Articles | Volume 17, issue 10
https://doi.org/10.5194/essd-17-5113-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
https://doi.org/10.5194/essd-17-5113-2025
© Author(s) 2025. This work is distributed under
the Creative Commons Attribution 4.0 License.
the Creative Commons Attribution 4.0 License.
Tracking county-level cooking emissions and their drivers in China from 1990 to 2021 with ensemble machine learning
Zeqi Li
State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
Shengyue Li
State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
Zhezhe Shi
State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
Dejia Yin
State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
Qingru Wu
State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
Fenfen Zhang
State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
Department of Environment, Yangtze Delta Region Institute of Tsinghua University, Zhejiang, Jiaxing 314006, China
Xiao Yun
China Energy Longyuan Environmental Protection Co., Ltd., Beijing 100039, China
National Engineering Research Center of New Energy Power Generation, North China Electric Power University, Beijing 102206, China
Guanghan Huang
Beijing Municipal Research Institute of Eco-Environmental Protection, Beijing 100037, China
Yun Zhu
Guangdong Provincial Key Laboratory of Atmos. Environ. and Pollution Control, College of Environment and Energy, South China University of Technology, Guangzhou 510006, China
State Key Joint Laboratory of Environmental Simulation and Pollution Control, School of Environment, Tsinghua University, Beijing 100084, China
State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex, Beijing 100084, China
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This work establishes the first emission inventory of carbonaceous aerosols from cooking, fireworks, sacrificial incense, joss paper burning, and barbecue, using multi-source datasets and tested emission factors. These emissions were concentrated in specific periods and areas. Positive and negative correlations between income and emissions were revealed in urban and rural regions. The dataset will be helpful for improving modeling studies and modifying corresponding emission control policies.
Lulu Cui, Di Wu, Shuxiao Wang, Qingcheng Xu, Ruolan Hu, and Jiming Hao
Atmos. Chem. Phys., 22, 11931–11944, https://doi.org/10.5194/acp-22-11931-2022, https://doi.org/10.5194/acp-22-11931-2022, 2022
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Mengying Li, Shaocai Yu, Xue Chen, Zhen Li, Yibo Zhang, Zhe Song, Weiping Liu, Pengfei Li, Xiaoye Zhang, Meigen Zhang, Yele Sun, Zirui Liu, Caiping Sun, Jingkun Jiang, Shuxiao Wang, Benjamin N. Murphy, Kiran Alapaty, Rohit Mathur, Daniel Rosenfeld, and John H. Seinfeld
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Jiandong Wang, Jia Xing, Shuxiao Wang, Rohit Mathur, Jiaping Wang, Yuqiang Zhang, Chao Liu, Jonathan Pleim, Dian Ding, Xing Chang, Jingkun Jiang, Peng Zhao, Shovan Kumar Sahu, Yuzhi Jin, David C. Wong, and Jiming Hao
Atmos. Chem. Phys., 22, 5147–5156, https://doi.org/10.5194/acp-22-5147-2022, https://doi.org/10.5194/acp-22-5147-2022, 2022
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Lin Huang, Song Liu, Zeyuan Yang, Jia Xing, Jia Zhang, Jiang Bian, Siwei Li, Shovan Kumar Sahu, Shuxiao Wang, and Tie-Yan Liu
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Accurate estimation of emissions is a prerequisite for effectively controlling air pollution, but current methods lack either sufficient data or a representation of nonlinearity. Here, we proposed a novel deep learning method to model the dual relationship between emissions and pollutant concentrations. Emissions can be updated by back-propagating the gradient of the loss function measuring the deviation between simulations and observations, resulting in better model performance.
Zhe Jiang, Hongrong Shi, Bin Zhao, Yu Gu, Yifang Zhu, Kazuyuki Miyazaki, Xin Lu, Yuqiang Zhang, Kevin W. Bowman, Takashi Sekiya, and Kuo-Nan Liou
Atmos. Chem. Phys., 21, 8693–8708, https://doi.org/10.5194/acp-21-8693-2021, https://doi.org/10.5194/acp-21-8693-2021, 2021
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We use the COVID-19 pandemic as a unique natural experiment to obtain a more robust understanding of the effectiveness of emission reductions toward air quality improvement by combining chemical transport simulations and observations. Our findings imply a shift from current control policies in California: a strengthened control on primary PM2.5 emissions and a well-balanced control on NOx and volatile organic compounds are needed to effectively and sustainably alleviate PM2.5 and O3 pollution.
Sunling Gong, Hongli Liu, Bihui Zhang, Jianjun He, Hengde Zhang, Yaqiang Wang, Shuxiao Wang, Lei Zhang, and Jie Wang
Atmos. Chem. Phys., 21, 2999–3013, https://doi.org/10.5194/acp-21-2999-2021, https://doi.org/10.5194/acp-21-2999-2021, 2021
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Surface concentrations of PM2.5 in China have had a declining trend since 2013 across the country. This research found that the control measures of emission reduction are the dominant factors in the PM2.5 declining trends in various regions. The contribution by the meteorology to the surface PM2.5 concentrations from 2013 to 2019 was not found to show a consistent trend, fluctuating positively or negatively by about 5% on the annual average and 10–20% for the fall–winter heavy-pollution seasons.
Brigitte Rooney, Yuan Wang, Jonathan H. Jiang, Bin Zhao, Zhao-Cheng Zeng, and John H. Seinfeld
Atmos. Chem. Phys., 20, 14597–14616, https://doi.org/10.5194/acp-20-14597-2020, https://doi.org/10.5194/acp-20-14597-2020, 2020
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Wildfires have become increasingly prevalent. Intense smoke consisting of particulate matter (PM) leads to an increased risk of morbidity and mortality. The record-breaking Camp Fire ravaged Northern California for two weeks in 2018. Here, we employ a comprehensive chemical transport model along with ground-based and satellite observations to characterize the PM concentrations across Northern California and to investigate the pollution sensitivity predictions to key parameters of the model.
Jia Xing, Siwei Li, Yueqi Jiang, Shuxiao Wang, Dian Ding, Zhaoxin Dong, Yun Zhu, and Jiming Hao
Atmos. Chem. Phys., 20, 14347–14359, https://doi.org/10.5194/acp-20-14347-2020, https://doi.org/10.5194/acp-20-14347-2020, 2020
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Quantifying emission changes is a prerequisite for assessment of control effectiveness in improving air quality. However, traditional bottom-up methods usually take months to perform and limit timely assessments. A novel method was developed by using a response model that provides real-time estimation of emission changes based on air quality observations. It was successfully applied to quantify emission changes on the North China Plain due to the COVID-19 pandemic shutdown.
Pengfei Han, Ning Zeng, Tom Oda, Xiaohui Lin, Monica Crippa, Dabo Guan, Greet Janssens-Maenhout, Xiaolin Ma, Zhu Liu, Yuli Shan, Shu Tao, Haikun Wang, Rong Wang, Lin Wu, Xiao Yun, Qiang Zhang, Fang Zhao, and Bo Zheng
Atmos. Chem. Phys., 20, 11371–11385, https://doi.org/10.5194/acp-20-11371-2020, https://doi.org/10.5194/acp-20-11371-2020, 2020
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An accurate estimation of China’s fossil-fuel CO2 emissions (FFCO2) is significant for quantification of carbon budget and emissions reductions towards the Paris Agreement goals. Here we assessed 9 global and regional inventories. Our findings highlight the significance of using locally measured coal emission factors. We call on the enhancement of physical measurements for validation and provide comprehensive information for inventory, monitoring, modeling, assimilation, and reducing emissions.
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Short summary
This study uses an ensemble machine learning model to predict long-term, high-resolution cooking activity data, establishing China’s first county-level cooking emission inventory spanning 1990–2021. It covers key pollutants such as polycyclic aromatic hydrocarbons. It reveals emissions’ long-term spatiotemporal trends and driving factors, such as population migration and economic growth, offering efficient control strategies. This dataset is crucial for air pollution and health impact studies.
This study uses an ensemble machine learning model to predict long-term, high-resolution cooking...
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