Articles | Volume 16, issue 8
https://doi.org/10.5194/essd-16-3781-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/essd-16-3781-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Retrieving ground-level PM2.5 concentrations in China (2013–2021) with a numerical-model-informed testbed to mitigate sample-imbalance-induced biases
Siwei Li
CORRESPONDING AUTHOR
Hubei Key Laboratory of Quantitative Remote Sensing of Land and Atmosphere, School of Remote Sensing and Information Engineering, Wuhan University, Hubei 430000, China
State Key Laboratory of Information Engineering in Surveying, Mapping and Remote Sensing, Wuhan University, Wuhan 430079, China
Hubei Luojia Laboratory, Wuhan University, Wuhan 430079, China
Yu Ding
Hubei Key Laboratory of Quantitative Remote Sensing of Land and Atmosphere, School of Remote Sensing and Information Engineering, Wuhan University, Hubei 430000, China
Jia Xing
CORRESPONDING AUTHOR
Department of Civil and Environmental Engineering, the University of Tennessee, Knoxville, TN 37996, USA
Joshua S. Fu
Department of Civil and Environmental Engineering, the University of Tennessee, Knoxville, TN 37996, USA
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Accurate estimation of emissions is a prerequisite for effectively controlling air pollution, but current methods lack either sufficient data or a representation of nonlinearity. Here, we proposed a novel deep learning method to model the dual relationship between emissions and pollutant concentrations. Emissions can be updated by back-propagating the gradient of the loss function measuring the deviation between simulations and observations, resulting in better model performance.
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Victoria A. Flood, Kimberly Strong, Cynthia H. Whaley, Kaley A. Walker, Thomas Blumenstock, James W. Hannigan, Johan Mellqvist, Justus Notholt, Mathias Palm, Amelie N. Röhling, Stephen Arnold, Stephen Beagley, Rong-You Chien, Jesper Christensen, Makoto Deushi, Srdjan Dobricic, Xinyi Dong, Joshua S. Fu, Michael Gauss, Wanmin Gong, Joakim Langner, Kathy S. Law, Louis Marelle, Tatsuo Onishi, Naga Oshima, David A. Plummer, Luca Pozzoli, Jean-Christophe Raut, Manu A. Thomas, Svetlana Tsyro, and Steven Turnock
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Hannah J. Rubin, Joshua S. Fu, Frank Dentener, Rui Li, Kan Huang, and Hongbo Fu
Atmos. Chem. Phys., 23, 7091–7102, https://doi.org/10.5194/acp-23-7091-2023, https://doi.org/10.5194/acp-23-7091-2023, 2023
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We update the 2010 global deposition budget for nitrogen (N) and sulfur (S) with new regional wet deposition measurements, improving the ensemble results of 11 global chemistry transport models from HTAP II. Our study demonstrates that a global measurement–model fusion approach can substantially improve N and S deposition model estimates at a regional scale and represents a step forward toward the WMO goal of global fusion products for accurately mapping harmful air pollution.
Cynthia H. Whaley, Kathy S. Law, Jens Liengaard Hjorth, Henrik Skov, Stephen R. Arnold, Joakim Langner, Jakob Boyd Pernov, Garance Bergeron, Ilann Bourgeois, Jesper H. Christensen, Rong-You Chien, Makoto Deushi, Xinyi Dong, Peter Effertz, Gregory Faluvegi, Mark Flanner, Joshua S. Fu, Michael Gauss, Greg Huey, Ulas Im, Rigel Kivi, Louis Marelle, Tatsuo Onishi, Naga Oshima, Irina Petropavlovskikh, Jeff Peischl, David A. Plummer, Luca Pozzoli, Jean-Christophe Raut, Tom Ryerson, Ragnhild Skeie, Sverre Solberg, Manu A. Thomas, Chelsea Thompson, Kostas Tsigaridis, Svetlana Tsyro, Steven T. Turnock, Knut von Salzen, and David W. Tarasick
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Maggie Chel-Gee Ooi, Ming-Tung Chuang, Joshua S. Fu, Steven S. Kong, Wei-Syun Huang, Sheng-Hsiang Wang, Sittichai Pimonsree, Andy Chan, Shantanu Kumar Pani, and Neng-Huei Lin
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Lin Huang, Song Liu, Zeyuan Yang, Jia Xing, Jia Zhang, Jiang Bian, Siwei Li, Shovan Kumar Sahu, Shuxiao Wang, and Tie-Yan Liu
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Syuichi Itahashi, Baozhu Ge, Keiichi Sato, Zhe Wang, Junichi Kurokawa, Jiani Tan, Kan Huang, Joshua S. Fu, Xuemei Wang, Kazuyo Yamaji, Tatsuya Nagashima, Jie Li, Mizuo Kajino, Gregory R. Carmichael, and Zifa Wang
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Na Zhao, Xinyi Dong, Kan Huang, Joshua S. Fu, Marianne Tronstad Lund, Kengo Sudo, Daven Henze, Tom Kucsera, Yun Fat Lam, Mian Chin, and Simone Tilmes
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Black carbon acts as a strong climate forcer, especially in vulnerable pristine regions such as the Arctic. This work utilizes ensemble modeling results from the task force Hemispheric Transport of Air Pollution Phase 2 to investigate the responses of Arctic black carbon and surface temperature to various source emission reductions. East Asia contributed the most to Arctic black carbon. The response of Arctic temperature to black carbon was substantially more sensitive than the global average.
Ling Huang, Yonghui Zhu, Hehe Zhai, Shuhui Xue, Tianyi Zhu, Yun Shao, Ziyi Liu, Chris Emery, Greg Yarwood, Yangjun Wang, Joshua Fu, Kun Zhang, and Li Li
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Numerical air quality models (AQMs) are being applied extensively to address diverse scientific and regulatory compliance associated with deteriorating air quality in China. For any AQM applications, model performance evaluation is a critical step that guarantees the robustness and reliability of the baseline modeling results and subsequent applications. We provided benchmarks for model performance evaluation of AQM applications in China to demonstrate model robustness.
Ming-Tung Chuang, Maggie Chel Gee Ooi, Neng-Huei Lin, Joshua S. Fu, Chung-Te Lee, Sheng-Hsiang Wang, Ming-Cheng Yen, Steven Soon-Kai Kong, and Wei-Syun Huang
Atmos. Chem. Phys., 20, 14947–14967, https://doi.org/10.5194/acp-20-14947-2020, https://doi.org/10.5194/acp-20-14947-2020, 2020
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This study evaluated the impact of Asian haze from the three biggest industrial regions on Taiwan and analyzed the process during transport. The production and removal process revealed the mechanisms of long-range transport. This is the first time that the brute force method and process analysis technique has been applied in a Community Multiscale Air Quality Modeling System. Also, this study simulated the interesting transboundary transport of pollutants from southern mainland China to Taiwan.
Hajime Akimoto, Tatsuya Nagashima, Natsumi Kawano, Li Jie, Joshua S. Fu, and Zifa Wang
Atmos. Chem. Phys., 20, 15003–15014, https://doi.org/10.5194/acp-20-15003-2020, https://doi.org/10.5194/acp-20-15003-2020, 2020
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In order to perform proper model simulation of ozone near the ground in the coastal area of northeastern Asia, it has been found that it is very important to select appropriate dry deposition velocities of ozone on the oceanic water of specific area of the northwestern Pacific. Empirical measurement of the mixing ratios and dry deposition flux of ozone over the ocean in this area is highly recommended.
Jia Xing, Siwei Li, Yueqi Jiang, Shuxiao Wang, Dian Ding, Zhaoxin Dong, Yun Zhu, and Jiming Hao
Atmos. Chem. Phys., 20, 14347–14359, https://doi.org/10.5194/acp-20-14347-2020, https://doi.org/10.5194/acp-20-14347-2020, 2020
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Quantifying emission changes is a prerequisite for assessment of control effectiveness in improving air quality. However, traditional bottom-up methods usually take months to perform and limit timely assessments. A novel method was developed by using a response model that provides real-time estimation of emission changes based on air quality observations. It was successfully applied to quantify emission changes on the North China Plain due to the COVID-19 pandemic shutdown.
Cited articles
Appel, K. W., Pouliot, G. A., Simon, H., Sarwar, G., Pye, H. O. T., Napelenok, S. L., Akhtar, F., and Roselle, S. J.: Evaluation of dust and trace metal estimates from the Community Multiscale Air Quality (CMAQ) model version 5.0, Geosci. Model Dev., 6, 883–899, https://doi.org/10.5194/gmd-6-883-2013, 2013.
Appel, K. W., Napelenok, S., Hogrefe, C., Pouliot, G., Foley, K. M., Roselle, S. J., Pleim, J., Bash, J., Pye, H. O. T., Heath, N., Murphy, B., and Mathur, R.: Overview and evaluation of the community multiscale air quality (CMAQ) modeling system version 5.2, in: Air Pollution Modeling and its Application XXV 35, Springer International Publishing, 69–73, https://doi.org/10.1007/978-3-319-57645-9_11, 2018.
Bai, K., Li, K., Guo, J., and Chang, N. B.: Multiscale and multisource data fusion for full-coverage PM2.5 concentration mapping: Can spatial pattern recognition come with modeling accuracy? ISPRS J. Photogramm., 184, 31–44, 2022.
Belgiu, M. and Drăguţ, L.: Random forest in remote sensing: A review of applications and future directions, ISPRS J. Photogramm., 114, 24–31, 2016.
Bellouin, N., Boucher, O., Haywood, J., and Reddy, M. S.: Global estimate of aerosol direct radiative forcing from satellite measurements. Nature, 438, 1138–1141, 2005.
Celarier, E. A., Brinksma, E. J., Gleason, J. F., Veefkind, J. P., Cede, A., Herman, J. R., Ionov, D., Goutail, F., Pommereau, J.-P., Lambert, J.-C., van Roozendael, M., Pinardi, G., Wittrock, F., Schönhardt, A., Richter, A., Ibrahim, O.W., Wagner, T., Bojkov, B., Mount, G., Spinei, E., Chen, C. M., Pongetti, T. J., Sander, S. P., Bucsela, E. J., Wenig, M. O., Swart, D. P. J., Volten, H., Kroon, M., and Levelt, P. F.: Validation of Ozone Monitoring Instrument nitrogen dioxide columns, J. Geophys. Res.-Atmos., 113, D15S15, https://doi.org/10.1029/2007JD008908, 2008.
Chen, D., Guo, H., Gu, X., Cheng, T., Yang, J., Zhan, Y., and Wei, X.: A spatial-neighborhood deep neural network model for PM2.5 estimation across China, IEEE T. Geosci. Remote, 61, 4105815, https://doi.org/10.1109/TGRS.2023.3317905, 2023.
Chen, T. and Guestrin, C.: XGBoost: A scalable tree boosting system, in: Proceedings of the 22nd acm sigkdd international conference on knowledge discovery and data mining, San Francisco, CA, USA, 13–17 August 2016, 785–794, https://doi.org/10.1145/2939672.2939785, 2016.
Ding, D., Xing, J., Wang, S., Chang, X., and Hao, J.: Impacts of emissions and meteorological changes on China's ozone pollution in the warm seasons of 2013 and 2017, Front. Environ. Sci. Eng., 13, 76, https://doi.org/10.1007/s11783-019-1160-1, 2019a.
Ding, D., Xing, J., Wang, S., Liu, K., and Hao, J.: Estimated Contributions of Emissions Controls, Meteorological Factors, Population Growth, and Changes in Baseline Mortality to Reductions in Ambient PM2.5 and PM2.5-Related Mortality in China, 2013–2017, Environ. Health Persp., 127, 67009, https://doi.org/10.1289/EHP4157, 2019b.
Ding, Y., Li, S., Xing, J., Li, X., Ma, X., Song, G., Teng, M., Yang, J., Dong, J., and Meng, S.: Retrieving hourly seamless PM2.5 concentration across China with physically informed spatiotemporal connection. Remote Sens. Environ., 301, 113901, https://doi.org/10.1016/j.rse.2023.113901, 2024.
Dong, L., Li, S., Yang, J., Shi, W., and Zhang, L.: Investigating the performance of satellite-based models in estimating the surface PM2.5 over China, Chemosphere, 256, 127051, https://doi.org/10.1016/j.chemosphere.2020.127051, 2020.
Guenther, A. B., Jiang, X., Heald, C. L., Sakulyanontvittaya, T., Duhl, T., Emmons, L. K., and Wang, X.: The Model of Emissions of Gases and Aerosols from Nature version 2.1 (MEGAN2.1): an extended and updated framework for modeling biogenic emissions, Geosci. Model Dev., 5, 1471–1492, https://doi.org/10.5194/gmd-5-1471-2012, 2012.
He, K., Zhang, X., Ren, S., and Sun, J.: Deep residual learning for image recognition, in: Proceedings of the IEEE conference on computer vision and pattern recognition, Las Vegas, Nevada, USA, 26 June–1 July 2016, 770–778, https://doi.org/10.48550/arXiv.1512.03385, 2016.
He, Q., Qin, K., Cohen, J. B., Loyola, D., Li, D., Shi, J., and Xue, Y.: Spatially and temporally coherent reconstruction of tropospheric NO2 over China combining OMI and GOME-2B measurements, Environ. Res. Lett., 15, 125011, https://doi.org/10.1088/1748-9326/abc7df, 2020.
Hoff, R. M. and Christopher, S. A.: Remote sensing of particulate pollution from space: have we reached the promised land?, J. Air Waste Manage., 59, 645–675, 2009.
Hu, X., Belle, J. H., Meng, X., Wildani, A., Waller, L. A., Strickland, M. J., and Liu, Y.: Estimating PM2.5 concentrations in the conterminous United States using the random forest approach, Environ. Sci. Technol., 51, 6936–6944, 2017.
Ke, G., Meng, Q., Finley, T., Wang, T., Chen, W., Ma, W., Ye, Q., and Liu, T. Y.: Lightgbm: A highly efficient gradient boosting decision tree, in: 31st Conference on Neural Information Processing Systems (NIPS 2017), Long Beach, CA, 2017, 12.4–12.9, USA3149 – 3157, https://dl.acm.org/doi/10.5555/3294996.3295074 (last access: 24 August 2024), 2017.
Kingma, D. P. and Ba, J.: Adam: A method for stochastic optimization, arXiv [preprint], https://doi.org/10.48550/arXiv.1412.6980, 2014.
Kong, L., Tang, X., Zhu, J., Wang, Z., Li, J., Wu, H., Wu, Q., Chen, H., Zhu, L., Wang, W., Liu, B., Wang, Q., Chen, D., Pan, Y., Song, T., Li, F., Zheng, H., Jia, G., Lu, M., Wu, L., and Carmichael, G. R.: A 6-year-long (2013–2018) high-resolution air quality reanalysis dataset in China based on the assimilation of surface observations from CNEMC, Earth Syst. Sci. Data, 13, 529–570, https://doi.org/10.5194/essd-13-529-2021, 2021.
Lelieveld, J., Evans, J. S., Fnais, M., Giannadaki, D., and Pozzer, A.: The contribution of outdoor air pollution sources to premature mortality on a global scale, Nature, 525, 367–371, 2015.
Li, S. and Xing, J.: DeepSAT4D: Deep learning empowers four-dimensional atmospheric chemical concentration and emission retrieval from satellite, The Innovation Geoscience, 2, 100061-1, https://doi.org/10.59717/j.xinn-geo.2024.100061, 2024.
Li, S., Ding, Y., Xing, J., and Fu, J.: Numerical model-informed testbed for surface PM2.5 concentration over China and its estimates during 2013–2021, Zenodo [code and data set], https://doi.org/10.5281/zenodo.11122294, 2024a.
Li, S., Ding, Y., Xing, J., and Fu, J.: Numerical model-informed testbed for surface PM2.5 concentration over China and its estimates during 2013–2021 Zenodo [data set], https://doi.org/10.5281/zenodo.12636976, 2024b.
Li, T., Shen, H., Yuan, Q., and Zhang, L.: Geographically and temporally weighted neural networks for satellite-based mapping of ground-level PM2.5. ISPRS J. Photogramm., 167, 178–188, 2020.
Lin, H., Li, S., Xing, J., He, T., Yang, J., and Wang, Q.: High resolution aerosol optical depth retrieval over urban areas from Landsat-8 OLI images, Atmos. Environ., 261, 118591, https://doi.org/10.1016/j.atmosenv.2021.118591, 2021.
Liu, X. H., Zhang, Y., Cheng, S. H., Xing, J., Zhang, Q., Streets, D. G., Jang, C., Wang W., and Hao, J. M.: Understanding of regional air pollution over China using CMAQ, part I performance evaluation and seasonal variation, Atmos. Environ., 44, 2415–2426, 2010.
Ma, Z., Dey, S., Christopher, S., Liu, R., Bi, J., Balyan, P., and Liu, Y.: A review of statistical methods used for developing large-scale and long-term PM2.5 models from satellite data, Remote Sens. Environ., 269, 112827, https://doi.org/10.1016/j.rse.2021.112827, 2022.
Martin, R. V., Jacob, D. J., Chance, K., Kurosu, T. P., Palmer, P. I., and Evans, M. J.: Global inventory of nitrogen oxide emissions constrained by space-based observations of NO2 columns, J. Geophys. Res.-Atmos., 108, 4537, https://doi.org/10.1029/2003JD003453, 2003.
Remer, L. A., Kleidman, R. G., Levy, R. C., Kaufman, Y. J., Tanré, D., Mattoo, S., Martins, J. V., Ichoku, C., Koren, I., Yu, H., and Holben, B. N.: Global aerosol climatology from the MODIS satellite sensors, J. Geophys. Res.-Atmos., 113, D14S07, https://doi.org/10.1029/2007JD009661, 2008.
Shin, M., Kang, Y., Park, S., Im, J., Yoo, C., and Quackenbush, L. J.: Estimating ground-level particulate matter concentrations using satellite-based data: A review, GIsci. Remote Sens., 57, 174–189, 2020.
Skamarock, W. C., Klemp, J. B., Dudhia, J., Gill, D. O., Barker, D. M., Duda, M. G., Huang, X.-Y., Wang, W., and Powers, J.G.: A Description of the Advanced Research WRF Version 3, NCAR Tech. Note, NCAR/TN-475+STR, 113 pp., https://doi.org/10.5065/D68S4MVH, 2008.
Tao, H., Xing, J., Zhou, H., Pleim, J., Ran, L., Chang, X., Wang, S., Chen, F., Zheng, H., and Li, J.: Impacts of improved modeling resolution on the simulation of meteorology, air quality, and human exposure to PM2.5, O3 in Beijing, China, J. Clean. Prod., 243, 118574, https://doi.org/10.1016/j.jclepro.2019.118574, 2020.
Teng, M., Li, S., Xing, J., Fan, C., Yang, J., Wang, S., Song, G., Ding. Y., Dong, J., and Wang, S.: 72-hour real-time forecasting of ambient PM2.5 by hybrid graph deep neural network with aggregated neighborhood spatiotemporal information, Environ. Int., 176, 107971, https://doi.org/10.1016/j.envint.2023.107971, 2023.
Wang, Z., Hu, B., Huang, B., Ma, Z., Biswas, A., Jiang, Y., and Shi, Z.: Predicting annual PM2.5 in mainland China from 2014 to 2020 using multi temporal satellite product: An improved deep learning approach with spatial generalization ability, ISPRS. J. Photogramm., 187, 141–158, 2022a.
Wang, Z., Li, R., Chen, Z., Yao, Q., Gao, B., Xu, M., Yang, L., Li, M., and Zhou, C.: The estimation of hourly PM2.5 concentrations across China based on a Spatial and Temporal Weighted Continuous Deep Neural Network (STWC-DNN), ISPRS. J. Photogramm., 190, 38–55, 2022b.
Wei, J., Li, Z., Chen, X., Li, C., Sun, Y., Wang, J., Lyapustin, A.,Brasseur, G., Jiang, M., Sun, L., Wang, T., Jung, C., Qiu, B., Fang, Liu, X., Hao, J., Wang, Y., Zhan, M., Song, X., and Liu, Y.: Separating Daily 1 km PM2.5 Inorganic Chemical Composition in China since 2000 via Deep Learning Integrating Ground, Satellite, and Model Data, Environ. Sci. Technol., 57, 18282–18295, https://doi.org/10.1021/acs.est.3c00272, 2023.
Xiao, Q., Chang, H. H., Geng, G., and Liu, Y.: An ensemble machine-learning model to predict historical PM2.5 concentrations in China from satellite data, Environ. Sci. Technol., 52, 13260–13269, 2018.
Xing, J., Zheng, S., Ding, D., Kelly, J. T., Wang, S., Li, S., Qin, T., Ma, M., Dong, Z., Jang, C., Zhu, Y., Zheng, H., Ren, L., Liu, T.-Y., and Hao, J.: Deep learning for prediction of the air quality response to emission changes, Environ. Sci. Technol., 54, 8589–8600, 2020.
Yan, X., Zang, Z., Luo, N., Jiang, Y., and Li, Z.: New interpretable deep learning model to monitor real-time PM2.5 concentrations from satellite data, Environ. Int., 144, 106060, https://doi.org/10.1016/j.envint.2020.106060, 2020.
Yarwood, G., Jung, J., Whitten, G. Z., Heo, G., Mellberg, J., and Estes, M.: Updates to the Carbon Bond mechanism for version 6 (CB6), in: 9th Annual CMAS Conference, Chapel Hill, NC, USA, 11–13 October 2010, https://cmascenter.org/conference/2010/abstracts/emery_updates_carbon_2010.pdf (last access: 19 August 2024), 2010.
Zheng, H., Zhao, B., Wang, S., Wang, T., Ding, D., Chang, X., Liu, K., Xing, J., Dong, Z., Aunan, K., Liu, T., Wu, X., Zhang, S., and Wu, Y.: Transition in source contributions of PM2.5 exposure and associated premature mortality in China during 2005–2015, Environ. Int., 132, 105111, https://doi.org/10.1016/j.envint.2019.105111, 2019.
Zhou, Z. H. and Feng, J.: Deep forest, Natl. Sci. Rev., 6, 74–86, 2019.
Zhong, J., Zhang, X., Gui, K., Wang, Y., Che, H., Shen, X., Zhang, L., Zhang, Y., Sun, J., and Zhang, W.: Robust prediction of hourly PM2.5 from meteorological data using LightGBM, Natl. Sci. Rev., 8, nwaa307, https://doi.org/10.1093/nsr/nwaa307, 2021.
Short summary
Surface PM2.5 data have gained widespread application in health assessments and related fields, while the inherent uncertainties in PM2.5 data persist due to the lack of ground-truth data across the space. This study provides a novel testbed, enabling comprehensive evaluation across the entire spatial domain. The optimized deep-learning model with spatiotemporal features successfully retrieved surface PM2.5 concentrations in China (2013–2021), with reduced biases induced by sample imbalance.
Surface PM2.5 data have gained widespread application in health assessments and related fields,...
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