Articles | Volume 14, issue 7
https://doi.org/10.5194/essd-14-3197-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/essd-14-3197-2022
© Author(s) 2022. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Reconstructing 6-hourly PM2.5 datasets from 1960 to 2020 in China
Junting Zhong
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Xiaoye Zhang
CORRESPONDING AUTHOR
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Center for Excellence in Regional Atmospheric Environment, IUE,
Chinese Academy of Sciences, Xiamen 361021, China
Ke Gui
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Jie Liao
National Meteorological Information Center, Beijing 100081, China
Ye Fei
National Meteorological Information Center, Beijing 100081, China
Lipeng Jiang
Earth System Numerical Prediction Center, Beijing 100081, China
Lifeng Guo
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Liangke Liu
Department of Earth System Science, Tsinghua University, Beijing
100084, China
Huizheng Che
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Yaqiang Wang
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Deying Wang
State Key Laboratory of Severe Weather & Key Laboratory of
Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences,
Beijing 100081, China
Zijiang Zhou
National Meteorological Information Center, Beijing 100081, China
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By combining long-term observational data analyses, synoptic classifications, and meteorology–chemistry coupled simulations, the complicated impacts of large-scale synoptic forcing and local boundary layer processes on the aerosol pollution in the Beijing–Tianjin–Hebei region have been investigated. The influences of the aerosol radiative effect on boundary layer structure and pollution were also examined. This study has important implications for better understanding pollution in China.
Zhe Jiang, Minzheng Duan, Huizheng Che, Wenxing Zhang, Teruyuki Nakajima, Makiko Hashimoto, Bin Chen, and Akihiro Yamazaki
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This study analyzed the aerosol optical properties derived by SKYRAD.pack versions 5.0 and 4.2 using the radiometer measurements over Qionghai and Yucheng in China, which are two new sites of SKYNET. The seasonal variability of the aerosol properties over the two sites were investigated based on SKYRAD.pack V5.0. The validation results provide valuable references for continued improvement of the retrieval algorithms of SKYNET and other aerosol observational networks.
Linlin Liang, Guenter Engling, Chang Liu, Wanyun Xu, Xuyan Liu, Yuan Cheng, Zhenyu Du, Gen Zhang, Junying Sun, and Xiaoye Zhang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-19, https://doi.org/10.5194/acp-2020-19, 2020
Revised manuscript not accepted
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Our study captured an episode with extreme biomass burning tracer level at an agricultural site in North China, with concentrations of levoglucosan as high as 4.37 μg m−3. Based on comparison of the chemical composition between different biomass burning periods, it appeared that biomass burning can obviously elevate the levels of organic components, but seems to have no significant effect on the production of secondary inorganic ions, although their precursors increased during the episode.
Jun Zhu, Xiangao Xia, Huizheng Che, Jun Wang, Zhiyuan Cong, Tianliang Zhao, Shichang Kang, Xuelei Zhang, Xingna Yu, and Yanlin Zhang
Atmos. Chem. Phys., 19, 14637–14656, https://doi.org/10.5194/acp-19-14637-2019, https://doi.org/10.5194/acp-19-14637-2019, 2019
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The long-term temporal–spatial variations of the aerosol optical properties over the Tibetan Plateau (TP) based on the multiple ground-based sun photometer sites and the MODIS product are presented. Besides, the aerosol pollution and aerosol transport processes over the TP are also analyzed by the observations and models. The results in this region could help reduce the assessment uncertainties of aerosol radiative forcing and provide more information on aerosol transportation.
Lei Li, Oleg Dubovik, Yevgeny Derimian, Gregory L. Schuster, Tatyana Lapyonok, Pavel Litvinov, Fabrice Ducos, David Fuertes, Cheng Chen, Zhengqiang Li, Anton Lopatin, Benjamin Torres, and Huizheng Che
Atmos. Chem. Phys., 19, 13409–13443, https://doi.org/10.5194/acp-19-13409-2019, https://doi.org/10.5194/acp-19-13409-2019, 2019
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A novel methodology to monitor atmospheric aerosol components using remote sensing is presented. The concept is realized within the GRASP (Generalized Retrieval of Aerosol and Surface Properties) project. Application to POLDER/PARASOL and AERONET observations yielded the spatial and temporal variability of absorbing and non-absorbing insoluble and soluble aerosol species in the fine and coarse size fractions. This presents the global-scale aerosol component derived from satellite measurements.
Renmin Yuan, Xiaoye Zhang, Hao Liu, Yu Gui, Bohao Shao, Xiaoping Tao, Yaqiang Wang, Junting Zhong, Yubin Li, and Zhiqiu Gao
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To understand the contribution of ground emission during heavy pollution in Beijing, Tianjin and Hebei, aerosol fluxes were estimated in Beijing and Gucheng areas. The results show that in the three stages of a heavy pollution process (transport, accumulative and removal stages: TS, AS and RS), the ground emissions in the TS and RS stages are stronger, while the ground discharge in the AS stage is weak. The weakened mass flux indicates that the already weak turbulence would be further weakened.
Huizheng Che, Xiangao Xia, Hujia Zhao, Oleg Dubovik, Brent N. Holben, Philippe Goloub, Emilio Cuevas-Agulló, Victor Estelles, Yaqiang Wang, Jun Zhu, Bing Qi, Wei Gong, Honglong Yang, Renjian Zhang, Leiku Yang, Jing Chen, Hong Wang, Yu Zheng, Ke Gui, Xiaochun Zhang, and Xiaoye Zhang
Atmos. Chem. Phys., 19, 11843–11864, https://doi.org/10.5194/acp-19-11843-2019, https://doi.org/10.5194/acp-19-11843-2019, 2019
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A full-scale description of ground-based aerosol microphysical and optical properties over China is presented. Moreover, the results have also provided significant information about optical and radiative aerosol properties for different types of sites covering a broad expanse of China. The results have considerable value for ground-truthing satellite observations and validating aerosol models.
Xianyi Yang, Huizheng Che, Hitoshi Irie, Quanliang Chen, Ke Gui, Ying Cai, Yu Zheng, Linchang An, Hujia Zhao, Lei Li, Yuanxin Liang, Yaqiang Wang, Hong Wang, and Xiaoye Zhang
Atmos. Meas. Tech. Discuss., https://doi.org/10.5194/amt-2019-339, https://doi.org/10.5194/amt-2019-339, 2019
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This study assesses the performance of SKYNET in comparison to AERONET (Aerosol Robotic Network) for retrieving aerosol optical properties (AOPs) in Beijing, China. SKYNET data retrieved by SR-CEReS analysis package are used to analyze a serious pollution event in winter over Beijing. The AOPs under three weather conditions (clean, dusty, haze) in Beijing are discussed. Measurements from the SKYNET skyradiometer can be used to analyze the AOPs over Beijing reasonably.
Huizheng Che, Ke Gui, Xiangao Xia, Yaqiang Wang, Brent N. Holben, Philippe Goloub, Emilio Cuevas-Agulló, Hong Wang, Yu Zheng, Hujia Zhao, and Xiaoye Zhang
Atmos. Chem. Phys., 19, 10497–10523, https://doi.org/10.5194/acp-19-10497-2019, https://doi.org/10.5194/acp-19-10497-2019, 2019
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A comprehensive assessment of the global and regional AOD trends over the past 37 years (1980–2016) is presented. AOD observations from both AERONET and CARSNET were used for the first time to assess the performance of the MERRA-2 AOD dataset on a global scale. Based on statistical models, we found the meteorological parameters explained a larger proportion of the regional AOD variability (20.4 %–2.8 %) when compared with emission factors (0 %%–56 %).
Hua Yu, Weijun Li, Yangmei Zhang, Peter Tunved, Manuel Dall'Osto, Xiaojing Shen, Junying Sun, Xiaoye Zhang, Jianchao Zhang, and Zongbo Shi
Atmos. Chem. Phys., 19, 10433–10446, https://doi.org/10.5194/acp-19-10433-2019, https://doi.org/10.5194/acp-19-10433-2019, 2019
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Interaction of anthropogenic particles with radiation and clouds plays an important role in Arctic climate change. The mixing state of different aerosols is a key parameter influencing such interactions. However, little is known of this parameter, preventing an accurate representation of this information in global models. Multi-microscopic techniques were used to find one general core–shell structure in which secondary sulfate particles were covered by organic coating in the Arctic atmosphere.
Yahui Che, Jie Guang, Gerrit de Leeuw, Yong Xue, Ling Sun, and Huizheng Che
Atmos. Meas. Tech., 12, 4091–4112, https://doi.org/10.5194/amt-12-4091-2019, https://doi.org/10.5194/amt-12-4091-2019, 2019
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The use of AOD data retrieved from ATSR-2, AATSR and AVHRR to produce a very long time series is investigated. The study is made over a small area in northern China with a large variation of AOD values. Sun photometer data from AERONET and CARSNET and radiance-derived AOD are used as reference. The results show that all data sets compare well. However, AVHRR underestimates high AOD (mainly occurring in summer) but performs better than (A)ATSR in winter.
Weijun Li, Lei Liu, Qi Yuan, Liang Xu, Yanhong Zhu, Bingbing Wang, Hua Yu, Xiaokun Ding, Jian Zhang, Dao Huang, Dantong Liu, Wei Hu, Daizhou Zhang, Pingqing Fu, Maosheng Yao, Min Hu, Xiaoye Zhang, and Zongbo Shi
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2019-539, https://doi.org/10.5194/acp-2019-539, 2019
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The real state of individual primary biological aerosol particles (PBAPs) derived from natural sources is under mystery, although many studies well evaluate the morphology, mixing state, and elemental composition of anthropogenic particles. It induces that some studies mislead some anthropogenic particles into biological particles through electron microscopy. Here we firstly estimate the full database of individual PBAPs through two microscopic instruments. The database is good for research.
Linlin Wang, Junkai Liu, Zhiqiu Gao, Yubin Li, Meng Huang, Sihui Fan, Xiaoye Zhang, Yuanjian Yang, Shiguang Miao, Han Zou, Yele Sun, Yong Chen, and Ting Yang
Atmos. Chem. Phys., 19, 6949–6967, https://doi.org/10.5194/acp-19-6949-2019, https://doi.org/10.5194/acp-19-6949-2019, 2019
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Urban boundary layer (UBL) affects the physical and chemical processes of the pollutants, and UBL structure can also be altered by pollutants. This paper presents the interactions between air pollution and the UBL structure by using the field data mainly collected from a 325 m meteorology tower, as well as from a Doppler wind lidar, during a severe heavy pollution event that occurred during 1–4 December 2016 in Beijing.
Junting Zhong, Xiaoye Zhang, Yaqiang Wang, Jizhi Wang, Xiaojing Shen, Hongsheng Zhang, Tijian Wang, Zhouqing Xie, Cheng Liu, Hengde Zhang, Tianliang Zhao, Junying Sun, Shaojia Fan, Zhiqiu Gao, Yubin Li, and Linlin Wang
Atmos. Chem. Phys., 19, 3287–3306, https://doi.org/10.5194/acp-19-3287-2019, https://doi.org/10.5194/acp-19-3287-2019, 2019
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In various haze regions in China, including the Guanzhong Plain, the middle and lower reaches of the Yangtze River, the Pearl River Delta, the Sichuan Basin, and the Northeast China Plain, heavy aerosol pollution episodes include inter-/trans-regional transport stages and cumulative stages (CSs). During CSs a two-way feedback mechanism exists between unfavorable meteorological conditions and cumulative aerosol pollution. This two-way feedback is further quantified and its magnitude is compared.
Angela Benedetti, Francesca Di Giuseppe, Luke Jones, Vincent-Henri Peuch, Samuel Rémy, and Xiaoye Zhang
Atmos. Chem. Phys., 19, 987–998, https://doi.org/10.5194/acp-19-987-2019, https://doi.org/10.5194/acp-19-987-2019, 2019
Hong Wang, Yue Peng, Xiaoye Zhang, Hongli Liu, Meng Zhang, Huizheng Che, Yanli Cheng, and Yu Zheng
Atmos. Chem. Phys., 18, 17717–17733, https://doi.org/10.5194/acp-18-17717-2018, https://doi.org/10.5194/acp-18-17717-2018, 2018
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The explosive growth (EG) of PM2.5 resulted in a PM2.5 maximum, which was generally underestimated by atmospheric chemical models due to the deficient description of the local
turbulence intermittent. The aerosol–radiation feedback (AF) and decrease in turbulence diffusion (DTD) may reduce the underestimation of PM2.5 EG by 20–25% and 14–20%, respectively. The modeled EG stage PM2.5 error was decreased from −40 to −51% to −11 to 2% by the combined effects of AF and DTD in Jing–Jin–Ji.
Yue Peng, Hong Wang, Yubin Li, Changwei Liu, Tianliang Zhao, Xiaoye Zhang, Zhiqiu Gao, Tong Jiang, Huizheng Che, and Meng Zhang
Atmos. Chem. Phys., 18, 17421–17435, https://doi.org/10.5194/acp-18-17421-2018, https://doi.org/10.5194/acp-18-17421-2018, 2018
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Two surface layer schemes are evaluated in eastern China based on observational flux data. The results indicate that the Li scheme better describes regional atmosphere stratification compared with the MM5 scheme, especially for the transition stage from unstable to stable atmosphere conditions, corresponding to PM2.5 accumulation. Our research suggests the potential improved possibilities for severe haze prediction in eastern China by coupling Li online into atmosphere chemical models.
Xiaoning Xie, Xiaodong Liu, Huizheng Che, Xiaoxun Xie, Xinzhou Li, Zhengguo Shi, Hongli Wang, Tianliang Zhao, and Yangang Liu
Atmos. Chem. Phys., 18, 12683–12698, https://doi.org/10.5194/acp-18-12683-2018, https://doi.org/10.5194/acp-18-12683-2018, 2018
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This study extends our previous investigation in dust–radiation interactions to investigate SRF and its feedbacks on the regional climate and the dust cycle over east Asia by use of the CAM4-BAM. Our results show that SRF increases the east Asian dust emissions significantly by 13.7 % in the spring, in contrast to −7.6 % of decreased dust emissions by DRF. Hence, a significant feature of SRF on the Tibetan Plateau can create a positive feedback loop to enhance the dust cycle over east Asia.
Xiaoye Zhang, Junting Zhong, Jizhi Wang, Yaqiang Wang, and Yanju Liu
Atmos. Chem. Phys., 18, 5991–5999, https://doi.org/10.5194/acp-18-5991-2018, https://doi.org/10.5194/acp-18-5991-2018, 2018
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The relation between interdecadal changes in weather conditions and climate warming is uncertain. Here, the decadal worsening of meteorological conditions since the 1960s in the Beijing area was found to be partly attributed to climate warming, which is defined by more warming in the higher layers of the boundary layer (BL) than the lower layers. This worsening may also partly be related to the impact on the increasing aerosol pollution (particularly after 2010).
Tianze Sun, Huizheng Che, Bing Qi, Yaqiang Wang, Yunsheng Dong, Xiangao Xia, Hong Wang, Ke Gui, Yu Zheng, Hujia Zhao, Qianli Ma, Rongguang Du, and Xiaoye Zhang
Atmos. Chem. Phys., 18, 2949–2971, https://doi.org/10.5194/acp-18-2949-2018, https://doi.org/10.5194/acp-18-2949-2018, 2018
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The Yangtze River Delta (YRD) region is a key hub in China with air pollution problems. We applied various data from observations and satellites, finding particles in summer prefer hygroscopic growth leading to high scatter. Transported scatter particles lead to a cooling effect which lowers the boundary layer, creating positive feedback. Transported pollutants over YRD are from the North China Plain, northwestern deserts, and southern biomass burning. This finding helps air quality control.
Bingliang Zhuang, Tijian Wang, Jane Liu, Huizheng Che, Yong Han, Yu Fu, Shu Li, Min Xie, Mengmeng Li, Pulong Chen, Huimin Chen, Xiu-qun Yang, and Jianning Sun
Atmos. Chem. Phys., 18, 1419–1436, https://doi.org/10.5194/acp-18-1419-2018, https://doi.org/10.5194/acp-18-1419-2018, 2018
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Aerosols have a significant influence on climate changes. Their uncertainties could be substantially reduced if observation data were used. The properties and the DRF of fractionated aerosols in the western Yangtze River Delta are investigated based on measurements. Results reveal the characteristics of the optical properties and DRFs of different types of fractionated aerosols, which can be further used to improve aerosol modelling performance in the eastern regions of China.
Xiaojing Shen, Junying Sun, Niku Kivekäs, Adam Kristensson, Xiaoye Zhang, Yangmei Zhang, Lu Zhang, Ruxia Fan, Xuefei Qi, Qianli Ma, and Huaigang Zhou
Atmos. Chem. Phys., 18, 587–599, https://doi.org/10.5194/acp-18-587-2018, https://doi.org/10.5194/acp-18-587-2018, 2018
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In this study we used the NanoMap method by applying back trajectories and particle number size distribution in different rural sites in China to evaluate the spatial distribution of NPF events and their occurrence probability. We found difference in the horizontal spatial distribution of new particle source areas was connected to typical meteorological conditions. The horizontal extent of NPF reached to larger than 500 km at two sites, favoured by the fast transport of northwesterly air masses.
Huizheng Che, Bing Qi, Hujia Zhao, Xiangao Xia, Thomas F. Eck, Philippe Goloub, Oleg Dubovik, Victor Estelles, Emilio Cuevas-Agulló, Luc Blarel, Yunfei Wu, Jun Zhu, Rongguang Du, Yaqiang Wang, Hong Wang, Ke Gui, Jie Yu, Yu Zheng, Tianze Sun, Quanliang Chen, Guangyu Shi, and Xiaoye Zhang
Atmos. Chem. Phys., 18, 405–425, https://doi.org/10.5194/acp-18-405-2018, https://doi.org/10.5194/acp-18-405-2018, 2018
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Sun photometer measurements from seven sites in the Yangtze River Delta (YRD) from 2011 to 2015 were used to characterize the climatology of aerosol microphysical and optical properties, calculate direct aerosol radiative forcing (DARF) and classify aerosols based on size and absorption. This study contributes to our understanding of aerosols and regional climate/air quality, and the results will be useful for validating satellite retrievals and for improving climate models and remote sensing.
Junting Zhong, Xiaoye Zhang, Yunsheng Dong, Yaqiang Wang, Cheng Liu, Jizhi Wang, Yangmei Zhang, and Haochi Che
Atmos. Chem. Phys., 18, 247–258, https://doi.org/10.5194/acp-18-247-2018, https://doi.org/10.5194/acp-18-247-2018, 2018
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Beijing heavy pollution episodes are characterized by the transport stage (TS) and the cumulative stage (CS). PM2.5 pollution formation in the TS is primarily caused by pollutants transported from the south of Beijing. PM2.5 cumulative explosive growth in the CS is dominated by stable atmospheric stratification due to the interaction of particulate matter (PM) and meteorological factors. The positive meteorological feedback on PM2.5 mass noted explains over 70% of cumulative explosive growth.
Ying Zhang, Zhengqiang Li, Yuhuan Zhang, Donghui Li, Lili Qie, Huizheng Che, and Hua Xu
Atmos. Meas. Tech., 10, 3203–3213, https://doi.org/10.5194/amt-10-3203-2017, https://doi.org/10.5194/amt-10-3203-2017, 2017
Shurui Chen, Liang Xu, Yinxiao Zhang, Bing Chen, Xinfeng Wang, Xiaoye Zhang, Mei Zheng, Jianmin Chen, Wenxing Wang, Yele Sun, Pingqing Fu, Zifa Wang, and Weijun Li
Atmos. Chem. Phys., 17, 1259–1270, https://doi.org/10.5194/acp-17-1259-2017, https://doi.org/10.5194/acp-17-1259-2017, 2017
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Many studies have focused on the unusually severe hazes instead of the more frequent light and moderate hazes (22–63 %) in winter in the North China Plain (NCP). The morphology, mixing state, and size of organic aerosols in the L & M hazes were characterized. We conclude that the direct emissions from residential coal stoves without any pollution controls in rural and urban outskirts contribute large amounts of primary OM particles to the regional L & M hazes in winter in the NCP.
Y. Q. Yang, J. Z. Wang, S. L. Gong, X. Y. Zhang, H. Wang, Y. Q. Wang, J. Wang, D. Li, and J. P. Guo
Atmos. Chem. Phys., 16, 1353–1364, https://doi.org/10.5194/acp-16-1353-2016, https://doi.org/10.5194/acp-16-1353-2016, 2016
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A new model, PLAM/h, has been developed and used in near-real-time air quality forecasts by considering both meteorology and pollutant emissions, based on the two-dimensional probability density function diagnosis model for emissions. The results show that combining the influence of regular meteorological conditions and emission factors together in the PLAM/h parameterization scheme is very effective in improving the forecasting ability for fog-haze weather in North China.
P. Wang, H. Wang, Y. Q. Wang, X. Y. Zhang, S. L. Gong, M. Xue, C. H. Zhou, H. L. Liu, X. Q. An, T. Niu, and Y. L. Cheng
Atmos. Chem. Phys., 16, 989–1002, https://doi.org/10.5194/acp-16-989-2016, https://doi.org/10.5194/acp-16-989-2016, 2016
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An ensemble optimal interpolation (EnOI) data assimilation technique is used to investigate the possibility of optimally recovering the spatially resolved emissions bias of BC. The inversed emission over China in January is 240.1 Gg, and annual emission is about 2539 Gg. Even though only monthly mean BC measurements are employed to inverse the emissions, the accuracy of the daily model simulation improves. We finds that EnOI is a useful and computation-free method to make top-down estimation.
C. Zhou, X. Zhang, S. Gong, Y. Wang, and M. Xue
Atmos. Chem. Phys., 16, 145–160, https://doi.org/10.5194/acp-16-145-2016, https://doi.org/10.5194/acp-16-145-2016, 2016
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A comprehensive aerosol-cloud-precipitation interaction (ACI) scheme from emissions to precipitation has been developed under the CMA chemical weather modeling system GRAPES/CUACE. The ACI for January 2013 has been studied using this model. The interactive microphysical properties of clouds improve the precipitation, showing 24 to 48 % enhancements of threat score for 6 h precipitation in all regions and reduction of the regional mean bias of temperature by 3 °C in certain precipitation events.
Y. Q. Wang, X. Y. Zhang, J. Y. Sun, X. C. Zhang, H. Z. Che, and Y. Li
Atmos. Chem. Phys., 15, 13585–13598, https://doi.org/10.5194/acp-15-13585-2015, https://doi.org/10.5194/acp-15-13585-2015, 2015
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Concentrations of PM10, PM2.5 and PM1 were monitored at 24 stations of CAWNET from 2006 to 2014. The average levels of particulate matter (PM) concentrations and relationships were investigated. Seasonal, interannual and diurnal variations of the PM were revealed. The effects of meteorological factors on the PM were discussed. The highest PM concentrations were observed at the stations of Xian, Zhengzhou and Gucheng, in Guanzhong and the Huabei Plain.
J.-W. Xu, R. V. Martin, A. van Donkelaar, J. Kim, M. Choi, Q. Zhang, G. Geng, Y. Liu, Z. Ma, L. Huang, Y. Wang, H. Chen, H. Che, P. Lin, and N. Lin
Atmos. Chem. Phys., 15, 13133–13144, https://doi.org/10.5194/acp-15-13133-2015, https://doi.org/10.5194/acp-15-13133-2015, 2015
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1. GOCI (Geostationary Ocean Color Imager) retrieval of AOD is consistent with AERONET AOD (RMSE=0.08-0.1)
2. GOCI-derived PM2.5 is in significant agreement with in situ observations (r2=0.66, rRMSE=18.3%)
3. Population-weighted GOCI-derived PM2.5 over eastern China for 2013 is 53.8 μg/m3, threatening the health of its more than 400 million residents
4. Secondary inorganics (SO42-, NO3-, NH4+) & organic matter are the most significant components of GOCI-derived PM2.5.
X. Y. Zhang, J. Z. Wang, Y. Q. Wang, H. L. Liu, J. Y. Sun, and Y. M. Zhang
Atmos. Chem. Phys., 15, 12935–12952, https://doi.org/10.5194/acp-15-12935-2015, https://doi.org/10.5194/acp-15-12935-2015, 2015
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No obvious changes were found in annual mean concentrations of major chemical components and PM10 in 2013, relative to 2012. But wintertime mass were quite different; approximately 60% of the winter mass increase from 2012 to 2013 can be attributed to severe meteorological conditions in the HBP area, and mass of chemical components exhibited a decline during 2006 to 2010, and then a rise till 2013. Coal-combustion was still the largest anthropogenic source of aerosol pollution in 2013 in China.
J. W. Chi, W. J. Li, D. Z. Zhang, J. C. Zhang, Y. T. Lin, X. J. Shen, J. Y. Sun, J. M. Chen, X. Y. Zhang, Y. M. Zhang, and W. X. Wang
Atmos. Chem. Phys., 15, 11341–11353, https://doi.org/10.5194/acp-15-11341-2015, https://doi.org/10.5194/acp-15-11341-2015, 2015
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Sea salt aerosols (SSA) are dominant particles in the Arctic atmosphere. Our result suggests that the hydrophilic MgCl2 coating in fresh SSA likely intrigued the heterogeneous reactions at the beginning of SSA and acidic gases in the Arctic. The content of organic matter increased in the aged SSA compared with the fresh SSA, which suggests organic acids (beside inorganic acids) participate in the ageing of SSA in the Arctic.
L. Zhang, J. Y. Sun, X. J. Shen, Y. M. Zhang, H. Che, Q. L. Ma, Y. W. Zhang, X. Y. Zhang, and J. A. Ogren
Atmos. Chem. Phys., 15, 8439–8454, https://doi.org/10.5194/acp-15-8439-2015, https://doi.org/10.5194/acp-15-8439-2015, 2015
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The aerosol hygroscopic properties at a rural background site in the Yangtze River delta of China was discussed. The results show the scattering coefficient and backscattering coefficient increased by 58 and 25% as relative humidity (RH) increased from 40 to 85%, while the hemispheric backscatter fraction decreased by 21%. Aerosol hygroscopic growth caused a 47% increase in calculated aerosol direct radiative forcing at 85% RH compared to the forcing at 40% RH. Nitrate played a vital role.
H. Che, X.-Y. Zhang, X. Xia, P. Goloub, B. Holben, H. Zhao, Y. Wang, X.-C. Zhang, H. Wang, L. Blarel, B. Damiri, R. Zhang, X. Deng, Y. Ma, T. Wang, F. Geng, B. Qi, J. Zhu, J. Yu, Q. Chen, and G. Shi
Atmos. Chem. Phys., 15, 7619–7652, https://doi.org/10.5194/acp-15-7619-2015, https://doi.org/10.5194/acp-15-7619-2015, 2015
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This work studied more than 10 years of measurements of aerosol optical depths (AODs) made for 50 sites of CARSNET compiled into a climatology of aerosol optical properties for China. It lets us see a detailed full-scale description of AOD observations over China. The results would benefit us a lot in comprehending the temporal and special distribution aerosol optical property over China. Also the data would be valuable to communities of aerosol satellite retrieval, modelling, etc.
C. Jiang, H. Wang, T. Zhao, T. Li, and H. Che
Atmos. Chem. Phys., 15, 5803–5814, https://doi.org/10.5194/acp-15-5803-2015, https://doi.org/10.5194/acp-15-5803-2015, 2015
Z. L. Wang, H. Zhang, and X. Y. Zhang
Atmos. Chem. Phys., 15, 3671–3685, https://doi.org/10.5194/acp-15-3671-2015, https://doi.org/10.5194/acp-15-3671-2015, 2015
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This study highlights that there are no effective ways to remove the black carbon exclusively without influencing the other co-emitted components, our results therefore indicate that a reduction in BC emission can lead to an unexpected warming on the Earth’s climate system in the future.
H. Wang, M. Xue, X. Y. Zhang, H. L. Liu, C. H. Zhou, S. C. Tan, H. Z. Che, B. Chen, and T. Li
Atmos. Chem. Phys., 15, 3257–3275, https://doi.org/10.5194/acp-15-3257-2015, https://doi.org/10.5194/acp-15-3257-2015, 2015
H. Wang, G. Y. Shi, X. Y. Zhang, S. L. Gong, S. C. Tan, B. Chen, H. Z. Che, and T. Li
Atmos. Chem. Phys., 15, 3277–3287, https://doi.org/10.5194/acp-15-3277-2015, https://doi.org/10.5194/acp-15-3277-2015, 2015
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Solar radiation reaching the ground decreases about 15% in Chinese 3JNS region and by 20 to 25% in the region with the highest AOD. Aerosol cools the PBL atmosphere but warms the atmosphere above it, leading to a more stable atmosphere that causes a decrease in turbulence diffusion of about 52% and in PBL height of about 33%; this results in a positive feedback on the PM2.5 concentration within the PBL and the surface as well as the haze formation.
Y. M. Zhang, X. Y. Zhang, J. Y. Sun, G. Y. Hu, X. J. Shen, Y. Q. Wang, T. T. Wang, D. Z. Wang, and Y. Zhao
Atmos. Chem. Phys., 14, 12237–12249, https://doi.org/10.5194/acp-14-12237-2014, https://doi.org/10.5194/acp-14-12237-2014, 2014
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An AMS was employed to measure the mass and size distributions of PM1 at an elevated site. Features of PM1 at four seasons, during different kinds of episodes including NPF, polluted, PBL, LFT and in-cloud, were discussed. The characterizations of PM1 at seven clusters of air masses were also analyzed. BBOA, CCOA and oxidized organic aerosols were resolved by AMS-PMF (positive matrix function). Almost half of OA were oxidized, and BBOA is 34% of OA in summer; CCOA is 22% of OA in winter as well.
K. Tsigaridis, N. Daskalakis, M. Kanakidou, P. J. Adams, P. Artaxo, R. Bahadur, Y. Balkanski, S. E. Bauer, N. Bellouin, A. Benedetti, T. Bergman, T. K. Berntsen, J. P. Beukes, H. Bian, K. S. Carslaw, M. Chin, G. Curci, T. Diehl, R. C. Easter, S. J. Ghan, S. L. Gong, A. Hodzic, C. R. Hoyle, T. Iversen, S. Jathar, J. L. Jimenez, J. W. Kaiser, A. Kirkevåg, D. Koch, H. Kokkola, Y. H Lee, G. Lin, X. Liu, G. Luo, X. Ma, G. W. Mann, N. Mihalopoulos, J.-J. Morcrette, J.-F. Müller, G. Myhre, S. Myriokefalitakis, N. L. Ng, D. O'Donnell, J. E. Penner, L. Pozzoli, K. J. Pringle, L. M. Russell, M. Schulz, J. Sciare, Ø. Seland, D. T. Shindell, S. Sillman, R. B. Skeie, D. Spracklen, T. Stavrakou, S. D. Steenrod, T. Takemura, P. Tiitta, S. Tilmes, H. Tost, T. van Noije, P. G. van Zyl, K. von Salzen, F. Yu, Z. Wang, Z. Wang, R. A. Zaveri, H. Zhang, K. Zhang, Q. Zhang, and X. Zhang
Atmos. Chem. Phys., 14, 10845–10895, https://doi.org/10.5194/acp-14-10845-2014, https://doi.org/10.5194/acp-14-10845-2014, 2014
J. Tao, J. Gao, L. Zhang, R. Zhang, H. Che, Z. Zhang, Z. Lin, J. Jing, J. Cao, and S.-C. Hsu
Atmos. Chem. Phys., 14, 8679–8699, https://doi.org/10.5194/acp-14-8679-2014, https://doi.org/10.5194/acp-14-8679-2014, 2014
H. Che, X. Xia, J. Zhu, Z. Li, O. Dubovik, B. Holben, P. Goloub, H. Chen, V. Estelles, E. Cuevas-Agulló, L. Blarel, H. Wang, H. Zhao, X. Zhang, Y. Wang, J. Sun, R. Tao, X. Zhang, and G. Shi
Atmos. Chem. Phys., 14, 2125–2138, https://doi.org/10.5194/acp-14-2125-2014, https://doi.org/10.5194/acp-14-2125-2014, 2014
A. Petzold, J. A. Ogren, M. Fiebig, P. Laj, S.-M. Li, U. Baltensperger, T. Holzer-Popp, S. Kinne, G. Pappalardo, N. Sugimoto, C. Wehrli, A. Wiedensohler, and X.-Y. Zhang
Atmos. Chem. Phys., 13, 8365–8379, https://doi.org/10.5194/acp-13-8365-2013, https://doi.org/10.5194/acp-13-8365-2013, 2013
H. Jiang, H. Liao, H. O. T. Pye, S. Wu, L. J. Mickley, J. H. Seinfeld, and X. Y. Zhang
Atmos. Chem. Phys., 13, 7937–7960, https://doi.org/10.5194/acp-13-7937-2013, https://doi.org/10.5194/acp-13-7937-2013, 2013
Related subject area
Domain: ESSD – Atmosphere | Subject: Atmospheric chemistry and physics
The Tibetan Plateau space-based tropospheric aerosol climatology: 2007–2020
PalVol v1: a proxy-based semi-stochastic ensemble reconstruction of volcanic stratospheric sulfur injection for the last glacial cycle (140 000–50 BP)
Ground- and ship-based microwave radiometer measurements during EUREC4A
Shortwave and longwave components of the surface radiation budget measured at the Thule High Arctic Atmospheric Observatory, Northern Greenland
Cloud condensation nuclei concentrations derived from the CAMS reanalysis
A merged continental planetary boundary layer height dataset based on high-resolution radiosonde measurements, ERA5 reanalysis, and GLDAS
High-resolution physicochemical dataset of atmospheric aerosols over the Tibetan Plateau and its surroundings
12 years of continuous atmospheric O2, CO2 and APO data from Weybourne Atmospheric Observatory in the United Kingdom
CLAAS-3: the third edition of the CM SAF cloud data record based on SEVIRI observations
Using machine learning to construct TOMCAT model and occultation measurement-based stratospheric methane (TCOM-CH4) and nitrous oxide (TCOM-N2O) profile data sets
A Level 3 Monthly Gridded Ice Cloud Dataset Derived from a Decade of CALIOP Measurements
High-resolution aerosol data from the top 3.8 kyr of the East Greenland Ice coring Project (EGRIP) ice core
Introduction to the NJIAS Himawari-8/9 cloud feature dataset for climate and typhoon research
A database of aircraft measurements of carbon monoxide (CO) with high temporal and spatial resolution during 2011–2021
DCMEX coordinated aircraft and ground observations: Microphysics, aerosol and dynamics during cumulonimbus development
Global Anthropogenic Emissions (CAMS-GLOB-ANT) for the Copernicus Atmosphere Monitoring Service Simulations of Air Quality Forecasts and Reanalyses
The Total Carbon Column Observing Network's GGG2020 Data Version
A first global height-resolved cloud condensation nuclei data set derived from spaceborne lidar measurements
A monthly 1° resolution dataset of daytime cloud fraction over the Arctic during 2000–2020 based on multiple satellite products
Network for the Detection of Atmospheric Composition Change (NDACC) Fourier transform infrared (FTIR) trace gas measurements at the University of Toronto Atmospheric Observatory from 2002 to 2020
Deconstruction of tropospheric chemical reactivity using aircraft measurements: the Atmospheric Tomography Mission (ATom) data
Spatial variability of Saharan dust deposition revealed through a citizen science campaign
Radiative sensitivity quantified by a new set of radiation flux kernels based on the ECMWF Reanalysis v5 (ERA5)
Updated observations of clouds by MODIS for global model assessment
An extensive database of airborne trace gas and meteorological observations from the Alpha Jet Atmospheric eXperiment (AJAX)
Two years of volatile organic compound online in situ measurements at the Site Instrumental de Recherche par Télédétection Atmosphérique (Paris region, France) using proton-transfer-reaction mass spectrometry
Global Ozone Monitoring Experiment-2 (GOME-2) daily and monthly level-3 products of atmospheric trace gas columns
Crowdsourced Doppler measurements of time standard stations demonstrating ionospheric variability
A machine learning approach to address air quality changes during the COVID-19 lockdown in Buenos Aires, Argentina
Version 2 of the global catalogue of large anthropogenic and volcanic SO2 sources and emissions derived from satellite measurements
World Wide Lightning Location Network (WWLLN) Global Lightning Climatology (WGLC) and time series, 2022 update
Long-term ash dispersal dataset of the Sakurajima Taisho eruption for ashfall disaster countermeasure
Full-coverage 250 m monthly aerosol optical depth dataset (2000–2019) amended with environmental covariates by an ensemble machine learning model over arid and semi-arid areas, NW China
The polar mesospheric cloud dataset of the Balloon Lidar Experiment (BOLIDE)
Multiyear emissions of carbonaceous aerosols from cooking, fireworks, sacrificial incense, joss paper burning, and barbecue as well as their key driving forces in China
Impacts of the proposal of the CNG2020 strategy on aircraft emissions of China–foreign routes
Northern hemispheric atmospheric ethane trends in the upper troposphere and lower stratosphere (2006–2016) with reference to methane and propane
New contributions of measurements in Europe to the global inventory of the stable isotopic composition of methane
International Monitoring System infrasound data products for atmospheric studies and civilian applications
A benchmark dataset of diurnal- and seasonal-scale radiation, heat, and CO2 fluxes in a typical East Asian monsoon region
Attenuated atmospheric backscatter profiles measured by the CO2 Sounder lidar in the 2017 ASCENDS/ABoVE airborne campaign
Climatology of aerosol component concentrations derived from multi-angular polarimetric POLDER-3 observations using GRASP algorithm
A 10-year global monthly averaged terrestrial net ecosystem exchange dataset inferred from the ACOS GOSAT v9 XCO2 retrievals (GCAS2021)
Honglin Pan, Jianping Huang, Jiming Li, Zhongwei Huang, Minzhong Wang, Ali Mamtimin, Wen Huo, Fan Yang, Tian Zhou, and Kanike Raghavendra Kumar
Earth Syst. Sci. Data, 16, 1185–1207, https://doi.org/10.5194/essd-16-1185-2024, https://doi.org/10.5194/essd-16-1185-2024, 2024
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We applied several correction procedures and rigorously checked for data quality constraints during the long observation period spanning almost 14 years (2007–2020). Nevertheless, some uncertainties remain, mainly due to technical constraints and limited documentation of the measurements. Even though not completely accurate, this strategy is expected to at least reduce the inaccuracy of the computed characteristic value of aerosol optical parameters.
Julie Christin Schindlbeck-Belo, Matthew Toohey, Marion Jegen, Steffen Kutterolf, and Kira Rehfeld
Earth Syst. Sci. Data, 16, 1063–1081, https://doi.org/10.5194/essd-16-1063-2024, https://doi.org/10.5194/essd-16-1063-2024, 2024
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Volcanic forcing of climate resulting from major explosive eruptions is a dominant natural driver of past climate variability. To support model studies of the potential impacts of explosive volcanism on climate variability across timescales, we present an ensemble reconstruction of volcanic stratospheric sulfur injection over the last 140 000 years that is based primarily on tephra records.
Sabrina Schnitt, Andreas Foth, Heike Kalesse-Los, Mario Mech, Claudia Acquistapace, Friedhelm Jansen, Ulrich Löhnert, Bernhard Pospichal, Johannes Röttenbacher, Susanne Crewell, and Bjorn Stevens
Earth Syst. Sci. Data, 16, 681–700, https://doi.org/10.5194/essd-16-681-2024, https://doi.org/10.5194/essd-16-681-2024, 2024
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This publication describes the microwave radiometric measurements performed during the EUREC4A campaign at Barbados Cloud Observatory (BCO) and aboard RV Meteor and RV Maria S Merian. We present retrieved integrated water vapor (IWV), liquid water path (LWP), and temperature and humidity profiles as a unified, quality-controlled, multi-site data set on a 3 s temporal resolution for a core period between 19 January 2020 and 14 February 2020.
Daniela Meloni, Filippo Calì Quaglia, Virginia Ciardini, Annalisa Di Bernardino, Tatiana Di Iorio, Antonio Iaccarino, Giovanni Muscari, Giandomenico Pace, Claudio Scarchilli, and Alcide di Sarra
Earth Syst. Sci. Data, 16, 543–566, https://doi.org/10.5194/essd-16-543-2024, https://doi.org/10.5194/essd-16-543-2024, 2024
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Solar and infrared radiation are key factors in determining Arctic climate. Only a few sites in the Arctic perform long-term measurements of the surface radiation budget (SRB). At the Thule High Arctic Atmospheric Observatory (THAAO, 76.5° N, 68.8° W) in Northern Greenland, solar and infrared irradiance measurements were started in 2009. These data are of paramount importance in studying the impact of the atmospheric (mainly clouds and aerosols) and surface (albedo) parameters on the SRB.
Karoline Block, Mahnoosh Haghighatnasab, Daniel G. Partridge, Philip Stier, and Johannes Quaas
Earth Syst. Sci. Data, 16, 443–470, https://doi.org/10.5194/essd-16-443-2024, https://doi.org/10.5194/essd-16-443-2024, 2024
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Aerosols being able to act as condensation nuclei for cloud droplets (CCNs) are a key element in cloud formation but very difficult to determine. In this study we present a new global vertically resolved CCN dataset for various humidity conditions and aerosols. It is obtained using an atmospheric model (CAMS reanalysis) that is fed by satellite observations of light extinction (AOD). We investigate and evaluate the abundance of CCNs in the atmosphere and their temporal and spatial occurrence.
Jianping Guo, Jian Zhang, Jia Shao, Tianmeng Chen, Kaixu Bai, Yuping Sun, Ning Li, Jingyan Wu, Rui Li, Jian Li, Qiyun Guo, Jason B. Cohen, Panmao Zhai, Xiaofeng Xu, and Fei Hu
Earth Syst. Sci. Data, 16, 1–14, https://doi.org/10.5194/essd-16-1-2024, https://doi.org/10.5194/essd-16-1-2024, 2024
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A global continental merged high-resolution (PBLH) dataset with good accuracy compared to radiosonde is generated via machine learning algorithms, covering the period from 2011 to 2021 with 3-hour and 0.25º resolution in space and time. The machine learning model takes parameters derived from the ERA5 reanalysis and GLDAS product as input, with PBLH biases between radiosonde and ERA5 as the learning targets. The merged PBLH is the sum of the predicted PBLH bias and the PBLH from ERA5.
Jianzhong Xu, Xinghua Zhang, Wenhui Zhao, Lixiang Zhai, Miao Zhao, Jinsen Shi, Junying Sun, Yanmei Liu, Conghui Xie, Yulong Tan, Kemei Li, Xinlei Ge, Qi Zhang, and Shichang Kang
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-506, https://doi.org/10.5194/essd-2023-506, 2023
Revised manuscript accepted for ESSD
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A comprehensive aerosol observation project was carried out in the Tibetan Plateau (TP) and its surrounding in recent years to investigate the properties and sources of atmospheric aerosols as well as their regional differences by performing multiple intensive field observations. The release of this dataset can provide basic and systematic data for related researches in atmospheric, cryospheric, and environmental sciences in this unique region.
Karina E. Adcock, Penelope A. Pickers, Andrew C. Manning, Grant L. Forster, Leigh S. Fleming, Thomas Barningham, Philip A. Wilson, Elena A. Kozlova, Marica Hewitt, Alex J. Etchells, and Andy J. Macdonald
Earth Syst. Sci. Data, 15, 5183–5206, https://doi.org/10.5194/essd-15-5183-2023, https://doi.org/10.5194/essd-15-5183-2023, 2023
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We present a 12-year time series of continuous atmospheric measurements of O2 and CO2 at the Weybourne Atmospheric Observatory in the United Kingdom. These measurements are combined into the term atmospheric potential oxygen (APO), a tracer that is not influenced by land biosphere processes. The datasets show a long-term increasing trend in CO2 and decreasing trends in O2 and APO between 2010 and 2021.
Nikos Benas, Irina Solodovnik, Martin Stengel, Imke Hüser, Karl-Göran Karlsson, Nina Håkansson, Erik Johansson, Salomon Eliasson, Marc Schröder, Rainer Hollmann, and Jan Fokke Meirink
Earth Syst. Sci. Data, 15, 5153–5170, https://doi.org/10.5194/essd-15-5153-2023, https://doi.org/10.5194/essd-15-5153-2023, 2023
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This paper describes CLAAS-3, the third edition of the Cloud property dAtAset using SEVIRI, which was created based on observations from geostationary Meteosat satellites. CLAAS-3 cloud properties are evaluated using a variety of reference datasets, with very good overall results. The demonstrated quality of CLAAS-3 ensures its usefulness in a wide range of applications, including studies of local- to continental-scale cloud processes and evaluation of climate models.
Sandip S. Dhomse and Martyn P. Chipperfield
Earth Syst. Sci. Data, 15, 5105–5120, https://doi.org/10.5194/essd-15-5105-2023, https://doi.org/10.5194/essd-15-5105-2023, 2023
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There are no long-term stratospheric profile data sets for two very important greenhouse gases: methane (CH4) and nitrous oxide (N2O). Along with radiative feedback, these species play an important role in controlling ozone loss in the stratosphere. Here, we use machine learning to fuse satellite measurements with a chemical model to construct long-term gap-free profile data sets for CH4 and N2O. We aim to construct similar data sets for other important trace gases (e.g. O3, Cly, NOy species).
David Winker, Xia Cai, Mark Vaughan, Anne Garnier, Brian Magill, Melody Avery, and Brian Getzewich
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-373, https://doi.org/10.5194/essd-2023-373, 2023
Revised manuscript accepted for ESSD
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Clouds play important roles in both weather and climate. We describe Version 1.0 of a monthly globally gridded ice cloud data product containing vertically resolved statistics on the occurrence and properties of ice clouds, built from the curtains of lidar profile data from the CALIPSO satellite acquired over a 10-year period. This product should provide significant value for cloud research and the evaluation of clouds simulated in weather and climate models.
Tobias Erhardt, Camilla Marie Jensen, Florian Adolphi, Helle Astrid Kjær, Remi Dallmayr, Birthe Twarloh, Melanie Behrens, Motohiro Hirabayashi, Kaori Fukuda, Jun Ogata, François Burgay, Federico Scoto, Ilaria Crotti, Azzurra Spagnesi, Niccoló Maffezzoli, Delia Segato, Chiara Paleari, Florian Mekhaldi, Raimund Muscheler, Sophie Darfeuil, and Hubertus Fischer
Earth Syst. Sci. Data, 15, 5079–5091, https://doi.org/10.5194/essd-15-5079-2023, https://doi.org/10.5194/essd-15-5079-2023, 2023
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The presented paper provides a 3.8 kyr long dataset of aerosol concentrations from the East Greenland Ice coring Project (EGRIP) ice core. The data consists of 1 mm depth-resolution profiles of calcium, sodium, ammonium, nitrate, and electrolytic conductivity as well as decadal averages of these profiles. Alongside the data a detailed description of the measurement setup as well as a discussion of the uncertainties are given.
Xiaoyong Zhuge, Xiaolei Zou, Lu Yu, Xin Li, Mingjian Zeng, Yilun Chen, Bing Zhang, Bin Yao, Fei Tang, Fengjiao Chen, and Wanlin Kan
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-414, https://doi.org/10.5194/essd-2023-414, 2023
Revised manuscript accepted for ESSD
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The Himawari-8/9 level-2 operational cloud product has a low spatial resolution and is available only during the daytime. To supplement this official dataset, a new dataset named the NJIAS Himawari-8/9 Cloud Feature Dataset (HCFD) was constructed. The NJIAS HCFD provides a comprehensive description of cloud features over the East Asia and west North Pacific regions for the years 2016–2022, by 30 retrieved cloud variables. The NJIAS HCDF has been demonstrated to outperform the official dataset.
Chaoyang Xue, Gisèle Krysztofiak, Vanessa Brocchi, Stéphane Chevrier, Michel Chartier, Patrick Jacquet, Claude Robert, and Valéry Catoire
Earth Syst. Sci. Data, 15, 4553–4569, https://doi.org/10.5194/essd-15-4553-2023, https://doi.org/10.5194/essd-15-4553-2023, 2023
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To understand tropospheric air pollution at regional and global scales, an infrared laser spectrometer called SPIRIT was used on aircraft to rapidly and accurately measure carbon monoxide (CO), an important indicator of air pollution, during the last decade. Measurements were taken for more than 200 flight hours over three continents. Levels of CO are mapped with 3D trajectories for each flight. Additionally, this can be used to validate model performance and satellite measurements.
Declan L. Finney, Alan M. Blyth, Martin Gallagher, Huihui Wu, Graeme Nott, Mike Biggerstaff, Richard G. Sonnenfeld, Martin Daily, Dan Walker, David Dufton, Keith Bower, Steven Boeing, Thomas Choularton, Jonathan Crosier, James Groves, Paul R. Field, Hugh Coe, Benjamin J. Murray, Gary Lloyd, Nicholas A. Marsden, Michael Flynn, Kezhen Hu, Naveneeth M. Thamban, Paul I. Williams, James B. McQuaid, Joseph Robinson, Gordon Carrie, Robert Moore, Graydon Aulich, Ralph R. Burton, and Paul J. Connolly
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-303, https://doi.org/10.5194/essd-2023-303, 2023
Revised manuscript accepted for ESSD
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Deep convective clouds are a source of large uncertainty in predictions of surface temperature response to carbon dioxide. It is the effect of clouds on incoming sunlight and outgoing heat that matters. The DCMEX 2022 campaign in New Mexico collected data with an aircraft, radars, and other instruments. They give new detail on the role of aerosol and cloud ice in cloud formation. Combined with satellite data, the dataset can be used to explore the cloud impact on sunlight and heat.
Antonin Soulie, Claire Granier, Sabine Darras, Nicolas Zilbermann, Thierno Doumbia, Marc Guevara, Jukka-Pekka Jalkanen, Sekou Keita, Cathy Liousse, Monica Crippa, Diego Guizzardi, Rachel Hoesly, and Steven Smith
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-306, https://doi.org/10.5194/essd-2023-306, 2023
Revised manuscript accepted for ESSD
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Anthropogenic emissions are the result of transportation, power generation, industrial, residential and commercial activities, waste treatment and agriculture practices. This paper describes the new CAMS-GLOB-ANT gridded inventory of 2000–2023 anthropogenic emissions of air pollutants and greenhouse gases. The methodology to generate the emissions is explained, and the datasets are analysed and compared with publicly available global and regional inventories for selected world regions.
Joshua L. Laughner, Geoffrey C. Toon, Joseph Mendonca, Christof Petri, Sébastien Roche, Debra Wunch, Jean-Francois Blavier, David W. T. Griffith, Pauli Heikkinen, Ralph F. Keeling, Matthäus Kiel, Rigel Kivi, Coleen M. Roehl, Britton B. Stephens, Bianca C. Baier, Huilin Chen, Yonghoon Choi, Nicholas M. Deutscher, Joshua P. DiGangi, Jochen Gross, Benedikt Herkommer, Pascal Jeseck, Thomas Laemmel, Xin Lan, Erin McGee, Kathryn McKain, John Miller, Isamu Morino, Justus Notholt, Hirofumi Ohyama, David F. Pollard, Markus Rettinger, Haris Riris, Constantina Rousogenous, Mahesh Kumar Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Steven C. Wofsy, Minqiang Zhou, and Paul O. Wennberg
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2023-331, https://doi.org/10.5194/essd-2023-331, 2023
Revised manuscript accepted for ESSD
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This paper describes a new version, called GGG2020, of a dataset containing column-integrated observations of greenhouse and related gases (including CO2, CH4, CO, and N2O) made by ground stations located around the world. Compared to the previous version (GGG2014), improvements have been made towards site-to-site consistency. This dataset plays a key role in validating space-based greenhouse gas observations and in understanding the carbon cycle.
Goutam Choudhury and Matthias Tesche
Earth Syst. Sci. Data, 15, 3747–3760, https://doi.org/10.5194/essd-15-3747-2023, https://doi.org/10.5194/essd-15-3747-2023, 2023
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Aerosols in the atmosphere that can form liquid cloud droplets are called cloud condensation nuclei (CCN). Accurate measurements of CCN, especially CCN of anthropogenic origin, are necessary to quantify the effect of anthropogenic aerosols on the present-day as well as future climate. In this paper, we describe a novel global 3D CCN data set calculated from satellite measurements. We also discuss the potential applications of the data in the context of aerosol–cloud interactions.
Xinyan Liu, Tao He, Shunlin Liang, Ruibo Li, Xiongxin Xiao, Rui Ma, and Yichuan Ma
Earth Syst. Sci. Data, 15, 3641–3671, https://doi.org/10.5194/essd-15-3641-2023, https://doi.org/10.5194/essd-15-3641-2023, 2023
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We proposed a data fusion strategy that combines the complementary features of multiple-satellite cloud fraction (CF) datasets and generated a continuous monthly 1° daytime cloud fraction product covering the entire Arctic during the sunlit months in 2000–2020. This study has positive significance for reducing the uncertainties for the assessment of surface radiation fluxes and improving the accuracy of research related to climate change and energy budgets, both regionally and globally.
Shoma Yamanouchi, Stephanie Conway, Kimberly Strong, Orfeo Colebatch, Erik Lutsch, Sébastien Roche, Jeffrey Taylor, Cynthia H. Whaley, and Aldona Wiacek
Earth Syst. Sci. Data, 15, 3387–3418, https://doi.org/10.5194/essd-15-3387-2023, https://doi.org/10.5194/essd-15-3387-2023, 2023
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Nineteen years of atmospheric composition measurements made at the University of Toronto Atmospheric Observatory (TAO; 43.66° N, 79.40° W; 174 m.a.s.l.) are presented. These are retrieved from Fourier transform infrared (FTIR) solar absorption spectra recorded with a spectrometer from May 2002 to December 2020. The retrievals have been optimized for fourteen species: O3, HCl, HF, HNO3, CH4, C2H6, CO, HCN, N2O, C2H2, H2CO, CH3OH, HCOOH, and NH3.
Michael J. Prather, Hao Guo, and Xin Zhu
Earth Syst. Sci. Data, 15, 3299–3349, https://doi.org/10.5194/essd-15-3299-2023, https://doi.org/10.5194/essd-15-3299-2023, 2023
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The Atmospheric Tomography Mission (ATom) measured the chemical composition in air parcels from 0–12 km altitude on 2 km horizontal by 80 m vertical scales for four seasons, resolving most scales of chemical heterogeneity. ATom is one of the first missions designed to calculate the chemical evolution of each parcel, providing semi-global diurnal budgets for ozone and methane. Observations covered the remote troposphere: Pacific and Atlantic Ocean basins, Southern Ocean, Arctic basin, Antarctica.
Marie Dumont, Simon Gascoin, Marion Réveillet, Didier Voisin, François Tuzet, Laurent Arnaud, Mylène Bonnefoy, Montse Bacardit Peñarroya, Carlo Carmagnola, Alexandre Deguine, Aurélie Diacre, Lukas Dürr, Olivier Evrard, Firmin Fontaine, Amaury Frankl, Mathieu Fructus, Laure Gandois, Isabelle Gouttevin, Abdelfateh Gherab, Pascal Hagenmuller, Sophia Hansson, Hervé Herbin, Béatrice Josse, Bruno Jourdain, Irene Lefevre, Gaël Le Roux, Quentin Libois, Lucie Liger, Samuel Morin, Denis Petitprez, Alvaro Robledano, Martin Schneebeli, Pascal Salze, Delphine Six, Emmanuel Thibert, Jürg Trachsel, Matthieu Vernay, Léo Viallon-Galinier, and Céline Voiron
Earth Syst. Sci. Data, 15, 3075–3094, https://doi.org/10.5194/essd-15-3075-2023, https://doi.org/10.5194/essd-15-3075-2023, 2023
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Saharan dust outbreaks have profound effects on ecosystems, climate, health, and the cryosphere, but the spatial deposition pattern of Saharan dust is poorly known. Following the extreme dust deposition event of February 2021 across Europe, a citizen science campaign was launched to sample dust on snow over the Pyrenees and the European Alps. This campaign triggered wide interest and over 100 samples. The samples revealed the high variability of the dust properties within a single event.
Han Huang and Yi Huang
Earth Syst. Sci. Data, 15, 3001–3021, https://doi.org/10.5194/essd-15-3001-2023, https://doi.org/10.5194/essd-15-3001-2023, 2023
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We present a newly generated set of ERA5-based radiative kernels and compare them with other published kernels for the top of the atmosphere and surface radiation budgets. For both, the discrepancies in sensitivity values are generally of small magnitude, except for temperature kernels for the surface, likely due to improper treatment in the perturbation experiments used for kernel computation. The kernel bias is not a major cause of the inter-GCM (general circulation model) feedback spread.
Robert Pincus, Paul A. Hubanks, Steven Platnick, Kerry Meyer, Robert E. Holz, Denis Botambekov, and Casey J. Wall
Earth Syst. Sci. Data, 15, 2483–2497, https://doi.org/10.5194/essd-15-2483-2023, https://doi.org/10.5194/essd-15-2483-2023, 2023
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This paper describes a new global dataset of cloud properties observed by a specific satellite program created to facilitate comparison with a matching observational proxy used in climate models. Statistics are accumulated over daily and monthly timescales on an equal-angle grid. Statistics include cloud detection, cloud-top pressure, and cloud optical properties. Joint histograms of several variable pairs are also available.
Emma L. Yates, Laura T. Iraci, Susan S. Kulawik, Ju-Mee Ryoo, Josette E. Marrero, Caroline L. Parworth, Jason M. St. Clair, Thomas F. Hanisco, Thao Paul V. Bui, Cecilia S. Chang, and Jonathan M. Dean-Day
Earth Syst. Sci. Data, 15, 2375–2389, https://doi.org/10.5194/essd-15-2375-2023, https://doi.org/10.5194/essd-15-2375-2023, 2023
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The Alpha Jet Atmospheric eXperiment (AJAX) flew scientific flights between 2011 and 2018 providing measurements of carbon dioxide, methane, ozone, formaldehyde, water vapor and meteorological parameters over California and Nevada, USA. AJAX was a multi-year, multi-objective, multi-instrument program with a variety of sampling strategies resulting in an extensive dataset of interest to a wide variety of users. AJAX measurements have been published at https://asdc.larc.nasa.gov/project/AJAX.
Leïla Simon, Valérie Gros, Jean-Eudes Petit, François Truong, Roland Sarda-Estève, Carmen Kalalian, Alexia Baudic, Caroline Marchand, and Olivier Favez
Earth Syst. Sci. Data, 15, 1947–1968, https://doi.org/10.5194/essd-15-1947-2023, https://doi.org/10.5194/essd-15-1947-2023, 2023
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Long-term measurements of volatile organic compounds (VOCs) have been set up to better characterize the atmospheric chemistry at the SIRTA national facility (Paris area, France). Results obtained from the first 2 years (2020–2021) confirm the importance of local sources for short-lived compounds and the role played by meteorology and air mass origins in the long-term analysis of VOCs. They also point to a substantial influence of anthropogenic on the monoterpene loadings.
Ka Lok Chan, Pieter Valks, Klaus-Peter Heue, Ronny Lutz, Pascal Hedelt, Diego Loyola, Gaia Pinardi, Michel Van Roozendael, François Hendrick, Thomas Wagner, Vinod Kumar, Alkis Bais, Ankie Piters, Hitoshi Irie, Hisahiro Takashima, Yugo Kanaya, Yongjoo Choi, Kihong Park, Jihyo Chong, Alexander Cede, Udo Frieß, Andreas Richter, Jianzhong Ma, Nuria Benavent, Robert Holla, Oleg Postylyakov, Claudia Rivera Cárdenas, and Mark Wenig
Earth Syst. Sci. Data, 15, 1831–1870, https://doi.org/10.5194/essd-15-1831-2023, https://doi.org/10.5194/essd-15-1831-2023, 2023
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This paper presents the theoretical basis as well as verification and validation of the Global Ozone Monitoring Experiment-2 (GOME-2) daily and monthly level-3 products.
Kristina Collins, John Gibbons, Nathaniel Frissell, Aidan Montare, David Kazdan, Darren Kalmbach, David Swartz, Robert Benedict, Veronica Romanek, Rachel Boedicker, William Liles, William Engelke, David G. McGaw, James Farmer, Gary Mikitin, Joseph Hobart, George Kavanagh, and Shibaji Chakraborty
Earth Syst. Sci. Data, 15, 1403–1418, https://doi.org/10.5194/essd-15-1403-2023, https://doi.org/10.5194/essd-15-1403-2023, 2023
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This paper summarizes radio data collected by citizen scientists, which can be used to analyze the charged part of Earth's upper atmosphere. The data are collected from several independent stations. We show ways to look at the data from one station or multiple stations over different periods of time and how it can be combined with data from other sources as well. The code provided to make these visualizations will still work if some data are missing or when more data are added in the future.
Melisa Diaz Resquin, Pablo Lichtig, Diego Alessandrello, Marcelo De Oto, Darío Gómez, Cristina Rössler, Paula Castesana, and Laura Dawidowski
Earth Syst. Sci. Data, 15, 189–209, https://doi.org/10.5194/essd-15-189-2023, https://doi.org/10.5194/essd-15-189-2023, 2023
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We explored the performance of the random forest algorithm to predict CO, NOx, PM10, SO2, and O3 air quality concentrations and comparatively assessed the monitored and modeled concentrations during the COVID-19 lockdown phases. We provide the first long-term O3 and SO2 observational dataset for an urban–residential area of Buenos Aires in more than a decade and study the responses of O3 to the reduction in the emissions of its precursors because of its relevance regarding emission control.
Vitali E. Fioletov, Chris A. McLinden, Debora Griffin, Ihab Abboud, Nickolay Krotkov, Peter J. T. Leonard, Can Li, Joanna Joiner, Nicolas Theys, and Simon Carn
Earth Syst. Sci. Data, 15, 75–93, https://doi.org/10.5194/essd-15-75-2023, https://doi.org/10.5194/essd-15-75-2023, 2023
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Sulfur dioxide (SO2) measurements from three satellite instruments were used to update and extend the previously developed global catalogue of large SO2 emission sources. This version 2 of the global catalogue covers the period of 2005–2021 and includes a total of 759 continuously emitting point sources. The catalogue data show an approximate 50 % decline in global SO2 emissions between 2005 and 2021, although emissions were relatively stable during the last 3 years.
Jed O. Kaplan and Katie Hong-Kiu Lau
Earth Syst. Sci. Data, 14, 5665–5670, https://doi.org/10.5194/essd-14-5665-2022, https://doi.org/10.5194/essd-14-5665-2022, 2022
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Global lightning strokes are recorded continuously by a network of ground-based stations. We consolidated these point observations into a map form and provide these as electronic datasets for research purposes. Here we extend our dataset to include lightning observations from 2021.
Haris Rahadianto, Hirokazu Tatano, Masato Iguchi, Hiroshi L. Tanaka, Tetsuya Takemi, and Sudip Roy
Earth Syst. Sci. Data, 14, 5309–5332, https://doi.org/10.5194/essd-14-5309-2022, https://doi.org/10.5194/essd-14-5309-2022, 2022
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We simulated the Taisho (1914) eruption of Sakurajima volcano under various weather conditions to show how a similar eruption would affect contemporary Japan in a worst-case scenario. We provide the dataset of projected airborne ash concentration and deposit over all of Japan to support risk assessment and planning for disaster management. Our work extends previous analyses of local risks to cover distal locations in Japan where a large population could be exposed to devastating impacts.
Xiangyue Chen, Hongchao Zuo, Zipeng Zhang, Xiaoyi Cao, Jikai Duan, Chuanmei Zhu, Zhe Zhang, and Jingzhe Wang
Earth Syst. Sci. Data, 14, 5233–5252, https://doi.org/10.5194/essd-14-5233-2022, https://doi.org/10.5194/essd-14-5233-2022, 2022
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Arid and semi-arid areas are data-scarce aerosol areas. We provide path-breaking, high-resolution, full coverage, and long time series AOD datasets (FEC AOD) to support the atmosphere and related studies in northwestern China. The FEC AOD effectively compensates for the deficiency and constraints of in situ observations and satellite AOD products. Meanwhile, FEC AOD products demonstrate a reliable accuracy and ability to capture long-term change information.
Natalie Kaifler, Bernd Kaifler, Markus Rapp, and David C. Fritts
Earth Syst. Sci. Data, 14, 4923–4934, https://doi.org/10.5194/essd-14-4923-2022, https://doi.org/10.5194/essd-14-4923-2022, 2022
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We measured polar mesospheric clouds (PMCs), our Earth’s highest clouds at the edge of space, with a Rayleigh lidar from a stratospheric balloon. We describe how we derive the cloud’s brightness and discuss the stability of the gondola pointing and the sensitivity of our measurements. We present our high-resolution PMC dataset that is used to study dynamical processes in the upper mesosphere, e.g. regarding gravity waves, mesospheric bores, vortex rings, and Kelvin–Helmholtz instabilities.
Yi Cheng, Shaofei Kong, Liquan Yao, Huang Zheng, Jian Wu, Qin Yan, Shurui Zheng, Yao Hu, Zhenzhen Niu, Yingying Yan, Zhenxing Shen, Guofeng Shen, Dantong Liu, Shuxiao Wang, and Shihua Qi
Earth Syst. Sci. Data, 14, 4757–4775, https://doi.org/10.5194/essd-14-4757-2022, https://doi.org/10.5194/essd-14-4757-2022, 2022
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This work establishes the first emission inventory of carbonaceous aerosols from cooking, fireworks, sacrificial incense, joss paper burning, and barbecue, using multi-source datasets and tested emission factors. These emissions were concentrated in specific periods and areas. Positive and negative correlations between income and emissions were revealed in urban and rural regions. The dataset will be helpful for improving modeling studies and modifying corresponding emission control policies.
Qiang Cui, Yilin Lei, and Bin Chen
Earth Syst. Sci. Data, 14, 4419–4433, https://doi.org/10.5194/essd-14-4419-2022, https://doi.org/10.5194/essd-14-4419-2022, 2022
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This paper calculates the emissions of six kinds of emissions from China’s foreign routes from 2014 to 2019, enriching the existing database. This paper applies the improved BFFM2-FOA-FPM method and ICAO method to calculate the emissions, which can combine CO2 and non-CO2 emissions calculations and calculate the aircraft types' emission intensity.
Mengze Li, Andrea Pozzer, Jos Lelieveld, and Jonathan Williams
Earth Syst. Sci. Data, 14, 4351–4364, https://doi.org/10.5194/essd-14-4351-2022, https://doi.org/10.5194/essd-14-4351-2022, 2022
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We present a northern hemispheric airborne measurement dataset of atmospheric ethane, propane and methane and temporal trends for the time period 2006–2016 in the upper troposphere and lower stratosphere. The growth rates of ethane, methane, and propane in the upper troposphere are -2.24, 0.33, and -0.78 % yr-1, respectively, and in the lower stratosphere they are -3.27, 0.26, and -4.91 % yr-1, respectively, in 2006–2016.
Malika Menoud, Carina van der Veen, Dave Lowry, Julianne M. Fernandez, Semra Bakkaloglu, James L. France, Rebecca E. Fisher, Hossein Maazallahi, Mila Stanisavljević, Jarosław Nęcki, Katarina Vinkovic, Patryk Łakomiec, Janne Rinne, Piotr Korbeń, Martina Schmidt, Sara Defratyka, Camille Yver-Kwok, Truls Andersen, Huilin Chen, and Thomas Röckmann
Earth Syst. Sci. Data, 14, 4365–4386, https://doi.org/10.5194/essd-14-4365-2022, https://doi.org/10.5194/essd-14-4365-2022, 2022
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Emission sources of methane (CH4) can be distinguished with measurements of CH4 stable isotopes. We present new measurements of isotope signatures of various CH4 sources in Europe, mainly anthropogenic, sampled from 2017 to 2020. The present database also contains the most recent update of the global signature dataset from the literature. The dataset improves CH4 source attribution and the understanding of the global CH4 budget.
Patrick Hupe, Lars Ceranna, Alexis Le Pichon, Robin S. Matoza, and Pierrick Mialle
Earth Syst. Sci. Data, 14, 4201–4230, https://doi.org/10.5194/essd-14-4201-2022, https://doi.org/10.5194/essd-14-4201-2022, 2022
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Sound waves with frequencies below the human hearing threshold can travel long distances through the atmosphere. A global network of sensors records such infrasound to detect clandestine nuclear tests in the atmosphere. These data are generally not public. This study provides four data products based on global infrasound signal detections to make infrasound data available to a broad community. This will advance the use of infrasound observations for scientific studies and civilian applications.
Zexia Duan, Zhiqiu Gao, Qing Xu, Shaohui Zhou, Kai Qin, and Yuanjian Yang
Earth Syst. Sci. Data, 14, 4153–4169, https://doi.org/10.5194/essd-14-4153-2022, https://doi.org/10.5194/essd-14-4153-2022, 2022
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Land–atmosphere interactions over the Yangtze River Delta (YRD) in China are becoming more varied and complex, as the area is experiencing rapid land use changes. In this paper, we describe a dataset of microclimate and eddy covariance variables at four sites in the YRD. This dataset has potential use cases in multiple research fields, such as boundary layer parametrization schemes, evaluation of remote sensing algorithms, and development of climate models in typical East Asian monsoon regions.
Xiaoli Sun, Paul T. Kolbeck, James B. Abshire, Stephan R. Kawa, and Jianping Mao
Earth Syst. Sci. Data, 14, 3821–3833, https://doi.org/10.5194/essd-14-3821-2022, https://doi.org/10.5194/essd-14-3821-2022, 2022
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We describe the measurement and data processing of the atmospheric backscatter profile data by our CO2 Sounder lidar from the 2017 ASCENDS/ABoVE airborne campaign. It is an additional data set from the column average CO2 mixing ratio measurements from laser sounding. It not only helps to interpret the CO2 mixing ratio measurement but also give a standalone data set for atmosphere backscattering study at 1572 nm wavelength.
Lei Li, Yevgeny Derimian, Cheng Chen, Xindan Zhang, Huizheng Che, Gregory L. Schuster, David Fuertes, Pavel Litvinov, Tatyana Lapyonok, Anton Lopatin, Christian Matar, Fabrice Ducos, Yana Karol, Benjamin Torres, Ke Gui, Yu Zheng, Yuanxin Liang, Yadong Lei, Jibiao Zhu, Lei Zhang, Junting Zhong, Xiaoye Zhang, and Oleg Dubovik
Earth Syst. Sci. Data, 14, 3439–3469, https://doi.org/10.5194/essd-14-3439-2022, https://doi.org/10.5194/essd-14-3439-2022, 2022
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A climatology of aerosol composition concentration derived from POLDER-3 observations using GRASP/Component is presented. The conceptual specifics of the GRASP/Component approach are in the direct retrieval of aerosol speciation without intermediate retrievals of aerosol optical characteristics. The dataset of satellite-derived components represents scarce but imperative information for validation and potential adjustment of chemical transport models.
Fei Jiang, Weimin Ju, Wei He, Mousong Wu, Hengmao Wang, Jun Wang, Mengwei Jia, Shuzhuang Feng, Lingyu Zhang, and Jing M. Chen
Earth Syst. Sci. Data, 14, 3013–3037, https://doi.org/10.5194/essd-14-3013-2022, https://doi.org/10.5194/essd-14-3013-2022, 2022
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A 10-year (2010–2019) global monthly terrestrial NEE dataset (GCAS2021) was inferred from the GOSAT ACOS v9 XCO2 product. It shows strong carbon sinks over eastern N. America, the Amazon, the Congo Basin, Europe, boreal forests, southern China, and Southeast Asia. It has good quality and can reflect the impacts of extreme climates and large-scale climate anomalies on carbon fluxes well. We believe that this dataset can contribute to regional carbon budget assessment and carbon dynamics research.
Cited articles
Bai, K., Li, K., Ma, M., Li, K., Li, Z., Guo, J., Chang, N.-B., Tan, Z., and Han, D.: LGHAP: the Long-term Gap-free High-resolution Air Pollutant concentration dataset, derived via tensor-flow-based multimodal data fusion, Earth Syst. Sci. Data, 14, 907–927, https://doi.org/10.5194/essd-14-907-2022, 2022.
Beelen, R., Hoek, G., Den Brandt, P. A. V., Goldbohm, R. A., Fischer, P.,
Schouten, L. J., Jerrett, M., Hughes, E., Armstrong, B., and Brunekreef, B.:
Long-term effects of traffic-related air pollution on mortality in a Dutch
cohort (NLCS-AIR study), Environ. Health Persp., 116, 196–202,
2007.
Chen, H., Huang, Y., Shen, H., Chen, Y., Ru, M., Chen, Y., Lin, N., Su, S.,
Zhuo, S., Zhong, Q., Wang, X., Liu, J., Li, B., and Tao, S.: Modeling
temporal variations in global residential energy consumption and pollutant
emissions, Appl. Energ., 184, 820–829, https://doi.org/10.1016/j.apenergy.2015.10.185, 2016.
Chen, J., Yin, J., Zang, L., Zhang, T., and Zhao, M.: Stacking machine
learning model for estimating hourly PM2.5 in China based on Himawari 8
aerosol optical depth data, Sci. Total Environ., 697, 134021,
https://doi.org/10.1016/j.scitotenv.2019.134021, 2019.
Chen, X., Zhang, L. W., Huang, J. J., Song, F. J., Zhang, L. P., Qian, Z.
M., Trevathan, E., Mao, H. J., Han, B., Vaughn, M., Chen, K. X., Liu, Y. M.,
Chen, J., Zhao, B. X., Jiang, G. H., Gu, Q., Bai, Z. P., Dong, G. H., and
Tang, N. J.: Long-term exposure to urban air pollution and lung cancer
mortality: A 12-year cohort study in Northern China, Sci. Total
Environ., 571, 855–861, https://doi.org/10.1016/j.scitotenv.2016.07.064, 2016.
CMA: Forecasting and Networking Department of China Meteorological
Administration released letter No.4: Notice on the adjustments of the haze
weather phenomenon observation and on the revision of the fog and haze
observation data, China Meteorological Administration (CMA), 2014.
Ervens, B., Turpin, B. J., and Weber, R. J.: Secondary organic aerosol formation in cloud droplets and aqueous particles (aqSOA): a review of laboratory, field and model studies, Atmos. Chem. Phys., 11, 11069–11102, https://doi.org/10.5194/acp-11-11069-2011, 2011.
Fang, X., Zou, B., Liu, X., Sternberg, T., and Zhai, L.: Satellite-based
ground PM2.5 estimation using timely structure adaptive modeling, Remote
Sens. Environ., 186, 152-163, https://doi.org/10.1016/j.rse.2016.08.027, 2016.
Gelaro, R., McCarty, W., Suárez, M. J., Todling, R., Molod, A., Takacs,
L., Randles, C. A., Darmenov, A., Bosilovich, M. G., and Reichle, R.: The
modern-era retrospective analysis for research and applications, version 2
(MERRA-2), J. Climate, 30, 5419–5454, 2017.
Geng, G., Xiao, Q., Liu, S., Liu, X., Cheng, J., Zheng, Y., Xue, T., Tong,
D., Zheng, B., Peng, Y., Huang, X., He, K., and Zhang, Q.: Tracking Air
Pollution in China: Near Real-Time PM2.5 Retrievals from Multisource Data
Fusion, Environ. Sci. Technol., 55, 12106–12115,
https://doi.org/10.1021/acs.est.1c01863, 2021.
Gui, K., Che, H., Zeng, Z., Wang, Y., Zhai, S., Wang, Z., Luo, M., Zhang,
L., Liao, T., Zhao, H., Li, L., Zheng, Y., and Zhang, X.: Construction of a
virtual PM2.5 observation network in China based on high-density surface
meteorological observations using the Extreme Gradient Boosting model,
Environ. Int., 141, 105801, https://doi.org/10.1016/j.envint.2020.105801, 2020.
Huang, C., Hu, J., Xue, T., Xu, H., and Wang, M.: High-Resolution
Spatiotemporal Modeling for Ambient PM2.5 Exposure Assessment in China from
2013 to 2019, Environ. Sci. Technol., 55, 2152–2162,
https://doi.org/10.1021/acs.est.0c05815, 2021.
Huang, Y., Shen, H., Chen, H., Wang, R., Zhang, Y., Su, S., Chen, Y., Lin,
N., Zhuo, S., Zhong, Q., Wang, X., Liu, J., Li, B., Liu, W., and Tao, S.:
Quantification of Global Primary Emissions of PM2.5, PM10, and TSP from
Combustion and Industrial Process Sources, Environ. Sci.
Technol., 48, 13834–13843, https://doi.org/10.1021/es503696k, 2014.
Huang, Y., Shen, H., Chen, Y., Zhong, Q., Chen, H., Wang, R., Shen, G., Liu,
J., Li, B., and Tao, S.: Global organic carbon emissions from primary
sources from 1960 to 2009, Atmos. Environ., 122, 505–512, https://doi.org/10.1016/j.atmosenv.2015.10.017, 2015.
Inness, A., Ades, M., Agustí-Panareda, A., Barré, J., Benedictow, A., Blechschmidt, A.-M., Dominguez, J. J., Engelen, R., Eskes, H., Flemming, J., Huijnen, V., Jones, L., Kipling, Z., Massart, S., Parrington, M., Peuch, V.-H., Razinger, M., Remy, S., Schulz, M., and Suttie, M.: The CAMS reanalysis of atmospheric composition, Atmos. Chem. Phys., 19, 3515–3556, https://doi.org/10.5194/acp-19-3515-2019, 2019.
Ke, G., Meng, Q., Finley, T., Wang, T., Chen, W., Ma, W., Ye, Q., and Liu,
T.-Y.: Lightgbm: A highly efficient gradient boosting decision tree,
Adv. Neural In., 3146–3154, 2017.
Kuang, Y., Zhao, C., Tao, J., Bian, Y., and Ma, N. J.: Impact of
aerosol hygroscopic growth on the direct aerosol radiative effect in summer
on North China Plain, Atmos. Environ., 147, 224–233, https://doi.org/10.1016/j.atmosenv.2016.10.013, 2016.
Liang, F., Xiao, Q., Huang, K., Yang, X., Liu, F., Li, J., Lu, X., Liu, Y.,
and Gu, D.: The 17-y spatiotemporal trend of PM2.5 and its mortality burden in China, P. Natl. Acad. Sci. USA, 117, 25601–25608,
https://doi.org/10.1073/pnas.1919641117, 2020.
Liu, M., Bi, J., and Ma, Z.: Visibility-Based PM2.5 Concentrations in China:
1957–1964 and 1973–2014, Environ. Sci. Technol., 51,
13161–13169, https://doi.org/10.1021/acs.est.7b03468, 2017.
Lynch, P., Reid, J. S., Westphal, D. L., Zhang, J., Hogan, T. F., Hyer, E. J., Curtis, C. A., Hegg, D. A., Shi, Y., Campbell, J. R., Rubin, J. I., Sessions, W. R., Turk, F. J., and Walker, A. L.: An 11-year global gridded aerosol optical thickness reanalysis (v1.0) for atmospheric and climate sciences, Geosci. Model Dev., 9, 1489–1522, https://doi.org/10.5194/gmd-9-1489-2016, 2016.
Ma, Z., Hu, X., Sayer, A. M., Levy, R., Zhang, Q., Xue, Y., Tong, S., Bi,
J., Huang, L., and Liu, Y.: Satellite-Based Spatiotemporal Trends in PM2.5
Concentrations: China, 2004–2013, Environ. Health Persp., 124,
184–192, https://doi.org/10.1289/ehp.1409481, 2016.
Pilinis, C., Seinfeld, J. H., and Grosjean, D.: Water content of atmospheric
aerosols, Atmos. Environ., 23, 1601–1606,
https://doi.org/10.1016/0004-6981(89)90419-8, 1989.
Pope, C. A., Burnett, R. T., Thun, M. J., Calle, E. E., Krewski, D., Ito,
K., and Thurston, G. D.: Lung cancer, cardiopulmonary mortality, and
long-term exposure to fine particulate air pollution, J.
Am. Medical Assoc., 287, 1132–1141, 2002.
Randles, C., Da Silva, A., Buchard, V., Colarco, P., Darmenov, A.,
Govindaraju, R., Smirnov, A., Holben, B., Ferrare, R., and Hair, J.: The
MERRA-2 aerosol reanalysis, 1980 onward. Part I: System description and data
assimilation evaluation, J. Climate, 30, 6823–6850, 2017.
van Donkelaar, A., Hammer, M. S., Bindle, L., Brauer, M., Brook, J. R.,
Garay, M. J., Hsu, N. C., Kalashnikova, O. V., Kahn, R. A., Lee, C., Levy,
R. C., Lyapustin, A., Sayer, A. M., and Martin, R. V.: Monthly Global
Estimates of Fine Particulate Matter and Their Uncertainty, Environ.
Sci. Technol., 55, 15287–15300, https://doi.org/10.1021/acs.est.1c05309, 2021.
Wang, B., Yuan, Q., Yang, Q., Zhu, L., Li, T., and Zhang, L.: Estimate
hourly PM2.5 concentrations from Himawari-8 TOA reflectance directly using
geo-intelligent long short-term memory network, Environ. Pollut.,
271, 116327, https://doi.org/10.1016/j.envpol.2020.116327,
2021.
Wang, R., Tao, S., Shen, H., Huang, Y., Chen, H., Balkanski, Y., Boucher,
O., Ciais, P., Shen, G., Li, W., Zhang, Y., Chen, Y., Lin, N., Su, S., Li,
B., Liu, J., and Liu, W.: Trend in Global Black Carbon Emissions from 1960
to 2007, Environ. Sci. Technol., 48, 6780–6787,
https://doi.org/10.1021/es5021422, 2014.
Wang, X., Dickinson, R. E., Su, L., Zhou, C., and Wang, K.: PM2.5 Pollution
in China and How It Has Been Exacerbated by Terrain and Meteorological
Conditions, B. Am. Meteorol. Soc., 99, 105–119,
https://doi.org/10.1175/bams-d-16-0301.1, 2018.
Wang, X., Zhang, R., and Yu, W.: The Effects of PM2.5 Concentrations and
Relative Humidity on Atmospheric Visibility in Beijing, J.
Geophys. Res.-Atmos., 124, 2235–2259, https://doi.org/10.1029/2018JD029269, 2019.
Wei, J., Li, Z., Lyapustin, A., Sun, L., Peng, Y., Xue, W., Su, T., and
Cribb, M.: Reconstructing 1-km-resolution high-quality PM2.5 data records
from 2000 to 2018 in China: spatiotemporal variations and policy
implications, Remote Sens. Environ., 252, 112136, https://doi.org/10.1016/j.rse.2020.112136, 2021a.
Wei, J., Li, Z., Pinker, R. T., Wang, J., Sun, L., Xue, W., Li, R., and Cribb, M.: Himawari-8-derived diurnal variations in ground-level PM2.5 pollution across China using the fast space-time Light Gradient Boosting Machine (LightGBM), Atmos. Chem. Phys., 21, 7863–7880, https://doi.org/10.5194/acp-21-7863-2021, 2021b.
Xiao, Q., Chang, H. H., Geng, G., and Liu, Y.: An Ensemble Machine-Learning
Model To Predict Historical PM2.5 Concentrations in China from Satellite
Data, Environ. Sci. Technol., 52, 13260–13269,
https://doi.org/10.1021/acs.est.8b02917, 2018.
Xue, T., Zheng, Y., Tong, D., Zheng, B., Li, X., Zhu, T., and Zhang, Q.:
Spatiotemporal continuous estimates of PM2.5 concentrations in China,
2000–2016: A machine learning method with inputs from satellites, chemical
transport model, and ground observations, Environ. Int., 123,
345–357, https://doi.org/10.1016/j.envint.2018.11.075, 2019.
Yan, X., Zang, Z., Luo, N., Jiang, Y., and Li, Z.: New interpretable deep
learning model to monitor real-time PM2.5 concentrations from satellite
data, Environ. Int., 144, 106060, https://doi.org/10.1016/j.envint.2020.106060, 2020.
Yumimoto, K., Tanaka, T. Y., Oshima, N., and Maki, T.: JRAero: the Japanese Reanalysis for Aerosol v1.0, Geosci. Model Dev., 10, 3225–3253, https://doi.org/10.5194/gmd-10-3225-2017, 2017.
Zhang, H. L., Wang, Y. G., Hu, J. L., Ying, Q., and Hu, X. M.: Relationships
between meteorological parameters and criteria air pollutants in three
megacities in China, Environ. Res., 140, 242–254,
https://doi.org/10.1016/j.envres.2015.04.004, 2015.
Zhang, Q., Streets, D. G., Carmichael, G. R., He, K. B., Huo, H., Kannari, A., Klimont, Z., Park, I. S., Reddy, S., Fu, J. S., Chen, D., Duan, L., Lei, Y., Wang, L. T., and Yao, Z. L.: Asian emissions in 2006 for the NASA INTEX-B mission, Atmos. Chem. Phys., 9, 5131–5153, https://doi.org/10.5194/acp-9-5131-2009, 2009.
Zhang, R., Li, Q., and Zhang, R.: Meteorological conditions for the
persistent severe fog and haze event over eastern China in January 2013,
Sci. China Earth Sci., 57, 26–35, https://doi.org/10.1007/s11430-013-4774-3, 2013a.
Zhang, X., Sun, J., Wang, Y., Li, W., Zhang, Q., Wang, W., Quan, J., Cao,
G., Wang, J., Yang, Y., and Zhang, Y.: Factors contributing to haze and fog
in China, Chinese Sci. B., 58, 1178, https://doi.org/10.1360/972013-150, 2013b.
Zheng, B., Tong, D., Li, M., Liu, F., Hong, C., Geng, G., Li, H., Li, X., Peng, L., Qi, J., Yan, L., Zhang, Y., Zhao, H., Zheng, Y., He, K., and Zhang, Q.: Trends in China's anthropogenic emissions since 2010 as the consequence of clean air actions, Atmos. Chem. Phys., 18, 14095–14111, https://doi.org/10.5194/acp-18-14095-2018, 2018.
Zheng, B., Cheng, J., Geng, G., Wang, X., Li, M., Shi, Q., Qi, J., Lei, Y.,
Zhang, Q., and He, K.: Mapping anthropogenic emissions in China at 1 km
spatial resolution and its application in air quality modeling, Sci.
Bull., 66, 612–620, https://doi.org/10.1016/j.scib.2020.12.008, 2021.
Zhong, J., Zhang, X., Wang, Y., Sun, J., Zhang, Y., Wang, J., Tan, K., Shen,
X., Che, H., and Zhang, L.: Relative contributions of boundary-layer
meteorological factors to the explosive growth of PM2.5 during the red-alert
heavy pollution episodes in Beijing in December 2016, J.
Meteorol. Res., 31, 809–819, https://doi.org/10.1007/s13351-017-7088-0, 2017.
Zhong, J., Zhang, X., Dong, Y., Wang, Y., Liu, C., Wang, J., Zhang, Y., and Che, H.: Feedback effects of boundary-layer meteorological factors on cumulative explosive growth of PM2.5 during winter heavy pollution episodes in Beijing from 2013 to 2016, Atmos. Chem. Phys., 18, 247–258, https://doi.org/10.5194/acp-18-247-2018, 2018.
Zhong, J., Zhang, X., Gui, K., Wang, Y., Che, H., Shen, X., Zhang, L.,
Zhang, Y., Sun, J., and Zhang, W.: Robust prediction of hourly PM2.5 from
meteorological data using LightGBM, National Sci. Rev., 8, nwaa307,
https://doi.org/10.1093/nsr/nwaa307, 2021.
Zhong, J., Zhang, X., Gui, K., Liao, J., Fei, Y., Jiang, L., Guo, L., Liu,
L., Che, H., Wang, Y., Wang, D., and Zhou, Z.: Reconstructing 6-hourly PM2.5
datasets from 1960 to 2020 in China, Zenodo [data set], https://doi.org/10.5281/zenodo.6372847, 2022.
Zhou, Z. and Zhang, G.: Typical severe dust storms in northern China during
1954–2002, Chinese Sci. B., 48, 2366–2370, 2003.
Zhu, W., Xu, X., Zheng, J., Yan, P., Wang, Y., and Cai, W.: The
characteristics of abnormal wintertime pollution events in the Jing-Jin-Ji
region and its relationships with meteorological factors, Sci.
Total Environ., 626, 887–898, 2018.
Short summary
Historical long-term PM2.5 records with high temporal resolution are essential but lacking for research and environmental management. Here, we reconstruct site-based and gridded PM2.5 datasets at 6-hour intervals from 1960 to 2020 that combine visibility, meteorological data, and emissions based on a machine learning model with extracted spatial features. These two PM2.5 datasets will lay the foundation of research studies associated with air pollution, climate change, and aerosol reanalysis.
Historical long-term PM2.5 records with high temporal resolution are essential but lacking for...
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