Articles | Volume 15, issue 6
https://doi.org/10.5194/essd-15-2667-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/essd-15-2667-2023
© Author(s) 2023. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Data description paper
| 
29 Jun 2023
Data description paper |
| 29 Jun 2023
| 29 Jun 2023
The HTAP_v3 emission mosaic: merging regional and global monthly emissions (2000–2018) to support air quality modelling and policies
Monica Crippa
CORRESPONDING AUTHOR
European Commission, Joint Research Centre (JRC), Ispra, Italy
Diego Guizzardi
European Commission, Joint Research Centre (JRC), Ispra, Italy
Tim Butler
Research Institute Sustainability, Helmholtz Centre Potsdam (RIFS
Potsdam), 14467 Potsdam, Germany
Terry Keating
U.S. Environmental Protection Agency, Washington DC 20460, USA
Rosa Wu
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada
Jacek Kaminski
Institute of Environmental Protection, National Research Institute, 00‐548 Warsaw,
Poland
Jeroen Kuenen
Department of Climate, Air and Sustainability, TNO, Utrecht, the
Netherlands
Junichi Kurokawa
Asia Center for Air Pollution Research (ACAP), 1182 Sowa, Nishi-ku,
Niigata-shi 950-2144, Japan
Satoru Chatani
Regional Environment Conservation Division, National Institute for Environmental Studies (NIES), Tsukuba,
305-8506, Japan
Tazuko Morikawa
Japan Automobile Research Institute (JARI), 2530 Karima, Tsukuba 305-0822, Japan
George Pouliot
US Environmental Protection Agency, 109 T.W. Alexander Drive, Research Triangle Park, NC 27711, United States
Jacinthe Racine
Air Quality Policy-Issue Response Section, Canadian Centre for
Meteorological and Environmental Prediction, Environment and Climate Change
Canada (ECCC), Dorval, Quebec, Canada
Michael D. Moran
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada
Zbigniew Klimont
International Institute for Applied Systems Analysis (IIASA),
Laxenburg, Austria
Patrick M. Manseau
Air Quality Policy-Issue Response Section, Canadian Centre for
Meteorological and Environmental Prediction, Environment and Climate Change
Canada (ECCC), Dorval, Quebec, Canada
Rabab Mashayekhi
Air Quality Policy-Issue Response Section, Canadian Centre for
Meteorological and Environmental Prediction, Environment and Climate Change
Canada (ECCC), Dorval, Quebec, Canada
Barron H. Henderson
US Environmental Protection Agency, 109 T.W. Alexander Drive, Research Triangle Park, NC 27711, United States
Steven J. Smith
Joint Global Change Research Institute, Pacific Northwest National
Lab, College Park, MD, USA
Harrison Suchyta
Joint Global Change Research Institute, Pacific Northwest National
Lab, College Park, MD, USA
Marilena Muntean
CORRESPONDING AUTHOR
European Commission, Joint Research Centre (JRC), Ispra, Italy
Efisio Solazzo
UniSystems Company, Milan, Italy
Manjola Banja
European Commission, Joint Research Centre (JRC), Ispra, Italy
Edwin Schaaf
European Commission, Joint Research Centre (JRC), Ispra, Italy
Federico Pagani
GFT Italia S.r.l., VIA SILE, 20139 Milan, Italy
Jung-Hun Woo
Department of Civil and Environmental Engineering, Konuk University, Seoul, South Korea
Department of Technology Fusion Engineering, Konuk University, Seoul, South Korea
Jinseok Kim
Department of Technology Fusion Engineering, Konuk University, Seoul, South Korea
Fabio Monforti-Ferrario
European Commission, Joint Research Centre (JRC), Ispra, Italy
Enrico Pisoni
European Commission, Joint Research Centre (JRC), Ispra, Italy
Junhua Zhang
Air Quality Research Division, Environment and Climate Change Canada, Toronto, Ontario, Canada
David Niemi
Air Quality Policy-Issue Response Section, Canadian Centre for
Meteorological and Environmental Prediction, Environment and Climate Change
Canada (ECCC), Dorval, Quebec, Canada
Mourad Sassi
Air Quality Policy-Issue Response Section, Canadian Centre for
Meteorological and Environmental Prediction, Environment and Climate Change
Canada (ECCC), Dorval, Quebec, Canada
Tabish Ansari
Research Institute Sustainability, Helmholtz Centre Potsdam (RIFS
Potsdam), 14467 Potsdam, Germany
Kristen Foley
US Environmental Protection Agency, 109 T.W. Alexander Drive, Research Triangle Park, NC 27711, United States
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Matthew J. McGrath, Ana Maria Roxana Petrescu, Philippe Peylin, Robbie M. Andrew, Bradley Matthews, Frank Dentener, Juraj Balkovič, Vladislav Bastrikov, Meike Becker, Gregoire Broquet, Philippe Ciais, Audrey Fortems-Cheiney, Raphael Ganzenmüller, Giacomo Grassi, Ian Harris, Matthew Jones, Jürgen Knauer, Matthias Kuhnert, Guillaume Monteil, Saqr Munassar, Paul I. Palmer, Glen P. Peters, Chunjing Qiu, Mart-Jan Schelhaas, Oksana Tarasova, Matteo Vizzarri, Karina Winkler, Gianpaolo Balsamo, Antoine Berchet, Peter Briggs, Patrick Brockmann, Frédéric Chevallier, Giulia Conchedda, Monica Crippa, Stijn N. C. Dellaert, Hugo A. C. Denier van der Gon, Sara Filipek, Pierre Friedlingstein, Richard Fuchs, Michael Gauss, Christoph Gerbig, Diego Guizzardi, Dirk Günther, Richard A. Houghton, Greet Janssens-Maenhout, Ronny Lauerwald, Bas Lerink, Ingrid T. Luijkx, Géraud Moulas, Marilena Muntean, Gert-Jan Nabuurs, Aurélie Paquirissamy, Lucia Perugini, Wouter Peters, Roberto Pilli, Julia Pongratz, Pierre Regnier, Marko Scholze, Yusuf Serengil, Pete Smith, Efisio Solazzo, Rona L. Thompson, Francesco N. Tubiello, Timo Vesala, and Sophia Walther
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Jan C. Minx, William F. Lamb, Robbie M. Andrew, Josep G. Canadell, Monica Crippa, Niklas Döbbeling, Piers M. Forster, Diego Guizzardi, Jos Olivier, Glen P. Peters, Julia Pongratz, Andy Reisinger, Matthew Rigby, Marielle Saunois, Steven J. Smith, Efisio Solazzo, and Hanqin Tian
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Ana Maria Roxana Petrescu, Matthew J. McGrath, Robbie M. Andrew, Philippe Peylin, Glen P. Peters, Philippe Ciais, Gregoire Broquet, Francesco N. Tubiello, Christoph Gerbig, Julia Pongratz, Greet Janssens-Maenhout, Giacomo Grassi, Gert-Jan Nabuurs, Pierre Regnier, Ronny Lauerwald, Matthias Kuhnert, Juraj Balkovič, Mart-Jan Schelhaas, Hugo A. C. Denier van der
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Efisio Solazzo, Monica Crippa, Diego Guizzardi, Marilena Muntean, Margarita Choulga, and Greet Janssens-Maenhout
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We conducted an extensive analysis of the structural uncertainty of the Emissions Database for Global Atmospheric Research (EDGAR) emission inventory of greenhouse gases, which adds a much needed reliability dimension to the accuracy of the emission estimates. The study undertakes in-depth analyses of the implication of aggregating emissions from different sources and/or countries on the accuracy. Results are presented for all emissions sectors according to IPCC definitions.
Xiaohui Lin, Wen Zhang, Monica Crippa, Shushi Peng, Pengfei Han, Ning Zeng, Lijun Yu, and Guocheng Wang
Earth Syst. Sci. Data, 13, 1073–1088, https://doi.org/10.5194/essd-13-1073-2021, https://doi.org/10.5194/essd-13-1073-2021, 2021
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CH4 is a potent greenhouse gas, and China’s anthropogenic CH4 emissions account for a large proportion of global total emissions. However, the existing estimates either focus on a specific sector or lag behind real time by several years. We collected and analyzed 12 datasets and compared them to reveal the spatiotemporal changes and their uncertainties. We further estimated the emissions from 1990–2019, and the estimates showed a robust trend in recent years when compared to top-down results.
Francesco Canonaco, Anna Tobler, Gang Chen, Yulia Sosedova, Jay Gates Slowik, Carlo Bozzetti, Kaspar Rudolf Daellenbach, Imad El Haddad, Monica Crippa, Ru-Jin Huang, Markus Furger, Urs Baltensperger, and André Stephan Henry Prévôt
Atmos. Meas. Tech., 14, 923–943, https://doi.org/10.5194/amt-14-923-2021, https://doi.org/10.5194/amt-14-923-2021, 2021
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Long-term ambient aerosol mass spectrometric data were analyzed with a statistical model (PMF) to obtain source contributions and fingerprints. The new aspects of this paper involve time-dependent source fingerprints by a rolling technique and the replacement of the full visual inspection of each run by a user-defined set of criteria to monitor the quality of each of these runs more efficiently. More reliable sources will finally provide better instruments for political mitigation strategies.
Erin E. McDuffie, Steven J. Smith, Patrick O'Rourke, Kushal Tibrewal, Chandra Venkataraman, Eloise A. Marais, Bo Zheng, Monica Crippa, Michael Brauer, and Randall V. Martin
Earth Syst. Sci. Data, 12, 3413–3442, https://doi.org/10.5194/essd-12-3413-2020, https://doi.org/10.5194/essd-12-3413-2020, 2020
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Global emission inventories are vital to understanding the impacts of air pollution on the environment, human health, and society. We update the open-source Community Emissions Data System (CEDS) to provide global gridded emissions of seven key air pollutants from 1970–2017 for 11 source sectors and multiple fuel types, including coal, solid biofuel, and liquid oil and natural gas. This dataset includes both monthly global gridded emissions and annual national totals.
Pengfei Han, Ning Zeng, Tom Oda, Xiaohui Lin, Monica Crippa, Dabo Guan, Greet Janssens-Maenhout, Xiaolin Ma, Zhu Liu, Yuli Shan, Shu Tao, Haikun Wang, Rong Wang, Lin Wu, Xiao Yun, Qiang Zhang, Fang Zhao, and Bo Zheng
Atmos. Chem. Phys., 20, 11371–11385, https://doi.org/10.5194/acp-20-11371-2020, https://doi.org/10.5194/acp-20-11371-2020, 2020
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An accurate estimation of China’s fossil-fuel CO2 emissions (FFCO2) is significant for quantification of carbon budget and emissions reductions towards the Paris Agreement goals. Here we assessed 9 global and regional inventories. Our findings highlight the significance of using locally measured coal emission factors. We call on the enhancement of physical measurements for validation and provide comprehensive information for inventory, monitoring, modeling, assimilation, and reducing emissions.
Philippe Thunis, Monica Crippa, Cornelis Cuvelier, Diego Guizzardi, Alexander De Meij, Gabriel Oreggioni, and Enrico Pisoni
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2020-144, https://doi.org/10.5194/essd-2020-144, 2020
Preprint withdrawn
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A comparison of emissions inventories for air quality modelling, in Europe, is presented. Among these inventories, EDGAR v5.0 for air pollutants is introduced and validated, through a simulation with the EMEP model.
Leyang Feng, Steven J. Smith, Caleb Braun, Monica Crippa, Matthew J. Gidden, Rachel Hoesly, Zbigniew Klimont, Margreet van Marle, Maarten van den Berg, and Guido R. van der Werf
Geosci. Model Dev., 13, 461–482, https://doi.org/10.5194/gmd-13-461-2020, https://doi.org/10.5194/gmd-13-461-2020, 2020
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We describe the methods used for generating gridded emission datasets produced for use by the modeling community, particularly for the Coupled Model Intercomparison Project Phase 6 (CMIP6). The development of three sets of gridded data (historical open burning, historical anthropogenic, and future scenarios) was coordinated to produce consistent data over 1750–2100. We discuss the methodologies used to produce these data along with limitations and potential for future work.
Alcide Zhao, Massimo A. Bollasina, Monica Crippa, and David S. Stevenson
Atmos. Chem. Phys., 19, 14517–14533, https://doi.org/10.5194/acp-19-14517-2019, https://doi.org/10.5194/acp-19-14517-2019, 2019
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Emissions of aerosols over the recent past have been regulated largely by two policy-relevant drivers: energy-use growth and technology advances. These generate large and competing impacts on global radiation balance and climate, particularly over Asia, Europe, and the Arctic. This may help better assess and interpret future climate projections, and hence inform future climate change impact reduction strategies. Yet, it is pressing to better constrain various uncertainties related to aerosols.
Greet Janssens-Maenhout, Monica Crippa, Diego Guizzardi, Marilena Muntean, Edwin Schaaf, Frank Dentener, Peter Bergamaschi, Valerio Pagliari, Jos G. J. Olivier, Jeroen A. H. W. Peters, John A. van Aardenne, Suvi Monni, Ulrike Doering, A. M. Roxana Petrescu, Efisio Solazzo, and Gabriel D. Oreggioni
Earth Syst. Sci. Data, 11, 959–1002, https://doi.org/10.5194/essd-11-959-2019, https://doi.org/10.5194/essd-11-959-2019, 2019
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In support of the Paris Agreement, EDGARv4.3.2 provides global annual estimates, broken down into IPCC-compliant source-sector levels, from 1970 to 2012. The anthropogenic CO2, CH4 and N2O emissions were calculated bottom up with international statistics and emission factors for 226 countries and spatially distributed. EDGARv4.3.2 is input for the top-down modelling of the Global Carbon Project and EU policy-making, needing GHG emission estimates for each country at the climate negotiations.
Monica Crippa, Greet Janssens-Maenhout, Diego Guizzardi, Rita Van Dingenen, and Frank Dentener
Atmos. Chem. Phys., 19, 5165–5186, https://doi.org/10.5194/acp-19-5165-2019, https://doi.org/10.5194/acp-19-5165-2019, 2019
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In this work we evaluate the contribution of the major anthropogenic emission sources to global air quality and human health, focusing on particulate matter (PM) concentrations because of their importance in populated areas and the proven cumulative negative effects on human health. We show that in order to improve air quality, regional policies should be implemented due to the transboundary features of PM pollution.
Rita Van Dingenen, Frank Dentener, Monica Crippa, Joana Leitao, Elina Marmer, Shilpa Rao, Efisio Solazzo, and Luana Valentini
Atmos. Chem. Phys., 18, 16173–16211, https://doi.org/10.5194/acp-18-16173-2018, https://doi.org/10.5194/acp-18-16173-2018, 2018
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The evaluation of air pollution impacts, including on human health, vegetation, climate, and ecosystem health, is an essential component in the design of policies that affect air quality directly or indirectly. We have developed a tool that allows for a fast screening of relevant air pollution impacts from given emission scenarios at the regional to global scale, bypassing expensive numerical modelling of complex atmospheric processes. This paper provides a full documentation of the methodology.
Monica Crippa, Diego Guizzardi, Marilena Muntean, Edwin Schaaf, Frank Dentener, John A. van Aardenne, Suvi Monni, Ulrike Doering, Jos G. J. Olivier, Valerio Pagliari, and Greet Janssens-Maenhout
Earth Syst. Sci. Data, 10, 1987–2013, https://doi.org/10.5194/essd-10-1987-2018, https://doi.org/10.5194/essd-10-1987-2018, 2018
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EDGAR v4.3.2 is a global bottom-up emission inventory providing consistent anthropogenic emissions of gaseous and particulate air pollutants for 1970–2012 (with annual and monthly resolution) and grid maps with 0.1° × 0.1° resolution. We compare world regions using per capita and per GDP emissions, implied emissions per unit of energy, and emission ratios of co-emitted pollutants. We also show the growth of high-emitting areas (e.g. China, India) and the implications for global air quality.
Greet Janssens-Maenhout, Monica Crippa, Diego Guizzardi, Marilena Muntean, Edwin Schaaf, Frank Dentener, Peter Bergamaschi, Valerio Pagliari, Jos G. J. Olivier, Jeroen A. H. W. Peters, John A. van Aardenne, Suvi Monni, Ulrike Doering, and A. M. Roxana Petrescu
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2017-79, https://doi.org/10.5194/essd-2017-79, 2017
Revised manuscript not accepted
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The Emissions Database for Global Atmospheric Research supports climate policy making with a global dataset at disaggregated country & source-sector level for 1970–2012. This dataset is not only unique in its space/time coverage, but also in its completeness & consistency of CO2, CH4 & N2O emissions compilation for all anthropogenic activities except land use. Comparison with UNFCCC values show that estimates are within the uncertainty range, but have an annual variation smaller than this range.
Ganlin Huang, Rosie Brook, Monica Crippa, Greet Janssens-Maenhout, Christian Schieberle, Chris Dore, Diego Guizzardi, Marilena Muntean, Edwin Schaaf, and Rainer Friedrich
Atmos. Chem. Phys., 17, 7683–7701, https://doi.org/10.5194/acp-17-7683-2017, https://doi.org/10.5194/acp-17-7683-2017, 2017
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In this study, a global speciated non-methane volatile organic compound (NMVOC) emission data set is developed by compiling and allocating region- and source-specific speciation profiles, i.e. distributions of NMVOC species, to the revised and extended Emissions Database for Global Atmospheric Research emission inventory, which can serve as input data for chemical transport models and health impact assessments. Species time series and high-resolution global grid maps for 1970–2012 are produced.
Giancarlo Ciarelli, Sebnem Aksoyoglu, Imad El Haddad, Emily A. Bruns, Monica Crippa, Laurent Poulain, Mikko Äijälä, Samara Carbone, Evelyn Freney, Colin O'Dowd, Urs Baltensperger, and André S. H. Prévôt
Atmos. Chem. Phys., 17, 7653–7669, https://doi.org/10.5194/acp-17-7653-2017, https://doi.org/10.5194/acp-17-7653-2017, 2017
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Organic aerosol (OA) comprises the main fraction of fine particulate matter (PM1). Using a new VBS parameterization, we performed model-based source apportionment studies to assess the importance of different emission sources to the total OA loads in Europe during winter periods. Our results indicate that residential wood burning emissions represent the major source of OA, followed by non-residential emission sources (i.e. traffic and industries).
Giancarlo Ciarelli, Sebnem Aksoyoglu, Monica Crippa, Jose-Luis Jimenez, Eriko Nemitz, Karine Sellegri, Mikko Äijälä, Samara Carbone, Claudia Mohr, Colin O'Dowd, Laurent Poulain, Urs Baltensperger, and André S. H. Prévôt
Atmos. Chem. Phys., 16, 10313–10332, https://doi.org/10.5194/acp-16-10313-2016, https://doi.org/10.5194/acp-16-10313-2016, 2016
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Recent studies based on aerosol mass spectrometer measurements revealed that the organic fraction dominates the non-refractory PM1 composition. However its representation in chemical transport models is still very challenging due to uncertainties in emission sources and formation pathways. In this study, a novel organic aerosol scheme was tested in the regional air quality model CAMx and results were compared with ambient measurements at 11 different sites in Europe.
Monica Crippa, Greet Janssens-Maenhout, Frank Dentener, Diego Guizzardi, Katerina Sindelarova, Marilena Muntean, Rita Van Dingenen, and Claire Granier
Atmos. Chem. Phys., 16, 3825–3841, https://doi.org/10.5194/acp-16-3825-2016, https://doi.org/10.5194/acp-16-3825-2016, 2016
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The interplay of European air quality policies and technological advancement to reduce anthropogenic emissions avoided a dramatic deterioration of air quality in Europe and beyond over the last 40 years (e.g. fuel quality directives reduced global SO2 emissions by 88 %, while the EURO standards led to a 50 % reduction of PM2.5). The story told by the EDGAR retrospective scenarios can be informative for designing multi-pollutant abatement policies also in emerging economies.
Christos Fountoukis, Athanasios G. Megaritis, Ksakousti Skyllakou, Panagiotis E. Charalampidis, Hugo A. C. Denier van der Gon, Monica Crippa, André S. H. Prévôt, Friederike Fachinger, Alfred Wiedensohler, Christodoulos Pilinis, and Spyros N. Pandis
Atmos. Chem. Phys., 16, 3727–3741, https://doi.org/10.5194/acp-16-3727-2016, https://doi.org/10.5194/acp-16-3727-2016, 2016
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We use PMCAMx with high grid resolution over Paris to simulate carbonaceous aerosol during the summer and winter MEGAPOLI campaigns. PMCAMx reproduces BC observations well. Addition of cooking organic aerosol emissions of 80 mg per day per capita is needed to reproduce the corresponding observations. While the oxygenated organic aerosol predictions during the summer are encouraging a major wintertime source appears to be missing.
Andrea Paciga, Eleni Karnezi, Evangelia Kostenidou, Lea Hildebrandt, Magda Psichoudaki, Gabriella J. Engelhart, Byong-Hyoek Lee, Monica Crippa, André S. H. Prévôt, Urs Baltensperger, and Spyros N. Pandis
Atmos. Chem. Phys., 16, 2013–2023, https://doi.org/10.5194/acp-16-2013-2016, https://doi.org/10.5194/acp-16-2013-2016, 2016
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We estimate the volatility distribution for the organic aerosol (OA) components during summer and winter field campaigns in Paris, France as part of the collaborative project MEGAPOLI. The OA factors (hydrocarbon like OA, cooking OA, marine OA, oxygenated OA) had a broad spectrum of volatilities with no direct link between the average volatility and average oxygen to carbon of the OA components.
K. R. Daellenbach, C. Bozzetti, A. Křepelová, F. Canonaco, R. Wolf, P. Zotter, P. Fermo, M. Crippa, J. G. Slowik, Y. Sosedova, Y. Zhang, R.-J. Huang, L. Poulain, S. Szidat, U. Baltensperger, I. El Haddad, and A. S. H. Prévôt
Atmos. Meas. Tech., 9, 23–39, https://doi.org/10.5194/amt-9-23-2016, https://doi.org/10.5194/amt-9-23-2016, 2016
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In this study, we developed an offline technique using the AMS for the characterization of the chemical fingerprints of aerosols collected on quartz filters, and evaluated the suitability of the organic mass spectral data for source apportionment. This technique may be used to enhance the AMS capabilities in measuring size-fractionated, spatially resolved long-term data sets.
G. Janssens-Maenhout, M. Crippa, D. Guizzardi, F. Dentener, M. Muntean, G. Pouliot, T. Keating, Q. Zhang, J. Kurokawa, R. Wankmüller, H. Denier van der Gon, J. J. P. Kuenen, Z. Klimont, G. Frost, S. Darras, B. Koffi, and M. Li
Atmos. Chem. Phys., 15, 11411–11432, https://doi.org/10.5194/acp-15-11411-2015, https://doi.org/10.5194/acp-15-11411-2015, 2015
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This paper provides monthly emission grid maps at 0.1deg x 0.1deg resolution with global coverage for air pollutants and aerosols anthropogenic emissions in 2008 and 2010.
Countries are consistently inter-compared with sector-specific implied emission factors, per capita emissions and emissions per unit of GDP.
The emission grid maps compose the reference emissions data set for the community modelling hemispheric transport of air pollution (HTAP).
M. Pikridas, J. Sciare, F. Freutel, S. Crumeyrolle, S.-L. von der Weiden-Reinmüller, A. Borbon, A. Schwarzenboeck, M. Merkel, M. Crippa, E. Kostenidou, M. Psichoudaki, L. Hildebrandt, G. J. Engelhart, T. Petäjä, A. S. H. Prévôt, F. Drewnick, U. Baltensperger, A. Wiedensohler, M. Kulmala, M. Beekmann, and S. N. Pandis
Atmos. Chem. Phys., 15, 10219–10237, https://doi.org/10.5194/acp-15-10219-2015, https://doi.org/10.5194/acp-15-10219-2015, 2015
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Aerosol size distribution measurements from three ground sites, two mobile laboratories, and one airplane are combined to investigate the spatial and temporal variability of ultrafine particles in and around Paris during the summer and winter MEGAPOLI campaigns. The role of nucleation as a particle source and the influence of Paris emissions on their surroundings are examined.
M. Beekmann, A. S. H. Prévôt, F. Drewnick, J. Sciare, S. N. Pandis, H. A. C. Denier van der Gon, M. Crippa, F. Freutel, L. Poulain, V. Ghersi, E. Rodriguez, S. Beirle, P. Zotter, S.-L. von der Weiden-Reinmüller, M. Bressi, C. Fountoukis, H. Petetin, S. Szidat, J. Schneider, A. Rosso, I. El Haddad, A. Megaritis, Q. J. Zhang, V. Michoud, J. G. Slowik, S. Moukhtar, P. Kolmonen, A. Stohl, S. Eckhardt, A. Borbon, V. Gros, N. Marchand, J. L. Jaffrezo, A. Schwarzenboeck, A. Colomb, A. Wiedensohler, S. Borrmann, M. Lawrence, A. Baklanov, and U. Baltensperger
Atmos. Chem. Phys., 15, 9577–9591, https://doi.org/10.5194/acp-15-9577-2015, https://doi.org/10.5194/acp-15-9577-2015, 2015
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A detailed characterization of air quality in the Paris (France) agglomeration, a megacity, during two summer and winter intensive campaigns and from additional 1-year observations, revealed that about 70% of the fine particulate matter (PM) at urban background is transported into the megacity from upwind regions. Unexpectedly, a major part of organic PM is of modern origin (woodburning and cooking activities, secondary formation from biogenic VOC).
B. Gantt, M. S. Johnson, M. Crippa, A. S. H. Prévôt, and N. Meskhidze
Geosci. Model Dev., 8, 619–629, https://doi.org/10.5194/gmd-8-619-2015, https://doi.org/10.5194/gmd-8-619-2015, 2015
W. Ait-Helal, A. Borbon, S. Sauvage, J. A. de Gouw, A. Colomb, V. Gros, F. Freutel, M. Crippa, C. Afif, U. Baltensperger, M. Beekmann, J.-F. Doussin, R. Durand-Jolibois, I. Fronval, N. Grand, T. Leonardis, M. Lopez, V. Michoud, K. Miet, S. Perrier, A. S. H. Prévôt, J. Schneider, G. Siour, P. Zapf, and N. Locoge
Atmos. Chem. Phys., 14, 10439–10464, https://doi.org/10.5194/acp-14-10439-2014, https://doi.org/10.5194/acp-14-10439-2014, 2014
L. Poulain, W. Birmili, F. Canonaco, M. Crippa, Z. J. Wu, S. Nordmann, G. Spindler, A. S. H. Prévôt, A. Wiedensohler, and H. Herrmann
Atmos. Chem. Phys., 14, 10145–10162, https://doi.org/10.5194/acp-14-10145-2014, https://doi.org/10.5194/acp-14-10145-2014, 2014
C. Fountoukis, A. G. Megaritis, K. Skyllakou, P. E. Charalampidis, C. Pilinis, H. A. C. Denier van der Gon, M. Crippa, F. Canonaco, C. Mohr, A. S. H. Prévôt, J. D. Allan, L. Poulain, T. Petäjä, P. Tiitta, S. Carbone, A. Kiendler-Scharr, E. Nemitz, C. O'Dowd, E. Swietlicki, and S. N. Pandis
Atmos. Chem. Phys., 14, 9061–9076, https://doi.org/10.5194/acp-14-9061-2014, https://doi.org/10.5194/acp-14-9061-2014, 2014
M. Crippa, F. Canonaco, V. A. Lanz, M. Äijälä, J. D. Allan, S. Carbone, G. Capes, D. Ceburnis, M. Dall'Osto, D. A. Day, P. F. DeCarlo, M. Ehn, A. Eriksson, E. Freney, L. Hildebrandt Ruiz, R. Hillamo, J. L. Jimenez, H. Junninen, A. Kiendler-Scharr, A.-M. Kortelainen, M. Kulmala, A. Laaksonen, A. A. Mensah, C. Mohr, E. Nemitz, C. O'Dowd, J. Ovadnevaite, S. N. Pandis, T. Petäjä, L. Poulain, S. Saarikoski, K. Sellegri, E. Swietlicki, P. Tiitta, D. R. Worsnop, U. Baltensperger, and A. S. H. Prévôt
Atmos. Chem. Phys., 14, 6159–6176, https://doi.org/10.5194/acp-14-6159-2014, https://doi.org/10.5194/acp-14-6159-2014, 2014
S.-L. von der Weiden-Reinmüller, F. Drewnick, M. Crippa, A. S. H. Prévôt, F. Meleux, U. Baltensperger, M. Beekmann, and S. Borrmann
Atmos. Meas. Tech., 7, 279–299, https://doi.org/10.5194/amt-7-279-2014, https://doi.org/10.5194/amt-7-279-2014, 2014
F. Canonaco, M. Crippa, J. G. Slowik, U. Baltensperger, and A. S. H. Prévôt
Atmos. Meas. Tech., 6, 3649–3661, https://doi.org/10.5194/amt-6-3649-2013, https://doi.org/10.5194/amt-6-3649-2013, 2013
R. M. Healy, J. Sciare, L. Poulain, M. Crippa, A. Wiedensohler, A. S. H. Prévôt, U. Baltensperger, R. Sarda-Estève, M. L. McGuire, C.-H. Jeong, E. McGillicuddy, I. P. O'Connor, J. R. Sodeau, G. J. Evans, and J. C. Wenger
Atmos. Chem. Phys., 13, 9479–9496, https://doi.org/10.5194/acp-13-9479-2013, https://doi.org/10.5194/acp-13-9479-2013, 2013
M. Crippa, F. Canonaco, J. G. Slowik, I. El Haddad, P. F. DeCarlo, C. Mohr, M. F. Heringa, R. Chirico, N. Marchand, B. Temime-Roussel, E. Abidi, L. Poulain, A. Wiedensohler, U. Baltensperger, and A. S. H. Prévôt
Atmos. Chem. Phys., 13, 8411–8426, https://doi.org/10.5194/acp-13-8411-2013, https://doi.org/10.5194/acp-13-8411-2013, 2013
M. Laborde, M. Crippa, T. Tritscher, Z. Jurányi, P. F. Decarlo, B. Temime-Roussel, N. Marchand, S. Eckhardt, A. Stohl, U. Baltensperger, A. S. H. Prévôt, E. Weingartner, and M. Gysel
Atmos. Chem. Phys., 13, 5831–5856, https://doi.org/10.5194/acp-13-5831-2013, https://doi.org/10.5194/acp-13-5831-2013, 2013
Q. J. Zhang, M. Beekmann, F. Drewnick, F. Freutel, J. Schneider, M. Crippa, A. S. H. Prevot, U. Baltensperger, L. Poulain, A. Wiedensohler, J. Sciare, V. Gros, A. Borbon, A. Colomb, V. Michoud, J.-F. Doussin, H. A. C. Denier van der Gon, M. Haeffelin, J.-C. Dupont, G. Siour, H. Petetin, B. Bessagnet, S. N. Pandis, A. Hodzic, O. Sanchez, C. Honoré, and O. Perrussel
Atmos. Chem. Phys., 13, 5767–5790, https://doi.org/10.5194/acp-13-5767-2013, https://doi.org/10.5194/acp-13-5767-2013, 2013
M. Crippa, P. F. DeCarlo, J. G. Slowik, C. Mohr, M. F. Heringa, R. Chirico, L. Poulain, F. Freutel, J. Sciare, J. Cozic, C. F. Di Marco, M. Elsasser, J. B. Nicolas, N. Marchand, E. Abidi, A. Wiedensohler, F. Drewnick, J. Schneider, S. Borrmann, E. Nemitz, R. Zimmermann, J.-L. Jaffrezo, A. S. H. Prévôt, and U. Baltensperger
Atmos. Chem. Phys., 13, 961–981, https://doi.org/10.5194/acp-13-961-2013, https://doi.org/10.5194/acp-13-961-2013, 2013
F. Freutel, J. Schneider, F. Drewnick, S.-L. von der Weiden-Reinmüller, M. Crippa, A. S. H. Prévôt, U. Baltensperger, L. Poulain, A. Wiedensohler, J. Sciare, R. Sarda-Estève, J. F. Burkhart, S. Eckhardt, A. Stohl, V. Gros, A. Colomb, V. Michoud, J. F. Doussin, A. Borbon, M. Haeffelin, Y. Morille, M. Beekmann, and S. Borrmann
Atmos. Chem. Phys., 13, 933–959, https://doi.org/10.5194/acp-13-933-2013, https://doi.org/10.5194/acp-13-933-2013, 2013
Hazel Cathcart, Julian Aherne, Michael D. Moran, Verica Savic-Jovcic, Paul A. Makar, and Amanda Cole
Biogeosciences, 22, 535–554, https://doi.org/10.5194/bg-22-535-2025, https://doi.org/10.5194/bg-22-535-2025, 2025
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Deposition from sulfur and nitrogen pollution can harm ecosystems, and recovery from this type of pollution can take decades or longer. To identify risk to Canadian soils, we created maps showing sensitivity to sulfur and nitrogen pollution. Results show that some ecosystems are at risk from acid and nutrient nitrogen deposition: 10 % of protected areas are receiving acid deposition beyond their damage threshold, and 70 % may be receiving nitrogen deposition that could cause biodiversity loss.
Natalie Brett, Kathy S. Law, Steve R. Arnold, Javier G. Fochesatto, Jean-Christophe Raut, Tatsuo Onishi, Robert Gilliam, Kathleen Fahey, Deanna Huff, George Pouliot, Brice Barret, Elsa Dieudonné, Roman Pohorsky, Julia Schmale, Andrea Baccarini, Slimane Bekki, Gianluca Pappaccogli, Federico Scoto, Stefano Decesari, Antonio Donateo, Meeta Cesler-Maloney, William Simpson, Patrice Medina, Barbara D'Anna, Brice Temime-Roussel, Joel Savarino, Sarah Albertin, Jingqiu Mao, Becky Alexander, Allison Moon, Peter F. DeCarlo, Vanessa Selimovic, Robert Yokelson, and Ellis S. Robinson
Atmos. Chem. Phys., 25, 1063–1104, https://doi.org/10.5194/acp-25-1063-2025, https://doi.org/10.5194/acp-25-1063-2025, 2025
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Processes influencing dispersion of local anthropogenic pollution in Arctic wintertime are investigated with Lagrangian dispersion modelling. Simulated power plant plume rise that considers temperature inversion layers improves results compared to observations (interior Alaska). Modelled surface concentrations are improved by representation of vertical mixing and emission estimates. Large increases in diesel vehicle emissions at temperatures reaching −35°C are required to reproduce observed NOx.
Wanmin Gong, Stephen R. Beagley, Kenjiro Toyota, Henrik Skov, Jesper Heile Christensen, Alexandru Lupu, Diane Pendlebury, Junhua Zhang, Ulas Im, Yugo Kanaya, Alfonso Saiz-Lopez, Roberto Sommariva, Peter Effertz, John W. Halfacre, Nis Jepsen, Rigel Kivi, Theodore K. Koenig, Katrin Müller, Claus Nordstrøm, Irina Petropavlovskikh, Paul B. Shepson, William R. Simpson, Sverre Solberg, Ralf M. Staebler, David W. Tarasick, Roeland Van Malderen, and Mika Vestenius
EGUsphere, https://doi.org/10.5194/egusphere-2024-3750, https://doi.org/10.5194/egusphere-2024-3750, 2025
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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This study showed that the springtime O3 depletion plays a critical role in driving the surface O3 seasonal cycle in Central Arctic. The O3 depletion events, while occurring most notably within the lowest few hundred metres above the Arctic Ocean, can induce a 5–7 % of loss in the pan-Arctic tropospheric O3 burden during springtime. The study also found an enhancement in O3 and NOy (mostly PAN) concentrations in the Arctic due to northern boreal wildfires, particularly at altitudes.
Alexander de Meij, Cornelis Cuvelier, Philippe Thunis, and Enrico Pisoni
EGUsphere, https://doi.org/10.5194/egusphere-2024-3690, https://doi.org/10.5194/egusphere-2024-3690, 2025
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
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We assess the relevance and utility indicators developed within FAIRMODE by evaluating 9 CAMS models in calculated air pollutant values. For NO2, the results highlight difficulties at traffic stations. For PM2.5 and PM10 the bias and Winter-Summer gradients reveal issues. O3 evaluation shows that e.g. seasonal gradients are useful. Overall, the indicators provide valuable insights into model limitations, yet there is a need to reconsider the strictness of some indicators for certain pollutants.
Xiao Lu, Yiming Liu, Jiayin Su, Xiang Weng, Tabish Ansari, Yuqiang Zhang, Guowen He, Yuqi Zhu, Haolin Wang, Ganquan Zeng, Jingyu Li, Cheng He, Shuai Li, Teerachai Amnuaylojaroen, Tim Butler, Qi Fan, Shaojia Fan, Grant L. Forster, Meng Gao, Jianlin Hu, Yugo Kanaya, Mohd Talib Latif, Keding Lu, Philippe Nédélec, Peer Nowack, Bastien Sauvage, Xiaobin Xu, Lin Zhang, Ke Li, Ja-Ho Koo, and Tatsuya Nagashima
EGUsphere, https://doi.org/10.5194/egusphere-2024-3702, https://doi.org/10.5194/egusphere-2024-3702, 2024
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This study analyzes summertime ozone trends in East and Southeast Asia derived from a comprehensive observational database spanning from 1995 to 2019, incorporating aircraft observations, ozonesonde data, and measurements from 2500 surface sites. Multiple models are applied to attribute to changes in anthropogenic emissions and climate. The results highlight increases in anthropogenic emission are the primary driver of ozone increases both in the free troposphere and at the surface.
Tabish Ansari, Aditya Nalam, Aurelia Lupaşcu, Carsten Hinz, Simon Grasse, and Tim Butler
EGUsphere, https://doi.org/10.5194/egusphere-2024-3752, https://doi.org/10.5194/egusphere-2024-3752, 2024
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Surface ozone can travel far from its sources. In recent decades, emissions of ozone-forming gases have decreased in North America and Europe but risen in Asia, alongside rising global methane levels. Using advanced modeling, this study reveals that while local reductions in nitrogen oxides have lowered summer ozone, increases in natural and foreign sources offset these gains. Methane remains important, but its ozone impact has declined with reduced local emissions.
Augustin Colette, Gaëlle Collin, François Besson, Etienne Blot, Vincent Guidard, Frederik Meleux, Adrien Royer, Valentin Petiot, Claire Miller, Oihana Fermond, Alizé Jeant, Mario Adani, Joaquim Arteta, Anna Benedictow, Robert Bergström, Dene Bowdalo, Jorgen Brandt, Gino Briganti, Ana C. Carvalho, Jesper Heile Christensen, Florian Couvidat, Ilia D’Elia, Massimo D’Isidoro, Hugo Denier van der Gon, Gaël Descombes, Enza Di Tomaso, John Douros, Jeronimo Escribano, Henk Eskes, Hilde Fagerli, Yalda Fatahi, Johannes Flemming, Elmar Friese, Lise Frohn, Michael Gauss, Camilla Geels, Guido Guarnieri, Marc Guevara, Antoine Guion, Jonathan Guth, Risto Hänninen, Kaj Hansen, Ulas Im, Ruud Janssen, Marine Jeoffrion, Mathieu Joly, Luke Jones, Oriol Jorba, Evgeni Kadantsev, Michael Kahnert, Jacek W. Kaminski, Rostislav Kouznetsov, Richard Kranenburg, Jeroen Kuenen, Anne Caroline Lange, Joachim Langner, Victor Lannuque, Francesca Macchia, Astrid Manders, Mihaela Mircea, Agnes Nyiri, Miriam Olid, Carlos Pérez García-Pando, Yuliia Palamarchuk, Antonio Piersanti, Blandine Raux, Miha Razinger, Lennard Robertson, Arjo Segers, Martijn Schaap, Pilvi Siljamo, David Simpson, Mikhail Sofiev, Anders Stangel, Joanna Struzewska, Carles Tena, Renske Timmermans, Thanos Tsikerdekis, Svetlana Tsyro, Svyatoslav Tyuryakov, Anthony Ung, Andreas Uppstu, Alvaro Valdebenito, Peter van Velthoven, Lina Vitali, Zhuyun Ye, Vincent-Henri Peuch, and Laurence Rouïl
EGUsphere, https://doi.org/10.5194/egusphere-2024-3744, https://doi.org/10.5194/egusphere-2024-3744, 2024
This preprint is open for discussion and under review for Geoscientific Model Development (GMD).
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The Copernicus Atmosphere Monitoring Service – Regional Production delivers daily forecasts, analyses, and reanalyses of air quality in Europe. The Service relies on a distributed modelling production by eleven leading European modelling teams following stringent requirements with an operational design which has no equivalent in the world. All the products are full, free, open and quality assured and disseminated with a high level of reliability.
T. Nash Skipper, Christian Hogrefe, Barron H. Henderson, Rohit Mathur, Kristen M. Foley, and Armistead G. Russell
Geosci. Model Dev., 17, 8373–8397, https://doi.org/10.5194/gmd-17-8373-2024, https://doi.org/10.5194/gmd-17-8373-2024, 2024
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Chemical transport model simulations are combined with ozone observations to estimate the bias in ozone attributable to US anthropogenic sources and individual sources of US background ozone: natural sources, non-US anthropogenic sources, and stratospheric ozone. Results indicate a positive bias correlated with US anthropogenic emissions during summer in the eastern US and a negative bias correlated with stratospheric ozone during spring.
Phuc Thi Minh Ha, Yugo Kanaya, Kazuyo Yamaji, Syuichi Itahashi, Satoru Chatani, Takashi Sekiya, Maria Dolores Andrés Hernández, John Philip Burrows, Hans Schlager, Michael Lichtenstern, Mira Poehlker, and Bruna Holanda
EGUsphere, https://doi.org/10.5194/egusphere-2024-2064, https://doi.org/10.5194/egusphere-2024-2064, 2024
This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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Black carbon and CO are important to climate change. EMeRGe airborne observation can identify the suitability of emission inventories used in CMAQv5.0.2 model for Asian polluted regions. GFEDv4.1s is suitable for fire emissions. Anthropogenic BC and CO emissions from Philippines (REASv2.1) are insufficient. The estimated Chinese emissions in 2018 are 0.65±0.25 TgBC, 166±65 TgCO and 12.4±4.8 PgCO2, suggesting a reduction and increment for China's BC and CO emissions in the HTAPv2.2z inventory.
T. Nash Skipper, Emma L. D'Ambro, Forwood C. Wiser, V. Faye McNeill, Rebecca H. Schwantes, Barron H. Henderson, Ivan R. Piletic, Colleen B. Baublitz, Jesse O. Bash, Andrew R. Whitehill, Lukas C. Valin, Asher P. Mouat, Jennifer Kaiser, Glenn M. Wolfe, Jason M. St. Clair, Thomas F. Hanisco, Alan Fried, Bryan K. Place, and Havala O.T. Pye
Atmos. Chem. Phys., 24, 12903–12924, https://doi.org/10.5194/acp-24-12903-2024, https://doi.org/10.5194/acp-24-12903-2024, 2024
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We develop the Community Regional Atmospheric Chemistry Multiphase Mechanism (CRACMM) version 2 to improve predictions of formaldehyde in ambient air compared to satellite-, aircraft-, and ground-based observations. With the updated chemistry, we estimate the cancer risk from inhalation exposure to ambient formaldehyde across the contiguous USA and predict that 40 % of this risk is controllable through reductions in anthropogenic emissions of nitrogen oxides and reactive organic carbon.
Kiyeon Kim, Kyung Man Han, Chul Han Song, Hyojun Lee, Ross Beardsley, Jinhyeok Yu, Greg Yarwood, Bonyoung Koo, Jasper Madalipay, Jung-Hun Woo, and Seogju Cho
Atmos. Chem. Phys., 24, 12575–12593, https://doi.org/10.5194/acp-24-12575-2024, https://doi.org/10.5194/acp-24-12575-2024, 2024
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We incorporated each HONO process into the current CMAQ modeling framework to enhance the accuracy of HONO mixing ratio predictions. These results expand our understanding of HONO photochemistry and identify crucial sources of HONO that impact the total HONO budget in Seoul, South Korea. Through this investigation, we contribute to resolving discrepancies in understanding chemical transport models, with implications for better air quality management and environmental protection in the region.
David C. Wong, Jeff Willison, Jonathan E. Pleim, Golam Sarwar, James Beidler, Russ Bullock, Jerold A. Herwehe, Rob Gilliam, Daiwen Kang, Christian Hogrefe, George Pouliot, and Hosein Foroutan
Geosci. Model Dev., 17, 7855–7866, https://doi.org/10.5194/gmd-17-7855-2024, https://doi.org/10.5194/gmd-17-7855-2024, 2024
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This work describe how we linked the meteorological Model for Prediction Across Scales – Atmosphere (MPAS-A) with the Community Multiscale Air Quality (CMAQ) air quality model to form a coupled modelling system. This could be used to study air quality or climate and air quality interaction at a global scale. This new model scales well in high-performance computing environments and performs well with respect to ground surface networks in terms of ozone and PM2.5.
Chris McLinden, Debora Griffin, Vitali Fioletov, Junhua Zhang, Enrico Dammers, Cristen Adams, Mallory Loria, Nicolay Krotkov, and Lok Lamsal
EGUsphere, https://doi.org/10.5194/egusphere-2024-2856, https://doi.org/10.5194/egusphere-2024-2856, 2024
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The Ozone Monitoring Instrument (OMI) was used to understand the evolution of NOx emissions from the Canadian oil sands. OMI NO2 combined with winds and reported stack emissions, found emissions from the heavy-hauler mine fleet increased by about 20 % since 2005, whereas the total oil sands mined nearly doubled. This difference is a result of emissions standards limiting NOx emissions becoming more stringent over this period confirming the efficacy of the policy enacting these standards.
Willem E. van Caspel, Zbigniew Klimont, Chris Heyes, and Hilde Fagerli
Atmos. Chem. Phys., 24, 11545–11563, https://doi.org/10.5194/acp-24-11545-2024, https://doi.org/10.5194/acp-24-11545-2024, 2024
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Methane in the atmosphere contributes to the production of ozone gas – an air pollutant and greenhouse gas. Our results highlight that simultaneous reductions in methane emissions help avoid offsetting the air pollution benefits already achieved by the already-approved precursor emission reductions by 2050 in the European Monitoring and Evaluation Programme region, while also playing an important role in bringing air pollution further down towards World Health Organization guideline limits.
Christos I. Efstathiou, Elizabeth Adams, Carlie J. Coats, Robert Zelt, Mark Reed, John McGee, Kristen M. Foley, Fahim I. Sidi, David C. Wong, Steven Fine, and Saravanan Arunachalam
Geosci. Model Dev., 17, 7001–7027, https://doi.org/10.5194/gmd-17-7001-2024, https://doi.org/10.5194/gmd-17-7001-2024, 2024
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We present a summary of enabling high-performance computing of the Community Multiscale Air Quality Model (CMAQ) – a state-of-the-science community multiscale air quality model – on two cloud computing platforms through documenting the technologies, model performance, scaling and relative merits. This may be a new paradigm for computationally intense future model applications. We initiated this work due to a need to leverage cloud computing advances and to ease the learning curve for new users.
Cynthia H. Whaley, Tim Butler, Jose A. Adame, Rupal Ambulkar, Stephen R. Arnold, Rebecca R. Buchholz, Benjamin Gaubert, Douglas S. Hamilton, Min Huang, Hayley Hung, Johannes W. Kaiser, Jacek W. Kaminski, Christophe Knote, Gerbrand Koren, Jean-Luc Kouassi, Meiyun Lin, Tianjia Liu, Jianmin Ma, Kasemsan Manomaiphiboon, Elisa Bergas Masso, Jessica L. McCarty, Mariano Mertens, Mark Parrington, Helene Peiro, Pallavi Saxena, Saurabh Sonwani, Vanisa Surapipith, Damaris Tan, Wenfu Tang, Veerachai Tanpipat, Kostas Tsigaridis, Christine Wiedinmyer, Oliver Wild, Yuanyu Xie, and Paquita Zuidema
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-126, https://doi.org/10.5194/gmd-2024-126, 2024
Revised manuscript under review for GMD
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The multi-model experiment design of the HTAP3 Fires project takes a multi-pollutant approach to improving our understanding of transboundary transport of wildland fire and agricultural burning emissions and their impacts. The experiments are designed with the goal of answering science policy questions related to fires. The options for the multi-model approach, including inputs, outputs, and model set up are discussed, and the official recommendations for the project are presented.
Sepehr Fathi, Paul Makar, Wanmin Gong, Junhua Zhang, Katherine Hayden, and Mark Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2024-1655, https://doi.org/10.5194/egusphere-2024-1655, 2024
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Our study explores the influence of water phase changes in plumes from industrial sources on atmospheric dispersion of emitted pollutants and air quality. Employing PRISM (Plume-Rise-Iterative-Stratified-Moist), a new method, we found that considering these effects significantly improves predictions of pollutant dispersion. This insight enhances our understanding of environmental impacts, enabling more accurate air quality modeling, and fostering more effective pollution management strategies.
Paul A. Makar, Philip Cheung, Christian Hogrefe, Ayodeji Akingunola, Ummugulsum Alyuz-Ozdemir, Jesse O. Bash, Michael D. Bell, Roberto Bellasio, Roberto Bianconi, Tim Butler, Hazel Cathcart, Olivia E. Clifton, Alma Hodzic, Iannis Koutsioukis, Richard Kranenburg, Aurelia Lupascu, Jason A. Lynch, Kester Momoh, Juan L. Perez-Camanyo, Jonathan Pleim, Young-Hee Ryu, Roberto San Jose, Donna Schwede, Thomas Scheuschner, Mark Shephard, Ranjeet Sokhi, and Stefano Galmarini
EGUsphere, https://doi.org/10.5194/egusphere-2024-2226, https://doi.org/10.5194/egusphere-2024-2226, 2024
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The large range of sulphur and nitrogen deposition estimates from air-quality models results in a large range of predicted impacts. We used models and deposition diagnostics to identify the processes controlling atmospheric sulphur and nitrogen deposition variability. Controlling factors included the uptake of gases and aerosols by droplets, rain, snow, etc., aerosol inorganic chemistry, particle dry deposition, ammonia bidirectional fluxes, and gas deposition via plant cuticles and soil.
Matthew J. Rowlinson, Mat J. Evans, Lucy J. Carpenter, Katie A. Read, Shalini Punjabi, Adedayo Adedeji, Luke Fakes, Ally Lewis, Ben Richmond, Neil Passant, Tim Murrells, Barron Henderson, Kelvin H. Bates, and Detlev Helmig
Atmos. Chem. Phys., 24, 8317–8342, https://doi.org/10.5194/acp-24-8317-2024, https://doi.org/10.5194/acp-24-8317-2024, 2024
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Ethane and propane are volatile organic compounds emitted from human activities which help to form ozone, a pollutant and greenhouse gas, and also affect the chemistry of the lower atmosphere. Atmospheric models tend to do a poor job of reproducing the abundance of these compounds in the atmosphere. By using regional estimates of their emissions, rather than globally consistent estimates, we can significantly improve the simulation of ethane in the model and make some improvement for propane.
Sara Louise Farrell, Havala O. T. Pye, Robert Gilliam, George Pouliot, Deanna Huff, Golam Sarwar, William Vizuete, Nicole Briggs, and Kathleen Fahey
EGUsphere, https://doi.org/10.5194/egusphere-2024-1550, https://doi.org/10.5194/egusphere-2024-1550, 2024
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In this work we implement heterogeneous sulfur chemistry into the Community Multiscale Air Quality (CMAQ) model. This new chemistry accounts for the formation of sulfate via aqueous oxidation of SO2 in aerosol liquid water and the formation of hydroxymethanesulfonate (HMS) – often confused by measurement techniques as sulfate. Model performance in predicting sulfur PM2.5 in Fairbanks, Alaska, and other places that experience dark and cold winters, is improved.
Cassandra J. Gaston, Joseph M. Prospero, Kristen Foley, Havala O. T. Pye, Lillian Custals, Edmund Blades, Peter Sealy, and James A. Christie
Atmos. Chem. Phys., 24, 8049–8066, https://doi.org/10.5194/acp-24-8049-2024, https://doi.org/10.5194/acp-24-8049-2024, 2024
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To understand how changing emissions have impacted aerosols in remote regions, we measured nitrate and sulfate in Barbados and compared them to model predictions from EPA’s Air QUAlity TimE Series (EQUATES). Nitrate was stable, except for spikes in 2008 and 2010 due to transported smoke. Sulfate decreased in the 1990s due to reductions in sulfur dioxide (SO2) in the US and Europe; then it increased in the 2000s, likely due to anthropogenic emissions from Africa.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter G. Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankararaman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Johann Engelbrecht, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbigniew Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
EGUsphere, https://doi.org/10.5194/egusphere-2024-1617, https://doi.org/10.5194/egusphere-2024-1617, 2024
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Aerosol particles are an important part of the Earth system, but their concentrations are spatially and temporally heterogeneous, as well as variable in size and composition. Here we present a new compilation of PM2.5 and PM10 aerosol observations, focusing on the spatial variability across different observational stations, including composition, and demonstrate a method for comparing the datasets to model output.
Kalyn Dorheim, Skylar Gering, Robert Gieseke, Corinne Hartin, Leeya Pressburger, Alexey N. Shiklomanov, Steven J. Smith, Claudia Tebaldi, Dawn L. Woodard, and Ben Bond-Lamberty
Geosci. Model Dev., 17, 4855–4869, https://doi.org/10.5194/gmd-17-4855-2024, https://doi.org/10.5194/gmd-17-4855-2024, 2024
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Hector is an easy-to-use, global climate–carbon cycle model. With its quick run time, Hector can provide climate information from a run in a fraction of a second. Hector models on a global and annual basis. Here, we present an updated version of the model, Hector V3. In this paper, we document Hector’s new features. Hector V3 is capable of reproducing historical observations, and its future temperature projections are consistent with those of more complex models.
Monica Crippa, Diego Guizzardi, Federico Pagani, Marcello Schiavina, Michele Melchiorri, Enrico Pisoni, Francesco Graziosi, Marilena Muntean, Joachim Maes, Lewis Dijkstra, Martin Van Damme, Lieven Clarisse, and Pierre Coheur
Earth Syst. Sci. Data, 16, 2811–2830, https://doi.org/10.5194/essd-16-2811-2024, https://doi.org/10.5194/essd-16-2811-2024, 2024
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Knowing where emissions occur is essential for planning effective emission reduction measures and atmospheric modelling. Disaggregating national emissions over high-resolution grids requires spatial proxies that contain information on the location of different emission sources. This work incorporates state-of-the-art spatial information to improve the spatial representation of global emissions with the Emissions Database for Global Atmospheric Research (EDGAR).
Hanqin Tian, Naiqing Pan, Rona L. Thompson, Josep G. Canadell, Parvadha Suntharalingam, Pierre Regnier, Eric A. Davidson, Michael Prather, Philippe Ciais, Marilena Muntean, Shufen Pan, Wilfried Winiwarter, Sönke Zaehle, Feng Zhou, Robert B. Jackson, Hermann W. Bange, Sarah Berthet, Zihao Bian, Daniele Bianchi, Alexander F. Bouwman, Erik T. Buitenhuis, Geoffrey Dutton, Minpeng Hu, Akihiko Ito, Atul K. Jain, Aurich Jeltsch-Thömmes, Fortunat Joos, Sian Kou-Giesbrecht, Paul B. Krummel, Xin Lan, Angela Landolfi, Ronny Lauerwald, Ya Li, Chaoqun Lu, Taylor Maavara, Manfredi Manizza, Dylan B. Millet, Jens Mühle, Prabir K. Patra, Glen P. Peters, Xiaoyu Qin, Peter Raymond, Laure Resplandy, Judith A. Rosentreter, Hao Shi, Qing Sun, Daniele Tonina, Francesco N. Tubiello, Guido R. van der Werf, Nicolas Vuichard, Junjie Wang, Kelley C. Wells, Luke M. Western, Chris Wilson, Jia Yang, Yuanzhi Yao, Yongfa You, and Qing Zhu
Earth Syst. Sci. Data, 16, 2543–2604, https://doi.org/10.5194/essd-16-2543-2024, https://doi.org/10.5194/essd-16-2543-2024, 2024
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Atmospheric concentrations of nitrous oxide (N2O), a greenhouse gas 273 times more potent than carbon dioxide, have increased by 25 % since the preindustrial period, with the highest observed growth rate in 2020 and 2021. This rapid growth rate has primarily been due to a 40 % increase in anthropogenic emissions since 1980. Observed atmospheric N2O concentrations in recent years have exceeded the worst-case climate scenario, underscoring the importance of reducing anthropogenic N2O emissions.
Marielle Saunois, Adrien Martinez, Benjamin Poulter, Zhen Zhang, Peter Raymond, Pierre Regnier, Joseph G. Canadell, Robert B. Jackson, Prabir K. Patra, Philippe Bousquet, Philippe Ciais, Edward J. Dlugokencky, Xin Lan, George H. Allen, David Bastviken, David J. Beerling, Dmitry A. Belikov, Donald R. Blake, Simona Castaldi, Monica Crippa, Bridget R. Deemer, Fraser Dennison, Giuseppe Etiope, Nicola Gedney, Lena Höglund-Isaksson, Meredith A. Holgerson, Peter O. Hopcroft, Gustaf Hugelius, Akihito Ito, Atul K. Jain, Rajesh Janardanan, Matthew S. Johnson, Thomas Kleinen, Paul Krummel, Ronny Lauerwald, Tingting Li, Xiangyu Liu, Kyle C. McDonald, Joe R. Melton, Jens Mühle, Jurek Müller, Fabiola Murguia-Flores, Yosuke Niwa, Sergio Noce, Shufen Pan, Robert J. Parker, Changhui Peng, Michel Ramonet, William J. Riley, Gerard Rocher-Ros, Judith A. Rosentreter, Motoki Sasakawa, Arjo Segers, Steven J. Smith, Emily H. Stanley, Joel Thanwerdas, Hanquin Tian, Aki Tsuruta, Francesco N. Tubiello, Thomas S. Weber, Guido van der Werf, Doug E. Worthy, Yi Xi, Yukio Yoshida, Wenxin Zhang, Bo Zheng, Qing Zhu, Qiuan Zhu, and Qianlai Zhuang
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-115, https://doi.org/10.5194/essd-2024-115, 2024
Revised manuscript under review for ESSD
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Methane (CH4) is the second most important human-influenced greenhouse gas in terms of climate forcing after carbon dioxide (CO2). A consortium of multi-disciplinary scientists synthesize and update the budget of the sources and sinks of CH4. This edition benefits from important progresses in estimating emissions from lakes and ponds, reservoirs, and streams and rivers. For the 2010s decade, global CH4 emissions are estimated at 575 Tg CH4 yr-1, including ~65 % from anthropogenic sources.
Ashu Dastoor, Hélène Angot, Johannes Bieser, Flora Brocza, Brock Edwards, Aryeh Feinberg, Xinbin Feng, Benjamin Geyman, Charikleia Gournia, Yipeng He, Ian M. Hedgecock, Ilia Ilyin, Terry Keating, Jane Kirk, Che-Jen Lin, Igor Lehnherr, Robert Mason, David McLagan, Marilena Muntean, Peter Rafaj, Eric M. Roy, Andrei Ryjkov, Noelle E. Selin, Francesco De Simone, Anne L. Soerensen, Frits Steenhuisen, Oleg Travnikov, Shuxiao Wang, Xun Wang, Simon Wilson, Rosa Wu, Qingru Wu, Yanxu Zhang, Jun Zhou, Wei Zhu, and Scott Zolkos
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-65, https://doi.org/10.5194/gmd-2024-65, 2024
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This paper introduces the Multi-Compartment Mercury (Hg) Modeling and Analysis Project (MCHgMAP) aimed to inform the effectiveness evaluations of two multilateral environmental agreements: the Minamata Convention on Mercury and Convention on Long-Range Transboundary Air Pollution. The experimental design exploits a variety of models (atmospheric, land, oceanic and multi-media mass balance models) to assess the short- and long-term influences of anthropogenic Hg releases in the environment.
Philippe Thunis, Jeroen Kuenen, Enrico Pisoni, Bertrand Bessagnet, Manjola Banja, Lech Gawuc, Karol Szymankiewicz, Diego Guizardi, Monica Crippa, Susana Lopez-Aparicio, Marc Guevara, Alexander De Meij, Sabine Schindlbacher, and Alain Clappier
Geosci. Model Dev., 17, 3631–3643, https://doi.org/10.5194/gmd-17-3631-2024, https://doi.org/10.5194/gmd-17-3631-2024, 2024
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An ensemble emission inventory is created with the aim of monitoring the status and progress made with the development of EU-wide inventories. This emission ensemble serves as a common benchmark for the screening and allows for the comparison of more than two inventories at a time. Because the emission “truth” is unknown, the approach does not tell which inventory is the closest to reality, but it identifies inconsistencies that require special attention.
Antonin Soulie, Claire Granier, Sabine Darras, Nicolas Zilbermann, Thierno Doumbia, Marc Guevara, Jukka-Pekka Jalkanen, Sekou Keita, Cathy Liousse, Monica Crippa, Diego Guizzardi, Rachel Hoesly, and Steven J. Smith
Earth Syst. Sci. Data, 16, 2261–2279, https://doi.org/10.5194/essd-16-2261-2024, https://doi.org/10.5194/essd-16-2261-2024, 2024
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Anthropogenic emissions are the result of transportation, power generation, industrial, residential and commercial activities as well as waste treatment and agriculture practices. This work describes the new CAMS-GLOB-ANT gridded inventory of 2000–2023 anthropogenic emissions of air pollutants and greenhouse gases. The methodology to generate the emissions is explained and the datasets are analysed and compared with publicly available global and regional inventories for selected world regions.
Edward C. Chan, Ilona J. Jäkel, Basit Khan, Martijn Schaap, Timothy M. Butler, Renate Forkel, and Sabine Banzhaf
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2024-61, https://doi.org/10.5194/gmd-2024-61, 2024
Revised manuscript accepted for GMD
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An enhanced emission module has been developed for the PALM model system, allowing greater levels of flexibility and performance in modelling emission sources across different sectors. A model for parametrized domestic emissions has also been included, for which an idealized model run is conducted for PM10. The results show that, in addition to individual sources and diurnal variations in energy consumption, vertical transport and urban topology play a role in the PM concentration distribution.
Meng Li, Junichi Kurokawa, Qiang Zhang, Jung-Hun Woo, Tazuko Morikawa, Satoru Chatani, Zifeng Lu, Yu Song, Guannan Geng, Hanwen Hu, Jinseok Kim, Owen R. Cooper, and Brian C. McDonald
Atmos. Chem. Phys., 24, 3925–3952, https://doi.org/10.5194/acp-24-3925-2024, https://doi.org/10.5194/acp-24-3925-2024, 2024
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In this work, we developed MIXv2, a mosaic Asian emission inventory for 2010–2017. With high spatial (0.1°) and monthly temporal resolution, MIXv2 integrates anthropogenic and open biomass burning emissions across seven sectors following a mosaic methodology. It provides CO2 emissions data alongside nine key pollutants and three chemical mechanisms. Our publicly accessible gridded monthly emissions data can facilitate long-term atmospheric and climate model analyses.
Fei Liu, Steffen Beirle, Joanna Joiner, Sungyeon Choi, Zhining Tao, K. Emma Knowland, Steven J. Smith, Daniel Q. Tong, Siqi Ma, Zachary T. Fasnacht, and Thomas Wagner
Atmos. Chem. Phys., 24, 3717–3728, https://doi.org/10.5194/acp-24-3717-2024, https://doi.org/10.5194/acp-24-3717-2024, 2024
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Using satellite data, we developed a coupled method independent of the chemical transport model to map NOx emissions across US cities. After validating our technique with synthetic data, we charted NOx emissions from 2018–2021 in 39 cities. Our results closely matched EPA estimates but also highlighted some inconsistencies in both magnitude and spatial distribution. This research can help refine strategies for monitoring and managing air quality.
Ville-Veikko Paunu, Niko Karvosenoja, David Segersson, Susana López-Aparicio, Ole-Kenneth Nielsen, Marlene Schmidt Plejdrup, Throstur Thorsteinsson, Dam Thanh Vo, Jeroen Kuenen, Hugo Denier van der Gon, Jukka-Pekka Jalkanen, Jørgen Brandt, and Camilla Geels
Earth Syst. Sci. Data, 16, 1453–1474, https://doi.org/10.5194/essd-16-1453-2024, https://doi.org/10.5194/essd-16-1453-2024, 2024
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Air pollution is an important cause of adverse health effects, even in Nordic countries. To assess their health impacts, emission inventories with high spatial resolution are needed. We studied how national data and methods for the spatial distribution of the emissions compare to a European level inventory. For road transport the methods are well established, but for machinery and off-road emissions the current recommendations for the spatial distribution of these emissions should be improved.
Aditya Nalam, Aura Lupascu, Tabish Ansari, and Timothy Butler
EGUsphere, https://doi.org/10.5194/egusphere-2024-432, https://doi.org/10.5194/egusphere-2024-432, 2024
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Tropospheric O3 molecules are labelled with the identity of their precursor source in CAM-Chem to quantify the contribution from various emission sources to the tropospheric O3 burden (TOB) and its trends. With an equatorward shift, anthropogenic NOx emissions become significantly more efficient at producing O3 and play a major role in driving TOB trends. This is due to larger convection at the tropics effectively lifting O3 and its precursors to the free troposphere where O3 lifetime is longer.
Kelvin H. Bates, Mathew J. Evans, Barron H. Henderson, and Daniel J. Jacob
Geosci. Model Dev., 17, 1511–1524, https://doi.org/10.5194/gmd-17-1511-2024, https://doi.org/10.5194/gmd-17-1511-2024, 2024
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Accurate representation of rates and products of chemical reactions in atmospheric models is crucial for simulating concentrations of pollutants and climate forcers. We update the widely used GEOS-Chem atmospheric chemistry model with reaction parameters from recent compilations of experimental data and demonstrate the implications for key atmospheric chemical species. The updates decrease tropospheric CO mixing ratios and increase stratospheric nitrogen oxide mixing ratios, among other changes.
Heather Simon, Christian Hogrefe, Andrew Whitehill, Kristen M. Foley, Jennifer Liljegren, Norm Possiel, Benjamin Wells, Barron H. Henderson, Lukas C. Valin, Gail Tonnesen, K. Wyat Appel, and Shannon Koplitz
Atmos. Chem. Phys., 24, 1855–1871, https://doi.org/10.5194/acp-24-1855-2024, https://doi.org/10.5194/acp-24-1855-2024, 2024
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We assess observed and modeled ozone weekend–weekday differences in the USA from 2002–2019. A subset of urban areas that were NOx-saturated at the beginning of the period transitioned to NOx-limited conditions. Multiple rural areas of California were NOx-limited for the entire period but become less influenced by local day-of-week emission patterns in more recent years. The model produces more NOx-saturated conditions than the observations but captures trends in weekend–weekday ozone patterns.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankarararman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Hannele Hakola, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbiginiw Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-1, https://doi.org/10.5194/essd-2024-1, 2024
Preprint withdrawn
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Aerosol particles can interact with incoming solar radiation and outgoing long wave radiation, change cloud properties, affect photochemistry, impact surface air quality, and when deposited impact surface albedo of snow and ice, and modulate carbon dioxide uptake by the land and ocean. Here we present a new compilation of aerosol observations including composition, a methodology for comparing the datasets to model output, and show the implications of these results using one model.
Alexander de Meij, Cornelis Cuvelier, Philippe Thunis, Enrico Pisoni, and Bertrand Bessagnet
Geosci. Model Dev., 17, 587–606, https://doi.org/10.5194/gmd-17-587-2024, https://doi.org/10.5194/gmd-17-587-2024, 2024
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In our study the robustness of the model responses to emission reductions in the EU is assessed when the emission data are changed. Our findings are particularly important to better understand the uncertainties associated to the emission inventories and how these uncertainties impact the level of accuracy of the resulting air quality modelling, which is a key for designing air quality plans. Also crucial is the choice of indicator to avoid misleading interpretations of the results.
Ruben Urraca, Greet Janssens-Maenhout, Nicolás Álamos, Lucas Berna-Peña, Monica Crippa, Sabine Darras, Stijn Dellaert, Hugo Denier van der Gon, Mark Dowell, Nadine Gobron, Claire Granier, Giacomo Grassi, Marc Guevara, Diego Guizzardi, Kevin Gurney, Nicolás Huneeus, Sekou Keita, Jeroen Kuenen, Ana Lopez-Noreña, Enrique Puliafito, Geoffrey Roest, Simone Rossi, Antonin Soulie, and Antoon Visschedijk
Earth Syst. Sci. Data, 16, 501–523, https://doi.org/10.5194/essd-16-501-2024, https://doi.org/10.5194/essd-16-501-2024, 2024
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CoCO2-MOSAIC 1.0 is a global mosaic of regional bottom-up inventories providing gridded (0.1×0.1) monthly emissions of anthropogenic CO2. Regional inventories include country-specific information and finer spatial resolution than global inventories. CoCO2-MOSAIC provides harmonized access to these datasets and can be considered as a regionally accepted reference to assess the quality of global inventories, as done in the current paper.
Hamza Ahsan, Hailong Wang, Jingbo Wu, Mingxuan Wu, Steven J. Smith, Susanne Bauer, Harrison Suchyta, Dirk Olivié, Gunnar Myhre, Hitoshi Matsui, Huisheng Bian, Jean-François Lamarque, Ken Carslaw, Larry Horowitz, Leighton Regayre, Mian Chin, Michael Schulz, Ragnhild Bieltvedt Skeie, Toshihiko Takemura, and Vaishali Naik
Atmos. Chem. Phys., 23, 14779–14799, https://doi.org/10.5194/acp-23-14779-2023, https://doi.org/10.5194/acp-23-14779-2023, 2023
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We examine the impact of the assumed effective height of SO2 injection, SO2 and BC emission seasonality, and the assumed fraction of SO2 emissions injected as SO4 on climate and chemistry model results. We find that the SO2 injection height has a large impact on surface SO2 concentrations and, in some models, radiative flux. These assumptions are a
hiddensource of inter-model variability and may be leading to bias in some climate model results.
Chi-Tsan Wang, Bok H. Baek, William Vizuete, Lawrence S. Engel, Jia Xing, Jaime Green, Marc Serre, Richard Strott, Jared Bowden, and Jung-Hun Woo
Earth Syst. Sci. Data, 15, 5261–5279, https://doi.org/10.5194/essd-15-5261-2023, https://doi.org/10.5194/essd-15-5261-2023, 2023
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Hazardous air pollutant (HAP) human exposure studies usually rely on local measurements or dispersion model methods, but those methods are limited under spatial and temporal conditions. We processed the US EPA emission data to simulate the hourly HAP emission patterns and applied the chemical transport model to simulate the HAP concentrations. The modeled HAP results exhibit good agreement (R is 0.75 and NMB is −5.6 %) with observational data.
Matthew J. McGrath, Ana Maria Roxana Petrescu, Philippe Peylin, Robbie M. Andrew, Bradley Matthews, Frank Dentener, Juraj Balkovič, Vladislav Bastrikov, Meike Becker, Gregoire Broquet, Philippe Ciais, Audrey Fortems-Cheiney, Raphael Ganzenmüller, Giacomo Grassi, Ian Harris, Matthew Jones, Jürgen Knauer, Matthias Kuhnert, Guillaume Monteil, Saqr Munassar, Paul I. Palmer, Glen P. Peters, Chunjing Qiu, Mart-Jan Schelhaas, Oksana Tarasova, Matteo Vizzarri, Karina Winkler, Gianpaolo Balsamo, Antoine Berchet, Peter Briggs, Patrick Brockmann, Frédéric Chevallier, Giulia Conchedda, Monica Crippa, Stijn N. C. Dellaert, Hugo A. C. Denier van der Gon, Sara Filipek, Pierre Friedlingstein, Richard Fuchs, Michael Gauss, Christoph Gerbig, Diego Guizzardi, Dirk Günther, Richard A. Houghton, Greet Janssens-Maenhout, Ronny Lauerwald, Bas Lerink, Ingrid T. Luijkx, Géraud Moulas, Marilena Muntean, Gert-Jan Nabuurs, Aurélie Paquirissamy, Lucia Perugini, Wouter Peters, Roberto Pilli, Julia Pongratz, Pierre Regnier, Marko Scholze, Yusuf Serengil, Pete Smith, Efisio Solazzo, Rona L. Thompson, Francesco N. Tubiello, Timo Vesala, and Sophia Walther
Earth Syst. Sci. Data, 15, 4295–4370, https://doi.org/10.5194/essd-15-4295-2023, https://doi.org/10.5194/essd-15-4295-2023, 2023
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Accurate estimation of fluxes of carbon dioxide from the land surface is essential for understanding future impacts of greenhouse gas emissions on the climate system. A wide variety of methods currently exist to estimate these sources and sinks. We are continuing work to develop annual comparisons of these diverse methods in order to clarify what they all actually calculate and to resolve apparent disagreement, in addition to highlighting opportunities for increased understanding.
Lea Fink, Matthias Karl, Volker Matthias, Sonia Oppo, Richard Kranenburg, Jeroen Kuenen, Sara Jutterström, Jana Moldanova, Elisa Majamäki, and Jukka-Pekka Jalkanen
Atmos. Chem. Phys., 23, 10163–10189, https://doi.org/10.5194/acp-23-10163-2023, https://doi.org/10.5194/acp-23-10163-2023, 2023
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The Mediterranean Sea is a heavily trafficked shipping area, and air quality monitoring stations in numerous cities along the Mediterranean coast have detected high levels of air pollutants originating from shipping emissions. The current study investigates how existing restrictions on shipping-related emissions to the atmosphere ensure compliance with legislation. Focus was laid on fine particles and particle species, which were simulated with five different chemical transport models.
Jean-Philippe Putaud, Enrico Pisoni, Alexander Mangold, Christoph Hueglin, Jean Sciare, Michael Pikridas, Chrysanthos Savvides, Jakub Ondracek, Saliou Mbengue, Alfred Wiedensohler, Kay Weinhold, Maik Merkel, Laurent Poulain, Dominik van Pinxteren, Hartmut Herrmann, Andreas Massling, Claus Nordstroem, Andrés Alastuey, Cristina Reche, Noemí Pérez, Sonia Castillo, Mar Sorribas, Jose Antonio Adame, Tuukka Petaja, Katrianne Lehtipalo, Jarkko Niemi, Véronique Riffault, Joel F. de Brito, Augustin Colette, Olivier Favez, Jean-Eudes Petit, Valérie Gros, Maria I. Gini, Stergios Vratolis, Konstantinos Eleftheriadis, Evangelia Diapouli, Hugo Denier van der Gon, Karl Espen Yttri, and Wenche Aas
Atmos. Chem. Phys., 23, 10145–10161, https://doi.org/10.5194/acp-23-10145-2023, https://doi.org/10.5194/acp-23-10145-2023, 2023
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Many European people are still exposed to levels of air pollution that can affect their health. COVID-19 lockdowns in 2020 were used to assess the impact of the reduction in human mobility on air pollution across Europe by comparing measurement data with values that would be expected if no lockdown had occurred. We show that lockdown measures did not lead to consistent decreases in the concentrations of fine particulate matter suspended in the air, and we investigate why.
Christian Hogrefe, Jesse O. Bash, Jonathan E. Pleim, Donna B. Schwede, Robert C. Gilliam, Kristen M. Foley, K. Wyat Appel, and Rohit Mathur
Atmos. Chem. Phys., 23, 8119–8147, https://doi.org/10.5194/acp-23-8119-2023, https://doi.org/10.5194/acp-23-8119-2023, 2023
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Under the umbrella of the fourth phase of the Air Quality Model Evaluation International Initiative (AQMEII4), this study applies AQMEII4 diagnostic tools to better characterize how dry deposition removes pollutants from the atmosphere in the widely used CMAQ model. The results illustrate how these tools can provide insights into similarities and differences between the two CMAQ dry deposition options that affect simulated pollutant budgets and ecosystem impacts from atmospheric pollution.
Marc Guevara, Hervé Petetin, Oriol Jorba, Hugo Denier van der Gon, Jeroen Kuenen, Ingrid Super, Claire Granier, Thierno Doumbia, Philippe Ciais, Zhu Liu, Robin D. Lamboll, Sabine Schindlbacher, Bradley Matthews, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 23, 8081–8101, https://doi.org/10.5194/acp-23-8081-2023, https://doi.org/10.5194/acp-23-8081-2023, 2023
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This study provides an intercomparison of European 2020 emission changes derived from official inventories, which are reported by countries under the framework of several international conventions and directives, and non-official near-real-time estimates, the use of which has significantly grown since the COVID-19 outbreak. The results of the work are used to produce recommendations on how best to approach and make use of near-real-time emissions for modelling and monitoring applications.
Marianne Tronstad Lund, Gunnar Myhre, Ragnhild Bieltvedt Skeie, Bjørn Hallvard Samset, and Zbigniew Klimont
Atmos. Chem. Phys., 23, 6647–6662, https://doi.org/10.5194/acp-23-6647-2023, https://doi.org/10.5194/acp-23-6647-2023, 2023
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Here we show that differences, in magnitude and trend, between recent global anthropogenic emission inventories have a notable influence on simulated regional abundances of anthropogenic aerosol over the 1990–2019 period. This, in turn, affects estimates of radiative forcing. Our findings form a basis for comparing existing and upcoming studies on anthropogenic aerosols using different emission inventories.
Havala O. T. Pye, Bryan K. Place, Benjamin N. Murphy, Karl M. Seltzer, Emma L. D'Ambro, Christine Allen, Ivan R. Piletic, Sara Farrell, Rebecca H. Schwantes, Matthew M. Coggon, Emily Saunders, Lu Xu, Golam Sarwar, William T. Hutzell, Kristen M. Foley, George Pouliot, Jesse Bash, and William R. Stockwell
Atmos. Chem. Phys., 23, 5043–5099, https://doi.org/10.5194/acp-23-5043-2023, https://doi.org/10.5194/acp-23-5043-2023, 2023
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Chemical mechanisms describe how emissions from vehicles, vegetation, and other sources are chemically transformed in the atmosphere to secondary products including criteria and hazardous air pollutants. The Community Regional Atmospheric Chemistry Multiphase Mechanism integrates gas-phase radical chemistry with pathways to fine-particle mass. New species were implemented, resulting in a bottom-up representation of organic aerosol, which is required for accurate source attribution of pollutants.
Qian Shu, Sergey L. Napelenok, William T. Hutzell, Kirk R. Baker, Barron H. Henderson, Benjamin N. Murphy, and Christian Hogrefe
Geosci. Model Dev., 16, 2303–2322, https://doi.org/10.5194/gmd-16-2303-2023, https://doi.org/10.5194/gmd-16-2303-2023, 2023
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Source attribution methods are generally used to determine culpability of precursor emission sources to ambient pollutant concentrations. However, source attribution of secondarily formed pollutants such as ozone and its precursors cannot be explicitly measured, making evaluation of source apportionment methods challenging. In this study, multiple apportionment approach comparisons show common features but still reveal wide variations in predicted sector contribution and species dependency.
Shixian Zhai, Daniel J. Jacob, Drew C. Pendergrass, Nadia K. Colombi, Viral Shah, Laura Hyesung Yang, Qiang Zhang, Shuxiao Wang, Hwajin Kim, Yele Sun, Jin-Soo Choi, Jin-Soo Park, Gan Luo, Fangqun Yu, Jung-Hun Woo, Younha Kim, Jack E. Dibb, Taehyoung Lee, Jin-Seok Han, Bruce E. Anderson, Ke Li, and Hong Liao
Atmos. Chem. Phys., 23, 4271–4281, https://doi.org/10.5194/acp-23-4271-2023, https://doi.org/10.5194/acp-23-4271-2023, 2023
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Anthropogenic fugitive dust in East Asia not only causes severe coarse particulate matter air pollution problems, but also affects fine particulate nitrate. Due to emission control efforts, coarse PM decreased steadily. We find that the decrease of coarse PM is a major driver for a lack of decrease of fine particulate nitrate, as it allows more nitric acid to form fine particulate nitrate. The continuing decrease of coarse PM requires more stringent ammonia and nitrogen oxides emission controls.
Ana Maria Roxana Petrescu, Chunjing Qiu, Matthew J. McGrath, Philippe Peylin, Glen P. Peters, Philippe Ciais, Rona L. Thompson, Aki Tsuruta, Dominik Brunner, Matthias Kuhnert, Bradley Matthews, Paul I. Palmer, Oksana Tarasova, Pierre Regnier, Ronny Lauerwald, David Bastviken, Lena Höglund-Isaksson, Wilfried Winiwarter, Giuseppe Etiope, Tuula Aalto, Gianpaolo Balsamo, Vladislav Bastrikov, Antoine Berchet, Patrick Brockmann, Giancarlo Ciotoli, Giulia Conchedda, Monica Crippa, Frank Dentener, Christine D. Groot Zwaaftink, Diego Guizzardi, Dirk Günther, Jean-Matthieu Haussaire, Sander Houweling, Greet Janssens-Maenhout, Massaer Kouyate, Adrian Leip, Antti Leppänen, Emanuele Lugato, Manon Maisonnier, Alistair J. Manning, Tiina Markkanen, Joe McNorton, Marilena Muntean, Gabriel D. Oreggioni, Prabir K. Patra, Lucia Perugini, Isabelle Pison, Maarit T. Raivonen, Marielle Saunois, Arjo J. Segers, Pete Smith, Efisio Solazzo, Hanqin Tian, Francesco N. Tubiello, Timo Vesala, Guido R. van der Werf, Chris Wilson, and Sönke Zaehle
Earth Syst. Sci. Data, 15, 1197–1268, https://doi.org/10.5194/essd-15-1197-2023, https://doi.org/10.5194/essd-15-1197-2023, 2023
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This study updates the state-of-the-art scientific overview of CH4 and N2O emissions in the EU27 and UK in Petrescu et al. (2021a). Yearly updates are needed to improve the different respective approaches and to inform on the development of formal verification systems. It integrates the most recent emission inventories, process-based model and regional/global inversions, comparing them with UNFCCC national GHG inventories, in support to policy to facilitate real-time verification procedures.
Robin N. Thor, Mariano Mertens, Sigrun Matthes, Mattia Righi, Johannes Hendricks, Sabine Brinkop, Phoebe Graf, Volker Grewe, Patrick Jöckel, and Steven Smith
Geosci. Model Dev., 16, 1459–1466, https://doi.org/10.5194/gmd-16-1459-2023, https://doi.org/10.5194/gmd-16-1459-2023, 2023
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We report on an inconsistency in the latitudinal distribution of aviation emissions between two versions of a data product which is widely used by researchers. From the available documentation, we do not expect such an inconsistency. We run a chemistry–climate model to compute the effect of the inconsistency in emissions on atmospheric chemistry and radiation and find that the radiative forcing associated with aviation ozone is 7.6 % higher when using the less recent version of the data.
Edward C. Chan, Joana Leitão, Andreas Kerschbaumer, and Timothy M. Butler
Geosci. Model Dev., 16, 1427–1444, https://doi.org/10.5194/gmd-16-1427-2023, https://doi.org/10.5194/gmd-16-1427-2023, 2023
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Yeti is a Handbook Emission Factors for Road Transport-based traffic emission inventory written in the Python 3 scripting language, which adopts a generalized treatment for activity data using traffic information of varying levels of detail introduced in a systematic and consistent manner, with the ability to maximize reusability. Thus, Yeti has been conceived and implemented with a high degree of data and process symmetry, allowing scalable and flexible execution while affording ease of use.
Lea Fink, Matthias Karl, Volker Matthias, Sonia Oppo, Richard Kranenburg, Jeroen Kuenen, Jana Moldanova, Sara Jutterström, Jukka-Pekka Jalkanen, and Elisa Majamäki
Atmos. Chem. Phys., 23, 1825–1862, https://doi.org/10.5194/acp-23-1825-2023, https://doi.org/10.5194/acp-23-1825-2023, 2023
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Potential ship impact on air pollution in the Mediterranean Sea was simulated with five chemistry transport models. An evaluation of the results for NO2 and O3 air concentrations and dry deposition is presented. Emission data, modeled year and domain were the same. Model run outputs were compared to measurements from background stations. We focused on comparing model outputs regarding the concentration of regulatory pollutants and the relative ship impact on total air pollution concentrations.
James D. East, Barron H. Henderson, Sergey L. Napelenok, Shannon N. Koplitz, Golam Sarwar, Robert Gilliam, Allen Lenzen, Daniel Q. Tong, R. Bradley Pierce, and Fernando Garcia-Menendez
Atmos. Chem. Phys., 22, 15981–16001, https://doi.org/10.5194/acp-22-15981-2022, https://doi.org/10.5194/acp-22-15981-2022, 2022
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We present a framework that uses a computer model of air quality, along with air pollution data from satellite instruments, to estimate emissions of nitrogen oxides (NOx) across the Northern Hemisphere. The framework, which advances current methods to infer emissions from satellite observations, provides observationally constrained NOx estimates, including in regions of the world where emissions are highly uncertain, and can improve simulations of air pollutants relevant for health and policy.
Felix Kleinert, Lukas H. Leufen, Aurelia Lupascu, Tim Butler, and Martin G. Schultz
Geosci. Model Dev., 15, 8913–8930, https://doi.org/10.5194/gmd-15-8913-2022, https://doi.org/10.5194/gmd-15-8913-2022, 2022
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We examine the effects of spatially aggregated upstream information as input for a deep learning model forecasting near-surface ozone levels. Using aggregated data from one upstream sector (45°) improves the forecast by ~ 10 % for 4 prediction days. Three upstream sectors improve the forecasts by ~ 14 % on the first 2 d only. Our results serve as an orientation for other researchers or environmental agencies focusing on pointwise time-series predictions, for example, due to regulatory purposes.
Johana Romero-Alvarez, Aurelia Lupaşcu, Douglas Lowe, Alba Badia, Scott Archer-Nicholls, Steve Dorling, Claire E. Reeves, and Tim Butler
Atmos. Chem. Phys., 22, 13797–13815, https://doi.org/10.5194/acp-22-13797-2022, https://doi.org/10.5194/acp-22-13797-2022, 2022
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As ozone can be transported across countries, efficient air quality management and regulatory policies rely on the assessment of local ozone production vs. transport. In our study, we investigate the origin of surface ozone in the UK and the contribution of the different source regions to regulatory ozone metrics. It is shown that emission controls would be necessary over western Europe to improve health-related metrics and over larger areas to reduce impacts on ecosystems.
Steven J. Smith, Erin E. McDuffie, and Molly Charles
Atmos. Chem. Phys., 22, 13201–13218, https://doi.org/10.5194/acp-22-13201-2022, https://doi.org/10.5194/acp-22-13201-2022, 2022
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Emissions into the atmosphere of greenhouse gases (GHGs) and air pollutants, quantified in emission inventories, impact human health, ecosystems, and the climate. We review how air pollutant and GHG inventory activities have historically been structured and their different uses and requirements. We discuss the benefits of increasing coordination between air pollutant and GHG inventory development efforts, but also caution that there are differences in appropriate methodologies and applications.
Sarah E. Benish, Jesse O. Bash, Kristen M. Foley, K. Wyat Appel, Christian Hogrefe, Robert Gilliam, and George Pouliot
Atmos. Chem. Phys., 22, 12749–12767, https://doi.org/10.5194/acp-22-12749-2022, https://doi.org/10.5194/acp-22-12749-2022, 2022
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We assess Community Multiscale Air Quality (CMAQ) model simulations of nitrogen and sulfur deposition over US climate regions to evaluate the model ability to reproduce long-term deposition trends and total deposition budgets. A measurement–model fusion technique is found to improve estimates of wet deposition. Emission controls set by the Clean Air Act successfully decreased oxidized nitrogen deposition across the US; we find increasing amounts of reduced nitrogen to the total nitrogen budget.
Johannes Quaas, Hailing Jia, Chris Smith, Anna Lea Albright, Wenche Aas, Nicolas Bellouin, Olivier Boucher, Marie Doutriaux-Boucher, Piers M. Forster, Daniel Grosvenor, Stuart Jenkins, Zbigniew Klimont, Norman G. Loeb, Xiaoyan Ma, Vaishali Naik, Fabien Paulot, Philip Stier, Martin Wild, Gunnar Myhre, and Michael Schulz
Atmos. Chem. Phys., 22, 12221–12239, https://doi.org/10.5194/acp-22-12221-2022, https://doi.org/10.5194/acp-22-12221-2022, 2022
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Pollution particles cool climate and offset part of the global warming. However, they are washed out by rain and thus their effect responds quickly to changes in emissions. We show multiple datasets to demonstrate that aerosol emissions and their concentrations declined in many regions influenced by human emissions, as did the effects on clouds. Consequently, the cooling impact on the Earth energy budget became smaller. This change in trend implies a relative warming.
Aurelia Lupaşcu, Noelia Otero, Andrea Minkos, and Tim Butler
Atmos. Chem. Phys., 22, 11675–11699, https://doi.org/10.5194/acp-22-11675-2022, https://doi.org/10.5194/acp-22-11675-2022, 2022
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Ground-level ozone is an important air pollutant that affects human health, ecosystems, and climate. Ozone is not emitted directly but rather formed in the atmosphere through chemical reactions involving two distinct precursors. Our results provide detailed information about the origin of ozone in Germany during two peak ozone events that took place in 2015 and 2018, thus improving our understanding of ground-level ozone.
Philippe Thunis, Alain Clappier, Enrico Pisoni, Bertrand Bessagnet, Jeroen Kuenen, Marc Guevara, and Susana Lopez-Aparicio
Geosci. Model Dev., 15, 5271–5286, https://doi.org/10.5194/gmd-15-5271-2022, https://doi.org/10.5194/gmd-15-5271-2022, 2022
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In this work, we propose a screening method to improve the quality of emission inventories, which are responsible for large uncertainties in air-quality modeling. The first step of screening consists of keeping only emission contributions that are relevant enough. In a second step, the method identifies large differences that provide evidence of methodological divergence or errors. We used the approach to compare two versions of the CAMS-REG European-scale inventory over 150 European cities.
Katherine R. Travis, James H. Crawford, Gao Chen, Carolyn E. Jordan, Benjamin A. Nault, Hwajin Kim, Jose L. Jimenez, Pedro Campuzano-Jost, Jack E. Dibb, Jung-Hun Woo, Younha Kim, Shixian Zhai, Xuan Wang, Erin E. McDuffie, Gan Luo, Fangqun Yu, Saewung Kim, Isobel J. Simpson, Donald R. Blake, Limseok Chang, and Michelle J. Kim
Atmos. Chem. Phys., 22, 7933–7958, https://doi.org/10.5194/acp-22-7933-2022, https://doi.org/10.5194/acp-22-7933-2022, 2022
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The 2016 Korea–United States Air Quality (KORUS-AQ) field campaign provided a unique set of observations to improve our understanding of PM2.5 pollution in South Korea. Models typically have errors in simulating PM2.5 in this region, which is of concern for the development of control measures. We use KORUS-AQ observations to improve our understanding of the mechanisms driving PM2.5 and the implications of model errors for determining PM2.5 that is attributable to local or foreign sources.
Marc Guevara, Hervé Petetin, Oriol Jorba, Hugo Denier van der Gon, Jeroen Kuenen, Ingrid Super, Jukka-Pekka Jalkanen, Elisa Majamäki, Lasse Johansson, Vincent-Henri Peuch, and Carlos Pérez García-Pando
Earth Syst. Sci. Data, 14, 2521–2552, https://doi.org/10.5194/essd-14-2521-2022, https://doi.org/10.5194/essd-14-2521-2022, 2022
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To control the spread of the COVID-19 disease, European governments implemented mobility restriction measures that resulted in an unprecedented drop in anthropogenic emissions. This work presents a dataset of emission adjustment factors that allows quantifying changes in 2020 European primary emissions per country and pollutant sector at the daily scale. The resulting dataset can be used as input in modelling studies aiming at quantifying the impact of COVID-19 on air quality levels.
Cynthia H. Whaley, Rashed Mahmood, Knut von Salzen, Barbara Winter, Sabine Eckhardt, Stephen Arnold, Stephen Beagley, Silvia Becagli, Rong-You Chien, Jesper Christensen, Sujay Manish Damani, Xinyi Dong, Konstantinos Eleftheriadis, Nikolaos Evangeliou, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Fabio Giardi, Wanmin Gong, Jens Liengaard Hjorth, Lin Huang, Ulas Im, Yugo Kanaya, Srinath Krishnan, Zbigniew Klimont, Thomas Kühn, Joakim Langner, Kathy S. Law, Louis Marelle, Andreas Massling, Dirk Olivié, Tatsuo Onishi, Naga Oshima, Yiran Peng, David A. Plummer, Olga Popovicheva, Luca Pozzoli, Jean-Christophe Raut, Maria Sand, Laura N. Saunders, Julia Schmale, Sangeeta Sharma, Ragnhild Bieltvedt Skeie, Henrik Skov, Fumikazu Taketani, Manu A. Thomas, Rita Traversi, Kostas Tsigaridis, Svetlana Tsyro, Steven Turnock, Vito Vitale, Kaley A. Walker, Minqi Wang, Duncan Watson-Parris, and Tahya Weiss-Gibbons
Atmos. Chem. Phys., 22, 5775–5828, https://doi.org/10.5194/acp-22-5775-2022, https://doi.org/10.5194/acp-22-5775-2022, 2022
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Air pollutants, like ozone and soot, play a role in both global warming and air quality. Atmospheric models are often used to provide information to policy makers about current and future conditions under different emissions scenarios. In order to have confidence in those simulations, in this study we compare simulated air pollution from 18 state-of-the-art atmospheric models to measured air pollution in order to assess how well the models perform.
Andrea Pozzer, Simon F. Reifenberg, Vinod Kumar, Bruno Franco, Matthias Kohl, Domenico Taraborrelli, Sergey Gromov, Sebastian Ehrhart, Patrick Jöckel, Rolf Sander, Veronica Fall, Simon Rosanka, Vlassis Karydis, Dimitris Akritidis, Tamara Emmerichs, Monica Crippa, Diego Guizzardi, Johannes W. Kaiser, Lieven Clarisse, Astrid Kiendler-Scharr, Holger Tost, and Alexandra Tsimpidi
Geosci. Model Dev., 15, 2673–2710, https://doi.org/10.5194/gmd-15-2673-2022, https://doi.org/10.5194/gmd-15-2673-2022, 2022
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A newly developed setup of the chemistry general circulation model EMAC (ECHAM5/MESSy for Atmospheric Chemistry) is evaluated here. A comprehensive organic degradation mechanism is used and coupled with a volatility base model.
The results show that the model reproduces most of the tracers and aerosols satisfactorily but shows discrepancies for oxygenated organic gases. It is also shown that this model configuration can be used for further research in atmospheric chemistry.
Sumanta Sarkhel, Gunter Stober, Jorge L. Chau, Steven M. Smith, Christoph Jacobi, Subarna Mondal, Martin G. Mlynczak, and James M. Russell III
Ann. Geophys., 40, 179–190, https://doi.org/10.5194/angeo-40-179-2022, https://doi.org/10.5194/angeo-40-179-2022, 2022
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A rare gravity wave event was observed on the night of 25 April 2017 over northern Germany. An all-sky airglow imager recorded an upward-propagating wave at different altitudes in mesosphere with a prominent wave front above 91 km and faintly observed below. Based on wind and satellite-borne temperature profiles close to the event location, we have found the presence of a leaky thermal duct layer in 85–91 km. The appearance of this duct layer caused the wave amplitudes to diminish below 91 km.
Noelia Otero, Oscar E. Jurado, Tim Butler, and Henning W. Rust
Atmos. Chem. Phys., 22, 1905–1919, https://doi.org/10.5194/acp-22-1905-2022, https://doi.org/10.5194/acp-22-1905-2022, 2022
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Surface ozone and temperature are strongly dependent and their extremes might be exacerbated by underlying climatological drivers, such as atmospheric blocking. Using an observational data set, we measure the dependence structure between ozone and temperature under the influence of atmospheric blocking. Blocks enhanced the probability of occurrence of compound ozone and temperature extremes over northwestern and central Europe, leading to greater health risks.
Jeroen Kuenen, Stijn Dellaert, Antoon Visschedijk, Jukka-Pekka Jalkanen, Ingrid Super, and Hugo Denier van der Gon
Earth Syst. Sci. Data, 14, 491–515, https://doi.org/10.5194/essd-14-491-2022, https://doi.org/10.5194/essd-14-491-2022, 2022
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This paper presents an 18-year time series for anthropogenic emissions for the main air pollutants in Europe, distinguishing 15 main source categories. It provides a complete overview of emissions to air and is designed to support air quality modelling. The data build where possible on official country total emissions used in the policy processes, but where necessary alternative data were used. The emission data are spatially distributed at high resolution (~ 6 km x 6 km) in a consistent way.
Fei Liu, Zhining Tao, Steffen Beirle, Joanna Joiner, Yasuko Yoshida, Steven J. Smith, K. Emma Knowland, and Thomas Wagner
Atmos. Chem. Phys., 22, 1333–1349, https://doi.org/10.5194/acp-22-1333-2022, https://doi.org/10.5194/acp-22-1333-2022, 2022
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In this work, we present a novel method to infer NOx emissions and lifetimes based on tropospheric NO2 observations together with reanalysis wind fields for cities located in polluted backgrounds. We evaluate the accuracy of the method using synthetic NO2 observations derived from a high-resolution model simulation. Our work provides an estimate for uncertainties in satellite-derived emissions inferred from chemical transport model (CTM)-independent approaches.
Mahtab Majdzadeh, Craig A. Stroud, Christopher Sioris, Paul A. Makar, Ayodeji Akingunola, Chris McLinden, Xiaoyi Zhao, Michael D. Moran, Ihab Abboud, and Jack Chen
Geosci. Model Dev., 15, 219–249, https://doi.org/10.5194/gmd-15-219-2022, https://doi.org/10.5194/gmd-15-219-2022, 2022
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A new lookup table for aerosol optical properties based on a Mie scattering code was calculated and adopted within an improved version of the photolysis module in the GEM-MACH in-line chemical transport model. The modified version of the photolysis module makes use of online interactive aerosol feedback and applies core-shell parameterizations to the black carbon absorption efficiency based on Bond et al. (2006) to the size bins with black carbon mass fraction of less than 40 %.
Xiao Lu, Daniel J. Jacob, Haolin Wang, Joannes D. Maasakkers, Yuzhong Zhang, Tia R. Scarpelli, Lu Shen, Zhen Qu, Melissa P. Sulprizio, Hannah Nesser, A. Anthony Bloom, Shuang Ma, John R. Worden, Shaojia Fan, Robert J. Parker, Hartmut Boesch, Ritesh Gautam, Deborah Gordon, Michael D. Moran, Frances Reuland, Claudia A. Octaviano Villasana, and Arlyn Andrews
Atmos. Chem. Phys., 22, 395–418, https://doi.org/10.5194/acp-22-395-2022, https://doi.org/10.5194/acp-22-395-2022, 2022
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We evaluate methane emissions and trends for 2010–2017 in the gridded national emission inventories for the United States, Canada, and Mexico by inversion of in situ and satellite methane observations. We find that anthropogenic methane emissions for all three countries are underestimated in the national inventories, largely driven by oil emissions. Anthropogenic methane emissions in the US peak in 2014, in contrast to the report of a steadily decreasing trend over 2010–2017 from the US EPA.
Philippe Thunis, Alain Clappier, Alexander de Meij, Enrico Pisoni, Bertrand Bessagnet, and Leonor Tarrason
Atmos. Chem. Phys., 21, 18195–18212, https://doi.org/10.5194/acp-21-18195-2021, https://doi.org/10.5194/acp-21-18195-2021, 2021
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Air pollution's origin in cities is still a point of discussion, and approaches to assess the city's responsibility for its pollution are not harmonized and thus not comparable, resulting in sometimes contradicting interpretations. We show that methodological choices can easily lead to differences of a factor of 2 in terms of responsibility outcome and stress that methodological choices and assumptions most often lead to a systematic and important underestimation of the city's responsibility.
Shixian Zhai, Daniel J. Jacob, Jared F. Brewer, Ke Li, Jonathan M. Moch, Jhoon Kim, Seoyoung Lee, Hyunkwang Lim, Hyun Chul Lee, Su Keun Kuk, Rokjin J. Park, Jaein I. Jeong, Xuan Wang, Pengfei Liu, Gan Luo, Fangqun Yu, Jun Meng, Randall V. Martin, Katherine R. Travis, Johnathan W. Hair, Bruce E. Anderson, Jack E. Dibb, Jose L. Jimenez, Pedro Campuzano-Jost, Benjamin A. Nault, Jung-Hun Woo, Younha Kim, Qiang Zhang, and Hong Liao
Atmos. Chem. Phys., 21, 16775–16791, https://doi.org/10.5194/acp-21-16775-2021, https://doi.org/10.5194/acp-21-16775-2021, 2021
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Geostationary satellite aerosol optical depth (AOD) has tremendous potential for monitoring surface fine particulate matter (PM2.5). Our study explored the physical relationship between AOD and PM2.5 by integrating data from surface networks, aircraft, and satellites with the GEOS-Chem chemical transport model. We quantitatively showed that accurate simulation of aerosol size distributions, boundary layer depths, relative humidity, coarse particles, and diurnal variations in PM2.5 are essential.
Margarita Choulga, Greet Janssens-Maenhout, Ingrid Super, Efisio Solazzo, Anna Agusti-Panareda, Gianpaolo Balsamo, Nicolas Bousserez, Monica Crippa, Hugo Denier van der Gon, Richard Engelen, Diego Guizzardi, Jeroen Kuenen, Joe McNorton, Gabriel Oreggioni, and Antoon Visschedijk
Earth Syst. Sci. Data, 13, 5311–5335, https://doi.org/10.5194/essd-13-5311-2021, https://doi.org/10.5194/essd-13-5311-2021, 2021
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People worry that growing man-made carbon dioxide (CO2) concentrations lead to climate change. Global models, use of observations, and datasets can help us better understand behaviour of CO2. Here a tool to compute uncertainty in man-made CO2 sources per country per year and month is presented. An example of all sources separated into seven groups (intensive and average energy, industry, humans, ground and air transport, others) is presented. Results will be used to predict CO2 concentrations.
Jan C. Minx, William F. Lamb, Robbie M. Andrew, Josep G. Canadell, Monica Crippa, Niklas Döbbeling, Piers M. Forster, Diego Guizzardi, Jos Olivier, Glen P. Peters, Julia Pongratz, Andy Reisinger, Matthew Rigby, Marielle Saunois, Steven J. Smith, Efisio Solazzo, and Hanqin Tian
Earth Syst. Sci. Data, 13, 5213–5252, https://doi.org/10.5194/essd-13-5213-2021, https://doi.org/10.5194/essd-13-5213-2021, 2021
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We provide a synthetic dataset on anthropogenic greenhouse gas (GHG) emissions for 1970–2018 with a fast-track extension to 2019. We show that GHG emissions continued to rise across all gases and sectors. Annual average GHG emissions growth slowed, but absolute decadal increases have never been higher in human history. We identify a number of data gaps and data quality issues in global inventories and highlight their importance for monitoring progress towards international climate goals.
Stefano Galmarini, Paul Makar, Olivia E. Clifton, Christian Hogrefe, Jesse O. Bash, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Tim Butler, Jason Ducker, Johannes Flemming, Alma Hodzic, Christopher D. Holmes, Ioannis Kioutsioukis, Richard Kranenburg, Aurelia Lupascu, Juan Luis Perez-Camanyo, Jonathan Pleim, Young-Hee Ryu, Roberto San Jose, Donna Schwede, Sam Silva, and Ralf Wolke
Atmos. Chem. Phys., 21, 15663–15697, https://doi.org/10.5194/acp-21-15663-2021, https://doi.org/10.5194/acp-21-15663-2021, 2021
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This technical note presents the research protocols for phase 4 of the Air Quality Model Evaluation International Initiative (AQMEII4). This initiative has three goals: (i) to define the state of wet and dry deposition in regional models, (ii) to evaluate how dry deposition influences air concentration and flux predictions, and (iii) to identify the causes for prediction differences. The evaluation compares LULC-specific dry deposition and effective conductances and fluxes.
Jessica L. McCarty, Juha Aalto, Ville-Veikko Paunu, Steve R. Arnold, Sabine Eckhardt, Zbigniew Klimont, Justin J. Fain, Nikolaos Evangeliou, Ari Venäläinen, Nadezhda M. Tchebakova, Elena I. Parfenova, Kaarle Kupiainen, Amber J. Soja, Lin Huang, and Simon Wilson
Biogeosciences, 18, 5053–5083, https://doi.org/10.5194/bg-18-5053-2021, https://doi.org/10.5194/bg-18-5053-2021, 2021
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Fires, including extreme fire seasons, and fire emissions are more common in the Arctic. A review and synthesis of current scientific literature find climate change and human activity in the north are fuelling an emerging Arctic fire regime, causing more black carbon and methane emissions within the Arctic. Uncertainties persist in characterizing future fire landscapes, and thus emissions, as well as policy-relevant challenges in understanding, monitoring, and managing Arctic fire regimes.
Albana Kona, Fabio Monforti-Ferrario, Paolo Bertoldi, Marta Giulia Baldi, Georgia Kakoulaki, Nadja Vetters, Christian Thiel, Giulia Melica, Eleonora Lo Vullo, Alessandra Sgobbi, Christofer Ahlgren, and Brieuc Posnic
Earth Syst. Sci. Data, 13, 3551–3564, https://doi.org/10.5194/essd-13-3551-2021, https://doi.org/10.5194/essd-13-3551-2021, 2021
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The Global Covenant of Mayors for Climate & Energy (GCoM), the largest international initiative to promote climate action at the city level, has collected a large amount of information on urban greenhouse gas emissions.
Here we present the harmonised, completed and verified GCoM emission dataset, originating from 6200 cities among its signatories, complemented with a set of useful ancillary data. This knowledge will contribute to covering the lack of consistent datasets of cities' emissions.
Edward C. Chan and Timothy M. Butler
Geosci. Model Dev., 14, 4555–4572, https://doi.org/10.5194/gmd-14-4555-2021, https://doi.org/10.5194/gmd-14-4555-2021, 2021
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A large-eddy simulation based chemical transport model is implemented for an idealized street canyon. The dynamics of the model are evaluated using stationary measurements. A transient model run is also conducted over a 24 h period, where variations of pollutant concentrations indicate dependence on emissions, background concentrations, and solar state. Comparison stationary model runs show changes in flow structure concentrations.
Ulas Im, Kostas Tsigaridis, Gregory Faluvegi, Peter L. Langen, Joshua P. French, Rashed Mahmood, Manu A. Thomas, Knut von Salzen, Daniel C. Thomas, Cynthia H. Whaley, Zbigniew Klimont, Henrik Skov, and Jørgen Brandt
Atmos. Chem. Phys., 21, 10413–10438, https://doi.org/10.5194/acp-21-10413-2021, https://doi.org/10.5194/acp-21-10413-2021, 2021
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Future (2015–2050) simulations of the aerosol burdens and their radiative forcing and climate impacts over the Arctic under various emission projections show that although the Arctic aerosol burdens are projected to decrease significantly by 10 to 60 %, regardless of the magnitude of aerosol reductions, surface air temperatures will continue to increase by 1.9–2.6 ℃, while sea-ice extent will continue to decrease, implying reductions of greenhouse gases are necessary to mitigate climate change.
Syuichi Itahashi, Baozhu Ge, Keiichi Sato, Zhe Wang, Junichi Kurokawa, Jiani Tan, Kan Huang, Joshua S. Fu, Xuemei Wang, Kazuyo Yamaji, Tatsuya Nagashima, Jie Li, Mizuo Kajino, Gregory R. Carmichael, and Zifa Wang
Atmos. Chem. Phys., 21, 8709–8734, https://doi.org/10.5194/acp-21-8709-2021, https://doi.org/10.5194/acp-21-8709-2021, 2021
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This study presents the detailed analysis of acid deposition over southeast Asia based on the Model Inter-Comparison Study for Asia (MICS-Asia) phase III. Simulated wet deposition is evaluated with observation data from the Acid Deposition Monitoring Network in East Asia (EANET). The difficulties of models to capture observations are related to the model performance on precipitation. The precipitation-adjusted approach was applied, and the distribution of wet deposition was successfully revised.
Benjamin N. Murphy, Christopher G. Nolte, Fahim Sidi, Jesse O. Bash, K. Wyat Appel, Carey Jang, Daiwen Kang, James Kelly, Rohit Mathur, Sergey Napelenok, George Pouliot, and Havala O. T. Pye
Geosci. Model Dev., 14, 3407–3420, https://doi.org/10.5194/gmd-14-3407-2021, https://doi.org/10.5194/gmd-14-3407-2021, 2021
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The algorithms for applying air pollution emission rates in the Community Multiscale Air Quality (CMAQ) model have been improved to better support users and developers. The new features accommodate emissions perturbation studies that are typical in atmospheric research and output a wealth of metadata for each model run so assumptions can be verified and documented. The new approach dramatically enhances the transparency and functionality of this critical aspect of atmospheric modeling.
Ana Maria Roxana Petrescu, Chunjing Qiu, Philippe Ciais, Rona L. Thompson, Philippe Peylin, Matthew J. McGrath, Efisio Solazzo, Greet Janssens-Maenhout, Francesco N. Tubiello, Peter Bergamaschi, Dominik Brunner, Glen P. Peters, Lena Höglund-Isaksson, Pierre Regnier, Ronny Lauerwald, David Bastviken, Aki Tsuruta, Wilfried Winiwarter, Prabir K. Patra, Matthias Kuhnert, Gabriel D. Oreggioni, Monica Crippa, Marielle Saunois, Lucia Perugini, Tiina Markkanen, Tuula Aalto, Christine D. Groot Zwaaftink, Hanqin Tian, Yuanzhi Yao, Chris Wilson, Giulia Conchedda, Dirk Günther, Adrian Leip, Pete Smith, Jean-Matthieu Haussaire, Antti Leppänen, Alistair J. Manning, Joe McNorton, Patrick Brockmann, and Albertus Johannes Dolman
Earth Syst. Sci. Data, 13, 2307–2362, https://doi.org/10.5194/essd-13-2307-2021, https://doi.org/10.5194/essd-13-2307-2021, 2021
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This study is topical and provides a state-of-the-art scientific overview of data availability from bottom-up and top-down CH4 and N2O emissions in the EU27 and UK. The data integrate recent emission inventories with process-based model data and regional/global inversions for the European domain, aiming at reconciling them with official country-level UNFCCC national GHG inventories in support to policy and to facilitate real-time verification procedures.
Ana Maria Roxana Petrescu, Matthew J. McGrath, Robbie M. Andrew, Philippe Peylin, Glen P. Peters, Philippe Ciais, Gregoire Broquet, Francesco N. Tubiello, Christoph Gerbig, Julia Pongratz, Greet Janssens-Maenhout, Giacomo Grassi, Gert-Jan Nabuurs, Pierre Regnier, Ronny Lauerwald, Matthias Kuhnert, Juraj Balkovič, Mart-Jan Schelhaas, Hugo A. C. Denier van der
Gon, Efisio Solazzo, Chunjing Qiu, Roberto Pilli, Igor B. Konovalov, Richard A. Houghton, Dirk Günther, Lucia Perugini, Monica Crippa, Raphael Ganzenmüller, Ingrid T. Luijkx, Pete Smith, Saqr Munassar, Rona L. Thompson, Giulia Conchedda, Guillaume Monteil, Marko Scholze, Ute Karstens, Patrick Brockmann, and Albertus Johannes Dolman
Earth Syst. Sci. Data, 13, 2363–2406, https://doi.org/10.5194/essd-13-2363-2021, https://doi.org/10.5194/essd-13-2363-2021, 2021
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This study is topical and provides a state-of-the-art scientific overview of data availability from bottom-up and top-down CO2 fossil emissions and CO2 land fluxes in the EU27+UK. The data integrate recent emission inventories with ecosystem data, land carbon models and regional/global inversions for the European domain, aiming at reconciling CO2 estimates with official country-level UNFCCC national GHG inventories in support to policy and facilitating real-time verification procedures.
K. Wyat Appel, Jesse O. Bash, Kathleen M. Fahey, Kristen M. Foley, Robert C. Gilliam, Christian Hogrefe, William T. Hutzell, Daiwen Kang, Rohit Mathur, Benjamin N. Murphy, Sergey L. Napelenok, Christopher G. Nolte, Jonathan E. Pleim, George A. Pouliot, Havala O. T. Pye, Limei Ran, Shawn J. Roselle, Golam Sarwar, Donna B. Schwede, Fahim I. Sidi, Tanya L. Spero, and David C. Wong
Geosci. Model Dev., 14, 2867–2897, https://doi.org/10.5194/gmd-14-2867-2021, https://doi.org/10.5194/gmd-14-2867-2021, 2021
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This paper details the scientific updates in the recently released CMAQ version 5.3 (and v5.3.1) and also includes operational and diagnostic evaluations of CMAQv5.3.1 against observations and the previous version of the CMAQ (v5.2.1). This work was done to improve the underlying science in CMAQ. This article is used to inform the CMAQ modeling community of the updates to the modeling system and the expected change in model performance from these updates (versus the previous model version).
Jean-Philippe Putaud, Luca Pozzoli, Enrico Pisoni, Sebastiao Martins Dos Santos, Friedrich Lagler, Guido Lanzani, Umberto Dal Santo, and Augustin Colette
Atmos. Chem. Phys., 21, 7597–7609, https://doi.org/10.5194/acp-21-7597-2021, https://doi.org/10.5194/acp-21-7597-2021, 2021
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To determine the impact of the COVID lockdown on air quality in northern Italy, measurements of atmospheric pollutants (NO2, PM10, O3, NO, SO2 ) were compared to the output of a model ignoring the lockdown. We found that NO2 decreased on average by −30 % to −40 %. Unlike NO2, PM10 was not significantly affected due to the compensation of decreased emissions from traffic by increased emissions from domestic heating and/or by changes in atmospheric chemistry enhancing secondary aerosol formation.
Qian Shu, Benjamin Murphy, Jonathan E. Pleim, Donna Schwede, Barron H. Henderson, Havala O.T. Pye, Keith Wyat Appel, Tanvir R. Khan, and Judith A. Perlinger
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2021-129, https://doi.org/10.5194/gmd-2021-129, 2021
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We have bridged the gap between dry deposition measurement and modeling by rigorous use of box and regional transport models and field measurements, but more efforts are needed. This study highlights that deviation among deposition schemes is most pronounced for small and large particles. This study better links model predictions to available real-world observations and incrementally reduces uncertainties in the magnitude of loss processes important for the lifecycle of air pollutants.
Efisio Solazzo, Monica Crippa, Diego Guizzardi, Marilena Muntean, Margarita Choulga, and Greet Janssens-Maenhout
Atmos. Chem. Phys., 21, 5655–5683, https://doi.org/10.5194/acp-21-5655-2021, https://doi.org/10.5194/acp-21-5655-2021, 2021
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We conducted an extensive analysis of the structural uncertainty of the Emissions Database for Global Atmospheric Research (EDGAR) emission inventory of greenhouse gases, which adds a much needed reliability dimension to the accuracy of the emission estimates. The study undertakes in-depth analyses of the implication of aggregating emissions from different sources and/or countries on the accuracy. Results are presented for all emissions sectors according to IPCC definitions.
Elena Macdonald, Noelia Otero, and Tim Butler
Atmos. Chem. Phys., 21, 4007–4023, https://doi.org/10.5194/acp-21-4007-2021, https://doi.org/10.5194/acp-21-4007-2021, 2021
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NO2 limit values are still regularly exceeded in many European cities despite decreasing emissions. Measurements of NOx concentrations from stations across Europe were systematically analysed to assess long-term changes observed in urban areas. We compared trends in concentration increments to trends in total and traffic emissions to find potential discrepancies. The results can help in evaluating inaccuracies in emission inventories and in improving spatial imbalances in data availability.
Xiaohui Lin, Wen Zhang, Monica Crippa, Shushi Peng, Pengfei Han, Ning Zeng, Lijun Yu, and Guocheng Wang
Earth Syst. Sci. Data, 13, 1073–1088, https://doi.org/10.5194/essd-13-1073-2021, https://doi.org/10.5194/essd-13-1073-2021, 2021
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CH4 is a potent greenhouse gas, and China’s anthropogenic CH4 emissions account for a large proportion of global total emissions. However, the existing estimates either focus on a specific sector or lag behind real time by several years. We collected and analyzed 12 datasets and compared them to reveal the spatiotemporal changes and their uncertainties. We further estimated the emissions from 1990–2019, and the estimates showed a robust trend in recent years when compared to top-down results.
Marc Guevara, Oriol Jorba, Carles Tena, Hugo Denier van der Gon, Jeroen Kuenen, Nellie Elguindi, Sabine Darras, Claire Granier, and Carlos Pérez García-Pando
Earth Syst. Sci. Data, 13, 367–404, https://doi.org/10.5194/essd-13-367-2021, https://doi.org/10.5194/essd-13-367-2021, 2021
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The temporal variability of atmospheric emissions is linked to changes in activity patterns, emission processes and meteorology. Accounting for the change in temporal emission characteristics is a key aspect for modelling the trends of air pollutants. This work presents a dataset of global and European emission temporal profiles to be used for air quality modelling purposes. The profiles were constructed considering the influences of local sociodemographic factors and climatological conditions.
Francesco Canonaco, Anna Tobler, Gang Chen, Yulia Sosedova, Jay Gates Slowik, Carlo Bozzetti, Kaspar Rudolf Daellenbach, Imad El Haddad, Monica Crippa, Ru-Jin Huang, Markus Furger, Urs Baltensperger, and André Stephan Henry Prévôt
Atmos. Meas. Tech., 14, 923–943, https://doi.org/10.5194/amt-14-923-2021, https://doi.org/10.5194/amt-14-923-2021, 2021
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Long-term ambient aerosol mass spectrometric data were analyzed with a statistical model (PMF) to obtain source contributions and fingerprints. The new aspects of this paper involve time-dependent source fingerprints by a rolling technique and the replacement of the full visual inspection of each run by a user-defined set of criteria to monitor the quality of each of these runs more efficiently. More reliable sources will finally provide better instruments for political mitigation strategies.
Kalyn Dorheim, Steven J. Smith, and Ben Bond-Lamberty
Geosci. Model Dev., 14, 365–375, https://doi.org/10.5194/gmd-14-365-2021, https://doi.org/10.5194/gmd-14-365-2021, 2021
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Simple climate models are frequently used in research and decision-making communities because of their tractability and low computational cost. Simple climate models are diverse, including highly idealized and process-based models. Here we present a hybrid approach that combines the strength of two types of simple climate models in a flexible framework. This hybrid approach has provided insights into the climate system and opens an avenue for investigating radiative forcing uncertainties.
Marc Guevara, Oriol Jorba, Albert Soret, Hervé Petetin, Dene Bowdalo, Kim Serradell, Carles Tena, Hugo Denier van der Gon, Jeroen Kuenen, Vincent-Henri Peuch, and Carlos Pérez García-Pando
Atmos. Chem. Phys., 21, 773–797, https://doi.org/10.5194/acp-21-773-2021, https://doi.org/10.5194/acp-21-773-2021, 2021
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Most European countries have imposed lockdowns to combat the spread of the COVID-19 pandemic. Such a socioeconomic disruption has resulted in a sudden drop of atmospheric emissions and air pollution levels. This study quantifies the daily reductions in national emissions and associated levels of nitrogen dioxide (NO2) due to the COVID-19 lockdowns in Europe, by making use of multiple open-access measured activity data as well as artificial intelligence and modelling techniques.
Erin E. McDuffie, Steven J. Smith, Patrick O'Rourke, Kushal Tibrewal, Chandra Venkataraman, Eloise A. Marais, Bo Zheng, Monica Crippa, Michael Brauer, and Randall V. Martin
Earth Syst. Sci. Data, 12, 3413–3442, https://doi.org/10.5194/essd-12-3413-2020, https://doi.org/10.5194/essd-12-3413-2020, 2020
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Global emission inventories are vital to understanding the impacts of air pollution on the environment, human health, and society. We update the open-source Community Emissions Data System (CEDS) to provide global gridded emissions of seven key air pollutants from 1970–2017 for 11 source sectors and multiple fuel types, including coal, solid biofuel, and liquid oil and natural gas. This dataset includes both monthly global gridded emissions and annual national totals.
Benjamin Gaubert, Louisa K. Emmons, Kevin Raeder, Simone Tilmes, Kazuyuki Miyazaki, Avelino F. Arellano Jr., Nellie Elguindi, Claire Granier, Wenfu Tang, Jérôme Barré, Helen M. Worden, Rebecca R. Buchholz, David P. Edwards, Philipp Franke, Jeffrey L. Anderson, Marielle Saunois, Jason Schroeder, Jung-Hun Woo, Isobel J. Simpson, Donald R. Blake, Simone Meinardi, Paul O. Wennberg, John Crounse, Alex Teng, Michelle Kim, Russell R. Dickerson, Hao He, Xinrong Ren, Sally E. Pusede, and Glenn S. Diskin
Atmos. Chem. Phys., 20, 14617–14647, https://doi.org/10.5194/acp-20-14617-2020, https://doi.org/10.5194/acp-20-14617-2020, 2020
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This study investigates carbon monoxide pollution in East Asia during spring using a numerical model, satellite remote sensing, and aircraft measurements. We found an underestimation of emission sources. Correcting the emission bias can improve air quality forecasting of carbon monoxide and other species including ozone. Results also suggest that controlling VOC and CO emissions, in addition to widespread NOx controls, can improve ozone pollution over East Asia.
Bart Degraeuwe, Enrico Pisoni, and Philippe Thunis
Geosci. Model Dev., 13, 5725–5736, https://doi.org/10.5194/gmd-13-5725-2020, https://doi.org/10.5194/gmd-13-5725-2020, 2020
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To make decisions on how to improve air quality, it is useful to identify the main sources of pollution for an area of interest. Often these sources of pollution are identified with complex models that, even if accurate, are time consuming and complex. In this work we use another approach, simplified models, to accomplish the same task. The results, computed with two different set of simplified models, show the main sources of pollution for selected cities, and the associated uncertainties.
Marianne T. Lund, Borgar Aamaas, Camilla W. Stjern, Zbigniew Klimont, Terje K. Berntsen, and Bjørn H. Samset
Earth Syst. Dynam., 11, 977–993, https://doi.org/10.5194/esd-11-977-2020, https://doi.org/10.5194/esd-11-977-2020, 2020
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Achieving the Paris Agreement temperature goals requires both near-zero levels of long-lived greenhouse gases and deep cuts in emissions of short-lived climate forcers (SLCFs). Here we quantify the near- and long-term global temperature impacts of emissions of individual SLCFs and CO2 from 7 economic sectors in 13 regions in order to provide the detailed knowledge needed to design efficient mitigation strategies at the sectoral and regional levels.
Junichi Kurokawa and Toshimasa Ohara
Atmos. Chem. Phys., 20, 12761–12793, https://doi.org/10.5194/acp-20-12761-2020, https://doi.org/10.5194/acp-20-12761-2020, 2020
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A long historical emission inventory of major air pollutants in Asia during 1950–2015 was developed as Regional Emission inventory in ASia version 3 (REASv3). Trends of emissions and changes in source contributions in countries and regions in Asia during these 6 decades were analyzed. REASv3 provides monthly gridded data with 0.25° by 0.25° resolution for major source categories as well as table of emissions by countries and sub-regions for major sectors and fuel types.
Zebedee R. J. Nicholls, Malte Meinshausen, Jared Lewis, Robert Gieseke, Dietmar Dommenget, Kalyn Dorheim, Chen-Shuo Fan, Jan S. Fuglestvedt, Thomas Gasser, Ulrich Golüke, Philip Goodwin, Corinne Hartin, Austin P. Hope, Elmar Kriegler, Nicholas J. Leach, Davide Marchegiani, Laura A. McBride, Yann Quilcaille, Joeri Rogelj, Ross J. Salawitch, Bjørn H. Samset, Marit Sandstad, Alexey N. Shiklomanov, Ragnhild B. Skeie, Christopher J. Smith, Steve Smith, Katsumasa Tanaka, Junichi Tsutsui, and Zhiang Xie
Geosci. Model Dev., 13, 5175–5190, https://doi.org/10.5194/gmd-13-5175-2020, https://doi.org/10.5194/gmd-13-5175-2020, 2020
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Computational limits mean that we cannot run our most comprehensive climate models for all applications of interest. In such cases, reduced complexity models (RCMs) are used. Here, researchers working on 15 different models present the first systematic community effort to evaluate and compare RCMs: the Reduced Complexity Model Intercomparison Project (RCMIP). Our research ensures that users of RCMs can more easily evaluate the strengths, weaknesses and limitations of their tools.
Amy E. Christiansen, Annmarie G. Carlton, and Barron H. Henderson
Atmos. Chem. Phys., 20, 11607–11624, https://doi.org/10.5194/acp-20-11607-2020, https://doi.org/10.5194/acp-20-11607-2020, 2020
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We quantify differences in surface-level fine particle mass (PM2.5) chemical composition in relation to satellite-derived cloud flags and find significant differences between clear-sky and cloud days. The work suggests that future analysis in this area is warranted.
Pengfei Han, Ning Zeng, Tom Oda, Xiaohui Lin, Monica Crippa, Dabo Guan, Greet Janssens-Maenhout, Xiaolin Ma, Zhu Liu, Yuli Shan, Shu Tao, Haikun Wang, Rong Wang, Lin Wu, Xiao Yun, Qiang Zhang, Fang Zhao, and Bo Zheng
Atmos. Chem. Phys., 20, 11371–11385, https://doi.org/10.5194/acp-20-11371-2020, https://doi.org/10.5194/acp-20-11371-2020, 2020
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An accurate estimation of China’s fossil-fuel CO2 emissions (FFCO2) is significant for quantification of carbon budget and emissions reductions towards the Paris Agreement goals. Here we assessed 9 global and regional inventories. Our findings highlight the significance of using locally measured coal emission factors. We call on the enhancement of physical measurements for validation and provide comprehensive information for inventory, monitoring, modeling, assimilation, and reducing emissions.
Tim Butler, Aurelia Lupascu, and Aditya Nalam
Atmos. Chem. Phys., 20, 10707–10731, https://doi.org/10.5194/acp-20-10707-2020, https://doi.org/10.5194/acp-20-10707-2020, 2020
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Ground-level ozone (O3) is not directly emitted; it is formed chemically in the atmosphere. Some ground-level O3 is transported from the stratosphere, but most O3 is produced from reactive precursors that are emitted by both natural and anthropogenic sources. We present the results of a novel source apportionment method for ground-level O3. Our results are consistent with previous work and also provide new insights. In particular, we highlight the roles of methane and international shipping.
Baozhu Ge, Syuichi Itahashi, Keiichi Sato, Danhui Xu, Junhua Wang, Fan Fan, Qixin Tan, Joshua S. Fu, Xuemei Wang, Kazuyo Yamaji, Tatsuya Nagashima, Jie Li, Mizuo Kajino, Hong Liao, Meigen Zhang, Zhe Wang, Meng Li, Jung-Hun Woo, Junichi Kurokawa, Yuepeng Pan, Qizhong Wu, Xuejun Liu, and Zifa Wang
Atmos. Chem. Phys., 20, 10587–10610, https://doi.org/10.5194/acp-20-10587-2020, https://doi.org/10.5194/acp-20-10587-2020, 2020
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Performances of the simulated deposition for different reduced N (Nr) species in China were conducted with the Model Inter-Comparison Study for Asia. Results showed that simulated wet deposition of oxidized N was overestimated in northeastern China and underestimated in south China, but Nr was underpredicted in all regions by all models. Oxidized N has larger uncertainties than Nr, indicating that the chemical reaction process is one of the most importance factors affecting model performance.
Satoru Chatani, Hikari Shimadera, Syuichi Itahashi, and Kazuyo Yamaji
Atmos. Chem. Phys., 20, 10311–10329, https://doi.org/10.5194/acp-20-10311-2020, https://doi.org/10.5194/acp-20-10311-2020, 2020
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Source sensitivities and apportionments of PM2.5 and ozone concentrations over Japan for 2016 were evaluated using multiple numerical techniques including BFM, HDDM, and ISAM, embedded in regional chemical transport models. Influences of stringent emission controls recently implemented in Asian countries were reflected. Differences between sensitivities and apportionments greatly helped distinguish various direct and indirect effects of emission sources on PM2.5 and ozone concentrations.
Amir H. Souri, Caroline R. Nowlan, Gonzalo González Abad, Lei Zhu, Donald R. Blake, Alan Fried, Andrew J. Weinheimer, Armin Wisthaler, Jung-Hun Woo, Qiang Zhang, Christopher E. Chan Miller, Xiong Liu, and Kelly Chance
Atmos. Chem. Phys., 20, 9837–9854, https://doi.org/10.5194/acp-20-9837-2020, https://doi.org/10.5194/acp-20-9837-2020, 2020
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For the first time, we provide a joint nonlinear optimal estimate of NOx and NMVOC emissions during the KORUS-AQ campaign by simultaneously incorporating SAO's new product of HCHO columns from OMPS and OMI tropospheric NO2 columns into a regional model. Results demonstrate a promising improvement in the performance of the model in terms of HCHO and NO2 concentrations, which in turn enables us to quantify the impact of the emission changes on different pathways of ozone formation and loss.
Noelia Otero, Henning W. Rust, and Tim Butler
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-691, https://doi.org/10.5194/acp-2020-691, 2020
Revised manuscript not accepted
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Surface ozone concentrations are strongly correlated with temperature in summertime. Using long-term measurements, we investigate changes in the observed relationship between ozone and temperature over Germany. We propose a new statistical approach based on Generalized Additive Models (GAMs) to describe ozone production rates as a function of nitrogen oxides (NOx) and temperature. Our results suggest that NOx reductions alone can not explain the changes in the temperature dependence of ozone.
Malte Meinshausen, Zebedee R. J. Nicholls, Jared Lewis, Matthew J. Gidden, Elisabeth Vogel, Mandy Freund, Urs Beyerle, Claudia Gessner, Alexander Nauels, Nico Bauer, Josep G. Canadell, John S. Daniel, Andrew John, Paul B. Krummel, Gunnar Luderer, Nicolai Meinshausen, Stephen A. Montzka, Peter J. Rayner, Stefan Reimann, Steven J. Smith, Marten van den Berg, Guus J. M. Velders, Martin K. Vollmer, and Ray H. J. Wang
Geosci. Model Dev., 13, 3571–3605, https://doi.org/10.5194/gmd-13-3571-2020, https://doi.org/10.5194/gmd-13-3571-2020, 2020
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This study provides the future greenhouse gas (GHG) concentrations under the new set of so-called SSP scenarios (the successors of the IPCC SRES and previous representative concentration pathway (RCP) scenarios). The projected CO2 concentrations range from 350 ppm for low-emission scenarios by 2150 to more than 2000 ppm under the high-emission scenarios. We also provide concentrations, latitudinal gradients, and seasonality for most of the other 42 considered GHGs.
Philippe Thunis, Monica Crippa, Cornelis Cuvelier, Diego Guizzardi, Alexander De Meij, Gabriel Oreggioni, and Enrico Pisoni
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2020-144, https://doi.org/10.5194/essd-2020-144, 2020
Preprint withdrawn
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A comparison of emissions inventories for air quality modelling, in Europe, is presented. Among these inventories, EDGAR v5.0 for air pollutants is introduced and validated, through a simulation with the EMEP model.
Yugo Kanaya, Kazuyo Yamaji, Takuma Miyakawa, Fumikazu Taketani, Chunmao Zhu, Yongjoo Choi, Yuichi Komazaki, Kohei Ikeda, Yutaka Kondo, and Zbigniew Klimont
Atmos. Chem. Phys., 20, 6339–6356, https://doi.org/10.5194/acp-20-6339-2020, https://doi.org/10.5194/acp-20-6339-2020, 2020
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Fundamental disagreements among bottom-up emission inventories exist about the sign of the black carbon emissions trend from China over the past decade. Our decadal observations on Fukue Island clearly indicate its rapid reduction, after correcting for interannual meteorological variability, which supports inventories reflecting governmental clean air actions after 2010. The reduction pace surpasses those of SSP1 scenarios for 2015–2030, suggesting highly successful emission control policies.
Pablo E. Saide, Meng Gao, Zifeng Lu, Daniel L. Goldberg, David G. Streets, Jung-Hun Woo, Andreas Beyersdorf, Chelsea A. Corr, Kenneth L. Thornhill, Bruce Anderson, Johnathan W. Hair, Amin R. Nehrir, Glenn S. Diskin, Jose L. Jimenez, Benjamin A. Nault, Pedro Campuzano-Jost, Jack Dibb, Eric Heim, Kara D. Lamb, Joshua P. Schwarz, Anne E. Perring, Jhoon Kim, Myungje Choi, Brent Holben, Gabriele Pfister, Alma Hodzic, Gregory R. Carmichael, Louisa Emmons, and James H. Crawford
Atmos. Chem. Phys., 20, 6455–6478, https://doi.org/10.5194/acp-20-6455-2020, https://doi.org/10.5194/acp-20-6455-2020, 2020
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Air quality forecasts over the Korean Peninsula captured aerosol optical depth but largely overpredicted surface PM during a Chinese haze transport event. Model deficiency was related to the calculation of optical properties. In order to improve it, aerosol size representation needs to be refined in the calculations, and the representation of aerosol properties, such as size distribution, chemical composition, refractive index, hygroscopicity parameter, and density, needs to be improved.
Hideo Shiogama, Ryuichi Hirata, Tomoko Hasegawa, Shinichiro Fujimori, Noriko N. Ishizaki, Satoru Chatani, Masahiro Watanabe, Daniel Mitchell, and Y. T. Eunice Lo
Earth Syst. Dynam., 11, 435–445, https://doi.org/10.5194/esd-11-435-2020, https://doi.org/10.5194/esd-11-435-2020, 2020
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Based on climate simulations, we suggested that historical warming increased chances of drought exceeding the severe 2015 event in equatorial Asia due to El Niño. The fire and fire emissions of CO2/PM2.5 will largely increase at 1.5 and 2 °C warming. If global warming reaches 3 °C, as is expected from the current mitigation policies, chances of fire and CO2/PM2.5 emissions exceeding the 2015 event become approximately 100 %. Future climate policy has to consider these climate change effects.
Sojin Lee, Chul Han Song, Kyung Man Han, Daven K. Henze, Kyunghwa Lee, Jinhyeok Yu, Jung-Hun Woo, Jia Jung, Yunsoo Choi, Pablo E. Saide, and Gregory R. Carmichael
Geosci. Model Dev. Discuss., https://doi.org/10.5194/gmd-2020-116, https://doi.org/10.5194/gmd-2020-116, 2020
Revised manuscript not accepted
Ana Maria Roxana Petrescu, Glen P. Peters, Greet Janssens-Maenhout, Philippe Ciais, Francesco N. Tubiello, Giacomo Grassi, Gert-Jan Nabuurs, Adrian Leip, Gema Carmona-Garcia, Wilfried Winiwarter, Lena Höglund-Isaksson, Dirk Günther, Efisio Solazzo, Anja Kiesow, Ana Bastos, Julia Pongratz, Julia E. M. S. Nabel, Giulia Conchedda, Roberto Pilli, Robbie M. Andrew, Mart-Jan Schelhaas, and Albertus J. Dolman
Earth Syst. Sci. Data, 12, 961–1001, https://doi.org/10.5194/essd-12-961-2020, https://doi.org/10.5194/essd-12-961-2020, 2020
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This study is topical and provides a state-of-the-art scientific overview of data availability from bottom-up GHG anthropogenic emissions from agriculture, forestry and other land use (AFOLU) in the EU28. The data integrate recent AFOLU emission inventories with ecosystem data and land carbon models, aiming at reconciling GHG budgets with official country-level UNFCCC inventories. We provide comprehensive emission assessments in support to policy, facilitating real-time verification procedures.
Cynthia H. Whaley, Elisabeth Galarneau, Paul A. Makar, Michael D. Moran, and Junhua Zhang
Atmos. Chem. Phys., 20, 2911–2925, https://doi.org/10.5194/acp-20-2911-2020, https://doi.org/10.5194/acp-20-2911-2020, 2020
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Benzene and polycyclic aromatic compounds are toxic air pollutants and ubiquitous in the environment. Using a chemical transport model, we have determined the net impact of vehicle emissions on ambient concentrations of these species. Traffic emissions were found to be a significant fraction of ambient pollution in the densely populated modelled region of North America. Our simulations demonstrate the air quality benefits that would result from transitioning to a zero-emission vehicle fleet.
Kyunghwa Lee, Jinhyeok Yu, Sojin Lee, Mieun Park, Hun Hong, Soon Young Park, Myungje Choi, Jhoon Kim, Younha Kim, Jung-Hun Woo, Sang-Woo Kim, and Chul H. Song
Geosci. Model Dev., 13, 1055–1073, https://doi.org/10.5194/gmd-13-1055-2020, https://doi.org/10.5194/gmd-13-1055-2020, 2020
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For the purpose of providing reliable and robust air quality predictions, an operational air quality prediction system was developed for the main air quality criteria species in South Korea (PM10, PM2.5, CO, O3 and SO2) by preparing the initial conditions for model simulations via data assimilation using satellite- and ground-based observations. The performance of the developed air quality prediction system was evaluated using ground in situ data during the KORUS-AQ campaign period.
Syuichi Itahashi, Baozhu Ge, Keiichi Sato, Joshua S. Fu, Xuemei Wang, Kazuyo Yamaji, Tatsuya Nagashima, Jie Li, Mizuo Kajino, Hong Liao, Meigen Zhang, Zhe Wang, Meng Li, Junichi Kurokawa, Gregory R. Carmichael, and Zifa Wang
Atmos. Chem. Phys., 20, 2667–2693, https://doi.org/10.5194/acp-20-2667-2020, https://doi.org/10.5194/acp-20-2667-2020, 2020
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This study gives an overview of acid deposition from the Model Inter-Comparison Study for Asia (MICS-Asia) phase III. Wet deposition simulated by a total of nine models is evaluated with observation data from the Acid Deposition Monitoring Network in East Asia (EANET). The total deposition maps comparing to emissions over Asia are presented. To seek a way to improve the model performance, ensemble approaches and the precipitation-adjusted method are discussed.
Zhining Tao, Mian Chin, Meng Gao, Tom Kucsera, Dongchul Kim, Huisheng Bian, Jun-ichi Kurokawa, Yuesi Wang, Zirui Liu, Gregory R. Carmichael, Zifa Wang, and Hajime Akimoto
Atmos. Chem. Phys., 20, 2319–2339, https://doi.org/10.5194/acp-20-2319-2020, https://doi.org/10.5194/acp-20-2319-2020, 2020
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One goal of the Model Inter-Comparison Study for Asia (MICS-Asia) Phase III is to identify strengths and weaknesses of current air quality models to provide insights into reducing uncertainties. This study identified that a 15 km grid would be the optimal horizontal resolution in terms of performance and resource usage to capture average and extreme air quality over East Asia and is thus suggested for use in future MICS-Asia modeling activities if the investigation domain remains the same.
Mark W. Shephard, Enrico Dammers, Karen E. Cady-Pereira, Shailesh K. Kharol, Jesse Thompson, Yonatan Gainariu-Matz, Junhua Zhang, Chris A. McLinden, Andrew Kovachik, Michael Moran, Shabtai Bittman, Christopher E. Sioris, Debora Griffin, Matthew J. Alvarado, Chantelle Lonsdale, Verica Savic-Jovcic, and Qiong Zheng
Atmos. Chem. Phys., 20, 2277–2302, https://doi.org/10.5194/acp-20-2277-2020, https://doi.org/10.5194/acp-20-2277-2020, 2020
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Presented is a description and survey demonstrating the capabilities of the CrIS ammonia product for monitoring, air quality forecast model evaluation, dry deposition estimates, and emission estimates of an agricultural hotspot.
Leyang Feng, Steven J. Smith, Caleb Braun, Monica Crippa, Matthew J. Gidden, Rachel Hoesly, Zbigniew Klimont, Margreet van Marle, Maarten van den Berg, and Guido R. van der Werf
Geosci. Model Dev., 13, 461–482, https://doi.org/10.5194/gmd-13-461-2020, https://doi.org/10.5194/gmd-13-461-2020, 2020
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We describe the methods used for generating gridded emission datasets produced for use by the modeling community, particularly for the Coupled Model Intercomparison Project Phase 6 (CMIP6). The development of three sets of gridded data (historical open burning, historical anthropogenic, and future scenarios) was coordinated to produce consistent data over 1750–2100. We discuss the methodologies used to produce these data along with limitations and potential for future work.
Meng Gao, Zhiwei Han, Zhining Tao, Jiawei Li, Jeong-Eon Kang, Kan Huang, Xinyi Dong, Bingliang Zhuang, Shu Li, Baozhu Ge, Qizhong Wu, Hyo-Jung Lee, Cheol-Hee Kim, Joshua S. Fu, Tijian Wang, Mian Chin, Meng Li, Jung-Hun Woo, Qiang Zhang, Yafang Cheng, Zifa Wang, and Gregory R. Carmichael
Atmos. Chem. Phys., 20, 1147–1161, https://doi.org/10.5194/acp-20-1147-2020, https://doi.org/10.5194/acp-20-1147-2020, 2020
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Topic 3 of the Model Inter-Comparison Study for Asia (MICS-Asia) Phase III examines how online coupled air quality models perform in simulating high aerosol pollution in the North China Plain region during wintertime haze events and evaluates the importance of aerosol radiative feedbacks. This paper discusses the estimates of aerosol radiative forcing, aerosol feedbacks, and possible causes for the differences among the models.
Hongbin Yu, Yang Yang, Hailong Wang, Qian Tan, Mian Chin, Robert C. Levy, Lorraine A. Remer, Steven J. Smith, Tianle Yuan, and Yingxi Shi
Atmos. Chem. Phys., 20, 139–161, https://doi.org/10.5194/acp-20-139-2020, https://doi.org/10.5194/acp-20-139-2020, 2020
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Emissions and long-range transport of mineral dust and
combustion-related aerosol from burning fossil fuels and biomass vary from year to year, driven by the evolution of the economy and changes in meteorological conditions and environmental regulations. This study offers both satellite and model perspectives on interannual variability and possible trends in combustion aerosol and dust in major continental outflow regions over the past 15 years (2003–2017).
Aurelia Lupaşcu and Tim Butler
Atmos. Chem. Phys., 19, 14535–14558, https://doi.org/10.5194/acp-19-14535-2019, https://doi.org/10.5194/acp-19-14535-2019, 2019
Alcide Zhao, Massimo A. Bollasina, Monica Crippa, and David S. Stevenson
Atmos. Chem. Phys., 19, 14517–14533, https://doi.org/10.5194/acp-19-14517-2019, https://doi.org/10.5194/acp-19-14517-2019, 2019
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Emissions of aerosols over the recent past have been regulated largely by two policy-relevant drivers: energy-use growth and technology advances. These generate large and competing impacts on global radiation balance and climate, particularly over Asia, Europe, and the Arctic. This may help better assess and interpret future climate projections, and hence inform future climate change impact reduction strategies. Yet, it is pressing to better constrain various uncertainties related to aerosols.
Adria K. Schwarber, Steven J. Smith, Corinne A. Hartin, Benjamin Aaron Vega-Westhoff, and Ryan Sriver
Earth Syst. Dynam., 10, 729–739, https://doi.org/10.5194/esd-10-729-2019, https://doi.org/10.5194/esd-10-729-2019, 2019
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Simple climate models (SCMs) underlie many important scientific and decision-making endeavors. This illustrates the need for their use to be rooted in a clear understanding of their fundamental responses. In this study, we provide a comprehensive assessment of model performance by evaluating the fundamental responses of several SCMs. We find biases in some responses, which have implications for decision science. We conclude by recommending a standard set of validation tests for any SCM.
Daiwen Kang, Kristen M. Foley, Rohit Mathur, Shawn J. Roselle, Kenneth E. Pickering, and Dale J. Allen
Geosci. Model Dev., 12, 4409–4424, https://doi.org/10.5194/gmd-12-4409-2019, https://doi.org/10.5194/gmd-12-4409-2019, 2019
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This paper provides a comprehensive evaluation of the lightning production schemes in CMAQ as described in https://www.geosci-model-dev.net/12/3071/2019/gmd-12-3071-2019.html on model performance. The impact of lightning NOx from different schemes is evaluated in time and space using both ground–level network measurements and aloft (ozonesonde and aircraft) observations. These results provide users the benchmark model performance when the lightning NOx production schemes are applied.
Lei Chen, Yi Gao, Meigen Zhang, Joshua S. Fu, Jia Zhu, Hong Liao, Jialin Li, Kan Huang, Baozhu Ge, Xuemei Wang, Yun Fat Lam, Chuan-Yao Lin, Syuichi Itahashi, Tatsuya Nagashima, Mizuo Kajino, Kazuyo Yamaji, Zifa Wang, and Jun-ichi Kurokawa
Atmos. Chem. Phys., 19, 11911–11937, https://doi.org/10.5194/acp-19-11911-2019, https://doi.org/10.5194/acp-19-11911-2019, 2019
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Simulated aerosol concentrations from 14 CTMs within the framework of MICS-Asia III are detailedly evaluated with an extensive set of measurements in East Asia. Similarities and differences among model performances are also analyzed. Although more considerable capacities for reproducing the aerosol concentrations and their variations are shown in current CTMs than those in MICS-Asia II, more efforts are needed to reduce diversities of simulated aerosol concentrations among air quality models.
Xiaoyi Zhao, Debora Griffin, Vitali Fioletov, Chris McLinden, Jonathan Davies, Akira Ogyu, Sum Chi Lee, Alexandru Lupu, Michael D. Moran, Alexander Cede, Martin Tiefengraber, and Moritz Müller
Atmos. Chem. Phys., 19, 10619–10642, https://doi.org/10.5194/acp-19-10619-2019, https://doi.org/10.5194/acp-19-10619-2019, 2019
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New nitrogen dioxide (NO2) retrieval algorithms are developed for Pandora zenith-sky measurements. A column-to-surface conversion look-up table was produced for the Pandora instruments; therefore, quick and practical Pandora-based surface NO2 concentration data can be obtained for air quality monitoring purposes. It is demonstrated that the surface NO2 concentration is controlled not only by the planetary boundary layer height but also by both boundary layer dynamics and photochemistry.
Jack Chen, Kerry Anderson, Radenko Pavlovic, Michael D. Moran, Peter Englefield, Dan K. Thompson, Rodrigo Munoz-Alpizar, and Hugo Landry
Geosci. Model Dev., 12, 3283–3310, https://doi.org/10.5194/gmd-12-3283-2019, https://doi.org/10.5194/gmd-12-3283-2019, 2019
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Emissions from wildland fires can cause significant impacts on regional air quality. We introduce the Canadian Forest Fire Emissions Prediction System and demonstrate its integration with Canada's FireWork operational air quality forecast system with biomass burning emissions. The coupled system shows improved skill in providing short-term, 48 h forecasts of surface air pollutant concentrations (PM2.5, O3, and NO2) from the impacts of regional wildland fires across the North American domain.
Daiwen Kang, Kenneth E. Pickering, Dale J. Allen, Kristen M. Foley, David C. Wong, Rohit Mathur, and Shawn J. Roselle
Geosci. Model Dev., 12, 3071–3083, https://doi.org/10.5194/gmd-12-3071-2019, https://doi.org/10.5194/gmd-12-3071-2019, 2019
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Lightning strikes produce significant amount of nitrogen oxides and the resulting atmospheric chemistry causes one of the primary air pollutants, ground-level ozone, to change. In this paper, we documented the evolution of scientific updates for lightning-induced nitrogen oxides schemes in the CMAQ model. The updated observation-based schemes are good for retrospective applications, while the parameterized scheme can estimate lightning nitrogen oxides for applications without observations.
Greet Janssens-Maenhout, Monica Crippa, Diego Guizzardi, Marilena Muntean, Edwin Schaaf, Frank Dentener, Peter Bergamaschi, Valerio Pagliari, Jos G. J. Olivier, Jeroen A. H. W. Peters, John A. van Aardenne, Suvi Monni, Ulrike Doering, A. M. Roxana Petrescu, Efisio Solazzo, and Gabriel D. Oreggioni
Earth Syst. Sci. Data, 11, 959–1002, https://doi.org/10.5194/essd-11-959-2019, https://doi.org/10.5194/essd-11-959-2019, 2019
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In support of the Paris Agreement, EDGARv4.3.2 provides global annual estimates, broken down into IPCC-compliant source-sector levels, from 1970 to 2012. The anthropogenic CO2, CH4 and N2O emissions were calculated bottom up with international statistics and emission factors for 226 countries and spatially distributed. EDGARv4.3.2 is input for the top-down modelling of the Global Carbon Project and EU policy-making, needing GHG emission estimates for each country at the climate negotiations.
Monica Crippa, Greet Janssens-Maenhout, Diego Guizzardi, Rita Van Dingenen, and Frank Dentener
Atmos. Chem. Phys., 19, 5165–5186, https://doi.org/10.5194/acp-19-5165-2019, https://doi.org/10.5194/acp-19-5165-2019, 2019
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In this work we evaluate the contribution of the major anthropogenic emission sources to global air quality and human health, focusing on particulate matter (PM) concentrations because of their importance in populated areas and the proven cumulative negative effects on human health. We show that in order to improve air quality, regional policies should be implemented due to the transboundary features of PM pollution.
Matthew J. Gidden, Keywan Riahi, Steven J. Smith, Shinichiro Fujimori, Gunnar Luderer, Elmar Kriegler, Detlef P. van Vuuren, Maarten van den Berg, Leyang Feng, David Klein, Katherine Calvin, Jonathan C. Doelman, Stefan Frank, Oliver Fricko, Mathijs Harmsen, Tomoko Hasegawa, Petr Havlik, Jérôme Hilaire, Rachel Hoesly, Jill Horing, Alexander Popp, Elke Stehfest, and Kiyoshi Takahashi
Geosci. Model Dev., 12, 1443–1475, https://doi.org/10.5194/gmd-12-1443-2019, https://doi.org/10.5194/gmd-12-1443-2019, 2019
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We present a suite of nine scenarios of future emissions trajectories of anthropogenic sources for use in CMIP6. Integrated assessment model results are provided for each scenario with consistent transitions from the historical data to future trajectories. We find that the set of scenarios enables the exploration of a variety of warming pathways. A wide range of scenario data products are provided for the CMIP6 scientific community including global, regional, and gridded emissions datasets.
Matthew Russell, Amir Hakami, Paul A. Makar, Ayodeji Akingunola, Junhua Zhang, Michael D. Moran, and Qiong Zheng
Atmos. Chem. Phys., 19, 4393–4417, https://doi.org/10.5194/acp-19-4393-2019, https://doi.org/10.5194/acp-19-4393-2019, 2019
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High-resolution air-quality forecast modeling results are compared for two different grid spacings for the Environment and Climate Change Canada GEM-MACH model. While the higher-resolution simulations have worse formal error scores, we show that the higher-resolution model nevertheless has the ability to better resolve plume maxima and has better performance when the evaluation occurs using new scoring metrics which operate on an equal-representative-area basis.
Debra Wunch, Dylan B. A. Jones, Geoffrey C. Toon, Nicholas M. Deutscher, Frank Hase, Justus Notholt, Ralf Sussmann, Thorsten Warneke, Jeroen Kuenen, Hugo Denier van der Gon, Jenny A. Fisher, and Joannes D. Maasakkers
Atmos. Chem. Phys., 19, 3963–3980, https://doi.org/10.5194/acp-19-3963-2019, https://doi.org/10.5194/acp-19-3963-2019, 2019
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We used five atmospheric observatories in Europe measuring total column dry-air mole fractions of methane and carbon monoxide to infer methane emissions in the area between the observatories. We find that the methane emissions are overestimated by the state-of-the-art inventories, and that this is likely due, at least in part, to the inventory disaggregation. We find that there is significant uncertainty in the carbon monoxide inventories that requires further investigation.
Stephanie Fiedler, Bjorn Stevens, Matthew Gidden, Steven J. Smith, Keywan Riahi, and Detlef van Vuuren
Geosci. Model Dev., 12, 989–1007, https://doi.org/10.5194/gmd-12-989-2019, https://doi.org/10.5194/gmd-12-989-2019, 2019
Yang Yang, Steven J. Smith, Hailong Wang, Catrin M. Mills, and Philip J. Rasch
Atmos. Chem. Phys., 19, 2405–2420, https://doi.org/10.5194/acp-19-2405-2019, https://doi.org/10.5194/acp-19-2405-2019, 2019
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Black carbon (BC) particles exert a potentially large warming influence on the
Earth system. We evaluate regional climate responses, non-linearity, and short-term transient responses to BC emission perturbations. We found that climate responses do not scale linearity with emissions and BC impacts temperature much faster than greenhouse gas forcing. Removing present-day BC emissions results in discernible surface temperature changes for only limited regions of the globe.
Katherine Calvin, Pralit Patel, Leon Clarke, Ghassem Asrar, Ben Bond-Lamberty, Ryna Yiyun Cui, Alan Di Vittorio, Kalyn Dorheim, Jae Edmonds, Corinne Hartin, Mohamad Hejazi, Russell Horowitz, Gokul Iyer, Page Kyle, Sonny Kim, Robert Link, Haewon McJeon, Steven J. Smith, Abigail Snyder, Stephanie Waldhoff, and Marshall Wise
Geosci. Model Dev., 12, 677–698, https://doi.org/10.5194/gmd-12-677-2019, https://doi.org/10.5194/gmd-12-677-2019, 2019
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This paper describes GCAM v5.1, an open source model that represents the linkages between energy, water, land, climate, and economic systems. GCAM examines the future evolution of these systems through the end of the 21st century. It can be used to examine, for example, how changes in population, income, or technology cost might alter crop production, energy demand, or water withdrawals, or how changes in one region’s demand for energy affect energy, water, and land in other regions.
Daniel L. Goldberg, Pablo E. Saide, Lok N. Lamsal, Benjamin de Foy, Zifeng Lu, Jung-Hun Woo, Younha Kim, Jinseok Kim, Meng Gao, Gregory Carmichael, and David G. Streets
Atmos. Chem. Phys., 19, 1801–1818, https://doi.org/10.5194/acp-19-1801-2019, https://doi.org/10.5194/acp-19-1801-2019, 2019
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Using satellite data, we are able to estimate the emissions of NOx (NOx=NO+NO2), a toxic group of air pollutants, in the Seoul metropolitan area. We first develop an enhanced satellite product that better observes NO2 in urban regions. Using this new product, we derive NOx emissions to be twice as large as the emissions reported by the South Korean government. The implication is that the measures taken to reduce NOx emissions in South Korea have not been as effective as regulators have thought.
Gabriele Curci, Ummugulsum Alyuz, Rocio Barò, Roberto Bianconi, Johannes Bieser, Jesper H. Christensen, Augustin Colette, Aidan Farrow, Xavier Francis, Pedro Jiménez-Guerrero, Ulas Im, Peng Liu, Astrid Manders, Laura Palacios-Peña, Marje Prank, Luca Pozzoli, Ranjeet Sokhi, Efisio Solazzo, Paolo Tuccella, Alper Unal, Marta G. Vivanco, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 19, 181–204, https://doi.org/10.5194/acp-19-181-2019, https://doi.org/10.5194/acp-19-181-2019, 2019
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Atmospheric carbonaceous aerosols are able to absorb solar radiation and they continue to contribute some of the largest uncertainties in projected climate change. One important detail is how the chemical species are arranged inside each particle, i.e. the knowledge of their mixing state. We use an ensemble of regional model simulations to test different mixing state assumptions and found that a combination of internal and external mixing may better reproduce sunphotometer observations.
Benjamin A. Nault, Pedro Campuzano-Jost, Douglas A. Day, Jason C. Schroder, Bruce Anderson, Andreas J. Beyersdorf, Donald R. Blake, William H. Brune, Yonghoon Choi, Chelsea A. Corr, Joost A. de Gouw, Jack Dibb, Joshua P. DiGangi, Glenn S. Diskin, Alan Fried, L. Gregory Huey, Michelle J. Kim, Christoph J. Knote, Kara D. Lamb, Taehyoung Lee, Taehyun Park, Sally E. Pusede, Eric Scheuer, Kenneth L. Thornhill, Jung-Hun Woo, and Jose L. Jimenez
Atmos. Chem. Phys., 18, 17769–17800, https://doi.org/10.5194/acp-18-17769-2018, https://doi.org/10.5194/acp-18-17769-2018, 2018
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Aerosol impacts visibility and human health in large cities. Sources of aerosols are still highly uncertain, especially for cities surrounded by numerous other cities. We use observations collected during the Korea–United States Air Quality study to determine sources of organic aerosol (OA). We find that secondary OA (SOA) is rapidly produced over Seoul, South Korea, and that the sources of the SOA originate from short-lived hydrocarbons, which originate from local emissions.
Rita Van Dingenen, Frank Dentener, Monica Crippa, Joana Leitao, Elina Marmer, Shilpa Rao, Efisio Solazzo, and Luana Valentini
Atmos. Chem. Phys., 18, 16173–16211, https://doi.org/10.5194/acp-18-16173-2018, https://doi.org/10.5194/acp-18-16173-2018, 2018
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The evaluation of air pollution impacts, including on human health, vegetation, climate, and ecosystem health, is an essential component in the design of policies that affect air quality directly or indirectly. We have developed a tool that allows for a fast screening of relevant air pollution impacts from given emission scenarios at the regional to global scale, bypassing expensive numerical modelling of complex atmospheric processes. This paper provides a full documentation of the methodology.
Xinyi Dong, Joshua S. Fu, Qingzhao Zhu, Jian Sun, Jiani Tan, Terry Keating, Takashi Sekiya, Kengo Sudo, Louisa Emmons, Simone Tilmes, Jan Eiof Jonson, Michael Schulz, Huisheng Bian, Mian Chin, Yanko Davila, Daven Henze, Toshihiko Takemura, Anna Maria Katarina Benedictow, and Kan Huang
Atmos. Chem. Phys., 18, 15581–15600, https://doi.org/10.5194/acp-18-15581-2018, https://doi.org/10.5194/acp-18-15581-2018, 2018
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We have applied the HTAP phase II multi-model data to investigate the long-range transport impacts on surface concentration and column density of PM from Europe and Russia, Belarus, and Ukraine to eastern Asia, with a special focus on the long-range transport contribution during haze episodes in China. We found that long-range transport plays a more important role in elevating the background concentration of surface PM during the haze days.
Monica Crippa, Diego Guizzardi, Marilena Muntean, Edwin Schaaf, Frank Dentener, John A. van Aardenne, Suvi Monni, Ulrike Doering, Jos G. J. Olivier, Valerio Pagliari, and Greet Janssens-Maenhout
Earth Syst. Sci. Data, 10, 1987–2013, https://doi.org/10.5194/essd-10-1987-2018, https://doi.org/10.5194/essd-10-1987-2018, 2018
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EDGAR v4.3.2 is a global bottom-up emission inventory providing consistent anthropogenic emissions of gaseous and particulate air pollutants for 1970–2012 (with annual and monthly resolution) and grid maps with 0.1° × 0.1° resolution. We compare world regions using per capita and per GDP emissions, implied emissions per unit of energy, and emission ratios of co-emitted pollutants. We also show the growth of high-emitting areas (e.g. China, India) and the implications for global air quality.
Marina Astitha, Ioannis Kioutsioukis, Ghezae Araya Fisseha, Roberto Bianconi, Johannes Bieser, Jesper H. Christensen, Owen R. Cooper, Stefano Galmarini, Christian Hogrefe, Ulas Im, Bryan Johnson, Peng Liu, Uarporn Nopmongcol, Irina Petropavlovskikh, Efisio Solazzo, David W. Tarasick, and Greg Yarwood
Atmos. Chem. Phys., 18, 13925–13945, https://doi.org/10.5194/acp-18-13925-2018, https://doi.org/10.5194/acp-18-13925-2018, 2018
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This work is unique in the detailed analyses of modeled ozone vertical profiles from sites in North America through the collaboration of four research groups from the US and EU. We assess the air quality models' performance and model inter-comparison for ozone vertical profiles and stratospheric ozone intrusions. Lastly, we designate the important role of lateral boundary conditions in the ozone vertical profiles using chemically inert tracers.
Jan Eiof Jonson, Michael Schulz, Louisa Emmons, Johannes Flemming, Daven Henze, Kengo Sudo, Marianne Tronstad Lund, Meiyun Lin, Anna Benedictow, Brigitte Koffi, Frank Dentener, Terry Keating, Rigel Kivi, and Yanko Davila
Atmos. Chem. Phys., 18, 13655–13672, https://doi.org/10.5194/acp-18-13655-2018, https://doi.org/10.5194/acp-18-13655-2018, 2018
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Focusing on Europe, this HTAP 2 study computes ozone in several global models when reducing anthropogenic emissions by 20 % in different world regions. The differences in model results are explored
by use of a novel stepwise approach combining a tracer, CO and ozone. For ozone the contributions from the rest of the world are larger than from Europe, with the largest contributions from North America and eastern Asia. Contributions do, however, depend on the choice of ozone metric.
Noelia Otero, Jana Sillmann, Kathleen A. Mar, Henning W. Rust, Sverre Solberg, Camilla Andersson, Magnuz Engardt, Robert Bergström, Bertrand Bessagnet, Augustin Colette, Florian Couvidat, Cournelius Cuvelier, Svetlana Tsyro, Hilde Fagerli, Martijn Schaap, Astrid Manders, Mihaela Mircea, Gino Briganti, Andrea Cappelletti, Mario Adani, Massimo D'Isidoro, María-Teresa Pay, Mark Theobald, Marta G. Vivanco, Peter Wind, Narendra Ojha, Valentin Raffort, and Tim Butler
Atmos. Chem. Phys., 18, 12269–12288, https://doi.org/10.5194/acp-18-12269-2018, https://doi.org/10.5194/acp-18-12269-2018, 2018
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This paper evaluates the capability of air-quality models to capture the observed relationship between surface ozone concentrations and meteorology over Europe. The air-quality models tended to overestimate the influence of maximum temperature and surface solar radiation. None of the air-quality models captured the strength of the observed relationship between ozone and relative humidity appropriately, underestimating the effect of relative humidity, a key factor in the ozone removal processes.
Jiani Tan, Joshua S. Fu, Frank Dentener, Jian Sun, Louisa Emmons, Simone Tilmes, Johannes Flemming, Toshihiko Takemura, Huisheng Bian, Qingzhao Zhu, Cheng-En Yang, and Terry Keating
Atmos. Chem. Phys., 18, 12223–12240, https://doi.org/10.5194/acp-18-12223-2018, https://doi.org/10.5194/acp-18-12223-2018, 2018
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Have contributions of hemispheric air pollution to deposition at global scale been overlooked in the past years? How do we assess the critical load for the acid deposition when we look for the demand of forest and crop? This study highlights the significant impact of hemispheric transport on deposition in coastal regions, open ocean and low-emission regions. Further research is proposed for improving ecosystem and human health in these regions, with regards to the enhanced hemispheric transport.
Wenfu Tang, Avelino F. Arellano, Joshua P. DiGangi, Yonghoon Choi, Glenn S. Diskin, Anna Agustí-Panareda, Mark Parrington, Sebastien Massart, Benjamin Gaubert, Youngjae Lee, Danbi Kim, Jinsang Jung, Jinkyu Hong, Je-Woo Hong, Yugo Kanaya, Mindo Lee, Ryan M. Stauffer, Anne M. Thompson, James H. Flynn, and Jung-Hun Woo
Atmos. Chem. Phys., 18, 11007–11030, https://doi.org/10.5194/acp-18-11007-2018, https://doi.org/10.5194/acp-18-11007-2018, 2018
Junhua Zhang, Michael D. Moran, Qiong Zheng, Paul A. Makar, Pegah Baratzadeh, George Marson, Peter Liu, and Shao-Meng Li
Atmos. Chem. Phys., 18, 10459–10481, https://doi.org/10.5194/acp-18-10459-2018, https://doi.org/10.5194/acp-18-10459-2018, 2018
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This paper discusses the development of new synthesized emissions inventories and the generation of air quality model-ready emissions files for the Athabasca Oil Sands Region of Alberta, Canada, using multiple emissions inventories, continuous emissions monitoring data, and inferred emission rates based on aircraft measurements. Novel facility-specific gridded spatial surrogate fields were generated to allocate emissions spatially within each huge mining facility.
Ciao-Kai Liang, J. Jason West, Raquel A. Silva, Huisheng Bian, Mian Chin, Yanko Davila, Frank J. Dentener, Louisa Emmons, Johannes Flemming, Gerd Folberth, Daven Henze, Ulas Im, Jan Eiof Jonson, Terry J. Keating, Tom Kucsera, Allen Lenzen, Meiyun Lin, Marianne Tronstad Lund, Xiaohua Pan, Rokjin J. Park, R. Bradley Pierce, Takashi Sekiya, Kengo Sudo, and Toshihiko Takemura
Atmos. Chem. Phys., 18, 10497–10520, https://doi.org/10.5194/acp-18-10497-2018, https://doi.org/10.5194/acp-18-10497-2018, 2018
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Emissions from one continent affect air quality and health elsewhere. Here we quantify the effects of intercontinental PM2.5 and ozone transport on human health using a new multi-model ensemble, evaluating the health effects of emissions from six world regions and three emission source sectors. Emissions from one region have significant health impacts outside of that source region; similarly, foreign emissions contribute significantly to air-pollution-related deaths in several world regions.
Marta G. Vivanco, Mark R. Theobald, Héctor García-Gómez, Juan Luis Garrido, Marje Prank, Wenche Aas, Mario Adani, Ummugulsum Alyuz, Camilla Andersson, Roberto Bellasio, Bertrand Bessagnet, Roberto Bianconi, Johannes Bieser, Jørgen Brandt, Gino Briganti, Andrea Cappelletti, Gabriele Curci, Jesper H. Christensen, Augustin Colette, Florian Couvidat, Cornelis Cuvelier, Massimo D'Isidoro, Johannes Flemming, Andrea Fraser, Camilla Geels, Kaj M. Hansen, Christian Hogrefe, Ulas Im, Oriol Jorba, Nutthida Kitwiroon, Astrid Manders, Mihaela Mircea, Noelia Otero, Maria-Teresa Pay, Luca Pozzoli, Efisio Solazzo, Svetlana Tsyro, Alper Unal, Peter Wind, and Stefano Galmarini
Atmos. Chem. Phys., 18, 10199–10218, https://doi.org/10.5194/acp-18-10199-2018, https://doi.org/10.5194/acp-18-10199-2018, 2018
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European wet and dry atmospheric deposition of N and S estimated by 14 air quality models was found to vary substantially. An ensemble of models meeting acceptability criteria was used to estimate the exceedances of the critical loads for N in habitats within the Natura 2000 network, as well as their lower and upper limits. Scenarios with 20 % emission reductions in different regions of the world showed that European emissions are responsible for most of the N and S deposition in Europe.
Paul A. Makar, Ayodeji Akingunola, Julian Aherne, Amanda S. Cole, Yayne-abeba Aklilu, Junhua Zhang, Isaac Wong, Katherine Hayden, Shao-Meng Li, Jane Kirk, Ken Scott, Michael D. Moran, Alain Robichaud, Hazel Cathcart, Pegah Baratzedah, Balbir Pabla, Philip Cheung, Qiong Zheng, and Dean S. Jeffries
Atmos. Chem. Phys., 18, 9897–9927, https://doi.org/10.5194/acp-18-9897-2018, https://doi.org/10.5194/acp-18-9897-2018, 2018
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Complex computer model output was compared to and fused with observation data, to estimate potential damage due to acidifying precipitation for ecosystems in the Canadian provinces of Alberta and Saskatchewan. Estimated deposition was compared to the maximum no-damage ecosystem capacity for sulfur and/or nitrogen uptake; these critical loads were exceeded, for areas between 10 000 and 330 000 square kilometres, depending on ecosystem type: ecosystem damage will occur at 2013 emission levels.
Tim Butler, Aurelia Lupascu, Jane Coates, and Shuai Zhu
Geosci. Model Dev., 11, 2825–2840, https://doi.org/10.5194/gmd-11-2825-2018, https://doi.org/10.5194/gmd-11-2825-2018, 2018
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This paper describes a method for determining origin of tropospheric ozone simulated in a global chemistry–climate model. This technique can show which precursor compounds were responsible for simulated ozone, and where they were emitted. In this paper we describe our technique, compare and contrast it with several other similar techniques, and use it to calculate the contribution of several different NOx and VOC precursor categories to the tropospheric ozone burden.
Steven T. Turnock, Oliver Wild, Frank J. Dentener, Yanko Davila, Louisa K. Emmons, Johannes Flemming, Gerd A. Folberth, Daven K. Henze, Jan E. Jonson, Terry J. Keating, Sudo Kengo, Meiyun Lin, Marianne Lund, Simone Tilmes, and Fiona M. O'Connor
Atmos. Chem. Phys., 18, 8953–8978, https://doi.org/10.5194/acp-18-8953-2018, https://doi.org/10.5194/acp-18-8953-2018, 2018
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A simple parameterisation was developed in this study to provide a rapid assessment of the impacts and uncertainties associated with future emission control strategies by predicting changes to surface ozone air quality and near-term climate forcing of ozone. Future emissions scenarios based on currently implemented legislation are shown to worsen surface ozone air quality and enhance near-term climate warming, with changes in methane becoming increasingly important in the future.
Ulas Im, Jesper Heile Christensen, Camilla Geels, Kaj Mantzius Hansen, Jørgen Brandt, Efisio Solazzo, Ummugulsum Alyuz, Alessandra Balzarini, Rocio Baro, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Augustin Colette, Gabriele Curci, Aidan Farrow, Johannes Flemming, Andrea Fraser, Pedro Jimenez-Guerrero, Nutthida Kitwiroon, Peng Liu, Uarporn Nopmongcol, Laura Palacios-Peña, Guido Pirovano, Luca Pozzoli, Marje Prank, Rebecca Rose, Ranjeet Sokhi, Paolo Tuccella, Alper Unal, Marta G. Vivanco, Greg Yarwood, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 18, 8929–8952, https://doi.org/10.5194/acp-18-8929-2018, https://doi.org/10.5194/acp-18-8929-2018, 2018
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We evaluate the impact of global and regional anthropogenic emission reductions on major air pollutant levels over Europe and North America, using a multi-model ensemble of regional chemistry and transport models. Results show that ozone levels are largely driven by long-range transport over both continents while other pollutants such as carbon monoxide or aerosols are mainly controlled by domestic sources. Use of multi-model ensembles can help to reduce the uncertainties in individual models.
Stefano Galmarini, Ioannis Kioutsioukis, Efisio Solazzo, Ummugulsum Alyuz, Alessandra Balzarini, Roberto Bellasio, Anna M. K. Benedictow, Roberto Bianconi, Johannes Bieser, Joergen Brandt, Jesper H. Christensen, Augustin Colette, Gabriele Curci, Yanko Davila, Xinyi Dong, Johannes Flemming, Xavier Francis, Andrea Fraser, Joshua Fu, Daven K. Henze, Christian Hogrefe, Ulas Im, Marta Garcia Vivanco, Pedro Jiménez-Guerrero, Jan Eiof Jonson, Nutthida Kitwiroon, Astrid Manders, Rohit Mathur, Laura Palacios-Peña, Guido Pirovano, Luca Pozzoli, Marie Prank, Martin Schultz, Rajeet S. Sokhi, Kengo Sudo, Paolo Tuccella, Toshihiko Takemura, Takashi Sekiya, and Alper Unal
Atmos. Chem. Phys., 18, 8727–8744, https://doi.org/10.5194/acp-18-8727-2018, https://doi.org/10.5194/acp-18-8727-2018, 2018
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An ensemble of model results relating to ozone concentrations in Europe in 2010 has been produced and studied. The novelty consists in the fact that the ensemble is made of results of models working at two different scales (regional and global), therefore contributing in detail two different parts of the atmospheric spectrum. The ensemble defined as a hybrid has been studied in detail and shown to bring additional value to the assessment of air quality.
Erika von Schneidemesser, Boris Bonn, Tim M. Butler, Christian Ehlers, Holger Gerwig, Hannele Hakola, Heidi Hellén, Andreas Kerschbaumer, Dieter Klemp, Claudia Kofahl, Jürgen Kura, Anja Lüdecke, Rainer Nothard, Axel Pietsch, Jörn Quedenau, Klaus Schäfer, James J. Schauer, Ashish Singh, Ana-Maria Villalobos, Matthias Wiegner, and Mark G. Lawrence
Atmos. Chem. Phys., 18, 8621–8645, https://doi.org/10.5194/acp-18-8621-2018, https://doi.org/10.5194/acp-18-8621-2018, 2018
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This paper provides an overview of the measurements done at an urban background site in Berlin from June-August of 2014. Results show that natural source contributions to ozone and particulate matter (PM) air pollutants are substantial. Large contributions of secondary aerosols formed in the atmosphere to PM10 concentrations were quantified. An analysis of the sources also identified contributions to PM from plant-based sources, vehicles, and a small contribution from wood burning.
Ayodeji Akingunola, Paul A. Makar, Junhua Zhang, Andrea Darlington, Shao-Meng Li, Mark Gordon, Michael D. Moran, and Qiong Zheng
Atmos. Chem. Phys., 18, 8667–8688, https://doi.org/10.5194/acp-18-8667-2018, https://doi.org/10.5194/acp-18-8667-2018, 2018
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We examine the manner in which air-quality models simulate lofting of buoyant plumes of emissions from stacks (plume rise) and the impact of the level of detail in algorithms simulating particles' variation in size (particle size distribution). The most commonly used plume rise algorithm underestimates the height of plumes compared to observations, while a revised algorithm has much better performance. A 12-bin size distribution reduced the forecast 2-bin size distribution bias error by 32 %.
Friderike Kuik, Andreas Kerschbaumer, Axel Lauer, Aurelia Lupascu, Erika von Schneidemesser, and Tim M. Butler
Atmos. Chem. Phys., 18, 8203–8225, https://doi.org/10.5194/acp-18-8203-2018, https://doi.org/10.5194/acp-18-8203-2018, 2018
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Modelled NOx concentrations are often underestimated compared to observations, and measurement studies show that reported NOx emissions in urban areas are often too low when the contribution from traffic is largest. This modelling study quantifies the underestimation of traffic NOx emissions in the Berlin–Brandenburg and finds that they are underestimated by ca. 50 % in the core urban area. More research is needed in order to more accurately understand real-world NOx emissions from traffic.
Chandra Venkataraman, Michael Brauer, Kushal Tibrewal, Pankaj Sadavarte, Qiao Ma, Aaron Cohen, Sreelekha Chaliyakunnel, Joseph Frostad, Zbigniew Klimont, Randall V. Martin, Dylan B. Millet, Sajeev Philip, Katherine Walker, and Shuxiao Wang
Atmos. Chem. Phys., 18, 8017–8039, https://doi.org/10.5194/acp-18-8017-2018, https://doi.org/10.5194/acp-18-8017-2018, 2018
Jiani Tan, Joshua S. Fu, Frank Dentener, Jian Sun, Louisa Emmons, Simone Tilmes, Kengo Sudo, Johannes Flemming, Jan Eiof Jonson, Sylvie Gravel, Huisheng Bian, Yanko Davila, Daven K. Henze, Marianne T. Lund, Tom Kucsera, Toshihiko Takemura, and Terry Keating
Atmos. Chem. Phys., 18, 6847–6866, https://doi.org/10.5194/acp-18-6847-2018, https://doi.org/10.5194/acp-18-6847-2018, 2018
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We study the distributions of sulfur and nitrogen deposition, which are associated with current environmental issues such as formation of acid rain and ecosystem eutrophication and result in widespread problems such as loss of environmental diversity, harming the crop yield and even food insecurity. According to our study, both the amount and distribution of sulfate and nitrogen deposition have changed significantly in the last decade, particularly in East Asia, South Asia and Southeast Asia.
Ulas Im, Jørgen Brandt, Camilla Geels, Kaj Mantzius Hansen, Jesper Heile Christensen, Mikael Skou Andersen, Efisio Solazzo, Ioannis Kioutsioukis, Ummugulsum Alyuz, Alessandra Balzarini, Rocio Baro, Roberto Bellasio, Roberto Bianconi, Johannes Bieser, Augustin Colette, Gabriele Curci, Aidan Farrow, Johannes Flemming, Andrea Fraser, Pedro Jimenez-Guerrero, Nutthida Kitwiroon, Ciao-Kai Liang, Uarporn Nopmongcol, Guido Pirovano, Luca Pozzoli, Marje Prank, Rebecca Rose, Ranjeet Sokhi, Paolo Tuccella, Alper Unal, Marta Garcia Vivanco, Jason West, Greg Yarwood, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 18, 5967–5989, https://doi.org/10.5194/acp-18-5967-2018, https://doi.org/10.5194/acp-18-5967-2018, 2018
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The impacts of air pollution on human health and their costs in Europe and the United States for the year 2010 ared modeled by a multi-model ensemble. In Europe, the number of premature deaths is calculated to be 414 000, while in the US it is estimated to be 160 000. Health impacts estimated by individual models can vary up to a factor of 3. Results show that the domestic emissions have the largest impact on premature deaths, compared to foreign sources.
Meng Gao, Zhiwei Han, Zirui Liu, Meng Li, Jinyuan Xin, Zhining Tao, Jiawei Li, Jeong-Eon Kang, Kan Huang, Xinyi Dong, Bingliang Zhuang, Shu Li, Baozhu Ge, Qizhong Wu, Yafang Cheng, Yuesi Wang, Hyo-Jung Lee, Cheol-Hee Kim, Joshua S. Fu, Tijian Wang, Mian Chin, Jung-Hun Woo, Qiang Zhang, Zifa Wang, and Gregory R. Carmichael
Atmos. Chem. Phys., 18, 4859–4884, https://doi.org/10.5194/acp-18-4859-2018, https://doi.org/10.5194/acp-18-4859-2018, 2018
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Topic 3 of the Model Inter-Comparison Study for Asia (MICS-Asia) Phase III examines how online coupled air quality models perform in simulating high aerosol pollution in the North China Plain region during wintertime haze events and evaluates the importance of aerosol radiative and microphysical feedbacks. A comprehensive overview of the MICS-ASIA III Topic 3 study design is presented.
Riinu Ots, Mathew R. Heal, Dominique E. Young, Leah R. Williams, James D. Allan, Eiko Nemitz, Chiara Di Marco, Anais Detournay, Lu Xu, Nga L. Ng, Hugh Coe, Scott C. Herndon, Ian A. Mackenzie, David C. Green, Jeroen J. P. Kuenen, Stefan Reis, and Massimo Vieno
Atmos. Chem. Phys., 18, 4497–4518, https://doi.org/10.5194/acp-18-4497-2018, https://doi.org/10.5194/acp-18-4497-2018, 2018
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The main hypothesis of this paper is that people who live in large cities in the UK disobey the
smoke control lawas it has not been actively enforced for decades now. However, the use of wood in residential heating has increased, partly due to renewable energy targets, but also for discretionary (i.e. pleasant fireplaces) reasons. Our study is based mainly in London, but similar struggles with urban air quality due to residential wood and coal burning are seen in other major European cities.
Christian Hogrefe, Peng Liu, George Pouliot, Rohit Mathur, Shawn Roselle, Johannes Flemming, Meiyun Lin, and Rokjin J. Park
Atmos. Chem. Phys., 18, 3839–3864, https://doi.org/10.5194/acp-18-3839-2018, https://doi.org/10.5194/acp-18-3839-2018, 2018
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This study quantifies the impacts of different representations of background ozone in state-of-the-science large-scale models on surface and aloft ozone burdens simulated by the CMAQ regional model over the United States. It also compares both the CMAQ simulations and the driving large-scale models to surface and upper air observations.
Meng Li, Zbigniew Klimont, Qiang Zhang, Randall V. Martin, Bo Zheng, Chris Heyes, Janusz Cofala, Yuxuan Zhang, and Kebin He
Atmos. Chem. Phys., 18, 3433–3456, https://doi.org/10.5194/acp-18-3433-2018, https://doi.org/10.5194/acp-18-3433-2018, 2018
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In this paper, we conducted a comprehensive evaluation of two widely used anthropogenic emission inventories over China, ECLIPSE and MIX, to explore the potential sources of uncertainties and find clues to improving emission inventories. We found that SO2 emission estimates are consistent between the two inventories (with 1 % differences), while NOx emissions in ECLIPSE's estimates are 16 % lower than those in MIX. Discrepancies at the sector and provincial levels are much higher.
Stephanie C. Pugliese, Jennifer G. Murphy, Felix R. Vogel, Michael D. Moran, Junhua Zhang, Qiong Zheng, Craig A. Stroud, Shuzhan Ren, Douglas Worthy, and Gregoire Broquet
Atmos. Chem. Phys., 18, 3387–3401, https://doi.org/10.5194/acp-18-3387-2018, https://doi.org/10.5194/acp-18-3387-2018, 2018
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We developed the Southern Ontario CO2 Emissions (SOCE) inventory, which identifies the spatial and temporal distribution (2.5 km and hourly, respectively) of CO2 emissions from seven source sectors. When the SOCE inventory was used with a chemistry transport model, we found strong agreement between modelled and measured mixing ratios. We were able to quantify that natural gas combustion contributes > 80 % of CO2 emissions at nighttime while on-road emissions contribute > 70 % during the day.
Rachel M. Hoesly, Steven J. Smith, Leyang Feng, Zbigniew Klimont, Greet Janssens-Maenhout, Tyler Pitkanen, Jonathan J. Seibert, Linh Vu, Robert J. Andres, Ryan M. Bolt, Tami C. Bond, Laura Dawidowski, Nazar Kholod, June-ichi Kurokawa, Meng Li, Liang Liu, Zifeng Lu, Maria Cecilia P. Moura, Patrick R. O'Rourke, and Qiang Zhang
Geosci. Model Dev., 11, 369–408, https://doi.org/10.5194/gmd-11-369-2018, https://doi.org/10.5194/gmd-11-369-2018, 2018
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Historical emission trends are key inputs to Earth systems and atmospheric chemistry models. We present a new data set of historical (1750–2014) anthropogenic gases (CO, CH4, NH3, NOx, SO2, NMVOCs, BC, OC, and CO2) developed with the Community Emissions Data System (CEDS). This improves on existing inventories as it uses consistent methods and data across emissions species, has annual resolution for a longer and more recent time series, and is designed to be transparent and reproducible.
Yuan You, Ralf M. Staebler, Samar G. Moussa, Yushan Su, Tony Munoz, Craig Stroud, Junhua Zhang, and Michael D. Moran
Atmos. Chem. Phys., 17, 14119–14143, https://doi.org/10.5194/acp-17-14119-2017, https://doi.org/10.5194/acp-17-14119-2017, 2017
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A novel approach for traffic emission measurements is shown to have the capacity to provide high-time-resolution accurate concentrations of key air pollutants. A top-down method for quantifying real-world emission rates produced vehicular emission factor estimates for carbon monoxide that agreed well with bottom-up values. Significant ammonia and hydrogen cyanide emissions were observed. The main factors modulating the concentrations were turbulent mixing and traffic density.
Hugo A. C. Denier van der Gon, Jeroen J. P. Kuenen, Greet Janssens-Maenhout, Ulrike Döring, Sander Jonkers, and Antoon Visschedijk
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2017-124, https://doi.org/10.5194/essd-2017-124, 2017
Revised manuscript has not been submitted
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A gridded European emission inventory for CO2 from fossil fuels and biofuels (2000–2014) is made to support carbon cycle modelling and city-scale identification of emissions. Future projections following a “business as usual” and a climate change scenario are included to study possible CO2 emission changes between Paris Agreement stocktake years (2023-2028-2033). The data can be used for testing GHG verification modelling and sensitivity tests for designing a future observational system.
Astrid M. M. Manders, Peter J. H. Builtjes, Lyana Curier, Hugo A. C. Denier van der Gon, Carlijn Hendriks, Sander Jonkers, Richard Kranenburg, Jeroen J. P. Kuenen, Arjo J. Segers, Renske M. A. Timmermans, Antoon J. H. Visschedijk, Roy J. Wichink Kruit, W. Addo J. van Pul, Ferd J. Sauter, Eric van der Swaluw, Daan P. J. Swart, John Douros, Henk Eskes, Erik van Meijgaard, Bert van Ulft, Peter van Velthoven, Sabine Banzhaf, Andrea C. Mues, Rainer Stern, Guangliang Fu, Sha Lu, Arnold Heemink, Nils van Velzen, and Martijn Schaap
Geosci. Model Dev., 10, 4145–4173, https://doi.org/10.5194/gmd-10-4145-2017, https://doi.org/10.5194/gmd-10-4145-2017, 2017
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The regional-scale air quality model LOTOS–EUROS has been developed by a consortium of Dutch institutes. Recently, version 2.0 of the model was released as an open-source version. Next to a technical description and model evaluation for 2012, this paper presents the model developments in context of the history of air quality modelling and provides an outlook for future directions. Key and innovative applications of LOTOS–EUROS are also highlighted.
Vitali Fioletov, Chris A. McLinden, Shailesh K. Kharol, Nickolay A. Krotkov, Can Li, Joanna Joiner, Michael D. Moran, Robert Vet, Antoon J. H. Visschedijk, and Hugo A. C. Denier van der Gon
Atmos. Chem. Phys., 17, 12597–12616, https://doi.org/10.5194/acp-17-12597-2017, https://doi.org/10.5194/acp-17-12597-2017, 2017
Rohit Mathur, Jia Xing, Robert Gilliam, Golam Sarwar, Christian Hogrefe, Jonathan Pleim, George Pouliot, Shawn Roselle, Tanya L. Spero, David C. Wong, and Jeffrey Young
Atmos. Chem. Phys., 17, 12449–12474, https://doi.org/10.5194/acp-17-12449-2017, https://doi.org/10.5194/acp-17-12449-2017, 2017
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We extend CMAQ's applicability to the entire Northern Hemisphere to enable consistent examination of interactions between atmospheric processes occurring on various spatial and temporal scales. Improvements were made in model process representation, structure, and input data sets that enable a range of model applications including episodic intercontinental pollutant transport, long-term trends in air pollution across the Northern Hemisphere, and air pollution–climate interactions.
Heiko Bozem, Tim M. Butler, Mark G. Lawrence, Hartwig Harder, Monica Martinez, Dagmar Kubistin, Jos Lelieveld, and Horst Fischer
Atmos. Chem. Phys., 17, 10565–10582, https://doi.org/10.5194/acp-17-10565-2017, https://doi.org/10.5194/acp-17-10565-2017, 2017
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We present airborne measurements and model simulations in the tropics and mid-latitudes during GABRIEL and HOOVER, respectively. Based only on in situ data net ozone formation/destruction tendencies (NOPR) are calculated and compared to a 3-D chemistry transport model. The NOPR is positive in the continental boundary layer and the upper troposphere above 6 km. In the marine boundary layer and the middle troposphere ozone destruction prevails. Fresh convection shows strong net ozone formation.
Efisio Solazzo, Christian Hogrefe, Augustin Colette, Marta Garcia-Vivanco, and Stefano Galmarini
Atmos. Chem. Phys., 17, 10435–10465, https://doi.org/10.5194/acp-17-10435-2017, https://doi.org/10.5194/acp-17-10435-2017, 2017
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The work here is conducted within the frame of AQMEII3 and promotes the use of diagnostic methods for the evaluation of air quality models. We highlight the need to move away from aggregated error metrics and to focus on the quality of the information that can be extracted from the model and the observation. This aids the understanding of the causes of model error, providing more useful information to model developers and users than can be gained from common evaluations.
Augustin Colette, Camilla Andersson, Astrid Manders, Kathleen Mar, Mihaela Mircea, Maria-Teresa Pay, Valentin Raffort, Svetlana Tsyro, Cornelius Cuvelier, Mario Adani, Bertrand Bessagnet, Robert Bergström, Gino Briganti, Tim Butler, Andrea Cappelletti, Florian Couvidat, Massimo D'Isidoro, Thierno Doumbia, Hilde Fagerli, Claire Granier, Chris Heyes, Zig Klimont, Narendra Ojha, Noelia Otero, Martijn Schaap, Katarina Sindelarova, Annemiek I. Stegehuis, Yelva Roustan, Robert Vautard, Erik van Meijgaard, Marta Garcia Vivanco, and Peter Wind
Geosci. Model Dev., 10, 3255–3276, https://doi.org/10.5194/gmd-10-3255-2017, https://doi.org/10.5194/gmd-10-3255-2017, 2017
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The EURODELTA-Trends numerical experiment has been designed to assess the capability of chemistry-transport models to capture the evolution of surface air quality over the 1990–2010 period in Europe. It also includes sensitivity experiments in order to analyse the relative contribution of (i) emission changes, (ii) meteorological variability, and (iii) boundary conditions to air quality trends. The article is a detailed presentation of the experiment design and participating models.
Jieying Ding, Kazuyuki Miyazaki, Ronald Johannes van der A, Bas Mijling, Jun-ichi Kurokawa, SeogYeon Cho, Greet Janssens-Maenhout, Qiang Zhang, Fei Liu, and Pieternel Felicitas Levelt
Atmos. Chem. Phys., 17, 10125–10141, https://doi.org/10.5194/acp-17-10125-2017, https://doi.org/10.5194/acp-17-10125-2017, 2017
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To evaluate the quality of the satellite-derived NOx emissions, we compare nine emission inventories of nitrogen oxides including four satellite-derived NOx inventories and bottom-up inventories for East Asia. The temporal and spatial distribution of NOx emissions over East Asia are evaluated. We analyse the differences in satellite-derived emissions from two different inversion methods. The paper ends with recommendations for future improvements of emission estimates.
Greet Janssens-Maenhout, Monica Crippa, Diego Guizzardi, Marilena Muntean, Edwin Schaaf, Frank Dentener, Peter Bergamaschi, Valerio Pagliari, Jos G. J. Olivier, Jeroen A. H. W. Peters, John A. van Aardenne, Suvi Monni, Ulrike Doering, and A. M. Roxana Petrescu
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2017-79, https://doi.org/10.5194/essd-2017-79, 2017
Revised manuscript not accepted
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The Emissions Database for Global Atmospheric Research supports climate policy making with a global dataset at disaggregated country & source-sector level for 1970–2012. This dataset is not only unique in its space/time coverage, but also in its completeness & consistency of CO2, CH4 & N2O emissions compilation for all anthropogenic activities except land use. Comparison with UNFCCC values show that estimates are within the uncertainty range, but have an annual variation smaller than this range.
Yang Yang, Hailong Wang, Steven J. Smith, Richard Easter, Po-Lun Ma, Yun Qian, Hongbin Yu, Can Li, and Philip J. Rasch
Atmos. Chem. Phys., 17, 8903–8922, https://doi.org/10.5194/acp-17-8903-2017, https://doi.org/10.5194/acp-17-8903-2017, 2017
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Sulfate has significant impacts on air quality and climate. Local sulfate pollution could result from remote influences, making domestic mitigation efforts inefficient. Using CESM with a sulfur source-tagging technique, we found that, over regions with relatively low emissions, sulfate concentrations are primarily attributed to non-local sources and sulfate indirect radiative forcing over the Southern Hemisphere is more sensitive to emission perturbation than the polluted Northern Hemisphere.
Zbigniew Klimont, Kaarle Kupiainen, Chris Heyes, Pallav Purohit, Janusz Cofala, Peter Rafaj, Jens Borken-Kleefeld, and Wolfgang Schöpp
Atmos. Chem. Phys., 17, 8681–8723, https://doi.org/10.5194/acp-17-8681-2017, https://doi.org/10.5194/acp-17-8681-2017, 2017
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This paper presents a comprehensive assessment of global anthropogenic emissions of particulate matter for 1990–2010. Global emissions have not changed much in this period, showing a strong decoupling from the increase in energy consumption (and carbon dioxide emissions). Regional trends were different – increase in East Asia and Africa and decline in Europe and North America. In 2010, 60 % of emissions originated in Asia and more than half from cooking and heating stoves.
Tatsuya Nagashima, Kengo Sudo, Hajime Akimoto, Junichi Kurokawa, and Toshimasa Ohara
Atmos. Chem. Phys., 17, 8231–8246, https://doi.org/10.5194/acp-17-8231-2017, https://doi.org/10.5194/acp-17-8231-2017, 2017
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We showed the large contribution of different source regions in Asia to the recent increasing trend in surface ozone over Japan by using a global chemical transport model. China accounted for the largest part of the increasing trend, not only through the domestic ozone production (36 %) but also the ozone production in the adjacent countries due to the ozone precursors emitted in China (10 %). Other factors such as temporal change in climate and methane concentration were also investigated.
Andrea Mues, Maheswar Rupakheti, Christoph Münkel, Axel Lauer, Heiko Bozem, Peter Hoor, Tim Butler, and Mark G. Lawrence
Atmos. Chem. Phys., 17, 8157–8176, https://doi.org/10.5194/acp-17-8157-2017, https://doi.org/10.5194/acp-17-8157-2017, 2017
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Ceilometer measurements taken in the Kathmandu Valley, Nepal, were used to study the temporal and spatial evolution of the mixing layer height in the valley. This provides important information on the vertical structure of the atmosphere and can thus also help to understand the mixing of air pollutants (e.g. black carbon) in the valley. The seasonal and diurnal cycles of the mixing layer were found to be highly dependent on meteorology and mainly anticorrelated to black carbon concentrations.
Reza Shaiganfar, Steffen Beirle, Hugo Denier van der Gon, Sander Jonkers, Jeroen Kuenen, Herve Petetin, Qijie Zhang, Matthias Beekmann, and Thomas Wagner
Atmos. Chem. Phys., 17, 7853–7890, https://doi.org/10.5194/acp-17-7853-2017, https://doi.org/10.5194/acp-17-7853-2017, 2017
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We determine NOx emissions for Paris in summer 2009 and winter 2009/2010 by combining car MAX-DOAS measurements of NO2 with wind fields. We compare the results with simulations from the CHIMERE model. We derive daily average NOx emissions for Paris of 4.0 × 1025 molecules s−1 for summer and of 6.9 × 1025 molecules s−1 in winter. These values are a factor of about 1.4 and 2.0 larger than the corresponding emissions in the MACC-III emission inventory.
Ganlin Huang, Rosie Brook, Monica Crippa, Greet Janssens-Maenhout, Christian Schieberle, Chris Dore, Diego Guizzardi, Marilena Muntean, Edwin Schaaf, and Rainer Friedrich
Atmos. Chem. Phys., 17, 7683–7701, https://doi.org/10.5194/acp-17-7683-2017, https://doi.org/10.5194/acp-17-7683-2017, 2017
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In this study, a global speciated non-methane volatile organic compound (NMVOC) emission data set is developed by compiling and allocating region- and source-specific speciation profiles, i.e. distributions of NMVOC species, to the revised and extended Emissions Database for Global Atmospheric Research emission inventory, which can serve as input data for chemical transport models and health impact assessments. Species time series and high-resolution global grid maps for 1970–2012 are produced.
Giancarlo Ciarelli, Sebnem Aksoyoglu, Imad El Haddad, Emily A. Bruns, Monica Crippa, Laurent Poulain, Mikko Äijälä, Samara Carbone, Evelyn Freney, Colin O'Dowd, Urs Baltensperger, and André S. H. Prévôt
Atmos. Chem. Phys., 17, 7653–7669, https://doi.org/10.5194/acp-17-7653-2017, https://doi.org/10.5194/acp-17-7653-2017, 2017
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Organic aerosol (OA) comprises the main fraction of fine particulate matter (PM1). Using a new VBS parameterization, we performed model-based source apportionment studies to assess the importance of different emission sources to the total OA loads in Europe during winter periods. Our results indicate that residential wood burning emissions represent the major source of OA, followed by non-residential emission sources (i.e. traffic and industries).
Eri Saikawa, Hankyul Kim, Min Zhong, Alexander Avramov, Yu Zhao, Greet Janssens-Maenhout, Jun-ichi Kurokawa, Zbigniew Klimont, Fabian Wagner, Vaishali Naik, Larry W. Horowitz, and Qiang Zhang
Atmos. Chem. Phys., 17, 6393–6421, https://doi.org/10.5194/acp-17-6393-2017, https://doi.org/10.5194/acp-17-6393-2017, 2017
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We analyze differences in existing air pollutant emission estimates to better understand the magnitude of emissions as well as the source regions and sectors of air pollution in China. We find large disagreements among the inventories, and we show that these differences have a significant impact on regional air quality simulations. Better understanding of air pollutant emissions at more disaggregated levels is essential for air pollution mitigation in China.
Min Huang, Gregory R. Carmichael, R. Bradley Pierce, Duseong S. Jo, Rokjin J. Park, Johannes Flemming, Louisa K. Emmons, Kevin W. Bowman, Daven K. Henze, Yanko Davila, Kengo Sudo, Jan Eiof Jonson, Marianne Tronstad Lund, Greet Janssens-Maenhout, Frank J. Dentener, Terry J. Keating, Hilke Oetjen, and Vivienne H. Payne
Atmos. Chem. Phys., 17, 5721–5750, https://doi.org/10.5194/acp-17-5721-2017, https://doi.org/10.5194/acp-17-5721-2017, 2017
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In support of the HTAP phase 2 experiment, we conducted a number of regional-scale Sulfur Transport and dEposition Model base and sensitivity simulations over North America during May–June 2010. The STEM chemical boundary conditions were downscaled from three (GEOS-Chem, RAQMS, and ECMWF C-IFS) global chemical transport models' simulations. Analyses were performed on large spatial–temporal scales relative to HTAP1 and also on subcontinental and event scales including the use of satellite data.
K. Wyat Appel, Sergey L. Napelenok, Kristen M. Foley, Havala O. T. Pye, Christian Hogrefe, Deborah J. Luecken, Jesse O. Bash, Shawn J. Roselle, Jonathan E. Pleim, Hosein Foroutan, William T. Hutzell, George A. Pouliot, Golam Sarwar, Kathleen M. Fahey, Brett Gantt, Robert C. Gilliam, Nicholas K. Heath, Daiwen Kang, Rohit Mathur, Donna B. Schwede, Tanya L. Spero, David C. Wong, and Jeffrey O. Young
Geosci. Model Dev., 10, 1703–1732, https://doi.org/10.5194/gmd-10-1703-2017, https://doi.org/10.5194/gmd-10-1703-2017, 2017
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The Community Multiscale Air Quality (CMAQ) model is a comprehensive multipollutant air quality modeling system. The CMAQ model is used extensively throughout the world to simulate air pollutants for many purposes, including regulatory and air quality forecasting applications. This work describes the scientific updates made to the latest version of the CMAQ modeling system (CMAQv5.1) and presents an evaluation of the new model against observations and results from the previous model version.
Yang Yang, Hailong Wang, Steven J. Smith, Po-Lun Ma, and Philip J. Rasch
Atmos. Chem. Phys., 17, 4319–4336, https://doi.org/10.5194/acp-17-4319-2017, https://doi.org/10.5194/acp-17-4319-2017, 2017
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The source attributions of black carbon (BC) in China are quantified using the Community Earth System Model by source tagging. BC impacts neighboring regions greatly. Transport is important in increasing BC during regional polluted days. Emissions outside China contribute 35 % of BC direct radiative forcing in China. Efficiency analysis shows that reduction in BC emissions over eastern China could have a greater benefit for regional air quality in China, especially in the winter haze season.
Efisio Solazzo, Roberto Bianconi, Christian Hogrefe, Gabriele Curci, Paolo Tuccella, Ummugulsum Alyuz, Alessandra Balzarini, Rocío Baró, Roberto Bellasio, Johannes Bieser, Jørgen Brandt, Jesper H. Christensen, Augistin Colette, Xavier Francis, Andrea Fraser, Marta Garcia Vivanco, Pedro Jiménez-Guerrero, Ulas Im, Astrid Manders, Uarporn Nopmongcol, Nutthida Kitwiroon, Guido Pirovano, Luca Pozzoli, Marje Prank, Ranjeet S. Sokhi, Alper Unal, Greg Yarwood, and Stefano Galmarini
Atmos. Chem. Phys., 17, 3001–3054, https://doi.org/10.5194/acp-17-3001-2017, https://doi.org/10.5194/acp-17-3001-2017, 2017
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As part of the third phase of AQMEII, this study uses timescale analysis to apportion error to the responsible processes, detect causes of model error, and identify the processes and scales that require dedicated investigations. The analysis tackles model performance gauging through measurement-to-model comparison, error decomposition, and time series analysis of model biases for ozone, CO, SO2, NO, NO2, PM10, PM2.5, wind speed, and temperature over Europe and North America.
Gunnar Myhre, Wenche Aas, Ribu Cherian, William Collins, Greg Faluvegi, Mark Flanner, Piers Forster, Øivind Hodnebrog, Zbigniew Klimont, Marianne T. Lund, Johannes Mülmenstädt, Cathrine Lund Myhre, Dirk Olivié, Michael Prather, Johannes Quaas, Bjørn H. Samset, Jordan L. Schnell, Michael Schulz, Drew Shindell, Ragnhild B. Skeie, Toshihiko Takemura, and Svetlana Tsyro
Atmos. Chem. Phys., 17, 2709–2720, https://doi.org/10.5194/acp-17-2709-2017, https://doi.org/10.5194/acp-17-2709-2017, 2017
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Over the past decades, the geographical distribution of emissions of substances that alter the atmospheric energy balance has changed due to economic growth and pollution regulations. Here, we show the resulting changes to aerosol and ozone abundances and their radiative forcing using recently updated emission data for the period 1990–2015, as simulated by seven global atmospheric composition models. The global mean radiative forcing is more strongly positive than reported in IPCC AR5.
William J. Collins, Jean-François Lamarque, Michael Schulz, Olivier Boucher, Veronika Eyring, Michaela I. Hegglin, Amanda Maycock, Gunnar Myhre, Michael Prather, Drew Shindell, and Steven J. Smith
Geosci. Model Dev., 10, 585–607, https://doi.org/10.5194/gmd-10-585-2017, https://doi.org/10.5194/gmd-10-585-2017, 2017
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We have designed a set of climate model experiments called the Aerosol Chemistry Model Intercomparison Project (AerChemMIP). These are designed to quantify the climate and air quality impacts of aerosols and chemically reactive gases in the climate models that are used to simulate past and future climate. We hope that many climate modelling centres will choose to run these experiments to help understand the contribution of aerosols and chemistry to climate change.
Bjorn Stevens, Stephanie Fiedler, Stefan Kinne, Karsten Peters, Sebastian Rast, Jobst Müsse, Steven J. Smith, and Thorsten Mauritsen
Geosci. Model Dev., 10, 433–452, https://doi.org/10.5194/gmd-10-433-2017, https://doi.org/10.5194/gmd-10-433-2017, 2017
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A simple analytic description of aerosol optical properties and their main effects on clouds is developed and described. The analytic description is easy to use and easy to modify and should aid experimentation to help understand how aerosol radiative and cloud interactions effect climate and circulation. The climatology is recommended for adoption by models participating in the sixth phase of the Coupled Model Intercomparison Project.
Stefano Galmarini, Brigitte Koffi, Efisio Solazzo, Terry Keating, Christian Hogrefe, Michael Schulz, Anna Benedictow, Jan Jurgen Griesfeller, Greet Janssens-Maenhout, Greg Carmichael, Joshua Fu, and Frank Dentener
Atmos. Chem. Phys., 17, 1543–1555, https://doi.org/10.5194/acp-17-1543-2017, https://doi.org/10.5194/acp-17-1543-2017, 2017
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We present an overview of the coordinated global numerical modelling experiments performed during 2012–2016 by the Task Force on Hemispheric Transport of Air Pollution (TF HTAP), the regional experiments by the Air Quality Model Evaluation International Initiative (AQMEII) over Europe and North America, and the Model Intercomparison Study for Asia (MICS-Asia). Given the organizational complexity of bringing together these three initiatives, the experiment organization is presented.
Meng Li, Qiang Zhang, Jun-ichi Kurokawa, Jung-Hun Woo, Kebin He, Zifeng Lu, Toshimasa Ohara, Yu Song, David G. Streets, Gregory R. Carmichael, Yafang Cheng, Chaopeng Hong, Hong Huo, Xujia Jiang, Sicong Kang, Fei Liu, Hang Su, and Bo Zheng
Atmos. Chem. Phys., 17, 935–963, https://doi.org/10.5194/acp-17-935-2017, https://doi.org/10.5194/acp-17-935-2017, 2017
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An anthropogenic emission inventory for Asia is developed for the years 2008 and 2010 to support the Model Inter-Comparison Study for Asia (MICS-Asia) and the Task Force on Hemispheric Transport of Air Pollution (TF HTAP) projects by a mosaic of up-to-date regional emission inventories. The total Asian emissions in 2010 are estimated as follows: 51.3 Tg SO2, 52.1 Tg NOx, 336.5 Tg CO, 67.0 Tg NMVOC, 28.7 Tg NH3, 31.7 Tg PM10, 22.7 Tg PM2.5, 3.5 Tg BC, 8.3 Tg OC, and 17.3 Pg CO2.
Ioannis Kioutsioukis, Ulas Im, Efisio Solazzo, Roberto Bianconi, Alba Badia, Alessandra Balzarini, Rocío Baró, Roberto Bellasio, Dominik Brunner, Charles Chemel, Gabriele Curci, Hugo Denier van der Gon, Johannes Flemming, Renate Forkel, Lea Giordano, Pedro Jiménez-Guerrero, Marcus Hirtl, Oriol Jorba, Astrid Manders-Groot, Lucy Neal, Juan L. Pérez, Guidio Pirovano, Roberto San Jose, Nicholas Savage, Wolfram Schroder, Ranjeet S. Sokhi, Dimiter Syrakov, Paolo Tuccella, Johannes Werhahn, Ralf Wolke, Christian Hogrefe, and Stefano Galmarini
Atmos. Chem. Phys., 16, 15629–15652, https://doi.org/10.5194/acp-16-15629-2016, https://doi.org/10.5194/acp-16-15629-2016, 2016
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Four ensemble methods are applied to two annual AQMEII datasets and their performance is compared for O3, NO2 and PM10. The goal of the study is to quantify to what extent we can extract predictable signals from an ensemble with superior skill at each station over the single models and the ensemble mean. The promotion of the right amount of accuracy and diversity within the ensemble results in an average additional skill of up to 31 % compared to using the full ensemble in an unconditional way.
Hui Zhong, Yu Zhao, Marilena Muntean, Lei Zhang, and Jie Zhang
Atmos. Chem. Phys., 16, 15119–15134, https://doi.org/10.5194/acp-16-15119-2016, https://doi.org/10.5194/acp-16-15119-2016, 2016
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A better understanding of the discrepancies in multi-scale emission inventories could provide indications for their limitations and further improvements. We develop a bottom-up inventory of Hg emissions for Jiangsu, China. Compared to the national and global inventories, the largest total Hg emissions and fraction of Hg2+ are estimated. The crucial parameters responsible for the differences include Hg contents in coals/materials, abatement rates of emission control devices, and activity levels.
Friderike Kuik, Axel Lauer, Galina Churkina, Hugo A. C. Denier van der Gon, Daniel Fenner, Kathleen A. Mar, and Tim M. Butler
Geosci. Model Dev., 9, 4339–4363, https://doi.org/10.5194/gmd-9-4339-2016, https://doi.org/10.5194/gmd-9-4339-2016, 2016
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The study evaluates the performance of a setup of the Weather Research and Forecasting model with chemistry and aerosols (WRF–Chem) for the Berlin–Brandenburg region of Germany. Its sensitivity to updating urban input parameters based on structural data for Berlin is tested, specifying land use classes on a sub-grid scale, downscaling the original emissions to a resolution of ca. 1 km by 1 km for Berlin based on proxy data and model resolution.
Carolina Cavazos Guerra, Axel Lauer, Andreas B. Herber, Tim M. Butler, Annette Rinke, and Klaus Dethloff
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2016-942, https://doi.org/10.5194/acp-2016-942, 2016
Revised manuscript has not been submitted
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Accurate description of the Arctic atmosphere is a challenge for the modelling comunity. We evaluate the performance of the Weather Research and Forecast model (WRF) in the Eurasian Arctic and analyse the implications of data to initialise the model and a land surface scheme. The results show that biases can be related to the quality of data used and in the case of black carbon concentrations, to emission data. More long term measurements are need for model Validation in the area.
Kathleen A. Mar, Narendra Ojha, Andrea Pozzer, and Tim M. Butler
Geosci. Model Dev., 9, 3699–3728, https://doi.org/10.5194/gmd-9-3699-2016, https://doi.org/10.5194/gmd-9-3699-2016, 2016
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Ground-level ozone is an air pollutant with adverse effects on human and ecosystem health and is also a climate forcer with a significant warming effect. This paper presents the setup and evaluation of a model for ozone air quality over Europe. Within the model evaluation, we compare the use of two commonly used photochemical schemes, and we conclude that uncertainties in the representation of chemistry are important to consider when using air quality models for policy applications.
Jane Coates, Kathleen A. Mar, Narendra Ojha, and Tim M. Butler
Atmos. Chem. Phys., 16, 11601–11615, https://doi.org/10.5194/acp-16-11601-2016, https://doi.org/10.5194/acp-16-11601-2016, 2016
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This modelling study reproduced the non-linear relationship of ozone, NOx and temperature using various chemical mechanisms previously determined from observational studies. Under urban conditions, faster reaction rates rather than increased isoprene emissions led to a slightly greater increase of ozone with temperature using different NOx conditions. This study also shows that the increase of ozone with temperature is more sensitive to atmospheric mixing than the choice of chemical mechanism.
Vitali E. Fioletov, Chris A. McLinden, Nickolay Krotkov, Can Li, Joanna Joiner, Nicolas Theys, Simon Carn, and Mike D. Moran
Atmos. Chem. Phys., 16, 11497–11519, https://doi.org/10.5194/acp-16-11497-2016, https://doi.org/10.5194/acp-16-11497-2016, 2016
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We introduce the first space-based catalogue of SO2 emission sources seen by OMI. The inventory contains about 500 sources. They account for about a half of all SO2 emissions; the remaining half is likely related to sources emitting less than 30 kt yr−1 and not detected by OMI. The sources are grouped by type (volcanoes, power plants, oil- and gas-related sources, and smelters) and country. The catalogue presented herein can be used for verification of available SO2 emission inventories.
B. Quennehen, J.-C. Raut, K. S. Law, N. Daskalakis, G. Ancellet, C. Clerbaux, S.-W. Kim, M. T. Lund, G. Myhre, D. J. L. Olivié, S. Safieddine, R. B. Skeie, J. L. Thomas, S. Tsyro, A. Bazureau, N. Bellouin, M. Hu, M. Kanakidou, Z. Klimont, K. Kupiainen, S. Myriokefalitakis, J. Quaas, S. T. Rumbold, M. Schulz, R. Cherian, A. Shimizu, J. Wang, S.-C. Yoon, and T. Zhu
Atmos. Chem. Phys., 16, 10765–10792, https://doi.org/10.5194/acp-16-10765-2016, https://doi.org/10.5194/acp-16-10765-2016, 2016
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This paper evaluates the ability of six global models and one regional model in reproducing short-lived pollutants (defined here as ozone and its precursors, aerosols and black carbon) concentrations over Asia using satellite, ground-based and airborne observations.
Key findings are that models homogeneously reproduce the trace gas observations although nitrous oxides are underestimated, whereas the aerosol distributions are heterogeneously reproduced, implicating important uncertainties.
Giancarlo Ciarelli, Sebnem Aksoyoglu, Monica Crippa, Jose-Luis Jimenez, Eriko Nemitz, Karine Sellegri, Mikko Äijälä, Samara Carbone, Claudia Mohr, Colin O'Dowd, Laurent Poulain, Urs Baltensperger, and André S. H. Prévôt
Atmos. Chem. Phys., 16, 10313–10332, https://doi.org/10.5194/acp-16-10313-2016, https://doi.org/10.5194/acp-16-10313-2016, 2016
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Recent studies based on aerosol mass spectrometer measurements revealed that the organic fraction dominates the non-refractory PM1 composition. However its representation in chemical transport models is still very challenging due to uncertainties in emission sources and formation pathways. In this study, a novel organic aerosol scheme was tested in the regional air quality model CAMx and results were compared with ambient measurements at 11 different sites in Europe.
Yuqiang Zhang, Jared H. Bowden, Zachariah Adelman, Vaishali Naik, Larry W. Horowitz, Steven J. Smith, and J. Jason West
Atmos. Chem. Phys., 16, 9533–9548, https://doi.org/10.5194/acp-16-9533-2016, https://doi.org/10.5194/acp-16-9533-2016, 2016
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Reducing greenhouse gas (GHG) emissions can also improve air quality. We estimate the co-benefits of global GHG mitigation for US air quality in 2050 at fine resolution by downscaling from a previous global study. Foreign GHG mitigation under RCP4.5 contributes more to the US O3 reduction (76 % of the total) than domestic mitigation and contributes 26 % of the PM2.5 reduction. Therefore, the US gains significantly greater air quality co-benefits by coordinating GHG controls internationally.
Giulia Ruggeri, Fabian A. Bernhard, Barron H. Henderson, and Satoshi Takahama
Atmos. Chem. Phys., 16, 8729–8747, https://doi.org/10.5194/acp-16-8729-2016, https://doi.org/10.5194/acp-16-8729-2016, 2016
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Functional groups provide an intermediate level of chemical resolution between full molecular speciation and elemental composition for describing complex mixtures and can be a useful metric in model–measurement comparison of reaction kinetics and secondary organic aerosol formation. We introduce tools to facilitate such comparisons and demonstrate its application in study of the photooxidation of two precursor volatile organic compounds and the gas–particle partitioning of their products.
Boris Bonn, Erika von Schneidemesser, Dorota Andrich, Jörn Quedenau, Holger Gerwig, Anja Lüdecke, Jürgen Kura, Axel Pietsch, Christian Ehlers, Dieter Klemp, Claudia Kofahl, Rainer Nothard, Andreas Kerschbaumer, Wolfgang Junkermann, Rüdiger Grote, Tobias Pohl, Konradin Weber, Birgit Lode, Philipp Schönberger, Galina Churkina, Tim M. Butler, and Mark G. Lawrence
Atmos. Chem. Phys., 16, 7785–7811, https://doi.org/10.5194/acp-16-7785-2016, https://doi.org/10.5194/acp-16-7785-2016, 2016
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The distribution of air pollutants (gases and particles) have been investigated in different environments in Potsdam, Germany. Remarkable variations of the pollutants have been observed for distances of tens of meters by bicycles, vans and aircraft. Vegetated areas caused reductions depending on the pollutants, the vegetation type and dimensions. Our measurements show the pollutants to be of predominantly local origin, resulting in a huge challenge for common models to resolve.
Pauli Paasonen, Kaarle Kupiainen, Zbigniew Klimont, Antoon Visschedijk, Hugo A. C. Denier van der Gon, and Markus Amann
Atmos. Chem. Phys., 16, 6823–6840, https://doi.org/10.5194/acp-16-6823-2016, https://doi.org/10.5194/acp-16-6823-2016, 2016
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In this paper we show the first results of size-segregated anthropogenic particle number emissions from the GAINS emission scenario model. The shares of different sources and their predicted changes from 2010 to 2030 are described, showing clear difference in sources dominating the particle number and mass emissions. We also point out the main uncertainties in number emissions. The GAINS particle number emissions can be applied in improving the evaluation of aerosol climate and health effects.
Riinu Ots, Dominique E. Young, Massimo Vieno, Lu Xu, Rachel E. Dunmore, James D. Allan, Hugh Coe, Leah R. Williams, Scott C. Herndon, Nga L. Ng, Jacqueline F. Hamilton, Robert Bergström, Chiara Di Marco, Eiko Nemitz, Ian A. Mackenzie, Jeroen J. P. Kuenen, David C. Green, Stefan Reis, and Mathew R. Heal
Atmos. Chem. Phys., 16, 6453–6473, https://doi.org/10.5194/acp-16-6453-2016, https://doi.org/10.5194/acp-16-6453-2016, 2016
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This study investigates the contribution of diesel vehicle emissions to organic aerosol formation and particulate matter concentrations in London. Comparisons of simulated pollutant concentrations with observations show good agreement and give confidence in the skill of the model applied. The contribution of diesel vehicle emissions, which are currently not included in official emissions inventories, is demonstrated to be substantial, indicating that more research on this topic is required.
Efisio Solazzo and Stefano Galmarini
Atmos. Chem. Phys., 16, 6263–6283, https://doi.org/10.5194/acp-16-6263-2016, https://doi.org/10.5194/acp-16-6263-2016, 2016
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A new technique to assess the quality of model results from a regional-scale air quality model is presented. The techniques are based on standard statistical parameters but work on spectral decomposition of model and measurement time series. This allows for the identification of scale-related processes for which the largest divergency between model and observed data is found. The technique is applied to the data collected during the second phase of the AQMEI Initiative.
Wolfgang Knorr, Frank Dentener, Stijn Hantson, Leiwen Jiang, Zbigniew Klimont, and Almut Arneth
Atmos. Chem. Phys., 16, 5685–5703, https://doi.org/10.5194/acp-16-5685-2016, https://doi.org/10.5194/acp-16-5685-2016, 2016
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Wildfires are generally expected to increase in frequency and severity due to climate change. For Europe this could mean increased air pollution levels during the summer. Until 2050, predicted changes are moderate, but under a scenario of strong climate change, these may increase considerably during the later part of the current century. In Portugal and several parts of the Mediterranean, emissions may become relevant for meeting WHO concentration targets.
Monica Crippa, Greet Janssens-Maenhout, Frank Dentener, Diego Guizzardi, Katerina Sindelarova, Marilena Muntean, Rita Van Dingenen, and Claire Granier
Atmos. Chem. Phys., 16, 3825–3841, https://doi.org/10.5194/acp-16-3825-2016, https://doi.org/10.5194/acp-16-3825-2016, 2016
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The interplay of European air quality policies and technological advancement to reduce anthropogenic emissions avoided a dramatic deterioration of air quality in Europe and beyond over the last 40 years (e.g. fuel quality directives reduced global SO2 emissions by 88 %, while the EURO standards led to a 50 % reduction of PM2.5). The story told by the EDGAR retrospective scenarios can be informative for designing multi-pollutant abatement policies also in emerging economies.
Christos Fountoukis, Athanasios G. Megaritis, Ksakousti Skyllakou, Panagiotis E. Charalampidis, Hugo A. C. Denier van der Gon, Monica Crippa, André S. H. Prévôt, Friederike Fachinger, Alfred Wiedensohler, Christodoulos Pilinis, and Spyros N. Pandis
Atmos. Chem. Phys., 16, 3727–3741, https://doi.org/10.5194/acp-16-3727-2016, https://doi.org/10.5194/acp-16-3727-2016, 2016
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We use PMCAMx with high grid resolution over Paris to simulate carbonaceous aerosol during the summer and winter MEGAPOLI campaigns. PMCAMx reproduces BC observations well. Addition of cooking organic aerosol emissions of 80 mg per day per capita is needed to reproduce the corresponding observations. While the oxygenated organic aerosol predictions during the summer are encouraging a major wintertime source appears to be missing.
Andrea Paciga, Eleni Karnezi, Evangelia Kostenidou, Lea Hildebrandt, Magda Psichoudaki, Gabriella J. Engelhart, Byong-Hyoek Lee, Monica Crippa, André S. H. Prévôt, Urs Baltensperger, and Spyros N. Pandis
Atmos. Chem. Phys., 16, 2013–2023, https://doi.org/10.5194/acp-16-2013-2016, https://doi.org/10.5194/acp-16-2013-2016, 2016
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We estimate the volatility distribution for the organic aerosol (OA) components during summer and winter field campaigns in Paris, France as part of the collaborative project MEGAPOLI. The OA factors (hydrocarbon like OA, cooking OA, marine OA, oxygenated OA) had a broad spectrum of volatilities with no direct link between the average volatility and average oxygen to carbon of the OA components.
S. Lee, C. H. Song, R. S. Park, M. E. Park, K. M. Han, J. Kim, M. Choi, Y. S. Ghim, and J.-H. Woo
Geosci. Model Dev., 9, 17–39, https://doi.org/10.5194/gmd-9-17-2016, https://doi.org/10.5194/gmd-9-17-2016, 2016
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We developed an integrated air quality modeling system using AOD data retrieved from a geostationary satellite sensor, GOCI (Geostationary Ocean Color Imager), over Northeast Asia with an application of the spatiotemporal-kriging (STK) method and conducted short-term hindcast runs using the developed system. It appears that the STK approach can greatly reduce not only the errors and biases of AOD and PM10 predictions but also the computational burden of a chemical weather forecast (CWF).
K. R. Daellenbach, C. Bozzetti, A. Křepelová, F. Canonaco, R. Wolf, P. Zotter, P. Fermo, M. Crippa, J. G. Slowik, Y. Sosedova, Y. Zhang, R.-J. Huang, L. Poulain, S. Szidat, U. Baltensperger, I. El Haddad, and A. S. H. Prévôt
Atmos. Meas. Tech., 9, 23–39, https://doi.org/10.5194/amt-9-23-2016, https://doi.org/10.5194/amt-9-23-2016, 2016
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In this study, we developed an offline technique using the AMS for the characterization of the chemical fingerprints of aerosols collected on quartz filters, and evaluated the suitability of the organic mass spectral data for source apportionment. This technique may be used to enhance the AMS capabilities in measuring size-fractionated, spatially resolved long-term data sets.
M. W. Shephard, C. A. McLinden, K. E. Cady-Pereira, M. Luo, S. G. Moussa, A. Leithead, J. Liggio, R. M. Staebler, A. Akingunola, P. Makar, P. Lehr, J. Zhang, D. K. Henze, D. B. Millet, J. O. Bash, L. Zhu, K. C. Wells, S. L. Capps, S. Chaliyakunnel, M. Gordon, K. Hayden, J. R. Brook, M. Wolde, and S.-M. Li
Atmos. Meas. Tech., 8, 5189–5211, https://doi.org/10.5194/amt-8-5189-2015, https://doi.org/10.5194/amt-8-5189-2015, 2015
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This study provides direct validations of Tropospheric Emission Spectrometer (TES) satellite retrieved profiles against coincident aircraft profiles of carbon monoxide, ammonia, methanol, and formic acid, all of which are of interest for air quality. The comparisons are performed over the Canadian oil sands region during an intensive field campaign in support of the Joint Canada-Alberta Implementation Plan for the Oil Sands Monitoring (JOSM). Initial model evaluations are also provided.
G. Janssens-Maenhout, M. Crippa, D. Guizzardi, F. Dentener, M. Muntean, G. Pouliot, T. Keating, Q. Zhang, J. Kurokawa, R. Wankmüller, H. Denier van der Gon, J. J. P. Kuenen, Z. Klimont, G. Frost, S. Darras, B. Koffi, and M. Li
Atmos. Chem. Phys., 15, 11411–11432, https://doi.org/10.5194/acp-15-11411-2015, https://doi.org/10.5194/acp-15-11411-2015, 2015
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This paper provides monthly emission grid maps at 0.1deg x 0.1deg resolution with global coverage for air pollutants and aerosols anthropogenic emissions in 2008 and 2010.
Countries are consistently inter-compared with sector-specific implied emission factors, per capita emissions and emissions per unit of GDP.
The emission grid maps compose the reference emissions data set for the community modelling hemispheric transport of air pollution (HTAP).
A. Stohl, B. Aamaas, M. Amann, L. H. Baker, N. Bellouin, T. K. Berntsen, O. Boucher, R. Cherian, W. Collins, N. Daskalakis, M. Dusinska, S. Eckhardt, J. S. Fuglestvedt, M. Harju, C. Heyes, Ø. Hodnebrog, J. Hao, U. Im, M. Kanakidou, Z. Klimont, K. Kupiainen, K. S. Law, M. T. Lund, R. Maas, C. R. MacIntosh, G. Myhre, S. Myriokefalitakis, D. Olivié, J. Quaas, B. Quennehen, J.-C. Raut, S. T. Rumbold, B. H. Samset, M. Schulz, Ø. Seland, K. P. Shine, R. B. Skeie, S. Wang, K. E. Yttri, and T. Zhu
Atmos. Chem. Phys., 15, 10529–10566, https://doi.org/10.5194/acp-15-10529-2015, https://doi.org/10.5194/acp-15-10529-2015, 2015
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This paper presents a summary of the findings of the ECLIPSE EU project. The project has investigated the climate and air quality impacts of short-lived climate pollutants (especially methane, ozone, aerosols) and has designed a global mitigation strategy that maximizes co-benefits between air quality and climate policy. Transient climate model simulations allowed quantifying the impacts on temperature (e.g., reduction in global warming by 0.22K for the decade 2041-2050) and precipitation.
M. Pikridas, J. Sciare, F. Freutel, S. Crumeyrolle, S.-L. von der Weiden-Reinmüller, A. Borbon, A. Schwarzenboeck, M. Merkel, M. Crippa, E. Kostenidou, M. Psichoudaki, L. Hildebrandt, G. J. Engelhart, T. Petäjä, A. S. H. Prévôt, F. Drewnick, U. Baltensperger, A. Wiedensohler, M. Kulmala, M. Beekmann, and S. N. Pandis
Atmos. Chem. Phys., 15, 10219–10237, https://doi.org/10.5194/acp-15-10219-2015, https://doi.org/10.5194/acp-15-10219-2015, 2015
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Aerosol size distribution measurements from three ground sites, two mobile laboratories, and one airplane are combined to investigate the spatial and temporal variability of ultrafine particles in and around Paris during the summer and winter MEGAPOLI campaigns. The role of nucleation as a particle source and the influence of Paris emissions on their surroundings are examined.
V. Marécal, V.-H. Peuch, C. Andersson, S. Andersson, J. Arteta, M. Beekmann, A. Benedictow, R. Bergström, B. Bessagnet, A. Cansado, F. Chéroux, A. Colette, A. Coman, R. L. Curier, H. A. C. Denier van der Gon, A. Drouin, H. Elbern, E. Emili, R. J. Engelen, H. J. Eskes, G. Foret, E. Friese, M. Gauss, C. Giannaros, J. Guth, M. Joly, E. Jaumouillé, B. Josse, N. Kadygrov, J. W. Kaiser, K. Krajsek, J. Kuenen, U. Kumar, N. Liora, E. Lopez, L. Malherbe, I. Martinez, D. Melas, F. Meleux, L. Menut, P. Moinat, T. Morales, J. Parmentier, A. Piacentini, M. Plu, A. Poupkou, S. Queguiner, L. Robertson, L. Rouïl, M. Schaap, A. Segers, M. Sofiev, L. Tarasson, M. Thomas, R. Timmermans, Á. Valdebenito, P. van Velthoven, R. van Versendaal, J. Vira, and A. Ung
Geosci. Model Dev., 8, 2777–2813, https://doi.org/10.5194/gmd-8-2777-2015, https://doi.org/10.5194/gmd-8-2777-2015, 2015
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This paper describes the air quality forecasting system over Europe put in place in the Monitoring Atmospheric Composition and Climate projects. It provides daily and 4-day forecasts and analyses for the previous day for major gas and particulate pollutants and their main precursors. These products are based on a multi-model approach using seven state-of-the-art models developed in Europe. An evaluation of the performance of the system is discussed in the paper.
M. Beekmann, A. S. H. Prévôt, F. Drewnick, J. Sciare, S. N. Pandis, H. A. C. Denier van der Gon, M. Crippa, F. Freutel, L. Poulain, V. Ghersi, E. Rodriguez, S. Beirle, P. Zotter, S.-L. von der Weiden-Reinmüller, M. Bressi, C. Fountoukis, H. Petetin, S. Szidat, J. Schneider, A. Rosso, I. El Haddad, A. Megaritis, Q. J. Zhang, V. Michoud, J. G. Slowik, S. Moukhtar, P. Kolmonen, A. Stohl, S. Eckhardt, A. Borbon, V. Gros, N. Marchand, J. L. Jaffrezo, A. Schwarzenboeck, A. Colomb, A. Wiedensohler, S. Borrmann, M. Lawrence, A. Baklanov, and U. Baltensperger
Atmos. Chem. Phys., 15, 9577–9591, https://doi.org/10.5194/acp-15-9577-2015, https://doi.org/10.5194/acp-15-9577-2015, 2015
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A detailed characterization of air quality in the Paris (France) agglomeration, a megacity, during two summer and winter intensive campaigns and from additional 1-year observations, revealed that about 70% of the fine particulate matter (PM) at urban background is transported into the megacity from upwind regions. Unexpectedly, a major part of organic PM is of modern origin (woodburning and cooking activities, secondary formation from biogenic VOC).
S. Eckhardt, B. Quennehen, D. J. L. Olivié, T. K. Berntsen, R. Cherian, J. H. Christensen, W. Collins, S. Crepinsek, N. Daskalakis, M. Flanner, A. Herber, C. Heyes, Ø. Hodnebrog, L. Huang, M. Kanakidou, Z. Klimont, J. Langner, K. S. Law, M. T. Lund, R. Mahmood, A. Massling, S. Myriokefalitakis, I. E. Nielsen, J. K. Nøjgaard, J. Quaas, P. K. Quinn, J.-C. Raut, S. T. Rumbold, M. Schulz, S. Sharma, R. B. Skeie, H. Skov, T. Uttal, K. von Salzen, and A. Stohl
Atmos. Chem. Phys., 15, 9413–9433, https://doi.org/10.5194/acp-15-9413-2015, https://doi.org/10.5194/acp-15-9413-2015, 2015
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The concentrations of sulfate, black carbon and other aerosols in the Arctic are characterized by high values in late winter and spring (so-called Arctic Haze) and low values in summer. Models have long been struggling to capture this seasonality. In this study, we evaluate sulfate and BC concentrations from different updated models and emissions against a comprehensive pan-Arctic measurement data set. We find that the models improved but still struggle to get the maximum concentrations.
J. Coates and T. M. Butler
Atmos. Chem. Phys., 15, 8795–8808, https://doi.org/10.5194/acp-15-8795-2015, https://doi.org/10.5194/acp-15-8795-2015, 2015
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We show that simplified chemical mechanisms break down VOC into smaller sized degradation products on the first day faster than the near-explicit MCM chemical mechanism which would lead to an underprediction of ozone levels downwind of VOC emissions, and an underestimation of the VOC contribution to tropospheric background ozone when using simplified chemical mechanisms in regional or global modelling studies.
K. M. Seltzer, W. Vizuete, and B. H. Henderson
Atmos. Chem. Phys., 15, 5973–5986, https://doi.org/10.5194/acp-15-5973-2015, https://doi.org/10.5194/acp-15-5973-2015, 2015
J.-P. Pietikäinen, K. Kupiainen, Z. Klimont, R. Makkonen, H. Korhonen, R. Karinkanta, A.-P. Hyvärinen, N. Karvosenoja, A. Laaksonen, H. Lihavainen, and V.-M. Kerminen
Atmos. Chem. Phys., 15, 5501–5519, https://doi.org/10.5194/acp-15-5501-2015, https://doi.org/10.5194/acp-15-5501-2015, 2015
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The global aerosol--climate model ECHAM-HAMMOZ is used to study the aerosol burden and forcing changes in the coming decades. We show that aerosol burdens overall can have a decreasing trend leading to reductions in the direct aerosol effect being globally 0.06--0.4W/m2 by 2030, whereas the aerosol indirect radiative effect could decline 0.25--0.82W/m2. We also show that the targeted emission reduction measures can be a much better choice for the climate than overall high reductions globally.
S. Banzhaf, M. Schaap, R. Kranenburg, A. M. M. Manders, A. J. Segers, A. J. H. Visschedijk, H. A. C. Denier van der Gon, J. J. P. Kuenen, E. van Meijgaard, L. H. van Ulft, J. Cofala, and P. J. H. Builtjes
Geosci. Model Dev., 8, 1047–1070, https://doi.org/10.5194/gmd-8-1047-2015, https://doi.org/10.5194/gmd-8-1047-2015, 2015
B. Gantt, M. S. Johnson, M. Crippa, A. S. H. Prévôt, and N. Meskhidze
Geosci. Model Dev., 8, 619–629, https://doi.org/10.5194/gmd-8-619-2015, https://doi.org/10.5194/gmd-8-619-2015, 2015
J. Xing, R. Mathur, J. Pleim, C. Hogrefe, C.-M. Gan, D. C. Wong, C. Wei, R. Gilliam, and G. Pouliot
Atmos. Chem. Phys., 15, 2723–2747, https://doi.org/10.5194/acp-15-2723-2015, https://doi.org/10.5194/acp-15-2723-2015, 2015
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Model-simulated air quality trends over the past 2 decades largely agree with those derived from observations. In the relative amounts of VOC and NOx emission controls in different regions across the northern hemisphere have led to significantly different trends in tropospheric O3. Differences in the historical changes in the relative amounts of NH3, NOx and SO2 emissions also impact the trends in inorganic particulate matter amounts and composition in China, the U.S. and Europe.
G. Curci, L. Ferrero, P. Tuccella, F. Barnaba, F. Angelini, E. Bolzacchini, C. Carbone, H. A. C. Denier van der Gon, M. C. Facchini, G. P. Gobbi, J. P. P. Kuenen, T. C. Landi, C. Perrino, M. G. Perrone, G. Sangiorgi, and P. Stocchi
Atmos. Chem. Phys., 15, 2629–2649, https://doi.org/10.5194/acp-15-2629-2015, https://doi.org/10.5194/acp-15-2629-2015, 2015
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Particulate matter (PM) at ground level is of primary concern for the quality of the air we breathe. Most direct sources of PM are near the ground, but an important fraction of PM is produced by photochemical processes happening also in the upper atmospheric layers. We investigated the contribution of those layers to the PM near the ground and found a significant impact. Nitrate is a major player in the “vertical direction”, owing to its sensitivity to ambient temperature and relative humidity.
E. Solazzo and S. Galmarini
Atmos. Chem. Phys., 15, 2535–2544, https://doi.org/10.5194/acp-15-2535-2015, https://doi.org/10.5194/acp-15-2535-2015, 2015
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Ensembles of results from multiple models require systematic screening according to well-defined and analytical principles described in the paper. The screening guarantees more robust conclusions especially in the case of scenario analysis.
W. Tang, D. S. Cohan, A. Pour-Biazar, L. N. Lamsal, A. T. White, X. Xiao, W. Zhou, B. H. Henderson, and B. F. Lash
Atmos. Chem. Phys., 15, 1601–1619, https://doi.org/10.5194/acp-15-1601-2015, https://doi.org/10.5194/acp-15-1601-2015, 2015
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A joint application of multiple satellite-derived model inputs to improve Texas O3 SIP modeling is demonstrated in this study. The GOES-retrieved clouds are applied to correct the modeled photolysis rates, and the DKF inversion approach is incorporated into the CAMx-DDM model to adjust NOx emissions using OMI NO2. Using both GOES-derived photolysis rates and OMI-constrained NOx emissions together improves O3 simulations and makes O3 more sensitive to NOx emissions in the O3 non-attainment areas.
H. S. Gadhavi, K. Renuka, V. Ravi Kiran, A. Jayaraman, A. Stohl, Z. Klimont, and G. Beig
Atmos. Chem. Phys., 15, 1447–1461, https://doi.org/10.5194/acp-15-1447-2015, https://doi.org/10.5194/acp-15-1447-2015, 2015
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Emission inventories are a key component of simulating past, present and future climate. In this article we have evaluated three black carbon emission inventories for emissions of India using observations made from a strategic location. Annual average simulated black carbon concentration is found to be 35% to 60% lower than observed concentration because of underestimation of emissions of southern India in the inventories.
T. F. Bidleman, L. M. Jantunen, H. Hung, J. Ma, G. A. Stern, B. Rosenberg, and J. Racine
Atmos. Chem. Phys., 15, 1411–1420, https://doi.org/10.5194/acp-15-1411-2015, https://doi.org/10.5194/acp-15-1411-2015, 2015
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Canadian Arctic air samples were analysed for enantiomers (mirror-image isomers) of pesticides α-hexachlorocyclohexane (α-HCH), trans-chlordane (TC) and cis-chlordane (CC). Annual cycles of enantiomer proportions suggested greater emission of microbially degraded residues from water and soil in warm vs. cold seasons. Enantiomer profiles may change in the future with rising contributions from secondary sources, monitoring them could increase the forensic capability in air monitoring programs.
J. J. P. Kuenen, A. J. H. Visschedijk, M. Jozwicka, and H. A. C. Denier van der Gon
Atmos. Chem. Phys., 14, 10963–10976, https://doi.org/10.5194/acp-14-10963-2014, https://doi.org/10.5194/acp-14-10963-2014, 2014
W. Ait-Helal, A. Borbon, S. Sauvage, J. A. de Gouw, A. Colomb, V. Gros, F. Freutel, M. Crippa, C. Afif, U. Baltensperger, M. Beekmann, J.-F. Doussin, R. Durand-Jolibois, I. Fronval, N. Grand, T. Leonardis, M. Lopez, V. Michoud, K. Miet, S. Perrier, A. S. H. Prévôt, J. Schneider, G. Siour, P. Zapf, and N. Locoge
Atmos. Chem. Phys., 14, 10439–10464, https://doi.org/10.5194/acp-14-10439-2014, https://doi.org/10.5194/acp-14-10439-2014, 2014
S. V. Henriksson, J.-P. Pietikäinen, A.-P. Hyvärinen, P. Räisänen, K. Kupiainen, J. Tonttila, R. Hooda, H. Lihavainen, D. O'Donnell, L. Backman, Z. Klimont, and A. Laaksonen
Atmos. Chem. Phys., 14, 10177–10192, https://doi.org/10.5194/acp-14-10177-2014, https://doi.org/10.5194/acp-14-10177-2014, 2014
L. Poulain, W. Birmili, F. Canonaco, M. Crippa, Z. J. Wu, S. Nordmann, G. Spindler, A. S. H. Prévôt, A. Wiedensohler, and H. Herrmann
Atmos. Chem. Phys., 14, 10145–10162, https://doi.org/10.5194/acp-14-10145-2014, https://doi.org/10.5194/acp-14-10145-2014, 2014
S. Safieddine, A. Boynard, P.-F. Coheur, D. Hurtmans, G. Pfister, B. Quennehen, J. L. Thomas, J.-C. Raut, K. S. Law, Z. Klimont, J. Hadji-Lazaro, M. George, and C. Clerbaux
Atmos. Chem. Phys., 14, 10119–10131, https://doi.org/10.5194/acp-14-10119-2014, https://doi.org/10.5194/acp-14-10119-2014, 2014
S. Chatani, M. Amann, A. Goel, J. Hao, Z. Klimont, A. Kumar, A. Mishra, S. Sharma, S. X. Wang, Y. X. Wang, and B. Zhao
Atmos. Chem. Phys., 14, 9259–9277, https://doi.org/10.5194/acp-14-9259-2014, https://doi.org/10.5194/acp-14-9259-2014, 2014
C. Fountoukis, A. G. Megaritis, K. Skyllakou, P. E. Charalampidis, C. Pilinis, H. A. C. Denier van der Gon, M. Crippa, F. Canonaco, C. Mohr, A. S. H. Prévôt, J. D. Allan, L. Poulain, T. Petäjä, P. Tiitta, S. Carbone, A. Kiendler-Scharr, E. Nemitz, C. O'Dowd, E. Swietlicki, and S. N. Pandis
Atmos. Chem. Phys., 14, 9061–9076, https://doi.org/10.5194/acp-14-9061-2014, https://doi.org/10.5194/acp-14-9061-2014, 2014
R. J. Park, S. K. Hong, H.-A. Kwon, S. Kim, A. Guenther, J.-H. Woo, and C. P. Loughner
Atmos. Chem. Phys., 14, 7929–7940, https://doi.org/10.5194/acp-14-7929-2014, https://doi.org/10.5194/acp-14-7929-2014, 2014
H.-K. Kim, J.-H. Woo, R. S. Park, C. H. Song, J.-H. Kim, S.-J. Ban, and J.-H. Park
Atmos. Chem. Phys., 14, 7461–7484, https://doi.org/10.5194/acp-14-7461-2014, https://doi.org/10.5194/acp-14-7461-2014, 2014
K. Markakis, M. Valari, A. Colette, O. Sanchez, O. Perrussel, C. Honore, R. Vautard, Z. Klimont, and S. Rao
Atmos. Chem. Phys., 14, 7323–7340, https://doi.org/10.5194/acp-14-7323-2014, https://doi.org/10.5194/acp-14-7323-2014, 2014
S. X. Wang, B. Zhao, S. Y. Cai, Z. Klimont, C. P. Nielsen, T. Morikawa, J. H. Woo, Y. Kim, X. Fu, J. Y. Xu, J. M. Hao, and K. B. He
Atmos. Chem. Phys., 14, 6571–6603, https://doi.org/10.5194/acp-14-6571-2014, https://doi.org/10.5194/acp-14-6571-2014, 2014
K. E. Yttri, C. Lund Myhre, S. Eckhardt, M. Fiebig, C. Dye, D. Hirdman, J. Ström, Z. Klimont, and A. Stohl
Atmos. Chem. Phys., 14, 6427–6442, https://doi.org/10.5194/acp-14-6427-2014, https://doi.org/10.5194/acp-14-6427-2014, 2014
M. Crippa, F. Canonaco, V. A. Lanz, M. Äijälä, J. D. Allan, S. Carbone, G. Capes, D. Ceburnis, M. Dall'Osto, D. A. Day, P. F. DeCarlo, M. Ehn, A. Eriksson, E. Freney, L. Hildebrandt Ruiz, R. Hillamo, J. L. Jimenez, H. Junninen, A. Kiendler-Scharr, A.-M. Kortelainen, M. Kulmala, A. Laaksonen, A. A. Mensah, C. Mohr, E. Nemitz, C. O'Dowd, J. Ovadnevaite, S. N. Pandis, T. Petäjä, L. Poulain, S. Saarikoski, K. Sellegri, E. Swietlicki, P. Tiitta, D. R. Worsnop, U. Baltensperger, and A. S. H. Prévôt
Atmos. Chem. Phys., 14, 6159–6176, https://doi.org/10.5194/acp-14-6159-2014, https://doi.org/10.5194/acp-14-6159-2014, 2014
D. Wen, L. Zhang, J. C. Lin, R. Vet, and M. D. Moran
Geosci. Model Dev., 7, 1037–1050, https://doi.org/10.5194/gmd-7-1037-2014, https://doi.org/10.5194/gmd-7-1037-2014, 2014
P. A. Makar, R. Nissen, A. Teakles, J. Zhang, Q. Zheng, M. D. Moran, H. Yau, and C. diCenzo
Geosci. Model Dev., 7, 1001–1024, https://doi.org/10.5194/gmd-7-1001-2014, https://doi.org/10.5194/gmd-7-1001-2014, 2014
X. Wang, L. Zhang, and M. D. Moran
Geosci. Model Dev., 7, 799–819, https://doi.org/10.5194/gmd-7-799-2014, https://doi.org/10.5194/gmd-7-799-2014, 2014
E. Galarneau, P. A. Makar, Q. Zheng, J. Narayan, J. Zhang, M. D. Moran, M. A. Bari, S. Pathela, A. Chen, and R. Chlumsky
Atmos. Chem. Phys., 14, 4065–4077, https://doi.org/10.5194/acp-14-4065-2014, https://doi.org/10.5194/acp-14-4065-2014, 2014
S. Itahashi, I. Uno, H. Irie, J.-I. Kurokawa, and T. Ohara
Atmos. Chem. Phys., 14, 3623–3635, https://doi.org/10.5194/acp-14-3623-2014, https://doi.org/10.5194/acp-14-3623-2014, 2014
C. Liu, S. Beirle, T. Butler, P. Hoor, C. Frankenberg, P. Jöckel, M. Penning de Vries, U. Platt, A. Pozzer, M. G. Lawrence, J. Lelieveld, H. Tost, and T. Wagner
Atmos. Chem. Phys., 14, 1717–1732, https://doi.org/10.5194/acp-14-1717-2014, https://doi.org/10.5194/acp-14-1717-2014, 2014
S.-L. von der Weiden-Reinmüller, F. Drewnick, M. Crippa, A. S. H. Prévôt, F. Meleux, U. Baltensperger, M. Beekmann, and S. Borrmann
Atmos. Meas. Tech., 7, 279–299, https://doi.org/10.5194/amt-7-279-2014, https://doi.org/10.5194/amt-7-279-2014, 2014
A. Mues, J. Kuenen, C. Hendriks, A. Manders, A. Segers, Y. Scholz, C. Hueglin, P. Builtjes, and M. Schaap
Atmos. Chem. Phys., 14, 939–955, https://doi.org/10.5194/acp-14-939-2014, https://doi.org/10.5194/acp-14-939-2014, 2014
M. E. Park, C. H. Song, R. S. Park, J. Lee, J. Kim, S. Lee, J.-H. Woo, G. R. Carmichael, T. F. Eck, B. N. Holben, S.-S. Lee, C. K. Song, and Y. D. Hong
Atmos. Chem. Phys., 14, 659–674, https://doi.org/10.5194/acp-14-659-2014, https://doi.org/10.5194/acp-14-659-2014, 2014
S. J. Smith and T. C. Bond
Atmos. Chem. Phys., 14, 537–549, https://doi.org/10.5194/acp-14-537-2014, https://doi.org/10.5194/acp-14-537-2014, 2014
S. J. Smith
Earth Syst. Dynam. Discuss., https://doi.org/10.5194/esdd-5-1-2014, https://doi.org/10.5194/esdd-5-1-2014, 2014
Revised manuscript has not been submitted
F. Canonaco, M. Crippa, J. G. Slowik, U. Baltensperger, and A. S. H. Prévôt
Atmos. Meas. Tech., 6, 3649–3661, https://doi.org/10.5194/amt-6-3649-2013, https://doi.org/10.5194/amt-6-3649-2013, 2013
Z. S. Stock, M. R. Russo, T. M. Butler, A. T. Archibald, M. G. Lawrence, P. J. Telford, N. L. Abraham, and J. A. Pyle
Atmos. Chem. Phys., 13, 12215–12231, https://doi.org/10.5194/acp-13-12215-2013, https://doi.org/10.5194/acp-13-12215-2013, 2013
J. Kurokawa, T. Ohara, T. Morikawa, S. Hanayama, G. Janssens-Maenhout, T. Fukui, K. Kawashima, and H. Akimoto
Atmos. Chem. Phys., 13, 11019–11058, https://doi.org/10.5194/acp-13-11019-2013, https://doi.org/10.5194/acp-13-11019-2013, 2013
L. Zhang, X. Wang, M. D. Moran, and J. Feng
Atmos. Chem. Phys., 13, 10005–10025, https://doi.org/10.5194/acp-13-10005-2013, https://doi.org/10.5194/acp-13-10005-2013, 2013
S. J. Smith and A. Rothwell
Biogeosciences, 10, 6323–6337, https://doi.org/10.5194/bg-10-6323-2013, https://doi.org/10.5194/bg-10-6323-2013, 2013
B. Zhao, S. X. Wang, H. Liu, J. Y. Xu, K. Fu, Z. Klimont, J. M. Hao, K. B. He, J. Cofala, and M. Amann
Atmos. Chem. Phys., 13, 9869–9897, https://doi.org/10.5194/acp-13-9869-2013, https://doi.org/10.5194/acp-13-9869-2013, 2013
G. Sarwar, J. Godowitch, B. H. Henderson, K. Fahey, G. Pouliot, W. T. Hutzell, R. Mathur, D. Kang, W. S. Goliff, and W. R. Stockwell
Atmos. Chem. Phys., 13, 9695–9712, https://doi.org/10.5194/acp-13-9695-2013, https://doi.org/10.5194/acp-13-9695-2013, 2013
R. M. Healy, J. Sciare, L. Poulain, M. Crippa, A. Wiedensohler, A. S. H. Prévôt, U. Baltensperger, R. Sarda-Estève, M. L. McGuire, C.-H. Jeong, E. McGillicuddy, I. P. O'Connor, J. R. Sodeau, G. J. Evans, and J. C. Wenger
Atmos. Chem. Phys., 13, 9479–9496, https://doi.org/10.5194/acp-13-9479-2013, https://doi.org/10.5194/acp-13-9479-2013, 2013
T. Stavrakou, J.-F. Müller, K. F. Boersma, R. J. van der A, J. Kurokawa, T. Ohara, and Q. Zhang
Atmos. Chem. Phys., 13, 9057–9082, https://doi.org/10.5194/acp-13-9057-2013, https://doi.org/10.5194/acp-13-9057-2013, 2013
A. Stohl, Z. Klimont, S. Eckhardt, K. Kupiainen, V. P. Shevchenko, V. M. Kopeikin, and A. N. Novigatsky
Atmos. Chem. Phys., 13, 8833–8855, https://doi.org/10.5194/acp-13-8833-2013, https://doi.org/10.5194/acp-13-8833-2013, 2013
M. Crippa, F. Canonaco, J. G. Slowik, I. El Haddad, P. F. DeCarlo, C. Mohr, M. F. Heringa, R. Chirico, N. Marchand, B. Temime-Roussel, E. Abidi, L. Poulain, A. Wiedensohler, U. Baltensperger, and A. S. H. Prévôt
Atmos. Chem. Phys., 13, 8411–8426, https://doi.org/10.5194/acp-13-8411-2013, https://doi.org/10.5194/acp-13-8411-2013, 2013
E. Solazzo, A. Riccio, I. Kioutsioukis, and S. Galmarini
Atmos. Chem. Phys., 13, 8315–8333, https://doi.org/10.5194/acp-13-8315-2013, https://doi.org/10.5194/acp-13-8315-2013, 2013
J. Xing, J. Pleim, R. Mathur, G. Pouliot, C. Hogrefe, C.-M. Gan, and C. Wei
Atmos. Chem. Phys., 13, 7531–7549, https://doi.org/10.5194/acp-13-7531-2013, https://doi.org/10.5194/acp-13-7531-2013, 2013
A. Colette, B. Bessagnet, R. Vautard, S. Szopa, S. Rao, S. Schucht, Z. Klimont, L. Menut, G. Clain, F. Meleux, G. Curci, and L. Rouïl
Atmos. Chem. Phys., 13, 7451–7471, https://doi.org/10.5194/acp-13-7451-2013, https://doi.org/10.5194/acp-13-7451-2013, 2013
S. Galmarini, I. Kioutsioukis, and E. Solazzo
Atmos. Chem. Phys., 13, 7153–7182, https://doi.org/10.5194/acp-13-7153-2013, https://doi.org/10.5194/acp-13-7153-2013, 2013
K. W. Appel, G. A. Pouliot, H. Simon, G. Sarwar, H. O. T. Pye, S. L. Napelenok, F. Akhtar, and S. J. Roselle
Geosci. Model Dev., 6, 883–899, https://doi.org/10.5194/gmd-6-883-2013, https://doi.org/10.5194/gmd-6-883-2013, 2013
M. Laborde, M. Crippa, T. Tritscher, Z. Jurányi, P. F. Decarlo, B. Temime-Roussel, N. Marchand, S. Eckhardt, A. Stohl, U. Baltensperger, A. S. H. Prévôt, E. Weingartner, and M. Gysel
Atmos. Chem. Phys., 13, 5831–5856, https://doi.org/10.5194/acp-13-5831-2013, https://doi.org/10.5194/acp-13-5831-2013, 2013
Q. J. Zhang, M. Beekmann, F. Drewnick, F. Freutel, J. Schneider, M. Crippa, A. S. H. Prevot, U. Baltensperger, L. Poulain, A. Wiedensohler, J. Sciare, V. Gros, A. Borbon, A. Colomb, V. Michoud, J.-F. Doussin, H. A. C. Denier van der Gon, M. Haeffelin, J.-C. Dupont, G. Siour, H. Petetin, B. Bessagnet, S. N. Pandis, A. Hodzic, O. Sanchez, C. Honoré, and O. Perrussel
Atmos. Chem. Phys., 13, 5767–5790, https://doi.org/10.5194/acp-13-5767-2013, https://doi.org/10.5194/acp-13-5767-2013, 2013
E. Solazzo, R. Bianconi, G. Pirovano, M. D. Moran, R. Vautard, C. Hogrefe, K. W. Appel, V. Matthias, P. Grossi, B. Bessagnet, J. Brandt, C. Chemel, J. H. Christensen, R. Forkel, X. V. Francis, A. B. Hansen, S. McKeen, U. Nopmongcol, M. Prank, K. N. Sartelet, A. Segers, J. D. Silver, G. Yarwood, J. Werhahn, J. Zhang, S. T. Rao, and S. Galmarini
Geosci. Model Dev., 6, 791–818, https://doi.org/10.5194/gmd-6-791-2013, https://doi.org/10.5194/gmd-6-791-2013, 2013
S. M. Burrows, P. J. Rayner, T. Butler, and M. G. Lawrence
Atmos. Chem. Phys., 13, 5473–5488, https://doi.org/10.5194/acp-13-5473-2013, https://doi.org/10.5194/acp-13-5473-2013, 2013
H. Irie, K. Yamaji, K. Ikeda, I. Uno, S. Itahashi, T. Ohara, and J. Kurokawa
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-14037-2013, https://doi.org/10.5194/acpd-13-14037-2013, 2013
Preprint withdrawn
D. Wen, J. C. Lin, L. Zhang, R. Vet, and M. D. Moran
Geosci. Model Dev., 6, 327–344, https://doi.org/10.5194/gmd-6-327-2013, https://doi.org/10.5194/gmd-6-327-2013, 2013
M. Crippa, P. F. DeCarlo, J. G. Slowik, C. Mohr, M. F. Heringa, R. Chirico, L. Poulain, F. Freutel, J. Sciare, J. Cozic, C. F. Di Marco, M. Elsasser, J. B. Nicolas, N. Marchand, E. Abidi, A. Wiedensohler, F. Drewnick, J. Schneider, S. Borrmann, E. Nemitz, R. Zimmermann, J.-L. Jaffrezo, A. S. H. Prévôt, and U. Baltensperger
Atmos. Chem. Phys., 13, 961–981, https://doi.org/10.5194/acp-13-961-2013, https://doi.org/10.5194/acp-13-961-2013, 2013
F. Freutel, J. Schneider, F. Drewnick, S.-L. von der Weiden-Reinmüller, M. Crippa, A. S. H. Prévôt, U. Baltensperger, L. Poulain, A. Wiedensohler, J. Sciare, R. Sarda-Estève, J. F. Burkhart, S. Eckhardt, A. Stohl, V. Gros, A. Colomb, V. Michoud, J. F. Doussin, A. Borbon, M. Haeffelin, Y. Morille, M. Beekmann, and S. Borrmann
Atmos. Chem. Phys., 13, 933–959, https://doi.org/10.5194/acp-13-933-2013, https://doi.org/10.5194/acp-13-933-2013, 2013
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Indicators of Global Climate Change 2022: annual update of large-scale indicators of the state of the climate system and human influence
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Kai Qin, Hongrui Gao, Xuancen Liu, Qin He, Pravash Tiwari, and Jason Blake Cohen
Earth Syst. Sci. Data, 16, 5287–5310, https://doi.org/10.5194/essd-16-5287-2024, https://doi.org/10.5194/essd-16-5287-2024, 2024
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Satellites have brought new opportunities for monitoring atmospheric NO2, although the results are limited by clouds and other factors, resulting in missing data. This work proposes a new process to obtain reliable data products with high coverage by reconstructing the raw data from multiple satellites. The results are validated in terms of traditional methods as well as variance maximization and demonstrate a good ability to reproduce known polluted and clean areas around the world.
Astrid Lampert, Rudolf Hankers, Thomas Feuerle, Thomas Rausch, Matthias Cremer, Maik Angermann, Mark Bitter, Jonas Füllgraf, Helmut Schulz, Ulf Bestmann, and Konrad B. Bärfuss
Earth Syst. Sci. Data, 16, 4777–4792, https://doi.org/10.5194/essd-16-4777-2024, https://doi.org/10.5194/essd-16-4777-2024, 2024
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We conducted flights above the North Sea and investigated changes in the wind field. The research aircraft measured wind speed, wind direction, temperature, humidity and sea surface at high resolution. Wind parks reduce the wind speed, and the data help to determine how long it takes for the wind speed to recover. The coast also plays an important role, and the wind speed varies with distance from the coast. The results help in wind park planning and better estimating the energy yield.
Liu Yan, Qiang Zhang, Bo Zheng, and Kebin He
Earth Syst. Sci. Data, 16, 4497–4509, https://doi.org/10.5194/essd-16-4497-2024, https://doi.org/10.5194/essd-16-4497-2024, 2024
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A new database of fuel-, vehicle-type-, and age-specific CO2 emissions from global on-road vehicles from 1970 to 2020 is developed with the fleet turnover model built in this study. Based on this database, the evolution of the global vehicle stock over 50 years is analyzed, the dominant emission contributors by vehicle and fuel type are identified, and the age distribution of on-road CO2 emissions is characterized further.
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Earth Syst. Sci. Data, 16, 4325–4350, https://doi.org/10.5194/essd-16-4325-2024, https://doi.org/10.5194/essd-16-4325-2024, 2024
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This study provides an overview of data availability from observation- and inventory-based CH4 emission estimates. It systematically compares them and provides recommendations for robust comparisons, aiming to steadily engage more parties in using observational methods to complement their UNFCCC submissions. Anticipating improvements in atmospheric modelling and observations, future developments need to resolve knowledge gaps in both approaches and to better quantify remaining uncertainty.
Mark Omara, Anthony Himmelberger, Katlyn MacKay, James P. Williams, Joshua Benmergui, Maryann Sargent, Steven C. Wofsy, and Ritesh Gautam
Earth Syst. Sci. Data, 16, 3973–3991, https://doi.org/10.5194/essd-16-3973-2024, https://doi.org/10.5194/essd-16-3973-2024, 2024
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We review, analyze, and synthesize previous peer-reviewed measurement-based data on facility-level oil and gas methane emissions and use these data to develop a high-resolution spatially explicit inventory of US basin-level and national methane emissions. This work provides an improved assessment of national methane emissions relative to government inventories in support of accurate and comprehensive methane emissions assessment, attribution, and mitigation.
Matthew W. Jones, Douglas I. Kelley, Chantelle A. Burton, Francesca Di Giuseppe, Maria Lucia F. Barbosa, Esther Brambleby, Andrew J. Hartley, Anna Lombardi, Guilherme Mataveli, Joe R. McNorton, Fiona R. Spuler, Jakob B. Wessel, John T. Abatzoglou, Liana O. Anderson, Niels Andela, Sally Archibald, Dolors Armenteras, Eleanor Burke, Rachel Carmenta, Emilio Chuvieco, Hamish Clarke, Stefan H. Doerr, Paulo M. Fernandes, Louis Giglio, Douglas S. Hamilton, Stijn Hantson, Sarah Harris, Piyush Jain, Crystal A. Kolden, Tiina Kurvits, Seppe Lampe, Sarah Meier, Stacey New, Mark Parrington, Morgane M. G. Perron, Yuquan Qu, Natasha S. Ribeiro, Bambang H. Saharjo, Jesus San-Miguel-Ayanz, Jacquelyn K. Shuman, Veerachai Tanpipat, Guido R. van der Werf, Sander Veraverbeke, and Gavriil Xanthopoulos
Earth Syst. Sci. Data, 16, 3601–3685, https://doi.org/10.5194/essd-16-3601-2024, https://doi.org/10.5194/essd-16-3601-2024, 2024
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This inaugural State of Wildfires report catalogues extreme fires of the 2023–2024 fire season. For key events, we analyse their predictability and drivers and attribute them to climate change and land use. We provide a seasonal outlook and decadal projections. Key anomalies occurred in Canada, Greece, and western Amazonia, with other high-impact events catalogued worldwide. Climate change significantly increased the likelihood of extreme fires, and mitigation is required to lessen future risk.
Yang Liu, Jie Chen, Yusheng Shi, Wei Zheng, Tianchan Shan, and Gang Wang
Earth Syst. Sci. Data, 16, 3495–3515, https://doi.org/10.5194/essd-16-3495-2024, https://doi.org/10.5194/essd-16-3495-2024, 2024
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Open biomass burning has a significant impact on regional and global air quality. To enhance the quantification of global emissions from open biomass burning, we have developed the Global Emissions Inventory from Open Biomass Burning (GEIOBB) dataset, which provides a global daily-scale database at 1 km resolution of multiple pollutant emissions. This database aids global-scale environmental analysis of biomass burning.
Nana Wu, Guannan Geng, Ruochong Xu, Shigan Liu, Xiaodong Liu, Qinren Shi, Ying Zhou, Yu Zhao, Huan Liu, Yu Song, Junyu Zheng, Qiang Zhang, and Kebin He
Earth Syst. Sci. Data, 16, 2893–2915, https://doi.org/10.5194/essd-16-2893-2024, https://doi.org/10.5194/essd-16-2893-2024, 2024
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The commonly used method for developing large-scale air pollutant emission datasets for China faces challenges due to limited availability of detailed parameter information. In this study, we develop an efficient integrated framework to gather such information by harmonizing seven heterogeneous inventories from five research institutions. Emission characterizations are analyzed and validated, demonstrating that the dataset provides more accurate emission magnitudes and spatiotemporal patterns.
Leonardo Hoinaski, Robson Will, and Camilo Bastos Ribeiro
Earth Syst. Sci. Data, 16, 2385–2405, https://doi.org/10.5194/essd-16-2385-2024, https://doi.org/10.5194/essd-16-2385-2024, 2024
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We introduce the Brazilian Atmospheric Inventories (BRAIN), the first comprehensive database for air quality studies in Brazil. The database encompasses hourly datasets of meteorology, emission sources, and ambient concentrations of multiple air pollutants covering the Brazilian territory. It combines local inventories, consolidated datasets, and internationally recommended models to provide essential data for developing air pollution control policies, even in data-scarce areas.
Ville-Veikko Paunu, Niko Karvosenoja, David Segersson, Susana López-Aparicio, Ole-Kenneth Nielsen, Marlene Schmidt Plejdrup, Throstur Thorsteinsson, Dam Thanh Vo, Jeroen Kuenen, Hugo Denier van der Gon, Jukka-Pekka Jalkanen, Jørgen Brandt, and Camilla Geels
Earth Syst. Sci. Data, 16, 1453–1474, https://doi.org/10.5194/essd-16-1453-2024, https://doi.org/10.5194/essd-16-1453-2024, 2024
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Air pollution is an important cause of adverse health effects, even in Nordic countries. To assess their health impacts, emission inventories with high spatial resolution are needed. We studied how national data and methods for the spatial distribution of the emissions compare to a European level inventory. For road transport the methods are well established, but for machinery and off-road emissions the current recommendations for the spatial distribution of these emissions should be improved.
Weijun Quan, Zhenfa Wang, Lin Qiao, Xiangdong Zheng, Junli Jin, Yinruo Li, Xiaomei Yin, Zhiqiang Ma, and Martin Wild
Earth Syst. Sci. Data, 16, 961–983, https://doi.org/10.5194/essd-16-961-2024, https://doi.org/10.5194/essd-16-961-2024, 2024
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Radiation components play important roles in various fields such as the Earth’s surface radiation budget, ecosystem productivity, and human health. In this study, a dataset consisting of quality-assured daily data of nine radiation components is presented based on the in situ measurements at the Shangdianzi regional GAW station in China during 2013–2022. The dataset can be applied in the validation of satellite products and numerical models and investigation of atmospheric radiation.
Ruben Urraca, Greet Janssens-Maenhout, Nicolás Álamos, Lucas Berna-Peña, Monica Crippa, Sabine Darras, Stijn Dellaert, Hugo Denier van der Gon, Mark Dowell, Nadine Gobron, Claire Granier, Giacomo Grassi, Marc Guevara, Diego Guizzardi, Kevin Gurney, Nicolás Huneeus, Sekou Keita, Jeroen Kuenen, Ana Lopez-Noreña, Enrique Puliafito, Geoffrey Roest, Simone Rossi, Antonin Soulie, and Antoon Visschedijk
Earth Syst. Sci. Data, 16, 501–523, https://doi.org/10.5194/essd-16-501-2024, https://doi.org/10.5194/essd-16-501-2024, 2024
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CoCO2-MOSAIC 1.0 is a global mosaic of regional bottom-up inventories providing gridded (0.1×0.1) monthly emissions of anthropogenic CO2. Regional inventories include country-specific information and finer spatial resolution than global inventories. CoCO2-MOSAIC provides harmonized access to these datasets and can be considered as a regionally accepted reference to assess the quality of global inventories, as done in the current paper.
Marc Guevara, Santiago Enciso, Carles Tena, Oriol Jorba, Stijn Dellaert, Hugo Denier van der Gon, and Carlos Pérez García-Pando
Earth Syst. Sci. Data, 16, 337–373, https://doi.org/10.5194/essd-16-337-2024, https://doi.org/10.5194/essd-16-337-2024, 2024
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A global dataset of emissions from thermal power plants was created for the year 2018. The resulting catalogue reports annual emissions of CO2 and co-emitted species (NOx, CO, SO2 and CH4) for more than 16000 individual facilities at their exact geographical locations. Information on the temporal and vertical distributions of the emissions is also provided at the facility level. The dataset is intended to support current and future satellite emission monitoring and inverse modelling efforts.
Pierre Friedlingstein, Michael O'Sullivan, Matthew W. Jones, Robbie M. Andrew, Dorothee C. E. Bakker, Judith Hauck, Peter Landschützer, Corinne Le Quéré, Ingrid T. Luijkx, Glen P. Peters, Wouter Peters, Julia Pongratz, Clemens Schwingshackl, Stephen Sitch, Josep G. Canadell, Philippe Ciais, Robert B. Jackson, Simone R. Alin, Peter Anthoni, Leticia Barbero, Nicholas R. Bates, Meike Becker, Nicolas Bellouin, Bertrand Decharme, Laurent Bopp, Ida Bagus Mandhara Brasika, Patricia Cadule, Matthew A. Chamberlain, Naveen Chandra, Thi-Tuyet-Trang Chau, Frédéric Chevallier, Louise P. Chini, Margot Cronin, Xinyu Dou, Kazutaka Enyo, Wiley Evans, Stefanie Falk, Richard A. Feely, Liang Feng, Daniel J. Ford, Thomas Gasser, Josefine Ghattas, Thanos Gkritzalis, Giacomo Grassi, Luke Gregor, Nicolas Gruber, Özgür Gürses, Ian Harris, Matthew Hefner, Jens Heinke, Richard A. Houghton, George C. Hurtt, Yosuke Iida, Tatiana Ilyina, Andrew R. Jacobson, Atul Jain, Tereza Jarníková, Annika Jersild, Fei Jiang, Zhe Jin, Fortunat Joos, Etsushi Kato, Ralph F. Keeling, Daniel Kennedy, Kees Klein Goldewijk, Jürgen Knauer, Jan Ivar Korsbakken, Arne Körtzinger, Xin Lan, Nathalie Lefèvre, Hongmei Li, Junjie Liu, Zhiqiang Liu, Lei Ma, Greg Marland, Nicolas Mayot, Patrick C. McGuire, Galen A. McKinley, Gesa Meyer, Eric J. Morgan, David R. Munro, Shin-Ichiro Nakaoka, Yosuke Niwa, Kevin M. O'Brien, Are Olsen, Abdirahman M. Omar, Tsuneo Ono, Melf Paulsen, Denis Pierrot, Katie Pocock, Benjamin Poulter, Carter M. Powis, Gregor Rehder, Laure Resplandy, Eddy Robertson, Christian Rödenbeck, Thais M. Rosan, Jörg Schwinger, Roland Séférian, T. Luke Smallman, Stephen M. Smith, Reinel Sospedra-Alfonso, Qing Sun, Adrienne J. Sutton, Colm Sweeney, Shintaro Takao, Pieter P. Tans, Hanqin Tian, Bronte Tilbrook, Hiroyuki Tsujino, Francesco Tubiello, Guido R. van der Werf, Erik van Ooijen, Rik Wanninkhof, Michio Watanabe, Cathy Wimart-Rousseau, Dongxu Yang, Xiaojuan Yang, Wenping Yuan, Xu Yue, Sönke Zaehle, Jiye Zeng, and Bo Zheng
Earth Syst. Sci. Data, 15, 5301–5369, https://doi.org/10.5194/essd-15-5301-2023, https://doi.org/10.5194/essd-15-5301-2023, 2023
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The Global Carbon Budget 2023 describes the methodology, main results, and data sets used to quantify the anthropogenic emissions of carbon dioxide (CO2) and their partitioning among the atmosphere, land ecosystems, and the ocean over the historical period (1750–2023). These living datasets are updated every year to provide the highest transparency and traceability in the reporting of CO2, the key driver of climate change.
Chi-Tsan Wang, Bok H. Baek, William Vizuete, Lawrence S. Engel, Jia Xing, Jaime Green, Marc Serre, Richard Strott, Jared Bowden, and Jung-Hun Woo
Earth Syst. Sci. Data, 15, 5261–5279, https://doi.org/10.5194/essd-15-5261-2023, https://doi.org/10.5194/essd-15-5261-2023, 2023
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Hazardous air pollutant (HAP) human exposure studies usually rely on local measurements or dispersion model methods, but those methods are limited under spatial and temporal conditions. We processed the US EPA emission data to simulate the hourly HAP emission patterns and applied the chemical transport model to simulate the HAP concentrations. The modeled HAP results exhibit good agreement (R is 0.75 and NMB is −5.6 %) with observational data.
Zeqi Li, Shuxiao Wang, Shengyue Li, Xiaochun Wang, Guanghan Huang, Xing Chang, Lyuyin Huang, Chengrui Liang, Yun Zhu, Haotian Zheng, Qian Song, Qingru Wu, Fenfen Zhang, and Bin Zhao
Earth Syst. Sci. Data, 15, 5017–5037, https://doi.org/10.5194/essd-15-5017-2023, https://doi.org/10.5194/essd-15-5017-2023, 2023
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This study developed the first full-volatility organic emission inventory for cooking sources in China, presenting high-resolution cooking emissions during 2015–2021. It identified the key subsectors and hotspots of cooking emissions, analyzed emission trends and drivers, and proposed future control strategies. The dataset is valuable for accurately simulating organic aerosol formation and evolution and for understanding the impact of organic emissions on air pollution and climate change.
Zi Huang, Jiaoyue Wang, Longfei Bing, Yijiao Qiu, Rui Guo, Ying Yu, Mingjing Ma, Le Niu, Dan Tong, Robbie M. Andrew, Pierre Friedlingstein, Josep G. Canadell, Fengming Xi, and Zhu Liu
Earth Syst. Sci. Data, 15, 4947–4958, https://doi.org/10.5194/essd-15-4947-2023, https://doi.org/10.5194/essd-15-4947-2023, 2023
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This is about global and regional cement process carbon emissions and CO2 uptake calculations from 1930 to 2019. The global cement production is rising to 4.4 Gt, causing processing carbon emission of 1.81 Gt (95% CI: 1.75–1.88 Gt CO2) in 2021. Plus, in 2021, cement’s carbon accumulated uptake (22.9 Gt, 95% CI: 19.6–22.6 Gt CO2) has offset 55.2% of cement process CO2 emissions (41.5 Gt, 95% CI: 38.7–47.1 Gt CO2) since 1930.
Wenjun Tang, Junmei He, Jingwen Qi, and Kun Yang
Earth Syst. Sci. Data, 15, 4537–4551, https://doi.org/10.5194/essd-15-4537-2023, https://doi.org/10.5194/essd-15-4537-2023, 2023
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In this study, we have developed a dense station-based, long-term dataset of daily surface solar radiation in China with high accuracy. The dataset consists of estimates of global, direct and diffuse radiation at 2473 meteorological stations from the 1950s to 2021. Validation indicates that our station-based radiation dataset clearly outperforms the satellite-based radiation products. Our dataset will contribute to climate change research and solar energy applications in the future.
Matthew J. McGrath, Ana Maria Roxana Petrescu, Philippe Peylin, Robbie M. Andrew, Bradley Matthews, Frank Dentener, Juraj Balkovič, Vladislav Bastrikov, Meike Becker, Gregoire Broquet, Philippe Ciais, Audrey Fortems-Cheiney, Raphael Ganzenmüller, Giacomo Grassi, Ian Harris, Matthew Jones, Jürgen Knauer, Matthias Kuhnert, Guillaume Monteil, Saqr Munassar, Paul I. Palmer, Glen P. Peters, Chunjing Qiu, Mart-Jan Schelhaas, Oksana Tarasova, Matteo Vizzarri, Karina Winkler, Gianpaolo Balsamo, Antoine Berchet, Peter Briggs, Patrick Brockmann, Frédéric Chevallier, Giulia Conchedda, Monica Crippa, Stijn N. C. Dellaert, Hugo A. C. Denier van der Gon, Sara Filipek, Pierre Friedlingstein, Richard Fuchs, Michael Gauss, Christoph Gerbig, Diego Guizzardi, Dirk Günther, Richard A. Houghton, Greet Janssens-Maenhout, Ronny Lauerwald, Bas Lerink, Ingrid T. Luijkx, Géraud Moulas, Marilena Muntean, Gert-Jan Nabuurs, Aurélie Paquirissamy, Lucia Perugini, Wouter Peters, Roberto Pilli, Julia Pongratz, Pierre Regnier, Marko Scholze, Yusuf Serengil, Pete Smith, Efisio Solazzo, Rona L. Thompson, Francesco N. Tubiello, Timo Vesala, and Sophia Walther
Earth Syst. Sci. Data, 15, 4295–4370, https://doi.org/10.5194/essd-15-4295-2023, https://doi.org/10.5194/essd-15-4295-2023, 2023
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Accurate estimation of fluxes of carbon dioxide from the land surface is essential for understanding future impacts of greenhouse gas emissions on the climate system. A wide variety of methods currently exist to estimate these sources and sinks. We are continuing work to develop annual comparisons of these diverse methods in order to clarify what they all actually calculate and to resolve apparent disagreement, in addition to highlighting opportunities for increased understanding.
Saroj Kumar Sahu, Poonam Mangaraj, and Gufran Beig
Earth Syst. Sci. Data, 15, 3183–3202, https://doi.org/10.5194/essd-15-3183-2023, https://doi.org/10.5194/essd-15-3183-2023, 2023
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The developed emission inventory identifies all the potential anthropogenic sources active in the Delhi NCR. The decadal change (2010–2020) and the changing policies have also been illustrated to observe the modulation in the sectorial emission trend. Emission hotspots with possible source-specific mitigation strategies have also been highlighted to improve the air quality of the Delhi NCR. The provided dataset is a vital tool for air quality and chemical transport modeling studies.
Steffen Beirle, Christian Borger, Adrian Jost, and Thomas Wagner
Earth Syst. Sci. Data, 15, 3051–3073, https://doi.org/10.5194/essd-15-3051-2023, https://doi.org/10.5194/essd-15-3051-2023, 2023
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We present a catalog of nitrogen oxide emissions from point sources (like power plants or metal smelters) based on satellite observations of NO2 combined with meteorological wind fields.
Piers M. Forster, Christopher J. Smith, Tristram Walsh, William F. Lamb, Robin Lamboll, Mathias Hauser, Aurélien Ribes, Debbie Rosen, Nathan Gillett, Matthew D. Palmer, Joeri Rogelj, Karina von Schuckmann, Sonia I. Seneviratne, Blair Trewin, Xuebin Zhang, Myles Allen, Robbie Andrew, Arlene Birt, Alex Borger, Tim Boyer, Jiddu A. Broersma, Lijing Cheng, Frank Dentener, Pierre Friedlingstein, José M. Gutiérrez, Johannes Gütschow, Bradley Hall, Masayoshi Ishii, Stuart Jenkins, Xin Lan, June-Yi Lee, Colin Morice, Christopher Kadow, John Kennedy, Rachel Killick, Jan C. Minx, Vaishali Naik, Glen P. Peters, Anna Pirani, Julia Pongratz, Carl-Friedrich Schleussner, Sophie Szopa, Peter Thorne, Robert Rohde, Maisa Rojas Corradi, Dominik Schumacher, Russell Vose, Kirsten Zickfeld, Valérie Masson-Delmotte, and Panmao Zhai
Earth Syst. Sci. Data, 15, 2295–2327, https://doi.org/10.5194/essd-15-2295-2023, https://doi.org/10.5194/essd-15-2295-2023, 2023
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This is a critical decade for climate action, but there is no annual tracking of the level of human-induced warming. We build on the Intergovernmental Panel on Climate Change assessment reports that are authoritative but published infrequently to create a set of key global climate indicators that can be tracked through time. Our hope is that this becomes an important annual publication that policymakers, media, scientists and the public can refer to.
Shengyue Li, Shuxiao Wang, Qingru Wu, Yanning Zhang, Daiwei Ouyang, Haotian Zheng, Licong Han, Xionghui Qiu, Yifan Wen, Min Liu, Yueqi Jiang, Dejia Yin, Kaiyun Liu, Bin Zhao, Shaojun Zhang, Ye Wu, and Jiming Hao
Earth Syst. Sci. Data, 15, 2279–2294, https://doi.org/10.5194/essd-15-2279-2023, https://doi.org/10.5194/essd-15-2279-2023, 2023
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This study compiled China's emission inventory of air pollutants and CO2 during 2005–2021 (ABaCAS-EI v2.0) based on unified emission-source framework. The emission trends and its drivers are analyzed. Key sectors and regions with higher synergistic reduction potential of air pollutants and CO2 are identified. Future control measures are suggested. The dataset and analyses provide insights into the synergistic reduction of air pollutants and CO2 emissions for China and other developing countries.
Wouter B. Mol, Wouter H. Knap, and Chiel C. van Heerwaarden
Earth Syst. Sci. Data, 15, 2139–2151, https://doi.org/10.5194/essd-15-2139-2023, https://doi.org/10.5194/essd-15-2139-2023, 2023
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We describe a dataset of detailed measurements of sunlight reaching the surface, recorded at a rate of one measurement per second for 10 years. The dataset includes detailed information on direct and scattered sunlight; classifications and statistics of variability; and observations of clouds, atmospheric composition, and wind. The dataset can be used to study how the atmosphere influences sunlight variability and to validate models that aim to predict this variability with greater accuracy.
Ana Maria Roxana Petrescu, Chunjing Qiu, Matthew J. McGrath, Philippe Peylin, Glen P. Peters, Philippe Ciais, Rona L. Thompson, Aki Tsuruta, Dominik Brunner, Matthias Kuhnert, Bradley Matthews, Paul I. Palmer, Oksana Tarasova, Pierre Regnier, Ronny Lauerwald, David Bastviken, Lena Höglund-Isaksson, Wilfried Winiwarter, Giuseppe Etiope, Tuula Aalto, Gianpaolo Balsamo, Vladislav Bastrikov, Antoine Berchet, Patrick Brockmann, Giancarlo Ciotoli, Giulia Conchedda, Monica Crippa, Frank Dentener, Christine D. Groot Zwaaftink, Diego Guizzardi, Dirk Günther, Jean-Matthieu Haussaire, Sander Houweling, Greet Janssens-Maenhout, Massaer Kouyate, Adrian Leip, Antti Leppänen, Emanuele Lugato, Manon Maisonnier, Alistair J. Manning, Tiina Markkanen, Joe McNorton, Marilena Muntean, Gabriel D. Oreggioni, Prabir K. Patra, Lucia Perugini, Isabelle Pison, Maarit T. Raivonen, Marielle Saunois, Arjo J. Segers, Pete Smith, Efisio Solazzo, Hanqin Tian, Francesco N. Tubiello, Timo Vesala, Guido R. van der Werf, Chris Wilson, and Sönke Zaehle
Earth Syst. Sci. Data, 15, 1197–1268, https://doi.org/10.5194/essd-15-1197-2023, https://doi.org/10.5194/essd-15-1197-2023, 2023
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This study updates the state-of-the-art scientific overview of CH4 and N2O emissions in the EU27 and UK in Petrescu et al. (2021a). Yearly updates are needed to improve the different respective approaches and to inform on the development of formal verification systems. It integrates the most recent emission inventories, process-based model and regional/global inversions, comparing them with UNFCCC national GHG inventories, in support to policy to facilitate real-time verification procedures.
Akash Biswal, Vikas Singh, Leeza Malik, Geetam Tiwari, Khaiwal Ravindra, and Suman Mor
Earth Syst. Sci. Data, 15, 661–680, https://doi.org/10.5194/essd-15-661-2023, https://doi.org/10.5194/essd-15-661-2023, 2023
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This paper presents detailed emission estimates of on-road traffic exhaust emissions of nine major pollutants for Delhi. We use advanced traffic data and emission factors as a function of speed to estimate emissions for each hour and 100 m × 100 m spatial resolution. We examine the source contribution according to the vehicle, fuel, road and Euro types to identify the most polluting vehicles. These data are useful for high-resolution air quality modelling for developing suitable strategies.
Auke M. van der Woude, Remco de Kok, Naomi Smith, Ingrid T. Luijkx, Santiago Botía, Ute Karstens, Linda M. J. Kooijmans, Gerbrand Koren, Harro A. J. Meijer, Gert-Jan Steeneveld, Ida Storm, Ingrid Super, Hubertus A. Scheeren, Alex Vermeulen, and Wouter Peters
Earth Syst. Sci. Data, 15, 579–605, https://doi.org/10.5194/essd-15-579-2023, https://doi.org/10.5194/essd-15-579-2023, 2023
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To monitor the progress towards the CO2 emission goals set out in the Paris Agreement, the European Union requires an independent validation of emitted CO2. For this validation, atmospheric measurements of CO2 can be used, together with first-guess estimates of CO2 emissions and uptake. To quickly inform end users, it is imperative that this happens in near real-time. To aid these efforts, we create estimates of European CO2 exchange at high resolution in near real time.
David F. Pollard, Frank Hase, Mahesh Kumar Sha, Darko Dubravica, Carlos Alberti, and Dan Smale
Earth Syst. Sci. Data, 14, 5427–5437, https://doi.org/10.5194/essd-14-5427-2022, https://doi.org/10.5194/essd-14-5427-2022, 2022
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We describe measurements made in Antarctica using an EM27/SUN, a near-infrared, portable, low-resolution spectrometer from which we can retrieve the average atmospheric concentration of several greenhouse gases. We show that these measurements are reliable and comparable to other, similar ground-based measurements. Comparisons to the ESA's Sentinel-5 precursor (S5P) satellite demonstrate the usefulness of these data for satellite validation.
Giacomo Grassi, Giulia Conchedda, Sandro Federici, Raul Abad Viñas, Anu Korosuo, Joana Melo, Simone Rossi, Marieke Sandker, Zoltan Somogyi, Matteo Vizzarri, and Francesco N. Tubiello
Earth Syst. Sci. Data, 14, 4643–4666, https://doi.org/10.5194/essd-14-4643-2022, https://doi.org/10.5194/essd-14-4643-2022, 2022
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Despite increasing attention on the role of land use CO2 fluxes in climate change mitigation, there are large differences in available databases. Here we present the most updated and complete compilation of land use CO2 data based on country submissions to United Nations Framework Convention on Climate Change and explain differences with other datasets. Our dataset brings clarity of land use CO2 fluxes and helps track country progress under the Paris Agreement.
Thorsten Hoeser, Stefanie Feuerstein, and Claudia Kuenzer
Earth Syst. Sci. Data, 14, 4251–4270, https://doi.org/10.5194/essd-14-4251-2022, https://doi.org/10.5194/essd-14-4251-2022, 2022
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The DeepOWT (Deep-learning-derived Offshore Wind Turbines) data set provides offshore wind energy infrastructure locations and their temporal deployment dynamics from July 2016 until June 2021 on a global scale. It differentiates between offshore wind turbines, platforms under construction, and offshore wind farm substations. It is derived by applying deep-learning-based object detection to Sentinel-1 imagery.
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Short summary
This study responds to the global and regional atmospheric modelling community's need for a mosaic of air pollutant emissions with global coverage, long time series, spatially distributed data at a high time resolution, and a high sectoral resolution in order to enhance the understanding of transboundary air pollution. The mosaic approach to integrating official regional emission inventories with a global inventory based on a consistent methodology ensures policy-relevant results.
This study responds to the global and regional atmospheric modelling community's need for a...
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