Articles | Volume 16, issue 4
https://doi.org/10.5194/essd-16-1875-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/essd-16-1875-2024
© Author(s) 2024. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Data description paper
| 
16 Apr 2024
Data description paper |
| 16 Apr 2024
| 16 Apr 2024
High-resolution physicochemical dataset of atmospheric aerosols over the Tibetan Plateau and its surroundings
Jianzhong Xu
CORRESPONDING AUTHOR
School of Oceanography, Shanghai Jiao Tong University, Shanghai 200030, China
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
Xinghua Zhang
CORRESPONDING AUTHOR
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
now at: College of Urban and Environmental Sciences, Northwest University, Xi'an 710127, China
Wenhui Zhao
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China
now at: Institute of Geochemistry, Chinese Academy of Sciences, Guangzhou 510640, China
Lixiang Zhai
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China
now at: College of Resources and Environmental Sciences, Gansu Agricultural University, Lanzhou 730000, China
Miao Zhong
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China
Jinsen Shi
Key Laboratory for Semi-Arid Climate Change of the Ministry of Education, College of Atmospheric Sciences, Lanzhou University, Lanzhou 730000, China
Junying Sun
Key Laboratory of Atmospheric Chemistry of CMA, Chinese Academy of Meteorological Sciences, Beijing 100081, China
Yanmei Liu
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
now at: College of Resources and Environment, Aba Teachers University, Wenchuan 623002, China
Conghui Xie
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
now at: State Key Joint Laboratory of Environmental Simulation and Pollution Control, College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China
Yulong Tan
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China
Kemei Li
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China
Xinlei Ge
Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing 210044, China
Department of Environmental Toxicology, University of California, Davis, CA 95616, USA
Shichang Kang
State Key Laboratory of Cryospheric Sciences, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China
College of Resources and Environment, University of Chinese Academy of Sciences, Beijing 100049, China
CAS Center for Excellence in Tibetan Plateau Earth Sciences, Beijing 100085, China
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Lan Ma, Reed Worland, Wenqing Jiang, Christopher Niedek, Chrystal Guzman, Keith J. Bein, Qi Zhang, and Cort Anastasio
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Wenqing Jiang, Christopher Niedek, Cort Anastasio, and Qi Zhang
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Atmos. Chem. Phys., 23, 5517–5531, https://doi.org/10.5194/acp-23-5517-2023, https://doi.org/10.5194/acp-23-5517-2023, 2023
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Huiming Lin, Yindong Tong, Long Chen, Chenghao Yu, Zhaohan Chu, Qianru Zhang, Xiufeng Yin, Qianggong Zhang, Shichang Kang, Junfeng Liu, James Schauer, Benjamin de Foy, and Xuejun Wang
Atmos. Chem. Phys., 23, 3937–3953, https://doi.org/10.5194/acp-23-3937-2023, https://doi.org/10.5194/acp-23-3937-2023, 2023
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Lhasa is the largest city in the Tibetan Plateau, and its atmospheric mercury concentrations represent the highest level of pollution in this region. Unexpectedly high concentrations of atmospheric mercury species were found. Combined with the trajectory analysis, the high atmospheric mercury concentrations may have originated from external long-range transport. Local sources, especially special mercury-related sources, are important factors influencing the variability of atmospheric mercury.
Nathaniel W. May, Noah Bernays, Ryan Farley, Qi Zhang, and Daniel A. Jaffe
Atmos. Chem. Phys., 23, 2747–2764, https://doi.org/10.5194/acp-23-2747-2023, https://doi.org/10.5194/acp-23-2747-2023, 2023
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Christopher R. Niedek, Fan Mei, Maria A. Zawadowicz, Zihua Zhu, Beat Schmid, and Qi Zhang
Atmos. Meas. Tech., 16, 955–968, https://doi.org/10.5194/amt-16-955-2023, https://doi.org/10.5194/amt-16-955-2023, 2023
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This novel micronebulization aerosol mass spectrometry (MS) technique requires a low sample volume (10 μL) and can quantify nanogram levels of organic and inorganic particulate matter (PM) components when used with 34SO4. This technique was successfully applied to PM samples collected from uncrewed atmospheric measurement platforms and provided chemical information that agrees well with real-time data from a co-located aerosol chemical speciation monitor and offline data from secondary ion MS.
Shaoyong Wang, Xiaobo He, Shichang Kang, Hui Fu, and Xiaofeng Hong
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This study used the sine-wave exponential model and long-term water stable isotopic data to estimate water mean residence time (MRT) and its influencing factors in a high-altitude permafrost catchment (5300 m a.s.l.) in the central Tibetan Plateau (TP). MRT for stream and supra-permafrost water was estimated at 100 and 255 d, respectively. Climate and vegetation factors affected the MRT of stream and supra-permafrost water mainly by changing the thickness of the permafrost active layer.
Yibei Wan, Xiangpeng Huang, Chong Xing, Qiongqiong Wang, Xinlei Ge, and Huan Yu
Atmos. Chem. Phys., 22, 15413–15423, https://doi.org/10.5194/acp-22-15413-2022, https://doi.org/10.5194/acp-22-15413-2022, 2022
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The organic compounds involved in continental new particle formation have been investigated in depth in the last 2 decades. In contrast, no prior work has studied the exact chemical composition of organic compounds and their role in coastal new particle formation. We present a complementary study to the ongoing laboratory and field research on iodine nucleation in the coastal atmosphere. This study provided a more complete story of coastal I-NPF from low-tide macroalgal emission.
Jizu Chen, Wentao Du, Shichang Kang, Xiang Qin, Weijun Sun, Yang Li, Yushuo Liu, Lihui Luo, and Youyan Jiang
The Cryosphere Discuss., https://doi.org/10.5194/tc-2022-179, https://doi.org/10.5194/tc-2022-179, 2022
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This study developed a dynamic deposition model of light absorbing particles (LAPs), which coupled with a surface energy and mass balance model. Based on the coupled model, we assessed atmospheric deposited BC effect on glacier melting, and quantified global warming and increment of emitted black carbon respective contributions to current accelerated glacier melting.
Chaman Gul, Shichang Kang, Siva Praveen Puppala, Xiaokang Wu, Cenlin He, Yangyang Xu, Inka Koch, Sher Muhammad, Rajesh Kumar, and Getachew Dubache
Atmos. Chem. Phys., 22, 8725–8737, https://doi.org/10.5194/acp-22-8725-2022, https://doi.org/10.5194/acp-22-8725-2022, 2022
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This work aims to understand concentrations, spatial variability, and potential source regions of light-absorbing impurities (black carbon aerosols, dust particles, and organic carbon) in the surface snow of central and western Himalayan glaciers and their impact on snow albedo and radiative forcing.
Xinghua Zhang, Wenhui Zhao, Lixiang Zhai, Miao Zhong, Jinsen Shi, Junying Sun, Yanmei Liu, Conghui Xie, Yulong Tan, Kemei Li, Xinlei Ge, Qi Zhang, Shichang Kang, and Jianzhong Xu
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2022-211, https://doi.org/10.5194/essd-2022-211, 2022
Manuscript not accepted for further review
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A comprehensive aerosol observation project was carried out in the Tibetan Plateau (TP) in recent years to investigate the properties and sources of atmospheric aerosols as well as their regional differences by performing multiple short-term intensive field observations. The real-time online high-time-resolution (hourly) data of aerosol properties in the different TP region are integrated in a new dataset and can provide supporting for related studies in in the TP.
Shijie Cui, Dan Dan Huang, Yangzhou Wu, Junfeng Wang, Fuzhen Shen, Jiukun Xian, Yunjiang Zhang, Hongli Wang, Cheng Huang, Hong Liao, and Xinlei Ge
Atmos. Chem. Phys., 22, 8073–8096, https://doi.org/10.5194/acp-22-8073-2022, https://doi.org/10.5194/acp-22-8073-2022, 2022
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Refractory black carbon (rBC) aerosols are important to air quality and climate change. rBC can mix with many other species, which can significantly change its properties and impacts. We used a specific set of techniques to exclusively characterize rBC-containing (rBCc) particles in Shanghai. We elucidated their composition, sources and size distributions and factors that affect their properties. Our findings are very valuable for advancing the understanding of BC and controlling BC pollution.
Xudong Li, Ye Tao, Longwei Zhu, Shuaishuai Ma, Shipeng Luo, Zhuzi Zhao, Ning Sun, Xinlei Ge, and Zhaolian Ye
Atmos. Chem. Phys., 22, 7793–7814, https://doi.org/10.5194/acp-22-7793-2022, https://doi.org/10.5194/acp-22-7793-2022, 2022
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This work has, for the first time, investigated the optical and chemical properties and oxidative potential of aqueous-phase photooxidation products of eugenol (a biomass-burning-emitted compound) and elucidated the interplay among these properties. Large mass yields exceeding 100 % were found, and the aqueous processing is a source of BrC (likely relevant with humic-like substances). We also show that aqueous processing can produce species that are more toxic than that of its precursor.
Jiaxing Sun, Yele Sun, Conghui Xie, Weiqi Xu, Chun Chen, Zhe Wang, Lei Li, Xubing Du, Fugui Huang, Yan Li, Zhijie Li, Xiaole Pan, Nan Ma, Wanyun Xu, Pingqing Fu, and Zifa Wang
Atmos. Chem. Phys., 22, 7619–7630, https://doi.org/10.5194/acp-22-7619-2022, https://doi.org/10.5194/acp-22-7619-2022, 2022
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We analyzed the chemical composition and mixing state of BC-containing particles at urban and rural sites in winter in the North China Plain and evaluated their impact on light absorption enhancement. BC was dominantly mixed with organic carbon, nitrate, and sulfate, and the mixing state evolved significantly as a function of relative humidity (RH) at both sites. The absorption enhancement depended strongly on coated secondary inorganic aerosol and was up to ~1.3–1.4 during aging processes.
Yongqin Liu, Pengcheng Fang, Bixi Guo, Mukan Ji, Pengfei Liu, Guannan Mao, Baiqing Xu, Shichang Kang, and Junzhi Liu
Earth Syst. Sci. Data, 14, 2303–2314, https://doi.org/10.5194/essd-14-2303-2022, https://doi.org/10.5194/essd-14-2303-2022, 2022
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Glaciers are an important pool of microorganisms, organic carbon, and nitrogen. This study constructed the first dataset of microbial abundance and total nitrogen in Tibetan Plateau (TP) glaciers and the first dataset of dissolved organic carbon in ice cores on the TP. These new data could provide valuable information for research on the glacier carbon and nitrogen cycle and help in assessing the potential impacts of glacier retreat due to global warming on downstream ecosystems.
Haoran Zhang, Nan Li, Keqin Tang, Hong Liao, Chong Shi, Cheng Huang, Hongli Wang, Song Guo, Min Hu, Xinlei Ge, Mindong Chen, Zhenxin Liu, Huan Yu, and Jianlin Hu
Atmos. Chem. Phys., 22, 5495–5514, https://doi.org/10.5194/acp-22-5495-2022, https://doi.org/10.5194/acp-22-5495-2022, 2022
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We developed a new algorithm with low economic/technique costs to identify primary and secondary components of PM2.5. Our model was shown to be reliable by comparison with different observation datasets. We systematically explored the patterns and changes in the secondary PM2.5 pollution in China at large spatial and time scales. We believe that this method is a promising tool for efficiently estimating primary and secondary PM2.5, and has huge potential for future PM mitigation.
Mukesh Rai, Shichang Kang, Junhua Yang, Maheswar Rupakheti, Dipesh Rupakheti, Lekhendra Tripathee, Yuling Hu, and Xintong Chen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2022-199, https://doi.org/10.5194/acp-2022-199, 2022
Revised manuscript not accepted
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Our study revealed distinctive seasonality with the maximum and minimum aerosol concentrations during the winter and summer seasons respectively. However, interestingly summer high (AOD > 0.8) was observed over South Asia. The highest aerosols are laden over South Asia and East China within 1–2 km, however, aerosol overshooting found up to 10 km due to the deep convection process. Whereas, integrated aerosol transport for OC during spring was found to be 5 times higher than the annual mean.
Huiming Lin, Yindong Tong, Chenghao Yu, Long Chen, Xiufeng Yin, Qianggong Zhang, Shichang Kang, Lun Luo, James Schauer, Benjamin de Foy, and Xuejun Wang
Atmos. Chem. Phys., 22, 2651–2668, https://doi.org/10.5194/acp-22-2651-2022, https://doi.org/10.5194/acp-22-2651-2022, 2022
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The Tibetan Plateau is known as
The Third Poleand is generally considered to be a clean area owing to its high altitude. However, it may receive be impacted by air pollutants transported from the Indian subcontinent. Pollutants generally enter the Tibetan Plateau in several ways. Among them is the Yarlung Zangbu–Brahmaputra Grand Canyon. In this study, we identified the influence of the Indian summer monsoon on the origin, transport, and behavior of mercury in this area.
Shichang Kang, Yulan Zhang, Pengfei Chen, Junming Guo, Qianggong Zhang, Zhiyuan Cong, Susan Kaspari, Lekhendra Tripathee, Tanguang Gao, Hewen Niu, Xinyue Zhong, Xintong Chen, Zhaofu Hu, Xiaofei Li, Yang Li, Bigyan Neupane, Fangping Yan, Dipesh Rupakheti, Chaman Gul, Wei Zhang, Guangming Wu, Ling Yang, Zhaoqing Wang, and Chaoliu Li
Earth Syst. Sci. Data, 14, 683–707, https://doi.org/10.5194/essd-14-683-2022, https://doi.org/10.5194/essd-14-683-2022, 2022
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The Tibetan Plateau is important to the Earth’s climate. However, systematically observed data here are scarce. To perform more integrated and in-depth investigations of the origins and distributions of atmospheric pollutants and their impacts on cryospheric change, systematic data of black carbon and organic carbon from the atmosphere, glaciers, snow cover, precipitation, and lake sediment cores over the plateau based on the Atmospheric Pollution and Cryospheric Change program are provided.
Jiaxing Sun, Zhe Wang, Wei Zhou, Conghui Xie, Cheng Wu, Chun Chen, Tingting Han, Qingqing Wang, Zhijie Li, Jie Li, Pingqing Fu, Zifa Wang, and Yele Sun
Atmos. Chem. Phys., 22, 561–575, https://doi.org/10.5194/acp-22-561-2022, https://doi.org/10.5194/acp-22-561-2022, 2022
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We analyzed 9-year measurements of BC and aerosol optical properties from 2012 to 2020 in Beijing, China. Our results showed large reductions in BC and light extinction coefficient due to the Clean Air Action Plan. As a response, both SSA and mass extinction efficiency (MEE) showed considerable increases, demonstrating a future challenge in visibility improvement. The primary and secondary BrC was also separated and quantified, and the changes in radiative forcing of BC and BrC were estimated.
Jinlei Chen, Shichang Kang, Wentao Du, Junming Guo, Min Xu, Yulan Zhang, Xinyue Zhong, Wei Zhang, and Jizu Chen
The Cryosphere, 15, 5473–5482, https://doi.org/10.5194/tc-15-5473-2021, https://doi.org/10.5194/tc-15-5473-2021, 2021
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Sea ice is retreating with rapid warming in the Arctic. It will continue and approach the worst predicted pathway released by the IPCC. The irreversible tipping point might show around 2060 when the oldest ice will have completely disappeared. It has a huge impact on human production. Ordinary merchant ships will be able to pass the Northeast Passage and Northwest Passage by the midcentury, and the opening time will advance to the next 10 years for icebreakers with moderate ice strengthening.
Clémence Rose, Martine Collaud Coen, Elisabeth Andrews, Yong Lin, Isaline Bossert, Cathrine Lund Myhre, Thomas Tuch, Alfred Wiedensohler, Markus Fiebig, Pasi Aalto, Andrés Alastuey, Elisabeth Alonso-Blanco, Marcos Andrade, Begoña Artíñano, Todor Arsov, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Juan Andrés Casquero-Vera, Sébastien Conil, Konstantinos Eleftheriadis, Olivier Favez, Harald Flentje, Maria I. Gini, Francisco Javier Gómez-Moreno, Martin Gysel-Beer, Anna Gannet Hallar, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Melita Keywood, Jeong Eun Kim, Sang-Woo Kim, Adam Kristensson, Markku Kulmala, Heikki Lihavainen, Neng-Huei Lin, Hassan Lyamani, Angela Marinoni, Sebastiao Martins Dos Santos, Olga L. Mayol-Bracero, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Jakub Ondracek, Marco Pandolfi, Noemi Pérez, Tuukka Petäjä, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Jean-Philippe Putaud, Fabienne Reisen, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Junying Sun, Pierre Tulet, Ville Vakkari, Pieter Gideon van Zyl, Fernando Velarde, Paolo Villani, Stergios Vratolis, Zdenek Wagner, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Vladimir Zdimal, and Paolo Laj
Atmos. Chem. Phys., 21, 17185–17223, https://doi.org/10.5194/acp-21-17185-2021, https://doi.org/10.5194/acp-21-17185-2021, 2021
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Aerosol particles are a complex component of the atmospheric system the effects of which are among the most uncertain in climate change projections. Using data collected at 62 stations, this study provides the most up-to-date picture of the spatial distribution of particle number concentration and size distribution worldwide, with the aim of contributing to better representation of aerosols and their interactions with clouds in models and, therefore, better evaluation of their impact on climate.
Fan Mei, Jian Wang, Shan Zhou, Qi Zhang, Sonya Collier, and Jianzhong Xu
Atmos. Chem. Phys., 21, 13019–13029, https://doi.org/10.5194/acp-21-13019-2021, https://doi.org/10.5194/acp-21-13019-2021, 2021
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This work focuses on understanding aerosol's ability to act as cloud condensation nuclei (CCN) and its variations with organic oxidation level and volatility using measurements at a rural site. Aerosol properties were examined from four air mass sources. The results help improve the accurate representation of aerosol from different ambient aerosol emissions, transformation pathways, and atmospheric processes in a climate model.
Yongkang Xue, Tandong Yao, Aaron A. Boone, Ismaila Diallo, Ye Liu, Xubin Zeng, William K. M. Lau, Shiori Sugimoto, Qi Tang, Xiaoduo Pan, Peter J. van Oevelen, Daniel Klocke, Myung-Seo Koo, Tomonori Sato, Zhaohui Lin, Yuhei Takaya, Constantin Ardilouze, Stefano Materia, Subodh K. Saha, Retish Senan, Tetsu Nakamura, Hailan Wang, Jing Yang, Hongliang Zhang, Mei Zhao, Xin-Zhong Liang, J. David Neelin, Frederic Vitart, Xin Li, Ping Zhao, Chunxiang Shi, Weidong Guo, Jianping Tang, Miao Yu, Yun Qian, Samuel S. P. Shen, Yang Zhang, Kun Yang, Ruby Leung, Yuan Qiu, Daniele Peano, Xin Qi, Yanling Zhan, Michael A. Brunke, Sin Chan Chou, Michael Ek, Tianyi Fan, Hong Guan, Hai Lin, Shunlin Liang, Helin Wei, Shaocheng Xie, Haoran Xu, Weiping Li, Xueli Shi, Paulo Nobre, Yan Pan, Yi Qin, Jeff Dozier, Craig R. Ferguson, Gianpaolo Balsamo, Qing Bao, Jinming Feng, Jinkyu Hong, Songyou Hong, Huilin Huang, Duoying Ji, Zhenming Ji, Shichang Kang, Yanluan Lin, Weiguang Liu, Ryan Muncaster, Patricia de Rosnay, Hiroshi G. Takahashi, Guiling Wang, Shuyu Wang, Weicai Wang, Xu Zhou, and Yuejian Zhu
Geosci. Model Dev., 14, 4465–4494, https://doi.org/10.5194/gmd-14-4465-2021, https://doi.org/10.5194/gmd-14-4465-2021, 2021
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The subseasonal prediction of extreme hydroclimate events such as droughts/floods has remained stubbornly low for years. This paper presents a new international initiative which, for the first time, introduces spring land surface temperature anomalies over high mountains to improve precipitation prediction through remote effects of land–atmosphere interactions. More than 40 institutions worldwide are participating in this effort. The experimental protocol and preliminary results are presented.
Kun Wang, Shohei Hattori, Mang Lin, Sakiko Ishino, Becky Alexander, Kazuki Kamezaki, Naohiro Yoshida, and Shichang Kang
Atmos. Chem. Phys., 21, 8357–8376, https://doi.org/10.5194/acp-21-8357-2021, https://doi.org/10.5194/acp-21-8357-2021, 2021
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Sulfate aerosols play an important climatic role and exert adverse effects on the ecological environment and human health. In this study, we present the triple oxygen isotopic composition of sulfate from the Mt. Everest region, southern Tibetan Plateau, and decipher the formation mechanisms of atmospheric sulfate in this pristine environment. The results indicate the important role of the S(IV) + O3 pathway in atmospheric sulfate formation promoted by conditions of high cloud water pH.
Xiaojing Shen, Junying Sun, Fangqun Yu, Ying Wang, Junting Zhong, Yangmei Zhang, Xinyao Hu, Can Xia, Sinan Zhang, and Xiaoye Zhang
Atmos. Chem. Phys., 21, 7039–7052, https://doi.org/10.5194/acp-21-7039-2021, https://doi.org/10.5194/acp-21-7039-2021, 2021
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In this work, we revealed the changes of PNSD and NPF events during the COVID-19 lockdown period in Beijing, China, to illustrate the impact of reduced primary emission and elavated atmospheric oxidized capicity on the nucleation and growth processes. The subsequent growth of nucleated particles and their contribution to the aerosol pollution formation were also explored, to highlight the necessity of controlling the nanoparticles in the future air quality management.
Mutian Ma, Laura-Hélèna Rivellini, YuXi Cui, Megan D. Willis, Rio Wilkie, Jonathan P. D. Abbatt, Manjula R. Canagaratna, Junfeng Wang, Xinlei Ge, and Alex K. Y. Lee
Atmos. Meas. Tech., 14, 2799–2812, https://doi.org/10.5194/amt-14-2799-2021, https://doi.org/10.5194/amt-14-2799-2021, 2021
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Chemical characterization of organic coatings is important to advance our understanding of the physio-chemical properties and atmospheric processing of black carbon (BC) particles. This work develops two approaches to improve the elemental analysis of oxygenated organic coatings using a soot-particle aerosol mass spectrometer. Analyzing ambient data with the new approaches indicated that secondary organics that coated on BC were likely less oxygenated compared to those externally mixed with BC.
Linlin Liang, Guenter Engling, Chang Liu, Wanyun Xu, Xuyan Liu, Yuan Cheng, Zhenyu Du, Gen Zhang, Junying Sun, and Xiaoye Zhang
Atmos. Chem. Phys., 21, 3181–3192, https://doi.org/10.5194/acp-21-3181-2021, https://doi.org/10.5194/acp-21-3181-2021, 2021
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A unique episode with extreme biomass burning (BB) impact, with daily concentration of levoglucosan as high as 4.37 µg m-3, was captured at an area upwind of Beijing. How this extreme BB pollution event was generated and what were the chemical properties of PM2.5 under this kind severe BB pollution level in the real atmospheric environment were both presented in this measurement report. Moreover, the variation of the ratios of BB tracers during different BB pollution periods was also exhibited.
Junfeng Wang, Jianhuai Ye, Dantong Liu, Yangzhou Wu, Jian Zhao, Weiqi Xu, Conghui Xie, Fuzhen Shen, Jie Zhang, Paul E. Ohno, Yiming Qin, Xiuyong Zhao, Scot T. Martin, Alex K. Y. Lee, Pingqing Fu, Daniel J. Jacob, Qi Zhang, Yele Sun, Mindong Chen, and Xinlei Ge
Atmos. Chem. Phys., 20, 14091–14102, https://doi.org/10.5194/acp-20-14091-2020, https://doi.org/10.5194/acp-20-14091-2020, 2020
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We compared the organics in total submicron matter and those coated on BC cores during summertime in Beijing and found large differences between them. Traffic-related OA was associated significantly with BC, while cooking-related OA did not coat BC. In addition, a factor likely originated from primary biomass burning OA was only identified in BC-containing particles. Such a unique BBOA requires further field and laboratory studies to verify its presence and elucidate its properties and impacts.
Lawrence I. Kleinman, Arthur J. Sedlacek III, Kouji Adachi, Peter R. Buseck, Sonya Collier, Manvendra K. Dubey, Anna L. Hodshire, Ernie Lewis, Timothy B. Onasch, Jeffery R. Pierce, John Shilling, Stephen R. Springston, Jian Wang, Qi Zhang, Shan Zhou, and Robert J. Yokelson
Atmos. Chem. Phys., 20, 13319–13341, https://doi.org/10.5194/acp-20-13319-2020, https://doi.org/10.5194/acp-20-13319-2020, 2020
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Aerosols from wildfires affect the Earth's temperature by absorbing light or reflecting it back into space. This study investigates time-dependent chemical, microphysical, and optical properties of aerosols generated by wildfires in the Pacific Northwest, USA. Wildfire smoke plumes were traversed by an instrumented aircraft at locations near the fire and up to 3.5 h travel time downwind. Although there was no net aerosol production, aerosol particles grew and became more efficient scatters.
Hwajin Kim, Qi Zhang, and Yele Sun
Atmos. Chem. Phys., 20, 11527–11550, https://doi.org/10.5194/acp-20-11527-2020, https://doi.org/10.5194/acp-20-11527-2020, 2020
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Severe spring haze and influences of long-range transport in the Seoul metropolitan area (SMA) in March 2019 were investigated. Simultaneous downwind (SMA) and upwind (Beijing) measurements using AMS and ACSM over the same period showed that PM species can be transported in approximately 2 d. Nitrate was the most responsible, and sulfate and two regional-transport-influenced SOAs also contributed. Enhancement of Pb also showed that the haze in the SMA was influenced by the regional transport.
María A. Burgos, Elisabeth Andrews, Gloria Titos, Angela Benedetti, Huisheng Bian, Virginie Buchard, Gabriele Curci, Zak Kipling, Alf Kirkevåg, Harri Kokkola, Anton Laakso, Julie Letertre-Danczak, Marianne T. Lund, Hitoshi Matsui, Gunnar Myhre, Cynthia Randles, Michael Schulz, Twan van Noije, Kai Zhang, Lucas Alados-Arboledas, Urs Baltensperger, Anne Jefferson, James Sherman, Junying Sun, Ernest Weingartner, and Paul Zieger
Atmos. Chem. Phys., 20, 10231–10258, https://doi.org/10.5194/acp-20-10231-2020, https://doi.org/10.5194/acp-20-10231-2020, 2020
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We investigate how well models represent the enhancement in scattering coefficients due to particle water uptake, and perform an evaluation of several implementation schemes used in ten Earth system models. Our results show the importance of the parameterization of hygroscopicity and model chemistry as drivers of some of the observed diversity amongst model estimates. The definition of dry conditions and the phenomena taking place in this relative humidity range also impact the model evaluation.
Paolo Laj, Alessandro Bigi, Clémence Rose, Elisabeth Andrews, Cathrine Lund Myhre, Martine Collaud Coen, Yong Lin, Alfred Wiedensohler, Michael Schulz, John A. Ogren, Markus Fiebig, Jonas Gliß, Augustin Mortier, Marco Pandolfi, Tuukka Petäja, Sang-Woo Kim, Wenche Aas, Jean-Philippe Putaud, Olga Mayol-Bracero, Melita Keywood, Lorenzo Labrador, Pasi Aalto, Erik Ahlberg, Lucas Alados Arboledas, Andrés Alastuey, Marcos Andrade, Begoña Artíñano, Stina Ausmeel, Todor Arsov, Eija Asmi, John Backman, Urs Baltensperger, Susanne Bastian, Olaf Bath, Johan Paul Beukes, Benjamin T. Brem, Nicolas Bukowiecki, Sébastien Conil, Cedric Couret, Derek Day, Wan Dayantolis, Anna Degorska, Konstantinos Eleftheriadis, Prodromos Fetfatzis, Olivier Favez, Harald Flentje, Maria I. Gini, Asta Gregorič, Martin Gysel-Beer, A. Gannet Hallar, Jenny Hand, Andras Hoffer, Christoph Hueglin, Rakesh K. Hooda, Antti Hyvärinen, Ivo Kalapov, Nikos Kalivitis, Anne Kasper-Giebl, Jeong Eun Kim, Giorgos Kouvarakis, Irena Kranjc, Radovan Krejci, Markku Kulmala, Casper Labuschagne, Hae-Jung Lee, Heikki Lihavainen, Neng-Huei Lin, Gunter Löschau, Krista Luoma, Angela Marinoni, Sebastiao Martins Dos Santos, Frank Meinhardt, Maik Merkel, Jean-Marc Metzger, Nikolaos Mihalopoulos, Nhat Anh Nguyen, Jakub Ondracek, Noemi Pérez, Maria Rita Perrone, Jean-Eudes Petit, David Picard, Jean-Marc Pichon, Veronique Pont, Natalia Prats, Anthony Prenni, Fabienne Reisen, Salvatore Romano, Karine Sellegri, Sangeeta Sharma, Gerhard Schauer, Patrick Sheridan, James Patrick Sherman, Maik Schütze, Andreas Schwerin, Ralf Sohmer, Mar Sorribas, Martin Steinbacher, Junying Sun, Gloria Titos, Barbara Toczko, Thomas Tuch, Pierre Tulet, Peter Tunved, Ville Vakkari, Fernando Velarde, Patricio Velasquez, Paolo Villani, Sterios Vratolis, Sheng-Hsiang Wang, Kay Weinhold, Rolf Weller, Margarita Yela, Jesus Yus-Diez, Vladimir Zdimal, Paul Zieger, and Nadezda Zikova
Atmos. Meas. Tech., 13, 4353–4392, https://doi.org/10.5194/amt-13-4353-2020, https://doi.org/10.5194/amt-13-4353-2020, 2020
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The paper establishes the fiducial reference of the GAW aerosol network providing the fully characterized value chain to the provision of four climate-relevant aerosol properties from ground-based sites. Data from almost 90 stations worldwide are reported for a reference year, 2017, providing a unique and very robust view of the variability of these variables worldwide. Current gaps in the GAW network are analysed and requirements for the Global Climate Monitoring System are proposed.
Martine Collaud Coen, Elisabeth Andrews, Andrés Alastuey, Todor Petkov Arsov, John Backman, Benjamin T. Brem, Nicolas Bukowiecki, Cédric Couret, Konstantinos Eleftheriadis, Harald Flentje, Markus Fiebig, Martin Gysel-Beer, Jenny L. Hand, András Hoffer, Rakesh Hooda, Christoph Hueglin, Warren Joubert, Melita Keywood, Jeong Eun Kim, Sang-Woo Kim, Casper Labuschagne, Neng-Huei Lin, Yong Lin, Cathrine Lund Myhre, Krista Luoma, Hassan Lyamani, Angela Marinoni, Olga L. Mayol-Bracero, Nikos Mihalopoulos, Marco Pandolfi, Natalia Prats, Anthony J. Prenni, Jean-Philippe Putaud, Ludwig Ries, Fabienne Reisen, Karine Sellegri, Sangeeta Sharma, Patrick Sheridan, James Patrick Sherman, Junying Sun, Gloria Titos, Elvis Torres, Thomas Tuch, Rolf Weller, Alfred Wiedensohler, Paul Zieger, and Paolo Laj
Atmos. Chem. Phys., 20, 8867–8908, https://doi.org/10.5194/acp-20-8867-2020, https://doi.org/10.5194/acp-20-8867-2020, 2020
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Long-term trends of aerosol radiative properties (52 stations) prove that aerosol load has significantly decreased over the last 20 years. Scattering trends are negative in Europe (EU) and North America (NA), not ss in Asia, and show a mix of positive and negative trends at polar stations. Absorption has mainly negative trends. The single scattering albedo has positive trends in Asia and eastern EU and negative in western EU and NA, leading to a global positive median trend of 0.02 % per year.
Shuang Yi, Chunqiao Song, Kosuke Heki, Shichang Kang, Qiuyu Wang, and Le Chang
The Cryosphere, 14, 2267–2281, https://doi.org/10.5194/tc-14-2267-2020, https://doi.org/10.5194/tc-14-2267-2020, 2020
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High-Asia glaciers have been observed to be retreating the fastest in the southeastern Tibeten Plateau, where vast amounts of glacier and snow feed the streamflow of the Brahmaputra. Here, we provide the first monthly glacier and snow mass balance during 2002–2017 based on satellite gravimetry. The results confirm previous long-term decreases but reveal strong seasonal variations. This work helps resolve previous divergent model estimates and underlines the importance of meltwater.
Lu Qi, Alexander L. Vogel, Sepideh Esmaeilirad, Liming Cao, Jing Zheng, Jean-Luc Jaffrezo, Paola Fermo, Anne Kasper-Giebl, Kaspar R. Daellenbach, Mindong Chen, Xinlei Ge, Urs Baltensperger, André S. H. Prévôt, and Jay G. Slowik
Atmos. Chem. Phys., 20, 7875–7893, https://doi.org/10.5194/acp-20-7875-2020, https://doi.org/10.5194/acp-20-7875-2020, 2020
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We present the first application of this online and offline strategy using the new extractive electrospray ionization time-of-flight mass spectrometer (EESI-TOF), which achieves increased chemical specificity relative to other online techniques. Measurement and source apportionment of 1 year of filter samples collected in Zurich, Switzerland, show seasonal contributions from fresh and aged wood combustion in winter and biogenic emission-derived SOA in summer, as well as other sources.
Jia Sun, Wolfram Birmili, Markus Hermann, Thomas Tuch, Kay Weinhold, Maik Merkel, Fabian Rasch, Thomas Müller, Alexander Schladitz, Susanne Bastian, Gunter Löschau, Josef Cyrys, Jianwei Gu, Harald Flentje, Björn Briel, Christoph Asbach, Heinz Kaminski, Ludwig Ries, Ralf Sohmer, Holger Gerwig, Klaus Wirtz, Frank Meinhardt, Andreas Schwerin, Olaf Bath, Nan Ma, and Alfred Wiedensohler
Atmos. Chem. Phys., 20, 7049–7068, https://doi.org/10.5194/acp-20-7049-2020, https://doi.org/10.5194/acp-20-7049-2020, 2020
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To evaluate the effectiveness of emission mitigation policies, we evaluated the trends of the size-resolved particle number concentrations and equivalent black carbon mass concentration at 16 observational sites for various environments in Germany (2009–2018). Overall, significant decrease trends are found for most of the parameters and sites. This study suggests that a combination of emission mitigation policies can effectively improve the air quality on large spatial scales such as in Germany.
Meixin Zhang, Chun Zhao, Zhiyuan Cong, Qiuyan Du, Mingyue Xu, Yu Chen, Ming Chen, Rui Li, Yunfei Fu, Lei Zhong, Shichang Kang, Delong Zhao, and Yan Yang
Atmos. Chem. Phys., 20, 5923–5943, https://doi.org/10.5194/acp-20-5923-2020, https://doi.org/10.5194/acp-20-5923-2020, 2020
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Analysis of multiple numerical experiments over the Himalayas and Tibetan Plateau (TP) shows that the complex topography results in 50 % stronger overall cross-Himalayan transport during the pre-monsoon season primarily due to the strengthened efficiency of near-surface meridional transport towards the TP, enhanced wind speed in some valleys and deeper valley channels associated with larger transported BC mass volume, which leads to 30–50 % stronger BC radiative heating over the TP.
Jianjun Li, Qi Zhang, Gehui Wang, Jin Li, Can Wu, Lang Liu, Jiayuan Wang, Wenqing Jiang, Lijuan Li, Kin Fai Ho, and Junji Cao
Atmos. Chem. Phys., 20, 4889–4904, https://doi.org/10.5194/acp-20-4889-2020, https://doi.org/10.5194/acp-20-4889-2020, 2020
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We examined light absorption properties and molecular composition of water-soluble (WS) and water-insoluble (WI) BrC in PM2.5 collected from northwest China. We found that photochemical formation contributes significantly to light absorption of WI-BrC in summer, whereas aqueous-phase reactions play an important role in secondary WS-BrC formation in winter. BrC was estimated to account for 1.36 % and 3.74 %, respectively, of total down-welling solar radiation in the UV range in summer and winter.
Linlin Liang, Guenter Engling, Chang Liu, Wanyun Xu, Xuyan Liu, Yuan Cheng, Zhenyu Du, Gen Zhang, Junying Sun, and Xiaoye Zhang
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2020-19, https://doi.org/10.5194/acp-2020-19, 2020
Revised manuscript not accepted
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Our study captured an episode with extreme biomass burning tracer level at an agricultural site in North China, with concentrations of levoglucosan as high as 4.37 μg m−3. Based on comparison of the chemical composition between different biomass burning periods, it appeared that biomass burning can obviously elevate the levels of organic components, but seems to have no significant effect on the production of secondary inorganic ions, although their precursors increased during the episode.
Jianjun Li, Gehui Wang, Qi Zhang, Jin Li, Can Wu, Wenqing Jiang, Tong Zhu, and Limin Zeng
Atmos. Chem. Phys., 19, 10481–10496, https://doi.org/10.5194/acp-19-10481-2019, https://doi.org/10.5194/acp-19-10481-2019, 2019
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In this study, we investigated molecular compositions of organic aerosols (OAs) in summertime PM2.5 at a rural site in the North China Plain. We found that regional emission from field biomass burning (BB) significantly affects the concentration and molecular distribution of aliphatic lipids, sugars, and terpene-derived SOA, but has limited influence on PAHs, hopenes, and phthalates. The contribution of BB to OA increased by more than 50 % during the period influenced by regional open-field BB.
Hua Yu, Weijun Li, Yangmei Zhang, Peter Tunved, Manuel Dall'Osto, Xiaojing Shen, Junying Sun, Xiaoye Zhang, Jianchao Zhang, and Zongbo Shi
Atmos. Chem. Phys., 19, 10433–10446, https://doi.org/10.5194/acp-19-10433-2019, https://doi.org/10.5194/acp-19-10433-2019, 2019
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Interaction of anthropogenic particles with radiation and clouds plays an important role in Arctic climate change. The mixing state of different aerosols is a key parameter influencing such interactions. However, little is known of this parameter, preventing an accurate representation of this information in global models. Multi-microscopic techniques were used to find one general core–shell structure in which secondary sulfate particles were covered by organic coating in the Arctic atmosphere.
Weiqi Xu, Conghui Xie, Eleni Karnezi, Qi Zhang, Junfeng Wang, Spyros N. Pandis, Xinlei Ge, Jingwei Zhang, Junling An, Qingqing Wang, Jian Zhao, Wei Du, Yanmei Qiu, Wei Zhou, Yao He, Ying Li, Jie Li, Pingqing Fu, Zifa Wang, Douglas R. Worsnop, and Yele Sun
Atmos. Chem. Phys., 19, 10205–10216, https://doi.org/10.5194/acp-19-10205-2019, https://doi.org/10.5194/acp-19-10205-2019, 2019
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We present the first aerosol volatility measurements in Beijing in summer using a thermodenuder coupled with aerosol mass spectrometers. Our results showed that organic aerosol (OA) comprised mainly semi-volatile organic compounds in summer, and the freshly oxidized secondary OA was the most volatile component. We also found quite different volatility distributions in black-carbon-containing primary and secondary OA, ambient OA, ambient secondary OA and the WRF-Chem model.
Lu Qi, Mindong Chen, Giulia Stefenelli, Veronika Pospisilova, Yandong Tong, Amelie Bertrand, Christoph Hueglin, Xinlei Ge, Urs Baltensperger, André S. H. Prévôt, and Jay G. Slowik
Atmos. Chem. Phys., 19, 8037–8062, https://doi.org/10.5194/acp-19-8037-2019, https://doi.org/10.5194/acp-19-8037-2019, 2019
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Current understanding of OA sources is limited by the chemical resolution of existing real-time measurement technology. We describe the first wintertime deployment of a novel extractive electrospray ionization time-of-flight mass spectrometer, which provides near-molecular OA measurements with high time resolution. We show that biomass combustion strongly influences winter OA. Via factor analysis, aging-dependent signatures and time contributions of biomass-combustion-derived OA are resolved.
Xinghua Zhang, Jianzhong Xu, Shichang Kang, Qi Zhang, and Junying Sun
Atmos. Chem. Phys., 19, 7897–7911, https://doi.org/10.5194/acp-19-7897-2019, https://doi.org/10.5194/acp-19-7897-2019, 2019
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Highly time resolved chemistry and sources of PM1 were measured by an Aerodyne HR-ToF-AMS at Waliguan Baseline Observatory, a high-altitude background station at the northeastern edge of Qinghai–Tibet Plateau (QTP), during summer 2017. Relatively higher mass concentration of PM1 and dominant sulfate contribution were observed in this site compared to those at other high-elevation sites in the southern or central QTP, indicating the different aerosol sources between them.
Dantong Liu, Rutambhara Joshi, Junfeng Wang, Chenjie Yu, James D. Allan, Hugh Coe, Michael J. Flynn, Conghui Xie, James Lee, Freya Squires, Simone Kotthaus, Sue Grimmond, Xinlei Ge, Yele Sun, and Pingqing Fu
Atmos. Chem. Phys., 19, 6749–6769, https://doi.org/10.5194/acp-19-6749-2019, https://doi.org/10.5194/acp-19-6749-2019, 2019
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This study provides source attribution and characterization of BC in the Beijing urban environment in both winter and summer. For the first time, the physically and chemically based source apportionments are compared to evaluate the primary source contribution and secondary processing of BC-containing particles. A method is proposed to isolate the BC from the transportation sector and coal combustion sources.
Richie Kaur, Jacqueline R. Labins, Scarlett S. Helbock, Wenqing Jiang, Keith J. Bein, Qi Zhang, and Cort Anastasio
Atmos. Chem. Phys., 19, 6579–6594, https://doi.org/10.5194/acp-19-6579-2019, https://doi.org/10.5194/acp-19-6579-2019, 2019
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We measured hydroxyl radical (•OH), singlet oxygen (1O2*), and organic triplets (3C*) in illuminated aqueous particle extracts. After measuring the impact of dilution on oxidant concentrations, we extrapolated our results to predict them in ambient particles – 1O2* and 3C* concentrations appear to be greatly enhanced, while •OH appears largely unchanged. Two of these oxidants (1O2*, 3C*) are not yet included in atmospheric models, and our results make it possible to include them in the future.
Junting Zhong, Xiaoye Zhang, Yaqiang Wang, Jizhi Wang, Xiaojing Shen, Hongsheng Zhang, Tijian Wang, Zhouqing Xie, Cheng Liu, Hengde Zhang, Tianliang Zhao, Junying Sun, Shaojia Fan, Zhiqiu Gao, Yubin Li, and Linlin Wang
Atmos. Chem. Phys., 19, 3287–3306, https://doi.org/10.5194/acp-19-3287-2019, https://doi.org/10.5194/acp-19-3287-2019, 2019
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In various haze regions in China, including the Guanzhong Plain, the middle and lower reaches of the Yangtze River, the Pearl River Delta, the Sichuan Basin, and the Northeast China Plain, heavy aerosol pollution episodes include inter-/trans-regional transport stages and cumulative stages (CSs). During CSs a two-way feedback mechanism exists between unfavorable meteorological conditions and cumulative aerosol pollution. This two-way feedback is further quantified and its magnitude is compared.
Xin Wan, Shichang Kang, Maheswar Rupakheti, Qianggong Zhang, Lekhendra Tripathee, Junming Guo, Pengfei Chen, Dipesh Rupakheti, Arnico K. Panday, Mark G. Lawrence, Kimitaka Kawamura, and Zhiyuan Cong
Atmos. Chem. Phys., 19, 2725–2747, https://doi.org/10.5194/acp-19-2725-2019, https://doi.org/10.5194/acp-19-2725-2019, 2019
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The sources of primary and secondary aerosols in the Hindu Kush–Himalayan–Tibetan Plateau region are not well known. Organic molecular tracers are useful for aerosol source apportionment. The characterization of molecular tracers were first systemically investigated and the contribution from primary and secondary sources to carbonaceous aerosols was estimated in the Kathmandu Valley. Our results demonstrate that biomass burning contributed a significant fraction to OC in the Kathmandu Valley.
Shan Zhou, Sonya Collier, Daniel A. Jaffe, and Qi Zhang
Atmos. Chem. Phys., 19, 1571–1585, https://doi.org/10.5194/acp-19-1571-2019, https://doi.org/10.5194/acp-19-1571-2019, 2019
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Regional background aerosols in the western US were studied from a mountaintop observatory during summer. Oxygenated organics and sulfate were dominant aerosol components. However, free tropospheric aerosols were more enriched in sulfate, frequently acidic, and comprised mainly of highly oxidized low-volatility organic species. In contrast, organic aerosols in the boundary-layer-influenced air masses were less oxidized and appeared to be semivolatile.
Yanqing An, Jianzhong Xu, Lin Feng, Xinghua Zhang, Yanmei Liu, Shichang Kang, Bin Jiang, and Yuhong Liao
Atmos. Chem. Phys., 19, 1115–1128, https://doi.org/10.5194/acp-19-1115-2019, https://doi.org/10.5194/acp-19-1115-2019, 2019
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Detailed molecular chemical composition of water-soluble organic matter in the Himalayas was characterized by positive electrospray ionization Fourier transform ion cyclotron resonance mass spectrometry for the first time. Many products formed from biogenic volatile organic compounds and biomass-burning-emitted compounds were found in the organic compounds, suggesting the important contribution of these two sources in the Himalayas.
Junfeng Wang, Dantong Liu, Xinlei Ge, Yangzhou Wu, Fuzhen Shen, Mindong Chen, Jian Zhao, Conghui Xie, Qingqing Wang, Weiqi Xu, Jie Zhang, Jianlin Hu, James Allan, Rutambhara Joshi, Pingqing Fu, Hugh Coe, and Yele Sun
Atmos. Chem. Phys., 19, 447–458, https://doi.org/10.5194/acp-19-447-2019, https://doi.org/10.5194/acp-19-447-2019, 2019
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This work is part of the UK-China APHH campaign. We used a laser-only Aerodyne soot particle aerosol mass spectrometer, for the first time, to investigate the concentrations, size distributions and chemical compositions for those ambient submicron aerosol particles only with black carbon as cores. Our findings are valuable to understand the BC properties and processes in the densely populated megacities.
Conghui Xie, Weiqi Xu, Junfeng Wang, Qingqing Wang, Dantong Liu, Guiqian Tang, Ping Chen, Wei Du, Jian Zhao, Yingjie Zhang, Wei Zhou, Tingting Han, Qingyun Bian, Jie Li, Pingqing Fu, Zifa Wang, Xinlei Ge, James Allan, Hugh Coe, and Yele Sun
Atmos. Chem. Phys., 19, 165–179, https://doi.org/10.5194/acp-19-165-2019, https://doi.org/10.5194/acp-19-165-2019, 2019
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We present the first simultaneous real-time online measurements of aerosol optical properties at ground level and at 260 m on a meteorological tower in urban Beijing in winter. The vertical similarities and differences in scattering and absorption coefficients were characterized. The increases in MAC of BC were mainly associated with the coating materials on rBC. Coal combustion was the dominant source contribution of brown carbon followed by biomass burning and SOA in winter in Beijing.
Zhiwen Dong, Shichang Kang, Dahe Qin, Yaping Shao, Sven Ulbrich, and Xiang Qin
The Cryosphere, 12, 3877–3890, https://doi.org/10.5194/tc-12-3877-2018, https://doi.org/10.5194/tc-12-3877-2018, 2018
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This study aimed to provide a first and unique record of physicochemical properties and mixing states of LAPs at the glacier and atmosphere interface over the northeastern Tibetan Plateau to determine the individual LAPs' structure aging and mixing state changes through the atmospheric deposition process from atmosphere to glacier–snowpack surface, thereby helping to characterize the LAPs' radiative forcing and climate effects in the cryosphere region.
Peng Sun, Wei Nie, Xuguang Chi, Yuning Xie, Xin Huang, Zheng Xu, Ximeng Qi, Zhengning Xu, Lei Wang, Tianyi Wang, Qi Zhang, and Aijun Ding
Atmos. Chem. Phys., 18, 17177–17190, https://doi.org/10.5194/acp-18-17177-2018, https://doi.org/10.5194/acp-18-17177-2018, 2018
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A total of 2 years of online measurement of particulate nitrate was conducted at the SORPES station in the western Yangtze River Delta, eastern China. Nitrate was found to be the major driver of haze pollution and behaved differently in different seasons. In summer, thermodynamic equilibrium and photochemical processes controlled nitrate formation. In winter, N2O5 hydrolysis was demonstrated to be a major contributor to the nitrate episodes.
Zhiyuan Cong, Shaopeng Gao, Wancang Zhao, Xin Wang, Guangming Wu, Yulan Zhang, Shichang Kang, Yongqin Liu, and Junfeng Ji
The Cryosphere, 12, 3177–3186, https://doi.org/10.5194/tc-12-3177-2018, https://doi.org/10.5194/tc-12-3177-2018, 2018
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Cryoconites from glaciers on the Tibetan Plateau and surrounding area were studied for iron oxides. We found that goethite is the predominant iron oxide form. Using the abundance, speciation and optical properties of iron oxides, the total light absorption was quantitatively attributed to goethite, hematite, black carbon and organic matter. Such findings are essential to understand the relative significance of anthropogenic and natural impacts.
Xintong Chen, Shichang Kang, Zhiyuan Cong, Junhua Yang, and Yaoming Ma
Atmos. Chem. Phys., 18, 12859–12875, https://doi.org/10.5194/acp-18-12859-2018, https://doi.org/10.5194/acp-18-12859-2018, 2018
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To understand the impact of transboundary atmospheric black carbon on the Mt. Everest region and depict the transport pathways in different spatiotemporal scales, we first investigated the concentration level, temporal variation, and sources of black carbon based on high-resolution (2-year) measurements at Qomolangma (Mt. Everest) Station (4276 m a.s.l.). Next, the WRF-Chem simulations were used to reveal the transport mechanisms of black carbon from southern Asia to the Mt. Everest region.
Martine Collaud Coen, Elisabeth Andrews, Diego Aliaga, Marcos Andrade, Hristo Angelov, Nicolas Bukowiecki, Marina Ealo, Paulo Fialho, Harald Flentje, A. Gannet Hallar, Rakesh Hooda, Ivo Kalapov, Radovan Krejci, Neng-Huei Lin, Angela Marinoni, Jing Ming, Nhat Anh Nguyen, Marco Pandolfi, Véronique Pont, Ludwig Ries, Sergio Rodríguez, Gerhard Schauer, Karine Sellegri, Sangeeta Sharma, Junying Sun, Peter Tunved, Patricio Velasquez, and Dominique Ruffieux
Atmos. Chem. Phys., 18, 12289–12313, https://doi.org/10.5194/acp-18-12289-2018, https://doi.org/10.5194/acp-18-12289-2018, 2018
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High altitude stations are often emphasized as free tropospheric measuring sites but they remain influenced by atmospheric boundary layer. An ABL-TopoIndex is defined from a topography analysis around the stations. This new index allows ranking stations as a function of the ABL influence due to topography or help to choose a new site to sample FT. The ABL-TopoIndex is validated by aerosol optical properties and number concentration measured at 29 high altitude stations of five continents.
Wei Zhou, Jian Zhao, Bin Ouyang, Archit Mehra, Weiqi Xu, Yuying Wang, Thomas J. Bannan, Stephen D. Worrall, Michael Priestley, Asan Bacak, Qi Chen, Conghui Xie, Qingqing Wang, Junfeng Wang, Wei Du, Yingjie Zhang, Xinlei Ge, Penglin Ye, James D. Lee, Pingqing Fu, Zifa Wang, Douglas Worsnop, Roderic Jones, Carl J. Percival, Hugh Coe, and Yele Sun
Atmos. Chem. Phys., 18, 11581–11597, https://doi.org/10.5194/acp-18-11581-2018, https://doi.org/10.5194/acp-18-11581-2018, 2018
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We present measurements of gas-phase N2O5 and ClNO2 by ToF-CIMS during summer in urban Beijing as part of the APHH campaign. High reactivity of N2O5 indicative of active nocturnal chemistry was observed. The lifetime of N2O5 as a function of aerosol surface area and relative humidity was characterized, and N2O5 uptake coefficients were estimated. We also found that the N2O5 loss in this study is mainly attributed to its indirect loss via reactions of NO3 with VOCs and NO.
Cenlin He, Mark G. Flanner, Fei Chen, Michael Barlage, Kuo-Nan Liou, Shichang Kang, Jing Ming, and Yun Qian
Atmos. Chem. Phys., 18, 11507–11527, https://doi.org/10.5194/acp-18-11507-2018, https://doi.org/10.5194/acp-18-11507-2018, 2018
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Snow albedo plays a key role in the Earth and climate system. It can be affected by impurities and snow properties. This study implements new parameterizations into a widely used snow model to account for effects of snow shape and black carbon–snow mixing state on snow albedo reduction in the Tibetan Plateau. This study points toward an imperative need for extensive measurements and improved model characterization of snow grain shape and aerosol–snow mixing state in Tibet and elsewhere.
Xiufeng Yin, Shichang Kang, Benjamin de Foy, Yaoming Ma, Yindong Tong, Wei Zhang, Xuejun Wang, Guoshuai Zhang, and Qianggong Zhang
Atmos. Chem. Phys., 18, 10557–10574, https://doi.org/10.5194/acp-18-10557-2018, https://doi.org/10.5194/acp-18-10557-2018, 2018
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Total gaseous mercury concentrations were measured at Nam Co Station on the inland Tibetan Plateau for ~ 3 years. The mean concentration of TGM during the entire monitoring period was 1.33 ± 0.24 ngm-3, ranking it the lowest in China and indicating the pristine atmospheric environment of the inland Tibetan Plateau. Variation of TGM at Nam Co was affected by regional surface reemission, vertical mixing and long-range transported atmospheric mercury, which was associated with the Indian monsoon.
Yele Sun, Weiqi Xu, Qi Zhang, Qi Jiang, Francesco Canonaco, André S. H. Prévôt, Pingqing Fu, Jie Li, John Jayne, Douglas R. Worsnop, and Zifa Wang
Atmos. Chem. Phys., 18, 8469–8489, https://doi.org/10.5194/acp-18-8469-2018, https://doi.org/10.5194/acp-18-8469-2018, 2018
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We present a 2–year analysis of organic aerosol (OA) from highly time–resolved measurements by an aerosol chemical speciation monitor in the megacity of Beijing. The sources of OA were analyzed with the advanced factor analysis of a multilinear engine (ME-2). Our results showed very different seasonal patterns, relative humidity and temperature dependence, and sources regions among different OA factors. The sources and processes of OA factors, and their roles in haze pollution are elucidated.
Hwajin Kim, Qi Zhang, and Jongbae Heo
Atmos. Chem. Phys., 18, 7149–7168, https://doi.org/10.5194/acp-18-7149-2018, https://doi.org/10.5194/acp-18-7149-2018, 2018
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Aerosol chemistry, sources and processes driving the observed temporal and diurnal variations of PM were studied in the Seoul Metropolitan Area (SMA) during spring 2016. An in-depth analysis of the data uncovered that air quality in SMA was influenced strongly by secondary aerosol formation. Also, it was found that the haze episode during spring was mainly caused by a combination of both regional and local factors, which is different from the winter haze mainly caused by intense local sources.
Kai Tang, Zhongwei Huang, Jianping Huang, Teruya Maki, Shuang Zhang, Atsushi Shimizu, Xiaojun Ma, Jinsen Shi, Jianrong Bi, Tian Zhou, Guoyin Wang, and Lei Zhang
Atmos. Chem. Phys., 18, 7131–7148, https://doi.org/10.5194/acp-18-7131-2018, https://doi.org/10.5194/acp-18-7131-2018, 2018
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To our knowledge, this is the first simultaneous field measurement of bioaerosols in dust events at four sites along the transport pathway of Asian dust. The samples were analyzed by means of fluorescence microscopy, scanning electron microscopy, and MiSeq sequencing analysis. The results indicate that dust clouds can carry many bacteria of various types into downwind regions, the alpha and beta diversity of which were investigated.
Hewen Niu, Shichang Kang, Hailong Wang, Rudong Zhang, Xixi Lu, Yun Qian, Rukumesh Paudyal, Shijin Wang, Xiaofei Shi, and Xingguo Yan
Atmos. Chem. Phys., 18, 6441–6460, https://doi.org/10.5194/acp-18-6441-2018, https://doi.org/10.5194/acp-18-6441-2018, 2018
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Deposition of light-absorbing carbonaceous aerosol on the surface of glaciers can greatly alter the energy fluxes of glaciers. Two years of continuous observations of carbonaceous aerosols in a glacierized region are analyzed. We mainly studied the light absorption properties of carbonaceous aerosol and have employed a global aerosol–climate model to estimate source attributions of atmospheric black carbon.
D. Rupakheti, S. Kang, Z. Cong, M. Rupakheti, L. Tripathee, A. K. Panday, and B. Holben
Int. Arch. Photogramm. Remote Sens. Spatial Inf. Sci., XLII-3, 1493–1497, https://doi.org/10.5194/isprs-archives-XLII-3-1493-2018, https://doi.org/10.5194/isprs-archives-XLII-3-1493-2018, 2018
Dean B. Atkinson, Mikhail Pekour, Duli Chand, James G. Radney, Katheryn R. Kolesar, Qi Zhang, Ari Setyan, Norman T. O'Neill, and Christopher D. Cappa
Atmos. Chem. Phys., 18, 5499–5514, https://doi.org/10.5194/acp-18-5499-2018, https://doi.org/10.5194/acp-18-5499-2018, 2018
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We use in situ measurements of particle light extinction to assess the performance of a typical aerosol remote retrieval method. The retrieved fine-mode fraction of extinction, a property commonly used to characterize the anthropogenic influence on the aerosol optical depth, compares well with the in situ measurements as does the retrieved effective fine-mode radius, which characterizes the average size of the particles that contribute most to scattering.
Chaman Gul, Siva Praveen Puppala, Shichang Kang, Bhupesh Adhikary, Yulan Zhang, Shaukat Ali, Yang Li, and Xiaofei Li
Atmos. Chem. Phys., 18, 4981–5000, https://doi.org/10.5194/acp-18-4981-2018, https://doi.org/10.5194/acp-18-4981-2018, 2018
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Snow and ice samples were collected from six glaciers and multiple mountain valleys from northern Pakistan. Samples were analyzed for black carbon and water-insoluble organic carbon. Relatively high concentrations of black carbon, organic carbon, and dust were reported. Snow albedo and radiative forcing were estimated for the snow samples. Possible source regions of pollutants were identified through various techniques.
Xinghua Zhang, Jianzhong Xu, Shichang Kang, Yanmei Liu, and Qi Zhang
Atmos. Chem. Phys., 18, 4617–4638, https://doi.org/10.5194/acp-18-4617-2018, https://doi.org/10.5194/acp-18-4617-2018, 2018
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Highly time and chemically resolved submicron aerosol properties were characterized online for the first time in a high-altitude site (Qomolangma station, 4276 m a.s.l.) in the northern Himalayas by using the Aerodyne HR-ToF-AMS. Biomass burning plumes were frequently observed and the dynamic processes (emissions, transport, and chemical processing) were characterized. The source and chemical composition of organic aerosol were further elucidated using positive matrix factorization analysis.
Haipeng Wang, Jianhui Chen, Shengda Zhang, David D. Zhang, Zongli Wang, Qinghai Xu, Shengqian Chen, Shijin Wang, Shichang Kang, and Fahu Chen
Clim. Past, 14, 383–396, https://doi.org/10.5194/cp-14-383-2018, https://doi.org/10.5194/cp-14-383-2018, 2018
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The chironomid-inferred temperature record from Gonghai Lake exhibits a stepwise decreasing trend since 4 ka. A cold event in the Era of Disunity, the Sui-Tang Warm Period, the Medieval Warm Period and the Little Ice Age can all be recognized in our record, as well as in many other temperature reconstructions in China. Local wars in Shanxi Province, documented in the historical literature during the past 2700 years, are statistically significantly correlated with changes in temperature.
Xin Wang, Hui Wen, Jinsen Shi, Jianrong Bi, Zhongwei Huang, Beidou Zhang, Tian Zhou, Kaiqi Fu, Quanliang Chen, and Jinyuan Xin
Atmos. Chem. Phys., 18, 2119–2138, https://doi.org/10.5194/acp-18-2119-2018, https://doi.org/10.5194/acp-18-2119-2018, 2018
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A ground-based mobile laboratory was deployed near the dust source regions over northwestern China.
We not only captured natural dust but also characterized the properties of anthropogenic soil dust produced by agricultural cultivations.
The results indicate that large differences were found between the optical and microphysical properties of anthropogenic and natural dust.
Yulan Zhang, Shichang Kang, Michael Sprenger, Zhiyuan Cong, Tanguang Gao, Chaoliu Li, Shu Tao, Xiaofei Li, Xinyue Zhong, Min Xu, Wenjun Meng, Bigyan Neupane, Xiang Qin, and Mika Sillanpää
The Cryosphere, 12, 413–431, https://doi.org/10.5194/tc-12-413-2018, https://doi.org/10.5194/tc-12-413-2018, 2018
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Light-absorbing impurities deposited on snow can reduce surface albedo and contribute to the near-worldwide melting of snowpack and ice. This study focused on the black carbon and mineral dust in snow cover on the Tibetan Plateau. We discussed their concentrations, distributions, possible sources, and albedo reduction and radiative forcing. Findings indicated that the impacts of black carbon and mineral dust need to be properly accounted for in future regional climate projections.
Yangzhou Wu, Xinlei Ge, Junfeng Wang, Yafei Shen, Zhaolian Ye, Shun Ge, Yun Wu, Huan Yu, and Mindong Chen
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acp-2018-75, https://doi.org/10.5194/acp-2018-75, 2018
Preprint withdrawn
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This work presents results regarding the secondary aerosol formations in suburan Nanjing, a site downwind of an industrial zone. We show that under such an industrialized environment, secondary species overwhelmingly dominate the fine particle mass, and moisture (relative humidity) is critical in enhancing formations of sulfate, nitrate and the most oxygenated portion of OA, while less oxygenated secondary OA was mainly driven by photochemical processing.
Xinyue Zhong, Tingjun Zhang, Shichang Kang, Kang Wang, Lei Zheng, Yuantao Hu, and Huijuan Wang
The Cryosphere, 12, 227–245, https://doi.org/10.5194/tc-12-227-2018, https://doi.org/10.5194/tc-12-227-2018, 2018
Xiaojing Shen, Junying Sun, Niku Kivekäs, Adam Kristensson, Xiaoye Zhang, Yangmei Zhang, Lu Zhang, Ruxia Fan, Xuefei Qi, Qianli Ma, and Huaigang Zhou
Atmos. Chem. Phys., 18, 587–599, https://doi.org/10.5194/acp-18-587-2018, https://doi.org/10.5194/acp-18-587-2018, 2018
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In this study we used the NanoMap method by applying back trajectories and particle number size distribution in different rural sites in China to evaluate the spatial distribution of NPF events and their occurrence probability. We found difference in the horizontal spatial distribution of new particle source areas was connected to typical meteorological conditions. The horizontal extent of NPF reached to larger than 500 km at two sites, favoured by the fast transport of northwesterly air masses.
Jianzhong Xu, Qi Zhang, Jinsen Shi, Xinlei Ge, Conghui Xie, Junfeng Wang, Shichang Kang, Ruixiong Zhang, and Yuhang Wang
Atmos. Chem. Phys., 18, 427–443, https://doi.org/10.5194/acp-18-427-2018, https://doi.org/10.5194/acp-18-427-2018, 2018
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This manuscript presents results from a comprehensive field study using an HR-AMS coupled with a suite of other instruments in central Tibetan Plateau. The study discusses the chemical composition, sources, and processes of submicron aerosol during the transition from pre-monsoon to monsoon. Organic aerosol was overall highly oxidized during the entire study with higher O / C ratios during the pre-monsoon period. Sensitivity of air pollution transport with synoptic process was also evaluated.
Lin Feng, Yanqing An, Jianzhong Xu, Shichang Kang, Xiaofei Li, Yongqiang Zhou, Yunlin Zhang, Bin Jiang, and Yuhong Liao
Biogeosciences Discuss., https://doi.org/10.5194/bg-2017-507, https://doi.org/10.5194/bg-2017-507, 2017
Revised manuscript not accepted
Gouri Prabhakar, Caroline L. Parworth, Xiaolu Zhang, Hwajin Kim, Dominique E. Young, Andreas J. Beyersdorf, Luke D. Ziemba, John B. Nowak, Timothy H. Bertram, Ian C. Faloona, Qi Zhang, and Christopher D. Cappa
Atmos. Chem. Phys., 17, 14747–14770, https://doi.org/10.5194/acp-17-14747-2017, https://doi.org/10.5194/acp-17-14747-2017, 2017
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This work assesses the processes that control the ambient concentrations of particulate nitrate in the the wintertime San Joaquin Valley of California through a combination of aircraft and surface measurements made during the DISCOVER-AQ study. We provide an observational demonstration of how nocturnal production and advection in aloft layers combines with daytime production and loss from entrainment and deposition to give rise to a distinct diurnal profile in surface nitrate concentrations.
Lauren Schmeisser, Elisabeth Andrews, John A. Ogren, Patrick Sheridan, Anne Jefferson, Sangeeta Sharma, Jeong Eun Kim, James P. Sherman, Mar Sorribas, Ivo Kalapov, Todor Arsov, Christo Angelov, Olga L. Mayol-Bracero, Casper Labuschagne, Sang-Woo Kim, András Hoffer, Neng-Huei Lin, Hao-Ping Chia, Michael Bergin, Junying Sun, Peng Liu, and Hao Wu
Atmos. Chem. Phys., 17, 12097–12120, https://doi.org/10.5194/acp-17-12097-2017, https://doi.org/10.5194/acp-17-12097-2017, 2017
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Three methods are used to classify aerosol type from aerosol optical properties measured in situ at 24 surface sites. Classification methods work best at sites with stable, homogenous aerosol at particularly polluted and dust-prone continental and marine sites. Classification methods are poor at remote marine and Arctic sites. Using these methods to extrapolate aerosol type from optical properties can help determine aerosol radiative forcing and improve aerosol satellite retrieval algorithms.
Chaoliu Li, Fangping Yan, Shichang Kang, Pengfei Chen, Xiaowen Han, Zhaofu Hu, Guoshuai Zhang, Ye Hong, Shaopeng Gao, Bin Qu, Zhejing Zhu, Jiwei Li, Bing Chen, and Mika Sillanpää
Atmos. Chem. Phys., 17, 11899–11912, https://doi.org/10.5194/acp-17-11899-2017, https://doi.org/10.5194/acp-17-11899-2017, 2017
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In this study, we found, due to contribution of carbonates, previously reported BC concentration in atmosphere of the Himalayas and Tibetan Plateau (HTP) were overestimated by around 39–52 %. Meanwhile, we found BC deposition of lake cores overestimated the atmospheric deposition of BC in the HTP; BC depositions of glacier region reflected actual values of 17.9 ± 5.3 mg m−2 a−1. The above results are critical for studying atmospheric distribution and chemical transport of BC in and around the HTP.
Xiufeng Yin, Shichang Kang, Benjamin de Foy, Zhiyuan Cong, Jiali Luo, Lang Zhang, Yaoming Ma, Guoshuai Zhang, Dipesh Rupakheti, and Qianggong Zhang
Atmos. Chem. Phys., 17, 11293–11311, https://doi.org/10.5194/acp-17-11293-2017, https://doi.org/10.5194/acp-17-11293-2017, 2017
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We presented 5-year surface ozone measurements at Nam Co in the inland Tibetan Plateau and made a synthesis comparison of diurnal and seasonal patterns on regional and hemispheric scales. Surface ozone at Nam Co is mainly dominated by natural processes and is less influenced by stratospheric intrusions and human activities than on the rim of the Tibetan Plateau. Ozone at Nam Co is representative of background that is valuable for studying ozone-related effects on large scales.
Benjamin N. Murphy, Matthew C. Woody, Jose L. Jimenez, Ann Marie G. Carlton, Patrick L. Hayes, Shang Liu, Nga L. Ng, Lynn M. Russell, Ari Setyan, Lu Xu, Jeff Young, Rahul A. Zaveri, Qi Zhang, and Havala O. T. Pye
Atmos. Chem. Phys., 17, 11107–11133, https://doi.org/10.5194/acp-17-11107-2017, https://doi.org/10.5194/acp-17-11107-2017, 2017
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We incorporate recent findings about the behavior of organic pollutants in urban airsheds into the Community Multiscale Air Quality (CMAQ) model to refine predictions of organic particulate pollution in the United States. The new techniques, which account for the volatility and ongoing chemistry of airborne organic compounds, substantially reduce biases, particularly in the winter time and near emission sources.
Dipesh Rupakheti, Bhupesh Adhikary, Puppala Siva Praveen, Maheswar Rupakheti, Shichang Kang, Khadak Singh Mahata, Manish Naja, Qianggong Zhang, Arnico Kumar Panday, and Mark G. Lawrence
Atmos. Chem. Phys., 17, 11041–11063, https://doi.org/10.5194/acp-17-11041-2017, https://doi.org/10.5194/acp-17-11041-2017, 2017
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For the first time, atmospheric composition was monitored during pre-monsoon season of 2013 at Lumbini (UNESCO world heritage site as birthplace of the Buddha). PM and O3 frequently exceeded WHO guidelines. Pollution concentration, diurnal characteristics and influence of open burning on air quality in Lumbini were investigated. Potential source regions were also identified. Results show that air pollution at this site is of a great concern, requiring prompt attention for mitigation.
Xin Wan, Shichang Kang, Quanlian Li, Dipesh Rupakheti, Qianggong Zhang, Junming Guo, Pengfei Chen, Lekhendra Tripathee, Maheswar Rupakheti, Arnico K. Panday, Wu Wang, Kimitaka Kawamura, Shaopeng Gao, Guangming Wu, and Zhiyuan Cong
Atmos. Chem. Phys., 17, 8867–8885, https://doi.org/10.5194/acp-17-8867-2017, https://doi.org/10.5194/acp-17-8867-2017, 2017
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Biomass burning (BB) tracers in the aerosols in Lumbini, northern IGP, were studied for the first time. The levoglucosan was the predominant tracer and BB significantly contributed to the air quality in Lumbini. Mixed crop residues and hardwood were main burning materials. BB emissions constituted large fraction of OC, especially during the post-monsoon season. The sources of BB aerosols in Lumbini varies seasonally due to the influence of local emissions and long-range transport.
Jianrong Bi, Jianping Huang, Jinsen Shi, Zhiyuan Hu, Tian Zhou, Guolong Zhang, Zhongwei Huang, Xin Wang, and Hongchun Jin
Atmos. Chem. Phys., 17, 7775–7792, https://doi.org/10.5194/acp-17-7775-2017, https://doi.org/10.5194/acp-17-7775-2017, 2017
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We conducted a field campaign on exploring dust aerosol in Dunhuang farmland nearby Gobi deserts. The anthropogenic dust produced by agricultural cultivations exerted a significant superimposed effect on elevated dust loadings. Strong south wind in daytime scavenged the pollution and weak northeast wind at night favorably accumulated air pollutants near the surface. The local emissions remarkably modified the absorptive and optical characteristics of mineral dust in desert source region.
Jinghao Zhai, Xiaohui Lu, Ling Li, Qi Zhang, Ci Zhang, Hong Chen, Xin Yang, and Jianmin Chen
Atmos. Chem. Phys., 17, 7481–7493, https://doi.org/10.5194/acp-17-7481-2017, https://doi.org/10.5194/acp-17-7481-2017, 2017
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The effective density, chemical composition, and optical properties of particles produced by burning rice straw were measured. Density distribution and single-particle mass spectrometry showed the size-dependent external mixing of black carbon, organic carbon, and potassium salts in biomass burning particles. Optical measurements indicated the significant presence of brown carbon in all particles. Though freshly emitted, light absorption enhancement was observed for particles larger than 200 nm.
Wei Pu, Xin Wang, Hailun Wei, Yue Zhou, Jinsen Shi, Zhiyuan Hu, Hongchun Jin, and Quanliang Chen
The Cryosphere, 11, 1213–1233, https://doi.org/10.5194/tc-11-1213-2017, https://doi.org/10.5194/tc-11-1213-2017, 2017
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We conducted a large field campaign to collect snow samples in Xinjiang. We measured insoluble light-absorbing particles with estimated black carbon concentrations of 10–150 ngg-1. We found a probable shift in emission sources with the progression of winter and dominated contributions of BC and OC to light absorption. A PMF model indicated an optimal three-factor/source solution that included industrial pollution, biomass burning, and soil dust.
Haiyan Li, Qi Zhang, Qiang Zhang, Chunrong Chen, Litao Wang, Zhe Wei, Shan Zhou, Caroline Parworth, Bo Zheng, Francesco Canonaco, André S. H. Prévôt, Ping Chen, Hongliang Zhang, Timothy J. Wallington, and Kebin He
Atmos. Chem. Phys., 17, 4751–4768, https://doi.org/10.5194/acp-17-4751-2017, https://doi.org/10.5194/acp-17-4751-2017, 2017
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The sources and aerosol evolution processes of severe pollution episodes were investigated in Handan during wintertime using real-time measurements. An in-depth analysis of the data uncovered that primary emissions from coal combustion and biomass burning together with secondary formation of sulfate (mainly from SO2 emitted by coal combustion) are important driving factors for haze evolution. Our findings provide useful insights into air pollution control in heavily polluted regions.
Zhaolian Ye, Jiashu Liu, Aijun Gu, Feifei Feng, Yuhai Liu, Chenglu Bi, Jianzhong Xu, Ling Li, Hui Chen, Yanfang Chen, Liang Dai, Quanfa Zhou, and Xinlei Ge
Atmos. Chem. Phys., 17, 2573–2592, https://doi.org/10.5194/acp-17-2573-2017, https://doi.org/10.5194/acp-17-2573-2017, 2017
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This work performed a thorough chemical characterization on the fine particulate matter (PM2.5) samples, collected during July 2015 to April 2016 across four seasons in Changzhou for the first time. In particular, an Aerodyne soot particle aerosol mass spectrometer (SP-AMS) was deployed offline to probe the chemical properties and sources of the water-soluble fraction of organic aerosols (WSOAs).
Pengfei Tian, Xianjie Cao, Lei Zhang, Naixiu Sun, Lu Sun, Timothy Logan, Jinsen Shi, Yuan Wang, Yuemeng Ji, Yun Lin, Zhongwei Huang, Tian Zhou, Yingying Shi, and Renyi Zhang
Atmos. Chem. Phys., 17, 2509–2523, https://doi.org/10.5194/acp-17-2509-2017, https://doi.org/10.5194/acp-17-2509-2017, 2017
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We have investigated the vertical distribution and optical properties of aerosols over China using long-term satellite observations from the Cloud–Aerosol Lidar with Orthogonal Polarization, ground-based lidar observations and Aerosol Robotic Network data. Our results provide key information on the long-term aerosol seasonal and spatial variations, optical properties, regional types, long-range transport and atmospheric stability in China for air quality and climate studies.
Shan Zhou, Sonya Collier, Daniel A. Jaffe, Nicole L. Briggs, Jonathan Hee, Arthur J. Sedlacek III, Lawrence Kleinman, Timothy B. Onasch, and Qi Zhang
Atmos. Chem. Phys., 17, 2477–2493, https://doi.org/10.5194/acp-17-2477-2017, https://doi.org/10.5194/acp-17-2477-2017, 2017
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Wildfire plumes in the western US were sampled at a high-elevation site in summer 2013. Three distinct BBOA types were identified, representing biomass burning OA with different degrees of atmospheric processing. Analysis of consecutive BB plumes transported from the same fire source showed that photooxidation led to enhanced mass fractions of aged BBOAs but negligible net OA production. A possible reason is that SOA formation was almost entirely balanced by BBOA volatilization during transport.
Xin Wang, Wei Pu, Yong Ren, Xuelei Zhang, Xueying Zhang, Jinsen Shi, Hongchun Jin, Mingkai Dai, and Quanliang Chen
Atmos. Chem. Phys., 17, 2279–2296, https://doi.org/10.5194/acp-17-2279-2017, https://doi.org/10.5194/acp-17-2279-2017, 2017
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A 2014 snow survey was performed across northeastern China to analyze light absorption of ILAPs in seasonal snow, and modeling studies were conducted to compare snow albedo reduction due to assumptions of internal–external mixing of BC in snow and different snow grain shapes. The results show that the simulated snow albedos from both SAMDS and SNICAR agree well with the observed values at low ILAP mixing ratios, but they tend to be higher than surface observations at high ILAP mixing ratios.
Hwajin Kim, Qi Zhang, Gwi-Nam Bae, Jin Young Kim, and Seung Bok Lee
Atmos. Chem. Phys., 17, 2009–2033, https://doi.org/10.5194/acp-17-2009-2017, https://doi.org/10.5194/acp-17-2009-2017, 2017
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We discuss characteristics, sources, and size distributions of the PM1 composition and OA components in Seoul, Korea, in winter. The serious pollution observed was caused by a combination of various factors, including meteorological conditions, emissions from local primary sources, secondary formation, and transport of air masses from upwind locations. This will be very useful for enacting effective PM reduction strategies for Korea as well as for the broader northern pan-Eurasian region.
Bin Liu, Zhiyuan Cong, Yuesi Wang, Jinyuan Xin, Xin Wan, Yuepeng Pan, Zirui Liu, Yonghong Wang, Guoshuai Zhang, Zhongyan Wang, Yongjie Wang, and Shichang Kang
Atmos. Chem. Phys., 17, 449–463, https://doi.org/10.5194/acp-17-449-2017, https://doi.org/10.5194/acp-17-449-2017, 2017
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The first observation net of background atmospheric aerosols of the Himalayas and Tibetan Plateau were conducted in 2011–2013, and the aerosol mass loadings were especially illustrated in this paper. Consequently, these terrestrial aerosol masses were strongly ecosystem-dependent, with various seasonality and diurnal cycles at these sites. These findings implicate that regional characteristics and fine-particle emissions need to be treated sensitively when assessing their climatic effects.
Jianlin Hu, Peng Wang, Qi Ying, Hongliang Zhang, Jianjun Chen, Xinlei Ge, Xinghua Li, Jingkun Jiang, Shuxiao Wang, Jie Zhang, Yu Zhao, and Yingyi Zhang
Atmos. Chem. Phys., 17, 77–92, https://doi.org/10.5194/acp-17-77-2017, https://doi.org/10.5194/acp-17-77-2017, 2017
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An annual simulation of secondary organic aerosol (SOA) concentrations in China with updated SOA formation pathways reveals that SOA can be a significant contributor to PM2.5 in major urban areas. Summer SOA is dominated by emissions from biogenic sources, while winter SOA is dominated by anthropogenic emissions such as alkanes and aromatic compounds. Reactive surface uptake of dicarbonyls throughout the year and isoprene epoxides in summer is the most important contributor.
Jianzhong Xu, Jinsen Shi, Qi Zhang, Xinlei Ge, Francesco Canonaco, André S. H. Prévôt, Matthias Vonwiller, Sönke Szidat, Jinming Ge, Jianmin Ma, Yanqing An, Shichang Kang, and Dahe Qin
Atmos. Chem. Phys., 16, 14937–14957, https://doi.org/10.5194/acp-16-14937-2016, https://doi.org/10.5194/acp-16-14937-2016, 2016
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This study deployed an AMS field study in Lanzhou, a city in northwestern China, evaluating the chemical composition, sources, and processes of urban aerosols during wintertime. In comparison with the results during summer in Lanzhou, the air pollution during winter was more severe and the sources were more complex. In addition, this paper estimates the contributions of fossil and non-fossil sources of organic carbon to primary and secondary organic carbon using the carbon isotopic method.
Hanna K. Lappalainen, Veli-Matti Kerminen, Tuukka Petäjä, Theo Kurten, Aleksander Baklanov, Anatoly Shvidenko, Jaana Bäck, Timo Vihma, Pavel Alekseychik, Meinrat O. Andreae, Stephen R. Arnold, Mikhail Arshinov, Eija Asmi, Boris Belan, Leonid Bobylev, Sergey Chalov, Yafang Cheng, Natalia Chubarova, Gerrit de Leeuw, Aijun Ding, Sergey Dobrolyubov, Sergei Dubtsov, Egor Dyukarev, Nikolai Elansky, Kostas Eleftheriadis, Igor Esau, Nikolay Filatov, Mikhail Flint, Congbin Fu, Olga Glezer, Aleksander Gliko, Martin Heimann, Albert A. M. Holtslag, Urmas Hõrrak, Juha Janhunen, Sirkku Juhola, Leena Järvi, Heikki Järvinen, Anna Kanukhina, Pavel Konstantinov, Vladimir Kotlyakov, Antti-Jussi Kieloaho, Alexander S. Komarov, Joni Kujansuu, Ilmo Kukkonen, Ella-Maria Duplissy, Ari Laaksonen, Tuomas Laurila, Heikki Lihavainen, Alexander Lisitzin, Alexsander Mahura, Alexander Makshtas, Evgeny Mareev, Stephany Mazon, Dmitry Matishov, Vladimir Melnikov, Eugene Mikhailov, Dmitri Moisseev, Robert Nigmatulin, Steffen M. Noe, Anne Ojala, Mari Pihlatie, Olga Popovicheva, Jukka Pumpanen, Tatjana Regerand, Irina Repina, Aleksei Shcherbinin, Vladimir Shevchenko, Mikko Sipilä, Andrey Skorokhod, Dominick V. Spracklen, Hang Su, Dmitry A. Subetto, Junying Sun, Arkady Y. Terzhevik, Yuri Timofeyev, Yuliya Troitskaya, Veli-Pekka Tynkkynen, Viacheslav I. Kharuk, Nina Zaytseva, Jiahua Zhang, Yrjö Viisanen, Timo Vesala, Pertti Hari, Hans Christen Hansson, Gennady G. Matvienko, Nikolai S. Kasimov, Huadong Guo, Valery Bondur, Sergej Zilitinkevich, and Markku Kulmala
Atmos. Chem. Phys., 16, 14421–14461, https://doi.org/10.5194/acp-16-14421-2016, https://doi.org/10.5194/acp-16-14421-2016, 2016
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After kick off in 2012, the Pan-Eurasian Experiment (PEEX) program has expanded fast and today the multi-disciplinary research community covers ca. 80 institutes and a network of ca. 500 scientists from Europe, Russia, and China. Here we introduce scientific topics relevant in this context. This is one of the first multi-disciplinary overviews crossing scientific boundaries, from atmospheric sciences to socio-economics and social sciences.
Fangping Yan, Shichang Kang, Chaoliu Li, Yulan Zhang, Xiang Qin, Yang Li, Xiaopeng Zhang, Zhaofu Hu, Pengfei Chen, Xiaofei Li, Bin Qu, and Mika Sillanpää
The Cryosphere, 10, 2611–2621, https://doi.org/10.5194/tc-10-2611-2016, https://doi.org/10.5194/tc-10-2611-2016, 2016
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DOC release of Laohugou Glacier No. 12 was 192 kg km−2 yr−1, of which 43.2 % could be decomposed and return to atmosphere as CO2 within 28 days, producing positive feedback in the warming process and influencing downstream ecosystems. Radiative forcing of snow pit DOC was calculated to be 0.43 W m−2, accounting for about 10 % of the radiative forcing caused by BC. Therefore, DOC is also a light-absorbing agent in glacierized regions, influencing the albedo of glacier surface and glacier melting.
Junfeng Wang, Xinlei Ge, Yanfang Chen, Yafei Shen, Qi Zhang, Yele Sun, Jianzhong Xu, Shun Ge, Huan Yu, and Mindong Chen
Atmos. Chem. Phys., 16, 9109–9127, https://doi.org/10.5194/acp-16-9109-2016, https://doi.org/10.5194/acp-16-9109-2016, 2016
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Highly time- and chemically resolved submicron aerosol properties were characterized online for the first time during springtime in Nanjing by using the Aerodyne SP-AMS. Both chemical and size information of black carbon together with other aerosol species were simultaneously determined. An in-depth analysis of the data elucidates the sources and evolution processes of the fine aerosols in the YRD region. Our findings are valuable for air quality remediation in the densely populated regions.
Yele Sun, Wei Du, Pingqing Fu, Qingqing Wang, Jie Li, Xinlei Ge, Qi Zhang, Chunmao Zhu, Lujie Ren, Weiqi Xu, Jian Zhao, Tingting Han, Douglas R. Worsnop, and Zifa Wang
Atmos. Chem. Phys., 16, 8309–8329, https://doi.org/10.5194/acp-16-8309-2016, https://doi.org/10.5194/acp-16-8309-2016, 2016
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We have a comprehensive characterization of the sources, variations and processes of submicron aerosols in Beijing in winter using HR-AMS and GC/MS measurements. The primary sources including traffic, cooking, biomass burning and coal combustion emissions, and secondary components were separated and quantified with PMF. Our results elucidated the important roles of primary emissions, particularly coal combustion, and aqueous-phase processing in the formation of severe air pollution in winter.
Shengyun Chen, Wenjie Liu, Qian Zhao, Lin Zhao, Qingbai Wu, Xingjie Lu, Shichang Kang, Xiang Qin, Shilong Chen, Jiawen Ren, and Dahe Qin
The Cryosphere Discuss., https://doi.org/10.5194/tc-2016-80, https://doi.org/10.5194/tc-2016-80, 2016
Revised manuscript not accepted
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Experimental warming was manipulated using open top chambers in alpine grassland ecosystem in the permafrost regions of the Qinghai-Tibet Plateau. The results revealed variations of earlier thawing, later freezing and longer freezing-thawing periods in shallow soil. Further, the estimated permafrost table declined under the warming scenarios. The work will be helpful to evaluate the stability of Qinghai-Tibet Railway/Highway and estimate the release of carbon under the future climate warming.
Christopher D. Cappa, Katheryn R. Kolesar, Xiaolu Zhang, Dean B. Atkinson, Mikhail S. Pekour, Rahul A. Zaveri, Alla Zelenyuk, and Qi Zhang
Atmos. Chem. Phys., 16, 6511–6535, https://doi.org/10.5194/acp-16-6511-2016, https://doi.org/10.5194/acp-16-6511-2016, 2016
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Measurements of size-dependent aerosol optical properties at visible wavelengths made during the 2010 CARES study are reported on, with a special focus on the characterization of supermicron particles. The relationships with and dependence upon particle composition, particle size, photochemical aging, water uptake and heating are discussed, along with broader implications of these in situ measurements for the interpretation of remote sensing products.
Dominique E. Young, Hwajin Kim, Caroline Parworth, Shan Zhou, Xiaolu Zhang, Christopher D. Cappa, Roger Seco, Saewung Kim, and Qi Zhang
Atmos. Chem. Phys., 16, 5427–5451, https://doi.org/10.5194/acp-16-5427-2016, https://doi.org/10.5194/acp-16-5427-2016, 2016
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Aerosol chemistry and the sources and processes driving the observed temporal and diurnal variations of PM were studied in a polluted urban environment during winter 2013. These results were compared to a similar campaign from winter 2010. Meteorology strongly influenced PM composition, both directly and indirectly. Nighttime reactions played a more important role in 2013 and the influence from a nighttime formed residual layer that mixed down in the morning was also much more intense in 2013.
Holger Baars, Thomas Kanitz, Ronny Engelmann, Dietrich Althausen, Birgit Heese, Mika Komppula, Jana Preißler, Matthias Tesche, Albert Ansmann, Ulla Wandinger, Jae-Hyun Lim, Joon Young Ahn, Iwona S. Stachlewska, Vassilis Amiridis, Eleni Marinou, Patric Seifert, Julian Hofer, Annett Skupin, Florian Schneider, Stephanie Bohlmann, Andreas Foth, Sebastian Bley, Anne Pfüller, Eleni Giannakaki, Heikki Lihavainen, Yrjö Viisanen, Rakesh Kumar Hooda, Sérgio Nepomuceno Pereira, Daniele Bortoli, Frank Wagner, Ina Mattis, Lucja Janicka, Krzysztof M. Markowicz, Peggy Achtert, Paulo Artaxo, Theotonio Pauliquevis, Rodrigo A. F. Souza, Ved Prakesh Sharma, Pieter Gideon van Zyl, Johan Paul Beukes, Junying Sun, Erich G. Rohwer, Ruru Deng, Rodanthi-Elisavet Mamouri, and Felix Zamorano
Atmos. Chem. Phys., 16, 5111–5137, https://doi.org/10.5194/acp-16-5111-2016, https://doi.org/10.5194/acp-16-5111-2016, 2016
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The findings from more than 10 years of global aerosol lidar measurements with Polly systems are summarized, and a data set of optical properties for specific aerosol types is given. An automated data retrieval algorithm for continuous Polly lidar observations is presented and discussed by means of a Saharan dust advection event in Leipzig, Germany. Finally, a statistic on the vertical aerosol distribution including the seasonal variability at PollyNET locations around the globe is presented.
Lu Yu, Jeremy Smith, Alexander Laskin, Katheryn M. George, Cort Anastasio, Julia Laskin, Ann M. Dillner, and Qi Zhang
Atmos. Chem. Phys., 16, 4511–4527, https://doi.org/10.5194/acp-16-4511-2016, https://doi.org/10.5194/acp-16-4511-2016, 2016
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The chemical evolution of SOA formed during aqueous reactions of phenolic compounds is studied via combined bulk and molecular analysis. Phenolic SOA evolve dynamically during photochemical aging, with different reaction mechanisms (oligomerization, fragmentation, and functionalization) leading to different generations of products that span an enormous range in volatilities and a large range in oxidation state and composition. Aqueous reactions of phenols are likely an important source of ELVOC.
Yang Li, Jizu Chen, Shichang Kang, Chaoliu Li, Bin Qu, Lekhendra Tripathee, Fangping Yan, Yulan Zhang, Junmin Guo, Chaman Gul, and Xiang Qin
The Cryosphere Discuss., https://doi.org/10.5194/tc-2016-32, https://doi.org/10.5194/tc-2016-32, 2016
Preprint withdrawn
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To our knowledge, this study constitutes the first quantitative dataset of the impacts of light absorbing particles (LAPs) on glacier ablation estimated directly from the northeastern edge of the Tibetan Plateau (TP).The average concentrations of black carbon (BC) and mineral dust (MD) in surface snow and ice at Laohugou Glacier No. 12 (LHG) were much higher than those detected in snow pits and ice cores in TP and Tien Shan mountains.
S. E. Pusede, K. C. Duffey, A. A. Shusterman, A. Saleh, J. L. Laughner, P. J. Wooldridge, Q. Zhang, C. L. Parworth, H. Kim, S. L. Capps, L. C. Valin, C. D. Cappa, A. Fried, J. Walega, J. B. Nowak, A. J. Weinheimer, R. M. Hoff, T. A. Berkoff, A. J. Beyersdorf, J. Olson, J. H. Crawford, and R. C. Cohen
Atmos. Chem. Phys., 16, 2575–2596, https://doi.org/10.5194/acp-16-2575-2016, https://doi.org/10.5194/acp-16-2575-2016, 2016
L. Kleinman, C. Kuang, A. Sedlacek, G. Senum, S. Springston, J. Wang, Q. Zhang, J. Jayne, J. Fast, J. Hubbe, J. Shilling, and R. Zaveri
Atmos. Chem. Phys., 16, 1729–1746, https://doi.org/10.5194/acp-16-1729-2016, https://doi.org/10.5194/acp-16-1729-2016, 2016
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Atmospheric measurements of total organic aerosol (OA) and tracers of anthropogenic and biogenic emissions are used to quantify synergistic effects (A–B interactions) between two classes of precursors in the formation of OA. Regressions are consistent with the Sacramento plume composed mainly of modern carbon, and OA correlating best with an anthropogenic tracer. It is found that meteorological conditions during a pollution episode can mimic effects of A–B interactions.
Y. Q. Wang, X. Y. Zhang, J. Y. Sun, X. C. Zhang, H. Z. Che, and Y. Li
Atmos. Chem. Phys., 15, 13585–13598, https://doi.org/10.5194/acp-15-13585-2015, https://doi.org/10.5194/acp-15-13585-2015, 2015
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Concentrations of PM10, PM2.5 and PM1 were monitored at 24 stations of CAWNET from 2006 to 2014. The average levels of particulate matter (PM) concentrations and relationships were investigated. Seasonal, interannual and diurnal variations of the PM were revealed. The effects of meteorological factors on the PM were discussed. The highest PM concentrations were observed at the stations of Xian, Zhengzhou and Gucheng, in Guanzhong and the Huabei Plain.
X. Y. Zhang, J. Z. Wang, Y. Q. Wang, H. L. Liu, J. Y. Sun, and Y. M. Zhang
Atmos. Chem. Phys., 15, 12935–12952, https://doi.org/10.5194/acp-15-12935-2015, https://doi.org/10.5194/acp-15-12935-2015, 2015
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No obvious changes were found in annual mean concentrations of major chemical components and PM10 in 2013, relative to 2012. But wintertime mass were quite different; approximately 60% of the winter mass increase from 2012 to 2013 can be attributed to severe meteorological conditions in the HBP area, and mass of chemical components exhibited a decline during 2006 to 2010, and then a rise till 2013. Coal-combustion was still the largest anthropogenic source of aerosol pollution in 2013 in China.
C. Chen, Y. L. Sun, W. Q. Xu, W. Du, L. B. Zhou, T. T. Han, Q. Q. Wang, P. Q. Fu, Z. F. Wang, Z. Q. Gao, Q. Zhang, and D. R. Worsnop
Atmos. Chem. Phys., 15, 12879–12895, https://doi.org/10.5194/acp-15-12879-2015, https://doi.org/10.5194/acp-15-12879-2015, 2015
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A comprehensive characterization of submicron aerosol composition and sources at 260m in urban Beijing during APEC 2014 is presented. Aerosol species were shown to decrease substantially by 40–80% during APEC, whereas the bulk composition was relatively similar to the result of synergetic controls of secondary precursors. Our results elucidated that the good air quality during APEC was the combined result of emission controls and meteorological effects, with the former playing the dominant role.
A. Lupascu, R. Easter, R. Zaveri, M. Shrivastava, M. Pekour, J. Tomlinson, Q. Yang, H. Matsui, A. Hodzic, Q. Zhang, and J. D. Fast
Atmos. Chem. Phys., 15, 12283–12313, https://doi.org/10.5194/acp-15-12283-2015, https://doi.org/10.5194/acp-15-12283-2015, 2015
J. W. Chi, W. J. Li, D. Z. Zhang, J. C. Zhang, Y. T. Lin, X. J. Shen, J. Y. Sun, J. M. Chen, X. Y. Zhang, Y. M. Zhang, and W. X. Wang
Atmos. Chem. Phys., 15, 11341–11353, https://doi.org/10.5194/acp-15-11341-2015, https://doi.org/10.5194/acp-15-11341-2015, 2015
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Sea salt aerosols (SSA) are dominant particles in the Arctic atmosphere. Our result suggests that the hydrophilic MgCl2 coating in fresh SSA likely intrigued the heterogeneous reactions at the beginning of SSA and acidic gases in the Arctic. The content of organic matter increased in the aged SSA compared with the fresh SSA, which suggests organic acids (beside inorganic acids) participate in the ageing of SSA in the Arctic.
Y. L. Sun, Z. F. Wang, W. Du, Q. Zhang, Q. Q. Wang, P. Q. Fu, X. L. Pan, J. Li, J. Jayne, and D. R. Worsnop
Atmos. Chem. Phys., 15, 10149–10165, https://doi.org/10.5194/acp-15-10149-2015, https://doi.org/10.5194/acp-15-10149-2015, 2015
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We conducted the first long-term real-time measurement of submicron aerosol composition in Beijing using an ACSM for 1 year. The seasonal variations of mass concentrations and chemical composition of submicron aerosol were investigated in detail, and the meteorological effects on aerosol chemistry, particularly temperature and relative humidity, were elucidated. Finally, the potential source areas of aerosol species during four seasons were identified.
L. Zhang, J. Y. Sun, X. J. Shen, Y. M. Zhang, H. Che, Q. L. Ma, Y. W. Zhang, X. Y. Zhang, and J. A. Ogren
Atmos. Chem. Phys., 15, 8439–8454, https://doi.org/10.5194/acp-15-8439-2015, https://doi.org/10.5194/acp-15-8439-2015, 2015
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The aerosol hygroscopic properties at a rural background site in the Yangtze River delta of China was discussed. The results show the scattering coefficient and backscattering coefficient increased by 58 and 25% as relative humidity (RH) increased from 40 to 85%, while the hemispheric backscatter fraction decreased by 21%. Aerosol hygroscopic growth caused a 47% increase in calculated aerosol direct radiative forcing at 85% RH compared to the forcing at 40% RH. Nitrate played a vital role.
S. Song, N. E. Selin, A. L. Soerensen, H. Angot, R. Artz, S. Brooks, E.-G. Brunke, G. Conley, A. Dommergue, R. Ebinghaus, T. M. Holsen, D. A. Jaffe, S. Kang, P. Kelley, W. T. Luke, O. Magand, K. Marumoto, K. A. Pfaffhuber, X. Ren, G.-R. Sheu, F. Slemr, T. Warneke, A. Weigelt, P. Weiss-Penzias, D. C. Wip, and Q. Zhang
Atmos. Chem. Phys., 15, 7103–7125, https://doi.org/10.5194/acp-15-7103-2015, https://doi.org/10.5194/acp-15-7103-2015, 2015
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A better knowledge of mercury (Hg) emission fluxes into the global atmosphere is important for assessing its human health impacts and evaluating the effectiveness of corresponding policy actions. We for the first time apply a top-down approach at a global scale to quantitatively estimate present-day mercury emission sources as well as key parameters in a chemical transport model, in order to better constrain the global biogeochemical cycle of mercury.
S. Kang, F. Wang, U. Morgenstern, Y. Zhang, B. Grigholm, S. Kaspari, M. Schwikowski, J. Ren, T. Yao, D. Qin, and P. A. Mayewski
The Cryosphere, 9, 1213–1222, https://doi.org/10.5194/tc-9-1213-2015, https://doi.org/10.5194/tc-9-1213-2015, 2015
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J. Z. Xu, Q. Zhang, Z. B. Wang, G. M. Yu, X. L. Ge, and X. Qin
Atmos. Chem. Phys., 15, 5069–5081, https://doi.org/10.5194/acp-15-5069-2015, https://doi.org/10.5194/acp-15-5069-2015, 2015
D. B. Atkinson, J. G. Radney, J. Lum, K. R. Kolesar, D. J. Cziczo, M. S. Pekour, Q. Zhang, A. Setyan, A. Zelenyuk, and C. D. Cappa
Atmos. Chem. Phys., 15, 4045–4061, https://doi.org/10.5194/acp-15-4045-2015, https://doi.org/10.5194/acp-15-4045-2015, 2015
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This work describes an analysis of measurements of the influence of water uptake on the light-scattering properties of sub- and supermicron-sized particles as observed in the Sacramento, CA, USA region during the 2010 CARES field campaign. The observations are used to derive campaign-average effective hygroscopicity parameters for submicron oxygenated organic aerosol and for supermicron particles, and the influence of chloride displacement reactions on particle hygroscopicity is examined.
L. Yu, J. Smith, A. Laskin, C. Anastasio, J. Laskin, and Q. Zhang
Atmos. Chem. Phys., 14, 13801–13816, https://doi.org/10.5194/acp-14-13801-2014, https://doi.org/10.5194/acp-14-13801-2014, 2014
J. Xu, Q. Zhang, M. Chen, X. Ge, J. Ren, and D. Qin
Atmos. Chem. Phys., 14, 12593–12611, https://doi.org/10.5194/acp-14-12593-2014, https://doi.org/10.5194/acp-14-12593-2014, 2014
Y. M. Zhang, X. Y. Zhang, J. Y. Sun, G. Y. Hu, X. J. Shen, Y. Q. Wang, T. T. Wang, D. Z. Wang, and Y. Zhao
Atmos. Chem. Phys., 14, 12237–12249, https://doi.org/10.5194/acp-14-12237-2014, https://doi.org/10.5194/acp-14-12237-2014, 2014
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An AMS was employed to measure the mass and size distributions of PM1 at an elevated site. Features of PM1 at four seasons, during different kinds of episodes including NPF, polluted, PBL, LFT and in-cloud, were discussed. The characterizations of PM1 at seven clusters of air masses were also analyzed. BBOA, CCOA and oxidized organic aerosols were resolved by AMS-PMF (positive matrix function). Almost half of OA were oxidized, and BBOA is 34% of OA in summer; CCOA is 22% of OA in winter as well.
K. Tsigaridis, N. Daskalakis, M. Kanakidou, P. J. Adams, P. Artaxo, R. Bahadur, Y. Balkanski, S. E. Bauer, N. Bellouin, A. Benedetti, T. Bergman, T. K. Berntsen, J. P. Beukes, H. Bian, K. S. Carslaw, M. Chin, G. Curci, T. Diehl, R. C. Easter, S. J. Ghan, S. L. Gong, A. Hodzic, C. R. Hoyle, T. Iversen, S. Jathar, J. L. Jimenez, J. W. Kaiser, A. Kirkevåg, D. Koch, H. Kokkola, Y. H Lee, G. Lin, X. Liu, G. Luo, X. Ma, G. W. Mann, N. Mihalopoulos, J.-J. Morcrette, J.-F. Müller, G. Myhre, S. Myriokefalitakis, N. L. Ng, D. O'Donnell, J. E. Penner, L. Pozzoli, K. J. Pringle, L. M. Russell, M. Schulz, J. Sciare, Ø. Seland, D. T. Shindell, S. Sillman, R. B. Skeie, D. Spracklen, T. Stavrakou, S. D. Steenrod, T. Takemura, P. Tiitta, S. Tilmes, H. Tost, T. van Noije, P. G. van Zyl, K. von Salzen, F. Yu, Z. Wang, Z. Wang, R. A. Zaveri, H. Zhang, K. Zhang, Q. Zhang, and X. Zhang
Atmos. Chem. Phys., 14, 10845–10895, https://doi.org/10.5194/acp-14-10845-2014, https://doi.org/10.5194/acp-14-10845-2014, 2014
J. D. Fast, J. Allan, R. Bahreini, J. Craven, L. Emmons, R. Ferrare, P. L. Hayes, A. Hodzic, J. Holloway, C. Hostetler, J. L. Jimenez, H. Jonsson, S. Liu, Y. Liu, A. Metcalf, A. Middlebrook, J. Nowak, M. Pekour, A. Perring, L. Russell, A. Sedlacek, J. Seinfeld, A. Setyan, J. Shilling, M. Shrivastava, S. Springston, C. Song, R. Subramanian, J. W. Taylor, V. Vinoj, Q. Yang, R. A. Zaveri, and Q. Zhang
Atmos. Chem. Phys., 14, 10013–10060, https://doi.org/10.5194/acp-14-10013-2014, https://doi.org/10.5194/acp-14-10013-2014, 2014
A. Setyan, C. Song, M. Merkel, W. B. Knighton, T. B. Onasch, M. R. Canagaratna, D. R. Worsnop, A. Wiedensohler, J. E. Shilling, and Q. Zhang
Atmos. Chem. Phys., 14, 6477–6494, https://doi.org/10.5194/acp-14-6477-2014, https://doi.org/10.5194/acp-14-6477-2014, 2014
C. Knote, A. Hodzic, J. L. Jimenez, R. Volkamer, J. J. Orlando, S. Baidar, J. Brioude, J. Fast, D. R. Gentner, A. H. Goldstein, P. L. Hayes, W. B. Knighton, H. Oetjen, A. Setyan, H. Stark, R. Thalman, G. Tyndall, R. Washenfelder, E. Waxman, and Q. Zhang
Atmos. Chem. Phys., 14, 6213–6239, https://doi.org/10.5194/acp-14-6213-2014, https://doi.org/10.5194/acp-14-6213-2014, 2014
H. Che, X. Xia, J. Zhu, Z. Li, O. Dubovik, B. Holben, P. Goloub, H. Chen, V. Estelles, E. Cuevas-Agulló, L. Blarel, H. Wang, H. Zhao, X. Zhang, Y. Wang, J. Sun, R. Tao, X. Zhang, and G. Shi
Atmos. Chem. Phys., 14, 2125–2138, https://doi.org/10.5194/acp-14-2125-2014, https://doi.org/10.5194/acp-14-2125-2014, 2014
Z. B. Wang, M. Hu, J. Y. Sun, Z. J. Wu, D. L. Yue, X. J. Shen, Y. M. Zhang, X. Y. Pei, Y. F. Cheng, and A. Wiedensohler
Atmos. Chem. Phys., 13, 12495–12506, https://doi.org/10.5194/acp-13-12495-2013, https://doi.org/10.5194/acp-13-12495-2013, 2013
F. Mei, A. Setyan, Q. Zhang, and J. Wang
Atmos. Chem. Phys., 13, 12155–12169, https://doi.org/10.5194/acp-13-12155-2013, https://doi.org/10.5194/acp-13-12155-2013, 2013
M. Gyawali, W. P. Arnott, R. A. Zaveri, C. Song, M. Pekour, B. Flowers, M. K. Dubey, A. Setyan, Q. Zhang, J. W. Harworth, J. G. Radney, D. B. Atkinson, S. China, C. Mazzoleni, K. Gorkowski, R. Subramanian, B. T. Jobson, and H. Moosmüller
Atmos. Chem. Phys. Discuss., https://doi.org/10.5194/acpd-13-7113-2013, https://doi.org/10.5194/acpd-13-7113-2013, 2013
Revised manuscript not accepted
Related subject area
Domain: ESSD – Atmosphere | Subject: Atmospheric chemistry and physics
ARMTRAJ: a set of multipurpose trajectory datasets augmenting the Atmospheric Radiation Measurement (ARM) user facility measurements
Atmospheric Radiation Measurement (ARM) airborne field campaign data products between 2013 and 2018
CREST: a Climate Data Record of Stratospheric Aerosols
Multiyear high-temporal-resolution measurements of submicron aerosols at 13 French urban sites: data processing and chemical composition
Large synthesis of in situ field measurements of the size distribution of mineral dust aerosols across their life cycles
A 10 km daily-level ultraviolet-radiation-predicting dataset based on machine learning models in China from 2005 to 2020
GHOST: a globally harmonised dataset of surface atmospheric composition measurements
Changes in air pollutant emissions in China during two clean-air action periods derived from the newly developed Inversed Emission Inventory for Chinese Air Quality (CAQIEI)
Version 1 NOAA-20/OMPS Nadir Mapper total column SO2 product: continuation of NASA long-term global data record
GERB Obs4MIPs: a dataset for evaluating diurnal and monthly variations in top-of-atmosphere radiative fluxes in climate models
Multiwavelength aerosol lidars at the Maïdo supersite, Réunion Island, France: instrument description, data processing chain, and quality assessment
PM2.5 concentrations based on near-surface visibility in the Northern Hemisphere from 1959 to 2022
MAP-IO: an atmospheric and marine observatory program on board Marion Dufresne over the Southern Ocean
Retrieving ground-level PM2.5 concentrations in China (2013–2021) with a numerical-model-informed testbed to mitigate sample-imbalance-induced biases
Reconstructing long-term (1980–2022) daily ground particulate matter concentrations in India (LongPMInd)
Calm ocean, stormy sea: Atmospheric and oceanographic observations of the Atlantic during the ARC ship campaign
A comprehensive in-situ and remote sensing data set collected during the HALO–(AC)3 aircraft campaign
Visibility-derived aerosol optical depth over global land from 1959 to 2021
Characterizing clouds with the CCClim dataset, a machine learning cloud class climatology
A Level 3 monthly gridded ice cloud dataset derived from 12 years of CALIOP measurements
IPB-MSA&SO4: a daily 0.25° resolution dataset of in situ-produced biogenic methanesulfonic acid and sulfate over the North Atlantic during 1998–2022 based on machine learning
Indicators of Global Climate Change 2023: annual update of key indicators of the state of the climate system and human influence
The Total Carbon Column Observing Network's GGG2020 data version
Global anthropogenic emissions (CAMS-GLOB-ANT) for the Copernicus Atmosphere Monitoring Service simulations of air quality forecasts and reanalyses
Deep Convective Microphysics Experiment (DCMEX) coordinated aircraft and ground observations: microphysics, aerosol, and dynamics during cumulonimbus development
Introduction to the NJIAS Himawari-8/9 Cloud Feature Dataset for climate and typhoon research
The Tibetan Plateau space-based tropospheric aerosol climatology: 2007–2020
PalVol v1: a proxy-based semi-stochastic ensemble reconstruction of volcanic stratospheric sulfur injection for the last glacial cycle (140 000–50 BP)
Ground- and ship-based microwave radiometer measurements during EUREC4A
Shortwave and longwave components of the surface radiation budget measured at the Thule High Arctic Atmospheric Observatory, Northern Greenland
Cloud condensation nuclei concentrations derived from the CAMS reanalysis
A merged continental planetary boundary layer height dataset based on high-resolution radiosonde measurements, ERA5 reanalysis, and GLDAS
12 years of continuous atmospheric O2, CO2 and APO data from Weybourne Atmospheric Observatory in the United Kingdom
CLAAS-3: the third edition of the CM SAF cloud data record based on SEVIRI observations
Using machine learning to construct TOMCAT model and occultation measurement-based stratospheric methane (TCOM-CH4) and nitrous oxide (TCOM-N2O) profile data sets
High-resolution aerosol data from the top 3.8 kyr of the East Greenland Ice coring Project (EGRIP) ice core
A database of aircraft measurements of carbon monoxide (CO) with high temporal and spatial resolution during 2011–2021
A first global height-resolved cloud condensation nuclei data set derived from spaceborne lidar measurements
A monthly 1° resolution dataset of daytime cloud fraction over the Arctic during 2000–2020 based on multiple satellite products
Network for the Detection of Atmospheric Composition Change (NDACC) Fourier transform infrared (FTIR) trace gas measurements at the University of Toronto Atmospheric Observatory from 2002 to 2020
Deconstruction of tropospheric chemical reactivity using aircraft measurements: the Atmospheric Tomography Mission (ATom) data
Spatial variability of Saharan dust deposition revealed through a citizen science campaign
Radiative sensitivity quantified by a new set of radiation flux kernels based on the ECMWF Reanalysis v5 (ERA5)
Updated observations of clouds by MODIS for global model assessment
An extensive database of airborne trace gas and meteorological observations from the Alpha Jet Atmospheric eXperiment (AJAX)
Two years of volatile organic compound online in situ measurements at the Site Instrumental de Recherche par Télédétection Atmosphérique (Paris region, France) using proton-transfer-reaction mass spectrometry
Global Ozone Monitoring Experiment-2 (GOME-2) daily and monthly level-3 products of atmospheric trace gas columns
Crowdsourced Doppler measurements of time standard stations demonstrating ionospheric variability
A machine learning approach to address air quality changes during the COVID-19 lockdown in Buenos Aires, Argentina
Version 2 of the global catalogue of large anthropogenic and volcanic SO2 sources and emissions derived from satellite measurements
Israel Silber, Jennifer M. Comstock, Michael R. Kieburtz, and Lynn M. Russell
Earth Syst. Sci. Data, 17, 29–42, https://doi.org/10.5194/essd-17-29-2025, https://doi.org/10.5194/essd-17-29-2025, 2025
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We present ARMTRAJ, a set of multipurpose trajectory datasets, which augments cloud, aerosol, and boundary layer studies utilizing the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) user facility data. ARMTRAJ data include ensemble run statistics that enhance consistency and serve as uncertainty metrics for air mass coordinates and state variables. ARMTRAJ will soon become a near real-time product that will accompany past, ongoing, and future ARM deployments.
Fan Mei, Jennifer M. Comstock, Mikhail S. Pekour, Jerome D. Fast, Krista L. Gaustad, Beat Schmid, Shuaiqi Tang, Damao Zhang, John E. Shilling, Jason M. Tomlinson, Adam C. Varble, Jian Wang, L. Ruby Leung, Lawrence Kleinman, Scot Martin, Sebastien C. Biraud, Brian D. Ermold, and Kenneth W. Burk
Earth Syst. Sci. Data, 16, 5429–5448, https://doi.org/10.5194/essd-16-5429-2024, https://doi.org/10.5194/essd-16-5429-2024, 2024
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Our study explores a comprehensive dataset from airborne field studies (2013–2018) conducted using the US Department of Energy's Gulfstream 1 (G-1). The 236 flights span diverse regions, including the Arctic, US Southern Great Plains, US West Coast, eastern North Atlantic, Amazon Basin in Brazil, and Sierras de Córdoba range in Argentina. This dataset provides unique insights into atmospheric dynamics, aerosols, and clouds and makes data available in a more accessible format.
Viktoria F. Sofieva, Alexei Rozanov, Monika Szelag, John P. Burrows, Christian Retscher, Robert Damadeo, Doug Degenstein, Landon A. Rieger, and Adam Bourassa
Earth Syst. Sci. Data, 16, 5227–5241, https://doi.org/10.5194/essd-16-5227-2024, https://doi.org/10.5194/essd-16-5227-2024, 2024
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Climate-related studies need information about the distribution of stratospheric aerosols, which influence the energy balance of the Earth’s atmosphere. In this work, we present a merged dataset of vertically resolved stratospheric aerosol extinction coefficients, which is derived from data of six limb and occultation satellite instruments. The created aerosol climate record covers the period from October 1984 to December 2023. It can be used in various climate-related studies.
Hasna Chebaicheb, Joel F. de Brito, Tanguy Amodeo, Florian Couvidat, Jean-Eudes Petit, Emmanuel Tison, Gregory Abbou, Alexia Baudic, Mélodie Chatain, Benjamin Chazeau, Nicolas Marchand, Raphaële Falhun, Florie Francony, Cyril Ratier, Didier Grenier, Romain Vidaud, Shouwen Zhang, Gregory Gille, Laurent Meunier, Caroline Marchand, Véronique Riffault, and Olivier Favez
Earth Syst. Sci. Data, 16, 5089–5109, https://doi.org/10.5194/essd-16-5089-2024, https://doi.org/10.5194/essd-16-5089-2024, 2024
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Long-term (2015–2021) quasi-continuous measurements have been obtained at 13 French urban sites using online mass spectrometry, to acquire the comprehensive chemical composition of submicron particulate matter. The results show their spatial and temporal differences and confirm the predominance of organics in France (40–60 %). These measurements can be used for many future studies, such as trend and epidemiological analyses, or comparisons with chemical transport models.
Paola Formenti and Claudia Di Biagio
Earth Syst. Sci. Data, 16, 4995–5007, https://doi.org/10.5194/essd-16-4995-2024, https://doi.org/10.5194/essd-16-4995-2024, 2024
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Particles from deserts and semi-vegetated areas (mineral dust) are important for Earth's climate and human health, notably depending on their size. In this paper we collect and make a synthesis of a body of these observations since 1972 in order to provide researchers modeling Earth's climate and developing satellite observations from space with a simple way of confronting their results and understanding their validity.
Yichen Jiang, Su Shi, Xinyue Li, Chang Xu, Haidong Kan, Bo Hu, and Xia Meng
Earth Syst. Sci. Data, 16, 4655–4672, https://doi.org/10.5194/essd-16-4655-2024, https://doi.org/10.5194/essd-16-4655-2024, 2024
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Limited ultraviolet (UV) measurements hindered further investigation of its health effects. This study used a machine learning algorithm to predict UV radiation with a daily and 10 km resolution of high accuracy in mainland China in 2005–2020. Then, uneven spatial distribution and population exposure risks as well as increased temporal trend of UV radiation were found in China. The long-term and high-quality UV dataset could further facilitate health-related research in the future.
Dene Bowdalo, Sara Basart, Marc Guevara, Oriol Jorba, Carlos Pérez García-Pando, Monica Jaimes Palomera, Olivia Rivera Hernandez, Melissa Puchalski, David Gay, Jörg Klausen, Sergio Moreno, Stoyka Netcheva, and Oksana Tarasova
Earth Syst. Sci. Data, 16, 4417–4495, https://doi.org/10.5194/essd-16-4417-2024, https://doi.org/10.5194/essd-16-4417-2024, 2024
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GHOST (Globally Harmonised Observations in Space and Time) represents one of the biggest collections of harmonised measurements of atmospheric composition at the surface. In total, 7 275 148 646 measurements from 1970 to 2023, from 227 different components, and from 38 reporting networks are compiled, parsed, and standardised. Components processed include gaseous species, total and speciated particulate matter, and aerosol optical properties.
Lei Kong, Xiao Tang, Zifa Wang, Jiang Zhu, Jianjun Li, Huangjian Wu, Qizhong Wu, Huansheng Chen, Lili Zhu, Wei Wang, Bing Liu, Qian Wang, Duohong Chen, Yuepeng Pan, Jie Li, Lin Wu, and Gregory R. Carmichael
Earth Syst. Sci. Data, 16, 4351–4387, https://doi.org/10.5194/essd-16-4351-2024, https://doi.org/10.5194/essd-16-4351-2024, 2024
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A new long-term inversed emission inventory for Chinese air quality (CAQIEI) is developed in this study, which contains constrained monthly emissions of NOx, SO2, CO, PM2.5, PM10, and NMVOCs in China from 2013 to 2020 with a horizontal resolution of 15 km. Emissions of different air pollutants and their changes during 2013–2020 were investigated and compared with previous emission inventories, which sheds new light on the complex variations of air pollutant emissions in China.
Can Li, Nickolay A. Krotkov, Joanna Joiner, Vitali Fioletov, Chris McLinden, Debora Griffin, Peter J. T. Leonard, Simon Carn, Colin Seftor, and Alexander Vasilkov
Earth Syst. Sci. Data, 16, 4291–4309, https://doi.org/10.5194/essd-16-4291-2024, https://doi.org/10.5194/essd-16-4291-2024, 2024
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Sulfur dioxide (SO2), a poisonous gas from human activities and volcanoes, causes air pollution, acid rain, and changes to climate and the ozone layer. Satellites have been used to monitor SO2 globally, including remote areas. Here we describe a new satellite SO2 dataset from the OMPS instrument that flies on the N20 satellite. Results show that the new dataset agrees well with the existing ones from other satellites and can help to continue the global monitoring of SO2 from space.
Jacqueline E. Russell, Richard J. Bantges, Helen E. Brindley, and Alejandro Bodas-Salcedo
Earth Syst. Sci. Data, 16, 4243–4266, https://doi.org/10.5194/essd-16-4243-2024, https://doi.org/10.5194/essd-16-4243-2024, 2024
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We present a dataset of top-of-atmosphere diurnally resolved reflected solar and emitted thermal energy for Earth system model evaluation. The multi-year, monthly hourly dataset, derived from observations made by the Geostationary Earth Radiation Budget instrument, covers the range 60° N–60° S, 60° E–60° W at 1° resolution. Comparison with two versions of the Hadley Centre Global Environmental Model highlight how the data can be used to assess updates to key model parameterizations.
Dominique Gantois, Guillaume Payen, Michaël Sicard, Valentin Duflot, Nelson Bègue, Nicolas Marquestaut, Thierry Portafaix, Sophie Godin-Beekmann, Patrick Hernandez, and Eric Golubic
Earth Syst. Sci. Data, 16, 4137–4159, https://doi.org/10.5194/essd-16-4137-2024, https://doi.org/10.5194/essd-16-4137-2024, 2024
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We describe three instruments that have been measuring interactions between aerosols (particles of various origin) and light over Réunion Island since 2012. Aerosols directly or indirectly influence the temperature in the atmosphere and can interact with clouds. Details are given on how we derived aerosol properties from our measurements and how we assessed the quality of our data before sharing them with the scientific community. A good correlation was found between the three instruments.
Hongfei Hao, Kaicun Wang, Guocan Wu, Jianbao Liu, and Jing Li
Earth Syst. Sci. Data, 16, 4051–4076, https://doi.org/10.5194/essd-16-4051-2024, https://doi.org/10.5194/essd-16-4051-2024, 2024
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In this study, daily PM2.5 concentrations are estimated from 1959 to 2022 using a machine learning method at more than 5000 terrestrial sites in the Northern Hemisphere based on hourly atmospheric visibility data, which are extracted from the Meteorological Terminal Aviation Routine Weather Report (METAR).
Pierre Tulet, Joel Van Baelen, Pierre Bosser, Jérome Brioude, Aurélie Colomb, Philippe Goloub, Andrea Pazmino, Thierry Portafaix, Michel Ramonet, Karine Sellegri, Melilotus Thyssen, Léa Gest, Nicolas Marquestaut, Dominique Mékiès, Jean-Marc Metzger, Gilles Athier, Luc Blarel, Marc Delmotte, Guillaume Desprairies, Mérédith Dournaux, Gaël Dubois, Valentin Duflot, Kevin Lamy, Lionel Gardes, Jean-François Guillemot, Valérie Gros, Joanna Kolasinski, Morgan Lopez, Olivier Magand, Erwan Noury, Manuel Nunes-Pinharanda, Guillaume Payen, Joris Pianezze, David Picard, Olivier Picard, Sandrine Prunier, François Rigaud-Louise, Michael Sicard, and Benjamin Torres
Earth Syst. Sci. Data, 16, 3821–3849, https://doi.org/10.5194/essd-16-3821-2024, https://doi.org/10.5194/essd-16-3821-2024, 2024
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The MAP-IO program aims to compensate for the lack of atmospheric and oceanographic observations in the Southern Ocean by equipping the ship Marion Dufresne with a set of 17 scientific instruments. This program collected 700 d of measurements under different latitudes, seasons, sea states, and weather conditions. These new data will support the calibration and validation of numerical models and the understanding of the atmospheric composition of this region of Earth.
Siwei Li, Yu Ding, Jia Xing, and Joshua S. Fu
Earth Syst. Sci. Data, 16, 3781–3793, https://doi.org/10.5194/essd-16-3781-2024, https://doi.org/10.5194/essd-16-3781-2024, 2024
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Surface PM2.5 data have gained widespread application in health assessments and related fields, while the inherent uncertainties in PM2.5 data persist due to the lack of ground-truth data across the space. This study provides a novel testbed, enabling comprehensive evaluation across the entire spatial domain. The optimized deep-learning model with spatiotemporal features successfully retrieved surface PM2.5 concentrations in China (2013–2021), with reduced biases induced by sample imbalance.
Shuai Wang, Mengyuan Zhang, Hui Zhao, Peng Wang, Sri Harsha Kota, Qingyan Fu, Cong Liu, and Hongliang Zhang
Earth Syst. Sci. Data, 16, 3565–3577, https://doi.org/10.5194/essd-16-3565-2024, https://doi.org/10.5194/essd-16-3565-2024, 2024
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Long-term, open-source, gap-free daily ground-level PM2.5 and PM10 datasets for India (LongPMInd) were reconstructed using a robust machine learning model to support health assessment and air quality management.
Laura Köhler, Julia Windmiller, Dariusz Baranowski, Michał Brennek, Michał Ciuryło, Lennéa Hayo, Daniel Kepski, Stefan Kinne, Beata Latos, Bertrand Lobo, Tobias Marke, Timo Nischik, Daria Paul, Piet Stammes, Artur Szkop, and Olaf Tuinder
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-275, https://doi.org/10.5194/essd-2024-275, 2024
Revised manuscript accepted for ESSD
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We present atmospheric and oceanic data from the ARC ship campaign in the Atlantic with the RV Maria S. Merian from Mindelo, Cape Verde, to Punta Arenas, Chile. Included instruments are the integrated ship sensors (DShip), a Humidity and Temperature Profiler, a Ceilometer, aerosol instruments, radiosondes, UAVs, and Conductivity, Temperature, and Depth scans. The data include three complete profiles of the Atlantic Intertropical Convergence Zone and a storm in the South Atlantic.
André Ehrlich, Susanne Crewell, Andreas Herber, Marcus Klingebiel, Christof Lüpkes, Mario Mech, Sebastian Becker, Stephan Borrmann, Heiko Bozem, Matthias Buschmann, Hans-Christian Clemen, Elena De La Torre Castro, Henning Dorff, Regis Dupuy, Oliver Eppers, Florian Ewald, Geet George, Andreas Giez, Sarah Grawe, Christophe Gourbeyre, Jörg Hartmann, Evelyn Jäkel, Philipp Joppe, Olivier Jourdan, Zsófia Jurányi, Benjamin Kirbus, Johannes Lucke, Anna E. Luebke, Maximilian Maahn, Nina Maherndl, Christian Mallaun, Johanna Mayer, Stephan Mertes, Guillaume Mioche, Manuel Moser, Hanno Müller, Veronika Pörtge, Nils Risse, Greg Roberts, Sophie Rosenburg, Johannes Röttenbacher, Michael Schäfer, Jonas Schaefer, Andreas Schäfler, Imke Schirmacher, Johannes Schneider, Sabrina Schnitt, Frank Stratmann, Christian Tatzelt, Christiane Voigt, Andreas Walbröl, Anna Weber, Bruno Wetzel, Martin Wirth, and Manfred Wendisch
Earth Syst. Sci. Data Discuss., https://doi.org/10.5194/essd-2024-281, https://doi.org/10.5194/essd-2024-281, 2024
Revised manuscript accepted for ESSD
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This paper provides an overview of the HALO–(AC)3 aircraft campaign data sets, the campaign specific instrument operation, data processing, and data quality. The data set comprises in-situ and remote sensing observations from three research aircraft, HALO, Polar 5, and Polar 6. All data are published in the PANGAEA database by instrument-separated data subsets. It is highlighted how the scientific analysis of the HALO–(AC)3 data benefits from the coordinated operation of three aircraft.
Hongfei Hao, Kaicun Wang, Chuanfeng Zhao, Guocan Wu, and Jing Li
Earth Syst. Sci. Data, 16, 3233–3260, https://doi.org/10.5194/essd-16-3233-2024, https://doi.org/10.5194/essd-16-3233-2024, 2024
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In this study, we employed a machine learning technique to derive daily aerosol optical depth from hourly visibility observations collected at more than 5000 airports worldwide from 1959 to 2021 combined with reanalysis meteorological parameters.
Arndt Kaps, Axel Lauer, Rémi Kazeroni, Martin Stengel, and Veronika Eyring
Earth Syst. Sci. Data, 16, 3001–3016, https://doi.org/10.5194/essd-16-3001-2024, https://doi.org/10.5194/essd-16-3001-2024, 2024
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CCClim displays observations of clouds in terms of cloud classes that have been in use for a long time. CCClim is a machine-learning-powered product based on multiple existing observational products from different satellites. We show that the cloud classes in CCClim are physically meaningful and can be used to study cloud characteristics in more detail. The goal of this is to make real-world clouds more easily understandable to eventually improve the simulation of clouds in climate models.
David Winker, Xia Cai, Mark Vaughan, Anne Garnier, Brian Magill, Melody Avery, and Brian Getzewich
Earth Syst. Sci. Data, 16, 2831–2855, https://doi.org/10.5194/essd-16-2831-2024, https://doi.org/10.5194/essd-16-2831-2024, 2024
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Clouds play important roles in both weather and climate. In this paper we describe version 1.0 of a unique global ice cloud data product derived from over 12 years of global spaceborne lidar measurements. This monthly gridded product provides a unique vertically resolved characterization of the occurrence and properties, optical and physical, of thin ice clouds and the tops of deep convective clouds. It should provide significant value for cloud research and model evaluation.
Karam Mansour, Stefano Decesari, Darius Ceburnis, Jurgita Ovadnevaite, Lynn M. Russell, Marco Paglione, Laurent Poulain, Shan Huang, Colin O'Dowd, and Matteo Rinaldi
Earth Syst. Sci. Data, 16, 2717–2740, https://doi.org/10.5194/essd-16-2717-2024, https://doi.org/10.5194/essd-16-2717-2024, 2024
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We propose and evaluate machine learning predictive algorithms to model freshly formed biogenic methanesulfonic acid and sulfate concentrations. The long-term constructed dataset covers the North Atlantic at an unprecedented resolution. The improved parameterization of biogenic sulfur aerosols at regional scales is essential for determining their radiative forcing, which could help further understand marine-aerosol–cloud interactions and reduce uncertainties in climate models
Piers M. Forster, Chris Smith, Tristram Walsh, William F. Lamb, Robin Lamboll, Bradley Hall, Mathias Hauser, Aurélien Ribes, Debbie Rosen, Nathan P. Gillett, Matthew D. Palmer, Joeri Rogelj, Karina von Schuckmann, Blair Trewin, Myles Allen, Robbie Andrew, Richard A. Betts, Alex Borger, Tim Boyer, Jiddu A. Broersma, Carlo Buontempo, Samantha Burgess, Chiara Cagnazzo, Lijing Cheng, Pierre Friedlingstein, Andrew Gettelman, Johannes Gütschow, Masayoshi Ishii, Stuart Jenkins, Xin Lan, Colin Morice, Jens Mühle, Christopher Kadow, John Kennedy, Rachel E. Killick, Paul B. Krummel, Jan C. Minx, Gunnar Myhre, Vaishali Naik, Glen P. Peters, Anna Pirani, Julia Pongratz, Carl-Friedrich Schleussner, Sonia I. Seneviratne, Sophie Szopa, Peter Thorne, Mahesh V. M. Kovilakam, Elisa Majamäki, Jukka-Pekka Jalkanen, Margreet van Marle, Rachel M. Hoesly, Robert Rohde, Dominik Schumacher, Guido van der Werf, Russell Vose, Kirsten Zickfeld, Xuebin Zhang, Valérie Masson-Delmotte, and Panmao Zhai
Earth Syst. Sci. Data, 16, 2625–2658, https://doi.org/10.5194/essd-16-2625-2024, https://doi.org/10.5194/essd-16-2625-2024, 2024
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This paper tracks some key indicators of global warming through time, from 1850 through to the end of 2023. It is designed to give an authoritative estimate of global warming to date and its causes. We find that in 2023, global warming reached 1.3 °C and is increasing at over 0.2 °C per decade. This is caused by all-time-high greenhouse gas emissions.
Joshua L. Laughner, Geoffrey C. Toon, Joseph Mendonca, Christof Petri, Sébastien Roche, Debra Wunch, Jean-Francois Blavier, David W. T. Griffith, Pauli Heikkinen, Ralph F. Keeling, Matthäus Kiel, Rigel Kivi, Coleen M. Roehl, Britton B. Stephens, Bianca C. Baier, Huilin Chen, Yonghoon Choi, Nicholas M. Deutscher, Joshua P. DiGangi, Jochen Gross, Benedikt Herkommer, Pascal Jeseck, Thomas Laemmel, Xin Lan, Erin McGee, Kathryn McKain, John Miller, Isamu Morino, Justus Notholt, Hirofumi Ohyama, David F. Pollard, Markus Rettinger, Haris Riris, Constantina Rousogenous, Mahesh Kumar Sha, Kei Shiomi, Kimberly Strong, Ralf Sussmann, Yao Té, Voltaire A. Velazco, Steven C. Wofsy, Minqiang Zhou, and Paul O. Wennberg
Earth Syst. Sci. Data, 16, 2197–2260, https://doi.org/10.5194/essd-16-2197-2024, https://doi.org/10.5194/essd-16-2197-2024, 2024
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This paper describes a new version, called GGG2020, of a data set containing column-integrated observations of greenhouse and related gases (including CO2, CH4, CO, and N2O) made by ground stations located around the world. Compared to the previous version (GGG2014), improvements have been made toward site-to-site consistency. This data set plays a key role in validating space-based greenhouse gas observations and in understanding the carbon cycle.
Antonin Soulie, Claire Granier, Sabine Darras, Nicolas Zilbermann, Thierno Doumbia, Marc Guevara, Jukka-Pekka Jalkanen, Sekou Keita, Cathy Liousse, Monica Crippa, Diego Guizzardi, Rachel Hoesly, and Steven J. Smith
Earth Syst. Sci. Data, 16, 2261–2279, https://doi.org/10.5194/essd-16-2261-2024, https://doi.org/10.5194/essd-16-2261-2024, 2024
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Anthropogenic emissions are the result of transportation, power generation, industrial, residential and commercial activities as well as waste treatment and agriculture practices. This work describes the new CAMS-GLOB-ANT gridded inventory of 2000–2023 anthropogenic emissions of air pollutants and greenhouse gases. The methodology to generate the emissions is explained and the datasets are analysed and compared with publicly available global and regional inventories for selected world regions.
Declan L. Finney, Alan M. Blyth, Martin Gallagher, Huihui Wu, Graeme J. Nott, Michael I. Biggerstaff, Richard G. Sonnenfeld, Martin Daily, Dan Walker, David Dufton, Keith Bower, Steven Böing, Thomas Choularton, Jonathan Crosier, James Groves, Paul R. Field, Hugh Coe, Benjamin J. Murray, Gary Lloyd, Nicholas A. Marsden, Michael Flynn, Kezhen Hu, Navaneeth M. Thamban, Paul I. Williams, Paul J. Connolly, James B. McQuaid, Joseph Robinson, Zhiqiang Cui, Ralph R. Burton, Gordon Carrie, Robert Moore, Steven J. Abel, Dave Tiddeman, and Graydon Aulich
Earth Syst. Sci. Data, 16, 2141–2163, https://doi.org/10.5194/essd-16-2141-2024, https://doi.org/10.5194/essd-16-2141-2024, 2024
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The DCMEX (Deep Convective Microphysics Experiment) project undertook an aircraft- and ground-based measurement campaign of New Mexico deep convective clouds during July–August 2022. The campaign coordinated a broad range of instrumentation measuring aerosol, cloud physics, radar signals, thermodynamics, dynamics, electric fields, and weather. The project's objectives included the utilisation of these data with satellite observations to study the anvil cloud radiative effect.
Xiaoyong Zhuge, Xiaolei Zou, Lu Yu, Xin Li, Mingjian Zeng, Yilun Chen, Bing Zhang, Bin Yao, Fei Tang, Fengjiao Chen, and Wanlin Kan
Earth Syst. Sci. Data, 16, 1747–1769, https://doi.org/10.5194/essd-16-1747-2024, https://doi.org/10.5194/essd-16-1747-2024, 2024
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The Himawari-8/9 level-2 operational cloud product has a low spatial resolution and is available only during the daytime. To supplement this official dataset, a new dataset named the NJIAS Himawari-8/9 Cloud Feature Dataset (HCFD) was constructed. The NJIAS HCFD provides a comprehensive description of cloud features over the East Asia and west North Pacific regions for the years 2016–2022 by 30 retrieved cloud variables. The NJIAS HCFD has been demonstrated to outperform the official dataset.
Honglin Pan, Jianping Huang, Jiming Li, Zhongwei Huang, Minzhong Wang, Ali Mamtimin, Wen Huo, Fan Yang, Tian Zhou, and Kanike Raghavendra Kumar
Earth Syst. Sci. Data, 16, 1185–1207, https://doi.org/10.5194/essd-16-1185-2024, https://doi.org/10.5194/essd-16-1185-2024, 2024
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We applied several correction procedures and rigorously checked for data quality constraints during the long observation period spanning almost 14 years (2007–2020). Nevertheless, some uncertainties remain, mainly due to technical constraints and limited documentation of the measurements. Even though not completely accurate, this strategy is expected to at least reduce the inaccuracy of the computed characteristic value of aerosol optical parameters.
Julie Christin Schindlbeck-Belo, Matthew Toohey, Marion Jegen, Steffen Kutterolf, and Kira Rehfeld
Earth Syst. Sci. Data, 16, 1063–1081, https://doi.org/10.5194/essd-16-1063-2024, https://doi.org/10.5194/essd-16-1063-2024, 2024
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Volcanic forcing of climate resulting from major explosive eruptions is a dominant natural driver of past climate variability. To support model studies of the potential impacts of explosive volcanism on climate variability across timescales, we present an ensemble reconstruction of volcanic stratospheric sulfur injection over the last 140 000 years that is based primarily on tephra records.
Sabrina Schnitt, Andreas Foth, Heike Kalesse-Los, Mario Mech, Claudia Acquistapace, Friedhelm Jansen, Ulrich Löhnert, Bernhard Pospichal, Johannes Röttenbacher, Susanne Crewell, and Bjorn Stevens
Earth Syst. Sci. Data, 16, 681–700, https://doi.org/10.5194/essd-16-681-2024, https://doi.org/10.5194/essd-16-681-2024, 2024
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This publication describes the microwave radiometric measurements performed during the EUREC4A campaign at Barbados Cloud Observatory (BCO) and aboard RV Meteor and RV Maria S Merian. We present retrieved integrated water vapor (IWV), liquid water path (LWP), and temperature and humidity profiles as a unified, quality-controlled, multi-site data set on a 3 s temporal resolution for a core period between 19 January 2020 and 14 February 2020.
Daniela Meloni, Filippo Calì Quaglia, Virginia Ciardini, Annalisa Di Bernardino, Tatiana Di Iorio, Antonio Iaccarino, Giovanni Muscari, Giandomenico Pace, Claudio Scarchilli, and Alcide di Sarra
Earth Syst. Sci. Data, 16, 543–566, https://doi.org/10.5194/essd-16-543-2024, https://doi.org/10.5194/essd-16-543-2024, 2024
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Solar and infrared radiation are key factors in determining Arctic climate. Only a few sites in the Arctic perform long-term measurements of the surface radiation budget (SRB). At the Thule High Arctic Atmospheric Observatory (THAAO, 76.5° N, 68.8° W) in Northern Greenland, solar and infrared irradiance measurements were started in 2009. These data are of paramount importance in studying the impact of the atmospheric (mainly clouds and aerosols) and surface (albedo) parameters on the SRB.
Karoline Block, Mahnoosh Haghighatnasab, Daniel G. Partridge, Philip Stier, and Johannes Quaas
Earth Syst. Sci. Data, 16, 443–470, https://doi.org/10.5194/essd-16-443-2024, https://doi.org/10.5194/essd-16-443-2024, 2024
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Aerosols being able to act as condensation nuclei for cloud droplets (CCNs) are a key element in cloud formation but very difficult to determine. In this study we present a new global vertically resolved CCN dataset for various humidity conditions and aerosols. It is obtained using an atmospheric model (CAMS reanalysis) that is fed by satellite observations of light extinction (AOD). We investigate and evaluate the abundance of CCNs in the atmosphere and their temporal and spatial occurrence.
Jianping Guo, Jian Zhang, Jia Shao, Tianmeng Chen, Kaixu Bai, Yuping Sun, Ning Li, Jingyan Wu, Rui Li, Jian Li, Qiyun Guo, Jason B. Cohen, Panmao Zhai, Xiaofeng Xu, and Fei Hu
Earth Syst. Sci. Data, 16, 1–14, https://doi.org/10.5194/essd-16-1-2024, https://doi.org/10.5194/essd-16-1-2024, 2024
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A global continental merged high-resolution (PBLH) dataset with good accuracy compared to radiosonde is generated via machine learning algorithms, covering the period from 2011 to 2021 with 3-hour and 0.25º resolution in space and time. The machine learning model takes parameters derived from the ERA5 reanalysis and GLDAS product as input, with PBLH biases between radiosonde and ERA5 as the learning targets. The merged PBLH is the sum of the predicted PBLH bias and the PBLH from ERA5.
Karina E. Adcock, Penelope A. Pickers, Andrew C. Manning, Grant L. Forster, Leigh S. Fleming, Thomas Barningham, Philip A. Wilson, Elena A. Kozlova, Marica Hewitt, Alex J. Etchells, and Andy J. Macdonald
Earth Syst. Sci. Data, 15, 5183–5206, https://doi.org/10.5194/essd-15-5183-2023, https://doi.org/10.5194/essd-15-5183-2023, 2023
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We present a 12-year time series of continuous atmospheric measurements of O2 and CO2 at the Weybourne Atmospheric Observatory in the United Kingdom. These measurements are combined into the term atmospheric potential oxygen (APO), a tracer that is not influenced by land biosphere processes. The datasets show a long-term increasing trend in CO2 and decreasing trends in O2 and APO between 2010 and 2021.
Nikos Benas, Irina Solodovnik, Martin Stengel, Imke Hüser, Karl-Göran Karlsson, Nina Håkansson, Erik Johansson, Salomon Eliasson, Marc Schröder, Rainer Hollmann, and Jan Fokke Meirink
Earth Syst. Sci. Data, 15, 5153–5170, https://doi.org/10.5194/essd-15-5153-2023, https://doi.org/10.5194/essd-15-5153-2023, 2023
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This paper describes CLAAS-3, the third edition of the Cloud property dAtAset using SEVIRI, which was created based on observations from geostationary Meteosat satellites. CLAAS-3 cloud properties are evaluated using a variety of reference datasets, with very good overall results. The demonstrated quality of CLAAS-3 ensures its usefulness in a wide range of applications, including studies of local- to continental-scale cloud processes and evaluation of climate models.
Sandip S. Dhomse and Martyn P. Chipperfield
Earth Syst. Sci. Data, 15, 5105–5120, https://doi.org/10.5194/essd-15-5105-2023, https://doi.org/10.5194/essd-15-5105-2023, 2023
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There are no long-term stratospheric profile data sets for two very important greenhouse gases: methane (CH4) and nitrous oxide (N2O). Along with radiative feedback, these species play an important role in controlling ozone loss in the stratosphere. Here, we use machine learning to fuse satellite measurements with a chemical model to construct long-term gap-free profile data sets for CH4 and N2O. We aim to construct similar data sets for other important trace gases (e.g. O3, Cly, NOy species).
Tobias Erhardt, Camilla Marie Jensen, Florian Adolphi, Helle Astrid Kjær, Remi Dallmayr, Birthe Twarloh, Melanie Behrens, Motohiro Hirabayashi, Kaori Fukuda, Jun Ogata, François Burgay, Federico Scoto, Ilaria Crotti, Azzurra Spagnesi, Niccoló Maffezzoli, Delia Segato, Chiara Paleari, Florian Mekhaldi, Raimund Muscheler, Sophie Darfeuil, and Hubertus Fischer
Earth Syst. Sci. Data, 15, 5079–5091, https://doi.org/10.5194/essd-15-5079-2023, https://doi.org/10.5194/essd-15-5079-2023, 2023
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The presented paper provides a 3.8 kyr long dataset of aerosol concentrations from the East Greenland Ice coring Project (EGRIP) ice core. The data consists of 1 mm depth-resolution profiles of calcium, sodium, ammonium, nitrate, and electrolytic conductivity as well as decadal averages of these profiles. Alongside the data a detailed description of the measurement setup as well as a discussion of the uncertainties are given.
Chaoyang Xue, Gisèle Krysztofiak, Vanessa Brocchi, Stéphane Chevrier, Michel Chartier, Patrick Jacquet, Claude Robert, and Valéry Catoire
Earth Syst. Sci. Data, 15, 4553–4569, https://doi.org/10.5194/essd-15-4553-2023, https://doi.org/10.5194/essd-15-4553-2023, 2023
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To understand tropospheric air pollution at regional and global scales, an infrared laser spectrometer called SPIRIT was used on aircraft to rapidly and accurately measure carbon monoxide (CO), an important indicator of air pollution, during the last decade. Measurements were taken for more than 200 flight hours over three continents. Levels of CO are mapped with 3D trajectories for each flight. Additionally, this can be used to validate model performance and satellite measurements.
Goutam Choudhury and Matthias Tesche
Earth Syst. Sci. Data, 15, 3747–3760, https://doi.org/10.5194/essd-15-3747-2023, https://doi.org/10.5194/essd-15-3747-2023, 2023
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Aerosols in the atmosphere that can form liquid cloud droplets are called cloud condensation nuclei (CCN). Accurate measurements of CCN, especially CCN of anthropogenic origin, are necessary to quantify the effect of anthropogenic aerosols on the present-day as well as future climate. In this paper, we describe a novel global 3D CCN data set calculated from satellite measurements. We also discuss the potential applications of the data in the context of aerosol–cloud interactions.
Xinyan Liu, Tao He, Shunlin Liang, Ruibo Li, Xiongxin Xiao, Rui Ma, and Yichuan Ma
Earth Syst. Sci. Data, 15, 3641–3671, https://doi.org/10.5194/essd-15-3641-2023, https://doi.org/10.5194/essd-15-3641-2023, 2023
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We proposed a data fusion strategy that combines the complementary features of multiple-satellite cloud fraction (CF) datasets and generated a continuous monthly 1° daytime cloud fraction product covering the entire Arctic during the sunlit months in 2000–2020. This study has positive significance for reducing the uncertainties for the assessment of surface radiation fluxes and improving the accuracy of research related to climate change and energy budgets, both regionally and globally.
Shoma Yamanouchi, Stephanie Conway, Kimberly Strong, Orfeo Colebatch, Erik Lutsch, Sébastien Roche, Jeffrey Taylor, Cynthia H. Whaley, and Aldona Wiacek
Earth Syst. Sci. Data, 15, 3387–3418, https://doi.org/10.5194/essd-15-3387-2023, https://doi.org/10.5194/essd-15-3387-2023, 2023
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Nineteen years of atmospheric composition measurements made at the University of Toronto Atmospheric Observatory (TAO; 43.66° N, 79.40° W; 174 m.a.s.l.) are presented. These are retrieved from Fourier transform infrared (FTIR) solar absorption spectra recorded with a spectrometer from May 2002 to December 2020. The retrievals have been optimized for fourteen species: O3, HCl, HF, HNO3, CH4, C2H6, CO, HCN, N2O, C2H2, H2CO, CH3OH, HCOOH, and NH3.
Michael J. Prather, Hao Guo, and Xin Zhu
Earth Syst. Sci. Data, 15, 3299–3349, https://doi.org/10.5194/essd-15-3299-2023, https://doi.org/10.5194/essd-15-3299-2023, 2023
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The Atmospheric Tomography Mission (ATom) measured the chemical composition in air parcels from 0–12 km altitude on 2 km horizontal by 80 m vertical scales for four seasons, resolving most scales of chemical heterogeneity. ATom is one of the first missions designed to calculate the chemical evolution of each parcel, providing semi-global diurnal budgets for ozone and methane. Observations covered the remote troposphere: Pacific and Atlantic Ocean basins, Southern Ocean, Arctic basin, Antarctica.
Marie Dumont, Simon Gascoin, Marion Réveillet, Didier Voisin, François Tuzet, Laurent Arnaud, Mylène Bonnefoy, Montse Bacardit Peñarroya, Carlo Carmagnola, Alexandre Deguine, Aurélie Diacre, Lukas Dürr, Olivier Evrard, Firmin Fontaine, Amaury Frankl, Mathieu Fructus, Laure Gandois, Isabelle Gouttevin, Abdelfateh Gherab, Pascal Hagenmuller, Sophia Hansson, Hervé Herbin, Béatrice Josse, Bruno Jourdain, Irene Lefevre, Gaël Le Roux, Quentin Libois, Lucie Liger, Samuel Morin, Denis Petitprez, Alvaro Robledano, Martin Schneebeli, Pascal Salze, Delphine Six, Emmanuel Thibert, Jürg Trachsel, Matthieu Vernay, Léo Viallon-Galinier, and Céline Voiron
Earth Syst. Sci. Data, 15, 3075–3094, https://doi.org/10.5194/essd-15-3075-2023, https://doi.org/10.5194/essd-15-3075-2023, 2023
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Saharan dust outbreaks have profound effects on ecosystems, climate, health, and the cryosphere, but the spatial deposition pattern of Saharan dust is poorly known. Following the extreme dust deposition event of February 2021 across Europe, a citizen science campaign was launched to sample dust on snow over the Pyrenees and the European Alps. This campaign triggered wide interest and over 100 samples. The samples revealed the high variability of the dust properties within a single event.
Han Huang and Yi Huang
Earth Syst. Sci. Data, 15, 3001–3021, https://doi.org/10.5194/essd-15-3001-2023, https://doi.org/10.5194/essd-15-3001-2023, 2023
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We present a newly generated set of ERA5-based radiative kernels and compare them with other published kernels for the top of the atmosphere and surface radiation budgets. For both, the discrepancies in sensitivity values are generally of small magnitude, except for temperature kernels for the surface, likely due to improper treatment in the perturbation experiments used for kernel computation. The kernel bias is not a major cause of the inter-GCM (general circulation model) feedback spread.
Robert Pincus, Paul A. Hubanks, Steven Platnick, Kerry Meyer, Robert E. Holz, Denis Botambekov, and Casey J. Wall
Earth Syst. Sci. Data, 15, 2483–2497, https://doi.org/10.5194/essd-15-2483-2023, https://doi.org/10.5194/essd-15-2483-2023, 2023
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This paper describes a new global dataset of cloud properties observed by a specific satellite program created to facilitate comparison with a matching observational proxy used in climate models. Statistics are accumulated over daily and monthly timescales on an equal-angle grid. Statistics include cloud detection, cloud-top pressure, and cloud optical properties. Joint histograms of several variable pairs are also available.
Emma L. Yates, Laura T. Iraci, Susan S. Kulawik, Ju-Mee Ryoo, Josette E. Marrero, Caroline L. Parworth, Jason M. St. Clair, Thomas F. Hanisco, Thao Paul V. Bui, Cecilia S. Chang, and Jonathan M. Dean-Day
Earth Syst. Sci. Data, 15, 2375–2389, https://doi.org/10.5194/essd-15-2375-2023, https://doi.org/10.5194/essd-15-2375-2023, 2023
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The Alpha Jet Atmospheric eXperiment (AJAX) flew scientific flights between 2011 and 2018 providing measurements of carbon dioxide, methane, ozone, formaldehyde, water vapor and meteorological parameters over California and Nevada, USA. AJAX was a multi-year, multi-objective, multi-instrument program with a variety of sampling strategies resulting in an extensive dataset of interest to a wide variety of users. AJAX measurements have been published at https://asdc.larc.nasa.gov/project/AJAX.
Leïla Simon, Valérie Gros, Jean-Eudes Petit, François Truong, Roland Sarda-Estève, Carmen Kalalian, Alexia Baudic, Caroline Marchand, and Olivier Favez
Earth Syst. Sci. Data, 15, 1947–1968, https://doi.org/10.5194/essd-15-1947-2023, https://doi.org/10.5194/essd-15-1947-2023, 2023
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Long-term measurements of volatile organic compounds (VOCs) have been set up to better characterize the atmospheric chemistry at the SIRTA national facility (Paris area, France). Results obtained from the first 2 years (2020–2021) confirm the importance of local sources for short-lived compounds and the role played by meteorology and air mass origins in the long-term analysis of VOCs. They also point to a substantial influence of anthropogenic on the monoterpene loadings.
Ka Lok Chan, Pieter Valks, Klaus-Peter Heue, Ronny Lutz, Pascal Hedelt, Diego Loyola, Gaia Pinardi, Michel Van Roozendael, François Hendrick, Thomas Wagner, Vinod Kumar, Alkis Bais, Ankie Piters, Hitoshi Irie, Hisahiro Takashima, Yugo Kanaya, Yongjoo Choi, Kihong Park, Jihyo Chong, Alexander Cede, Udo Frieß, Andreas Richter, Jianzhong Ma, Nuria Benavent, Robert Holla, Oleg Postylyakov, Claudia Rivera Cárdenas, and Mark Wenig
Earth Syst. Sci. Data, 15, 1831–1870, https://doi.org/10.5194/essd-15-1831-2023, https://doi.org/10.5194/essd-15-1831-2023, 2023
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This paper presents the theoretical basis as well as verification and validation of the Global Ozone Monitoring Experiment-2 (GOME-2) daily and monthly level-3 products.
Kristina Collins, John Gibbons, Nathaniel Frissell, Aidan Montare, David Kazdan, Darren Kalmbach, David Swartz, Robert Benedict, Veronica Romanek, Rachel Boedicker, William Liles, William Engelke, David G. McGaw, James Farmer, Gary Mikitin, Joseph Hobart, George Kavanagh, and Shibaji Chakraborty
Earth Syst. Sci. Data, 15, 1403–1418, https://doi.org/10.5194/essd-15-1403-2023, https://doi.org/10.5194/essd-15-1403-2023, 2023
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This paper summarizes radio data collected by citizen scientists, which can be used to analyze the charged part of Earth's upper atmosphere. The data are collected from several independent stations. We show ways to look at the data from one station or multiple stations over different periods of time and how it can be combined with data from other sources as well. The code provided to make these visualizations will still work if some data are missing or when more data are added in the future.
Melisa Diaz Resquin, Pablo Lichtig, Diego Alessandrello, Marcelo De Oto, Darío Gómez, Cristina Rössler, Paula Castesana, and Laura Dawidowski
Earth Syst. Sci. Data, 15, 189–209, https://doi.org/10.5194/essd-15-189-2023, https://doi.org/10.5194/essd-15-189-2023, 2023
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We explored the performance of the random forest algorithm to predict CO, NOx, PM10, SO2, and O3 air quality concentrations and comparatively assessed the monitored and modeled concentrations during the COVID-19 lockdown phases. We provide the first long-term O3 and SO2 observational dataset for an urban–residential area of Buenos Aires in more than a decade and study the responses of O3 to the reduction in the emissions of its precursors because of its relevance regarding emission control.
Vitali E. Fioletov, Chris A. McLinden, Debora Griffin, Ihab Abboud, Nickolay Krotkov, Peter J. T. Leonard, Can Li, Joanna Joiner, Nicolas Theys, and Simon Carn
Earth Syst. Sci. Data, 15, 75–93, https://doi.org/10.5194/essd-15-75-2023, https://doi.org/10.5194/essd-15-75-2023, 2023
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Sulfur dioxide (SO2) measurements from three satellite instruments were used to update and extend the previously developed global catalogue of large SO2 emission sources. This version 2 of the global catalogue covers the period of 2005–2021 and includes a total of 759 continuously emitting point sources. The catalogue data show an approximate 50 % decline in global SO2 emissions between 2005 and 2021, although emissions were relatively stable during the last 3 years.
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Short summary
A comprehensive aerosol observation project was carried out in the Tibetan Plateau (TP) and its surroundings in recent years to investigate the properties and sources of atmospheric aerosols as well as their regional differences by performing multiple intensive field observations. The release of this dataset can provide basic and systematic data for related research in the atmospheric, cryospheric, and environmental sciences in this unique region.
A comprehensive aerosol observation project was carried out in the Tibetan Plateau (TP) and its...
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