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<article xmlns:xlink="http://www.w3.org/1999/xlink" xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:oasis="http://docs.oasis-open.org/ns/oasis-exchange/table" xml:lang="en" dtd-version="3.0" article-type="data-paper">
  <front>
    <journal-meta><journal-id journal-id-type="publisher">ESSD</journal-id><journal-title-group>
    <journal-title>Earth System Science Data</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ESSD</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Earth Syst. Sci. Data</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1866-3516</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/essd-15-3001-2023</article-id><title-group><article-title>Radiative sensitivity quantified by a new set of radiation flux kernels
based on the ECMWF Reanalysis v5 (ERA5)</article-title><alt-title>A new set of radiative kernels based on ERA5</alt-title>
      </title-group><?xmltex \runningtitle{A new set of radiative kernels based on ERA5}?><?xmltex \runningauthor{H. Huang and Y. Huang}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes">
          <name><surname>Huang</surname><given-names>Han</given-names></name>
          <email>han.huang2@mcgill.ca</email>
        <ext-link>https://orcid.org/0000-0002-9143-6453</ext-link></contrib>
        <contrib contrib-type="author" corresp="yes">
          <name><surname>Huang</surname><given-names>Yi</given-names></name>
          <email>yi.huang@mcgill.ca</email>
        <ext-link>https://orcid.org/0000-0002-5065-4198</ext-link></contrib>
        <aff id="aff1"><institution>Department of Atmospheric and Oceanic Sciences, McGill University, Montréal,
Canada</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Han Huang (han.huang2@mcgill.ca) and Yi Huang (yi.huang@mcgill.ca)</corresp></author-notes><pub-date><day>13</day><month>July</month><year>2023</year></pub-date>
      
      <volume>15</volume>
      <issue>7</issue>
      <fpage>3001</fpage><lpage>3021</lpage>
      <history>
        <date date-type="received"><day>29</day><month>December</month><year>2022</year></date>
           <date date-type="rev-request"><day>10</day><month>February</month><year>2023</year></date>
           <date date-type="rev-recd"><day>7</day><month>June</month><year>2023</year></date>
           <date date-type="accepted"><day>12</day><month>June</month><year>2023</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2023 Han Huang</copyright-statement>
        <copyright-year>2023</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023.html">This article is available from https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023.html</self-uri><self-uri xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023.pdf">The full text article is available as a PDF file from https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023.pdf</self-uri>
      <abstract><title>Abstract</title>

      <p id="d1e89">Radiative sensitivity, i.e., the response of the radiative flux to climate
perturbations, is essential to understanding climate change and variability.
The sensitivity kernels computed by radiative transfer models have been
broadly used for assessing the climate forcing and feedbacks for global
warming. As these assessments are largely focused on the top of atmosphere
(TOA) radiation budget, less attention has been paid to the surface
radiation budget or the associated surface radiative sensitivity kernels.
Based on the fifth generation European Center for Medium-Range Weather
Forecasts atmospheric reanalysis (ERA5), we produce a new set of radiative
kernels for both the TOA and surface radiative fluxes, which is made
available at <ext-link xlink:href="https://doi.org/10.17632/vmg3s67568" ext-link-type="DOI">10.17632/vmg3s67568</ext-link> (Huang
and Huang, 2023). By comparing these with other published radiative kernels, we
find that the TOA kernels are generally in agreement in terms of global mean
radiative sensitivity and analyzed overall feedback strength. The
unexplained residual in the radiation closure tests is found to be generally
within 10 % of the total feedback, no matter which kernel dataset is used.
The uncertainty in the TOA feedbacks caused by inter-kernel differences, as
measured by the standard deviation of the global mean feedback parameter
value, is much smaller than the inter-climate model spread of the feedback
values. However, we find relatively larger discrepancies in the surface
kernels. The newly generated ERA5 kernel outperforms many other datasets in
closing the surface energy budget, achieving a radiation closure comparable
to the TOA feedback decomposition, which confirms the validity of the kernel
method for the surface radiation budget analysis. In addition, by
investigating the ERA5 kernel values computed from the atmospheric states of
different years, we notice some apparent interannual differences, which
demonstrates the dependence of radiative sensitivities on the mean climate
state and partly explains the inter-dataset kernel value differences. In
this paper, we provide a detailed description of how ERA5 kernels are
generated and considerations to ensure proper use of them in feedback
quantifications.</p>
  </abstract>
    
<funding-group>
<award-group id="gs1">
<funding-source>Natural Sciences and Engineering Research Council of Canada</funding-source>
<award-id>RGPIN-2019-04511</award-id>
</award-group>
<award-group id="gs2">
<funding-source>Fonds Québécois de la Recherche sur la Nature et les Technologies</funding-source>
<award-id>2021-PR-283823</award-id>
</award-group>
</funding-group>
</article-meta>
  </front>
<body>
      

<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d1e104">Radiative kernels measure the sensitivity of radiative fluxes to the
perturbation of feedback variables, such as temperature, water vapor, albedo
and cloud  (e.g., Soden and Held, 2006; Huang et al., 2007; Shell et al.,
2008; Previdi, 2010; Zelinka et al., 2012; Block and Mauritsen, 2013; Yue et
al., 2016; Huang et al., 2017; Pendergrass et al., 2018; Thorsen et al.,
2018; Kramer et al., 2019b; Smith et al., 2020). Compared to the partial
radiative perturbation method   (e.g., Wetherald and Manabe, 1988),
which is precise but computationally expensive, the kernel method deploys a
set of precalculated radiative kernels with simple arithmetic
multiplications in feedback quantification and thus is computationally
highly efficient, which has greatly facilitated the analysis of radiative
feedbacks in global climate models (GCMs)  (e.g., Soden and Held, 2006;
Soden et al., 2008; Jonko et al., 2012; Vial et al., 2013; Zhang and Huang,
2014; Dong et al., 2020; Zelinka et al., 2020; Chao and Dessler, 2021) as
well as in observations  (e.g., Dessler, 2010; Kolly and Huang, 2018;
Zhang et al., 2019; H. Huang et al., 2021). These analyses have helped
dissect and understand the climate sensitivity differences among the GCMs,
such as those in Coupled Model Intercomparison Projects CMIP5 (Taylor
et al., 2012) and CMIP6 (Eyring et al., 2016). For example,<?pagebreak page3002?> Zelinka et
al. (2020) attributed the higher climate sensitivity in the CMIP6 models to
their more positive extratropical cloud feedback. The kernel-enabled
feedback analyses have also provided insights into the energetics of the
climate variations such as the El Niño and Southern Oscillation (ENSO, e.g.,
Dessler et al., 2010; Kolly and Huang, 2018; H. Huang et al., 2021), the
Madden–Julian Oscillation (MJO, e.g., Zhang et al., 2019), and the Arctic sea
ice interannual variability  (e.g., Huang et al., 2019), despite the
approximate nature of the kernel method and the known limits of its accuracy
(e.g., Colman and Mcavaney, 1997; Huang and Huang, 2021).</p>
      <p id="d1e107">Multiple sets of radiative kernels have been developed to date, using
different radiation codes and based on different atmospheric state datasets
ranging from GCMs to global reanalysis and satellite datasets, for both
non-cloud variables  (e.g., Soden and Held, 2006; Shell et al., 2008;
Huang et al., 2017; Thorsen et al., 2018; Bright and O'Halloran, 2019;
Donohoe et al., 2020) and cloud properties  (e.g., Zelinka et al., 2012;
Zhou et al., 2013; Yue et al., 2016; Zhang et al., 2021; Zhou et al., 2022).
As the conventional feedback analyses are mostly concerned with the
radiation energy budget change at the top of the atmosphere (TOA), most existing kernels have been
developed and tested to address that need, i.e., to measure the feedback
contributions to the TOA radiation changes. Although the radiative
sensitivity depends on the atmospheric states as well as the radiative
transfer codes used to compute the kernel values  (e.g., Collins et al.,
2006; Huang and Wang, 2019; Pincus et al., 2020), it has been noted that the
global mean TOA feedback quantification is insensitive to which kernel
dataset is used, as the diagnosed feedback values are close to each other
when measured by different kernel datasets  (e.g., Soden et al., 2008;
Jonko et al., 2012; Vial et al., 2013; Zelinka et al., 2020). However, as
there is increasing interest in regional climate change and associated
feedback (e.g., Kolly and Huang, 2018; Huang et al., 2019; Zhang et al.,
2019), it becomes important to know how the kernels (dis)agree at regional
scales. The generation of the global radiative kernels usually requires
radiative transfer computation based on a large number of instantaneous
atmospheric profiles. Due to this computational cost, many kernel datasets
are generated based on the atmospheric data from an arbitrary calendar year.
Given the known interannual climate differences, e.g., between El Niño
to La Niña years, this warrants investigations to ascertain whether the
kernels may differ in important ways for regional feedback assessments.</p>
      <p id="d1e110">On the other hand, fewer feedback studies have addressed the surface
radiation budget, although its importance has been recognized for such
problems as the precipitation change  (Previdi, 2010; Pendergrass and
Hartmann, 2014; Myhre et al., 2018) and oceanic energy transport (e.g.,
Zhang and Huang, 2014; Huang et al., 2017). The surface budget analysis
requires the use of surface kernels, which are not always available from the
published kernel datasets. Few of them have been subject to
intercomparisons or rigorous validation. As explained below in this paper,
the computation and use of them require different care to the TOA kernels.
Possibly due to the lack of such recognition, there exist considerable
discrepancies between the existing surface kernels, and some surface-budget-centered analyses reported alarmingly large non-closure in their
radiation budget analyses (e.g., Vargas Zeppetello et al., 2019),
calling into question the validity of the kernel method for surface radiation
budget analysis. Hence, we are motivated to examine the radiative
sensitivity quantified by different kernels, especially for the surface
budget.</p>
      <p id="d1e113">In this work, we produce a new set of radiative kernels for both the TOA and
surface radiation fluxes based on the fifth generation European Center for
Medium-Range Weather Forecasts atmospheric reanalysis (ERA5, Hersbach et
al., 2020), which demonstrates superior accuracy in the quantification of
various atmospheric states  (e.g., Graham et al., 2019; Wright et
al., 2020), and document the key considerations in the kernel computation
procedure. We intercompare the kernels computed from ERA5 to the other
previously generated ones and investigate the interannual variation in the
kernel values due to their atmospheric state dependency. In addition,
applying a selected set of kernels to analyzing the feedback in the CMIP6
models, we intercompare the discrepancies in quantified feedbacks across the
GCMs and across different kernels.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Construction of ERA5 radiative kernels</title>
<sec id="Ch1.S2.SS1">
  <label>2.1</label><title>Radiative transfer model and atmospheric dataset</title>
      <p id="d1e131">We use the GCM version of the rapid radiative transfer model (RRTMG)
(Mlawer et al., 1997) to calculate the radiative kernels. RRTMG conducts
radiative transfer calculations in 16 longwave (LW) spectral bands and 14
shortwave (SW) bands. The accuracy of this model has been extensively
validated against the line-by-line calculations (e.g., Collins et al., 2006).</p>
      <?pagebreak page3003?><p id="d1e134">Input data required by RRTMG, including surface pressure, skin temperature,
air temperature, water vapor, albedo, ozone concentration, cloud fraction,
cloud liquid water content and cloud ice content, are taken from the
instantaneous (as opposed to monthly mean) data of ERA5, with
a horizontal resolution of 2.5<inline-formula><mml:math id="M1" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> by 2.5<inline-formula><mml:math id="M2" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> and 37 vertical pressure
levels between 1 and 1000 hPa. To ensure the accuracy of radiative
kernels in the upper atmosphere (Smith et al., 2020), we patch five layers of
the US standard profile above 1 hPa in the LW calculations. Other required
input variables, such as the effective radii of cloud liquid droplets and ice
crystals are taken from the 3-hourly synoptic TOA and surface fluxes and
the cloud product of the Clouds and Earth's Radiant Energy System (CERES)
(Doelling et al., 2013) with a horizontal resolution of 1<inline-formula><mml:math id="M3" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> and
then interpolated to the same resolution as the ERA5 data (2.5<inline-formula><mml:math id="M4" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>). A
random cloud overlapping scheme is used in our all-sky calculation.
Sensitivity tests have been conducted to determine the necessary temporal
sampling for a proper representation of the diurnal cycle, and 6-hourly and
3-hourly instantaneous profiles are adopted for LW and SW radiative transfer
calculations, respectively, to limit the root-mean-squared error in the
computed diurnal mean flux biases to less than 1 %.</p>
</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><title>Radiative kernel computation</title>
      <p id="d1e181">Radiative kernels in essence measure the change in radiative flux to unit
perturbation of atmospheric variables, i.e., <inline-formula><mml:math id="M5" display="inline"><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:mo>∂</mml:mo><mml:mi>R</mml:mi></mml:mrow><mml:mrow><mml:mo>∂</mml:mo><mml:mi>X</mml:mi></mml:mrow></mml:mfrac></mml:mstyle></mml:math></inline-formula>, where <inline-formula><mml:math id="M6" display="inline"><mml:mi>R</mml:mi></mml:math></inline-formula> is either the upwelling irradiance flux at the TOA or
upwelling and downwelling irradiance flux at the surface, <inline-formula><mml:math id="M7" display="inline"><mml:mi>X</mml:mi></mml:math></inline-formula> represents the
aforementioned feedback variables, <inline-formula><mml:math id="M8" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the radiative kernel of
variable <inline-formula><mml:math id="M9" display="inline"><mml:mi>X</mml:mi></mml:math></inline-formula>. Note that for each radiative flux, <inline-formula><mml:math id="M10" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> varies with the
time and geographic and vertical locations of the perturbed variable and is in
general a four-dimensional (4D) data array. Note also that all radiative
fluxes and kernel values are defined as downward positive.</p>
      <p id="d1e245">Following previous studies, we compute non-cloud radiative kernels
including the LW kernels of surface temperature (<inline-formula><mml:math id="M11" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), air temperature
(<inline-formula><mml:math id="M12" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and water vapor (WV LW), and the SW kernels of surface albedo
(ALB) and water vapor (WV SW). To calculate the kernels, we use the
partial radiative perturbation experiments, conducting two radiative
transfer computations, one without perturbation (control run) and the other
with a perturbation of one atmospheric variable; the difference between
these two computations is used to calculate the radiative kernel value. In
both experiments, the upward, downward and net radiative fluxes at TOA
and the surface are saved at each time instance and location. Then <inline-formula><mml:math id="M13" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> can be obtained by differencing the saved radiative fluxes between
the perturbed and unperturbed experiments. Dividing <inline-formula><mml:math id="M14" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> with the
perturbation of variable <inline-formula><mml:math id="M15" display="inline"><mml:mi>X</mml:mi></mml:math></inline-formula> (<inline-formula><mml:math id="M16" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>X</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>), the instantaneous radiative
kernel <inline-formula><mml:math id="M17" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is calculated as
            <disp-formula id="Ch1.E1" content-type="numbered"><label>1</label><mml:math id="M18" display="block"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>X</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
          Applying such perturbation computations to all the relevant variables (see
the Appendix for a detailed discussion of the procedure), we obtain
instantaneous radiative kernels of these dimensionalities: the surface
temperature and albedo kernels are 3D arrays (time; latitude: 73;
longitude: 144), and the air temperature and water vapor kernels are
4D arrays (time; level: 37; latitude: 73; longitude: 144).</p>
      <p id="d1e361">To account for possible interannual variability in the radiative kernel
values, we compute the kernels using atmospheric data of 5 calendar
years: from the year 2011 to the year 2015. Among these years, 2011 is a strong La
Niña year, and 2015 is a strong El Niño year. Monthly or annual mean
kernels are then averaged from the instantaneous computations. For example,
the LW annual mean kernel of 2011 is obtained as <inline-formula><mml:math id="M19" display="inline"><mml:mrow><mml:mi>K</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mn mathvariant="normal">365</mml:mn><mml:mo>⋅</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:mfrac></mml:mstyle><mml:munderover><mml:mo movablelimits="false">∑</mml:mo><mml:mrow><mml:mi>i</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow><mml:mrow><mml:mn mathvariant="normal">365</mml:mn><mml:mo>⋅</mml:mo><mml:mn mathvariant="normal">4</mml:mn></mml:mrow></mml:munderover><mml:msub><mml:mi>K</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (365 is the number of days of a year
and 4 is because 6-hourly data are used for LW calculations) and the SW
kernels, <inline-formula><mml:math id="M20" display="inline"><mml:mrow><mml:mi>K</mml:mi><mml:mo>=</mml:mo><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mn mathvariant="normal">365</mml:mn><mml:mo>⋅</mml:mo><mml:mn mathvariant="normal">8</mml:mn></mml:mrow></mml:mfrac></mml:mstyle><mml:munderover><mml:mo movablelimits="false">∑</mml:mo><mml:mrow><mml:mi>i</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow><mml:mrow><mml:mn mathvariant="normal">365</mml:mn><mml:mo>⋅</mml:mo><mml:mn mathvariant="normal">8</mml:mn></mml:mrow></mml:munderover><mml:msub><mml:mi>K</mml:mi><mml:mi>i</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (8 is
because 3-hourly data are used for SW calculations), where the index <inline-formula><mml:math id="M21" display="inline"><mml:mi>i</mml:mi></mml:math></inline-formula>
represents the time slices included in the averaging. A similar averaging
procedure is applied to monthly mean kernels. The analyses in this work are
based on multi-year averaged monthly mean kernels if not otherwise stated.</p>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Characterization of ERA5 kernels</title>
      <p id="d1e466">In this section, we first present the all-sky TOA and surface radiative
sensitivity kernels quantified from the ERA5 in Figs. 1 to 4 (see the
clear-sky kernels in Figs. S1 and S2 in the Supplement). The atmospheric radiation flux
kernels, i.e., the change in radiation flux convergence in the atmosphere
due to the perturbation of feedback variables and measured by differencing
TOA and surface kernels, are shown in Figs. S3 and S4 for interested
readers. Then, we compare ERA5 kernels with the other kernel datasets, and we
examine the interannual variability in the ERA5 kernel values, due to the
dependency of radiative sensitivity on the background atmospheric state.</p>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><title>Distribution of radiative sensitivity</title>
      <p id="d1e476">Figure 1 summarizes the spatial distribution of all-sky ERA5 kernels for TOA
and the surface, and Fig. 2 illustrates the vertical cross-sections of zonal
mean air temperature, water vapor LW and water vapor SW kernels in all sky (see Figs. S1 and S2 for results in clear sky). For the surface temperature
kernels, an increase in surface temperature leads to more upwelling longwave
radiation (i.e., OLR) both at the surface and TOA; therefore the kernel is
negative. The TOA flux sensitivity in clear sky (Fig. S1a) is stronger
than that in all sky (Fig. 1a) due to the absence of cloud, and the value
increases with latitude, due to the decreasing concentration of water vapor
from the tropics to the poles. The all-sky TOA sensitivity is strongly
influenced by clouds, showing, for example, the fingerprint of the Intertropical Convergence Zone (ITCZ) in
the tropical oceans (Fig. 1a). The locations with less atmospheric
absorption due to less water vapor or cloud, e.g., the Tibetan Plateau
and Sahara regions, show relatively stronger sensitivity (Fig. 1a).
For the surface flux kernels, the increase in surface temperature enhances
the upward emission according to the Planck function, and thus the
distribution follows that of surface temperature for both clear sky and all sky (Fig. 1b).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1" specific-use="star"><?xmltex \currentcnt{1}?><?xmltex \def\figurename{Figure}?><label>Figure 1</label><caption><p id="d1e481">All-sky (left) TOA and (right) surface ERA5 kernels of <bold>(a, b)</bold> surface temperature (<inline-formula><mml:math id="M22" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(c, d)</bold> air temperature (<inline-formula><mml:math id="M23" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(e, f)</bold> water vapor longwave (WV LW), <bold>(g, h)</bold> water vapor shortwave (WV SW)
and <bold>(i, j)</bold> surface albedo (ALB). Note that for <inline-formula><mml:math id="M24" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, WV LW and
WV SW kernels, vertically integrated values are shown, which represents
the sensitivity of radiative flux to a whole-column atmospheric
perturbation. Note that the color bar ranges differ among panels.</p></caption>
          <?xmltex \igopts{width=298.753937pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f01.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2" specific-use="star"><?xmltex \currentcnt{2}?><?xmltex \def\figurename{Figure}?><label>Figure 2</label><caption><p id="d1e541">All-sky (left) TOA and (right) surface ERA5 vertically resolved
and zonally averaged kernels of <bold>(a, b)</bold> air temperature (<inline-formula><mml:math id="M25" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(c, d)</bold> water vapor longwave (WV LW) and <bold>(e, f)</bold> water vapor shortwave (WV
SW); units: W m<inline-formula><mml:math id="M26" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M27" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> 100 hPa<inline-formula><mml:math id="M28" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. Note that nonlinear color bars are
used for surface air temperature and water vapor LW kernels and that the color bar
ranges differ among panels.</p></caption>
          <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f02.png"/>

        </fig>

      <?pagebreak page3005?><p id="d1e608">For air temperature kernels, the increase in air temperature increases the
OLR at TOA and also the downwelling flux at the surface, so the TOA and surface
kernels take negative and positive signs, respectively. The TOA kernel has
maximum values in the tropics, due to the higher air temperature (Planck
function) and more abundant cloud and water vapor (higher emissivity) there,
and generally decreases in magnitude with latitude (Fig. 1c). Unlike the
TOA flux kernel, which shows comparable sensitivity to air temperature at
nearly all vertical levels, the surface flux is mainly sensitive to the
bottom layers (Fig. 2b).</p>
      <p id="d1e611">For water vapor LW kernels, an increase in water vapor reduces OLR at TOA and
increases downwelling radiation at the surface, so that the TOA and surface
kernels are both positive in sign. The vertically integrated kernel values
(Fig. 1e and f) generally follow the temperature distribution, for
example, decreasing in magnitude with latitude. In both cases, the kernel
magnitude is dampened by clouds in all sky. The vertically resolved kernels
show a maximum sensitivity of TOA flux to the upper troposphere (Fig. 2c)
and maximum sensitivity of surface flux to the bottom layers (Fig. 2d). In terms of the atmospheric radiation (the convergence of the
TOA and surface radiation fluxes in the atmosphere), the increase in water
vapor concentration absorbs more LW in the upper troposphere than what it
emits, but the opposite is true in the lower troposphere (Fig. S4c). Such
features were discussed in previous works (e.g., Huang et al., 2007).</p>
      <p id="d1e614">For water vapor SW kernels, an increase in water vapor absorbs solar
radiation and thus reduces both the upwelling (reflected) SW flux at TOA and
the downwelling SW flux at the surface. As a result, the two kernels take
positive and negative signs, respectively. Note that the magnitude of the SW
kernels is much weaker than that of the LW kernels because water vapor
absorbs the LW flux more significantly than the SW flux. One noticeable
feature of the TOA kernel in clear sky (Fig. S1g) is that the magnitude
over the land is stronger than that over the ocean because the relatively
higher albedo over the land reflects more SW radiation and thus enhances the
absorption by the water vapor in the atmosphere. For this reason, over
reflective surfaces such as the Sahara and the Tibetan Plateau as well
as the poles, the sensitivity is maximized. Unlike the TOA kernel, the
distribution of surface kernel follows the distribution of background water
vapor<?pagebreak page3006?> concentration, with noticeable dampening by clouds (Figs. 1h and 2f).</p>
      <p id="d1e617">For surface albedo kernels, an increase in surface albedo leads to more
upwelling (reflected) SW flux both at the surface and TOA; therefore, the kernel
is of negative sign. In clear sky, the sensitivity strength follows the
pattern of solar insolation, with some local maxima, e.g., in the Sahara and the Tibetan Plateau (Fig. S1i and j) due to the relatively lower
water vapor concentration. In all sky, the distribution is again influenced
by cloud patterns; for example, in the ITCZ region, the strength is much
reduced as clouds reduce the solar radiation reaching the surface and thus
the sensitivity to surface albedo change (Fig. 1i and j).</p>
</sec>
<sec id="Ch1.S3.SS2">
  <label>3.2</label><title>Comparison of ERA5 kernels with other datasets</title>
      <p id="d1e628">To examine the discrepancies between different kernel datasets, we select
six previously published ones for comparison. Table 1 summarizes their
resolutions and the datasets based on which they are computed, including the
GCMs (GFDL kernel, Soden et al., 2008; CAM3 kernel, Shell et al., 2008; CAM5 kernel, Pendergrass et al., 2018; HadGEM3 kernel, Smith et al., 2020), a global
reanalysis (ERAi kernel, Huang et al., 2017) and satellite observations of cloud
fields from CloudSat/CALIPSO combined with thermodynamic fields from
reanalyses (Kramer et al., 2019b). This list is meant to be representative
instead of exhaustive.</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T1" specific-use="star"><?xmltex \currentcnt{1}?><label>Table 1</label><caption><p id="d1e634">Summary of radiative kernels compared in this work. Datasets with <inline-formula><mml:math id="M29" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula>
only have TOA kernels.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="left"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Radiative</oasis:entry>
         <oasis:entry colname="col2">Horizontal resolution</oasis:entry>
         <oasis:entry colname="col3">Vertical</oasis:entry>
         <oasis:entry colname="col4">Reference</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">kernels</oasis:entry>
         <oasis:entry colname="col2">(lat <inline-formula><mml:math id="M30" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> long)</oasis:entry>
         <oasis:entry colname="col3">levels</oasis:entry>
         <oasis:entry colname="col4"/>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">GFDL<inline-formula><mml:math id="M31" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">2 <inline-formula><mml:math id="M32" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2.5</oasis:entry>
         <oasis:entry colname="col3">17 (pressure level)</oasis:entry>
         <oasis:entry colname="col4">Soden et al. (2008)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CAM3<inline-formula><mml:math id="M33" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">2.8 <inline-formula><mml:math id="M34" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2.8</oasis:entry>
         <oasis:entry colname="col3">17 (pressure level)</oasis:entry>
         <oasis:entry colname="col4">Shell et al. (2008)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ERAi</oasis:entry>
         <oasis:entry colname="col2">2.5 <inline-formula><mml:math id="M35" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2.5</oasis:entry>
         <oasis:entry colname="col3">24 (pressure level)</oasis:entry>
         <oasis:entry colname="col4">Huang et al. (2017)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CAM5</oasis:entry>
         <oasis:entry colname="col2">0.94 <inline-formula><mml:math id="M36" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1.25</oasis:entry>
         <oasis:entry colname="col3">30 (hybrid level)</oasis:entry>
         <oasis:entry colname="col4">Pendergrass et al. (2018)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">or 17 (pressure level)</oasis:entry>
         <oasis:entry colname="col4"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CloudSat</oasis:entry>
         <oasis:entry colname="col2">2 <inline-formula><mml:math id="M37" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2.5</oasis:entry>
         <oasis:entry colname="col3">17 (pressure level)</oasis:entry>
         <oasis:entry colname="col4">Kramer et al. (2019b)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HadGEM3</oasis:entry>
         <oasis:entry colname="col2">1.25 <inline-formula><mml:math id="M38" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1.9</oasis:entry>
         <oasis:entry colname="col3">85 (hybrid level)</oasis:entry>
         <oasis:entry colname="col4">Smith et al. (2020)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">or 19 (pressure level)</oasis:entry>
         <oasis:entry colname="col4"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ERA5</oasis:entry>
         <oasis:entry colname="col2">2.5 <inline-formula><mml:math id="M39" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2.5</oasis:entry>
         <oasis:entry colname="col3">37 (pressure level)</oasis:entry>
         <oasis:entry colname="col4">This study</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table><?xmltex \gdef\@currentlabel{1}?></table-wrap>

      <p id="d1e897">To facilitate an intercomparison, these kernel datasets are interpolated to
the same horizontal and vertical resolutions as those of the ERA5 kernel
when illustrated in Figs. 3 and 4 (see Figs. S5 and S6 for clear sky) and
are uploaded to the same data repository of ERA5 kernels. Note that the CAM5
and HadGEM3 kernels have two versions, with one defined at the raw hybrid
levels and the other interpolated to pressure levels. To retain the accuracy
of them as much as possible, the hybrid level version is used for the
interpolation and comparison in Figs. 3 and 4, while in Sect. 4, the
pressure level version is used for quantifying the feedbacks of CMIP6
models. The GFDL and CAM3 kernels are only available for TOA fluxes and are
excluded for surface kernel comparisons.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3" specific-use="star"><?xmltex \currentcnt{3}?><?xmltex \def\figurename{Figure}?><label>Figure 3</label><caption><p id="d1e903">Contour plot: fractional discrepancies as measured by the
normalized standard deviation of the kernels by Eq. (3); line plot: zonal mean distribution of multi-kernels in all sky.</p></caption>
          <?xmltex \igopts{width=469.470472pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f03.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4" specific-use="star"><?xmltex \currentcnt{4}?><?xmltex \def\figurename{Figure}?><label>Figure 4</label><caption><p id="d1e914">Contour plot: cross-section of fraction discrepancies of the
radiative kernels; line plot: global mean vertically resolved kernels from
multi-datasets in all sky.</p></caption>
          <?xmltex \igopts{width=469.470472pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f04.png"/>

        </fig>

      <p id="d1e923">Here we use the standard deviation (SD) and its normalized value
(<inline-formula><mml:math id="M40" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="normal">SD</mml:mi><mml:mo>∗</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>) to measure the spread of the inter-kernel dataset
differences:

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M41" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="Ch1.E2"><mml:mtd><mml:mtext>2</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msub><mml:mi mathvariant="normal">SD</mml:mi><mml:mi>X</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msqrt><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:mi>n</mml:mi><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:mfrac></mml:mstyle><mml:munderover><mml:mo movablelimits="false">∑</mml:mo><mml:mrow><mml:mi>i</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow><mml:mi>n</mml:mi></mml:munderover><mml:msup><mml:mfenced close=")" open="("><mml:mrow><mml:msubsup><mml:mi>K</mml:mi><mml:mi>X</mml:mi><mml:mi>i</mml:mi></mml:msubsup><mml:mo>-</mml:mo><mml:mover accent="true"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:mrow></mml:mfenced><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:mrow></mml:msqrt><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="Ch1.E3"><mml:mtd><mml:mtext>3</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msubsup><mml:mi mathvariant="normal">SD</mml:mi><mml:mi>X</mml:mi><mml:mo>∗</mml:mo></mml:msubsup><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi mathvariant="normal">SD</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow><mml:mover accent="true"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mn mathvariant="normal">100</mml:mn><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

            where <inline-formula><mml:math id="M42" display="inline"><mml:mi>n</mml:mi></mml:math></inline-formula> is the total number of kernel datasets. <inline-formula><mml:math id="M43" display="inline"><mml:mrow><mml:msubsup><mml:mi>K</mml:mi><mml:mi>X</mml:mi><mml:mi>i</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> is the radiative
kernel of variable <inline-formula><mml:math id="M44" display="inline"><mml:mi>X</mml:mi></mml:math></inline-formula> from the <inline-formula><mml:math id="M45" display="inline"><mml:mi>i</mml:mi></mml:math></inline-formula>th dataset. <inline-formula><mml:math id="M46" display="inline"><mml:mover accent="true"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> is the
multi-dataset mean of radiative kernel <inline-formula><mml:math id="M47" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. Note that <inline-formula><mml:math id="M48" display="inline"><mml:mover accent="true"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow><mml:mo mathvariant="normal">‾</mml:mo></mml:mover></mml:math></inline-formula> does
not represent the “truth” value but a reference value used to measure the
spread of multi-kernel values. The vertically integrated and the vertically
resolved but zonally averaged distributions of fractional discrepancy
(<inline-formula><mml:math id="M49" display="inline"><mml:mrow><mml:msup><mml:mi mathvariant="normal">SD</mml:mi><mml:mo>∗</mml:mo></mml:msup></mml:mrow></mml:math></inline-formula>) are shown in Figs. 3 and 4, respectively. The zonal mean
kernel values from respective multi-datasets are shown in line plots in
Figs. 3 and 4. Note that some kernels exhibit abnormal values, such as the
surface and air temperature kernel of the surface flux in the CAM5 and
CloudSat kernels (see the Appendix Fig. A2), indicating inconsistent
computation of their values, and thus are excluded in the corresponding
<inline-formula><mml:math id="M50" display="inline"><mml:mrow><mml:msubsup><mml:mi mathvariant="normal">SD</mml:mi><mml:mi>X</mml:mi><mml:mo>∗</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> statistics in Figs. 3 and 4. See more discussions in the Appendix.</p>
      <p id="d1e1144">The comparisons identify the following relatively larger differences in
kernel values. Among the TOA kernels, the surface temperature and albedo
kernels show relatively large discrepancies in the Arctic, Southern Ocean
and over some continental regions in the tropics in all sky (Fig. 3a and
q), with the maximum discrepancy exceeding 30 %. The air temperature
kernel shows larger discrepancies in the lower troposphere and tropical
tropopause region (Fig. 4a). These kernel differences are likely due to
the differences in cloud fields. The water vapor LW kernel also shows
noticeable fractional differences, for example, over the Antarctic region
(Figs. 3i and 4e). The water vapor SW kernel shows differences in the
tropical mid-troposphere and over the Antarctic in both clear sky and all sky (Figs. 4i and S6i), leading to strong variations in the vertical
integration of sensitivity (Figs. 3m and S5m), with a spread exceeding
30 %. The noticeable periodic equatorial pattern in Fig. S5m is caused
by the CAM3 kernel, likely due to a coarser temporal resolution that does
not resolve the diurnal cycle of solar insolation in the kernel
computation well.</p>
      <p id="d1e1147">For the surface kernels, the most prominent differences exist in SW
radiative kernels (Figs. 3 and 4), especially in the polar regions. The
discrepancy in the water vapor SW kernel reaches 30 % for vertically
integrated values (Fig. 3o), with noticeable differences through the
troposphere (Fig. 4k). The surface albedo kernel differences are much
larger in all sky than that in clear sky (Figs. 3 and S5), indicating that
the cause is in cloud fields, and are also noticeable in the Arctic region
due to sea ice variations (Fig. 3s). In the LW, the water vapor kernels
exhibit noticeable differences in the central Pacific, Southern Ocean and
Arctic in all sky (Fig. 3k), where again the difference in cloud field is
likely the cause. The air temperature kernels show noticeable discrepancies
in the bottom layers (Fig. 4d), which may be caused by inconsistency in
the kernel computation and vertical resolutions (see the discussions in
the Appendix).</p>
      <?pagebreak page3008?><p id="d1e1151">In summary, the differences among radiative kernel datasets are generally
smaller in clear sky than in all sky and, in most cases, are within
10 % of the radiative kernel values. However, there are some notable
regional discrepancies, for example, in the surface temperature kernel in
the tropics (Fig. 3a), in the surface albedo kernel in the Arctic (Fig. 3q) and in the water vapor SW kernel in the Antarctic region (Fig. 3m).
As different kernel datasets are calculated using different data sources,
the discrepancies detected here are likely due to the state dependency in
the kernels, which differs between the kernel datasets. To ascertain the
state-dependency-caused kernel uncertainty, we next examine the ERA5 kernels
computed from different years, i.e., from different atmospheric states, to
investigate how much difference in radiative sensitivity can result from the
change in atmospheric state.</p>
</sec>
<sec id="Ch1.S3.SS3">
  <label>3.3</label><title>Interannual variation in kernel values</title>
      <p id="d1e1162">The intercomparison above identified several prominent inter-dataset
differences in the kernel values. For example, there are noticeable
differences in the values of surface temperature, albedo and water vapor
kernels in the central Pacific and Arctic regions. One possible reason that
may account for such differences is the atmospheric state dependency of the
kernel values. Besides the inter-model differences in the different GCM
climatology, interannual variations in the atmospheric states, such as
cloudiness variations in the central Pacific region during the ENSO cycle,
may affect the radiative sensitivity as some radiative kernels are
calculated using 1 arbitrary year's data. To test this hypothesis, we use
the ENSO and sea ice loss cases to demonstrate the changes in radiative
sensitivity with a focus on the central Pacific and Arctic regions, respectively.
In the ENSO case, the variation is defined as the difference in annual mean
kernel values between 2015 and the 5-year mean (from 2011 to 2015), which have annual mean sea surface temperature anomalies in the Niño 3.4 region
(5<inline-formula><mml:math id="M51" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N–5<inline-formula><mml:math id="M52" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S, 190–240<inline-formula><mml:math id="M53" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> E) over <inline-formula><mml:math id="M54" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>2.0 K. In the sea ice loss case, the variation is
calculated as the difference in September between the years 2012 and 2013, as the
sea ice cover in 2012 was reported to be the lowest level in the satellite
observation era. In addition, we further show the comparison between ERA5
and ERAi kernels (in Fig. 5), which was also calculated by RRTMG and
averaged from 5-year calculations (2008–2012), to compare the inter-kernel
difference and interannual difference in kernel values.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5" specific-use="star"><?xmltex \currentcnt{5}?><?xmltex \def\figurename{Figure}?><label>Figure 5</label><caption><p id="d1e1201">Differences in climate states and all-sky kernel values (left)
between an arbitrary year (2015) and a 5-year mean of ERA5 and (right)
between the 5-year means of ERA5 and ERAi datasets: <bold>(a, g)</bold> skin temperature,
<bold>(b, h)</bold> total-column water vapor (TCWV), <bold>(c, i)</bold> total cloud cover (TCC), <bold>(d, j)</bold> TOA skin temperature kernel, <bold>(e, k)</bold> TOA vertically integrated water vapor
LW kernel and <bold>(f, l)</bold> TOA vertically integrated water vapor SW kernel. Note
that the color bar ranges differ among panels.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f05.png"/>

        </fig>

      <p id="d1e1229">To save space, here we only highlight the most prominent differences. Figure 5a–c show the differences in skin temperature, total-column water vapor and
total cloud cover due to ENSO, and Fig. 5d–f summarize the corresponding
differences in all-sky TOA kernels. As the skin temperature in the central
Pacific warms over 2 K (Fig. 5a) during ENSO, the increases in water vapor
concentration and cloud fraction (Fig. 5b and c) reduce the sensitivity of
TOA flux to surface temperature change by about 0.2 W m<inline-formula><mml:math id="M55" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M56" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
(about 33 %) (Fig. 5d). The moistening in the central Pacific (Fig. 5b) enhances the TOA water vapor LW sensitivity in the clear sky (Fig. S7b),
while in all sky the enhanced convection and associated total cloud cover in
this region lead to a weakened TOA water vapor LW radiative sensitivity
(Fig. 5e) despite the moist anomaly, and the decrease is contributed from almost the whole troposphere (Fig. S8c). The water vapor SW
kernel discrepancy is less pronounced (Fig. 5f).</p>
      <p id="d1e1257">Comparing the 5-year averaged all-sky ERA5 and ERAi kernels, we find that
the atmospheric state differences also exist between the atmospheric
datasets on which the kernels are computed. For example, ERA5 shows
similar, but less pronounced, warming anomalies in sea surface temperature
in the central Pacific compared to ERAi, partly due to the strong El Niño
year (2015) included in the ERA5 dataset. ERA5 data also show more water
vapor and cloud cover (Fig. 5h and i). Although the total-column water
vapor and total cloud cover are higher in ERA5 (Fig. 5h and i), their
differences are complex and vertically non-uniform (Fig. S8d and e),
which leads to a slight strengthening of surface temperature kernels
compared with ERAi (Fig. 5j). It is also<?pagebreak page3010?> noticed that the ERA5 water vapor
SW kernel shows lower sensitivity (Fig. 5l), which mainly comes from the
contributions in the mid- to low troposphere (Fig. S8f). The difference noticed
in Fig. S8f corresponds to the discrepancy noticed in Fig. 4i, which
are both in the mid- to low troposphere, and the corresponding clear sky have far fewer differences (Fig. S7), suggesting that the
difference in clouds might be the main cause of the all-sky kernel
differences, which also correspond to the discrepancies shown in the
multi-kernel comparisons in Fig. 3a, i, and m.</p>
      <p id="d1e1260">In the sea ice loss case, the reduction in sea ice in the Arctic region
(Fig. 6a) leads to a significant decrease in radiative sensitivity to
surface albedo in the areas with noticeable sea ice retreats (Fig. 6d and
f), with the maximum difference exceeding 30 % of the radiative kernel
value, because of the nonlinear dependency of the reflected solar radiation
on the surface albedo (e.g., see Y. Huang et al., 2021, Figs. 3 and  6).
The cloud cover changes also contribute to changes in surface albedo kernel
values due to the coupling effect between cloud and surface albedo (see
Y. Huang et al., 2021), which for example is seen in Siberia and the western coastline of Europe. The change in sea ice also leads to a significant
decrease in the TOA sensitivity and an increase in surface sensitivity to
water vapor in the sea ice loss region (Fig. 6c and e), with the
maximum changes exceeding 80 % for the surface. All these results confirm the
state dependency of radiative kernels (e.g.,  Riihelä et al., 2021).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6"><?xmltex \currentcnt{6}?><?xmltex \def\figurename{Figure}?><label>Figure 6</label><caption><p id="d1e1265">September differences between 2012 and 2013 in <bold>(a)</bold> sea ice
concentration, <bold>(b)</bold> total cloud cover (TCC), and the differences in <bold>(c, e)</bold>
water vapor SW kernels for TOA and surface fluxes (units: W m<inline-formula><mml:math id="M57" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M58" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and <bold>(d, f)</bold> surface albedo kernels for TOA and surface fluxes (units: W m<inline-formula><mml:math id="M59" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> 1 %<inline-formula><mml:math id="M60" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). Note that the color bar ranges differ among panels.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f06.png"/>

        </fig>

      <p id="d1e1335">In summary, these quantitatively large interannual differences, as well as
their locations, verify that some discrepancies between the radiative
kernels are caused by the difference in atmospheric states and partly
explain the inter-dataset kernel differences seen in Figs. 3 and 4.
Nevertheless, it ought to be noted that the differences are localized and
because of that do not cause significant differences in the global mean
feedback values (see Sect. 4). The results above also show that kernel
values based on 1 arbitrary year may be regionally different. If only 1 year's atmospheric profiles are used to generate radiative kernels, we
recommend selecting a year without significant anomalies in atmospheric
states, e.g., due to El Niño or severe sea ice loss, so that the computed
kernel values better represent the radiative sensitivity climatology.</p>
</sec>
</sec>
<sec id="Ch1.S4">
  <label>4</label><title>Feedback quantification</title>
      <p id="d1e1347">In this section, we apply different kernels to quantifying the radiative
feedbacks in one quadrupling CO<inline-formula><mml:math id="M61" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> experiment (abrupt4xCO<inline-formula><mml:math id="M62" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) of CMIP6
models. This experiment is selected because it has been used by a number of
studies for forcing and feedback analyses (e.g., Zelinka et al., 2020),
which we can compare our results to. The CMIP6 models used in this
assessment are listed in Table 2. Note that the standard outputs at 19
pressure levels from the models and correspondingly the kernel values,
including CAM5 and HadGEM3, provided at the pressure levels are used in this
section.</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T2" specific-use="star"><?xmltex \currentcnt{2}?><label>Table 2</label><caption><p id="d1e1371">Summary of CMIP6 models used in this study.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="left"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Models</oasis:entry>
         <oasis:entry colname="col2">Horizontal resolution</oasis:entry>
         <oasis:entry colname="col3">Vertical levels</oasis:entry>
         <oasis:entry colname="col4">Reference</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">(lat <inline-formula><mml:math id="M63" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> long)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">CESM2</oasis:entry>
         <oasis:entry colname="col2">0.9 <inline-formula><mml:math id="M64" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1.25</oasis:entry>
         <oasis:entry colname="col3">32 levels to 2.26 hPa</oasis:entry>
         <oasis:entry colname="col4">Danabasoglu et al. (2020)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CNRM-CM6-1</oasis:entry>
         <oasis:entry colname="col2">1.4 <inline-formula><mml:math id="M65" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1.4</oasis:entry>
         <oasis:entry colname="col3">91 levels to 0.01 hPa</oasis:entry>
         <oasis:entry colname="col4">Voldoire et al. (2019)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC-Earth3</oasis:entry>
         <oasis:entry colname="col2">0.7 <inline-formula><mml:math id="M66" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col3">91 levels to 90 km</oasis:entry>
         <oasis:entry colname="col4">Döscher et al. (2022)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HadGEM3-GC31-LL</oasis:entry>
         <oasis:entry colname="col2">1.25 <inline-formula><mml:math id="M67" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1.875</oasis:entry>
         <oasis:entry colname="col3">85 levels to 85 km</oasis:entry>
         <oasis:entry colname="col4">Williams et al. (2018)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">IPSL-CM6A-LR</oasis:entry>
         <oasis:entry colname="col2">1.3 <inline-formula><mml:math id="M68" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2.5</oasis:entry>
         <oasis:entry colname="col3">79 levels to 80 km</oasis:entry>
         <oasis:entry colname="col4">Boucher et al. (2020)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MPI-ESM1-2-LR</oasis:entry>
         <oasis:entry colname="col2">1.875 <inline-formula><mml:math id="M69" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1.875</oasis:entry>
         <oasis:entry colname="col3">47 levels to 0.01 hPa</oasis:entry>
         <oasis:entry colname="col4">Mauritsen et al. (2019)</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table><?xmltex \gdef\@currentlabel{2}?></table-wrap>

<sec id="Ch1.S4.SS1">
  <label>4.1</label><title>Analysis procedure</title>
      <?pagebreak page3011?><p id="d1e1568">To quantify the radiative feedbacks, data from two experiments as documented
by Eyring et al. (2016) and Pincus et al. (2016) are used: abrupt4xCO<inline-formula><mml:math id="M70" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
simulations with an instantaneous quadrupling of CO<inline-formula><mml:math id="M71" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration of the year
1850 and piClim-4xCO<inline-formula><mml:math id="M72" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> simulations with sea surface temperature (SST) and sea ice concentrations fixed
at the climatology of a pre-industrial control experiment and the CO<inline-formula><mml:math id="M73" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration quadrupled. In each experiment, a 20-year period at the end of
the simulation in each model is used. For example, in the models where the
abrupt4xCO<inline-formula><mml:math id="M74" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> simulation is longer than 150 years, the simulations from the
last 20 years rather than those from years 131 to 150 are used for the
calculation. To exclude the effect of rapid adjustments, the radiative
feedbacks in this study are measured using the difference in feedback
variables between the abrupt4xCO<inline-formula><mml:math id="M75" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and piClim-4xCO<inline-formula><mml:math id="M76" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> experiments and
vertically integrated from the surface to the model top. Note that these
treatments are different from some other studies, e.g., Zelinka et al. (2020), which used the piControl (pre-industrial control) simulation as the climatology baseline and
vertical integration from the surface to the tropopause, although the
quantitative differences in the diagnosed global mean feedback values are
small.</p>
      <p id="d1e1635">To detail the analysis procedure, firstly, all variables including radiative
fluxes and atmospheric variables from CMIP6 models are interpolated to the
horizontal and vertical resolution of the kernel itself. Note that for CAM3,
GFDL, CloudSat and CAM5 kernels, they only have 17 pressure levels, which is
two layers (1 and 5 hPa) fewer than the CMIP6 standard model output. To
address this issue, the contribution of the two missing layers is calculated
using other kernels (e.g., ERA5) and found to have a negligible effect on the
global mean feedback value. Hence, when using these three kernels, the
contributions from 10 hPa above are ignored.</p>
      <p id="d1e1638">Secondly, the non-cloud radiative feedback of variable <inline-formula><mml:math id="M77" display="inline"><mml:mi>X</mml:mi></mml:math></inline-formula> (<inline-formula><mml:math id="M78" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)
is calculated as
            <disp-formula id="Ch1.E4" content-type="numbered"><label>4</label><mml:math id="M79" display="block"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>X</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          with units in W m<inline-formula><mml:math id="M80" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, where <inline-formula><mml:math id="M81" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the monthly mean radiative kernel
of variable <inline-formula><mml:math id="M82" display="inline"><mml:mi>X</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M83" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>X</mml:mi></mml:mrow></mml:math></inline-formula> is the monthly mean anomaly of <inline-formula><mml:math id="M84" display="inline"><mml:mi>X</mml:mi></mml:math></inline-formula> measured
by the difference between abrupt4xCO<inline-formula><mml:math id="M85" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and piClim-4xCO<inline-formula><mml:math id="M86" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and
represents the anomalies of surface temperature (<inline-formula><mml:math id="M87" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), air
temperature (<inline-formula><mml:math id="M88" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), water vapor (<inline-formula><mml:math id="M89" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi mathvariant="normal">WV</mml:mi></mml:mrow></mml:math></inline-formula>) and surface albedo
(<inline-formula><mml:math id="M90" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi mathvariant="normal">ALB</mml:mi></mml:mrow></mml:math></inline-formula>). For the 2D radiative kernels (surface temperature and
surface albedo), <inline-formula><mml:math id="M91" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M92" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>X</mml:mi></mml:mrow></mml:math></inline-formula> have just single layer values and
<inline-formula><mml:math id="M93" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is simply the product of these two terms. For the 3D
radiative kernels (air temperature and water vapor), both <inline-formula><mml:math id="M94" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M95" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>X</mml:mi></mml:mrow></mml:math></inline-formula> are vectors of pressure levels and <inline-formula><mml:math id="M96" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the dot
product of <inline-formula><mml:math id="M97" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M98" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>X</mml:mi></mml:mrow></mml:math></inline-formula> and is integrated from TOA to 1000 hPa.
Note that if <inline-formula><mml:math id="M99" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is normalized with unit pressure thickness (e.g., W m<inline-formula><mml:math id="M100" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M101" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> 100 hPa<inline-formula><mml:math id="M102" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), the layer thickness must be taken into
account when calculating <inline-formula><mml:math id="M103" display="inline"><mml:mrow><mml:mi>d</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. See the Appendix for further discussion on
the application of thickness-weighted kernels.</p>
      <p id="d1e1953">Finally, cloud feedbacks are diagnosed using the adjusted cloud-radiative
forcing method (Shell et al., 2008). Here we compute the residual term in
clear sky as
            <disp-formula id="Ch1.E5" content-type="numbered"><label>5</label><mml:math id="M104" display="block"><mml:mrow><mml:msup><mml:mi mathvariant="normal">res</mml:mi><mml:mi>o</mml:mi></mml:msup><mml:mo>=</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msup><mml:mi>R</mml:mi><mml:mi>o</mml:mi></mml:msup><mml:mo>-</mml:mo><mml:mo movablelimits="false">∑</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>R</mml:mi><mml:mi>X</mml:mi><mml:mi>o</mml:mi></mml:msubsup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          which represents the unexplained part of radiation budget change, and,
assuming the all-sky decomposition has the same non-closure residual, the
cloud feedback is measured as
            <disp-formula id="Ch1.E6" content-type="numbered"><label>6</label><mml:math id="M105" display="block"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>R</mml:mi><mml:mo>-</mml:mo><mml:mo movablelimits="false">∑</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msup><mml:mi mathvariant="normal">res</mml:mi><mml:mi>o</mml:mi></mml:msup><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
          where the superscript <inline-formula><mml:math id="M106" display="inline"><mml:mi>o</mml:mi></mml:math></inline-formula> represents clear-sky quantities. <inline-formula><mml:math id="M107" display="inline"><mml:mrow><mml:mo>∑</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>R</mml:mi><mml:mi>X</mml:mi><mml:mi>o</mml:mi></mml:msubsup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M108" display="inline"><mml:mrow><mml:mo>∑</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are the sum of non-cloud feedbacks
in clear sky and all sky, respectively, diagnosed by multiplying the
radiative kernel with the atmospheric responses measured as the difference
between abrupt4xCO<inline-formula><mml:math id="M109" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and piClim-4xCO<inline-formula><mml:math id="M110" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> experiments. <inline-formula><mml:math id="M111" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msup><mml:mi>R</mml:mi><mml:mi>o</mml:mi></mml:msup></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M112" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>R</mml:mi></mml:mrow></mml:math></inline-formula> are the total radiation change in clear sky and
all sky, respectively, calculated as the difference in the GCM-simulated
radiative fluxes between two experiments. It is worth noting that <inline-formula><mml:math id="M113" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">C</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> measured according to Eq. (6) is essentially the part of total
radiation change not explained by the non-cloud feedbacks and is equivalent
to the other formulations of the adjusted cloud radiative effect method
(e.g., Soden et al., 2008; Huang, 2013). Interested readers can
refer to, for example, Huang (2013) for a detailed formulation and
explanations of the method.</p>
      <p id="d1e2126">The feedback parameters, <inline-formula><mml:math id="M114" display="inline"><mml:mrow><mml:msub><mml:mi mathvariant="italic">λ</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, in the units of W m<inline-formula><mml:math id="M115" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M116" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, are then obtained by normalizing the feedback flux changes <inline-formula><mml:math id="M117" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> by the global mean surface temperature change <inline-formula><mml:math id="M118" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">S</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in the
abrupt4xCO<inline-formula><mml:math id="M119" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> experiment:
            <disp-formula id="Ch1.E7" content-type="numbered"><label>7</label><mml:math id="M120" display="block"><mml:mrow><mml:msub><mml:mi mathvariant="italic">λ</mml:mi><mml:mi>X</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">S</mml:mi></mml:msub><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula></p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F7" specific-use="star"><?xmltex \currentcnt{7}?><?xmltex \def\figurename{Figure}?><label>Figure 7</label><caption><p id="d1e2232">The residuals (res<inline-formula><mml:math id="M121" display="inline"><mml:msup><mml:mi/><mml:mi>o</mml:mi></mml:msup></mml:math></inline-formula>) in the multi-model mean TOA feedback
decomposition when different kernels are used: LW (left column); SW (middle column); net (right column), the sum of LW and SW. The three
line plots in the bottom row are the zonal mean residuals. Numbers in the right corner in each panel are the spatial root-mean-square values.</p></caption>
          <?xmltex \igopts{width=455.244094pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f07.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F8"><?xmltex \currentcnt{8}?><?xmltex \def\figurename{Figure}?><label>Figure 8</label><caption><p id="d1e2252">Global mean TOA feedback parameters in all sky diagnosed by the
kernels listed in Table 1 across CMIP6 models. Dot marks represent
multi-model mean values computed from different kernel datasets. Stars
represent the multi-kernel mean results computed from different GCMs.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f08.png"/>

        </fig>

</sec>
<sec id="Ch1.S4.SS2">
  <label>4.2</label><title>TOA feedbacks</title>
      <?pagebreak page3013?><p id="d1e2270">The residual term (res<inline-formula><mml:math id="M122" display="inline"><mml:msup><mml:mi/><mml:mi>o</mml:mi></mml:msup></mml:math></inline-formula>) measures the unexplained radiation change in
the feedback analysis and provides a useful overall indication of the
soundness of the feedback quantification. Figure 7 illustrates the residual
term for the TOA flux decomposition when different kernels are used to
diagnose the multi-model mean feedbacks. In terms of the global mean, all
residual terms are of small magnitude, no matter which kernel dataset is
used (Fig. 8 and Table S1). However, there are some noticeable local
residuals, especially for the SW budget, e.g., in the Arctic region and
around the Antarctic continent where sea ice changes the most (middle column in
Fig. 7). While the non-zero magnitude of the residual is partly due to
nonlinearity in the radiation decomposition, e.g., possible coupling between
surface albedo and water vapor (Y. Huang et al., 2021), the spread
among the kernel results as evidenced by the line plots of Fig. 7 is
attributable to the discrepancies in the SW radiative kernels as revealed by
the comparisons in Sect. 3. In the LW, the residual is generally small
compared with the total feedback. In summary, the residual terms for the TOA
budget are small in terms of the global mean feedback strengths, confirming
the validity of the radiative kernels for feedback quantification. Here, we
use the spatial root-mean square (rms) of the residuals to quantify the
regional biases, which are shown by the numbers in the right corner of each
panel in Fig. 7. For LW, results from ERA5, ERAi and CAM5 kernels show
relatively smaller regional biases compared to those from HadGM3, CloudSat
and CAM3 kernels. For SW, all kernel datasets have similar regional
non-closures, for example, in the polar regions (Figs. 7 and 8). This is
largely caused by the nonlinearity in albedo feedback and also the coupling
effect between water vapor and surface albedo feedbacks (Y. Huang et al.,
2021; Block and Mauritsen, 2013). In summary, these results suggest that
for the TOA feedback quantification, the performance of the ERA5 kernel is
comparable to the other datasets.</p>
      <p id="d1e2282">Figure 8 compares the spreads of feedback values resulting from the
differences in kernels and those from the different projections of GCMs. In
general, feedbacks from different kernel datasets overlap each other, even
for cloud feedbacks, indicating a good consistency between the results
computed from different kernel datasets. However, the spread across the GCMs
is considerably larger, suggesting the overall feedback uncertainty is
dominated by inter-model spread rather than the kernel uncertainty. The
values of the feedbacks from each model and kernel datasets are shown in
Tables S1 and S2 for readers who are interested. These results are consistent
with other published results. For example, compared with the results of
Zelinka et al. (2020) based on the ERAi kernel, the kernel-diagnosed overall
feedback parameter in the two results is <inline-formula><mml:math id="M123" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.87  and <inline-formula><mml:math id="M124" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.85 W m<inline-formula><mml:math id="M125" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M126" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the CNRM-CM6-1 model and <inline-formula><mml:math id="M127" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.81
and <inline-formula><mml:math id="M128" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.84 W m<inline-formula><mml:math id="M129" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M130" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the HadGEM3-GC3-LL model.</p>
      <p id="d1e2362">In summary, in terms of TOA feedback values, the inter-kernel differences
lead to a small uncertainty in the analyzed non-cloud feedbacks; the
kernel-induced uncertainty in cloud feedback is relatively larger (Table S2), with the inter-kernel spread in cloud LW feedback coming almost equally from
the spread in surface and air temperature feedback and water vapor LW
feedback (as measured by the <inline-formula><mml:math id="M131" display="inline"><mml:mrow><mml:mo>∑</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>R</mml:mi><mml:mi>X</mml:mi><mml:mi>o</mml:mi></mml:msubsup><mml:mo>-</mml:mo><mml:mo>∑</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>X</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
terms in Eq. 6) and the inter-kernel spread in cloud SW feedback coming more
from the spread in surface albedo feedback than from water vapor SW feedback
(not shown). Despite this, this uncertainty is considerably less than the
inter-GCM cloud feedback spread.</p>
</sec>
<sec id="Ch1.S4.SS3">
  <label>4.3</label><title>Surface feedbacks</title>
      <p id="d1e2401">Next, we examine how the inter-kernel differences lead to uncertainty in the
analyzed surface feedbacks.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9" specific-use="star"><?xmltex \currentcnt{9}?><?xmltex \def\figurename{Figure}?><label>Figure 9</label><caption><p id="d1e2406">Similar to Fig. 7 but for the surface feedback analysis.</p></caption>
          <?xmltex \igopts{width=469.470472pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f09.png"/>

        </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F10"><?xmltex \currentcnt{10}?><?xmltex \def\figurename{Figure}?><label>Figure 10</label><caption><p id="d1e2417">Similar to Fig. 8 but for the surface feedback parameter.</p></caption>
          <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f10.png"/>

        </fig>

      <p id="d1e2427">Figure 9 shows the residual distribution. We find that when the ERA5 and
ERAi kernels are used for the feedback analysis, the non-closure residual in
the surface budget is comparable in magnitude to the TOA analysis. This
suggests that the surface kernels afford a valid tool for the surface
feedback analysis. However, some prominent biases are noticed for other
kernel datasets. For example, the HadGEM3 kernels particularly show an
underestimation in air temperature feedback, likely due to a biased
sensitivity of the bottom atmospheric layer (see the Appendix for more
discussions). The sum of global mean surface and air temperature feedback
parameters measured by the HadGEM3 kernel is around <inline-formula><mml:math id="M132" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>3.70 W m<inline-formula><mml:math id="M133" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M134" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
(Table S4, compared to around <inline-formula><mml:math id="M135" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.0 W m<inline-formula><mml:math id="M136" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M137" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> measured by the other
kernels), and the non-closure residual is as large as 3.0 W m<inline-formula><mml:math id="M138" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M139" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Table S3, compared to <inline-formula><mml:math id="M140" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.1 W m<inline-formula><mml:math id="M141" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M142" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the others). For
this reason, the result from the HadGEM3 kernel is excluded for the multi-kernel
statistics in Fig. 10, Table S3 and S4 but listed in a separate row for
comparison. From either the<?pagebreak page3014?> spatial distribution of residual terms or the
spatial rms residuals, the ERA5 kernel and ERAi kernel show a superior
performance than the other datasets. The use of ERA5 kernels may be advantageous
for diagnosing the surface radiation budget, considering that ERA5 data are a
newer-version reanalysis dataset from ECMWF compared with ERAi, and their quality has been widely validated.</p>
      <p id="d1e2548">Figure 10 compares the inter-model and inter-kernel spreads for the surface
feedbacks. Unlike the results for TOA, the inter-kernel spread can be as
large as the inter-model spread, for example, in LW surface temperature
feedback, air temperature feedback and water vapor feedback. The sum of air
temperature and surface temperature feedbacks shows better consistency
compared with the respective components (except for the HadGEM3 kernel), and
the respective air temperature and surface temperature feedbacks quantified
by the ERA5 kernel are stronger than the results from the other kernels.
These discrepancies are due to the reason discussed in the Appendix – a
possibly wrong quantification of surface temperature effect. In SW, the
multi-kernel results are close to each other, showing smaller inter-kernel
spreads than the inter-model spreads.</p>
      <?pagebreak page3015?><p id="d1e2551">In summary, we find the surface feedback decomposition can achieve a similar
level of radiation closure to the TOA analysis when using ERA5 kernels,
confirming the validity of kernels for diagnosing the surface radiative
feedback. However, the results qualitatively vary depending on which kernel
dataset is used, indicating errors in the computation of some kernels.</p>
</sec>
</sec>
<sec id="Ch1.S5">
  <label>5</label><title>Data availability</title>
      <p id="d1e2564">The datasets containing the multi-year averaged monthly mean TOA and surface
kernels for surface temperature, air temperature, surface albedo and water
vapor (LW and SW) are available at
<ext-link xlink:href="https://doi.org/10.17632/vmg3s67568" ext-link-type="DOI">10.17632/vmg3s67568</ext-link> (Huang and Huang, 2023). Other
kernel datasets used in this study, interpolated to the same horizontal and
vertical grids as the ERA5 kernels, are also provided at this link.</p>
</sec>
<sec id="Ch1.S6" sec-type="conclusions">
  <label>6</label><title>Conclusions and discussions</title>
      <p id="d1e2578">In this paper, we present a newly generated set of ERA5-based radiative
kernels of surface and air temperatures, water vapor, and surface albedo, for
both TOA and surface radiation fluxes. We also compare them with other
published kernels, including the kernel-diagnosed radiative feedbacks for
both the TOA and surface radiation budgets.</p>
      <p id="d1e2581">For the TOA kernels, the results here demonstrate general consistency among
the different kernel datasets, and the discrepancies are generally within
10 % in terms of vertically integrated or globally averaged radiative
sensitivity, although some relatively larger regional differences are
noticed, including those in the surface temperature kernel in the tropics
(Fig. 3a), those in the surface albedo kernel in the Arctic (Fig. 3q)
and those in the water vapor shortwave kernel over Antarctica (Fig. 3m),
which is partly due to the dependence of radiative sensitivity on background
climate states.</p>
      <p id="d1e2584">For the surface kernels, more prominent inter-kernel differences are found.
For example, the differences in the water vapor shortwave kernel in the
Antarctic (Fig. 3o) and in the surface albedo kernel in the Arctic (Fig. 3s) can reach 30 % of the kernel value itself. Some kernels have
considerably biased air temperature sensitivity values in the bottom
atmospheric layers, which is likely due to improper treatment in the
perturbation experiments used for kernel computation (see the Appendix). The
differences in both TOA and surface kernels discovered here emphasize the
importance of validating the radiative sensitivity as noted by Huang and
Wang (2019) and Pincus et al. (2020).</p>
      <p id="d1e2587">The investigation of interannual variability in ERA5 kernels validates the
dependence of radiative sensitivity on atmospheric state and the further
comparison between ERAi and ERA5 kernels (Fig. 5) reveals the effects of
clouds on the kernel values, which might explain the discrepancies between
multi-kernel datasets (Fig. 3).</p>
      <p id="d1e2591">Applying the different kernels to quantifying the TOA and surface radiative
feedbacks, we find that for TOA feedback quantification, the ERA5 kernels
are as accurate as other kernel datasets, while for surface feedback, ERA5
and ERAi kernels show superior accuracy compared with other datasets.
Considering the strengths of the ERA5 dataset in representing the
atmospheric states, we recommend the use of ERA5 kernels.</p>
      <p id="d1e2594">In addition, we compare the feedback differences caused by using different
kernels and also the inter-GCM spread of the feedback values (when measured
by the same kernel). We find the kernel difference is not a major cause of
the inter-GCM TOA feedback spread (Figs. 7 and 8). This finding is
consistent with the previous assessments (e.g., Soden et al., 2008; Jonko et
al., 2012; Vial et al., 2013).</p>
      <p id="d1e2597">Radiation closure tests show that the unexplained residuals are generally
within 10 % of the total feedback for both TOA and surface analyses in
terms of the global mean feedback, confirming the validity of the kernels
for feedback quantification for both budgets. This suggests that the large
non-closure residuals reported in some previous studies (e.g., Vargas
Zeppetello et al., 2019) are likely due to kernel inaccuracy rather than
the limitation of the kernel method. However, there are more significant
local non-closures, for example, in the shortwave in the Arctic region and
around the Antarctic continent, which is contributed, but cannot be fully
explained, by the kernel uncertainty. This points to the accuracy limit of
the kernel (linear) method and calls for more advanced methods, such as the
neural network method (Zhu et al., 2019), for local feedback analysis.</p>
</sec>

      
      </body>
    <back><app-group>

<?pagebreak page3016?><app id="App1.Ch1.S1">
  <?xmltex \currentcnt{A}?><label>Appendix A</label><title/>
      <p id="d1e2610">The ERA5 kernels are computed following Eq. (1) and the approach outlined in Sect. 2.2.</p>
<sec id="App1.Ch1.S1.SS1">
  <label>A1</label><title>Surface variable kernels</title>
      <p id="d1e2620">To execute the partial radiative perturbation computations, the
perturbations are prescribed as the following: for the 2D feedback
variables, the surface temperature is increased by 1 K and the albedo is
increased by 0.01 at each location. Hence, the units of the two kernels,
<inline-formula><mml:math id="M143" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>  and <inline-formula><mml:math id="M144" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi mathvariant="normal">ALB</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are W m<inline-formula><mml:math id="M145" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M146" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and W m<inline-formula><mml:math id="M147" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> %<inline-formula><mml:math id="M148" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>,
respectively. When applying them to feedback quantification, their feedbacks
are quantified as

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M149" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="App1.Ch1.S1.E8"><mml:mtd><mml:mtext>A1</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">S</mml:mi></mml:msub><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="App1.Ch1.S1.E9"><mml:mtd><mml:mtext>A2</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">ALB</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>K</mml:mi><mml:mi mathvariant="normal">ALB</mml:mi></mml:msub><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi mathvariant="normal">ALB</mml:mi><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

            where <inline-formula><mml:math id="M150" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">S</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> should be measured in the units of K and <inline-formula><mml:math id="M151" display="inline"><mml:mi mathvariant="normal">Δ</mml:mi></mml:math></inline-formula>ALB in absolute values divided by 1 %.</p>
</sec>
<sec id="App1.Ch1.S1.SS2">
  <label>A2</label><title>Water vapor kernel</title>
      <p id="d1e2801">For the 3D feedback variables, the perturbations are applied to each of the
37 pressure layers (from 1 to 1000 hPa) and one layer at a time. For the
water vapor kernel, a 10 % incremental perturbation of the water vapor
concentration is used. To adapt to the convention used in the majority of
the existing kernels, we convert the units of the kernels to represent the
radiative flux change corresponding to an increase in water vapor
concentration that conserves the relative humidity of the layer under a 1 K
increase in air temperature, i.e., converting the units from W (m<inline-formula><mml:math id="M152" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>
<inline-formula><mml:math id="M153" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="italic">%</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula> 100 hPa)<inline-formula><mml:math id="M154" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to W (m<inline-formula><mml:math id="M155" display="inline"><mml:mrow><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula> 100 hPa)<inline-formula><mml:math id="M156" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>:

                <disp-formula specific-use="gather" content-type="numbered"><mml:math id="M157" display="block"><mml:mtable displaystyle="true"><mml:mlabeledtr id="App1.Ch1.S1.E10"><mml:mtd><mml:mtext>A3</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle class="stylechange" displaystyle="true"/><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="italic">%</mml:mi></mml:mrow></mml:msubsup><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="italic">%</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mlabeledtr><mml:mlabeledtr id="App1.Ch1.S1.E11"><mml:mtd><mml:mtext>A4</mml:mtext></mml:mtd><mml:mtd><mml:mrow><mml:mstyle displaystyle="true" class="stylechange"/><mml:mtable class="split" rowspacing="0.2ex" displaystyle="true" columnalign="right left"><mml:mtr><mml:mtd><mml:mrow><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="italic">%</mml:mi></mml:mrow></mml:msubsup><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="italic">%</mml:mi></mml:mrow></mml:msubsup></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:mo>=</mml:mo><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="italic">%</mml:mi></mml:mrow></mml:msubsup><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mi mathvariant="italic">%</mml:mi></mml:mrow></mml:msubsup></mml:mrow><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfenced></mml:mrow><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:mrow></mml:mfenced><mml:mo>-</mml:mo><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfenced></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:mrow></mml:mtd></mml:mlabeledtr></mml:mtable></mml:math></disp-formula>

            where <inline-formula><mml:math id="M158" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> is the unperturbed water vapor concentration in units of kg kg<inline-formula><mml:math id="M159" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. <inline-formula><mml:math id="M160" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow><mml:mo>+</mml:mo><mml:mn mathvariant="normal">10</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="italic">%</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula> is a 10 % increment in water vapor
concentration. <inline-formula><mml:math id="M161" display="inline"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mfenced open="(" close=")"><mml:mi>T</mml:mi></mml:mfenced></mml:mrow></mml:math></inline-formula> is the saturated water vapor pressure
under temperature <inline-formula><mml:math id="M162" display="inline"><mml:mi>T</mml:mi></mml:math></inline-formula> and can be measured by empirical formulas; hence,
<inline-formula><mml:math id="M163" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula> can be measured as <inline-formula><mml:math id="M164" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>[</mml:mo><mml:mstyle displaystyle="false"><mml:mfrac style="text"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:mrow></mml:mfenced></mml:mrow><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfenced></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula>. Accordingly, when the water vapor
kernel is used for water vapor feedback quantification, the feedback is
measured as
            <disp-formula id="App1.Ch1.S1.E12" content-type="numbered"><label>A5</label><mml:math id="M165" display="block"><mml:mtable class="split" rowspacing="0.2ex" displaystyle="true" columnalign="right left"><mml:mtr><mml:mtd><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>q</mml:mi></mml:msub></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mo>=</mml:mo><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msup><mml:mi>q</mml:mi><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msup><mml:mo>=</mml:mo><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi></mml:mrow><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:mo>=</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi></mml:mrow><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfenced></mml:mrow><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mfenced open="(" close=")"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mrow class="unit"><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:mrow></mml:mfenced><mml:mo>-</mml:mo><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mfenced close=")" open="("><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfenced></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:math></disp-formula>
          where <inline-formula><mml:math id="M166" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi><mml:mo>=</mml:mo><mml:mi>q</mml:mi><mml:mo>-</mml:mo><mml:msub><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> measures the change in water vapor concentration
and is normalized by <inline-formula><mml:math id="M167" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msubsup><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula> to give the factor that is
multipliable with the <inline-formula><mml:math id="M168" display="inline"><mml:mrow><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup></mml:mrow></mml:math></inline-formula> kernel value. If using the
Clapeyron–Clausius relation, the above expression can be further
approximated as
            <disp-formula id="App1.Ch1.S1.E13" content-type="numbered"><label>A6</label><mml:math id="M169" display="block"><mml:mtable class="split" rowspacing="0.2ex" displaystyle="true" columnalign="right left"><mml:mtr><mml:mtd><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mi>q</mml:mi></mml:msub></mml:mrow></mml:mtd><mml:mtd><mml:mrow><mml:mo>=</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi></mml:mrow><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mo>(</mml:mo><mml:mi mathvariant="normal">d</mml:mi><mml:msub><mml:mi>e</mml:mi><mml:mi mathvariant="normal">s</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:mi mathvariant="normal">d</mml:mi><mml:mi>T</mml:mi><mml:mo>)</mml:mo><mml:mo>⋅</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mrow class="unit"><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:mrow></mml:mfrac></mml:mstyle></mml:mrow></mml:mtd></mml:mtr><mml:mtr><mml:mtd/><mml:mtd><mml:mrow><mml:mo>=</mml:mo><mml:msubsup><mml:mi>K</mml:mi><mml:mi>q</mml:mi><mml:mrow class="unit"><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mspace linebreak="nobreak" width="0.125em"/><mml:mi mathvariant="normal">K</mml:mi></mml:mrow></mml:msubsup><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>q</mml:mi></mml:mrow><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mi>L</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>⋅</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:msubsup><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn><mml:mn mathvariant="normal">2</mml:mn></mml:msubsup></mml:mrow><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mi>K</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:mtd></mml:mtr></mml:mtable></mml:math></disp-formula>
          where <inline-formula><mml:math id="M170" display="inline"><mml:mrow><mml:msub><mml:mi>R</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M171" display="inline"><mml:mrow><mml:msub><mml:mi>L</mml:mi><mml:mi mathvariant="normal">v</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are the gas constant and specific latent heat of
water vapor, respectively. Note that when the kernels are used, <inline-formula><mml:math id="M172" display="inline"><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M173" display="inline"><mml:mrow><mml:msub><mml:mi>q</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula> typically take their values from the base climate appropriate to the
application, e.g., the unperturbed climate of a GCM experiment, not
necessarily the dataset used for kernel computation.</p>
</sec>
<sec id="App1.Ch1.S1.SS3">
  <label>A3</label><title>Air temperature kernel</title>
      <p id="d1e3731">For the air temperature kernel, to be consistent with the “inhomogeneous
path treatment” that accounts for the vertically non-uniform temperature
distribution within each discrete atmospheric layer (Mlawer et al., 1997),
perturbations are added not only to the layer-mean temperature but also to the
temperature at the exiting boundary of radiative fluxes of interest (i.e.,
the upper boundary of each layer for the TOA flux and the lower boundary for
the surface flux) to appropriately represent the physical temperature
perturbation in each layer.</p>
      <p id="d1e3734">A meaningful test to validate the validity of the air temperature kernel is
a vertical sum test, i.e., a linear additivity test to verify the vertical
integration of the kernel values reproducing the flux change, either at TOA or the surface, in response to a whole-column air temperature increase of 1 K.
Figure A1 shows that the ERA5 kernel passes this test well. However, as
shown by Fig. 9, some kernels (e.g., HadGEM3 kernel) show a much weaker
radiative response at the surface, possibly due to improper treatment of the air
temperature perturbation in the kernel computation, which may lead to an
underestimated air temperature feedback and large biases in the surface
feedback analysis.</p>

      <?xmltex \floatpos{t}?><fig id="App1.Ch1.S1.F11" specific-use="star"><?xmltex \currentcnt{A1}?><?xmltex \def\figurename{Figure}?><label>Figure A1</label><caption><p id="d1e3739">Monthly mean TOA and surface radiation flux change in response to
a <inline-formula><mml:math id="M174" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1 K air temperature perturbation throughout the vertical column: <bold>(a, b)</bold> computed by a radiation model, RRTMG; <bold>(c, d)</bold> difference in the vertical sum of
air temperature kernels compared to truth in <bold>(a)</bold>, <bold>(b)</bold>; <bold>(e, f)</bold> comparison of
the zonal mean.</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f11.png"/>

        </fig>

      <p id="d1e3772">Another challenge in the computation of air temperature kernels for surface
flux is that the surface in radiative transfer models is also the lower
boundary of the lowermost atmospheric layer. If the effects of the surface
temperature perturbation on the emission of the surface and that of the
lowermost atmospheric layer are not distinguished, this may lead to improper
interpretation and use of the surface temperature kernel. In our ERA5
kernel, the two effects are considered separately: according to radiative
transfer theory, an increase in surface skin temperature only affects the
surface upward emission; an increase in air temperature only affects the
downward radiation. In some other kernels such as CAM5, these effects are
not distinguished, so that the kernel value represents the net effect, i.e.,
a change in the sum of both<?pagebreak page3017?> downward and upward fluxes. As a result, in Fig. 10, we
see stronger air temperature and surface temperature feedbacks quantified
from ERA5 kernels than from other kernels, and in Table S4, we can only
report the sum of surface and air temperature feedbacks.</p>

      <?xmltex \floatpos{t}?><fig id="App1.Ch1.S1.F12" specific-use="star"><?xmltex \currentcnt{A2}?><?xmltex \def\figurename{Figure}?><label>Figure A2</label><caption><p id="d1e3777">Comparison of annual mean surface kernels for ERA5, CAM5,
CloudSat and HadGEM3 for <bold>(a, b)</bold> the vertically integrated air temperature
kernel values and <bold>(c, d)</bold> sum of surface and air temperature kernels.
</p></caption>
          <?xmltex \igopts{width=341.433071pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f12.png"/>

        </fig>

      <p id="d1e3792">Figure A2 shows the comparison of vertically integrated air temperature
kernels and the sum of surface and air temperature kernels between ERA5,
CAM5, HadGEM3 and CloudSat. Although the strength of the vertically integrated
air temperature kernel for CAM5 is much weaker than that for ERA5 (Fig. A2a and b), the sum of surface and air temperature kernels between these two
datasets is in good agreement (Fig. A2c and d), which warns us that the
seemingly right temperature feedback quantified by some kernels might come
from the misattribution of surface temperature contributions. Another
noticeable feature in Fig. A2 is that the HadGEM3 kernel shows an
underestimation in the vertical integration of the air temperature kernel and an
overestimation in the sum of surface and air temperature kernels, likely due
to mistreatment of the bottom layer, and this accounts for the biased
surface feedback analysis as shown in Fig. 9. Similar issues were noticed
in Kramer et al. (2019a).</p>
</sec>
<sec id="App1.Ch1.S1.SS4">
  <label>A4</label><title>Time averaging</title>
      <p id="d1e3804">As described in Sect. 2.2, all the kernels provided for feedback analysis
are averaged from instantaneous kernel values over each calendar month and,
in the ERA5 kernel, over multiple years. This is to ensure proper sampling
of radiative sensitivity values under different atmospheric states, so that
the kernels are representative of mean radiative sensitivity and thus can be
readily multiplied with monthly mean climate responses (<inline-formula><mml:math id="M175" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>X</mml:mi></mml:mrow></mml:math></inline-formula>) to
evaluate climate feedbacks.</p>
      <p id="d1e3817">If the kernels are computed for fixed pressure levels, and if the pressure
of any of these levels of an instantaneous atmospheric profile is higher
than the surface pressure (i.e., the level is below the surface) at a time
instance, this potentially creates inconsistency in the averaging procedure.
To address this concern, we set the kernel value to 0 (as opposed to
a missing value) before averaging. This is to ensure that when multiplied with
the monthly mean climate response (<inline-formula><mml:math id="M176" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:mi>X</mml:mi></mml:mrow></mml:math></inline-formula>), the contribution of a
pressure layer (e.g., that<?pagebreak page3018?> centered at 1000 hPa) is effectively counted only
for the fraction of time the layer exists (when surface pressure is higher
than 1000 hPa). Otherwise, the feedback quantification needs to be further
weighted with the fraction of time (<inline-formula><mml:math id="M177" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>) when the pressure layer exists. For
example, if the surface pressure is larger than 1000 hPa only for half of
the time in a month (<inline-formula><mml:math id="M178" display="inline"><mml:mrow><mml:mi>f</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:math></inline-formula>), the radiation flux anomaly contributed by the
layer centered at 1000 hPa is
            <disp-formula id="App1.Ch1.S1.E14" content-type="numbered"><label>A7</label><mml:math id="M179" display="block"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>R</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>1000 hPa</mml:mtext></mml:msub></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:msubsup><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>1000 hPa</mml:mtext></mml:msub></mml:mrow><mml:mo>∗</mml:mo></mml:msubsup><mml:mo>⋅</mml:mo><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>T</mml:mi><mml:mtext>1000 hPa</mml:mtext></mml:msub><mml:mo>⋅</mml:mo><mml:mi>f</mml:mi><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
          Here, <inline-formula><mml:math id="M180" display="inline"><mml:mrow><mml:msubsup><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>1000 hPa</mml:mtext></mml:msub></mml:mrow><mml:mo>∗</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> represents the kernel value averaged from
the time instances when the layer exists. Our averaging scheme is
essentially to provide a kernel <inline-formula><mml:math id="M181" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>1000 hPa</mml:mtext></mml:msub></mml:mrow></mml:msub><mml:mo>=</mml:mo><mml:msubsup><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mtext>1000 hPa</mml:mtext></mml:msub></mml:mrow><mml:mo>∗</mml:mo></mml:msubsup><mml:mo>⋅</mml:mo><mml:mi>f</mml:mi></mml:mrow></mml:math></inline-formula>, so that it can be simply multiplied with <inline-formula><mml:math id="M182" display="inline"><mml:mrow><mml:mi mathvariant="normal">Δ</mml:mi><mml:msub><mml:mi>T</mml:mi><mml:mtext>1000 hPa</mml:mtext></mml:msub></mml:mrow></mml:math></inline-formula>
to obtain the same result.</p>

      <?xmltex \floatpos{t}?><fig id="App1.Ch1.S1.F13"><?xmltex \currentcnt{A3}?><?xmltex \def\figurename{Figure}?><label>Figure A3</label><caption><p id="d1e3959">Zonal mean monthly mean air temperature kernels for surface flux
from ERA5 in clear sky. Black line is the result from the whole-column
perturbation computation by RRTMG, providing a “truth” for comparison. Red
dashed line is the kernel weighted with fraction of time (<inline-formula><mml:math id="M183" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>) and
blue dotted line represents results without weights (<inline-formula><mml:math id="M184" display="inline"><mml:mrow><mml:msubsup><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow><mml:mo>∗</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula>).</p></caption>
          <?xmltex \igopts{width=227.622047pt}?><graphic xlink:href="https://essd.copernicus.org/articles/15/3001/2023/essd-15-3001-2023-f13.png"/>

        </fig>

      <p id="d1e4001">Figure A3 illustrates the differences between <inline-formula><mml:math id="M185" display="inline"><mml:mrow><mml:msubsup><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow><mml:mo>∗</mml:mo></mml:msubsup></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M186" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mrow><mml:msub><mml:mi>T</mml:mi><mml:mi mathvariant="normal">a</mml:mi></mml:msub></mml:mrow></mml:msub></mml:mrow></mml:math></inline-formula>, in terms of their vertically integrated value. Such a difference is pronounced over the Southern Oceans (around 60<inline-formula><mml:math id="M187" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S), where the surface
pressure value varies considerably. This likely explains why Fig. 3h shows
noticeable differences in the air temperature kernel in this region.</p>
</sec>
<sec id="App1.Ch1.S1.SS5">
  <label>A5</label><title>Layer-specified and layer-thickness-normalized radiative kernels</title>
      <p id="d1e4053">We generate two versions of vertically resolved air temperature kernels – the
water vapor LW and SW kernels – one with values corresponding to specified
vertical layers, i.e., in the units of W m<inline-formula><mml:math id="M188" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M189" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, and another with
unit-layer thickness (e.g., as shown in Figs. 2 and 4), i.e., in W m<inline-formula><mml:math id="M190" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> K<inline-formula><mml:math id="M191" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> 100 hPa<inline-formula><mml:math id="M192" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The latter properly portrays the vertical
distribution of radiative sensitivity to perturbations in the unit thickness
layers, while the former may be more convenient to use in feedback
quantifications. For TOA budget analyses, these two versions of kernels lead
to little difference in practice due to limited contributions from the
bottom atmospheric layer. However, for surface budget analyses, we recommend
using the layer-specified kernels, as the surface kernels typically show
the strongest sensitivity to the perturbations in the bottom layers, which can
be best accounted for in the non-normalized kernels. Otherwise, the
difference in surface pressure between ERA5 and GCMs needs to be carefully
treated to avoid errors caused, for example,  by missing the radiative
contribution from the bottom layer of the atmosphere. To illustrate this
issue in an example, consider a location (latitude–longitude grid point)
where the surface pressure is 960 hPa in a GCM and the lowermost level of
the<?pagebreak page3019?> non-zero value of the ERA5 air temperature kernel is located at 975 hPa. Had the
air temperature change been set to 0 or an NaN (not a number) value due to the GCM ground
level being above 975 hPa, the contribution to the surface radiation change
from the air temperature change in the bottom layer of the atmosphere would
not be included, which might have led to a biased quantification of the feedback.
We recommend interpolating the air temperature changes from the GCM vertical
coordinate to the kernel vertical coordinate, using surface values to
replace the missing levels (e.g., the 975 hPa level in the above example)
before multiplying with the kernel values when computing the feedbacks of
air temperature and water vapor.</p><supplementary-material position="anchor"><p id="d1e4115">The supplement related to this article is available online at: <inline-supplementary-material xlink:href="https://doi.org/10.5194/essd-15-3001-2023-supplement" xlink:title="pdf">https://doi.org/10.5194/essd-15-3001-2023-supplement</inline-supplementary-material>.</p></supplementary-material>
</sec>
</app>
  </app-group><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d1e4127">HH and YH led the design of this research and the writing of the paper.
HH produced the ERA5 radiative kernel and provided calculations of the
inter-kernel comparison and feedback analysis.</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e4133">The contact author has declared that neither of the authors has any competing interests.</p>
  </notes><notes notes-type="disclaimer"><title>Disclaimer</title>

      <p id="d1e4139">Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e4145">We thank Mark Zelinka, Ryan Kramer and one anonymous reviewer for their
helpful reviews.   Han Huang thanks Yonggang Liu, Jun Yang and Qiang
Wei for hosting her visit at Peking University, during which time part of
this work was completed.</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d1e4150">This research has been supported by the Natural Sciences and Engineering Research Council of Canada (grant no. RGPIN-2019-04511) and the Fonds de Recherche du Québec Nature et
technologies (grant no. 2021-PR-283823).</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d1e4156">This paper was edited by Tobias Gerken and reviewed by Mark Zelinka, Ryan Kramer, and one anonymous referee.</p>
  </notes><ref-list>
    <title>References</title>

      <ref id="bib1.bib1"><label>1</label><?label 1?><mixed-citation>Block, K. and Mauritsen, T.: Forcing and feedback in the MPI-ESM-LR coupled
model under abruptly quadrupled CO<inline-formula><mml:math id="M193" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, J. Adv. Model. Earth
Sy., 5, 676–691, 2013.</mixed-citation></ref>
      <ref id="bib1.bib2"><label>2</label><?label 1?><mixed-citation>Boucher, O., Servonnat, J., Albright, A. L., Aumont, O., Balkanski, Y.,
Bastrikov, V., Bekki, S., Bonnet, R., Bony, S., and Bopp, L.: Presentation
and evaluation of the IPSL-CM6A-LR climate model, J. Adv.
Model. Earth Sy., 12, e2019MS002010, <ext-link xlink:href="https://doi.org/10.1029/2019MS002010" ext-link-type="DOI">10.1029/2019MS002010</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib3"><label>3</label><?label 1?><mixed-citation>Bright, R. M. and O'Halloran, T. L.: Developing a monthly radiative kernel for surface albedo change from satellite climatologies of Earth's shortwave radiation budget: CACK v1.0, Geosci. Model Dev., 12, 3975–3990, <ext-link xlink:href="https://doi.org/10.5194/gmd-12-3975-2019" ext-link-type="DOI">10.5194/gmd-12-3975-2019</ext-link>, 2019.</mixed-citation></ref>
      <ref id="bib1.bib4"><label>4</label><?label 1?><mixed-citation>Chao, L.-W. and Dessler, A. E.: An assessment of climate feedbacks in
observations and climate models using different energy balance frameworks,
J. Climate, 34, 9763–9773, 2021.</mixed-citation></ref>
      <ref id="bib1.bib5"><label>5</label><?label 1?><mixed-citation>Collins, W., Ramaswamy, V., Schwarzkopf, M. D., Sun, Y., Portmann, R. W.,
Fu, Q., Casanova, S., Dufresne, J. L., Fillmore, D. W., and Forster, P.:
Radiative forcing by well-mixed greenhouse gases: Estimates from climate
models in the Intergovernmental Panel on Climate Change (IPCC) Fourth
Assessment Report (AR4), J. Geophys. Res.-Atmos., 111, D14317, <ext-link xlink:href="https://doi.org/10.1029/2005JD006713" ext-link-type="DOI">10.1029/2005JD006713</ext-link>,
2006.</mixed-citation></ref>
      <ref id="bib1.bib6"><label>6</label><?label 1?><mixed-citation>Colman, R. and McAvaney, B.: A study of general circulation model climate
feedbacks determined from perturbed sea surface temperature experiments,
J. Geophys. Res.-Atmos., 102, 19383–19402, 1997.</mixed-citation></ref>
      <ref id="bib1.bib7"><label>7</label><?label 1?><mixed-citation>Danabasoglu, G., Lamarque, J. F., Bacmeister, J., Bailey, D., DuVivier, A.,
Edwards, J., Emmons, L., Fasullo, J., Garcia, R., and Gettelman, A.: The
community earth system model version 2 (CESM2), J. Adv.
Model. Earth Sy., 12, e2019MS001916, <ext-link xlink:href="https://doi.org/10.1029/2019MS001916" ext-link-type="DOI">10.1029/2019MS001916</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib8"><label>8</label><?label 1?><mixed-citation>Dessler, A. E.: A determination of the cloud feedback from climate
variations over the past decade, Science, 330, 1523–1527, 2010.</mixed-citation></ref>
      <ref id="bib1.bib9"><label>9</label><?label 1?><mixed-citation>Doelling, D. R., Loeb, N. G., Keyes, D. F., Nordeen, M. L., Morstad, D.,
Nguyen, C., Wielicki, B. A., Young, D. F., and Sun, M.: Geostationary
enhanced temporal interpolation for CERES flux products, J.
Atmos. Ocean. Tech., 30, 1072–1090, 2013.</mixed-citation></ref>
      <ref id="bib1.bib10"><label>10</label><?label 1?><mixed-citation>Dong, Y., Armour, K. C., Zelinka, M. D., Proistosescu, C., Battisti, D. S.,
Zhou, C., and Andrews, T.: Intermodel spread in the pattern effect and its
contribution to climate sensitivity in CMIP5 and CMIP6 models, J.
Climate, 33, 7755–7775, 2020.</mixed-citation></ref>
      <ref id="bib1.bib11"><label>11</label><?label 1?><mixed-citation>Donohoe, A., Blanchard-Wrigglesworth, E., Schweiger, A., and Rasch, P. J.:
The effect of atmospheric transmissivity on model and observational
estimates of the sea ice albedo feedback, J. Climate, 33, 5743–5765,
2020.</mixed-citation></ref>
      <?pagebreak page3020?><ref id="bib1.bib12"><label>12</label><?label 1?><mixed-citation>Döscher, R., Acosta, M., Alessandri, A., Anthoni, P., Arsouze, T., Bergman, T., Bernardello, R., Boussetta, S., Caron, L.-P., Carver, G., Castrillo, M., Catalano, F., Cvijanovic, I., Davini, P., Dekker, E., Doblas-Reyes, F. J., Docquier, D., Echevarria, P., Fladrich, U., Fuentes-Franco, R., Gröger, M., v. Hardenberg, J., Hieronymus, J., Karami, M. P., Keskinen, J.-P., Koenigk, T., Makkonen, R., Massonnet, F., Ménégoz, M., Miller, P. A., Moreno-Chamarro, E., Nieradzik, L., van Noije, T., Nolan, P., O'Donnell, D., Ollinaho, P., van den Oord, G., Ortega, P., Prims, O. T., Ramos, A., Reerink, T., Rousset, C., Ruprich-Robert, Y., Le Sager, P., Schmith, T., Schrödner, R., Serva, F., Sicardi, V., Sloth Madsen, M., Smith, B., Tian, T., Tourigny, E., Uotila, P., Vancoppenolle, M., Wang, S., Wårlind, D., Willén, U., Wyser, K., Yang, S., Yepes-Arbós, X., and Zhang, Q.: The EC-Earth3 Earth system model for the Coupled Model Intercomparison Project 6, Geosci. Model Dev., 15, 2973–3020, <ext-link xlink:href="https://doi.org/10.5194/gmd-15-2973-2022" ext-link-type="DOI">10.5194/gmd-15-2973-2022</ext-link>, 2022.</mixed-citation></ref>
      <ref id="bib1.bib13"><label>13</label><?label 1?><mixed-citation>Eyring, V., Bony, S., Meehl, G. A., Senior, C. A., Stevens, B., Stouffer, R. J., and Taylor, K. E.: Overview of the Coupled Model Intercomparison Project Phase 6 (CMIP6) experimental design and organization, Geosci. Model Dev., 9, 1937–1958, <ext-link xlink:href="https://doi.org/10.5194/gmd-9-1937-2016" ext-link-type="DOI">10.5194/gmd-9-1937-2016</ext-link>, 2016.</mixed-citation></ref>
      <ref id="bib1.bib14"><label>14</label><?label 1?><mixed-citation>Graham, R. M., Hudson, S. R., and Maturilli, M.: Improved performance of
ERA5 in Arctic gateway relative to four global atmospheric reanalyses,
Geophys. Res. Lett., 46, 6138–6147, 2019.</mixed-citation></ref>
      <ref id="bib1.bib15"><label>15</label><?label 1?><mixed-citation>Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A.,
Muñoz-Sabater, J., Nicolas, J., Peubey, C., Radu, R., and Schepers, D.:
The ERA5 global reanalysis, Q. J. Roy. Meteorol.
Soc., 146, 1999–2049, 2020.</mixed-citation></ref>
      <ref id="bib1.bib16"><label>16</label><?label 1?><mixed-citation>Huang, H. and Huang, Y.: Nonlinear coupling between longwave radiative
climate feedbacks, J. Geophys. Res.-Atmos., 126,
e2020JD033995, <ext-link xlink:href="https://doi.org/10.1029/2020JD033995" ext-link-type="DOI">10.1029/2020JD033995</ext-link>, 2021.</mixed-citation></ref>
      <ref id="bib1.bib17"><label>17</label><?label 1?><mixed-citation>Huang, H. and Huang, Y.: Data for ERA5 radiative kernels, Mendeley [data set], <ext-link xlink:href="https://doi.org/10.17632/vmg3s67568" ext-link-type="DOI">10.17632/vmg3s67568</ext-link>, 2023.</mixed-citation></ref>
      <ref id="bib1.bib18"><label>18</label><?label 1?><mixed-citation>Huang, H., Huang, Y., and Hu, Y.: Quantifying the energetic feedbacks in
ENSO, Clim. Dynam., 56, 139–153, 2021.</mixed-citation></ref>
      <ref id="bib1.bib19"><label>19</label><?label 1?><mixed-citation>Huang, Y.: On the longwave climate feedbacks, J. Climate, 26,
7603–7610, 2013.</mixed-citation></ref>
      <ref id="bib1.bib20"><label>20</label><?label 1?><mixed-citation>Huang, Y. and Wang, Y.: How does radiation code accuracy matter?, J.
Geophys. Res.-Atmos., 124, 10742–10752, 2019.</mixed-citation></ref>
      <ref id="bib1.bib21"><label>21</label><?label 1?><mixed-citation>Huang, Y., Ramaswamy, V., and Soden, B.: An investigation of the sensitivity
of the clear-sky outgoing longwave radiation to atmospheric temperature and
water vapor, J. Geophys. Res.-Atmos., 112, D05104, <ext-link xlink:href="https://doi.org/10.1029/2005JD006906" ext-link-type="DOI">10.1029/2005JD006906</ext-link>, 2007.</mixed-citation></ref>
      <ref id="bib1.bib22"><label>22</label><?label 1?><mixed-citation>Huang, Y., Xia, Y., and Tan, X.: On the pattern of CO<inline-formula><mml:math id="M194" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> radiative forcing and
poleward energy transport, J. Geophys. Res.-Atmos.,
122, 10578–10593, 2017.</mixed-citation></ref>
      <ref id="bib1.bib23"><label>23</label><?label 1?><mixed-citation>Huang, Y., Chou, G., Xie, Y., and Soulard, N.: Radiative control of the
interannual variability of Arctic sea ice, Geophys. Res. Lett., 46,
9899–9908, 2019.</mixed-citation></ref>
      <ref id="bib1.bib24"><label>24</label><?label 1?><mixed-citation>Huang, Y., Huang, H., and Shakirova, A.: The nonlinear radiative feedback
effects in the Arctic warming, Front. Earth Sci., 651, <ext-link xlink:href="https://doi.org/10.3389/feart.2021.693779" ext-link-type="DOI">10.3389/feart.2021.693779</ext-link>, 2021.</mixed-citation></ref>
      <ref id="bib1.bib25"><label>25</label><?label 1?><mixed-citation>Jonko, A. K., Shell, K. M., Sanderson, B. M., and Danabasoglu, G.: Climate
feedbacks in CCSM3 under changing CO<inline-formula><mml:math id="M195" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> forcing. Part I: Adapting the linear
radiative kernel technique to feedback calculations for a broad range of
forcings, J. Climate, 25, 5260–5272, 2012.</mixed-citation></ref>
      <ref id="bib1.bib26"><label>26</label><?label 1?><mixed-citation>Kolly, A. and Huang, Y.: The radiative feedback during the ENSO cycle:
Observations versus models, J. Geophys. Res.-Atmos.,
123, 9097–9108, 2018.</mixed-citation></ref>
      <ref id="bib1.bib27"><label>27</label><?label 1?><mixed-citation>Kramer, R. J., Soden, B. J., and Pendergrass, A. G.: Evaluating Climate
Model Simulations of the Radiative Forcing and Radiative Response at Earth's
Surface, J. Climate, 32, 4089–4102, 2019a.</mixed-citation></ref>
      <ref id="bib1.bib28"><label>28</label><?label 1?><mixed-citation>Kramer, R. J., Matus, A. V., Soden, B. J., and L'Ecuyer, T. S.:
Observation-based radiative kernels from CloudSat/CALIPSO, J.
Geophys. Res.-Atmos., 124, 5431–5444, 2019b.</mixed-citation></ref>
      <ref id="bib1.bib29"><label>29</label><?label 1?><mixed-citation>Mauritsen, T., Bader, J., Becker, T., Behrens, J., Bittner, M., Brokopf, R.,
Brovkin, V., Claussen, M., Crueger, T., and Esch, M.: Developments in the
MPI-M Earth System Model version 1.2 (MPI-ESM1. 2) and its response to
increasing CO<inline-formula><mml:math id="M196" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, J. Adv. Model. Earth Sy., 11, 998–1038,
2019.</mixed-citation></ref>
      <ref id="bib1.bib30"><label>30</label><?label 1?><mixed-citation>Mlawer, E. J., Taubman, S. J., Brown, P. D., Iacono, M. J., and Clough, S.
A.: Radiative transfer for inhomogeneous atmospheres: RRTM, a validated
correlated-k model for the longwave, J. Geophys. Res.-Atmos., 102, 16663–16682, 1997.</mixed-citation></ref>
      <ref id="bib1.bib31"><label>31</label><?label 1?><mixed-citation>Myhre, G., Kramer, R., Smith, C., Hodnebrog, Ø., Forster, P., Soden, B.,
Samset, B., Stjern, C., Andrews, T., and Boucher, O.: Quantifying the
importance of rapid adjustments for global precipitation changes,
Geophys. Res. Lett., 45, 11399–11405, 2018.</mixed-citation></ref>
      <ref id="bib1.bib32"><label>32</label><?label 1?><mixed-citation>Pendergrass, A. G. and Hartmann, D. L.: The atmospheric energy constraint on
global-mean precipitation change, J. Climate, 27, 757–768, 2014.</mixed-citation></ref>
      <ref id="bib1.bib33"><label>33</label><?label 1?><mixed-citation>Pendergrass, A. G., Conley, A., and Vitt, F. M.: Surface and top-of-atmosphere radiative feedback kernels for CESM-CAM5, Earth Syst. Sci. Data, 10, 317–324, <ext-link xlink:href="https://doi.org/10.5194/essd-10-317-2018" ext-link-type="DOI">10.5194/essd-10-317-2018</ext-link>, 2018.</mixed-citation></ref>
      <ref id="bib1.bib34"><label>34</label><?label 1?><mixed-citation>Pincus, R., Buehler, S. A., Brath, M., Crevoisier, C., Jamil, O., Franklin
Evans, K., Manners, J., Menzel, R. L., Mlawer, E. J., and Paynter, D.:
Benchmark calculations of radiative forcing by greenhouse gases, J.
Geophys. Res.-Atmos., 125, e2020JD033483, <ext-link xlink:href="https://doi.org/10.1029/2020JD033483" ext-link-type="DOI">10.1029/2020JD033483</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib35"><label>35</label><?label 1?><mixed-citation>Previdi, M.: Radiative feedbacks on global precipitation, Environ.
Res. Lett., 5, 025211, <ext-link xlink:href="https://doi.org/10.1088/1748-9326/5/2/025211" ext-link-type="DOI">10.1088/1748-9326/5/2/025211</ext-link>, 2010.</mixed-citation></ref>
      <ref id="bib1.bib36"><label>36</label><?label 1?><mixed-citation>Riihelä, A., Bright, R. M., and Anttila, K.: Recent strengthening of
snow and ice albedo feedback driven by Antarctic sea-ice loss, Nat.
Geosci., 14, 832–836, 2021.</mixed-citation></ref>
      <ref id="bib1.bib37"><label>37</label><?label 1?><mixed-citation>Shell, K. M., Kiehl, J. T., and Shields, C. A.: Using the radiative kernel
technique to calculate climate feedbacks in NCAR's Community Atmospheric
Model, J. Climate, 21, 2269–2282, 2008.</mixed-citation></ref>
      <ref id="bib1.bib38"><label>38</label><?label 1?><mixed-citation>Smith, C. J., Kramer, R. J., and Sima, A.: The HadGEM3-GA7.1 radiative kernel: the importance of a well-resolved stratosphere, Earth Syst. Sci. Data, 12, 2157–2168, <ext-link xlink:href="https://doi.org/10.5194/essd-12-2157-2020" ext-link-type="DOI">10.5194/essd-12-2157-2020</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib39"><label>39</label><?label 1?><mixed-citation>Soden, B. J. and Held, I. M.: An assessment of climate feedbacks in coupled
ocean–atmosphere models, J. Climate, 19, 3354–3360, 2006.</mixed-citation></ref>
      <ref id="bib1.bib40"><label>40</label><?label 1?><mixed-citation>Soden, B. J., Held, I. M., Colman, R., Shell, K. M., Kiehl, J. T., and
Shields, C. A.: Quantifying climate feedbacks using radiative kernels,
J. Climate, 21, 3504–3520, 2008.</mixed-citation></ref>
      <ref id="bib1.bib41"><label>41</label><?label 1?><mixed-citation>Taylor, K. E., Stouffer, R. J., and Meehl, G. A.: An overview of CMIP5 and
the experiment design, B. Am. Meteorol. Soc., 93,
485–498, 2012.</mixed-citation></ref>
      <ref id="bib1.bib42"><label>42</label><?label 1?><mixed-citation>Thorsen, T. J., Kato, S., Loeb, N. G., and Rose, F. G.: Observation-based
decomposition of radiative perturbations and radiative kernels, J.
Climate, 31, 10039–10058, 2018.</mixed-citation></ref>
      <ref id="bib1.bib43"><label>43</label><?label 1?><mixed-citation>Vargas Zeppetello, L., Donohoe, A., and Battisti, D.: Does surface
temperature respond to or determine downwelling longwave radiation?,
Geophys. Res. Lett., 46, 2781–2789, 2019.</mixed-citation></ref>
      <ref id="bib1.bib44"><label>44</label><?label 1?><mixed-citation>Vial, J., Dufresne, J.-L., and Bony, S.: On the interpretation of
inter-model spread in CMIP5 climate sensitivity estimates, Clim. Dynam.,
41, 3339–3362, 2013.</mixed-citation></ref>
      <ref id="bib1.bib45"><label>45</label><?label 1?><mixed-citation>Voldoire, A., Saint-Martin, D., Sénési, S., Decharme, B., Alias, A.,
Chevallier, M., Colin, J., Guérémy, J. F., Michou, M., and Moine, M.
P.: Evaluation of CMIP6 deck experiments with CNRM-CM6-1, J.
Adv. Model. Earth Sy., 11, 2177–2213, 2019.</mixed-citation></ref>
      <ref id="bib1.bib46"><label>46</label><?label 1?><mixed-citation>Wetherald, R. and Manabe, S.: Cloud feedback processes in a general
circulation model, J. Atmos. Sci., 45, 1397–1416, 1988.</mixed-citation></ref>
      <ref id="bib1.bib47"><label>47</label><?label 1?><mixed-citation>Williams, K., Copsey, D., Blockley, E., Bodas-Salcedo, A., Calvert, D.,
Comer, R., Davis, P., Graham, T., Hewitt, H., and Hill, R.: The Met Office
global coupled model 3.0 and 3.1 (GC3. 0 an<?pagebreak page3021?>d GC3. 1) configurations, J.
Adv. Model. Earth Sy., 10, 357–380, 2018.</mixed-citation></ref>
      <ref id="bib1.bib48"><label>48</label><?label 1?><mixed-citation>Wright, J. S., Sun, X., Konopka, P., Krüger, K., Legras, B., Molod, A. M., Tegtmeier, S., Zhang, G. J., and Zhao, X.: Differences in tropical high clouds among reanalyses: origins and radiative impacts, Atmos. Chem. Phys., 20, 8989–9030, <ext-link xlink:href="https://doi.org/10.5194/acp-20-8989-2020" ext-link-type="DOI">10.5194/acp-20-8989-2020</ext-link>, 2020.</mixed-citation></ref>
      <ref id="bib1.bib49"><label>49</label><?label 1?><mixed-citation>Yue, Q., Kahn, B. H., Fetzer, E. J., Schreier, M., Wong, S., Chen, X., and
Huang, X.: Observation-based longwave cloud radiative kernels derived from
the A-Train, J. Climate, 29, 2023–2040, 2016.</mixed-citation></ref>
      <ref id="bib1.bib50"><label>50</label><?label 1?><mixed-citation>Zelinka, M. D., Klein, S. A., and Hartmann, D. L.: Computing and
partitioning cloud feedbacks using cloud property histograms. Part I: Cloud
radiative kernels, J. Climate, 25, 3715–3735, 2012.</mixed-citation></ref>
      <ref id="bib1.bib51"><label>51</label><?label 1?><mixed-citation>Zelinka, M. D., Myers, T. A., McCoy, D. T., Po-Chedley, S., Caldwell, P. M.,
Ceppi, P., Klein, S. A., and Taylor, K. E.: Causes of higher climate
sensitivity in CMIP6 models, Geophys. Res. Lett., 47,  e2019GL085782, <ext-link xlink:href="https://doi.org/10.1029/2019GL085782" ext-link-type="DOI">10.1029/2019GL085782</ext-link>,
2020.
</mixed-citation></ref><?xmltex \hack{\newpage}?>
      <ref id="bib1.bib52"><label>52</label><?label 1?><mixed-citation>Zhang, B., Kramer, R. J., and Soden, B. J.: Radiative feedbacks associated
with the Madden–Julian oscillation, J. Climate, 32, 7055–7065,
2019.</mixed-citation></ref>
      <ref id="bib1.bib53"><label>53</label><?label 1?><mixed-citation>Zhang, M. and Huang, Y.: Radiative forcing of quadrupling CO<inline-formula><mml:math id="M197" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, J.
Climate, 27, 2496–2508, 2014.</mixed-citation></ref>
      <ref id="bib1.bib54"><label>54</label><?label 1?><mixed-citation>Zhang, Y., Jin, Z., and Sikand, M.: The top-of-atmosphere, surface and
atmospheric cloud radiative kernels based on ISCCP-H datasets: method and
evaluation, J. Geophys. Res.-Atmos., 126,
e2021JD035053, <ext-link xlink:href="https://doi.org/10.1029/2021JD035053" ext-link-type="DOI">10.1029/2021JD035053</ext-link>, 2021.</mixed-citation></ref>
      <ref id="bib1.bib55"><label>55</label><?label 1?><mixed-citation>Zhou, C., Zelinka, M. D., Dessler, A. E., and Yang, P.: An analysis of the
short-term cloud feedback using MODIS data, J. Climate, 26,
4803–4815, 2013.</mixed-citation></ref>
      <ref id="bib1.bib56"><label>56</label><?label 1?><mixed-citation>Zhou, C., Liu, Y., and Wang, Q.: Calculating the climatology and anomalies
of surface cloud radiative effect using cloud property histograms and cloud
radiative kernels, Adv. Atmos. Sci., 39, 2124-2136, 2022.</mixed-citation></ref>

  </ref-list></back>
    <!--<article-title-html>Radiative sensitivity quantified by a new set of radiation flux kernels based on the ECMWF Reanalysis v5 (ERA5)</article-title-html>
<abstract-html/>
<ref-html id="bib1.bib1"><label>1</label><mixed-citation>
      
Block, K. and Mauritsen, T.: Forcing and feedback in the MPI-ESM-LR coupled
model under abruptly quadrupled CO<sub>2</sub>, J. Adv. Model. Earth
Sy., 5, 676–691, 2013.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib2"><label>2</label><mixed-citation>
      Boucher, O., Servonnat, J., Albright, A. L., Aumont, O., Balkanski, Y.,
Bastrikov, V., Bekki, S., Bonnet, R., Bony, S., and Bopp, L.: Presentation
and evaluation of the IPSL-CM6A-LR climate model, J. Adv.
Model. Earth Sy., 12, e2019MS002010, <a href="https://doi.org/10.1029/2019MS002010" target="_blank">https://doi.org/10.1029/2019MS002010</a>, 2020.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib3"><label>3</label><mixed-citation>
      Bright, R. M. and O'Halloran, T. L.: Developing a monthly radiative kernel for surface albedo change from satellite climatologies of Earth's shortwave radiation budget: CACK v1.0, Geosci. Model Dev., 12, 3975–3990, <a href="https://doi.org/10.5194/gmd-12-3975-2019" target="_blank">https://doi.org/10.5194/gmd-12-3975-2019</a>, 2019.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib4"><label>4</label><mixed-citation>
      Chao, L.-W. and Dessler, A. E.: An assessment of climate feedbacks in
observations and climate models using different energy balance frameworks,
J. Climate, 34, 9763–9773, 2021.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib5"><label>5</label><mixed-citation>
      Collins, W., Ramaswamy, V., Schwarzkopf, M. D., Sun, Y., Portmann, R. W.,
Fu, Q., Casanova, S., Dufresne, J. L., Fillmore, D. W., and Forster, P.:
Radiative forcing by well-mixed greenhouse gases: Estimates from climate
models in the Intergovernmental Panel on Climate Change (IPCC) Fourth
Assessment Report (AR4), J. Geophys. Res.-Atmos., 111, D14317, <a href="https://doi.org/10.1029/2005JD006713" target="_blank">https://doi.org/10.1029/2005JD006713</a>,
2006.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib6"><label>6</label><mixed-citation>
      Colman, R. and McAvaney, B.: A study of general circulation model climate
feedbacks determined from perturbed sea surface temperature experiments,
J. Geophys. Res.-Atmos., 102, 19383–19402, 1997.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib7"><label>7</label><mixed-citation>
      Danabasoglu, G., Lamarque, J. F., Bacmeister, J., Bailey, D., DuVivier, A.,
Edwards, J., Emmons, L., Fasullo, J., Garcia, R., and Gettelman, A.: The
community earth system model version 2 (CESM2), J. Adv.
Model. Earth Sy., 12, e2019MS001916, <a href="https://doi.org/10.1029/2019MS001916" target="_blank">https://doi.org/10.1029/2019MS001916</a>, 2020.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib8"><label>8</label><mixed-citation>
      Dessler, A. E.: A determination of the cloud feedback from climate
variations over the past decade, Science, 330, 1523–1527, 2010.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib9"><label>9</label><mixed-citation>
      Doelling, D. R., Loeb, N. G., Keyes, D. F., Nordeen, M. L., Morstad, D.,
Nguyen, C., Wielicki, B. A., Young, D. F., and Sun, M.: Geostationary
enhanced temporal interpolation for CERES flux products, J.
Atmos. Ocean. Tech., 30, 1072–1090, 2013.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib10"><label>10</label><mixed-citation>
      Dong, Y., Armour, K. C., Zelinka, M. D., Proistosescu, C., Battisti, D. S.,
Zhou, C., and Andrews, T.: Intermodel spread in the pattern effect and its
contribution to climate sensitivity in CMIP5 and CMIP6 models, J.
Climate, 33, 7755–7775, 2020.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib11"><label>11</label><mixed-citation>
      Donohoe, A., Blanchard-Wrigglesworth, E., Schweiger, A., and Rasch, P. J.:
The effect of atmospheric transmissivity on model and observational
estimates of the sea ice albedo feedback, J. Climate, 33, 5743–5765,
2020.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib12"><label>12</label><mixed-citation>
      Döscher, R., Acosta, M., Alessandri, A., Anthoni, P., Arsouze, T., Bergman, T., Bernardello, R., Boussetta, S., Caron, L.-P., Carver, G., Castrillo, M., Catalano, F., Cvijanovic, I., Davini, P., Dekker, E., Doblas-Reyes, F. J., Docquier, D., Echevarria, P., Fladrich, U., Fuentes-Franco, R., Gröger, M., v. Hardenberg, J., Hieronymus, J., Karami, M. P., Keskinen, J.-P., Koenigk, T., Makkonen, R., Massonnet, F., Ménégoz, M., Miller, P. A., Moreno-Chamarro, E., Nieradzik, L., van Noije, T., Nolan, P., O'Donnell, D., Ollinaho, P., van den Oord, G., Ortega, P., Prims, O. T., Ramos, A., Reerink, T., Rousset, C., Ruprich-Robert, Y., Le Sager, P., Schmith, T., Schrödner, R., Serva, F., Sicardi, V., Sloth Madsen, M., Smith, B., Tian, T., Tourigny, E., Uotila, P., Vancoppenolle, M., Wang, S., Wårlind, D., Willén, U., Wyser, K., Yang, S., Yepes-Arbós, X., and Zhang, Q.: The EC-Earth3 Earth system model for the Coupled Model Intercomparison Project 6, Geosci. Model Dev., 15, 2973–3020, <a href="https://doi.org/10.5194/gmd-15-2973-2022" target="_blank">https://doi.org/10.5194/gmd-15-2973-2022</a>, 2022.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib13"><label>13</label><mixed-citation>
      Eyring, V., Bony, S., Meehl, G. A., Senior, C. A., Stevens, B., Stouffer, R. J., and Taylor, K. E.: Overview of the Coupled Model Intercomparison Project Phase 6 (CMIP6) experimental design and organization, Geosci. Model Dev., 9, 1937–1958, <a href="https://doi.org/10.5194/gmd-9-1937-2016" target="_blank">https://doi.org/10.5194/gmd-9-1937-2016</a>, 2016.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib14"><label>14</label><mixed-citation>
      Graham, R. M., Hudson, S. R., and Maturilli, M.: Improved performance of
ERA5 in Arctic gateway relative to four global atmospheric reanalyses,
Geophys. Res. Lett., 46, 6138–6147, 2019.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib15"><label>15</label><mixed-citation>
      Hersbach, H., Bell, B., Berrisford, P., Hirahara, S., Horányi, A.,
Muñoz-Sabater, J., Nicolas, J., Peubey, C., Radu, R., and Schepers, D.:
The ERA5 global reanalysis, Q. J. Roy. Meteorol.
Soc., 146, 1999–2049, 2020.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib16"><label>16</label><mixed-citation>
      Huang, H. and Huang, Y.: Nonlinear coupling between longwave radiative
climate feedbacks, J. Geophys. Res.-Atmos., 126,
e2020JD033995, <a href="https://doi.org/10.1029/2020JD033995" target="_blank">https://doi.org/10.1029/2020JD033995</a>, 2021.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib17"><label>17</label><mixed-citation>
      Huang, H. and Huang, Y.: Data for ERA5 radiative kernels, Mendeley [data set], <a href="https://doi.org/10.17632/vmg3s67568" target="_blank">https://doi.org/10.17632/vmg3s67568</a>, 2023.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib18"><label>18</label><mixed-citation>
      Huang, H., Huang, Y., and Hu, Y.: Quantifying the energetic feedbacks in
ENSO, Clim. Dynam., 56, 139–153, 2021.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib19"><label>19</label><mixed-citation>
      Huang, Y.: On the longwave climate feedbacks, J. Climate, 26,
7603–7610, 2013.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib20"><label>20</label><mixed-citation>
      Huang, Y. and Wang, Y.: How does radiation code accuracy matter?, J.
Geophys. Res.-Atmos., 124, 10742–10752, 2019.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib21"><label>21</label><mixed-citation>
      Huang, Y., Ramaswamy, V., and Soden, B.: An investigation of the sensitivity
of the clear-sky outgoing longwave radiation to atmospheric temperature and
water vapor, J. Geophys. Res.-Atmos., 112, D05104, <a href="https://doi.org/10.1029/2005JD006906" target="_blank">https://doi.org/10.1029/2005JD006906</a>, 2007.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib22"><label>22</label><mixed-citation>
      Huang, Y., Xia, Y., and Tan, X.: On the pattern of CO<sub>2</sub> radiative forcing and
poleward energy transport, J. Geophys. Res.-Atmos.,
122, 10578–10593, 2017.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib23"><label>23</label><mixed-citation>
      Huang, Y., Chou, G., Xie, Y., and Soulard, N.: Radiative control of the
interannual variability of Arctic sea ice, Geophys. Res. Lett., 46,
9899–9908, 2019.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib24"><label>24</label><mixed-citation>
      Huang, Y., Huang, H., and Shakirova, A.: The nonlinear radiative feedback
effects in the Arctic warming, Front. Earth Sci., 651, <a href="https://doi.org/10.3389/feart.2021.693779" target="_blank">https://doi.org/10.3389/feart.2021.693779</a>, 2021.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib25"><label>25</label><mixed-citation>
      Jonko, A. K., Shell, K. M., Sanderson, B. M., and Danabasoglu, G.: Climate
feedbacks in CCSM3 under changing CO<sub>2</sub> forcing. Part I: Adapting the linear
radiative kernel technique to feedback calculations for a broad range of
forcings, J. Climate, 25, 5260–5272, 2012.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib26"><label>26</label><mixed-citation>
      Kolly, A. and Huang, Y.: The radiative feedback during the ENSO cycle:
Observations versus models, J. Geophys. Res.-Atmos.,
123, 9097–9108, 2018.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib27"><label>27</label><mixed-citation>
      Kramer, R. J., Soden, B. J., and Pendergrass, A. G.: Evaluating Climate
Model Simulations of the Radiative Forcing and Radiative Response at Earth's
Surface, J. Climate, 32, 4089–4102, 2019a.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib28"><label>28</label><mixed-citation>
      Kramer, R. J., Matus, A. V., Soden, B. J., and L'Ecuyer, T. S.:
Observation-based radiative kernels from CloudSat/CALIPSO, J.
Geophys. Res.-Atmos., 124, 5431–5444, 2019b.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib29"><label>29</label><mixed-citation>
      Mauritsen, T., Bader, J., Becker, T., Behrens, J., Bittner, M., Brokopf, R.,
Brovkin, V., Claussen, M., Crueger, T., and Esch, M.: Developments in the
MPI-M Earth System Model version 1.2 (MPI-ESM1. 2) and its response to
increasing CO<sub>2</sub>, J. Adv. Model. Earth Sy., 11, 998–1038,
2019.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib30"><label>30</label><mixed-citation>
      Mlawer, E. J., Taubman, S. J., Brown, P. D., Iacono, M. J., and Clough, S.
A.: Radiative transfer for inhomogeneous atmospheres: RRTM, a validated
correlated-k model for the longwave, J. Geophys. Res.-Atmos., 102, 16663–16682, 1997.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib31"><label>31</label><mixed-citation>
      Myhre, G., Kramer, R., Smith, C., Hodnebrog, Ø., Forster, P., Soden, B.,
Samset, B., Stjern, C., Andrews, T., and Boucher, O.: Quantifying the
importance of rapid adjustments for global precipitation changes,
Geophys. Res. Lett., 45, 11399–11405, 2018.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib32"><label>32</label><mixed-citation>
      Pendergrass, A. G. and Hartmann, D. L.: The atmospheric energy constraint on
global-mean precipitation change, J. Climate, 27, 757–768, 2014.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib33"><label>33</label><mixed-citation>
      Pendergrass, A. G., Conley, A., and Vitt, F. M.: Surface and top-of-atmosphere radiative feedback kernels for CESM-CAM5, Earth Syst. Sci. Data, 10, 317–324, <a href="https://doi.org/10.5194/essd-10-317-2018" target="_blank">https://doi.org/10.5194/essd-10-317-2018</a>, 2018.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib34"><label>34</label><mixed-citation>
      Pincus, R., Buehler, S. A., Brath, M., Crevoisier, C., Jamil, O., Franklin
Evans, K., Manners, J., Menzel, R. L., Mlawer, E. J., and Paynter, D.:
Benchmark calculations of radiative forcing by greenhouse gases, J.
Geophys. Res.-Atmos., 125, e2020JD033483, <a href="https://doi.org/10.1029/2020JD033483" target="_blank">https://doi.org/10.1029/2020JD033483</a>, 2020.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib35"><label>35</label><mixed-citation>
      Previdi, M.: Radiative feedbacks on global precipitation, Environ.
Res. Lett., 5, 025211, <a href="https://doi.org/10.1088/1748-9326/5/2/025211" target="_blank">https://doi.org/10.1088/1748-9326/5/2/025211</a>, 2010.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib36"><label>36</label><mixed-citation>
      Riihelä, A., Bright, R. M., and Anttila, K.: Recent strengthening of
snow and ice albedo feedback driven by Antarctic sea-ice loss, Nat.
Geosci., 14, 832–836, 2021.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib37"><label>37</label><mixed-citation>
      Shell, K. M., Kiehl, J. T., and Shields, C. A.: Using the radiative kernel
technique to calculate climate feedbacks in NCAR's Community Atmospheric
Model, J. Climate, 21, 2269–2282, 2008.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib38"><label>38</label><mixed-citation>
      Smith, C. J., Kramer, R. J., and Sima, A.: The HadGEM3-GA7.1 radiative kernel: the importance of a well-resolved stratosphere, Earth Syst. Sci. Data, 12, 2157–2168, <a href="https://doi.org/10.5194/essd-12-2157-2020" target="_blank">https://doi.org/10.5194/essd-12-2157-2020</a>, 2020.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib39"><label>39</label><mixed-citation>
      Soden, B. J. and Held, I. M.: An assessment of climate feedbacks in coupled
ocean–atmosphere models, J. Climate, 19, 3354–3360, 2006.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib40"><label>40</label><mixed-citation>
      Soden, B. J., Held, I. M., Colman, R., Shell, K. M., Kiehl, J. T., and
Shields, C. A.: Quantifying climate feedbacks using radiative kernels,
J. Climate, 21, 3504–3520, 2008.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib41"><label>41</label><mixed-citation>
      Taylor, K. E., Stouffer, R. J., and Meehl, G. A.: An overview of CMIP5 and
the experiment design, B. Am. Meteorol. Soc., 93,
485–498, 2012.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib42"><label>42</label><mixed-citation>
      Thorsen, T. J., Kato, S., Loeb, N. G., and Rose, F. G.: Observation-based
decomposition of radiative perturbations and radiative kernels, J.
Climate, 31, 10039–10058, 2018.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib43"><label>43</label><mixed-citation>
      Vargas Zeppetello, L., Donohoe, A., and Battisti, D.: Does surface
temperature respond to or determine downwelling longwave radiation?,
Geophys. Res. Lett., 46, 2781–2789, 2019.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib44"><label>44</label><mixed-citation>
      Vial, J., Dufresne, J.-L., and Bony, S.: On the interpretation of
inter-model spread in CMIP5 climate sensitivity estimates, Clim. Dynam.,
41, 3339–3362, 2013.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib45"><label>45</label><mixed-citation>
      Voldoire, A., Saint-Martin, D., Sénési, S., Decharme, B., Alias, A.,
Chevallier, M., Colin, J., Guérémy, J. F., Michou, M., and Moine, M.
P.: Evaluation of CMIP6 deck experiments with CNRM-CM6-1, J.
Adv. Model. Earth Sy., 11, 2177–2213, 2019.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib46"><label>46</label><mixed-citation>
      Wetherald, R. and Manabe, S.: Cloud feedback processes in a general
circulation model, J. Atmos. Sci., 45, 1397–1416, 1988.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib47"><label>47</label><mixed-citation>
      Williams, K., Copsey, D., Blockley, E., Bodas-Salcedo, A., Calvert, D.,
Comer, R., Davis, P., Graham, T., Hewitt, H., and Hill, R.: The Met Office
global coupled model 3.0 and 3.1 (GC3. 0 and GC3. 1) configurations, J.
Adv. Model. Earth Sy., 10, 357–380, 2018.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib48"><label>48</label><mixed-citation>
      Wright, J. S., Sun, X., Konopka, P., Krüger, K., Legras, B., Molod, A. M., Tegtmeier, S., Zhang, G. J., and Zhao, X.: Differences in tropical high clouds among reanalyses: origins and radiative impacts, Atmos. Chem. Phys., 20, 8989–9030, <a href="https://doi.org/10.5194/acp-20-8989-2020" target="_blank">https://doi.org/10.5194/acp-20-8989-2020</a>, 2020.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib49"><label>49</label><mixed-citation>
      Yue, Q., Kahn, B. H., Fetzer, E. J., Schreier, M., Wong, S., Chen, X., and
Huang, X.: Observation-based longwave cloud radiative kernels derived from
the A-Train, J. Climate, 29, 2023–2040, 2016.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib50"><label>50</label><mixed-citation>
      Zelinka, M. D., Klein, S. A., and Hartmann, D. L.: Computing and
partitioning cloud feedbacks using cloud property histograms. Part I: Cloud
radiative kernels, J. Climate, 25, 3715–3735, 2012.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib51"><label>51</label><mixed-citation>
      Zelinka, M. D., Myers, T. A., McCoy, D. T., Po-Chedley, S., Caldwell, P. M.,
Ceppi, P., Klein, S. A., and Taylor, K. E.: Causes of higher climate
sensitivity in CMIP6 models, Geophys. Res. Lett., 47,  e2019GL085782, <a href="https://doi.org/10.1029/2019GL085782" target="_blank">https://doi.org/10.1029/2019GL085782</a>,
2020.


    </mixed-citation></ref-html>
<ref-html id="bib1.bib52"><label>52</label><mixed-citation>
      Zhang, B., Kramer, R. J., and Soden, B. J.: Radiative feedbacks associated
with the Madden–Julian oscillation, J. Climate, 32, 7055–7065,
2019.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib53"><label>53</label><mixed-citation>
      Zhang, M. and Huang, Y.: Radiative forcing of quadrupling CO<sub>2</sub>, J.
Climate, 27, 2496–2508, 2014.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib54"><label>54</label><mixed-citation>
      Zhang, Y., Jin, Z., and Sikand, M.: The top-of-atmosphere, surface and
atmospheric cloud radiative kernels based on ISCCP-H datasets: method and
evaluation, J. Geophys. Res.-Atmos., 126,
e2021JD035053, <a href="https://doi.org/10.1029/2021JD035053" target="_blank">https://doi.org/10.1029/2021JD035053</a>, 2021.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib55"><label>55</label><mixed-citation>
      Zhou, C., Zelinka, M. D., Dessler, A. E., and Yang, P.: An analysis of the
short-term cloud feedback using MODIS data, J. Climate, 26,
4803–4815, 2013.

    </mixed-citation></ref-html>
<ref-html id="bib1.bib56"><label>56</label><mixed-citation>
      Zhou, C., Liu, Y., and Wang, Q.: Calculating the climatology and anomalies
of surface cloud radiative effect using cloud property histograms and cloud
radiative kernels, Adv. Atmos. Sci., 39, 2124-2136, 2022.

    </mixed-citation></ref-html>--></article>
