Articles | Volume 13, issue 7
https://doi.org/10.5194/essd-13-3281-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/essd-13-3281-2021
© Author(s) 2021. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Observations from the NOAA P-3 aircraft during ATOMIC
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, Colorado, USA
NOAA Physical Sciences Laboratory, Boulder, Colorado, USA
Chris W. Fairall
NOAA Physical Sciences Laboratory, Boulder, Colorado, USA
Adriana Bailey
National Center for Atmospheric Research, Boulder, Colorado, USA
Haonan Chen
Cooperative Institute for Research in the Atmosphere, Colorado State University, Fort Collins, Colorado, USA
NOAA Physical Sciences Laboratory, Boulder, Colorado, USA
Patrick Y. Chuang
Department of Earth and Planetary Sciences, University of California Santa Cruz, Santa Cruz, California, USA
Gijs de Boer
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, Colorado, USA
NOAA Physical Sciences Laboratory, Boulder, Colorado, USA
Graham Feingold
NOAA Chemical Sciences Laboratory, Boulder, Colorado, USA
Dean Henze
College of Earth, Ocean, and Atmospheric Science, Oregon State University, Corvallis, Oregon, USA
Quinn T. Kalen
NOAA Aircraft Operations Center, Lakeland, Florida, USA
Jan Kazil
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, Colorado, USA
NOAA Chemical Sciences Laboratory, Boulder, Colorado, USA
Mason Leandro
Department of Earth and Planetary Sciences, University of California Santa Cruz, Santa Cruz, California, USA
Ashley Lundry
NOAA Aircraft Operations Center, Lakeland, Florida, USA
Ken Moran
Cooperative Institute for Research in Environmental Sciences, University of Colorado Boulder, Boulder, Colorado, USA
NOAA Physical Sciences Laboratory, Boulder, Colorado, USA
Dana A. Naeher
NOAA Aircraft Operations Center, Lakeland, Florida, USA
David Noone
College of Earth, Ocean, and Atmospheric Science, Oregon State University, Corvallis, Oregon, USA
Department of Physics, University of Auckland, Auckland, New Zealand
Akshar J. Patel
NOAA Aircraft Operations Center, Lakeland, Florida, USA
Sergio Pezoa
NOAA Physical Sciences Laboratory, Boulder, Colorado, USA
Ivan PopStefanija
ProSensing, Amherst, Massachusetts, USA
Elizabeth J. Thompson
NOAA Physical Sciences Laboratory, Boulder, Colorado, USA
James Warnecke
NOAA Aircraft Operations Center, Lakeland, Florida, USA
Paquita Zuidema
Rosenstiel School of Marine and Atmospheric Science, University of Miami, Miami, Florida, USA
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EGUsphere, https://doi.org/10.5194/egusphere-2025-2605, https://doi.org/10.5194/egusphere-2025-2605, 2025
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Fabian Hoffmann, Yao-Sheng Chen, and Graham Feingold
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Clouds reflect a substantial portion of the incoming solar radiation back into space. This capacity is determined by the number of cloud droplets, which in turn is influenced by the number of aerosol particles, forming the basis for aerosol–cloud–climate interactions. In this study, we use a simple entrainment parameterization to understand the effect of aerosol on cloud water in weakly and non-precipitating stratocumulus.
Abdulamid A. Fakoya, Jens Redemann, Pablo E. Saide, Lan Gao, Logan T. Mitchell, Calvin Howes, Amie Dobracki, Ian Chang, Gonzalo A. Ferrada, Kristina Pistone, Samuel E. Leblanc, Michal Segal-Rozenhaimer, Arthur J. Sedlacek III, Thomas Eck, Brent Holben, Pawan Gupta, Elena Lind, Paquita Zuidema, Gregory Carmichael, and Connor J. Flynn
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This preprint is open for discussion and under review for Atmospheric Chemistry and Physics (ACP).
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We explore how climate change and aerosol affect the evolution of marine low-clouds. Using high-resolution simulations, we find that warming has a stronger impact on these clouds, but aerosol becomes more important after the clouds form precipitation. Our results suggest that attempts to brighten these clouds using aerosol may become less effective in a warmer future due to the decrease in cloud cover.
Yao-Sheng Chen, Prasanth Prabhakaran, Fabian Hoffmann, Jan Kazil, Takanobu Yamaguchi, and Graham Feingold
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Aidan D. Pantoya, Stephanie R. Simonsen, Elisabeth Andrews, Ross Burgener, Christopher J. Cox, Gijs de Boer, Bryan D. Thomas, and Naruki Hiranuma
Aerosol Research, 3, 253–270, https://doi.org/10.5194/ar-3-253-2025, https://doi.org/10.5194/ar-3-253-2025, 2025
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We present continuous ice-nucleating particle data that were measured in the Alaskan Arctic from October 2021 to December 2023. We found a greater efficiency in the arctic immersion freezing during fall compared to those found previously at two mid-latitude sites, together with profound freezing efficiencies in spring, presumably due to arctic haze events. Our study will be useful for improving atmospheric models to simulate cloud feedback and determine their impact on the global radiative energy budget.
Florian Tornow, Ann Fridlind, George Tselioudis, Brian Cairns, Andrew Ackerman, Seethala Chellappan, David Painemal, Paquita Zuidema, Christiane Voigt, Simon Kirschler, and Armin Sorooshian
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Graham Feingold, Franziska Glassmeier, Jianhao Zhang, and Fabian Hoffmann
EGUsphere, https://doi.org/10.5194/egusphere-2025-1869, https://doi.org/10.5194/egusphere-2025-1869, 2025
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Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, P. Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankararaman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Johann Engelbrecht, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbigniew Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gómez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal L. Weagle, and Xi Zhao
Atmos. Chem. Phys., 25, 4665–4702, https://doi.org/10.5194/acp-25-4665-2025, https://doi.org/10.5194/acp-25-4665-2025, 2025
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Brian J. Butterworth, Brent G. T. Else, Kristina A. Brown, Christopher J. Mundy, William J. Williams, Lina M. Rotermund, and Gijs de Boer
EGUsphere, https://doi.org/10.5194/egusphere-2025-1802, https://doi.org/10.5194/egusphere-2025-1802, 2025
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Meloë S. F. Kacenelenbogen, Ralph Kuehn, Nandana Amarasinghe, Kerry Meyer, Edward Nowottnick, Mark Vaughan, Hong Chen, Sebastian Schmidt, Richard Ferrare, John Hair, Robert Levy, Hongbin Yu, Paquita Zuidema, Robert Holz, and Willem Marais
EGUsphere, https://doi.org/10.5194/egusphere-2025-1403, https://doi.org/10.5194/egusphere-2025-1403, 2025
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Aerosols perturb the radiation balance of the Earth-atmosphere system. To reduce the uncertainty in quantifying present-day climate change, we combine two satellite sensors and a model to assess the aerosol effects on radiation in all-sky conditions. Satellite-based and coincident aircraft measurements of aerosol radiative effects agree well over the Southeast Atlantic. This constitutes a crucial first evaluation before we apply our method to more years and regions of the world.
Christopher J. Cox, Janet M. Intrieri, Brian J. Butterworth, Gijs de Boer, Michael R. Gallagher, Jonathan Hamilton, Erik Hulm, Tilden Meyers, Sara M. Morris, Jackson Osborn, P. Ola G. Persson, Benjamin Schmatz, Matthew D. Shupe, and James M. Wilczak
Earth Syst. Sci. Data, 17, 1481–1499, https://doi.org/10.5194/essd-17-1481-2025, https://doi.org/10.5194/essd-17-1481-2025, 2025
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Snow is an essential water resource in the intermountain western United States, and predictions are made using models. We made observations to validate, constrain, and develop the models. The data are from the Study of Precipitation, the Lower Atmosphere and Surface for Hydrometeorology (SPLASH) campaign in Colorado's East River valley, 2021–2023. The measurements include meteorology and variables that quantify energy transfer between the atmosphere and surface. The data are available publicly.
Eric Giuffrida, Kate Johnson, Tyler Tatro, Paquita Zuidema, and Hamish Gordon
EGUsphere, https://doi.org/10.5194/egusphere-2025-511, https://doi.org/10.5194/egusphere-2025-511, 2025
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Smoke aerosols emitted from summer African fires periodically travel across the ocean and interact with one of Earth’s largest permanent cloud decks. Researchers quantify the heating and cooling effects of this interaction using climate models. However, the use of different historical weather matching methods has produced a large variation in results. Here we test method variations commonly used today, and conclude on new guidelines for achieving the most accurate results.
Isabel L. McCoy, Sunil Baidar, Paquita Zuidema, Jan Kazil, W. Alan Brewer, Wayne M. Angevine, and Graham Feingold
EGUsphere, https://doi.org/10.5194/egusphere-2025-520, https://doi.org/10.5194/egusphere-2025-520, 2025
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We use ship observations to investigate the dynamics of small clouds over the tropical oceans. When these cumulus clouds cluster together, they become more efficient at moving moisture into the cloud layer due to strengthened vertical air motions. This encourages further clustering and sustains clouds against diurnal variations in their environment. Greater resilience to environmental changes has implications for cumulus feedback on the climate, a significant uncertainty in future projections.
Kira Zeider, Kayla McCauley, Sanja Dmitrovic, Leong Wai Siu, Yonghoon Choi, Ewan C. Crosbie, Joshua P. DiGangi, Glenn S. Diskin, Simon Kirschler, John B. Nowak, Michael A. Shook, Kenneth L. Thornhill, Christiane Voigt, Edward L. Winstead, Luke D. Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 25, 2407–2422, https://doi.org/10.5194/acp-25-2407-2025, https://doi.org/10.5194/acp-25-2407-2025, 2025
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In situ aircraft data collected over the northwest Atlantic Ocean are utilized to compare aerosol conditions and turbulence between near-surface and below-cloud-base altitudes for different regimes of coupling strength between those two levels, along with how cloud microphysical properties vary across those regimes. Stronger coupling yields more homogenous aerosol structure vertically along with higher cloud drop concentrations and sea salt influence in clouds.
Amie Dobracki, Ernie R. Lewis, Arthur J. Sedlacek III, Tyler Tatro, Maria A. Zawadowicz, and Paquita Zuidema
Atmos. Chem. Phys., 25, 2333–2363, https://doi.org/10.5194/acp-25-2333-2025, https://doi.org/10.5194/acp-25-2333-2025, 2025
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Biomass-burning aerosol is commonly present in the marine boundary layer over the southeast Atlantic Ocean between June and October. Our research indicates that burning conditions, aerosol transport pathways, and prolonged oxidation processes (heterogeneous and aqueous phases) determine the chemical, microphysical, and optical properties of the boundary layer aerosol. Notably, we find that the aerosol optical properties can be estimated from the chemical properties alone.
Haochi Che, Lu Zhang, Michal Segal-Rozenhaimer, Caroline Dang, Paquita Zuidema, and Arthur J. Sedlacek III
EGUsphere, https://doi.org/10.5194/egusphere-2024-3304, https://doi.org/10.5194/egusphere-2024-3304, 2024
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We investigated how biomass burning (BB) affects cloud formation in the southeast Atlantic. We found that aerosol hygroscopicity, which influences cloud droplet formation, varied monthly and differed significantly between 2016 and 2017, due to changes in sulfate aerosols. These changes were driven by BB burning conditions, which were likely influenced by meteorological factors. This study highlights the important role of BB in shaping aerosol properties and clouds in the region.
Fabian Hoffmann, Franziska Glassmeier, and Graham Feingold
Atmos. Chem. Phys., 24, 13403–13412, https://doi.org/10.5194/acp-24-13403-2024, https://doi.org/10.5194/acp-24-13403-2024, 2024
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Clouds constitute a major cooling influence on Earth's climate system by reflecting a large fraction of the incident solar radiation back to space. This ability is controlled by the number of cloud droplets, which is governed by the number of aerosol particles in the atmosphere, laying the foundation for so-called aerosol–cloud–climate interactions. In this study, a simple model to understand the effect of aerosol on cloud water is developed and applied.
Yao-Sheng Chen, Jianhao Zhang, Fabian Hoffmann, Takanobu Yamaguchi, Franziska Glassmeier, Xiaoli Zhou, and Graham Feingold
Atmos. Chem. Phys., 24, 12661–12685, https://doi.org/10.5194/acp-24-12661-2024, https://doi.org/10.5194/acp-24-12661-2024, 2024
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Marine stratocumulus cloud is a type of shallow cloud that covers the vast areas of Earth's surface. It plays an important role in Earth's energy balance by reflecting solar radiation back to space. We used numerical models to simulate a large number of marine stratocumuli with different characteristics. We found that how the clouds develop throughout the day is affected by the level of humidity in the air above the clouds and how closely the clouds connect to the ocean surface.
Randall Chiu, Florian Obersteiner, Alessandro Franchin, Teresa Campos, Adriana Bailey, Christopher Webster, Andreas Zahn, and Rainer Volkamer
Atmos. Meas. Tech., 17, 5731–5746, https://doi.org/10.5194/amt-17-5731-2024, https://doi.org/10.5194/amt-17-5731-2024, 2024
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The ozone sink into oceans and marine clouds is seldom studied and highly uncertain. Calculations suggest O3 destruction at aqueous surfaces (ocean, droplets) may be strongly accelerated, but field evidence is missing. Here we compare three fast airborne O3 instruments to measure eddy covariance fluxes of O3 over the remote ocean, in clear and cloudy air. We find O3 fluxes below clouds are consistently directed into clouds, while O3 fluxes into oceans are much smaller and spatially variable.
Jianhao Zhang, Yao-Sheng Chen, Takanobu Yamaguchi, and Graham Feingold
Atmos. Chem. Phys., 24, 10425–10440, https://doi.org/10.5194/acp-24-10425-2024, https://doi.org/10.5194/acp-24-10425-2024, 2024
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Quantifying cloud response to aerosol perturbations presents a major challenge in understanding the human impact on climate. Using a large number of process-resolving simulations of marine stratocumulus, we show that solar heating drives a negative feedback mechanism that buffers the persistent negative trend in cloud water adjustment after sunrise. This finding has implications for the dependence of the cloud cooling effect on the timing of deliberate aerosol perturbations.
Kristina Pistone, Eric M. Wilcox, Paquita Zuidema, Marco Giordano, James Podolske, Samuel E. LeBlanc, Meloë Kacenelenbogen, Steven G. Howell, and Steffen Freitag
Atmos. Chem. Phys., 24, 7983–8005, https://doi.org/10.5194/acp-24-7983-2024, https://doi.org/10.5194/acp-24-7983-2024, 2024
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The springtime southeast Atlantic atmosphere contains lots of smoke from continental fires. This smoke travels with water vapor; more smoke means more humidity. We use aircraft observations and models to describe how the values change through the season and over the region. We sort the atmosphere into different types by vertical structure and amount of smoke and humidity. Since our work shows how frequently these components coincide, it helps to better quantify heating effects over this region.
Laura Bianco, Bianca Adler, Ludovic Bariteau, Irina V. Djalalova, Timothy Myers, Sergio Pezoa, David D. Turner, and James M. Wilczak
Atmos. Meas. Tech., 17, 3933–3948, https://doi.org/10.5194/amt-17-3933-2024, https://doi.org/10.5194/amt-17-3933-2024, 2024
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The Tropospheric Remotely Observed Profiling via Optimal Estimation physical retrieval is used to retrieve temperature and humidity profiles from various combinations of passive and active remote sensing instruments, surface platforms, and numerical weather prediction models. The retrieved profiles are assessed against collocated radiosonde in non-cloudy conditions to assess the sensitivity of the retrievals to different input combinations. Case studies with cloudy conditions are also inspected.
Francesca Lappin, Gijs de Boer, Petra Klein, Jonathan Hamilton, Michelle Spencer, Radiance Calmer, Antonio R. Segales, Michael Rhodes, Tyler M. Bell, Justin Buchli, Kelsey Britt, Elizabeth Asher, Isaac Medina, Brian Butterworth, Leia Otterstatter, Madison Ritsch, Bryony Puxley, Angelina Miller, Arianna Jordan, Ceu Gomez-Faulk, Elizabeth Smith, Steven Borenstein, Troy Thornberry, Brian Argrow, and Elizabeth Pillar-Little
Earth Syst. Sci. Data, 16, 2525–2541, https://doi.org/10.5194/essd-16-2525-2024, https://doi.org/10.5194/essd-16-2525-2024, 2024
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This article provides an overview of the lower-atmospheric dataset collected by two uncrewed aerial systems near the Gulf of Mexico coastline south of Houston, TX, USA, as part of the TRacking Aerosol Convection interactions ExpeRiment (TRACER) campaign. The data were collected through boundary layer transitions, through sea breeze circulations, and in the pre- and near-storm environment to understand how these processes influence the coastal environment.
Stephanie Fiedler, Vaishali Naik, Fiona M. O'Connor, Christopher J. Smith, Paul Griffiths, Ryan J. Kramer, Toshihiko Takemura, Robert J. Allen, Ulas Im, Matthew Kasoar, Angshuman Modak, Steven Turnock, Apostolos Voulgarakis, Duncan Watson-Parris, Daniel M. Westervelt, Laura J. Wilcox, Alcide Zhao, William J. Collins, Michael Schulz, Gunnar Myhre, and Piers M. Forster
Geosci. Model Dev., 17, 2387–2417, https://doi.org/10.5194/gmd-17-2387-2024, https://doi.org/10.5194/gmd-17-2387-2024, 2024
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Climate scientists want to better understand modern climate change. Thus, climate model experiments are performed and compared. The results of climate model experiments differ, as assessed in the latest Intergovernmental Panel on Climate Change (IPCC) assessment report. This article gives insights into the challenges and outlines opportunities for further improving the understanding of climate change. It is based on views of a group of experts in atmospheric composition–climate interactions.
Leah Bertrand, Jennifer E. Kay, John Haynes, and Gijs de Boer
Earth Syst. Sci. Data, 16, 1301–1316, https://doi.org/10.5194/essd-16-1301-2024, https://doi.org/10.5194/essd-16-1301-2024, 2024
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The vertical structure of clouds has a major impact on global energy flows, air circulation, and the hydrologic cycle. Two satellite instruments, CloudSat radar and CALIPSO lidar, have taken complementary measurements of cloud vertical structure for over a decade. Here, we present the 3S-GEOPROF-COMB product, a globally gridded satellite data product combining CloudSat and CALIPSO observations of cloud vertical structure.
Prasanth Prabhakaran, Fabian Hoffmann, and Graham Feingold
Atmos. Chem. Phys., 24, 1919–1937, https://doi.org/10.5194/acp-24-1919-2024, https://doi.org/10.5194/acp-24-1919-2024, 2024
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In this study, we explore the impact of deliberate aerosol perturbation in the northeast Pacific region using large-eddy simulations. Our results show that cloud reflectivity is sensitive to the aerosol sprayer arrangement in the pristine system, whereas in the polluted system it is largely proportional to the total number of aerosol particles injected. These insights would aid in assessing the efficiency of various aerosol injection strategies for climate intervention applications.
Natalie M. Mahowald, Longlei Li, Julius Vira, Marje Prank, Douglas S. Hamilton, Hitoshi Matsui, Ron L. Miller, Louis Lu, Ezgi Akyuz, Daphne Meidan, Peter Hess, Heikki Lihavainen, Christine Wiedinmyer, Jenny Hand, Maria Grazia Alaimo, Célia Alves, Andres Alastuey, Paulo Artaxo, Africa Barreto, Francisco Barraza, Silvia Becagli, Giulia Calzolai, Shankarararman Chellam, Ying Chen, Patrick Chuang, David D. Cohen, Cristina Colombi, Evangelia Diapouli, Gaetano Dongarra, Konstantinos Eleftheriadis, Corinne Galy-Lacaux, Cassandra Gaston, Dario Gomez, Yenny González Ramos, Hannele Hakola, Roy M. Harrison, Chris Heyes, Barak Herut, Philip Hopke, Christoph Hüglin, Maria Kanakidou, Zsofia Kertesz, Zbiginiw Klimont, Katriina Kyllönen, Fabrice Lambert, Xiaohong Liu, Remi Losno, Franco Lucarelli, Willy Maenhaut, Beatrice Marticorena, Randall V. Martin, Nikolaos Mihalopoulos, Yasser Morera-Gomez, Adina Paytan, Joseph Prospero, Sergio Rodríguez, Patricia Smichowski, Daniela Varrica, Brenna Walsh, Crystal Weagle, and Xi Zhao
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-1, https://doi.org/10.5194/essd-2024-1, 2024
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Aerosol particles can interact with incoming solar radiation and outgoing long wave radiation, change cloud properties, affect photochemistry, impact surface air quality, and when deposited impact surface albedo of snow and ice, and modulate carbon dioxide uptake by the land and ocean. Here we present a new compilation of aerosol observations including composition, a methodology for comparing the datasets to model output, and show the implications of these results using one model.
Gina C. Jozef, John J. Cassano, Sandro Dahlke, Mckenzie Dice, Christopher J. Cox, and Gijs de Boer
Atmos. Chem. Phys., 24, 1429–1450, https://doi.org/10.5194/acp-24-1429-2024, https://doi.org/10.5194/acp-24-1429-2024, 2024
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Observations collected during MOSAiC were used to identify the range in vertical structure and stability of the central Arctic lower atmosphere through a self-organizing map analysis. Characteristics of wind features (such as low-level jets) and atmospheric moisture features (such as clouds) were analyzed in the context of the varying vertical structure and stability. Thus, the results of this paper give an overview of the thermodynamic and kinematic features of the central Arctic atmosphere.
Dean Henze, David Noone, and Darin Toohey
Atmos. Chem. Phys., 23, 15269–15288, https://doi.org/10.5194/acp-23-15269-2023, https://doi.org/10.5194/acp-23-15269-2023, 2023
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The interaction between biomass burning aerosols and clouds remains challenging to accurately determine from observations. This is in part because of difficulties distinguishing aerosol differences due to precipitation versus dilution processes from the observations. This study addresses the challenge by utilizing atmospheric heavy water isotope ratios to constrain mixing versus precipitation processes during a field campaign (ORACLES) and in turn explain observed aerosol concentrations.
Gina C. Jozef, Robert Klingel, John J. Cassano, Björn Maronga, Gijs de Boer, Sandro Dahlke, and Christopher J. Cox
Earth Syst. Sci. Data, 15, 4983–4995, https://doi.org/10.5194/essd-15-4983-2023, https://doi.org/10.5194/essd-15-4983-2023, 2023
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Observations from the MOSAiC expedition relating to lower-atmospheric temperature, wind, stability, moisture, and surface radiation budget from radiosondes, a meteorological tower, radiation station, and ceilometer were compiled to create a dataset which describes the thermodynamic and kinematic state of the central Arctic lower atmosphere between October 2019 and September 2020. This paper describes the methods used to develop this lower-atmospheric properties dataset.
Calvin Howes, Pablo E. Saide, Hugh Coe, Amie Dobracki, Steffen Freitag, Jim M. Haywood, Steven G. Howell, Siddhant Gupta, Janek Uin, Mary Kacarab, Chongai Kuang, L. Ruby Leung, Athanasios Nenes, Greg M. McFarquhar, James Podolske, Jens Redemann, Arthur J. Sedlacek, Kenneth L. Thornhill, Jenny P. S. Wong, Robert Wood, Huihui Wu, Yang Zhang, Jianhao Zhang, and Paquita Zuidema
Atmos. Chem. Phys., 23, 13911–13940, https://doi.org/10.5194/acp-23-13911-2023, https://doi.org/10.5194/acp-23-13911-2023, 2023
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To better understand smoke properties and its interactions with clouds, we compare the WRF-CAM5 model with observations from ORACLES, CLARIFY, and LASIC field campaigns in the southeastern Atlantic in August 2017. The model transports and mixes smoke well but does not fully capture some important processes. These include smoke chemical and physical aging over 4–12 days, smoke removal by rain, sulfate particle formation, aerosol activation into cloud droplets, and boundary layer turbulence.
Gina C. Jozef, John J. Cassano, Sandro Dahlke, Mckenzie Dice, Christopher J. Cox, and Gijs de Boer
Atmos. Chem. Phys., 23, 13087–13106, https://doi.org/10.5194/acp-23-13087-2023, https://doi.org/10.5194/acp-23-13087-2023, 2023
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Observations from the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) were used to determine the frequency of occurrence of various central Arctic lower atmospheric stability regimes and how the stability regimes transition between each other. Wind and radiation observations were analyzed in the context of stability regime and season to reveal the relationships between Arctic atmospheric stability and mechanically and radiatively driven turbulent forcings.
Mampi Sarkar, Adriana Bailey, Peter Blossey, Simon P. de Szoeke, David Noone, Estefanía Quiñones Meléndez, Mason D. Leandro, and Patrick Y. Chuang
Atmos. Chem. Phys., 23, 12671–12690, https://doi.org/10.5194/acp-23-12671-2023, https://doi.org/10.5194/acp-23-12671-2023, 2023
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We study rain evaporation characteristics below shallow cumulus clouds over the North Atlantic Ocean by pairing isotope observations with a microphysical model. The modeled fraction of rain mass that evaporates below the cloud strongly depends on the raindrop size and distribution width. Moreover, the higher the rain mass fraction evaporated, the greater the change in deuterium excess. In this way, rain evaporation could be studied independently using only isotope and microphysical observations.
Armin Sorooshian, Mikhail D. Alexandrov, Adam D. Bell, Ryan Bennett, Grace Betito, Sharon P. Burton, Megan E. Buzanowicz, Brian Cairns, Eduard V. Chemyakin, Gao Chen, Yonghoon Choi, Brian L. Collister, Anthony L. Cook, Andrea F. Corral, Ewan C. Crosbie, Bastiaan van Diedenhoven, Joshua P. DiGangi, Glenn S. Diskin, Sanja Dmitrovic, Eva-Lou Edwards, Marta A. Fenn, Richard A. Ferrare, David van Gilst, Johnathan W. Hair, David B. Harper, Miguel Ricardo A. Hilario, Chris A. Hostetler, Nathan Jester, Michael Jones, Simon Kirschler, Mary M. Kleb, John M. Kusterer, Sean Leavor, Joseph W. Lee, Hongyu Liu, Kayla McCauley, Richard H. Moore, Joseph Nied, Anthony Notari, John B. Nowak, David Painemal, Kasey E. Phillips, Claire E. Robinson, Amy Jo Scarino, Joseph S. Schlosser, Shane T. Seaman, Chellappan Seethala, Taylor J. Shingler, Michael A. Shook, Kenneth A. Sinclair, William L. Smith Jr., Douglas A. Spangenberg, Snorre A. Stamnes, Kenneth L. Thornhill, Christiane Voigt, Holger Vömel, Andrzej P. Wasilewski, Hailong Wang, Edward L. Winstead, Kira Zeider, Xubin Zeng, Bo Zhang, Luke D. Ziemba, and Paquita Zuidema
Earth Syst. Sci. Data, 15, 3419–3472, https://doi.org/10.5194/essd-15-3419-2023, https://doi.org/10.5194/essd-15-3419-2023, 2023
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The NASA Aerosol Cloud meTeorology Interactions oVer the western ATlantic Experiment (ACTIVATE) produced a unique dataset for research into aerosol–cloud–meteorology interactions. HU-25 Falcon and King Air aircraft conducted systematic and spatially coordinated flights over the northwest Atlantic Ocean. This paper describes the ACTIVATE flight strategy, instrument and complementary dataset products, data access and usage details, and data application notes.
Robert Pincus, Paul A. Hubanks, Steven Platnick, Kerry Meyer, Robert E. Holz, Denis Botambekov, and Casey J. Wall
Earth Syst. Sci. Data, 15, 2483–2497, https://doi.org/10.5194/essd-15-2483-2023, https://doi.org/10.5194/essd-15-2483-2023, 2023
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This paper describes a new global dataset of cloud properties observed by a specific satellite program created to facilitate comparison with a matching observational proxy used in climate models. Statistics are accumulated over daily and monthly timescales on an equal-angle grid. Statistics include cloud detection, cloud-top pressure, and cloud optical properties. Joint histograms of several variable pairs are also available.
Ulrike Egerer, John J. Cassano, Matthew D. Shupe, Gijs de Boer, Dale Lawrence, Abhiram Doddi, Holger Siebert, Gina Jozef, Radiance Calmer, Jonathan Hamilton, Christian Pilz, and Michael Lonardi
Atmos. Meas. Tech., 16, 2297–2317, https://doi.org/10.5194/amt-16-2297-2023, https://doi.org/10.5194/amt-16-2297-2023, 2023
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This paper describes how measurements from a small uncrewed aircraft system can be used to estimate the vertical turbulent heat energy exchange between different layers in the atmosphere. This is particularly important for the atmosphere in the Arctic, as turbulent exchange in this region is often suppressed but is still important to understand how the atmosphere interacts with sea ice. We present three case studies from the MOSAiC field campaign in Arctic sea ice in 2020.
Amie Dobracki, Paquita Zuidema, Steven G. Howell, Pablo Saide, Steffen Freitag, Allison C. Aiken, Sharon P. Burton, Arthur J. Sedlacek III, Jens Redemann, and Robert Wood
Atmos. Chem. Phys., 23, 4775–4799, https://doi.org/10.5194/acp-23-4775-2023, https://doi.org/10.5194/acp-23-4775-2023, 2023
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Southern Africa produces approximately one-third of the world’s carbon from fires. The thick smoke layer can flow westward, interacting with the southeastern Atlantic cloud deck. The net radiative impact can alter regional circulation patterns, impacting rainfall over Africa. We find that the smoke is highly absorbing of sunlight, mostly because it contains more black carbon than smoke over the Northern Hemisphere.
Hong Chen, K. Sebastian Schmidt, Steven T. Massie, Vikas Nataraja, Matthew S. Norgren, Jake J. Gristey, Graham Feingold, Robert E. Holz, and Hironobu Iwabuchi
Atmos. Meas. Tech., 16, 1971–2000, https://doi.org/10.5194/amt-16-1971-2023, https://doi.org/10.5194/amt-16-1971-2023, 2023
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We introduce the Education and Research 3D Radiative Transfer Toolbox (EaR3T) and propose a radiance self-consistency approach for quantifying and mitigating 3D bias in legacy airborne and spaceborne imagery retrievals due to spatially inhomogeneous clouds and surfaces.
Ian Chang, Lan Gao, Connor J. Flynn, Yohei Shinozuka, Sarah J. Doherty, Michael S. Diamond, Karla M. Longo, Gonzalo A. Ferrada, Gregory R. Carmichael, Patricia Castellanos, Arlindo M. da Silva, Pablo E. Saide, Calvin Howes, Zhixin Xue, Marc Mallet, Ravi Govindaraju, Qiaoqiao Wang, Yafang Cheng, Yan Feng, Sharon P. Burton, Richard A. Ferrare, Samuel E. LeBlanc, Meloë S. Kacenelenbogen, Kristina Pistone, Michal Segal-Rozenhaimer, Kerry G. Meyer, Ju-Mee Ryoo, Leonhard Pfister, Adeyemi A. Adebiyi, Robert Wood, Paquita Zuidema, Sundar A. Christopher, and Jens Redemann
Atmos. Chem. Phys., 23, 4283–4309, https://doi.org/10.5194/acp-23-4283-2023, https://doi.org/10.5194/acp-23-4283-2023, 2023
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Abundant aerosols are present above low-level liquid clouds over the southeastern Atlantic during late austral spring. The model simulation differences in the proportion of aerosol residing in the planetary boundary layer and in the free troposphere can greatly affect the regional aerosol radiative effects. This study examines the aerosol loading and fractional aerosol loading in the free troposphere among various models and evaluates them against measurements from the NASA ORACLES campaign.
Yabin Gou, Haonan Chen, Hong Zhu, and Lulin Xue
Atmos. Chem. Phys., 23, 2439–2463, https://doi.org/10.5194/acp-23-2439-2023, https://doi.org/10.5194/acp-23-2439-2023, 2023
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This article investigates the complex precipitation microphysics associated with super typhoon Lekima using a host of in situ and remote sensing observations, including rain gauge and disdrometer data, as well as polarimetric radar observations. The impacts of precipitation microphysics on multi-source data consistency and radar precipitation estimation are quantified. It is concluded that the dynamical precipitation microphysical processes must be considered in radar precipitation estimation.
Adriana Bailey, Franziska Aemisegger, Leonie Villiger, Sebastian A. Los, Gilles Reverdin, Estefanía Quiñones Meléndez, Claudia Acquistapace, Dariusz B. Baranowski, Tobias Böck, Sandrine Bony, Tobias Bordsdorff, Derek Coffman, Simon P. de Szoeke, Christopher J. Diekmann, Marina Dütsch, Benjamin Ertl, Joseph Galewsky, Dean Henze, Przemyslaw Makuch, David Noone, Patricia K. Quinn, Michael Rösch, Andreas Schneider, Matthias Schneider, Sabrina Speich, Bjorn Stevens, and Elizabeth J. Thompson
Earth Syst. Sci. Data, 15, 465–495, https://doi.org/10.5194/essd-15-465-2023, https://doi.org/10.5194/essd-15-465-2023, 2023
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One of the novel ways EUREC4A set out to investigate trade wind clouds and their coupling to the large-scale circulation was through an extensive network of isotopic measurements in water vapor, precipitation, and seawater. Samples were taken from the island of Barbados, from aboard two aircraft, and from aboard four ships. This paper describes the full collection of EUREC4A isotopic in situ data and guides readers to complementary remotely sensed water vapor isotope ratios.
Haley M. Royer, Mira L. Pöhlker, Ovid Krüger, Edmund Blades, Peter Sealy, Nurun Nahar Lata, Zezhen Cheng, Swarup China, Andrew P. Ault, Patricia K. Quinn, Paquita Zuidema, Christopher Pöhlker, Ulrich Pöschl, Meinrat Andreae, and Cassandra J. Gaston
Atmos. Chem. Phys., 23, 981–998, https://doi.org/10.5194/acp-23-981-2023, https://doi.org/10.5194/acp-23-981-2023, 2023
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This paper presents atmospheric particle chemical composition and measurements of aerosol water uptake properties collected at Ragged Point, Barbados, during the winter of 2020. The result of this study indicates the importance of small African smoke particles for cloud droplet formation in the tropical North Atlantic and highlights the large spatial and temporal pervasiveness of smoke over the Atlantic Ocean.
Jianhao Zhang and Graham Feingold
Atmos. Chem. Phys., 23, 1073–1090, https://doi.org/10.5194/acp-23-1073-2023, https://doi.org/10.5194/acp-23-1073-2023, 2023
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Using observations from space, we show maps of potential brightness changes in marine warm clouds in response to increases in cloud droplet concentrations. The environmental and aerosol conditions in which these clouds reside covary differently in each ocean basin, leading to distinct evolutions of cloud brightness changes. This work stresses the central importance of the covariability between meteorology and aerosol for scaling up the radiative response of cloud brightness changes.
Jonathan Hamilton, Gijs de Boer, Abhiram Doddi, and Dale A. Lawrence
Atmos. Meas. Tech., 15, 6789–6806, https://doi.org/10.5194/amt-15-6789-2022, https://doi.org/10.5194/amt-15-6789-2022, 2022
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The DataHawk2 is a small, low-cost, rugged, uncrewed aircraft system (UAS) used to observe the thermodynamic and turbulence structures of the lower atmosphere, supporting an advanced understanding of the physical processes that regulate weather and climate. This paper discusses the development, performance, and sensing capabilities of the DataHawk2 using data collected during several recent field deployments.
Ju-Mee Ryoo, Leonhard Pfister, Rei Ueyama, Paquita Zuidema, Robert Wood, Ian Chang, and Jens Redemann
Atmos. Chem. Phys., 22, 14209–14241, https://doi.org/10.5194/acp-22-14209-2022, https://doi.org/10.5194/acp-22-14209-2022, 2022
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The variability in the meteorological fields during each deployment is highly modulated at a daily to synoptic timescale. This paper, along with part 1, the climatological overview paper, provides a meteorological context for interpreting the airborne measurements gathered during the three ORACLES deployments. This study supports related studies focusing on the detailed investigation of the processes controlling stratocumulus decks, aerosol lifting, transport, and their interactions.
Paul A. Barrett, Steven J. Abel, Hugh Coe, Ian Crawford, Amie Dobracki, James Haywood, Steve Howell, Anthony Jones, Justin Langridge, Greg M. McFarquhar, Graeme J. Nott, Hannah Price, Jens Redemann, Yohei Shinozuka, Kate Szpek, Jonathan W. Taylor, Robert Wood, Huihui Wu, Paquita Zuidema, Stéphane Bauguitte, Ryan Bennett, Keith Bower, Hong Chen, Sabrina Cochrane, Michael Cotterell, Nicholas Davies, David Delene, Connor Flynn, Andrew Freedman, Steffen Freitag, Siddhant Gupta, David Noone, Timothy B. Onasch, James Podolske, Michael R. Poellot, Sebastian Schmidt, Stephen Springston, Arthur J. Sedlacek III, Jamie Trembath, Alan Vance, Maria A. Zawadowicz, and Jianhao Zhang
Atmos. Meas. Tech., 15, 6329–6371, https://doi.org/10.5194/amt-15-6329-2022, https://doi.org/10.5194/amt-15-6329-2022, 2022
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To better understand weather and climate, it is vital to go into the field and collect observations. Often measurements take place in isolation, but here we compared data from two aircraft and one ground-based site. This was done in order to understand how well measurements made on one platform compared to those made on another. Whilst this is easy to do in a controlled laboratory setting, it is more challenging in the real world, and so these comparisons are as valuable as they are rare.
Michael S. Diamond, Pablo E. Saide, Paquita Zuidema, Andrew S. Ackerman, Sarah J. Doherty, Ann M. Fridlind, Hamish Gordon, Calvin Howes, Jan Kazil, Takanobu Yamaguchi, Jianhao Zhang, Graham Feingold, and Robert Wood
Atmos. Chem. Phys., 22, 12113–12151, https://doi.org/10.5194/acp-22-12113-2022, https://doi.org/10.5194/acp-22-12113-2022, 2022
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Smoke from southern Africa blankets the southeast Atlantic from June-October, overlying a major transition region between overcast and scattered clouds. The smoke affects Earth's radiation budget by absorbing sunlight and changing cloud properties. We investigate these effects in regional climate and large eddy simulation models based on international field campaigns. We find that large-scale circulation changes more strongly affect cloud transitions than smoke microphysical effects in our case.
Vikas Nataraja, Sebastian Schmidt, Hong Chen, Takanobu Yamaguchi, Jan Kazil, Graham Feingold, Kevin Wolf, and Hironobu Iwabuchi
Atmos. Meas. Tech., 15, 5181–5205, https://doi.org/10.5194/amt-15-5181-2022, https://doi.org/10.5194/amt-15-5181-2022, 2022
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A convolutional neural network (CNN) is introduced to retrieve cloud optical thickness (COT) from passive cloud imagery. The CNN, trained on large eddy simulations from the Sulu Sea, learns from spatial information at multiple scales to reduce cloud inhomogeneity effects. By considering the spatial context of a pixel, the CNN outperforms the traditional independent pixel approximation (IPA) across several cloud morphology metrics.
Edward Gryspeerdt, Franziska Glassmeier, Graham Feingold, Fabian Hoffmann, and Rebecca J. Murray-Watson
Atmos. Chem. Phys., 22, 11727–11738, https://doi.org/10.5194/acp-22-11727-2022, https://doi.org/10.5194/acp-22-11727-2022, 2022
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The response of clouds to changes in aerosol remains a large uncertainty in our understanding of the climate. Studies typically look at aerosol and cloud processes in snapshot images, measuring all properties at the same time. Here we use multiple images to characterise how cloud temporal development responds to aerosol. We find a reduction in liquid water path with increasing aerosol, party due to feedbacks. This suggests the aerosol impact on cloud water may be weaker than in previous studies.
Fan Mei, Mikhail S. Pekour, Darielle Dexheimer, Gijs de Boer, RaeAnn Cook, Jason Tomlinson, Beat Schmid, Lexie A. Goldberger, Rob Newsom, and Jerome D. Fast
Earth Syst. Sci. Data, 14, 3423–3438, https://doi.org/10.5194/essd-14-3423-2022, https://doi.org/10.5194/essd-14-3423-2022, 2022
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This work focuses on an expanding number of data sets observed using ARM TBS (133 flights) and UAS (seven flights) platforms by the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility. These data streams provide new perspectives on spatial variability of atmospheric and surface parameters, helping to address critical science questions in Earth system science research, such as the aerosol–cloud interaction in the boundary layer.
Caroline Dang, Michal Segal-Rozenhaimer, Haochi Che, Lu Zhang, Paola Formenti, Jonathan Taylor, Amie Dobracki, Sara Purdue, Pui-Shan Wong, Athanasios Nenes, Arthur Sedlacek III, Hugh Coe, Jens Redemann, Paquita Zuidema, Steven Howell, and James Haywood
Atmos. Chem. Phys., 22, 9389–9412, https://doi.org/10.5194/acp-22-9389-2022, https://doi.org/10.5194/acp-22-9389-2022, 2022
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Transmission electron microscopy was used to analyze aged African smoke particles and how the smoke interacts with the marine atmosphere. We found that the volatility of organic aerosol increases with biomass burning plume age, that black carbon is often mixed with potassium salts and that the marine atmosphere can incorporate Na and Cl into smoke particles. Marine salts are more processed when mixed with smoke plumes, and there are interesting Cl-rich yet Na-absent marine particles.
Gina Jozef, John Cassano, Sandro Dahlke, and Gijs de Boer
Atmos. Meas. Tech., 15, 4001–4022, https://doi.org/10.5194/amt-15-4001-2022, https://doi.org/10.5194/amt-15-4001-2022, 2022
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During the MOSAiC expedition, meteorological conditions over the lowest 1 km of the atmosphere were sampled with the DataHawk2 uncrewed aircraft system. These data were used to identify the best method for atmospheric boundary layer height detection by comparing visually identified subjective boundary layer height to that identified by several objective automated detection methods. The results show a bulk Richardson number-based approach gives the best estimate of boundary layer height.
Haochi Che, Michal Segal-Rozenhaimer, Lu Zhang, Caroline Dang, Paquita Zuidema, Arthur J. Sedlacek III, Xiaoye Zhang, and Connor Flynn
Atmos. Chem. Phys., 22, 8767–8785, https://doi.org/10.5194/acp-22-8767-2022, https://doi.org/10.5194/acp-22-8767-2022, 2022
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A 17-month in situ study on Ascension Island found low single-scattering albedo and strong absorption enhancement of the marine boundary layer aerosols during biomass burnings on the African continent, along with apparent patterns of regular monthly variability. We further discuss the characteristics and drivers behind these changes and find that biomass burning conditions in Africa may be the main factor influencing the optical properties of marine boundary aerosols.
Patricia A. Cleary, Gijs de Boer, Joseph P. Hupy, Steven Borenstein, Jonathan Hamilton, Ben Kies, Dale Lawrence, R. Bradley Pierce, Joe Tirado, Aidan Voon, and Timothy Wagner
Earth Syst. Sci. Data, 14, 2129–2145, https://doi.org/10.5194/essd-14-2129-2022, https://doi.org/10.5194/essd-14-2129-2022, 2022
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A field campaign, WiscoDISCO-21, was conducted at the shoreline of Lake Michigan to better understand the role of marine air in pollutants. Two uncrewed aircraft systems were equipped with sensors for meteorological variables and ozone. A Doppler lidar instrument at a ground station measured horizontal and vertical winds. The overlap of observations from multiple instruments allowed for a unique mapping of the meteorology and pollutants as a marine air mass moved over land.
Christopher D. Wallis, Mason D. Leandro, Patrick Y. Chuang, and Anthony S. Wexler
Atmos. Meas. Tech., 15, 2547–2556, https://doi.org/10.5194/amt-15-2547-2022, https://doi.org/10.5194/amt-15-2547-2022, 2022
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Measuring emissions from stacks requires techniques to address a broad range of conditions and measurement challenges. Here we describe an instrument package held by a crane above a stack to characterize both wet droplet and dried aerosol emissions from cooling tower spray drift in situ. The instrument package characterizes the velocity, size distribution, and concentration of the wet droplet emissions and the mass concentration and elemental composition of the dried PM2.5 and PM10 emissions.
Andreas Schneider, Tobias Borsdorff, Joost aan de Brugh, Alba Lorente, Franziska Aemisegger, David Noone, Dean Henze, Rigel Kivi, and Jochen Landgraf
Atmos. Meas. Tech., 15, 2251–2275, https://doi.org/10.5194/amt-15-2251-2022, https://doi.org/10.5194/amt-15-2251-2022, 2022
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This paper presents an extended H₂O/HDO total column dataset from short-wave infrared measurements by TROPOMI including cloudy and clear-sky scenes. Coverage is tremendously increased compared to previous TROPOMI HDO datasets. The new dataset is validated against recent ground-based FTIR measurements from TCCON and against aircraft measurements over the ocean. The use of the new dataset is demonstrated with a case study of a cold air outbreak in January 2020.
Dean Henze, David Noone, and Darin Toohey
Earth Syst. Sci. Data, 14, 1811–1829, https://doi.org/10.5194/essd-14-1811-2022, https://doi.org/10.5194/essd-14-1811-2022, 2022
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The heavy isotope ratios of water vapor can provide information on the movement of water in the atmosphere, such as water vapor's origin of evaporation (e.g., land vs. sea), or detection of prior precipitation in an air mass. This paper presents the water vapor isotope dataset collected via aircraft as part of the NASA ORACLES project. The data are presented to demonstrate their potential for providing a comprehensive perspective on moisture transport in this region.
Graham Feingold, Tom Goren, and Takanobu Yamaguchi
Atmos. Chem. Phys., 22, 3303–3319, https://doi.org/10.5194/acp-22-3303-2022, https://doi.org/10.5194/acp-22-3303-2022, 2022
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The evaluation of radiative forcing associated with aerosol–cloud interactions remains a significant source of uncertainty in future climate projections. Using high-resolution numerical model output, we mimic typical satellite retrieval methodologies to show that data aggregation can introduce significant error (hundreds of percent) in the cloud albedo susceptibility metric. Spatial aggregation errors tend to be countered by temporal aggregation errors.
Jianhao Zhang, Xiaoli Zhou, Tom Goren, and Graham Feingold
Atmos. Chem. Phys., 22, 861–880, https://doi.org/10.5194/acp-22-861-2022, https://doi.org/10.5194/acp-22-861-2022, 2022
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Oceanic liquid-form clouds are effective sunlight reflectors. Their brightness is highly sensitive to changes in the amount of aerosol particles in the atmosphere and the state of the atmosphere they reside in. This study quantifies this sensitivity using long-term satellite observations and finds an overall cloud brightening (a cooling effect) potential and an essential role of the covarying meteorological conditions in governing this sensitivity for northeastern Pacific stratocumulus.
Matthew W. Christensen, Andrew Gettelman, Jan Cermak, Guy Dagan, Michael Diamond, Alyson Douglas, Graham Feingold, Franziska Glassmeier, Tom Goren, Daniel P. Grosvenor, Edward Gryspeerdt, Ralph Kahn, Zhanqing Li, Po-Lun Ma, Florent Malavelle, Isabel L. McCoy, Daniel T. McCoy, Greg McFarquhar, Johannes Mülmenstädt, Sandip Pal, Anna Possner, Adam Povey, Johannes Quaas, Daniel Rosenfeld, Anja Schmidt, Roland Schrödner, Armin Sorooshian, Philip Stier, Velle Toll, Duncan Watson-Parris, Robert Wood, Mingxi Yang, and Tianle Yuan
Atmos. Chem. Phys., 22, 641–674, https://doi.org/10.5194/acp-22-641-2022, https://doi.org/10.5194/acp-22-641-2022, 2022
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Trace gases and aerosols (tiny airborne particles) are released from a variety of point sources around the globe. Examples include volcanoes, industrial chimneys, forest fires, and ship stacks. These sources provide opportunistic experiments with which to quantify the role of aerosols in modifying cloud properties. We review the current state of understanding on the influence of aerosol on climate built from the wide range of natural and anthropogenic laboratories investigated in recent decades.
Gijs de Boer, Steven Borenstein, Radiance Calmer, Christopher Cox, Michael Rhodes, Christopher Choate, Jonathan Hamilton, Jackson Osborn, Dale Lawrence, Brian Argrow, and Janet Intrieri
Earth Syst. Sci. Data, 14, 19–31, https://doi.org/10.5194/essd-14-19-2022, https://doi.org/10.5194/essd-14-19-2022, 2022
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This article provides a summary of the collection of atmospheric data over the near-coastal zone upwind of Barbados during the ATOMIC and EUREC4A field campaigns. These data were collected to improve our understanding of the structure and dynamics of the lower atmosphere in the tropical trade-wind regime over the Atlantic Ocean and the influence of that portion of the atmosphere on the development and maintenance of clouds.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Michal Segal Rozenhaimer, Meloë Kacenelenbogen, Yohei Shinozuka, Connor Flynn, Rich Ferrare, Sharon Burton, Chris Hostetler, Marc Mallet, and Paquita Zuidema
Atmos. Meas. Tech., 15, 61–77, https://doi.org/10.5194/amt-15-61-2022, https://doi.org/10.5194/amt-15-61-2022, 2022
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This work presents heating rates derived from aircraft observations from the 2016 and 2017 field campaigns of ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS). We separate the total heating rates into aerosol and gas (primarily water vapor) absorption and explore some of the co-variability of heating rate profiles and their primary drivers, leading to the development of a new concept: the heating rate efficiency (HRE; the heating rate per unit aerosol extinction).
Sarah J. Doherty, Pablo E. Saide, Paquita Zuidema, Yohei Shinozuka, Gonzalo A. Ferrada, Hamish Gordon, Marc Mallet, Kerry Meyer, David Painemal, Steven G. Howell, Steffen Freitag, Amie Dobracki, James R. Podolske, Sharon P. Burton, Richard A. Ferrare, Calvin Howes, Pierre Nabat, Gregory R. Carmichael, Arlindo da Silva, Kristina Pistone, Ian Chang, Lan Gao, Robert Wood, and Jens Redemann
Atmos. Chem. Phys., 22, 1–46, https://doi.org/10.5194/acp-22-1-2022, https://doi.org/10.5194/acp-22-1-2022, 2022
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Between July and October, biomass burning smoke is advected over the southeastern Atlantic Ocean, leading to climate forcing. Model calculations of forcing by this plume vary significantly in both magnitude and sign. This paper compares aerosol and cloud properties observed during three NASA ORACLES field campaigns to the same in four models. It quantifies modeled biases in properties key to aerosol direct radiative forcing and evaluates how these biases propagate to biases in forcing.
Amie Dobracki, Paquita Zuidema, Steve Howell, Pablo Saide, Steffen Freitag, Allison C. Aiken, Sharon P. Burton, Arthur J. Sedlacek III, Jens Redemann, and Robert Wood
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2021-1081, https://doi.org/10.5194/acp-2021-1081, 2022
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The global maximum of shortwave-absorbing aerosol above cloud occurs above the southeast Atlantic, where the biomass-burning aerosol provides a distinct aerosol radiative warming of regional climate. The smoke aerosols are unusually highly absorbing of sunlight. This study seeks to understand the cause. We conclude the aerosol is already strongly absorbing at the fire emission source, but that chemical aging, through encouraging a net loss of organic aerosol, also contributes.
Ju-Mee Ryoo, Leonhard Pfister, Rei Ueyama, Paquita Zuidema, Robert Wood, Ian Chang, and Jens Redemann
Atmos. Chem. Phys., 21, 16689–16707, https://doi.org/10.5194/acp-21-16689-2021, https://doi.org/10.5194/acp-21-16689-2021, 2021
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Part 1 of the meteorological overview paper highlights the anomalous meteorological characteristics during the ORACLES deployment compared to the climatological mean at monthly timescales. The upper-level wave disturbance and the associated anomalous circulation explain the weakening of AEJ-S through the reduction of the strength of the heat low over the land during August 2017. This may also help explain the anomalously low aerosol optical depth observed in the August 2017 ORACLES deployment.
Raphaela Vogel, Heike Konow, Hauke Schulz, and Paquita Zuidema
Atmos. Chem. Phys., 21, 16609–16630, https://doi.org/10.5194/acp-21-16609-2021, https://doi.org/10.5194/acp-21-16609-2021, 2021
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The shallow cumulus clouds that populate the trade-wind regions can produce substantial amounts of rain. Before reaching the surface, part of the rain can evaporate and form pools of cold air that spread at the surface as density currents. We use 10 years of data from Barbados to show that such cold pools occur on 3 out of 4 d, that cold-pool periods are 90 % cloudier relative to the average winter conditions, and that they are connected to specific patterns of mesoscale cloud organization.
Geet George, Bjorn Stevens, Sandrine Bony, Robert Pincus, Chris Fairall, Hauke Schulz, Tobias Kölling, Quinn T. Kalen, Marcus Klingebiel, Heike Konow, Ashley Lundry, Marc Prange, and Jule Radtke
Earth Syst. Sci. Data, 13, 5253–5272, https://doi.org/10.5194/essd-13-5253-2021, https://doi.org/10.5194/essd-13-5253-2021, 2021
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Dropsondes measure atmospheric parameters such as temperature, pressure, humidity and horizontal winds. The EUREC4A field campaign deployed 1215 dropsondes during January–February 2020 in the north Atlantic trade-wind region in order to characterize the thermodynamic and the dynamic structure of the atmosphere, primarily at horizontal scales of ~ 200 km. We present JOANNE, the dataset that provides these dropsonde measurements and thereby a rich characterization of the trade-wind atmosphere.
Zixia Liu, Martin Osborne, Karen Anderson, Jamie D. Shutler, Andy Wilson, Justin Langridge, Steve H. L. Yim, Hugh Coe, Suresh Babu, Sreedharan K. Satheesh, Paquita Zuidema, Tao Huang, Jack C. H. Cheng, and James Haywood
Atmos. Meas. Tech., 14, 6101–6118, https://doi.org/10.5194/amt-14-6101-2021, https://doi.org/10.5194/amt-14-6101-2021, 2021
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This paper first validates the performance of an advanced aerosol observation instrument POPS against a reference instrument and examines any biases introduced by operating it on a quadcopter drone. The results show the POPS performs relatively well on the ground. The impact of the UAV rotors on the POPS is small at low wind speeds, but when operating under higher wind speeds, larger discrepancies occur. It appears that the POPS measures sub-micron aerosol particles more accurately on the UAV.
Bjorn Stevens, Sandrine Bony, David Farrell, Felix Ament, Alan Blyth, Christopher Fairall, Johannes Karstensen, Patricia K. Quinn, Sabrina Speich, Claudia Acquistapace, Franziska Aemisegger, Anna Lea Albright, Hugo Bellenger, Eberhard Bodenschatz, Kathy-Ann Caesar, Rebecca Chewitt-Lucas, Gijs de Boer, Julien Delanoë, Leif Denby, Florian Ewald, Benjamin Fildier, Marvin Forde, Geet George, Silke Gross, Martin Hagen, Andrea Hausold, Karen J. Heywood, Lutz Hirsch, Marek Jacob, Friedhelm Jansen, Stefan Kinne, Daniel Klocke, Tobias Kölling, Heike Konow, Marie Lothon, Wiebke Mohr, Ann Kristin Naumann, Louise Nuijens, Léa Olivier, Robert Pincus, Mira Pöhlker, Gilles Reverdin, Gregory Roberts, Sabrina Schnitt, Hauke Schulz, A. Pier Siebesma, Claudia Christine Stephan, Peter Sullivan, Ludovic Touzé-Peiffer, Jessica Vial, Raphaela Vogel, Paquita Zuidema, Nicola Alexander, Lyndon Alves, Sophian Arixi, Hamish Asmath, Gholamhossein Bagheri, Katharina Baier, Adriana Bailey, Dariusz Baranowski, Alexandre Baron, Sébastien Barrau, Paul A. Barrett, Frédéric Batier, Andreas Behrendt, Arne Bendinger, Florent Beucher, Sebastien Bigorre, Edmund Blades, Peter Blossey, Olivier Bock, Steven Böing, Pierre Bosser, Denis Bourras, Pascale Bouruet-Aubertot, Keith Bower, Pierre Branellec, Hubert Branger, Michal Brennek, Alan Brewer, Pierre-Etienne Brilouet, Björn Brügmann, Stefan A. Buehler, Elmo Burke, Ralph Burton, Radiance Calmer, Jean-Christophe Canonici, Xavier Carton, Gregory Cato Jr., Jude Andre Charles, Patrick Chazette, Yanxu Chen, Michal T. Chilinski, Thomas Choularton, Patrick Chuang, Shamal Clarke, Hugh Coe, Céline Cornet, Pierre Coutris, Fleur Couvreux, Susanne Crewell, Timothy Cronin, Zhiqiang Cui, Yannis Cuypers, Alton Daley, Gillian M. Damerell, Thibaut Dauhut, Hartwig Deneke, Jean-Philippe Desbios, Steffen Dörner, Sebastian Donner, Vincent Douet, Kyla Drushka, Marina Dütsch, André Ehrlich, Kerry Emanuel, Alexandros Emmanouilidis, Jean-Claude Etienne, Sheryl Etienne-Leblanc, Ghislain Faure, Graham Feingold, Luca Ferrero, Andreas Fix, Cyrille Flamant, Piotr Jacek Flatau, Gregory R. Foltz, Linda Forster, Iulian Furtuna, Alan Gadian, Joseph Galewsky, Martin Gallagher, Peter Gallimore, Cassandra Gaston, Chelle Gentemann, Nicolas Geyskens, Andreas Giez, John Gollop, Isabelle Gouirand, Christophe Gourbeyre, Dörte de Graaf, Geiske E. de Groot, Robert Grosz, Johannes Güttler, Manuel Gutleben, Kashawn Hall, George Harris, Kevin C. Helfer, Dean Henze, Calvert Herbert, Bruna Holanda, Antonio Ibanez-Landeta, Janet Intrieri, Suneil Iyer, Fabrice Julien, Heike Kalesse, Jan Kazil, Alexander Kellman, Abiel T. Kidane, Ulrike Kirchner, Marcus Klingebiel, Mareike Körner, Leslie Ann Kremper, Jan Kretzschmar, Ovid Krüger, Wojciech Kumala, Armin Kurz, Pierre L'Hégaret, Matthieu Labaste, Tom Lachlan-Cope, Arlene Laing, Peter Landschützer, Theresa Lang, Diego Lange, Ingo Lange, Clément Laplace, Gauke Lavik, Rémi Laxenaire, Caroline Le Bihan, Mason Leandro, Nathalie Lefevre, Marius Lena, Donald Lenschow, Qiang Li, Gary Lloyd, Sebastian Los, Niccolò Losi, Oscar Lovell, Christopher Luneau, Przemyslaw Makuch, Szymon Malinowski, Gaston Manta, Eleni Marinou, Nicholas Marsden, Sebastien Masson, Nicolas Maury, Bernhard Mayer, Margarette Mayers-Als, Christophe Mazel, Wayne McGeary, James C. McWilliams, Mario Mech, Melina Mehlmann, Agostino Niyonkuru Meroni, Theresa Mieslinger, Andreas Minikin, Peter Minnett, Gregor Möller, Yanmichel Morfa Avalos, Caroline Muller, Ionela Musat, Anna Napoli, Almuth Neuberger, Christophe Noisel, David Noone, Freja Nordsiek, Jakub L. Nowak, Lothar Oswald, Douglas J. Parker, Carolyn Peck, Renaud Person, Miriam Philippi, Albert Plueddemann, Christopher Pöhlker, Veronika Pörtge, Ulrich Pöschl, Lawrence Pologne, Michał Posyniak, Marc Prange, Estefanía Quiñones Meléndez, Jule Radtke, Karim Ramage, Jens Reimann, Lionel Renault, Klaus Reus, Ashford Reyes, Joachim Ribbe, Maximilian Ringel, Markus Ritschel, Cesar B. Rocha, Nicolas Rochetin, Johannes Röttenbacher, Callum Rollo, Haley Royer, Pauline Sadoulet, Leo Saffin, Sanola Sandiford, Irina Sandu, Michael Schäfer, Vera Schemann, Imke Schirmacher, Oliver Schlenczek, Jerome Schmidt, Marcel Schröder, Alfons Schwarzenboeck, Andrea Sealy, Christoph J. Senff, Ilya Serikov, Samkeyat Shohan, Elizabeth Siddle, Alexander Smirnov, Florian Späth, Branden Spooner, M. Katharina Stolla, Wojciech Szkółka, Simon P. de Szoeke, Stéphane Tarot, Eleni Tetoni, Elizabeth Thompson, Jim Thomson, Lorenzo Tomassini, Julien Totems, Alma Anna Ubele, Leonie Villiger, Jan von Arx, Thomas Wagner, Andi Walther, Ben Webber, Manfred Wendisch, Shanice Whitehall, Anton Wiltshire, Allison A. Wing, Martin Wirth, Jonathan Wiskandt, Kevin Wolf, Ludwig Worbes, Ethan Wright, Volker Wulfmeyer, Shanea Young, Chidong Zhang, Dongxiao Zhang, Florian Ziemen, Tobias Zinner, and Martin Zöger
Earth Syst. Sci. Data, 13, 4067–4119, https://doi.org/10.5194/essd-13-4067-2021, https://doi.org/10.5194/essd-13-4067-2021, 2021
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The EUREC4A field campaign, designed to test hypothesized mechanisms by which clouds respond to warming and benchmark next-generation Earth-system models, is presented. EUREC4A comprised roughly 5 weeks of measurements in the downstream winter trades of the North Atlantic – eastward and southeastward of Barbados. It was the first campaign that attempted to characterize the full range of processes and scales influencing trade wind clouds.
Jianhao Zhang and Paquita Zuidema
Atmos. Chem. Phys., 21, 11179–11199, https://doi.org/10.5194/acp-21-11179-2021, https://doi.org/10.5194/acp-21-11179-2021, 2021
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The subtropical Atlantic hosts one of the planet's largest marine low cloud decks and interacts with biomass burning aerosol from approximately July through October. This study clarifies how the monthly evolution in meteorology and the biomass burning aerosol vertical structure affects the seasonal cycle in its low cloud fraction, such that the July–October evolution in low cloud cover and morphology are reinforced, when compared to scenarios with less aerosol present.
Hossein Dadashazar, David Painemal, Majid Alipanah, Michael Brunke, Seethala Chellappan, Andrea F. Corral, Ewan Crosbie, Simon Kirschler, Hongyu Liu, Richard H. Moore, Claire Robinson, Amy Jo Scarino, Michael Shook, Kenneth Sinclair, K. Lee Thornhill, Christiane Voigt, Hailong Wang, Edward Winstead, Xubin Zeng, Luke Ziemba, Paquita Zuidema, and Armin Sorooshian
Atmos. Chem. Phys., 21, 10499–10526, https://doi.org/10.5194/acp-21-10499-2021, https://doi.org/10.5194/acp-21-10499-2021, 2021
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This study investigates the seasonal cycle of cloud drop number concentration (Nd) over the western North Atlantic Ocean (WNAO) using multiple datasets. Reasons for the puzzling discrepancy between the seasonal cycles of Nd and aerosol concentration were identified. Results indicate that Nd is highest in winter (when aerosol proxy values are often lowest) due to conditions both linked to cold-air outbreaks and that promote greater droplet activation.
Kristina Pistone, Paquita Zuidema, Robert Wood, Michael Diamond, Arlindo M. da Silva, Gonzalo Ferrada, Pablo E. Saide, Rei Ueyama, Ju-Mee Ryoo, Leonhard Pfister, James Podolske, David Noone, Ryan Bennett, Eric Stith, Gregory Carmichael, Jens Redemann, Connor Flynn, Samuel LeBlanc, Michal Segal-Rozenhaimer, and Yohei Shinozuka
Atmos. Chem. Phys., 21, 9643–9668, https://doi.org/10.5194/acp-21-9643-2021, https://doi.org/10.5194/acp-21-9643-2021, 2021
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Using aircraft-based measurements off the Atlantic coast of Africa, we found the springtime smoke plume was strongly correlated with the amount of water vapor in the atmosphere (more smoke indicated more humidity). We see the same general feature in satellite-assimilated and free-running models. Our analysis suggests this relationship is not caused by the burning but originates due to coincident continental meteorology plus fires. This air is transported over the ocean without further mixing.
David Brus, Jani Gustafsson, Osku Kemppinen, Gijs de Boer, and Anne Hirsikko
Earth Syst. Sci. Data, 13, 2909–2922, https://doi.org/10.5194/essd-13-2909-2021, https://doi.org/10.5194/essd-13-2909-2021, 2021
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This publication summarizes measurements collected and datasets generated by the Finnish Meteorological Institute and Kansas State University teams during the LAPSE-RATE campaign that took place in San Luis Valley, Colorado, during summer 2018. We provide an overview of the rotorcraft and offer insights into the payloads that were used. We describe the teams’ scientific goals, flight strategies, and the datasets, including a description of the measurement validation techniques applied.
Christina J. Williamson, Agnieszka Kupc, Andrew Rollins, Jan Kazil, Karl D. Froyd, Eric A. Ray, Daniel M. Murphy, Gregory P. Schill, Jeff Peischl, Chelsea Thompson, Ilann Bourgeois, Thomas B. Ryerson, Glenn S. Diskin, Joshua P. DiGangi, Donald R. Blake, Thao Paul V. Bui, Maximilian Dollner, Bernadett Weinzierl, and Charles A. Brock
Atmos. Chem. Phys., 21, 9065–9088, https://doi.org/10.5194/acp-21-9065-2021, https://doi.org/10.5194/acp-21-9065-2021, 2021
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Aerosols in the stratosphere influence climate by scattering and absorbing sunlight and through chemical reactions occurring on the particles’ surfaces. We observed more nucleation mode aerosols (small aerosols, with diameters below 12 nm) in the mid- and high-latitude lowermost stratosphere (8–13 km) in the Northern Hemisphere (NH) than in the Southern Hemisphere. The most likely cause of this is aircraft emissions, which are concentrated in the NH at similar altitudes to our observations.
Gijs de Boer, Cory Dixon, Steven Borenstein, Dale A. Lawrence, Jack Elston, Daniel Hesselius, Maciej Stachura, Roger Laurence III, Sara Swenson, Christopher M. Choate, Abhiram Doddi, Aiden Sesnic, Katherine Glasheen, Zakariya Laouar, Flora Quinby, Eric Frew, and Brian M. Argrow
Earth Syst. Sci. Data, 13, 2515–2528, https://doi.org/10.5194/essd-13-2515-2021, https://doi.org/10.5194/essd-13-2515-2021, 2021
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This paper describes data collected by uncrewed aircraft operated by the University of Colorado Boulder and Black Swift Technologies during the Lower Atmospheric Profiling Studies at Elevation – A Remotely-piloted Aircraft Team Experiment (LAPSE-RATE) field campaign. This effort was conducted in the San Luis Valley of Colorado in July 2018 and included intensive observing of the atmospheric boundary layer. This paper describes data collected by four aircraft operated by these entities.
Patricia K. Quinn, Elizabeth J. Thompson, Derek J. Coffman, Sunil Baidar, Ludovic Bariteau, Timothy S. Bates, Sebastien Bigorre, Alan Brewer, Gijs de Boer, Simon P. de Szoeke, Kyla Drushka, Gregory R. Foltz, Janet Intrieri, Suneil Iyer, Chris W. Fairall, Cassandra J. Gaston, Friedhelm Jansen, James E. Johnson, Ovid O. Krüger, Richard D. Marchbanks, Kenneth P. Moran, David Noone, Sergio Pezoa, Robert Pincus, Albert J. Plueddemann, Mira L. Pöhlker, Ulrich Pöschl, Estefania Quinones Melendez, Haley M. Royer, Malgorzata Szczodrak, Jim Thomson, Lucia M. Upchurch, Chidong Zhang, Dongxiao Zhang, and Paquita Zuidema
Earth Syst. Sci. Data, 13, 1759–1790, https://doi.org/10.5194/essd-13-1759-2021, https://doi.org/10.5194/essd-13-1759-2021, 2021
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ATOMIC took place in the northwestern tropical Atlantic during January and February of 2020 to gather information on shallow atmospheric convection, the effects of aerosols and clouds on the ocean surface energy budget, and mesoscale oceanic processes. Measurements made from the NOAA RV Ronald H. Brown and assets it deployed (instrumented mooring and uncrewed seagoing vehicles) are described herein to advance widespread use of the data by the ATOMIC and broader research communities.
Anna Lea Albright, Benjamin Fildier, Ludovic Touzé-Peiffer, Robert Pincus, Jessica Vial, and Caroline Muller
Earth Syst. Sci. Data, 13, 617–630, https://doi.org/10.5194/essd-13-617-2021, https://doi.org/10.5194/essd-13-617-2021, 2021
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A number of climate mysteries are rooted in uncertainties in how clouds respond to their environment in the trades, the global belt of easterly winds. Differences in radiative heating play a role in the couplings between clouds and their environment. We calculate radiative profiles from 2580 dropsondes and radiosondes from the EUREC4A field campaign (downstream Atlantic trades, winter 2020). We describe the method, assess uncertainty, and discuss radiative heating variability on multiple scales.
Jessie M. Creamean, Gijs de Boer, Hagen Telg, Fan Mei, Darielle Dexheimer, Matthew D. Shupe, Amy Solomon, and Allison McComiskey
Atmos. Chem. Phys., 21, 1737–1757, https://doi.org/10.5194/acp-21-1737-2021, https://doi.org/10.5194/acp-21-1737-2021, 2021
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Arctic clouds play a role in modulating sea ice extent. Importantly, aerosols facilitate cloud formation, and thus it is crucial to understand the interactions between aerosols and clouds. Vertical measurements of aerosols and clouds are needed to tackle this issue. We present results from balloon-borne measurements of aerosols and clouds over the course of 2 years in northern Alaska. These data shed light onto the vertical distributions of aerosols relative to clouds spanning multiple seasons.
Jens Redemann, Robert Wood, Paquita Zuidema, Sarah J. Doherty, Bernadette Luna, Samuel E. LeBlanc, Michael S. Diamond, Yohei Shinozuka, Ian Y. Chang, Rei Ueyama, Leonhard Pfister, Ju-Mee Ryoo, Amie N. Dobracki, Arlindo M. da Silva, Karla M. Longo, Meloë S. Kacenelenbogen, Connor J. Flynn, Kristina Pistone, Nichola M. Knox, Stuart J. Piketh, James M. Haywood, Paola Formenti, Marc Mallet, Philip Stier, Andrew S. Ackerman, Susanne E. Bauer, Ann M. Fridlind, Gregory R. Carmichael, Pablo E. Saide, Gonzalo A. Ferrada, Steven G. Howell, Steffen Freitag, Brian Cairns, Brent N. Holben, Kirk D. Knobelspiesse, Simone Tanelli, Tristan S. L'Ecuyer, Andrew M. Dzambo, Ousmane O. Sy, Greg M. McFarquhar, Michael R. Poellot, Siddhant Gupta, Joseph R. O'Brien, Athanasios Nenes, Mary Kacarab, Jenny P. S. Wong, Jennifer D. Small-Griswold, Kenneth L. Thornhill, David Noone, James R. Podolske, K. Sebastian Schmidt, Peter Pilewskie, Hong Chen, Sabrina P. Cochrane, Arthur J. Sedlacek, Timothy J. Lang, Eric Stith, Michal Segal-Rozenhaimer, Richard A. Ferrare, Sharon P. Burton, Chris A. Hostetler, David J. Diner, Felix C. Seidel, Steven E. Platnick, Jeffrey S. Myers, Kerry G. Meyer, Douglas A. Spangenberg, Hal Maring, and Lan Gao
Atmos. Chem. Phys., 21, 1507–1563, https://doi.org/10.5194/acp-21-1507-2021, https://doi.org/10.5194/acp-21-1507-2021, 2021
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Southern Africa produces significant biomass burning emissions whose impacts on regional and global climate are poorly understood. ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) is a 5-year NASA investigation designed to study the key processes that determine these climate impacts. The main purpose of this paper is to familiarize the broader scientific community with the ORACLES project, the dataset it produced, and the most important initial findings.
Gijs de Boer, Sean Waugh, Alexander Erwin, Steven Borenstein, Cory Dixon, Wafa'a Shanti, Adam Houston, and Brian Argrow
Earth Syst. Sci. Data, 13, 155–169, https://doi.org/10.5194/essd-13-155-2021, https://doi.org/10.5194/essd-13-155-2021, 2021
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This paper provides an overview of measurements collected in south-central Colorado (USA) during the 2018 LAPSE-RATE campaign. The measurements described in this article were collected by mobile surface vehicles, including cars, trucks, and vans, and include measurements of thermodynamic quantities (e.g., temperature, humidity, pressure) and winds. These measurements can be used to study the evolution of the atmospheric boundary layer at a high-elevation site under a variety of conditions.
Sabrina P. Cochrane, K. Sebastian Schmidt, Hong Chen, Peter Pilewskie, Scott Kittelman, Jens Redemann, Samuel LeBlanc, Kristina Pistone, Meloë Kacenelenbogen, Michal Segal Rozenhaimer, Yohei Shinozuka, Connor Flynn, Amie Dobracki, Paquita Zuidema, Steven Howell, Steffen Freitag, and Sarah Doherty
Atmos. Meas. Tech., 14, 567–593, https://doi.org/10.5194/amt-14-567-2021, https://doi.org/10.5194/amt-14-567-2021, 2021
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Based on observations from the 2016 and 2017 field campaigns of ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS), this work establishes an observationally driven link from mid-visible aerosol optical depth (AOD) and other scene parameters to broadband shortwave irradiance (and by extension the direct aerosol radiative effect, DARE). The majority of the case-to-case DARE variability within the ORACLES dataset is attributable to the dependence on AOD and scene albedo.
Jim M. Haywood, Steven J. Abel, Paul A. Barrett, Nicolas Bellouin, Alan Blyth, Keith N. Bower, Melissa Brooks, Ken Carslaw, Haochi Che, Hugh Coe, Michael I. Cotterell, Ian Crawford, Zhiqiang Cui, Nicholas Davies, Beth Dingley, Paul Field, Paola Formenti, Hamish Gordon, Martin de Graaf, Ross Herbert, Ben Johnson, Anthony C. Jones, Justin M. Langridge, Florent Malavelle, Daniel G. Partridge, Fanny Peers, Jens Redemann, Philip Stier, Kate Szpek, Jonathan W. Taylor, Duncan Watson-Parris, Robert Wood, Huihui Wu, and Paquita Zuidema
Atmos. Chem. Phys., 21, 1049–1084, https://doi.org/10.5194/acp-21-1049-2021, https://doi.org/10.5194/acp-21-1049-2021, 2021
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Every year, the seasonal cycle of biomass burning from agricultural practices in Africa creates a huge plume of smoke that travels many thousands of kilometres over the Atlantic Ocean. This study provides an overview of a measurement campaign called the cloud–aerosol–radiation interaction and forcing for year 2017 (CLARIFY-2017) and documents the rationale, deployment strategy, observations, and key results from the campaign which utilized the heavily equipped FAAM atmospheric research aircraft.
Yingzhao Ma, Xun Sun, Haonan Chen, Yang Hong, and Yinsheng Zhang
Hydrol. Earth Syst. Sci., 25, 359–374, https://doi.org/10.5194/hess-25-359-2021, https://doi.org/10.5194/hess-25-359-2021, 2021
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A two-stage blending approach is proposed for the data fusion of multiple satellite precipitation estimates (SPEs), which firstly reduces the systematic errors of original SPEs based on a Bayesian correction model and then merges the bias-corrected SPEs with a Bayesian weighting model. The model is evaluated in the warm season of 2010–2014 in the northeastern Tibetan Plateau. Results show that the blended SPE is greatly improved compared with the original SPEs, even in heavy rainfall events.
David Brus, Jani Gustafsson, Ville Vakkari, Osku Kemppinen, Gijs de Boer, and Anne Hirsikko
Atmos. Chem. Phys., 21, 517–533, https://doi.org/10.5194/acp-21-517-2021, https://doi.org/10.5194/acp-21-517-2021, 2021
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This paper summarizes Finnish Meteorological Institute and Kansas State University unmanned aerial vehicle measurements during the summer 2018 Lower Atmospheric Process Studies at Elevation – a Remotely-piloted Aircraft Team Experiment (LAPSE-RATE) campaign in the San Luis Valley, providing an overview of the rotorcraft deployed, payloads, scientific goals and flight strategies and presenting observations of atmospheric thermodynamics and aerosol and gas parameters in the vertical column.
Robert Jackson, Scott Collis, Valentin Louf, Alain Protat, Die Wang, Scott Giangrande, Elizabeth J. Thompson, Brenda Dolan, and Scott W. Powell
Atmos. Meas. Tech., 14, 53–69, https://doi.org/10.5194/amt-14-53-2021, https://doi.org/10.5194/amt-14-53-2021, 2021
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About 4 years of 2D video disdrometer data in Darwin are used to develop and validate rainfall retrievals for tropical convection in C- and X-band radars in Darwin. Using blended techniques previously used for Colorado and Manus and Gan islands, with modified coefficients in each estimator, provided the most optimal results. Using multiple radar observables to develop a rainfall retrieval provided a greater advantage than using a single observable, including using specific attenuation.
Gijs de Boer, Adam Houston, Jamey Jacob, Phillip B. Chilson, Suzanne W. Smith, Brian Argrow, Dale Lawrence, Jack Elston, David Brus, Osku Kemppinen, Petra Klein, Julie K. Lundquist, Sean Waugh, Sean C. C. Bailey, Amy Frazier, Michael P. Sama, Christopher Crick, David Schmale III, James Pinto, Elizabeth A. Pillar-Little, Victoria Natalie, and Anders Jensen
Earth Syst. Sci. Data, 12, 3357–3366, https://doi.org/10.5194/essd-12-3357-2020, https://doi.org/10.5194/essd-12-3357-2020, 2020
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This paper provides an overview of the Lower Atmospheric Profiling Studies at Elevation – a Remotely-piloted Aircraft Team Experiment (LAPSE-RATE) field campaign, held from 14 to 20 July 2018. This field campaign spanned a 1-week deployment to Colorado's San Luis Valley, involving over 100 students, scientists, engineers, pilots, and outreach coordinators. This overview paper provides insight into the campaign for a special issue focused on the datasets collected during LAPSE-RATE.
Johannes Quaas, Antti Arola, Brian Cairns, Matthew Christensen, Hartwig Deneke, Annica M. L. Ekman, Graham Feingold, Ann Fridlind, Edward Gryspeerdt, Otto Hasekamp, Zhanqing Li, Antti Lipponen, Po-Lun Ma, Johannes Mülmenstädt, Athanasios Nenes, Joyce E. Penner, Daniel Rosenfeld, Roland Schrödner, Kenneth Sinclair, Odran Sourdeval, Philip Stier, Matthias Tesche, Bastiaan van Diedenhoven, and Manfred Wendisch
Atmos. Chem. Phys., 20, 15079–15099, https://doi.org/10.5194/acp-20-15079-2020, https://doi.org/10.5194/acp-20-15079-2020, 2020
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Anthropogenic pollution particles – aerosols – serve as cloud condensation nuclei and thus increase cloud droplet concentration and the clouds' reflection of sunlight (a cooling effect on climate). This Twomey effect is poorly constrained by models and requires satellite data for better quantification. The review summarizes the challenges in properly doing so and outlines avenues for progress towards a better use of aerosol retrievals and better retrievals of droplet concentrations.
Agnieszka Kupc, Christina J. Williamson, Anna L. Hodshire, Jan Kazil, Eric Ray, T. Paul Bui, Maximilian Dollner, Karl D. Froyd, Kathryn McKain, Andrew Rollins, Gregory P. Schill, Alexander Thames, Bernadett B. Weinzierl, Jeffrey R. Pierce, and Charles A. Brock
Atmos. Chem. Phys., 20, 15037–15060, https://doi.org/10.5194/acp-20-15037-2020, https://doi.org/10.5194/acp-20-15037-2020, 2020
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Tropical upper troposphere over the Atlantic and Pacific oceans is a major source region of new particles. These particles are associated with the outflow from deep convection. We investigate the processes that govern the formation of these particles and their initial growth and show that none of the formation schemes commonly used in global models are consistent with observations. Using newer schemes indicates that organic compounds are likely important as nucleating and initial growth agents.
Marc Mallet, Fabien Solmon, Pierre Nabat, Nellie Elguindi, Fabien Waquet, Dominique Bouniol, Andrew Mark Sayer, Kerry Meyer, Romain Roehrig, Martine Michou, Paquita Zuidema, Cyrille Flamant, Jens Redemann, and Paola Formenti
Atmos. Chem. Phys., 20, 13191–13216, https://doi.org/10.5194/acp-20-13191-2020, https://doi.org/10.5194/acp-20-13191-2020, 2020
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This paper presents numerical simulations using two regional climate models to study the impact of biomass fire plumes from central Africa on the radiative balance of this region. The results indicate that biomass fires can either warm the regional climate when they are located above low clouds or cool it when they are located above land. They can also alter sea and land surface temperatures by decreasing solar radiation at the surface. Finally, they can also modify the atmospheric dynamics.
Yohei Shinozuka, Pablo E. Saide, Gonzalo A. Ferrada, Sharon P. Burton, Richard Ferrare, Sarah J. Doherty, Hamish Gordon, Karla Longo, Marc Mallet, Yan Feng, Qiaoqiao Wang, Yafang Cheng, Amie Dobracki, Steffen Freitag, Steven G. Howell, Samuel LeBlanc, Connor Flynn, Michal Segal-Rosenhaimer, Kristina Pistone, James R. Podolske, Eric J. Stith, Joseph Ryan Bennett, Gregory R. Carmichael, Arlindo da Silva, Ravi Govindaraju, Ruby Leung, Yang Zhang, Leonhard Pfister, Ju-Mee Ryoo, Jens Redemann, Robert Wood, and Paquita Zuidema
Atmos. Chem. Phys., 20, 11491–11526, https://doi.org/10.5194/acp-20-11491-2020, https://doi.org/10.5194/acp-20-11491-2020, 2020
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In the southeast Atlantic, well-defined smoke plumes from Africa advect over marine boundary layer cloud decks; both are most extensive around September, when most of the smoke resides in the free troposphere. A framework is put forth for evaluating the performance of a range of global and regional atmospheric composition models against observations made during the NASA ORACLES (ObseRvations of Aerosols above CLouds and their intEractionS) airborne mission in September 2016.
Yohei Shinozuka, Meloë S. Kacenelenbogen, Sharon P. Burton, Steven G. Howell, Paquita Zuidema, Richard A. Ferrare, Samuel E. LeBlanc, Kristina Pistone, Stephen Broccardo, Jens Redemann, K. Sebastian Schmidt, Sabrina P. Cochrane, Marta Fenn, Steffen Freitag, Amie Dobracki, Michal Segal-Rosenheimer, and Connor J. Flynn
Atmos. Chem. Phys., 20, 11275–11285, https://doi.org/10.5194/acp-20-11275-2020, https://doi.org/10.5194/acp-20-11275-2020, 2020
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To help satellite retrieval of aerosols and studies of their radiative effects, we demonstrate that daytime aerosol optical depth over low-level clouds is similar to that in neighboring clear skies at the same heights. Based on recent airborne lidar and sun photometer observations above the southeast Atlantic, the mean AOD difference at 532 nm is between 0 and -0.01, when comparing the cloudy and clear sides of cloud edges, with each up to 20 km wide.
Adeyemi A. Adebiyi, Paquita Zuidema, Ian Chang, Sharon P. Burton, and Brian Cairns
Atmos. Chem. Phys., 20, 11025–11043, https://doi.org/10.5194/acp-20-11025-2020, https://doi.org/10.5194/acp-20-11025-2020, 2020
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Over the southeast Atlantic, interactions between the low-level clouds and the overlying smoke aerosols have previously been highlighted, but no study has yet focused on the presence of the mid-level clouds that complicate the aerosol–cloud interactions. Here we show that these optically thin super-cooled mid-level clouds are relatively common, and they frequently occur at the top of the smoke layer between August and October with significant radiative impacts on the low-level clouds.
Samantha J. Kramer, Claudia Alvarez, Anne E. Barkley, Peter R. Colarco, Lillian Custals, Rodrigo Delgadillo, Cassandra J. Gaston, Ravi Govindaraju, and Paquita Zuidema
Atmos. Chem. Phys., 20, 10047–10062, https://doi.org/10.5194/acp-20-10047-2020, https://doi.org/10.5194/acp-20-10047-2020, 2020
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Comparisons of sea salt and size-resolved dust mass concentration measurements over southeast Florida to those from the MERRA-2/GEOS-5 FP aerosol reanalysis show the reanalysis depicts excessive sea salt and puts too much dust in larger intermediate sizes than do the measurements. The vertical distribution of the dust mass is approximately correct. The incorrect reanalysis aerosol speciation and dust sizes have implications for the modeling of their transport, deposition, and radiative impact.
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Li, L., Heymsfield, G. M., Tian, L., and Racette, P. E.: Measurements of Ocean Surface Backscattering Using an Airborne 94-GHz Cloud Radar – Implication for Calibration of Airborne and Spaceborne W-Band Radars, J. Atmos. Ocean. Tech., 22, 1033–1045, https://doi.org/10.1175/JTECH1722.1, 2005. a
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NOAA Aircraft Operations Center and NOAA Physical Sciences Laboratory:
ATOMIC Aircraft Flight Level Navigation Meteorology: Wind Speed, Relative Humidity, Aircraft Parameters, and Other Measurements Taken from N43 Aircraft in the North Atlantic Ocean, Barbados: Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign 2020-01-17 to 2020-02-11 (NCEI Accession 0220621), NOAA National Centers for Environmental Information [data set], https://doi.org/10.25921/7jf5-wv54, 2020. a, b
NOAA Physical Sciences Laboratory: ATOMIC aircraft AXBT: Subsurface ocean temperature measurements from Airborne eXpendable BathyThermographs (AXBT) deployed from N43 aircraft, Barbados: Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign 2020-01-19 to 2020-02-11 (NCEI Accession 0220436), NOAA National Centers for Environmental Information [data set], https://doi.org/10.25921/pe39-sx75, 2020a. a, b
NOAA Physical Sciences Laboratory: ATOMIC aircraft remote sensing cloud, rain, wind, wave: Cloud and precipitation parameters and 10-meter wind speed estimated from remote sensing instruments aboard N43 aircraft in the North Atlantic Ocean, Barbados: Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign 2020-01-17 to 2020-02-11 (NCEI Accession 0220625), NOAA National Centers for Environmental Information [data set], https://doi.org/10.25921/x9q5-9745, 2020b. a, b
NOAA Physical Sciences Laboratory: ATOMIC aircraft W-band radar: Reflectivity, Doppler velocity, and spectral width taken from W-band radar abouard N43 aircraft in the North Atlantic Ocean, Barbados: Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign 2020-01-17 to 2020-02-11 (NCEI Accession 0220624), NOAA National Centers for Environmental Information [data set], https://doi.org/10.25921/n1hc-dc30, 2020c. a, b
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Quinn, P. K., Thompson, E. J., Coffman, D. J., Baidar, S., Bariteau, L., Bates, T. S., Bigorre, S., Brewer, A., de Boer, G., de Szoeke, S. P., Drushka, K., Foltz, G. R., Intrieri, J., Iyer, S., Fairall, C. W., Gaston, C. J., Jansen, F., Johnson, J. E., Krüger, O. O., Marchbanks, R. D., Moran, K. P., Noone, D., Pezoa, S., Pincus, R., Plueddemann, A. J., Pöhlker, M. L., Pöschl, U., Quinones Melendez, E., Royer, H. M., Szczodrak, M., Thomson, J., Upchurch, L. M., Zhang, C., Zhang, D., and Zuidema, P.: Measurements from the RV Ronald H. Brown and related platforms as part of the Atlantic Tradewind Ocean-Atmosphere Mesoscale Interaction Campaign (ATOMIC), Earth Syst. Sci. Data, 13, 1759–1790, https://doi.org/10.5194/essd-13-1759-2021, 2021. a, b, c, d, e, f, g, h
Sapp, J., Alsweiss, S., Jelenak, Z., Chang, P., and Carswell, J.: Stepped Frequency Microwave Radiometer Wind-Speed Retrieval Improvements, Remote Sens., 11, 214, https://doi.org/10.3390/rs11030214, 2019. a
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Short summary
This paper describes observations taken from a research aircraft during a field experiment in the western Atlantic Ocean during January and February 2020. The plane made 11 flights, most 8-9 h long, and measured the properties of the atmosphere and ocean with a combination of direct measurements, sensors falling from the plane to profile the atmosphere and ocean, and remote sensing measurements of clouds and the ocean surface.
This paper describes observations taken from a research aircraft during a field experiment in...
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