Here we present a global dataset of air concentration and depositional flux measurements of atmospheric ⁷Be and ²¹⁰Pb. The dataset could be used to better understand the transport processes of air masses and depositional processes of aerosols. This dataset not only lays a solid foundation to develop better parameterizations contributing to future modeling efforts but also supplies a basic parameter for tracing soil erosion, particle dynamics, and ocean surface process using ⁷Be and/or ²¹⁰Pb.