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  <front>
    <journal-meta><journal-id journal-id-type="publisher">ESSD</journal-id><journal-title-group>
    <journal-title>Earth System Science Data</journal-title>
    <abbrev-journal-title abbrev-type="publisher">ESSD</abbrev-journal-title><abbrev-journal-title abbrev-type="nlm-ta">Earth Syst. Sci. Data</abbrev-journal-title>
  </journal-title-group><issn pub-type="epub">1866-3516</issn><publisher>
    <publisher-name>Copernicus Publications</publisher-name>
    <publisher-loc>Göttingen, Germany</publisher-loc>
  </publisher></journal-meta>
    <article-meta>
      <article-id pub-id-type="doi">10.5194/essd-14-1917-2022</article-id><title-group><article-title>Global Carbon Budget 2021</article-title><alt-title>Global Carbon Budget 2021</alt-title>
      </title-group><?xmltex \runningtitle{Global Carbon Budget 2021}?><?xmltex \runningauthor{P. Friedlingstein et al.}?>
      <contrib-group>
        <contrib contrib-type="author" corresp="yes" rid="aff1 aff2">
          <name><surname>Friedlingstein</surname><given-names>Pierre</given-names></name>
          <email>p.friedlingstein@exeter.ac.uk</email>
        <ext-link>https://orcid.org/0000-0003-3309-4739</ext-link></contrib>
        <contrib contrib-type="author" corresp="no" rid="aff3">
          <name><surname>Jones</surname><given-names>Matthew W.</given-names></name>
          
        </contrib>
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          <name><surname>O'Sullivan</surname><given-names>Michael</given-names></name>
          
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        <contrib contrib-type="author" corresp="no" rid="aff4">
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          <name><surname>Le Quéré</surname><given-names>Corinne</given-names></name>
          
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          <name><surname>Peters</surname><given-names>Glen P.</given-names></name>
          
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          <name><surname>Peters</surname><given-names>Wouter</given-names></name>
          
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          <name><surname>Pongratz</surname><given-names>Julia</given-names></name>
          
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          <name><surname>Sitch</surname><given-names>Stephen</given-names></name>
          
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          <name><surname>Ciais</surname><given-names>Philippe</given-names></name>
          
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          <name><surname>Jackson</surname><given-names>Rob B.</given-names></name>
          
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          <name><surname>Alin</surname><given-names>Simone R.</given-names></name>
          
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          <name><surname>Anthoni</surname><given-names>Peter</given-names></name>
          
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        <contrib contrib-type="author" corresp="no" rid="aff17">
          <name><surname>Bates</surname><given-names>Nicholas R.</given-names></name>
          
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          <name><surname>Becker</surname><given-names>Meike</given-names></name>
          
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          <name><surname>Bellouin</surname><given-names>Nicolas</given-names></name>
          
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          <name><surname>Bopp</surname><given-names>Laurent</given-names></name>
          
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          <name><surname>Chau</surname><given-names>Thi Tuyet Trang</given-names></name>
          
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          <name><surname>Chevallier</surname><given-names>Frédéric</given-names></name>
          
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          <name><surname>Chini</surname><given-names>Louise P.</given-names></name>
          
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          <name><surname>Cronin</surname><given-names>Margot</given-names></name>
          
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          <name><surname>Currie</surname><given-names>Kim I.</given-names></name>
          
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          <name><surname>Decharme</surname><given-names>Bertrand</given-names></name>
          
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          <name><surname>Djeutchouang</surname><given-names>Laique M.</given-names></name>
          
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          <name><surname>Dou</surname><given-names>Xinyu</given-names></name>
          
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          <name><surname>Evans</surname><given-names>Wiley</given-names></name>
          
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          <name><surname>Feely</surname><given-names>Richard A.</given-names></name>
          
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          <name><surname>Feng</surname><given-names>Liang</given-names></name>
          
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          <name><surname>Gasser</surname><given-names>Thomas</given-names></name>
          
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          <name><surname>Gilfillan</surname><given-names>Dennis</given-names></name>
          
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          <name><surname>Gkritzalis</surname><given-names>Thanos</given-names></name>
          
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          <name><surname>Grassi</surname><given-names>Giacomo</given-names></name>
          
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          <name><surname>Gregor</surname><given-names>Luke</given-names></name>
          
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          <name><surname>Gruber</surname><given-names>Nicolas</given-names></name>
          
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          <name><surname>Gürses</surname><given-names>Özgür</given-names></name>
          
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          <name><surname>Harris</surname><given-names>Ian</given-names></name>
          
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          <name><surname>Houghton</surname><given-names>Richard A.</given-names></name>
          
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        <contrib contrib-type="author" corresp="no" rid="aff21">
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          <name><surname>Iida</surname><given-names>Yosuke</given-names></name>
          
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          <name><surname>Ilyina</surname><given-names>Tatiana</given-names></name>
          
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          <name><surname>Luijkx</surname><given-names>Ingrid T.</given-names></name>
          
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          <name><surname>Jain</surname><given-names>Atul</given-names></name>
          
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          <name><surname>Jones</surname><given-names>Steve D.</given-names></name>
          
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        <contrib contrib-type="author" corresp="no" rid="aff39">
          <name><surname>Kato</surname><given-names>Etsushi</given-names></name>
          
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          <name><surname>Kennedy</surname><given-names>Daniel</given-names></name>
          
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          <name><surname>Klein Goldewijk</surname><given-names>Kees</given-names></name>
          
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          <name><surname>Knauer</surname><given-names>Jürgen</given-names></name>
          
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          <name><surname>Korsbakken</surname><given-names>Jan Ivar</given-names></name>
          
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          <name><surname>Lauvset</surname><given-names>Siv K.</given-names></name>
          
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          <name><surname>Liu</surname><given-names>Junjie</given-names></name>
          
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          <name><surname>Marland</surname><given-names>Gregg</given-names></name>
          
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          <name><surname>McGuire</surname><given-names>Patrick C.</given-names></name>
          
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        <contrib contrib-type="author" corresp="no" rid="aff51">
          <name><surname>Melton</surname><given-names>Joe R.</given-names></name>
          
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          <name><surname>Munro</surname><given-names>David R.</given-names></name>
          
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          <name><surname>Nabel</surname><given-names>Julia E. M. S.</given-names></name>
          
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          <name><surname>Nakaoka</surname><given-names>Shin-Ichiro</given-names></name>
          
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          <name><surname>Niwa</surname><given-names>Yosuke</given-names></name>
          
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          <name><surname>Resplandy</surname><given-names>Laure</given-names></name>
          
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          <name><surname>Robertson</surname><given-names>Eddy</given-names></name>
          
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          <name><surname>Rosan</surname><given-names>Thais M.</given-names></name>
          
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          <name><surname>Sutton</surname><given-names>Adrienne J.</given-names></name>
          
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          <name><surname>Sweeney</surname><given-names>Colm</given-names></name>
          
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          <name><surname>Tanhua</surname><given-names>Toste</given-names></name>
          
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          <name><surname>Tans</surname><given-names>Pieter P.</given-names></name>
          
        </contrib>
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          <name><surname>Tian</surname><given-names>Hanqin</given-names></name>
          
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          <name><surname>Tilbrook</surname><given-names>Bronte</given-names></name>
          
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        <contrib contrib-type="author" corresp="no" rid="aff67">
          <name><surname>Tubiello</surname><given-names>Francesco</given-names></name>
          
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        <contrib contrib-type="author" corresp="no" rid="aff68">
          <name><surname>van der Werf</surname><given-names>Guido R.</given-names></name>
          
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        <aff id="aff1"><label>1</label><institution>College of Engineering, Mathematics and Physical Sciences, University of Exeter, Exeter EX4 4QF, UK</institution>
        </aff>
        <aff id="aff2"><label>2</label><institution>Laboratoire de Météorologie Dynamique, Institut Pierre-Simon Laplace, CNRS-ENS-UPMC-X, Paris, France</institution>
        </aff>
        <aff id="aff3"><label>3</label><institution>Tyndall Centre for Climate Change Research, School of Environmental Sciences, University of East Anglia, Norwich Research Park, Norwich NR4 7TJ, UK</institution>
        </aff>
        <aff id="aff4"><label>4</label><institution>CICERO Center for International Climate Research, Oslo 0349, Norway</institution>
        </aff>
        <aff id="aff5"><label>5</label><institution>School of Environmental Sciences, University of East Anglia, Norwich Research Park, Norwich NR4 7TJ, UK</institution>
        </aff>
        <aff id="aff6"><label>6</label><institution>Alfred-Wegener-Institut, Helmholtz-Zentrum für Polar- und Meeresforschung, Am Handelshafen 12,<?xmltex \hack{\break}?> 27570 Bremerhaven, Germany </institution>
        </aff>
        <aff id="aff7"><label>7</label><institution>Wageningen University, Environmental Sciences Group, P.O. Box 47, 6700AA, Wageningen, the Netherlands</institution>
        </aff>
        <aff id="aff8"><label>8</label><institution>University of Groningen, Centre for Isotope Research, Groningen, the Netherlands</institution>
        </aff>
        <aff id="aff9"><label>9</label><institution>Ludwig-Maximilians-Universität München, Luisenstr. 37, 80333 München, Germany</institution>
        </aff>
        <aff id="aff10"><label>10</label><institution>Max Planck Institute for Meteorology, Bundesstr. 53, 20146 Hamburg, Germany</institution>
        </aff>
        <aff id="aff11"><label>11</label><institution>College of Life and Environmental Sciences, University of Exeter, Exeter EX4 4RJ, UK</institution>
        </aff>
        <aff id="aff12"><label>12</label><institution>CSIRO Oceans and Atmosphere, Canberra, ACT 2101, Australia</institution>
        </aff>
        <aff id="aff13"><label>13</label><institution>Laboratoire des Sciences du Climat et de l’Environnement, LSCE/IPSL, CEA-CNRS-UVSQ, <?xmltex \hack{\break}?> Université Paris-Saclay,  91198 Gif-sur-Yvette, France</institution>
        </aff>
        <aff id="aff14"><label>14</label><institution>Department of Earth System Science, Woods Institute for the Environment, and Precourt Institute for Energy, Stanford University, Stanford, CA 94305–2210, USA</institution>
        </aff>
        <aff id="aff15"><label>15</label><institution>National Oceanic &amp; Atmospheric Administration, Pacific Marine Environmental Laboratory (NOAA/PMEL), 7600 Sand Point Way NE, Seattle, WA 98115, USA</institution>
        </aff>
        <aff id="aff16"><label>16</label><institution>Karlsruhe Institute of Technology, Institute of Meteorology and Climate Research/Atmospheric Environmental Research, 82467 Garmisch-Partenkirchen, Germany</institution>
        </aff>
        <aff id="aff17"><label>17</label><institution>Bermuda Institute of Ocean Sciences (BIOS), 17 Biological Lane, Ferry Reach, St. Georges, GEO1, Bermuda</institution>
        </aff>
        <aff id="aff18"><label>18</label><institution>Geophysical Institute, University of Bergen, Bergen, Norway</institution>
        </aff>
        <aff id="aff19"><label>19</label><institution>Bjerknes Centre for Climate Research, Bergen, Norway</institution>
        </aff>
        <aff id="aff20"><label>20</label><institution>Department of Meteorology, University of Reading, Reading, UK</institution>
        </aff>
        <aff id="aff21"><label>21</label><institution>Department of Geographical Sciences, University of Maryland, College Park, MD 20742, USA</institution>
        </aff>
        <aff id="aff22"><label>22</label><institution>Marine Institute, Galway, Ireland </institution>
        </aff>
        <aff id="aff23"><label>23</label><institution>NIWA, Union Place West, Dunedin, New Zealand</institution>
        </aff>
        <aff id="aff24"><label>24</label><institution>CNRM, Université de Toulouse, Météo-France, CNRS, Toulouse, France</institution>
        </aff>
        <aff id="aff25"><label>25</label><institution>Department of Oceanography, University of Cape Town, Cape Town, 7701, South Africa</institution>
        </aff>
        <aff id="aff26"><label>26</label><institution>SOCCO, Council for Scientific and Industrial Research, Cape Town, 7700, South Africa</institution>
        </aff>
        <aff id="aff27"><label>27</label><institution>Department of Earth System Science, Tsinghua University, Beijing, China</institution>
        </aff>
        <aff id="aff28"><label>28</label><institution>Hakai Institute, Heriot Bay, BC, Canada</institution>
        </aff>
        <aff id="aff29"><label>29</label><institution>National Centre for Earth Observation, University of Edinburgh, Edinburgh, UK </institution>
        </aff>
        <aff id="aff30"><label>30</label><institution>International Institute for Applied Systems Analysis (IIASA), Schlossplatz 1
2361 Laxenburg, Austria</institution>
        </aff>
        <aff id="aff31"><label>31</label><institution>North Carolina School for Science and Mathematics, Durham, NC, USA</institution>
        </aff>
        <aff id="aff32"><label>32</label><institution>Flanders Marine Institute (VLIZ), InnovOceanSite, Wandelaarkaai 7, 8400 Ostend, Belgium</institution>
        </aff>
        <aff id="aff33"><label>33</label><institution>European Commission, Joint Research Centre, 21027 Ispra (VA), Italy</institution>
        </aff>
        <aff id="aff34"><label>34</label><institution>Environmental Physics Group, ETH Zürich, Institute of Biogeochemistry and Pollutant Dynamics and Center for Climate Systems Modeling (C2SM), 8092 Zurich, Switzerland</institution>
        </aff>
        <aff id="aff35"><label>35</label><institution>NCAS-Climate, Climatic Research Unit, School of Environmental Sciences, University of East Anglia, Norwich Research Park, Norwich, NR4 7TJ, UK</institution>
        </aff>
        <aff id="aff36"><label>36</label><institution>Woodwell Climate Research Center, Falmouth, MA 02540, USA</institution>
        </aff>
        <aff id="aff37"><label>37</label><institution>Atmosphere and Ocean Department, Japan Meteorological Agency, Minato-Ku, Tokyo 105-8431, Japan</institution>
        </aff>
        <aff id="aff38"><label>38</label><institution>Department of Atmospheric Sciences, University of Illinois, Urbana, IL 61821, USA</institution>
        </aff>
        <aff id="aff39"><label>39</label><institution>Institute of Applied Energy (IAE), Minato-ku, Tokyo 105-0003, Japan</institution>
        </aff>
        <aff id="aff40"><label>40</label><institution>National Center for Atmospheric Research, Climate and Global Dynamics, <?xmltex \hack{\break}?> Terrestrial Sciences Section, Boulder, CO 80305, USA</institution>
        </aff>
        <aff id="aff41"><label>41</label><institution>Utrecht University, Faculty of Geosciences, Department IMEW, Copernicus Institute of Sustainable Development, Heidelberglaan 2, P.O. Box 80115, 3508 TC, Utrecht, the Netherlands</institution>
        </aff>
        <aff id="aff42"><label>42</label><institution>Hawkesbury Institute for the Environment, Western Sydney University, Penrith, New South Wales, Australia</institution>
        </aff>
        <aff id="aff43"><label>43</label><institution>GEOMAR Helmholtz Centre for Ocean Research Kiel, Düsternbrooker Weg 20, 24105 Kiel, Germany</institution>
        </aff>
        <aff id="aff44"><label>44</label><institution>NORCE Norwegian Research Centre, Jahnebakken 5, 5007 Bergen, Norway</institution>
        </aff>
        <aff id="aff45"><label>45</label><institution>LOCEAN/IPSL laboratory, Sorbonne Université, CNRS/IRD/MNHN, Paris, France</institution>
        </aff>
        <aff id="aff46"><label>46</label><institution>Climate and Environmental Physics, Physics Institute and Oeschger Centre for Climate Change Research, University of Bern, Bern, Switzerland</institution>
        </aff>
        <aff id="aff47"><label>47</label><institution>Jet Propulsion Laboratory, California Institute of Technology, Pasadena, CA, USA</institution>
        </aff>
        <aff id="aff48"><label>48</label><institution>Research Institute for Environment, Energy, and Economics, Appalachian State University,<?xmltex \hack{\break}?>  Boone, NC, USA</institution>
        </aff>
        <aff id="aff49"><label>49</label><institution>Department of Geological and Environmental Sciences, Appalachian State University, <?xmltex \hack{\break}?> Boone, NC, USA</institution>
        </aff>
        <aff id="aff50"><label>50</label><institution>Department of Meteorology, Department of Geography &amp; Environmental Science,<?xmltex \hack{\break}?>  National Centre for Atmospheric Science, University of Reading, Reading, UK</institution>
        </aff>
        <aff id="aff51"><label>51</label><institution>Climate Research Division, Environment and Climate Change Canada, Victoria, BC, Canada</institution>
        </aff>
        <aff id="aff52"><label>52</label><institution>Cooperative Institute for Research in Environmental Sciences, University of Colorado,<?xmltex \hack{\break}?> Boulder, CO 80305, USA</institution>
        </aff>
        <aff id="aff53"><label>53</label><institution>National Oceanic &amp; Atmospheric Administration/Global Monitoring Laboratory (NOAA/GML),<?xmltex \hack{\break}?>  Boulder, CO 80305, USA</institution>
        </aff>
        <aff id="aff54"><label>54</label><institution>Max Planck Institute for Biogeochemistry, Jena, Germany</institution>
        </aff>
        <aff id="aff55"><label>55</label><institution>Earth System Division, National Institute for Environmental Studies, 16-2 Onogawa,<?xmltex \hack{\break}?> Tsukuba, Ibaraki, 305-8506, Japan</institution>
        </aff>
        <aff id="aff56"><label>56</label><institution>Meteorological Research Institute, 1-1 Nagamine, Tsukuba, Ibaraki, 305-0052, Japan</institution>
        </aff>
        <aff id="aff57"><label>57</label><institution>Japan Fisheries Research and Education Agency, 2-12-4 Fukuura, Kanazawa-Ku, Yokohama 236-8648, Japan</institution>
        </aff>
        <aff id="aff58"><label>58</label><institution>National Oceanic &amp; Atmospheric Administration/Atlantic Oceanographic <?xmltex \hack{\break}?>&amp; Meteorological Laboratory (NOAA/AOML), Miami, FL 33149, USA</institution>
        </aff>
        <aff id="aff59"><label>59</label><institution>NASA Goddard Space Flight Center, Biospheric Sciences Laboratory, Greenbelt, MD 20771, USA</institution>
        </aff>
        <aff id="aff60"><label>60</label><institution>Leibniz Institute for Baltic Sea Research Warnemuende (IOW), Seestrasse 15, 18119 Rostock, Germany</institution>
        </aff>
        <aff id="aff61"><label>61</label><institution>Princeton University, Department of Geosciences and Princeton Environmental Institute, Princeton, NJ, USA</institution>
        </aff>
        <aff id="aff62"><label>62</label><institution>Met Office Hadley Centre, FitzRoy Road, Exeter EX1 3PB, UK</institution>
        </aff>
        <aff id="aff63"><label>63</label><institution>National Oceanic and Atmospheric Administration, Earth System Research Laboratory (NOAA ESRL), Boulder, CO 80305, USA</institution>
        </aff>
        <aff id="aff64"><label>64</label><institution>School of Forestry and Wildlife Sciences, Auburn University, 602 Ducan Drive, Auburn, AL 36849, USA</institution>
        </aff>
        <aff id="aff65"><label>65</label><institution>CSIRO Oceans and Atmosphere, P.O. Box 1538, Hobart, Tasmania 7001, Australia</institution>
        </aff>
        <aff id="aff66"><label>66</label><institution>Australian Antarctic Partnership Program, University of Tasmania, Hobart, Australia</institution>
        </aff>
        <aff id="aff67"><label>67</label><institution>Statistics Division, Food and Agriculture Organization of the United Nations, <?xmltex \hack{\break}?>Via Terme di Caracalla, Rome 00153, Italy</institution>
        </aff>
        <aff id="aff68"><label>68</label><institution>Faculty of Earth and Life Sciences, VU University, Amsterdam, the Netherlands</institution>
        </aff>
        <aff id="aff69"><label>69</label><institution>School of Atmospheric Sciences, Sun Yat-sen University, Zhuhai, Guangdong 510245, China</institution>
        </aff>
        <aff id="aff70"><label>70</label><institution>School of Environmental Science and Engineering, Nanjing University of Information Science and Technology (NUIST), Nanjing, China</institution>
        </aff>
      </contrib-group>
      <author-notes><corresp id="corr1">Pierre Friedlingstein (p.friedlingstein@exeter.ac.uk)</corresp></author-notes><pub-date><day>26</day><month>April</month><year>2022</year></pub-date>
      
      <volume>14</volume>
      <issue>4</issue>
      <fpage>1917</fpage><lpage>2005</lpage>
      <history>
        <date date-type="received"><day>28</day><month>October</month><year>2021</year></date>
           <date date-type="rev-request"><day>4</day><month>November</month><year>2021</year></date>
           <date date-type="rev-recd"><day>15</day><month>March</month><year>2022</year></date>
           <date date-type="accepted"><day>15</day><month>March</month><year>2022</year></date>
      </history>
      <permissions>
        <copyright-statement>Copyright: © 2022 Pierre Friedlingstein et al.</copyright-statement>
        <copyright-year>2022</copyright-year>
      <license license-type="open-access"><license-p>This work is licensed under the Creative Commons Attribution 4.0 International License. To view a copy of this licence, visit <ext-link ext-link-type="uri" xlink:href="https://creativecommons.org/licenses/by/4.0/">https://creativecommons.org/licenses/by/4.0/</ext-link></license-p></license></permissions><self-uri xlink:href="https://essd.copernicus.org/articles/essd-14-1917-2022.html">This article is available from https://essd.copernicus.org/articles/essd-14-1917-2022.html</self-uri><self-uri xlink:href="https://essd.copernicus.org/articles/essd-14-1917-2022.pdf">The full text article is available as a PDF file from https://essd.copernicus.org/articles/essd-14-1917-2022.pdf</self-uri>
      <abstract><title>Abstract</title>

      <p id="d1e1444">Accurate assessment of anthropogenic carbon dioxide (CO<inline-formula><mml:math id="M1" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) emissions and
their redistribution among the atmosphere, ocean, and terrestrial biosphere
in a changing climate is critical to better understand the global carbon
cycle, support the development of climate policies, and project future
climate change. Here we describe and synthesize datasets and methodology to
quantify the five major components of the global carbon budget and their
uncertainties. Fossil CO<inline-formula><mml:math id="M2" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (<inline-formula><mml:math id="M3" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) are based on energy
statistics and cement production data, while emissions from land-use change
(<inline-formula><mml:math id="M4" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), mainly deforestation, are based on land use and land-use change
data and bookkeeping models. Atmospheric CO<inline-formula><mml:math id="M5" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration is measured
directly, and its growth rate (<inline-formula><mml:math id="M6" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is computed from the annual
changes in concentration. The ocean CO<inline-formula><mml:math id="M7" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M8" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is estimated
with global ocean biogeochemistry models and observation-based
data products. The terrestrial CO<inline-formula><mml:math id="M9" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M10" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is estimated with
dynamic global vegetation models. The resulting carbon budget imbalance
(<inline-formula><mml:math id="M11" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), the difference between the estimated total emissions and the
estimated changes in the atmosphere, ocean, and terrestrial biosphere, is a
measure of imperfect data and understanding of the contemporary carbon
cycle. All uncertainties are reported as <inline-formula><mml:math id="M12" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M13" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>. For the first
time, an approach is shown to reconcile the difference in our <inline-formula><mml:math id="M14" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
estimate with the one from national greenhouse gas inventories, supporting
the assessment of collective countries' climate progress.</p>

      <p id="d1e1585">For the year 2020, <inline-formula><mml:math id="M15" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> declined by 5.4 % relative to 2019, with
fossil emissions at 9.5 <inline-formula><mml:math id="M16" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M17" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (9.3 <inline-formula><mml:math id="M18" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M19" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> when the cement carbonation sink is included), and <inline-formula><mml:math id="M20" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> was 0.9 <inline-formula><mml:math id="M21" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M22" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, for a total anthropogenic CO<inline-formula><mml:math id="M23" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emission of
10.2 <inline-formula><mml:math id="M24" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8 GtC yr<inline-formula><mml:math id="M25" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (37.4 <inline-formula><mml:math id="M26" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 2.9 GtCO<inline-formula><mml:math id="M27" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>). Also, for
2020, <inline-formula><mml:math id="M28" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> was 5.0 <inline-formula><mml:math id="M29" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2 GtC yr<inline-formula><mml:math id="M30" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (2.4 <inline-formula><mml:math id="M31" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.1 ppm yr<inline-formula><mml:math id="M32" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), <inline-formula><mml:math id="M33" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> was 3.0 <inline-formula><mml:math id="M34" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M35" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, and <inline-formula><mml:math id="M36" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
was 2.9 <inline-formula><mml:math id="M37" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1 GtC yr<inline-formula><mml:math id="M38" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, with a <inline-formula><mml:math id="M39" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of <inline-formula><mml:math id="M40" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.8 GtC yr<inline-formula><mml:math id="M41" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The
global atmospheric CO<inline-formula><mml:math id="M42" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration averaged over 2020 reached 412.45 <inline-formula><mml:math id="M43" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.1 ppm. Preliminary data for 2021 suggest a rebound in <inline-formula><mml:math id="M44" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
relative to 2020 of <inline-formula><mml:math id="M45" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.8 % (4.2 % to 5.4 %) globally.</p>

      <p id="d1e1889">Overall, the mean and trend in the components of the global carbon budget
are consistently estimated over the period 1959–2020, but discrepancies of
up to 1 GtC yr<inline-formula><mml:math id="M46" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> persist for the representation of annual to
semi-decadal variability in CO<inline-formula><mml:math id="M47" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes. Comparison of estimates from
multiple approaches and observations shows (1) a persistent large
uncertainty in the estimate of land-use changes emissions, (2) a low
agreement between the different methods on the magnitude of the land
CO<inline-formula><mml:math id="M48" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux in the northern extra-tropics, and (3) a discrepancy between
the different methods on the strength of the ocean sink over the last
decade. This living data update documents changes in the methods and datasets used in this new global carbon budget and the progress in understanding
of the global carbon cycle compared with previous publications of this dataset (Friedlingstein et al., 2020, 2019; Le
Quéré et al., 2018b, a, 2016, 2015b, a, 2014, 2013). The
data presented in this work are available at <ext-link xlink:href="https://doi.org/10.18160/gcp-2021" ext-link-type="DOI">10.18160/gcp-2021</ext-link> (Friedlingstein et al., 2021).</p>
  </abstract>
    </article-meta>
  </front>
<body>
      

<sec id="Ch1.Sx1" specific-use="unnumbered">
  <title>Executive summary</title>
      <p id="d1e1932">Global fossil CO<inline-formula><mml:math id="M49" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (excluding cement carbonation) in 2021 are
returning towards their 2019 levels after decreasing 5.4 % in 2020. The
2020 decrease was 0.52 GtC yr<inline-formula><mml:math id="M50" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (1.9 GtCO<inline-formula><mml:math id="M51" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M52" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), bringing
2020 emissions to 9.5 <inline-formula><mml:math id="M53" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M54" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (34.8 <inline-formula><mml:math id="M55" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1.8 GtCO<inline-formula><mml:math id="M56" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M57" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), comparable to the emissions level of 2012. Preliminary estimates
based on data available in March 2022 suggest fossil CO<inline-formula><mml:math id="M58" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
rebounded 4.8 % in 2021 (4.2 % to 5.4 %), bringing emissions to 9.9 GtC yr<inline-formula><mml:math id="M59" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (36.4 GtCO<inline-formula><mml:math id="M60" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M61" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), back to about the same level as
in 2019 (10.0 <inline-formula><mml:math id="M62" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M63" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 36.7 <inline-formula><mml:math id="M64" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1.8 GtCO<inline-formula><mml:math id="M65" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M66" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). Emissions from coal and gas in 2021 are expected to have
rebounded above 2019 levels, while emissions from oil were still below their
2019 level. Emissions are expected to have been 5.7 % higher in 2021 than
in 2019 in China, reaching 3.0 GtC (11.1 GtCO<inline-formula><mml:math id="M67" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>), and also higher in
India with a 3.2 % increase in 2021 relative to 2019, reaching 0.74 GtC
(2.7 GtCO<inline-formula><mml:math id="M68" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>). In contrast, projected 2021 emissions in the United States
(1.4 GtC, 5.0 GtCO<inline-formula><mml:math id="M69" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>), European Union (0.8 GtC, 2.8 GtCO<inline-formula><mml:math id="M70" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>), and the
rest of the world (4.0 GtC, 14.8 GtCO<inline-formula><mml:math id="M71" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, in aggregate) remained
respectively 4.5 %, 5.3 %, and 4.0 % below their 2019 levels. These
changes in 2021 emissions reflect the stringency of the COVID-19 confinement
levels in 2020 and the pre-covid background trends in emissions in these
countries.</p>
      <p id="d1e2161">Fossil CO<inline-formula><mml:math id="M72" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions significantly decreased in 23 countries during the
decade 2010–2019. Altogether, these 23 countries contribute to about 2.5 GtC yr<inline-formula><mml:math id="M73" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> fossil fuel CO<inline-formula><mml:math id="M74" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions over the last decade, only about
one-quarter of world CO<inline-formula><mml:math id="M75" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fossil emissions.</p>
      <p id="d1e2203">Global CO<inline-formula><mml:math id="M76" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from land use, land-use change, and forestry (LUC)
converge based on revised data of land-use change and show a small decrease
over the past two decades. Near-constant gross emissions estimated at 3.8 <inline-formula><mml:math id="M77" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6 GtC yr<inline-formula><mml:math id="M78" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the 2011–2020 decade are only partly offset by
growing carbon removals on managed land of 2.7 <inline-formula><mml:math id="M79" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M80" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>,
resulting in the net emissions in managed land of 1.1 <inline-formula><mml:math id="M81" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M82" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (4.1 <inline-formula><mml:math id="M83" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 2.6 GtCO<inline-formula><mml:math id="M84" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M85" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). These net emissions decreased
by 0.2 GtC in 2020 compared to 2019 levels, with large uncertainty.
Preliminary estimates for emissions in 2021 suggest a 0.1 GtC decrease for
2021, giving net emissions of 0.8 GtC yr<inline-formula><mml:math id="M86" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (2.9 GtCO<inline-formula><mml:math id="M87" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M88" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). The
small decrease in net LUC emissions amidst large uncertainty prohibits
robust conclusions concerning trend changes of total anthropogenic
emissions. For the first time, we link the global carbon budget models'
estimates to the official country reporting of national greenhouse gases
inventories. While the global carbon budget distinguishes anthropogenic from
natural drivers of land carbon fluxes, country reporting is area-based and
attributes part of the natural terrestrial sink on managed land to the
land-use sector. Accounting for this redistribution, the two approaches are
shown to be consistent with each other.
<?xmltex \hack{\newpage}?>
The remaining carbon budget for a 50 % likelihood to limit global warming
to 1.5, 1.7, and 2 <inline-formula><mml:math id="M89" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C has respectively
reduced to 120 GtC (420 GtCO<inline-formula><mml:math id="M90" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>), 210 GtC (770 GtCO<inline-formula><mml:math id="M91" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) and 350 GtC
(1270 GtCO<inline-formula><mml:math id="M92" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) from the beginning of 2022, equivalent to 11, 20, and 32 years, assuming 2021 emissions levels. Total anthropogenic emissions were
10.4 GtC yr<inline-formula><mml:math id="M93" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (38.0 GtCO<inline-formula><mml:math id="M94" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M95" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) in 2020, with a preliminary
estimate of 10.7 GtC yr<inline-formula><mml:math id="M96" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (39.3 GtCO<inline-formula><mml:math id="M97" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M98" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) for 2021. The
remaining carbon budget to keep global temperatures below these climate
targets has shrunk by 21 GtC (77 GtCO<inline-formula><mml:math id="M99" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) since the release of the IPCC
AR6 Working Group 1 assessment. Reaching zero CO<inline-formula><mml:math id="M100" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions by 2050
entails cutting total anthropogenic CO<inline-formula><mml:math id="M101" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions by about 0.4 GtC (1.4 GtCO<inline-formula><mml:math id="M102" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) each year on average, comparable to the decrease during 2020,
highlighting the scale of the action needed.</p>
      <p id="d1e2477">The concentration of CO<inline-formula><mml:math id="M103" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> in the atmosphere is set to reach 414.7 ppm in
2021, 50 % above pre-industrial levels. The atmospheric CO<inline-formula><mml:math id="M104" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth
was 5.1 <inline-formula><mml:math id="M105" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.02 GtC yr<inline-formula><mml:math id="M106" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during the decade 2011–2020 (47 % of
total CO<inline-formula><mml:math id="M107" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions) with a preliminary 2021 growth rate estimate of
around 5 GtC yr<inline-formula><mml:math id="M108" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p>
      <p id="d1e2540">The ocean CO<inline-formula><mml:math id="M109" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink resumed a more rapid growth in the past decade after
low or no growth during the 1991–2002 period. However, the growth of the
ocean CO<inline-formula><mml:math id="M110" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink in the past decade has an uncertainty of a factor of
3, with estimates based on data products and estimates based on models
showing an ocean sink increase of 0.9 and 0.3 GtC yr<inline-formula><mml:math id="M111" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> since 2010, respectively. The discrepancy in the trend originates from all
latitudes but is largest in the Southern Ocean. The ocean CO<inline-formula><mml:math id="M112" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink was
2.8 <inline-formula><mml:math id="M113" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M114" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during the decade 2011–2020 (26 % of total
CO<inline-formula><mml:math id="M115" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions), with a preliminary 2021 estimate of around 2.9 GtC yr<inline-formula><mml:math id="M116" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p>
      <p id="d1e2623">The land CO<inline-formula><mml:math id="M117" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink continued to increase during the 2011–2020 period
primarily in response to increased atmospheric CO<inline-formula><mml:math id="M118" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, albeit with large
interannual variability. The land CO<inline-formula><mml:math id="M119" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink was 3.1 <inline-formula><mml:math id="M120" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6 GtC yr<inline-formula><mml:math id="M121" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during the 2011–2020 decade (29 % of total CO<inline-formula><mml:math id="M122" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions),
0.5 GtC yr<inline-formula><mml:math id="M123" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> larger than during the previous decade (2000–2009), with a
preliminary 2021 estimate of around 3.3 GtC yr<inline-formula><mml:math id="M124" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. Year-to-year
variability in the land sink is about 1 GtC yr<inline-formula><mml:math id="M125" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, making small annual
changes in anthropogenic emissions hard to detect in global atmospheric
CO<inline-formula><mml:math id="M126" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration.</p>
</sec>
<sec id="Ch1.S1" sec-type="intro">
  <label>1</label><title>Introduction</title>
      <p id="d1e2735">The concentration of carbon dioxide (CO<inline-formula><mml:math id="M127" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) in the atmosphere has
increased from approximately 277 parts per million (ppm) in 1750 (Joos and
Spahni, 2008), the beginning of the industrial era, to 412.4 <inline-formula><mml:math id="M128" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.1 ppm
in 2020 (Dlugokencky and Tans, 2022; Fig. 1). The atmospheric CO<inline-formula><mml:math id="M129" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
increase above pre-industrial levels was, initially, primarily caused by the
release of carbon to the atmosphere from deforestation and other land-use
change activities (Canadell et al., 2022). While emissions from fossil fuels
started before the Industrial Era, they became the dominant source of
anthropogenic emissions to the atmosphere from around 1950 and their
relative share has continued to increase until the present. Anthropogenic
emissions occur on top of an active natural carbon cycle that circulates
carbon between the reservoirs of the atmosphere, ocean, and terrestrial
biosphere on timescales from sub-daily to millennial, while exchanges with
geologic reservoirs occur on longer timescales (Archer et al., 2009).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F1"><?xmltex \currentcnt{1}?><?xmltex \def\figurename{Figure}?><label>Figure 1</label><caption><p id="d1e2765">Surface average atmospheric CO<inline-formula><mml:math id="M130" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration (ppm). Since
1980, monthly data are from NOAA/ESRL (Dlugokencky and Tans, 2022) and are
based on an average of direct atmospheric CO<inline-formula><mml:math id="M131" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements from
multiple stations in the marine boundary layer (Masarie and Tans, 1995). The
1958–1979 monthly data are from the Scripps Institution of Oceanography,
based on an average of direct atmospheric CO<inline-formula><mml:math id="M132" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements from the
Mauna Loa and South Pole stations (Keeling et al., 1976). To account for the
difference of mean CO<inline-formula><mml:math id="M133" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and seasonality between the NOAA/ESRL and the
Scripps station networks used here, the Scripps surface average (from two
stations) was de-seasonalized and adjusted to match the NOAA/ESRL surface
average (from multiple stations) by adding the mean difference of 0.667 ppm,
calculated here from overlapping data during 1980–2012.</p></caption>
        <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f01.png"/>

      </fig>

      <p id="d1e2810">The global carbon budget (GCB) presented here refers to the mean,
variations, and trends in the perturbation of CO<inline-formula><mml:math id="M134" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> in the environment,
referenced to the beginning of the Industrial Era (defined here as 1750).
This paper describes the components of the global carbon cycle over the
historical period with a stronger focus on the recent period (since 1958,
onset of atmospheric CO<inline-formula><mml:math id="M135" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements), the last decade (2011–2020),
the last year (2020), and the current year (2021). We quantify the input of
CO<inline-formula><mml:math id="M136" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> to the atmosphere by emissions from human activities, the growth
rate of atmospheric CO<inline-formula><mml:math id="M137" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration, and the resulting changes in the
storage of carbon in the land and ocean reservoirs in response to increasing
atmospheric CO<inline-formula><mml:math id="M138" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> levels, climate change and variability, and other
anthropogenic and natural changes (Fig. 2). An understanding of this
perturbation budget over time and the underlying variability and trends of
the natural carbon cycle is necessary to understand the response of natural
sinks to changes in climate, CO<inline-formula><mml:math id="M139" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, and land-use change drivers, and to
quantify emissions compatible with a given climate stabilization target.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F2" specific-use="star"><?xmltex \currentcnt{2}?><?xmltex \def\figurename{Figure}?><label>Figure 2</label><caption><p id="d1e2871">Schematic representation of the overall perturbation of the global carbon cycle caused by anthropogenic activities, averaged globally for the decade 2011–2020. See legends for the corresponding arrows and units. The uncertainty in the atmospheric CO<inline-formula><mml:math id="M140" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth rate is very small (<inline-formula><mml:math id="M141" display="inline"><mml:mo lspace="0mm">±</mml:mo></mml:math></inline-formula>0.02 GtC yr<inline-formula><mml:math id="M142" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and is neglected for the figure. The anthropogenic perturbation occurs on top of an active carbon cycle, with fluxes and stocks represented in the background and taken from Canadell et al. (2022) for all numbers, except for the carbon stocks in coasts which is from a literature review of coastal marine sediments (Price and Warren, 2016). </p></caption>
        <?xmltex \igopts{width=412.564961pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f02.png"/>

      </fig>

      <p id="d1e2908">The components of the CO<inline-formula><mml:math id="M143" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> budget that are reported annually in this
paper include separate and independent estimates for the CO<inline-formula><mml:math id="M144" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
from (1) fossil fuel combustion and oxidation from all energy and industrial
processes, also including cement production and carbonation (<inline-formula><mml:math id="M145" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; GtC yr<inline-formula><mml:math id="M146" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>); (2) the emissions resulting from deliberate human activities
on land, including those leading to land-use change (<inline-formula><mml:math id="M147" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; GtC yr<inline-formula><mml:math id="M148" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>); and their partitioning among (3) the growth rate of atmospheric
CO<inline-formula><mml:math id="M149" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration (<inline-formula><mml:math id="M150" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; GtC yr<inline-formula><mml:math id="M151" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), and the uptake of
CO<inline-formula><mml:math id="M152" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (the “CO<inline-formula><mml:math id="M153" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sinks”) in (4) the ocean (<inline-formula><mml:math id="M154" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; GtC yr<inline-formula><mml:math id="M155" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and (5) on land (<inline-formula><mml:math id="M156" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; GtC yr<inline-formula><mml:math id="M157" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). The CO<inline-formula><mml:math id="M158" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sinks
as defined here conceptually include the response of the land (including
inland waters and estuaries) and ocean (including coasts and territorial
seas) to elevated CO<inline-formula><mml:math id="M159" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and changes in climate and other environmental
conditions, although in practice not all processes are fully accounted for
(see Sect. 2.7). Global emissions and their partitioning among the
atmosphere, ocean, and land are in reality in balance. Due to the combination
of imperfect spatial and/or temporal data coverage, errors in each estimate,
and smaller terms not included in our budget estimate (discussed in Sect. 2.7), the independent estimates (1) to (5) above do not necessarily add up
to zero. We therefore (a) additionally assess a set of global atmospheric
inverse model results that by design close the global carbon balance (see
Sect. 2.6), and (b) estimate a budget imbalance (<inline-formula><mml:math id="M160" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), which is a
measure of the mismatch between the estimated emissions and the estimated
changes in the atmosphere, land, and ocean, as follows:
          <disp-formula id="Ch1.E1" content-type="numbered"><label>1</label><mml:math id="M161" display="block"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:mo>(</mml:mo><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
        <inline-formula><mml:math id="M162" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is usually reported in ppm yr<inline-formula><mml:math id="M163" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, which we convert to units of
carbon mass per year, GtC yr<inline-formula><mml:math id="M164" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, using 1 ppm <inline-formula><mml:math id="M165" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 2.124 GtC (Ballantyne
et al., 2012; Table 1). All quantities are presented in units of gigatonnes
of carbon (GtC, 10<inline-formula><mml:math id="M166" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">15</mml:mn></mml:msup></mml:math></inline-formula> gC), which is the same as petagrammes of carbon
(PgC; Table 1). Units of gigatonnes of CO<inline-formula><mml:math id="M167" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (or billion tonnes of
CO<inline-formula><mml:math id="M168" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) used in policy are equal to 3.664 multiplied by the value in units
of GtC.</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T1" specific-use="star"><?xmltex \currentcnt{1}?><label>Table 1</label><caption><p id="d1e3229">Factors used to convert carbon in various units (by convention, Unit 1 <inline-formula><mml:math id="M169" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> Unit <inline-formula><mml:math id="M170" display="inline"><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mo>×</mml:mo></mml:mrow></mml:math></inline-formula> conversion).</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="4">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Unit 1</oasis:entry>
         <oasis:entry colname="col2">Unit 2</oasis:entry>
         <oasis:entry colname="col3">Conversion</oasis:entry>
         <oasis:entry colname="col4">Source</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">GtC (gigatonnes of carbon)</oasis:entry>
         <oasis:entry colname="col2">ppm (parts per million)<inline-formula><mml:math id="M176" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">2.124<inline-formula><mml:math id="M177" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4">Ballantyne et al. (2012)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GtC (gigatonnes of carbon)</oasis:entry>
         <oasis:entry colname="col2">PgC (petagrammes of carbon)</oasis:entry>
         <oasis:entry colname="col3">1</oasis:entry>
         <oasis:entry colname="col4">SI unit conversion</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GtCO<inline-formula><mml:math id="M178" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (gigatonnes of carbon dioxide)</oasis:entry>
         <oasis:entry colname="col2">GtC (gigatonnes of carbon)</oasis:entry>
         <oasis:entry colname="col3">3.664</oasis:entry>
         <oasis:entry colname="col4">44.01/12.011 in mass equivalent</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GtC (gigatonnes of carbon)</oasis:entry>
         <oasis:entry colname="col2">MtC (megatonnes of carbon)</oasis:entry>
         <oasis:entry colname="col3">1000</oasis:entry>
         <oasis:entry colname="col4">SI unit conversion</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table><table-wrap-foot><p id="d1e3249"><inline-formula><mml:math id="M171" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula> Measurements of atmospheric CO<inline-formula><mml:math id="M172" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration have units of dry-air mole fraction; “ppm” is an abbreviation for micromole per mole of dry air. <inline-formula><mml:math id="M173" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> The use of a factor of 2.124 assumes that all the atmosphere is well mixed within 1 year. In reality, only the troposphere is well mixed, and the growth rate of CO<inline-formula><mml:math id="M174" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration in the less well-mixed stratosphere is not measured by sites from the NOAA network. Using a factor of 2.124 makes the approximation that the growth rate of CO<inline-formula><mml:math id="M175" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration in the stratosphere is equal to that of the troposphere on a yearly basis.</p></table-wrap-foot></table-wrap>

      <p id="d1e3416">We also include a quantification of <inline-formula><mml:math id="M179" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> by country, computed with both
territorial and consumption-based accounting (see Sect. 2), and discuss
missing terms from sources other than the combustion of fossil fuels (see
Sect. 2.7).</p>
      <p id="d1e3430">The global CO<inline-formula><mml:math id="M180" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> budget has been assessed by the Intergovernmental Panel
on Climate Change (IPCC) in all assessment reports (Prentice et al., 2001;
Schimel et al., 1995; Watson et al., 1990; Denman et al., 2007; Ciais et
al., 2013; Canadell et al., 2022), and by others (e.g. Ballantyne et al.,
2012). The Global Carbon Project (GCP, <uri>https://www.globalcarbonproject.org</uri>, last
access: 11 March 2022) has coordinated this cooperative community effort for
the annual publication of global carbon budgets for the year 2005 (Raupach
et al., 2007; including fossil emissions only), year 2006 (Canadell et al.,
2007), year 2007 (GCP, 2007), year 2008 (Le Quéré et al., 2009),
year 2009 (Friedlingstein et al., 2010), year 2010 (Peters et al., 2012b),
year 2012 (Le Quéré et al., 2013; Peters et al., 2013), year 2013
(Le Quéré et al., 2014), year 2014 (Le Quéré et al., 2015a;
Friedlingstein et al., 2014), year 2015 (Jackson et al., 2016; Le
Quéré et al., 2015b), year 2016 (Le Quéré et al., 2016),
year 2017 (Le Quéré et al., 2018a; Peters et al., 2017), year 2018
(Le Quéré et al., 2018b; Jackson et al., 2018), year 2019
(Friedlingstein et al., 2019; Jackson et al., 2019; Peters et al., 2020), and
more recently the year 2020 (Friedlingstein et al., 2020; Le Quéré
et al., 2021). Each of these papers updated previous estimates with the
latest available information for the entire time series.</p>
      <p id="d1e3446">We adopt a range of <inline-formula><mml:math id="M181" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1 standard deviation (<inline-formula><mml:math id="M182" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>) to report the
uncertainties in our estimates, representing a likelihood of 68 % that the
true value will be within the provided range if the errors have a Gaussian
distribution, and no bias is assumed. This choice reflects the difficulty of
characterizing the uncertainty in the CO<inline-formula><mml:math id="M183" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes between the atmosphere
and the ocean and land reservoirs individually, particularly on an annual
basis, as well as the difficulty of updating the CO<inline-formula><mml:math id="M184" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from
land-use change. A likelihood of 68 % provides an indication of our
current capability to quantify each term and its uncertainty given the
available information. The uncertainties reported here combine statistical
analysis of the underlying data, assessments of uncertainties in the
generation of the datasets, and expert judgement of the likelihood of
results lying outside this range. The limitations of current information are
discussed in the paper and have been examined in detail elsewhere
(Ballantyne et al., 2015; Zscheischler et al., 2017). We also use a
qualitative assessment of confidence level to characterize the annual
estimates from each term based on the type, amount, quality, and consistency
of the evidence as defined by the IPCC (Stocker et al., 2013).</p>
      <p id="d1e3481">This paper provides a detailed description of the datasets and methodology
used to compute the global carbon budget estimates for the industrial
period, from 1750 to 2020, and in more detail for the period since 1959. It
also provides decadal averages starting in 1960 including the most recent
decade (2011–2020), results for the year 2020, and a projection for the year
2021. Finally, it provides cumulative emissions from fossil fuels and
land-use change since the year 1750, the pre-industrial period; and since
the year 1850, the reference year for historical simulations in IPCC AR6
(Eyring et al., 2016). This paper is updated every year using the format of
“living data” to keep a record of budget versions and the changes in new
data, revision of data, and changes in methodology that lead to changes in
estimates of the carbon budget. Additional materials associated with the
release of each new version will be posted at the Global Carbon Project
(GCP) website (<uri>http://www.globalcarbonproject.org/carbonbudget</uri>, last access:
11 March 2022), with fossil fuel emissions also available through the Global
Carbon Atlas (<uri>http://www.globalcarbonatlas.org</uri>, last access: 11 March 2022).
With this approach, we aim to provide the highest transparency and
traceability in the reporting of CO<inline-formula><mml:math id="M185" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, the key driver of climate change.</p>
</sec>
<sec id="Ch1.S2">
  <label>2</label><title>Methods</title>
      <p id="d1e3507">Multiple organizations and research groups around the world generated the
original measurements and data used to complete the global carbon budget.
The effort presented here is thus mainly one of synthesis, where results
from individual groups are collated, analysed, and evaluated for
consistency. We facilitate access to original data with the understanding
that primary datasets will be referenced in future work (see Table 2 for
how to cite the datasets). Descriptions of the measurements, models, and
methodologies follow below, and detailed descriptions of each component are
provided elsewhere.</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T2" specific-use="star"><?xmltex \currentcnt{2}?><label>Table 2</label><caption><p id="d1e3513">How to cite the individual components of the global carbon budget presented here.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.93}[.93]?><oasis:tgroup cols="2">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Component</oasis:entry>
         <oasis:entry colname="col2">Primary reference</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">Global fossil CO<inline-formula><mml:math id="M186" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (EFOS), total and by fuel type</oasis:entry>
         <oasis:entry colname="col2">Andrew and Peters (2021)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">National territorial fossil CO<inline-formula><mml:math id="M187" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (EFOS)</oasis:entry>
         <oasis:entry colname="col2">Gilfillan and Marland (2021), UNFCCC (2021a)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">National consumption-based fossil CO<inline-formula><mml:math id="M188" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (EFOS) by country (consumption)</oasis:entry>
         <oasis:entry colname="col2">Peters et al. (2011b) updated as described in this paper</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Net land-use change flux (<inline-formula><mml:math id="M189" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">This paper (see Table 4 for individual model references).</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Growth rate in atmospheric CO<inline-formula><mml:math id="M190" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration (GATM)</oasis:entry>
         <oasis:entry colname="col2">Dlugokencky and Tans (2022)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Ocean and land CO<inline-formula><mml:math id="M191" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sinks (<inline-formula><mml:math id="M192" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M193" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">This paper (see Table 4 for individual model references).</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

      <p id="d1e3673">This is the 16th version of the global carbon budget and the 10th revised
version in the format of a living data update in <italic>Earth System Science Data</italic>.
It builds on the latest published global carbon budget of Friedlingstein et
al. (2020). The main changes are as follows: the inclusion of (1) data to year 2020 and
a projection for the global carbon budget for year 2021, (2) a Kaya analysis
to identify the driving factors behind the recent trends in fossil fuel
emissions (changes in population, GDP per person, energy use per GDP, and
CO<inline-formula><mml:math id="M194" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions per unit energy), (3) an estimate of the ocean sink from
models and data products combined, (4) an assessment of the relative
contributions of increased atmospheric CO<inline-formula><mml:math id="M195" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and climate change in
driving the land and ocean sinks, and (5) an assessment of the current
trends in anthropogenic emissions and implications for the remaining carbon
budget for specific climate targets. The main methodological differences
between recent annual carbon budgets (2016–2020) are summarized in Table 3
and previous changes since 2006 are provided in Table A7.</p>

<?xmltex \floatpos{p}?><table-wrap id="Ch1.T3" specific-use="star" orientation="landscape"><?xmltex \currentcnt{3}?><label>Table 3</label><caption><p id="d1e3701">Main methodological changes in the global carbon budget since 2017. Methodological changes introduced in one year are kept for the following years unless noted. Empty cells mean there were no methodological changes introduced that year. Table A7 lists methodological changes from the first global carbon budget publication up to 2016.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.8}[.8]?><oasis:tgroup cols="8">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="3.2cm"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="3.2cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="3.2cm"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="3.2cm"/>
     <oasis:colspec colnum="5" colname="col5" align="justify" colwidth="3.2cm"/>
     <oasis:colspec colnum="6" colname="col6" align="justify" colwidth="3.1cm"/>
     <oasis:colspec colnum="7" colname="col7" align="justify" colwidth="3.1cm"/>
     <oasis:colspec colnum="8" colname="col8" align="justify" colwidth="3.1cm"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Publication year</oasis:entry>
         <oasis:entry rowsep="1" namest="col2" nameend="col3" align="center">Fossil fuel emissions </oasis:entry>
         <oasis:entry colname="col4">LUC emissions</oasis:entry>
         <oasis:entry rowsep="1" namest="col5" nameend="col7" align="center">Reservoirs </oasis:entry>
         <oasis:entry colname="col8">Uncertainty and other <?xmltex \hack{\hfill\break}?>changes</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">Global</oasis:entry>
         <oasis:entry colname="col3">Country (territorial)</oasis:entry>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5">Atmosphere</oasis:entry>
         <oasis:entry colname="col6">Ocean</oasis:entry>
         <oasis:entry colname="col7">Land</oasis:entry>
         <oasis:entry colname="col8"/>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2017</oasis:entry>
         <oasis:entry colname="col2">Projection includes<?xmltex \hack{\hfill\break}?>India-specific data</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Average of two bookkeeping models; use of 12 DGVMs</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">Based on eight models that match the observed sink for the 1990s; no longer normalized</oasis:entry>
         <oasis:entry colname="col7">Based on 15 models that meet observation-based criteria (see Sect. 2.5)</oasis:entry>
         <oasis:entry colname="col8">Land multi-model average now used in main carbon budget, with the carbon imbalance presented separately; new table of key uncertainties</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Le Quéré et al. (2018a) GCB2017</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2018</oasis:entry>
         <oasis:entry colname="col2">Revision in cement<?xmltex \hack{\hfill\break}?>emissions; projection<?xmltex \hack{\hfill\break}?>includes EU-specific <?xmltex \hack{\hfill\break}?>data</oasis:entry>
         <oasis:entry colname="col3">Aggregation of overseas territories into governing nations for total of 213 countries</oasis:entry>
         <oasis:entry colname="col4">Average of two bookkeeping models; use of 16 DGVMs</oasis:entry>
         <oasis:entry colname="col5">Use of four atmospheric inversions</oasis:entry>
         <oasis:entry colname="col6">Based on seven models</oasis:entry>
         <oasis:entry colname="col7">Based on 16 models; revised atmospheric forcing from CRUNCEP to CRU-JRA-55</oasis:entry>
         <oasis:entry colname="col8">Introduction of metrics for evaluation of individual models using observations</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Le Quéré et al. (2018b) GCB2018</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2019</oasis:entry>
         <oasis:entry colname="col2">Global emissions calculated as sum of all countries plus bunkers, rather than taken directly from CDIAC.</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Average of two bookkeeping models; use of 15 DGVMs</oasis:entry>
         <oasis:entry colname="col5">Use of three atmospheric inversions</oasis:entry>
         <oasis:entry colname="col6">Based on nine models</oasis:entry>
         <oasis:entry colname="col7">Based on 16 models</oasis:entry>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Friedlingstein et <?xmltex \hack{\hfill\break}?>al. (2019) GCB2019</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2020</oasis:entry>
         <oasis:entry colname="col2">Cement carbonation now included in the EFOS estimate, reducing EFOS by about 0.2 GtC yr<inline-formula><mml:math id="M196" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the last decade</oasis:entry>
         <oasis:entry colname="col3">India's emissions from Andrew (2020b: India); Corrections to Netherland Antilles and Aruba and Soviet emissions before 1950 as per Andrew (2020a: CO<inline-formula><mml:math id="M197" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>); China's coal emissions in 2019 derived from official statistics, emissions now shown for EU27 instead of EU28.Projection for 2020 based on assessment of four approaches.</oasis:entry>
         <oasis:entry colname="col4">Average of three bookkeeping models; use of 17 DGVMs. Estimate of gross land-use sources and sinks provided</oasis:entry>
         <oasis:entry colname="col5">Use of six atmospheric inversions</oasis:entry>
         <oasis:entry colname="col6">Based on nine models. River flux revised and partitioned NH, tropics, SH</oasis:entry>
         <oasis:entry colname="col7">Based on 17 models</oasis:entry>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Friedlingstein et<?xmltex \hack{\hfill\break}?>al. (2020) GCB2020</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2021</oasis:entry>
         <oasis:entry colname="col2">Projections are no longer an assessment of four approaches.</oasis:entry>
         <oasis:entry colname="col3">Official data included for a number of additional countries, new estimates for South Korea, added emissions from lime production in China.</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M198" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate compared to the estimates adopted in national GHG inventories (NGHGIs)</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">Average of means of eight models and means of seven data products. Current year prediction of <inline-formula><mml:math id="M199" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> using a feed-forward neural network method</oasis:entry>
         <oasis:entry colname="col7">Current year prediction of <inline-formula><mml:math id="M200" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> using a feed-forward neural network method</oasis:entry>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Friedlingstein et <?xmltex \hack{\hfill\break}?>al. (2021) GCB2021 <?xmltex \hack{\hfill\break}?>(this study)</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<sec id="Ch1.S2.SS1">
  <label>2.1</label><?xmltex \opttitle{Fossil CO${}_{{2}}$ emissions ($E_{\mathrm{FOS}}$)}?><title>Fossil CO<inline-formula><mml:math id="M201" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (<inline-formula><mml:math id="M202" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</title>
<sec id="Ch1.S2.SS1.SSS1">
  <label>2.1.1</label><title>Historical period 1850–2020</title>
      <p id="d1e4120">The estimates of global and national fossil CO<inline-formula><mml:math id="M203" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (<inline-formula><mml:math id="M204" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)
include the oxidation of fossil fuels through both combustion (e.g.
transport, heating) and chemical oxidation (e.g. carbon anode decomposition
in aluminium refining) activities, and the decomposition of carbonates in
industrial processes (e.g. the production of cement). We also include
CO<inline-formula><mml:math id="M205" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> uptake from the cement carbonation process. Several emissions
sources are not estimated or not fully covered: coverage of emissions from
lime production are not global, and decomposition of carbonates in glass and
ceramic production are included only for the “Annex 1” countries of the
United Nations Framework Convention on Climate Change (UNFCCC) due to a lack of
activity data. These omissions are considered to be minor. Short-cycle
carbon emissions – for example from combustion of biomass – are not included
here but are accounted for in the CO<inline-formula><mml:math id="M206" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from land use (see
Sect. 2.2).</p>
      <p id="d1e4161">Our estimates of fossil CO<inline-formula><mml:math id="M207" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions are derived using the standard
approach of activity data and emission factors, relying on data collection
by many other parties. Our goal is to produce the best estimate of this
flux, and we therefore use a prioritization framework to combine data from
different sources that have used different methods, while being careful to
avoid double counting and undercounting of emissions sources. The CDIAC-FF
emissions dataset, derived largely from UN energy data, forms the
foundation, and we extend emissions to year Y-1 using energy growth rates
reported by BP. We then proceed to replace estimates using data from what we
consider to be superior sources, for example Annex 1 countries' official
submissions to the UNFCCC. All data points are potentially subject to
revision, not just the latest year. For full details see Andrew and Peters (2021).</p>
      <p id="d1e4173">Other estimates of global fossil CO<inline-formula><mml:math id="M208" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions exist, and these are
compared by Andrew (2020a). The most common reason for differences in
estimates of global fossil CO<inline-formula><mml:math id="M209" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions is a difference in which
emissions sources are included in the datasets. Datasets such as those
published by BP energy company, the US Energy Information Administration,
and the International Energy Agency's “CO<inline-formula><mml:math id="M210" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from fuel
combustion” are all generally limited to emissions from combustion of fossil
fuels. In contrast, datasets such as PRIMAP-hist, CEDS, EDGAR, and GCP's
dataset aim to include all sources of fossil CO<inline-formula><mml:math id="M211" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions. See Andrew (2020a) for detailed comparisons and discussion.</p>
      <p id="d1e4212">Cement absorbs CO<inline-formula><mml:math id="M212" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> from the atmosphere over its lifetime, a process
known as “cement carbonation”. We estimate this CO<inline-formula><mml:math id="M213" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink as the average
of two studies in the literature (Cao et al., 2020; Guo et al., 2021). Both
studies use the same model, developed by Xi et al. (2016), with different
parameterizations and input data. Since carbonation is a function of both
current and previous cement production, we extend these estimates by 1 year to 2020 by using the growth rate derived from the smoothed cement
emissions (10-year smoothing) fitted to the carbonation data.</p>
      <p id="d1e4234">We use the Kaya identity for a simple decomposition of CO<inline-formula><mml:math id="M214" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
into the key drivers (Raupach et al., 2007). While there are variations
(Peters et al., 2017), we focus here on a decomposition of CO<inline-formula><mml:math id="M215" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
into population, GDP per person, energy use per GDP, and CO<inline-formula><mml:math id="M216" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
per energy use. Multiplying these individual components together returns the
CO<inline-formula><mml:math id="M217" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions. Using the decomposition, it is possible to attribute the
change in CO<inline-formula><mml:math id="M218" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions to the change in each of the drivers. This
method gives a first-order understanding of what causes CO<inline-formula><mml:math id="M219" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
to change each year.</p>
</sec>
<sec id="Ch1.S2.SS1.SSS2">
  <label>2.1.2</label><title>2021 projection</title>
      <p id="d1e4300">We provide a projection of global CO<inline-formula><mml:math id="M220" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions in 2021 by combining
separate projections for China, the USA, the EU, India, and for all other countries
combined. The methods are different for each of these. For China we combine
monthly fossil fuel production data from the National Bureau of Statistics,
import and export data from the Customs Administration, and monthly coal
consumption estimates from SX Coal (2021), giving us partial data for the
growth rates to date of natural gas, petroleum, and cement, and of the
consumption itself for raw coal. We then use a regression model to project
full-year emissions based on historical observations. For the USA our
projection is taken directly from the Energy Information Administration's
(EIA) Short-Term Energy Outlook (EIA, 2022), combined with the year-to-date
growth rate of cement production. For the EU we use monthly energy data from
Eurostat to derive estimates of monthly CO<inline-formula><mml:math id="M221" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions through July,
with coal emissions extended first through September using a statistical
relationship with reported electricity generation from coal and other
factors, then through December assuming normal seasonal patterns. EU
emissions from natural gas – a strongly seasonal cycle – are extended
through December using bias-adjusted Holt–Winters exponential smoothing
(Chatfield, 1978). EU emissions from oil are derived using the EIA's
projection of oil consumption for Europe. EU cement emissions are based on
available year-to-date data from two of the largest producers, Germany and
Poland. India's projected emissions are derived from estimates through
August (September for coal) using the methods of Andrew (2020b) and
extrapolated assuming normal seasonal patterns. Emissions for the rest of
the world are derived using projected growth in economic production from the
IMF (2022) combined with extrapolated changes in emissions intensity of
economic production. More details on the <inline-formula><mml:math id="M222" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> methodology and its 2021
projection can be found in Appendix C1.</p>
</sec>
</sec>
<sec id="Ch1.S2.SS2">
  <label>2.2</label><?xmltex \opttitle{CO${}_{{2}}$ emissions from land use, land-use change, and forestry ($E_{\mathrm{LUC}}$)}?><title>CO<inline-formula><mml:math id="M223" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from land use, land-use change, and forestry (<inline-formula><mml:math id="M224" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</title>
      <p id="d1e4362">The net CO<inline-formula><mml:math id="M225" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux from land use, land-use change, and forestry
(<inline-formula><mml:math id="M226" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, called land-use change emissions in the rest of the text)
includes CO<inline-formula><mml:math id="M227" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes from deforestation, afforestation, logging and
forest degradation (including harvest activity), shifting cultivation (cycle
of cutting forest for agriculture, then abandoning), and regrowth of forests
following wood harvest or abandonment of agriculture. Emissions from peat
burning and drainage are added from external datasets.</p>
      <p id="d1e4394">Three bookkeeping approaches (updated estimates of BLUE (Hansis et al.,
2015), OSCAR (Gasser et al., 2020), and H&amp;N2017 (Houghton and Nassikas,
2017)) were used to quantify gross sources and sinks and the resulting net
<inline-formula><mml:math id="M228" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. Uncertainty estimates were derived from the dynamic global
vegetation model (DGVM) ensemble for the time period prior to 1960, using
for the recent decades an uncertainty range of <inline-formula><mml:math id="M229" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.7 GtC yr<inline-formula><mml:math id="M230" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, which
is a semi-quantitative measure for annual and decadal emissions and reflects
our best value judgement that there is at least 68 % chance (<inline-formula><mml:math id="M231" display="inline"><mml:mo lspace="0mm">±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M232" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>) that the true land-use change emission lies within the given
range, for the range of processes considered here. This uncertainty range
had been increased from 0.5 GtC yr<inline-formula><mml:math id="M233" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> after new bookkeeping models were
included that indicated a larger spread than assumed before (Le
Quéré et al., 2018). Projections for 2021 are based on fire activity
from tropical deforestation and degradation as well as emissions from peat
fires and drainage.</p>
      <p id="d1e4454">Our <inline-formula><mml:math id="M234" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimates follow the definition of global carbon cycle models
of CO<inline-formula><mml:math id="M235" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes related to land use and land management and differ from
IPCC definitions adopted in national GHG inventories (NGHGIs) for reporting
under the UNFCCC, which additionally generally include, through adoption of
the IPCC so-called managed land proxy approach, the terrestrial fluxes
occurring on land defined by countries as managed. This partly includes
fluxes due to environmental change (e.g. atmospheric CO<inline-formula><mml:math id="M236" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> increase),
which are part of <inline-formula><mml:math id="M237" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in our definition. This causes the global
emission estimates to be smaller for NGHGIs than for the global carbon budget
definition (Grassi et al., 2018). The same is the case for the Food
Agriculture Organization (FAO) estimates of carbon fluxes on forest land,
which include, compared to <inline-formula><mml:math id="M238" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, both anthropogenic and natural
sources on managed land (Tubiello et al., 2021). Using the approach outlined
in Grassi et al. (2021), here we map as additional information the two
definitions to each other, to provide a comparison of the anthropogenic
carbon budget to the official country reporting to the climate convention.
More details on the <inline-formula><mml:math id="M239" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> methodology can be found in Appendix C2.</p>
</sec>
<sec id="Ch1.S2.SS3">
  <label>2.3</label><?xmltex \opttitle{Growth rate in atmospheric CO${}_{{2}}$ concentration ($G_{\mathrm{ATM}}$)}?><title>Growth rate in atmospheric CO<inline-formula><mml:math id="M240" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration (<inline-formula><mml:math id="M241" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</title>
<sec id="Ch1.S2.SS3.SSS1">
  <label>2.3.1</label><title>Historical period</title>
      <p id="d1e4556">The rate of growth of the atmospheric CO<inline-formula><mml:math id="M242" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration is provided
for years 1959–2020 by the US National Oceanic and Atmospheric
Administration Earth System Research Laboratory (NOAA/ESRL; Dlugokencky and
Tans, 2022), which is updated from Ballantyne et al. (2012) and includes
recent revisions to the calibration scale of atmospheric CO<inline-formula><mml:math id="M243" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
measurements (Hall et al., 2021). For the 1959–1979 period, the global
growth rate is based on measurements of atmospheric CO<inline-formula><mml:math id="M244" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration
averaged from the Mauna Loa and South Pole stations, as observed by the
CO<inline-formula><mml:math id="M245" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> Program at Scripps Institution of Oceanography (Keeling et al.,
1976). For the 1980–2020 time period, the global growth rate is based on the
average of multiple stations selected from the marine boundary layer sites
with well-mixed background air (Ballantyne et al., 2012), after fitting each
station with a smoothed curve as a function of time, and averaging by
latitude band (Masarie and Tans, 1995). The annual growth rate is estimated
by Dlugokencky and Tans (2022) from atmospheric CO<inline-formula><mml:math id="M246" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration by
taking the average of the most recent December–January months corrected for
the average seasonal cycle and subtracting this same average 1 year
earlier. The growth rate in units of ppm yr<inline-formula><mml:math id="M247" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> is converted to units
of GtC yr<inline-formula><mml:math id="M248" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> by multiplying by a factor of 2.124 GtC ppm<inline-formula><mml:math id="M249" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, assuming
instantaneous mixing of CO<inline-formula><mml:math id="M250" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> throughout the atmosphere (Ballantyne et
al., 2012).</p>
      <p id="d1e4650">Starting in 2020, NOAA/ESRL now provides estimates of atmospheric CO<inline-formula><mml:math id="M251" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations with respect to a new calibration scale, referred to as
WMO-CO<inline-formula><mml:math id="M252" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-X2019, in line with the recommendation of the World Meteorological
Organization (WMO) Global Atmosphere Watch (GAW) community (Hall et al.,
2021). The WMO-CO<inline-formula><mml:math id="M253" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-X2019 scale improves upon the earlier WMO-CO<inline-formula><mml:math id="M254" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-X2007 scale
by including a broader set of standards, which contain CO<inline-formula><mml:math id="M255" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> in a wider
range of concentrations that span the range 250–800 ppm (versus 250–520 ppm
for WMO-CO<inline-formula><mml:math id="M256" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-X2007). In addition, NOAA/ESRL made two minor corrections to the
analytical procedure used to quantify CO<inline-formula><mml:math id="M257" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations, fixing an
error in the second virial coefficient of CO<inline-formula><mml:math id="M258" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and accounting for loss
of a small amount of CO<inline-formula><mml:math id="M259" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> to materials in the manometer during the
measurement process. The difference in concentrations measured using
WMO-CO<inline-formula><mml:math id="M260" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-X2019 versus WMO-CO<inline-formula><mml:math id="M261" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-X2007 is <inline-formula><mml:math id="M262" display="inline"><mml:mrow><mml:mo>∼</mml:mo><mml:mo>+</mml:mo></mml:mrow></mml:math></inline-formula>0.18 ppm at 400 ppm
and the observational record of atmospheric CO<inline-formula><mml:math id="M263" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations have
been revised accordingly. The revisions have been applied retrospectively in
all cases where the calibrations were performed by NOAA/ESRL, thus affecting
measurements made by members of the WMO-GAW programme and other regionally
coordinated programmes (e.g. Integrated Carbon Observing System, ICOS).
Changes to the CO<inline-formula><mml:math id="M264" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations measured across these networks
propagate to the global mean CO<inline-formula><mml:math id="M265" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations. Comparing the
estimates of <inline-formula><mml:math id="M266" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> made by Dlugokencky and Tans (2020), used in the
Global Carbon Budget 2020 (Friedlingstein et al., 2020), with updated
estimates from Dlugokencky and Tans (2022), used here, we find that
<inline-formula><mml:math id="M267" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> reduced on average by <inline-formula><mml:math id="M268" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.06 GtC yr<inline-formula><mml:math id="M269" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during 2010–2019 and by
<inline-formula><mml:math id="M270" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.01 GtC yr<inline-formula><mml:math id="M271" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during 1959–2019 due to the new calibration. These
changes are well within the uncertainty ranges reported below. Hence the
change in analytical procedures made by NOAA/ESRL has a negligible impact on
the atmospheric growth rate <inline-formula><mml:math id="M272" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e4863">The uncertainty around the atmospheric growth rate is due to four main
factors. First, the long-term reproducibility of reference gas standards
(around 0.03 ppm for 1<inline-formula><mml:math id="M273" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> from the 1980s; Dlugokencky and Tans, 2022).
Second, small unexplained systematic analytical errors that may have a
duration of several months to 2 years come and go. They have been
simulated by randomizing both the duration and the magnitude (determined
from the existing evidence) in a Monte Carlo procedure. Third, the network
composition of the marine boundary layer with some sites coming or going,
gaps in the time series at each site, etc. (Dlugokencky and Tans, 2022). The
latter uncertainty was estimated by NOAA/ESRL with a Monte Carlo method by
constructing 100 “alternative” networks (Masarie and Tans, 1995; NOAA/ESRL,
2019). The second and third uncertainties, summed in quadrature, add up to
0.085 ppm on average (Dlugokencky and Tans, 2022). Fourth, the uncertainty
associated with using the average CO<inline-formula><mml:math id="M274" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration from a surface
network to approximate the true atmospheric average CO<inline-formula><mml:math id="M275" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration
(mass-weighted, in three dimensions) as needed to assess the total atmospheric
CO<inline-formula><mml:math id="M276" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> burden. In reality, CO<inline-formula><mml:math id="M277" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> variations measured at the stations
will not exactly track changes in total atmospheric burden, with offsets in
magnitude and phasing due to vertical and horizontal mixing. This effect
must be very small on decadal and longer timescales, when the atmosphere
can be considered well mixed. Preliminary estimates suggest this effect
would increase the annual uncertainty, but a full analysis is not yet
available. We therefore maintain an uncertainty around the annual growth
rate based on the multiple stations' dataset ranges between 0.11 and 0.72 GtC yr<inline-formula><mml:math id="M278" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, with a mean of 0.61 GtC yr<inline-formula><mml:math id="M279" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for 1959–1979 and 0.17 GtC yr<inline-formula><mml:math id="M280" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for 1980–2020, when a larger set of stations were available as
provided by Dlugokencky and Tans (2022), but recognize further exploration of
this uncertainty is required. At this time, we estimate the uncertainty of
the decadal averaged growth rate after 1980 at 0.02 GtC yr<inline-formula><mml:math id="M281" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> based on
the calibration and the annual growth rate uncertainty but stretched over a
10-year interval. For years prior to 1980, we estimate the decadal averaged
uncertainty to be 0.07 GtC yr<inline-formula><mml:math id="M282" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> based on a factor proportional to the
annual uncertainty prior and after 1980 (<inline-formula><mml:math id="M283" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.02</mml:mn><mml:mo>×</mml:mo><mml:mo>[</mml:mo><mml:mn mathvariant="normal">0.61</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">0.17</mml:mn><mml:mo>]</mml:mo></mml:mrow></mml:math></inline-formula> GtC yr<inline-formula><mml:math id="M284" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>).</p>
      <p id="d1e5003">We assign a high confidence to the annual estimates of <inline-formula><mml:math id="M285" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> because
they are based on direct measurements from multiple and consistent
instruments and stations distributed around the world (Ballantyne et al.,
2012; Hall et al., 2021).</p>
      <p id="d1e5018">To estimate the total carbon accumulated in the atmosphere since 1750 or
1850, we use an atmospheric CO<inline-formula><mml:math id="M286" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration of 277 <inline-formula><mml:math id="M287" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 3 ppm or
286 <inline-formula><mml:math id="M288" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 3 ppm, respectively, based on a cubic spline fit to ice core
data (Joos and Spahni, 2008). For the construction of the cumulative budget
shown in Fig. 3, we use the fitted estimates of CO<inline-formula><mml:math id="M289" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration
from Joos and Spahni (2008) to estimate the annual atmospheric growth rate
using the conversion factors shown in Table 1. The uncertainty of <inline-formula><mml:math id="M290" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>3 ppm (converted to <inline-formula><mml:math id="M291" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M292" display="inline"><mml:mrow><mml:mi mathvariant="italic">σ</mml:mi><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> is taken directly from the IPCC's AR5
assessment (Ciais et al., 2013). Typical uncertainties in the growth rate in
atmospheric CO<inline-formula><mml:math id="M293" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration from ice core data are equivalent to
<inline-formula><mml:math id="M294" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.1–0.15 GtC yr<inline-formula><mml:math id="M295" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> as evaluated from the Law Dome data
(Etheridge et al., 1996) for individual 20-year intervals over the period
from 1850 to 1960 (Bruno and Joos, 1997).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F3" specific-use="star"><?xmltex \currentcnt{3}?><?xmltex \def\figurename{Figure}?><label>Figure 3</label><caption><p id="d1e5108">Combined components of the global carbon budget illustrated in
Fig. 2 as a function of time, for fossil CO<inline-formula><mml:math id="M296" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (<inline-formula><mml:math id="M297" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>,
including a small sink from cement carbonation; grey) and emissions from
land-use change (<inline-formula><mml:math id="M298" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; brown), as well as their partitioning among the
atmosphere (<inline-formula><mml:math id="M299" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; cyan), ocean (<inline-formula><mml:math id="M300" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; blue), and land
(<inline-formula><mml:math id="M301" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; green). Panel <bold>(a)</bold> shows annual estimates of each flux and panel
<bold>(b)</bold> the cumulative flux (the sum of all prior annual fluxes) since the year
1850. The partitioning is based on nearly independent estimates from
observations (for <inline-formula><mml:math id="M302" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and from process model ensembles constrained by
data (for <inline-formula><mml:math id="M303" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M304" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and does not exactly add up to the sum
of the emissions, resulting in a budget imbalance (BI<inline-formula><mml:math id="M305" display="inline"><mml:msub><mml:mi/><mml:mi mathvariant="normal">M</mml:mi></mml:msub></mml:math></inline-formula>) which is
represented by the difference between the bottom red line (mirroring total
emissions) and the sum of carbon fluxes in the ocean, land, and atmosphere
reservoirs. All data are in GtC yr<inline-formula><mml:math id="M306" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> <bold>(a)</bold> and GtC <bold>(b)</bold>. The
<inline-formula><mml:math id="M307" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimates are primarily from Gilfillan and Marland (2021), with
uncertainty of about <inline-formula><mml:math id="M308" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>5 % (<inline-formula><mml:math id="M309" display="inline"><mml:mo lspace="0mm">±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M310" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>). The <inline-formula><mml:math id="M311" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
estimates are from three bookkeeping models (Table 4) with uncertainties of
about <inline-formula><mml:math id="M312" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M313" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The <inline-formula><mml:math id="M314" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimates prior to 1959 are
from Joos and Spahni (2008) with uncertainties equivalent to about <inline-formula><mml:math id="M315" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.1–0.15 GtC yr<inline-formula><mml:math id="M316" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and from Dlugokencky and Tans (2022) since 1959
with uncertainties of about <inline-formula><mml:math id="M317" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.07 GtC yr<inline-formula><mml:math id="M318" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>  during 1959–1979 and
<inline-formula><mml:math id="M319" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.02 GtC yr<inline-formula><mml:math id="M320" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> since 1980. The <inline-formula><mml:math id="M321" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate is the
average from Khatiwala et al. (2013) and DeVries (2014) with uncertainty of
about <inline-formula><mml:math id="M322" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>30 % prior to 1959, and the average of an ensemble of models
and an ensemble of <inline-formula><mml:math id="M323" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M324" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data products (Table 4) with uncertainties of
about <inline-formula><mml:math id="M325" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.4 GtC yr<inline-formula><mml:math id="M326" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> since 1959. The <inline-formula><mml:math id="M327" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate is the
average of an ensemble of models (Table 4) with uncertainties of about
<inline-formula><mml:math id="M328" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1 GtC yr<inline-formula><mml:math id="M329" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. See the text for more details of each component and
their uncertainties. </p></caption>
            <?xmltex \igopts{width=412.564961pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f03.png"/>

          </fig>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T4" specific-use="star"><?xmltex \currentcnt{4}?><label>Table 4</label><caption><p id="d1e5469">References for the process models, <inline-formula><mml:math id="M330" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M331" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based ocean data products, and atmospheric inversions. All models and products are updated with new data to the end of year 2020, and the atmospheric forcing for the DGVMs has been updated as described in Sect. C2.2.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.85}[.85]?><oasis:tgroup cols="3">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="8cm"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Model/data name</oasis:entry>
         <oasis:entry colname="col2">Reference</oasis:entry>
         <oasis:entry colname="col3">Change from Global Carbon Budget 2020 (Friedlingstein et al., 2020)</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col3">Bookkeeping models for land-use change emissions </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BLUE</oasis:entry>
         <oasis:entry colname="col2">Hansis et al. (2015)</oasis:entry>
         <oasis:entry colname="col3">No change to model, but simulations performed with updated LUH2 forcing.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Updated H&amp;N2017</oasis:entry>
         <oasis:entry colname="col2">Houghton and Nassikas (2017)</oasis:entry>
         <oasis:entry colname="col3">Adjustment to treatment of harvested wood products. Update to FRA2020 and 2021 FAOSTAT for forest cover and land-use areas. Forest loss in excess of increases in cropland and pastures represented an increase in shifting cultivation. Extra-tropical peatland drainage emissions added (based on Qiu et al., 2021).</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">OSCAR</oasis:entry>
         <oasis:entry colname="col2">Gasser et al. (2020)</oasis:entry>
         <oasis:entry colname="col3">Update to OSCAR3.1.2, which provides finer resolution (96 countries and regions). LUH2-GCB2019 input data replaced by LUH2-GCB2021. FRA2015 (Houghton  and Nassikas, 2017) still used as a second driving dataset, with emissions from FRA2015 extended to 2020. Constraining based on this year's budget data.</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col3">Dynamic global vegetation models </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CABLE-POP</oasis:entry>
         <oasis:entry colname="col2">Haverd et al. (2018)</oasis:entry>
         <oasis:entry colname="col3">Changes in parameterization, minor bug fixes.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CLASSIC</oasis:entry>
         <oasis:entry colname="col2">Melton et al. (2020)<inline-formula><mml:math id="M332" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Non-structural carbohydrates are now explicitly simulated.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CLM5.0</oasis:entry>
         <oasis:entry colname="col2">Lawrence et al. (2019)</oasis:entry>
         <oasis:entry colname="col3">No change.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">DLEM</oasis:entry>
         <oasis:entry colname="col2">Tian et al. (2015)<inline-formula><mml:math id="M333" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Updated algorithms for land-use change processes.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">IBIS</oasis:entry>
         <oasis:entry colname="col2">Yuan et al. (2014)<inline-formula><mml:math id="M334" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Several changes in parameterization; dynamic carbon allocation scheme.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ISAM</oasis:entry>
         <oasis:entry colname="col2">Meiyappan et al. (2015)<inline-formula><mml:math id="M335" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">ISAM now accounting for vertically resolved soil biogeochemistry (carbon and nitrogen) module (Shu et al., 2020).</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ISBA-CTRIP</oasis:entry>
         <oasis:entry colname="col2">Delire et al. (2020)<inline-formula><mml:math id="M336" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">e</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Updated spin-up protocol <inline-formula><mml:math id="M337" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> model name updated (SURFEXv8 in GCB2017) <inline-formula><mml:math id="M338" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> inclusion of crop harvesting module.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">JSBACH</oasis:entry>
         <oasis:entry colname="col2">Reick et al. (2021)<inline-formula><mml:math id="M339" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">f</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Wood product pools per plant functional type.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">JULES-ES</oasis:entry>
         <oasis:entry colname="col2">Wiltshire et al. (2021)<inline-formula><mml:math id="M340" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">g</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Version 1.1, inclusion of interactive fire; Burton et al. (2019).</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LPJ-GUESS</oasis:entry>
         <oasis:entry colname="col2">Smith et al. (2014)<inline-formula><mml:math id="M341" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">h</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">No code change. Using updated LUH2 and climate forcings.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LPJ</oasis:entry>
         <oasis:entry colname="col2">Poulter et al. (2011)<inline-formula><mml:math id="M342" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">i</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Updated soil data from FAO to HWSD v2.0.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LPX-Bern</oasis:entry>
         <oasis:entry colname="col2">Lienert and Joos (2018)</oasis:entry>
         <oasis:entry colname="col3">No change.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">OCN</oasis:entry>
         <oasis:entry colname="col2">Zaehle and Friend (2010)<inline-formula><mml:math id="M343" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">No change (uses r294).</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ORCHIDEEv3</oasis:entry>
         <oasis:entry colname="col2">Vuichard et al. (2019)<inline-formula><mml:math id="M344" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">k</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Updated growth respiration scheme (revision 7267).</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">SDGVM</oasis:entry>
         <oasis:entry colname="col2">Walker et al. (2017)<inline-formula><mml:math id="M345" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">l</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">No changes from version used in Friedlingstein et al. (2019), except for properly switching from grasslands to pasture in the blending of the ESA data with LUH2; this change affects mostly the semi-arid lands.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">VISIT</oasis:entry>
         <oasis:entry colname="col2">Kato et al. (2013)<inline-formula><mml:math id="M346" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">m</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Minor bug fix on CH<inline-formula><mml:math id="M347" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> emissions of last few years.</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">YIBs</oasis:entry>
         <oasis:entry colname="col2">Yue and Unger (2015)</oasis:entry>
         <oasis:entry colname="col3">Inclusion of nutrient limit with down-regulation approach of Arora et al. (2009).</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col3">Global ocean biogeochemistry models </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">NEMO-PlankTOM12</oasis:entry>
         <oasis:entry colname="col2">Wright et al. (2021)<inline-formula><mml:math id="M348" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">n</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Updated biochemical model to include 12 functional types. Change to spin-up, now using a looped 1990.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MICOM-HAMOCC (NorESM-OCv1.2)</oasis:entry>
         <oasis:entry colname="col2">Schwinger et al. (2016)</oasis:entry>
         <oasis:entry colname="col3">No change.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MPIOM-HAMOCC6</oasis:entry>
         <oasis:entry colname="col2">Lacroix et al. (2021)</oasis:entry>
         <oasis:entry colname="col3">Added riverine fluxes; CMIP6 model version including modifications and bug-fixes in HAMOCC and MPIOM.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">NEMO3.6-PISCESv2-gas (CNRM)</oasis:entry>
         <oasis:entry colname="col2">Berthet et al. (2019)<inline-formula><mml:math id="M349" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">o</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">small bug fixes; updated model spin-up (new forcings); atm forcing is now JRA55-Do including 2020 year and varying riverine freshwater inputs.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">FESOM-2.1-REcoM2</oasis:entry>
         <oasis:entry colname="col2">Hauck et al. (2020)<inline-formula><mml:math id="M350" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">p</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Updated physical model version FESOM2.1, and including second zooplankton and second detritus group. Used new atmospheric CO<inline-formula><mml:math id="M351" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> time series provided by GCB.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MOM6-COBALT (Princeton)</oasis:entry>
         <oasis:entry colname="col2">Liao et al. (2020)</oasis:entry>
         <oasis:entry colname="col3">Adjustment of the piston velocity prefactor (0.337 to 0.251 cph m<inline-formula><mml:math id="M352" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> s<inline-formula><mml:math id="M353" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). MOM6 update from GitHub version b748b1b (2018-10-03) to version 69a096b (2021-02-24). Updated model spin-up and simulation using JRA55-do v1.5. Used new atmospheric CO<inline-formula><mml:math id="M354" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> time series provided by GCB.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CESM-ETHZ</oasis:entry>
         <oasis:entry colname="col2">Doney et al. (2009)</oasis:entry>
         <oasis:entry colname="col3">No change in the model. Used new atmospheric CO<inline-formula><mml:math id="M355" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> time series provided by GCB.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">NEMO-PISCES (IPSL)</oasis:entry>
         <oasis:entry colname="col2">Aumont et al. (2015)</oasis:entry>
         <oasis:entry colname="col3">No change.</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T5" specific-use="star"><?xmltex \currentcnt{4}?><label>Table 4</label><caption><p id="d1e6081">Continued.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.85}[.85]?><oasis:tgroup cols="3">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="8cm"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Model/data name</oasis:entry>
         <oasis:entry colname="col2">Reference</oasis:entry>
         <oasis:entry colname="col3">Change from Global Carbon Budget 2020 (Friedlingstein et al., 2020)</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col3">Ocean <inline-formula><mml:math id="M378" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M379" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Landschützer (MPI-SOMFFN)</oasis:entry>
         <oasis:entry colname="col2">Landschützer et al. (2016)</oasis:entry>
         <oasis:entry colname="col3">Update to SOCATv2021 measurements and time period 1982–2020; the estimate now covers the full open ocean and coastal domain as well as the Arctic Ocean extension described in Landschützer et al. (2020).</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Rödenbeck (Jena-MLS)</oasis:entry>
         <oasis:entry colname="col2">Rödenbeck et al. (2014)</oasis:entry>
         <oasis:entry colname="col3">Update to SOCATv2021 measurements, time period extended to 1957–2020, involvement of a multi-linear regression for extrapolation (combined with an explicitly interannual correction), use of OCIM (DeVries, 2014) as decadal prior, carbonate chemistry parameterization now time-dependent, grid resolution increased to <inline-formula><mml:math id="M380" display="inline"><mml:mrow><mml:mn mathvariant="normal">2.5</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M381" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>, adjustable degrees of freedom now also covering shallow areas and Arctic, some numerical revisions.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CMEMS-LSCE-FFNNv2</oasis:entry>
         <oasis:entry colname="col2">Chau et al. (2022)</oasis:entry>
         <oasis:entry colname="col3">Update to SOCATv2021 measurements and time period 1985–2020. The CMEMS-LSCE-FFNNv2 product now covers both the open ocean and coastal regions (see in Chau et al., 2022, for model description and evaluation).</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CSIR-ML6</oasis:entry>
         <oasis:entry colname="col2">Gregor et al. (2019)</oasis:entry>
         <oasis:entry colname="col3">Updated to SOCATv2021. Reconstruction now spans the period 1985–2020 and includes updates using the SeaFlux protocols (Fay et al., 2021).</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Watson et al.</oasis:entry>
         <oasis:entry colname="col2">Watson et al. (2020)</oasis:entry>
         <oasis:entry colname="col3">Updated to SOCAT v2021. A monthly climatology of the skin temperature deviation as calculated for years 2003–2011 is now used in place of a single global average figure. SOM calculation updated to treat the Arctic as a separate biome.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">NIES-NN</oasis:entry>
         <oasis:entry colname="col2">Zeng et al. (2014)</oasis:entry>
         <oasis:entry colname="col3">New this year.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">JMA-MLR</oasis:entry>
         <oasis:entry colname="col2">Iida et al. (2021)</oasis:entry>
         <oasis:entry colname="col3">New this year.</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">OS-ETHZ-GRaCER</oasis:entry>
         <oasis:entry colname="col2">Gregor and Gruber (2021)</oasis:entry>
         <oasis:entry colname="col3">New this year.</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col3">Atmospheric inversions </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CAMS</oasis:entry>
         <oasis:entry colname="col2">Chevallier et al. (2005)<inline-formula><mml:math id="M382" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">q</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">No change.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CarbonTracker Europe (CTE)</oasis:entry>
         <oasis:entry colname="col2">van der Laan-Luijkx et al. (2017)</oasis:entry>
         <oasis:entry colname="col3">No change.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Jena CarboScope</oasis:entry>
         <oasis:entry colname="col2">Rödenbeck et al. (2018)<inline-formula><mml:math id="M383" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">r</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">No change.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UoE in situ</oasis:entry>
         <oasis:entry colname="col2">Feng et al. (2016)<inline-formula><mml:math id="M384" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">s</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Fossil fuels now from GCP-GridFEDv2021.2.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">NISMON-CO<inline-formula><mml:math id="M385" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Niwa et al. (2017)<inline-formula><mml:math id="M386" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">t</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Some inversion parameters were changed.</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CMS-Flux</oasis:entry>
         <oasis:entry colname="col2">Liu et al. (2021)</oasis:entry>
         <oasis:entry colname="col3">New this year.</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table><?xmltex \begin{scaleboxenv}{.83}[.83]?><table-wrap-foot><p id="d1e6084"><inline-formula><mml:math id="M356" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula> See also Asaadi et al. (2018).
<inline-formula><mml:math id="M357" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> See also Tian et al. (2011).
<inline-formula><mml:math id="M358" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula> The dynamic carbon allocation scheme was presented by Xia et al. (2015).
<inline-formula><mml:math id="M359" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula> See also Jain et al. (2013). Soil biogeochemistry is updated based on Shu et al. (2020).
<inline-formula><mml:math id="M360" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">e</mml:mi></mml:msup></mml:math></inline-formula> See also Decharme et al. (2019) and Seferian et al. (2019).
<inline-formula><mml:math id="M361" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">f</mml:mi></mml:msup></mml:math></inline-formula> Mauritsen et al. (2019).
<inline-formula><mml:math id="M362" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">g</mml:mi></mml:msup></mml:math></inline-formula> See also Sellar et al. (2019) and Burton et al. (2019). JULES-ES is the Earth System configuration of the Joint UK Land Environment Simulator as used in the UK Earth System Model (UKESM).
<inline-formula><mml:math id="M363" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">h</mml:mi></mml:msup></mml:math></inline-formula> to account for the differences between the derivation of shortwave radiation from CRU cloudiness and DSWRF from CRUJRA, the photosynthesis scaling parameter <inline-formula><mml:math id="M364" display="inline"><mml:mrow><mml:mi mathvariant="italic">α</mml:mi><mml:mi>a</mml:mi></mml:mrow></mml:math></inline-formula> was modified (<inline-formula><mml:math id="M365" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>15 %) to yield similar results.
<inline-formula><mml:math id="M366" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">i</mml:mi></mml:msup></mml:math></inline-formula> Compared to published version, decreased LPJ wood harvest efficiency so that 50 % of biomass was removed off-site compared to 85 % used in the 2012 budget. Residue management of managed grasslands increased so that 100  % of harvested grass enters the litter pool.
<inline-formula><mml:math id="M367" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula> See also Zaehle et al. (2011).
<inline-formula><mml:math id="M368" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">k</mml:mi></mml:msup></mml:math></inline-formula> See also Zaehle and Friend (2010) and Krinner et al. (2005).
<inline-formula><mml:math id="M369" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">l</mml:mi></mml:msup></mml:math></inline-formula> See also Woodward and Lomas (2004).
<inline-formula><mml:math id="M370" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">m</mml:mi></mml:msup></mml:math></inline-formula> See also Ito and Inatomi (2012).
<inline-formula><mml:math id="M371" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">n</mml:mi></mml:msup></mml:math></inline-formula> See also Buitenhuis et al. (2013).
<inline-formula><mml:math id="M372" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">o</mml:mi></mml:msup></mml:math></inline-formula> See also Séférian et al. (2019).
<inline-formula><mml:math id="M373" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">p</mml:mi></mml:msup></mml:math></inline-formula> See also Schourup-Kristensen et al. (2014).
<inline-formula><mml:math id="M374" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">q</mml:mi></mml:msup></mml:math></inline-formula> See also Remaud et al. (2018).
<inline-formula><mml:math id="M375" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">r</mml:mi></mml:msup></mml:math></inline-formula> See also Rodenbeck et al. (2003).
<inline-formula><mml:math id="M376" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">s</mml:mi></mml:msup></mml:math></inline-formula> See also Feng et al. (2009) and Palmer et al. (2019).
<inline-formula><mml:math id="M377" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">t</mml:mi></mml:msup></mml:math></inline-formula> See also Niwa et al. (2020).</p></table-wrap-foot><?xmltex \end{scaleboxenv}?></table-wrap>

</sec>
<sec id="Ch1.S2.SS3.SSS2">
  <label>2.3.2</label><title>2021 projection</title>
      <p id="d1e6581">We provide an assessment of <inline-formula><mml:math id="M387" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for 2021 based on the monthly
calculated global atmospheric CO<inline-formula><mml:math id="M388" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration (GLO) through August
(Dlugokencky and Tans, 2022), and bias-adjusted Holt–Winters exponential
smoothing with additive seasonality (Chatfield, 1978) to project to January
2022. Additional analysis suggests that the first half of the year (the
boreal winter–spring–summer transition) shows more interannual variability
than the second half of the year (the boreal summer–autumn–winter
transition), so that the exact projection method applied to the second half
of the year has a relatively smaller impact on the projection of the full
year. Uncertainty is estimated from past variability using the standard
deviation of the last 5 years' monthly growth rates.</p>
</sec>
</sec>
<sec id="Ch1.S2.SS4">
  <label>2.4</label><?xmltex \opttitle{Ocean CO${}_{{2}}$ sink}?><title>Ocean CO<inline-formula><mml:math id="M389" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink</title>
      <p id="d1e6623">The reported estimate of the global ocean anthropogenic CO<inline-formula><mml:math id="M390" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink
<inline-formula><mml:math id="M391" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is derived as the average of two estimates. The first estimate
is derived as the mean over an ensemble of eight global ocean
biogeochemistry models (GOBMs, Tables 4 and A2). The second estimate is
obtained as the mean over an ensemble of seven observation-based
data products (Tables 4 and  A3). An eighth product (Watson et al.,
2020) is shown but is not included in the ensemble average as it differs
from the other products by adjusting the flux to a cool, salty ocean surface
skin (see Appendix C3.1 for a discussion of the Watson product). The GOBMs
simulate both the natural and anthropogenic CO<inline-formula><mml:math id="M392" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> cycles in the ocean.
They constrain the anthropogenic air–sea CO<inline-formula><mml:math id="M393" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux (the dominant
component of <inline-formula><mml:math id="M394" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) by the transport of carbon into the ocean
interior, which is also the controlling factor of present-day ocean carbon
uptake in the real world. They cover the full globe and all seasons and were
recently evaluated against surface ocean carbon observations, suggesting
they are suitable to estimate the annual ocean carbon sink (Hauck et al.,
2020). The data products are tightly linked to observations of <inline-formula><mml:math id="M395" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M396" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
(fugacity of CO<inline-formula><mml:math id="M397" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, which equals <inline-formula><mml:math id="M398" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M399" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> corrected for the non-ideal
behaviour of the gas; Pfeil et al., 2013), which carry imprints of temporal
and spatial variability but are also sensitive to uncertainties in
gas-exchange parameterizations and data sparsity. Their asset is the
assessment of interannual and spatial variability (Hauck et al., 2020). We
further use two diagnostic ocean models to estimate <inline-formula><mml:math id="M400" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> over the
industrial era (1781–1958).</p>
      <p id="d1e6728">The global <inline-formula><mml:math id="M401" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M402" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based flux estimates were adjusted to remove the
pre-industrial ocean source of CO<inline-formula><mml:math id="M403" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> to the atmosphere of 0.61 GtC yr<inline-formula><mml:math id="M404" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> from river input to the ocean (the average of 0.45 <inline-formula><mml:math id="M405" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.18 GtC yr<inline-formula><mml:math id="M406" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> by Jacobson et al., 2007, and 0.78 <inline-formula><mml:math id="M407" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.41 GtC yr<inline-formula><mml:math id="M408" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
by Resplandy et al., 2018), to satisfy our definition of <inline-formula><mml:math id="M409" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Hauck et al., 2020). The river flux adjustment was distributed over the
latitudinal bands using the regional distribution of Aumont et al. (2001;
north: 0.16 GtC yr<inline-formula><mml:math id="M410" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, tropics: 0.15 GtC yr<inline-formula><mml:math id="M411" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, south: 0.30 GtC yr<inline-formula><mml:math id="M412" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), acknowledging that the boundaries of Aumont et al. (2001; namely
20<inline-formula><mml:math id="M413" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S and 20<inline-formula><mml:math id="M414" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N) are not consistent with the boundaries
otherwise used in the GCB (30<inline-formula><mml:math id="M415" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S and 30<inline-formula><mml:math id="M416" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N). A recent
modelling study (Lacroix et al., 2020) suggests that more of the riverine
outgassing is located in the tropics than in the Southern Ocean, and hence
this regional distribution is associated with a major uncertainty.
Anthropogenic perturbations of river carbon and nutrient transport to the
ocean are not considered (see Sect. 2.7).</p>
      <p id="d1e6891">We derive <inline-formula><mml:math id="M417" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from GOBMs by using a simulation (sim A) with
historical forcing of climate and atmospheric CO<inline-formula><mml:math id="M418" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, accounting for model
biases and drift from a control simulation (sim B) with constant atmospheric
CO<inline-formula><mml:math id="M419" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and normal-year climate forcing. A third simulation (sim C) with
historical atmospheric CO<inline-formula><mml:math id="M420" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> increase and normal-year climate forcing is
used to attribute the ocean sink to CO<inline-formula><mml:math id="M421" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (sim C minus sim B) and climate
(sim A minus sim C) effects. Data products are adjusted to represent the
full ocean area by a simple scaling approach when coverage is below 98 %.
GOBMs and data products fall within the observational constraints over the
1990s (2.2 <inline-formula><mml:math id="M422" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M423" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Ciais et al., 2013) after applying
adjustments.</p>
      <p id="d1e6962">We assign an uncertainty of <inline-formula><mml:math id="M424" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.4 GtC yr<inline-formula><mml:math id="M425" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to the ocean sink
based on a combination of random (ensemble standard deviation) and
systematic uncertainties (GOBMs bias in anthropogenic carbon accumulation,
previously reported uncertainties in <inline-formula><mml:math id="M426" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M427" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products; see
Sect. C3.3). We assess a medium confidence level to the annual ocean
CO<inline-formula><mml:math id="M428" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink and its uncertainty because it is based on multiple lines of
evidence, it is consistent with ocean interior carbon estimates (Gruber et
al., 2019; see Sect. 3.5.5), and the results are consistent in that the
interannual variability in the GOBMs and data-based estimates are all
generally small compared to the variability in the growth rate of
atmospheric CO<inline-formula><mml:math id="M429" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration. We refrain from assigning a high
confidence because of the systematic deviation between the GOBM and
data product trends since around 2002. More details on the <inline-formula><mml:math id="M430" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
methodology can be found in Appendix C3.</p>
      <p id="d1e7030">The ocean CO<inline-formula><mml:math id="M431" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink forecast for the year 2021 is based on the annual
historical and estimated 2021 atmospheric CO<inline-formula><mml:math id="M432" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration
(Dlugokencky and Tans, 2021), historical and estimated 2021 annual global
fossil fuel emissions from this year's carbon budget, and the spring (March,
April, May) oceanic Niño index (ONI) (NCEP, 2021). Using a
non-linear regression approach, i.e. a feed-forward neural network,
atmospheric CO<inline-formula><mml:math id="M433" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, the ONI, and the fossil fuel emissions are used
as training data to best match the annual ocean CO<inline-formula><mml:math id="M434" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (i.e. combined
<inline-formula><mml:math id="M435" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate from GOBMs and data products) from 1959 through 2020
from this year's carbon budget. Using this relationship, the 2021
<inline-formula><mml:math id="M436" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> can then be estimated from the projected 2021 input data using
the non-linear relationship established during the network training. To
avoid overfitting, the neural network was trained with a variable number of
hidden neurons (varying between 2–5), and 20 % of the randomly selected
training data were withheld for independent internal testing. Based on the
best output performance (tested using the 20 % withheld input data), the
best performing number of neurons was selected. In a second step, we trained
the network 10 times using the best number of neurons identified in step 1
and different sets of randomly selected training data. The mean of the 10
training runs is considered our best forecast, whereas the standard deviation of
the 10 ensembles provides a first-order estimate of the forecast
uncertainty. This uncertainty is then combined with the <inline-formula><mml:math id="M437" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
uncertainty (0.4 GtC yr<inline-formula><mml:math id="M438" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) to estimate the overall uncertainty of the
2021 prediction.</p>
</sec>
<sec id="Ch1.S2.SS5">
  <label>2.5</label><?xmltex \opttitle{Terrestrial CO${}_{{2}}$ sink}?><title>Terrestrial CO<inline-formula><mml:math id="M439" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink</title>
      <p id="d1e7133">The terrestrial land sink (<inline-formula><mml:math id="M440" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is thought to be due to the combined
effects of fertilization by rising atmospheric CO<inline-formula><mml:math id="M441" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and N inputs on
plant growth, as well as the effects of climate change such as the
lengthening of the growing season in northern temperate and boreal areas.
<inline-formula><mml:math id="M442" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> does not include land sinks directly resulting from land use and
land-use change (e.g. regrowth of vegetation) as these are part of the
land-use flux (<inline-formula><mml:math id="M443" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), although system boundaries make it difficult to exactly
attribute CO<inline-formula><mml:math id="M444" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes on land between <inline-formula><mml:math id="M445" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M446" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Erb et al., 2013).</p>
      <p id="d1e7210"><inline-formula><mml:math id="M447" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is estimated from the multi-model mean of 17 DGVMs (Table A1). As
described in Appendix C4, DGVM simulations include all climate variability
and CO<inline-formula><mml:math id="M448" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> effects over land, with 12 DGVMs also including the effect of N
inputs. The DGVM estimate of <inline-formula><mml:math id="M449" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> does not include the export of
carbon to aquatic systems or its historical perturbation, which is discussed
in Appendix D3. See Appendix C4 for DGVM evaluation and uncertainty
assessment for <inline-formula><mml:math id="M450" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, using the International Land Model Benchmarking
system (ILAMB; Collier et al., 2018). More details on the <inline-formula><mml:math id="M451" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
methodology can be found in Appendix C4.</p>
      <p id="d1e7265">Like the ocean forecast, the land CO<inline-formula><mml:math id="M452" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M453" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) forecast is
based on the annual historical and estimated 2021 atmospheric CO<inline-formula><mml:math id="M454" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration (Dlugokencky and Tans 2021), historical and estimated 2021
annual global fossil fuel emissions from this year's carbon budget, and the
summer (June, July, August) ONI (NCEP, 2021). All training data are
again used to best match <inline-formula><mml:math id="M455" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from 1959 through 2020 from this year's
carbon budget using a feed-forward neural network. To avoid overfitting, the
neural network was trained with a variable number of hidden neurons (varying
between 2–15), larger than for <inline-formula><mml:math id="M456" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> prediction due to the stronger
land carbon interannual variability. As done for <inline-formula><mml:math id="M457" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, a pre-training step selects the optimal number of hidden neurons based on 20 % withheld input
data, and in a second step, an ensemble of 10 forecasts is produced to
provide the mean forecast plus uncertainty. This uncertainty is then
combined with the <inline-formula><mml:math id="M458" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> uncertainty for 2020 (1.0 GtC yr<inline-formula><mml:math id="M459" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) to
estimate the overall uncertainty of the 2021 prediction.</p>
</sec>
<sec id="Ch1.S2.SS6">
  <label>2.6</label><title>The atmospheric perspective</title>
      <p id="d1e7363">The worldwide network of in situ atmospheric measurements and satellite-derived atmospheric CO<inline-formula><mml:math id="M460" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> column (xCO<inline-formula><mml:math id="M461" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) observations put a strong
constraint on changes in the atmospheric abundance of CO<inline-formula><mml:math id="M462" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>. This is true
globally (hence our large confidence in <inline-formula><mml:math id="M463" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), but also regionally in
regions with sufficient observational density found mostly in the
extra-tropics. This allows atmospheric inversion methods to constrain the
magnitude and location of the combined total surface CO<inline-formula><mml:math id="M464" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes from
all sources, including fossil and land-use change emissions and land and
ocean CO<inline-formula><mml:math id="M465" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes. The inversions assume <inline-formula><mml:math id="M466" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> to be well known, and
they solve for the spatial and temporal distribution of land and ocean
fluxes from the residual gradients of CO<inline-formula><mml:math id="M467" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> between stations that are not
explained by fossil fuel emissions. By design, such systems close the
carbon balance (<inline-formula><mml:math id="M468" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>) and thus provide an additional perspective
on the independent estimates of the ocean and land fluxes.</p>
      <p id="d1e7458">This year's release includes six inversion systems that are described in
Table A4. Each system is rooted in Bayesian inversion principles but uses
slightly different methodologies. These differences concern the selection of
atmospheric CO<inline-formula><mml:math id="M469" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data and the choice of a priori fluxes to refine with
these data. They also differ in spatial and temporal resolution, assumed
correlation structures, and mathematical approach of the models (see
references in Table A4 for details). Importantly, the systems use a variety
of transport models, which was demonstrated to be a driving factor behind
differences in atmospheric inversion-based flux estimates, and specifically
their distribution across latitudinal bands (Gaubert et al., 2019; Schuh et
al., 2019). Multiple inversion systems (UoE, CTE, and CAMS) were previously
tested with satellite xCO<inline-formula><mml:math id="M470" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> retrievals from GOSAT or OCO-2 measurements,
but their results at the larger scales (as discussed in this work) did not
deviate substantially from their in situ counterparts and are therefore not
separately included. One inversion this year (CMS-Flux) used ACOS-GOSAT v9
retrievals between July 2009 and December 2014 and OCO-2 b10 retrievals between
January to December 2015, in addition to the in situ observational CO<inline-formula><mml:math id="M471" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> mole
fraction records.</p>
      <p id="d1e7488">The original products delivered by the inverse modellers were modified to
facilitate the comparison to the other elements of the budget, specifically
on three accounts: (1) global total fossil fuel emissions, (2) riverine CO<inline-formula><mml:math id="M472" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
transport, and (3) cement carbonation CO<inline-formula><mml:math id="M473" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> uptake. Details are given
below. We note that with these adjustments the inverse results no longer
represent the net atmosphere–surface exchange over land–ocean areas as
sensed by atmospheric observations. Instead, for land, they become the net
uptake of CO<inline-formula><mml:math id="M474" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> by vegetation and soils that is not exported by fluvial
systems, similar to the DGVM estimates. For oceans, they become the net
uptake of anthropogenic CO<inline-formula><mml:math id="M475" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, similar to the GOBMs estimates.</p>
      <p id="d1e7527">The inversion systems prescribe global fossil fuel emissions based on the
GCP's Gridded Fossil Emissions Dataset version 2021.2 (GCP-GridFEDv2021.2;
Jones et al., 2021b), which is an update to 2019 of the first version of
GCP-GridFED presented by Jones et al. (2021a). GCP-GridFEDv2021.2 scales
gridded estimates of CO<inline-formula><mml:math id="M476" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from EDGARv4.3.2 (Janssens-Maenhout
et al., 2019) within national territories to match national emissions
estimates provided by the GCB for the years 1959–2020, which were compiled
following the methodology described in Sect. 2.1 with all datasets
available on 14 August 2021 (Robbie Andrew, personal communication, 2021). Small differences between the
systems due to for instance regridding to the transport model resolution are
corrected for in the latitudinal partitioning we present, to ensure
agreement with the estimate of <inline-formula><mml:math id="M477" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in this budget. We also note that
the ocean fluxes used as prior by five out of six inversions are part of the
suite of the ocean process model or <inline-formula><mml:math id="M478" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M479" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data products listed in Sect. 2.4. Although these fluxes are further adjusted by the atmospheric
inversions, it makes the inversion estimates of the ocean fluxes not
completely independent of <inline-formula><mml:math id="M480" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> assessed here.</p>
      <p id="d1e7578">To facilitate comparisons to the independent <inline-formula><mml:math id="M481" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M482" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, we
used the same corrections for transport and outgassing of carbon transported
from land to ocean, as done for the observation-based estimates of
<inline-formula><mml:math id="M483" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (see Appendix C3). Furthermore, the inversions did not
include a cement carbonation sink (see Sect. 2.1), and therefore this GCB
component is implicitly part of their total land sink estimate. In the
numbers presented in this budget, each year's global carbonation sink from
cement was subtracted from each year's estimated land sink in each
inversion, distributed proportionally to fossil fuel emissions per region
(north, tropics, and south).</p>
      <p id="d1e7614">The atmospheric inversions are evaluated using vertical profiles of
atmospheric CO<inline-formula><mml:math id="M484" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations (Fig. B4). More than 30 aircraft
programmes over the globe, either regular programmes or repeated surveys over at
least 9 months, have been used to assess model performance (with space–time
observational coverage sparse in the SH and tropics, and denser in NH
mid-latitudes; Table A6). The six models are compared to the independent
aircraft CO<inline-formula><mml:math id="M485" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements between 2 and 7 km above sea level between
2001 and 2020. Results are shown in Fig. B4 and discussed in Sect. 3.7.</p>
      <p id="d1e7635">With a relatively small ensemble (<inline-formula><mml:math id="M486" display="inline"><mml:mrow><mml:mi>N</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">6</mml:mn></mml:mrow></mml:math></inline-formula>) of systems that moreover share some
a priori fluxes used with one another, or with the process-based models, it
is difficult to justify using their mean and standard deviation as a metric
for uncertainty across the ensemble. We therefore report their full range
(min–max) without their mean. More details on the atmospheric inversions
methodology can be found in Appendix C5.</p>
</sec>
<sec id="Ch1.S2.SS7">
  <label>2.7</label><title>Processes not included in the global carbon budget</title>
      <p id="d1e7658">The contribution of anthropogenic CO and CH<inline-formula><mml:math id="M487" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> to the global carbon
budget is not fully accounted for in Eq. (1) and is described in Appendix D1. The contributions of other carbonates to CO<inline-formula><mml:math id="M488" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions is described
in Appendix D2. The contribution of anthropogenic changes in river fluxes is
conceptually included in Eq. (1) in <inline-formula><mml:math id="M489" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and in <inline-formula><mml:math id="M490" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, but it is
not represented in the process models used to quantify these fluxes. This
effect is discussed in Appendix D3. Similarly, the loss of additional sink
capacity from reduced forest cover is missing in the combination of
approaches used here to estimate both land fluxes (<inline-formula><mml:math id="M491" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M492" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)
and its potential effect is discussed and quantified in Appendix D4.</p>
</sec>
</sec>
<sec id="Ch1.S3">
  <label>3</label><title>Results</title>
      <p id="d1e7733">For each component of the global carbon budget, we present results for three
different time periods: the full historical period, from 1850 to 2020; the
six decades in which we have atmospheric concentration records from Mauna
Loa (1960–2020), with a specific focus on last year (2020); and the projection
for the current year (2021). Subsequently, we assess the combined
constraints from the budget components (often referred to as a bottom-up
budget) against the top-down constraints from inverse modelling of
atmospheric observations. We do this for the global balance of the last
decade, as well as for a regional breakdown of land and ocean sinks by broad
latitude bands.
<?xmltex \hack{\newpage}?></p>
<sec id="Ch1.S3.SS1">
  <label>3.1</label><?xmltex \opttitle{Fossil CO${}_{{2}}$ emissions}?><title>Fossil CO<inline-formula><mml:math id="M493" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions</title>
<sec id="Ch1.S3.SS1.SSS1">
  <label>3.1.1</label><title>Historical period 1850–2020</title>
      <p id="d1e7761">Cumulative fossil CO<inline-formula><mml:math id="M494" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions for 1850–2020 were 455 <inline-formula><mml:math id="M495" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 25 GtC,
including the cement carbonation sink (Fig. 3, Table 8).</p>
      <p id="d1e7780">In this period, 46 % of fossil CO<inline-formula><mml:math id="M496" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions came from coal, 35 %
from oil, 14 % from natural gas, 3 % from decomposition of carbonates,
and 1 % from flaring.</p>
      <p id="d1e7792">In 1850, the UK accounted for 62 % of global fossil CO<inline-formula><mml:math id="M497" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions. In
1891 the combined cumulative emissions of the current members of the
European Union reached and subsequently surpassed the level of the UK. Since
1917 US cumulative emissions have been the largest. Over the entire period
1850–2020, US cumulative emissions amounted to 110 GtC (25 % of world
total), the EU's to 80 GtC (18 %), and China's to 60 GtC (14 %).</p>
      <p id="d1e7804">There are three additional global datasets that include all sources of
fossil CO<inline-formula><mml:math id="M498" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions: CDIAC-FF (Gilfillan and Marland, 2021), CEDS
version v_2021_04_21 (Hoesly et
al., 2018; O'Rourke et al., 2021), and PRIMAP-hist version 2.3.1
(Gütschow et al., 2016, 2021), although these datasets are not
independent. CDIAC-FF has the lowest cumulative emissions over 1750–2018 at
437 GtC, GCP has 443 GtC, CEDS 445 GtC, PRIMAP-hist TP 453 GtC, and
PRIMAP-hist CR 455 GtC. CDIAC-FF excludes emissions from lime production,
while neither CDIAC-FF nor GCP explicitly include emissions from
international bunker fuels prior to 1950. CEDS has higher emissions from
international shipping in recent years, while PRIMAP-hist has higher
fugitive emissions than the other datasets. However, in general these four
datasets are in relative agreement with total historical global emissions
of fossil CO<inline-formula><mml:math id="M499" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F4" specific-use="star"><?xmltex \currentcnt{4}?><?xmltex \def\figurename{Figure}?><label>Figure 4</label><caption><p id="d1e7828">Components of the global carbon budget and their uncertainties as
a function of time, presented individually for <bold>(a)</bold> fossil CO<inline-formula><mml:math id="M500" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
(<inline-formula><mml:math id="M501" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(b)</bold> growth rate in atmospheric CO<inline-formula><mml:math id="M502" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration
(<inline-formula><mml:math id="M503" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(c)</bold> emissions from land-use change (<inline-formula><mml:math id="M504" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(d)</bold> the land
CO<inline-formula><mml:math id="M505" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M506" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(e)</bold> the ocean CO<inline-formula><mml:math id="M507" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M508" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), and <bold>(f)</bold>
the budget imbalance that is not accounted for by the other terms. Positive
values of <inline-formula><mml:math id="M509" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M510" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> represent a flux from the atmosphere to
land or the ocean. All data are in GtC yr<inline-formula><mml:math id="M511" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> with the uncertainty bounds
representing <inline-formula><mml:math id="M512" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1 standard deviation in shaded colour. Data sources are
as in Fig. 3. The red dots indicate our projections for the year 2021 and
the red error bars the uncertainty in the projections (see methods). </p></caption>
            <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f04.png"/>

          </fig>

      <?xmltex \floatpos{t}?><fig id="Ch1.F5" specific-use="star"><?xmltex \currentcnt{5}?><?xmltex \def\figurename{Figure}?><label>Figure 5</label><caption><p id="d1e7992">Fossil CO<inline-formula><mml:math id="M513" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions for <bold>(a)</bold> the globe, including an
uncertainty of <inline-formula><mml:math id="M514" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>5 % (grey shading) and a projection through the
year 2021 (red dot and uncertainty range); <bold>(b)</bold> territorial (solid lines) and
consumption (dashed lines) emissions for the top three country emitters
(USA, China, India) and for the European Union (EU27); <bold>(c)</bold> global emissions
by fuel type, including coal, oil, gas, and cement, and cement minus cement
carbonation (dashed); and <bold>(d)</bold> per capita emissions the world and for the
large emitters as in panel <bold>(b)</bold>. Territorial emissions are primarily from
Gilfillan and Marland (2021) except national data for the USA and EU27 for
1990–2018, which are reported by the countries to the UNFCCC as detailed in
the text; consumption-based emissions are updated from Peters et al. (2011b). See Sect. 2.1 and Appendix C1 for details of the calculations
and data sources. </p></caption>
            <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f05.png"/>

          </fig>

</sec>
<sec id="Ch1.S3.SS1.SSS2">
  <label>3.1.2</label><title>Recent period 1960–2020</title>
      <p id="d1e8041">Global fossil CO<inline-formula><mml:math id="M515" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions, <inline-formula><mml:math id="M516" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (including the cement
carbonation sink), have increased every decade from an average of 3.0 <inline-formula><mml:math id="M517" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2 GtC yr<inline-formula><mml:math id="M518" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the decade of the 1960s to an average of 9.5 <inline-formula><mml:math id="M519" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M520" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during 2011–2020 (Table 6, Figs. 2, 4 and 5). The
growth rate in these emissions decreased between the 1960s and the 1990s,
from 4.3 % yr<inline-formula><mml:math id="M521" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the 1960s (1960–1969), 3.2 % yr<inline-formula><mml:math id="M522" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the
1970s (1970–1979), and 1.6 % yr<inline-formula><mml:math id="M523" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the 1980s (1980–1989), to 0.9 % yr<inline-formula><mml:math id="M524" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the 1990s (1990–1999). After this period, the growth rate began
increasing again in the 2000s at an average growth rate of 3.0 % yr<inline-formula><mml:math id="M525" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, decreasing to 0.6 % yr<inline-formula><mml:math id="M526" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the last decade (2011–2020).
China's emissions increased by <inline-formula><mml:math id="M527" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.0 % yr<inline-formula><mml:math id="M528" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> on average over the last
10 years, dominating the global trend, followed by India's emissions increase
by <inline-formula><mml:math id="M529" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.9 % yr<inline-formula><mml:math id="M530" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, while emissions decreased in EU27 by <inline-formula><mml:math id="M531" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.9 % yr<inline-formula><mml:math id="M532" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, and in the USA by <inline-formula><mml:math id="M533" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.1 % yr<inline-formula><mml:math id="M534" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. Figure 6 illustrates the
spatial distribution of fossil fuel emissions for the 2011–2020 period.</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F6" specific-use="star"><?xmltex \currentcnt{6}?><?xmltex \def\figurename{Figure}?><label>Figure 6</label><caption><p id="d1e8255">The 2011–2020 decadal mean components of the global carbon budget,
presented for <bold>(a)</bold> fossil CO<inline-formula><mml:math id="M535" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (<inline-formula><mml:math id="M536" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(b)</bold> land-use change
emissions (<inline-formula><mml:math id="M537" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(c)</bold> the ocean CO<inline-formula><mml:math id="M538" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M539" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), and <bold>(d)</bold>
the land CO<inline-formula><mml:math id="M540" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M541" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). Positive values for <inline-formula><mml:math id="M542" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M543" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> represent a flux to the atmosphere, whereas positive values of
<inline-formula><mml:math id="M544" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M545" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> represent a flux from the atmosphere to the ocean
or the land. In all panels, yellow/red (green/blue) colours represent a flux
from (into) the land–ocean to (from) the atmosphere. All units are in kgC m<inline-formula><mml:math id="M546" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> yr<inline-formula><mml:math id="M547" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. Note the different scales in each panel. <inline-formula><mml:math id="M548" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> data
shown are from GCP-GridFEDv2021.2. <inline-formula><mml:math id="M549" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> data shown are only from BLUE as
the updated H&amp;N2017 and OSCAR do not resolve gridded fluxes. <inline-formula><mml:math id="M550" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
data shown are the average of GOBMs and data product means, using GOBMs
simulation A; no adjustment for bias and drift is applied to the gridded fields
(see Sect. 2.4). <inline-formula><mml:math id="M551" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> data shown are the average of DGVMs for
simulation S2 (see Sect. 2.5).</p></caption>
            <?xmltex \igopts{width=412.564961pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f06.png"/>

          </fig>

      <p id="d1e8462"><inline-formula><mml:math id="M552" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> includes the uptake of CO<inline-formula><mml:math id="M553" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> by cement via carbonation which
has increased with increasing stocks of cement products, from an average of
20 MtC yr<inline-formula><mml:math id="M554" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (0.02 GtC yr<inline-formula><mml:math id="M555" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) in the 1960s to an average of 200 MtC yr<inline-formula><mml:math id="M556" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (0.2 GtC yr<inline-formula><mml:math id="M557" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) during 2011–2020 (Fig. 5).</p>
</sec>
<sec id="Ch1.S3.SS1.SSS3">
  <label>3.1.3</label><title>Final year 2020</title>
      <p id="d1e8540">Global fossil CO<inline-formula><mml:math id="M558" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions were 5.4 % lower in 2020 than in 2019,
because of the COVID-19 pandemic, with a decline of 0.5 GtC to reach 9.5 <inline-formula><mml:math id="M559" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC (9.3 <inline-formula><mml:math id="M560" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC when including the cement carbonation
sink) in 2020 (Fig. 5), distributed among coal (40 %), oil (32 %),
natural gas (21 %), cement (5 %), and others (2 %). Compared to the
previous year, 2020 emissions from coal, oil, and gas declined by 4.4 %,
9.7 %, and 2.3 % respectively, while emissions from cement increased by
0.8 %. All growth rates presented are adjusted for the leap year, unless
stated otherwise.</p>
      <p id="d1e8566">In 2020, the largest absolute contributions to global fossil CO<inline-formula><mml:math id="M561" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
emissions were from China (31 %), the USA (14 %), the EU27 (7 %), and
India (7 %). These four regions account for 59 % of global CO<inline-formula><mml:math id="M562" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
emissions, while the rest of the world contributed 41 %, including
international aviation and marine bunker fuels (2.9 % of the total).
Growth rates for these countries from 2019 to 2020 were <inline-formula><mml:math id="M563" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.4 % (China),
<inline-formula><mml:math id="M564" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>10.6 % (USA), <inline-formula><mml:math id="M565" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>10.9 % (EU27), and <inline-formula><mml:math id="M566" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>7.3 % (India), with <inline-formula><mml:math id="M567" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>7.0 % for
the rest of the world. The per capita fossil CO<inline-formula><mml:math id="M568" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions in 2020 were
1.2 tC person<inline-formula><mml:math id="M569" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> yr<inline-formula><mml:math id="M570" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the globe, and were 3.9 (USA), 2.0
(China), 1.6 (EU27) and 0.5 (India) tC per person per year for the four
highest emitting countries (Fig. 5).</p>
      <p id="d1e8656">The COVID-19-induced decline in emissions of <inline-formula><mml:math id="M571" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>5.4 % in 2020 is close to
the projected decline of <inline-formula><mml:math id="M572" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>6.7 %, which was the median of four approaches,
published in Friedlingstein et al. (2020) (Table 7). Of the four approaches, the “GCP”
method was closest at <inline-formula><mml:math id="M573" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>5.8 %. That method was based on national emissions
projections for China, the USA, the EU27, and India using reported monthly
activity data when available and projections of gross domestic product
corrected for trends in fossil fuel intensity (<inline-formula><mml:math id="M574" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) for the rest of
the world. Of the regions, the projection for the EU27 was the least accurate,
and the reasons for this are discussed by Andrew (2021).</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T6" specific-use="star"><?xmltex \currentcnt{5}?><label>Table 5</label><caption><p id="d1e8695">Comparison of results from the bookkeeping method and
budget residuals with results from the DGVMs and inverse estimates for
different periods, the last decade, and the last year available. All values
are in GtC yr<inline-formula><mml:math id="M575" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The DGVM uncertainties represent <inline-formula><mml:math id="M576" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M577" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> of the decadal or annual (for 2020 only) estimates from
the individual DGVMs: for the inverse models the range of available results
is given. All values are rounded to the nearest 0.1 GtC and therefore
columns do not necessarily add to zero. </p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.88}[.88]?><oasis:tgroup cols="8">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:colspec colnum="7" colname="col7" align="right"/>
     <oasis:colspec colnum="8" colname="col8" align="right"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry rowsep="1" namest="col2" nameend="col8" align="center">Mean (GtC yr<inline-formula><mml:math id="M580" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">1960s</oasis:entry>
         <oasis:entry colname="col3">1970s</oasis:entry>
         <oasis:entry colname="col4">1980s</oasis:entry>
         <oasis:entry colname="col5">1990s</oasis:entry>
         <oasis:entry colname="col6">2000s</oasis:entry>
         <oasis:entry colname="col7">2011–2020</oasis:entry>
         <oasis:entry colname="col8">2020</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col8">Land-use change emissions (<inline-formula><mml:math id="M581" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Bookkeeping method – net flux (1a)</oasis:entry>
         <oasis:entry colname="col2">1.6 <inline-formula><mml:math id="M582" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col3">1.3 <inline-formula><mml:math id="M583" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col4">1.2 <inline-formula><mml:math id="M584" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col5">1.3 <inline-formula><mml:math id="M585" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col6">1.2 <inline-formula><mml:math id="M586" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col7">1.1 <inline-formula><mml:math id="M587" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col8">0.9 <inline-formula><mml:math id="M588" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Bookkeeping method – source</oasis:entry>
         <oasis:entry colname="col2">3.4 <inline-formula><mml:math id="M589" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
         <oasis:entry colname="col3">3.3 <inline-formula><mml:math id="M590" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col4">3.4 <inline-formula><mml:math id="M591" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col5">3.6 <inline-formula><mml:math id="M592" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
         <oasis:entry colname="col6">3.7 <inline-formula><mml:math id="M593" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
         <oasis:entry colname="col7">3.8 <inline-formula><mml:math id="M594" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
         <oasis:entry colname="col8">3.6 <inline-formula><mml:math id="M595" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Bookkeeping method – sink</oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M596" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.9 <inline-formula><mml:math id="M597" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M598" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.0 <inline-formula><mml:math id="M599" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M600" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.1 <inline-formula><mml:math id="M601" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M602" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.3 <inline-formula><mml:math id="M603" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M604" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.5 <inline-formula><mml:math id="M605" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M606" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.7 <inline-formula><mml:math id="M607" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M608" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.8 <inline-formula><mml:math id="M609" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">DGVMs – net flux (1b)</oasis:entry>
         <oasis:entry colname="col2">1.6 <inline-formula><mml:math id="M610" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col3">1.3 <inline-formula><mml:math id="M611" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col4">1.4 <inline-formula><mml:math id="M612" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col5">1.4 <inline-formula><mml:math id="M613" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col6">1.4 <inline-formula><mml:math id="M614" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col7">1.5 <inline-formula><mml:math id="M615" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col8">1.4 <inline-formula><mml:math id="M616" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col8">Terrestrial sink (<inline-formula><mml:math id="M617" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Residual sink from global budget (<inline-formula><mml:math id="M618" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub><mml:mo>-</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">1.8 <inline-formula><mml:math id="M619" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col3">1.9 <inline-formula><mml:math id="M620" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col4">1.6 <inline-formula><mml:math id="M621" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
         <oasis:entry colname="col5">2.5 <inline-formula><mml:math id="M622" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
         <oasis:entry colname="col6">2.7 <inline-formula><mml:math id="M623" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
         <oasis:entry colname="col7">2.8 <inline-formula><mml:math id="M624" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
         <oasis:entry colname="col8">2.1 <inline-formula><mml:math id="M625" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M626" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) (2a)</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">DGVMs (2b)</oasis:entry>
         <oasis:entry colname="col2">1.2 <inline-formula><mml:math id="M627" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col3">2.0 <inline-formula><mml:math id="M628" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col4">1.8 <inline-formula><mml:math id="M629" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col5">2.3 <inline-formula><mml:math id="M630" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col6">2.6 <inline-formula><mml:math id="M631" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col7">3.1 <inline-formula><mml:math id="M632" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
         <oasis:entry colname="col8">2.9 <inline-formula><mml:math id="M633" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1.0</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col8">Total land fluxes (<inline-formula><mml:math id="M634" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GCB2021 Budget (2b-1a)</oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M635" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.4 <inline-formula><mml:math id="M636" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col3">0.8 <inline-formula><mml:math id="M637" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col4">0.5 <inline-formula><mml:math id="M638" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
         <oasis:entry colname="col5">1.0 <inline-formula><mml:math id="M639" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col6">1.4 <inline-formula><mml:math id="M640" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
         <oasis:entry colname="col7">1.9 <inline-formula><mml:math id="M641" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
         <oasis:entry colname="col8">2.0 <inline-formula><mml:math id="M642" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1.2</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Budget constraint (2a-1a)</oasis:entry>
         <oasis:entry colname="col2">0.2 <inline-formula><mml:math id="M643" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col3">0.6 <inline-formula><mml:math id="M644" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col4">0.3 <inline-formula><mml:math id="M645" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col5">1.2 <inline-formula><mml:math id="M646" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col6">1.5 <inline-formula><mml:math id="M647" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
         <oasis:entry colname="col7">1.7 <inline-formula><mml:math id="M648" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
         <oasis:entry colname="col8">1.3 <inline-formula><mml:math id="M649" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">DGVMs – net (2b-1b)</oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M650" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.4 <inline-formula><mml:math id="M651" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
         <oasis:entry colname="col3">0.7 <inline-formula><mml:math id="M652" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col4">0.3 <inline-formula><mml:math id="M653" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col5">0.9 <inline-formula><mml:math id="M654" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col6">1.2 <inline-formula><mml:math id="M655" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col7">1.6 <inline-formula><mml:math id="M656" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
         <oasis:entry colname="col8">1.5 <inline-formula><mml:math id="M657" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Inversions<inline-formula><mml:math id="M658" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">–</oasis:entry>
         <oasis:entry colname="col3">–</oasis:entry>
         <oasis:entry colname="col4">0.5–0.6 (2)</oasis:entry>
         <oasis:entry colname="col5">0.9–1.2 (3)</oasis:entry>
         <oasis:entry colname="col6">1.3–1.8 (3)</oasis:entry>
         <oasis:entry colname="col7">1.3–2.0 (6)</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M659" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.1–1.3 (6)</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table><table-wrap-foot><p id="d1e8724"><inline-formula><mml:math id="M578" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula> Estimates are adjusted for the pre-industrial influence of river fluxes, for the cement carbonation sink, and adjusted to common <inline-formula><mml:math id="M579" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Sect. 2.6). The ranges given include<?xmltex \hack{\break}?> varying numbers (in parentheses) of inversions in each decade (Table A4).</p></table-wrap-foot></table-wrap>

</sec>
<sec id="Ch1.S3.SS1.SSS4">
  <label>3.1.4</label><title>Year 2021 projection</title>
      <p id="d1e9738">Globally, we estimate that global fossil CO<inline-formula><mml:math id="M660" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions will rebound
4.8 % in 2021 (4.2 % to 5.4 %) to 9.9 GtC (36.4 GtCO<inline-formula><mml:math id="M661" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>), returning to
near their 2019 emission levels of 10.0 GtC (36.7 GtCO<inline-formula><mml:math id="M662" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>). Global
increases in 2021 emissions per fuel types are <inline-formula><mml:math id="M663" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>6.3 % (range 5.5 % to
7.0 %) for coal, <inline-formula><mml:math id="M664" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.0 % (range 2.6 % to 5.4 %) for oil, <inline-formula><mml:math id="M665" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.8 %
(range 2.8 % to 4.8 %) for natural gas, and <inline-formula><mml:math id="M666" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.2 % (range 1.7 % to
4.6 %) for cement.</p>
      <p id="d1e9797">For China, projected fossil emissions in 2021 are expected to increase by
4.3 % (range 3.0 % to 5.4 %) compared with 2020 emissions, bringing
2021 emissions for China to around 3.0 GtC yr<inline-formula><mml:math id="M667" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (11.1 GtCO<inline-formula><mml:math id="M668" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M669" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). Chinese emissions appear to have risen in both 2020 and 2021
despite the economic disruptions of COVID-19. Increases in fuel-specific
projections for China are <inline-formula><mml:math id="M670" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.1 % for coal, <inline-formula><mml:math id="M671" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.4 % for oil,
<inline-formula><mml:math id="M672" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>12.8 % natural gas, and a decrease of 0.1 % for cement.</p>
      <p id="d1e9855">For the USA, the Energy Information Administration (EIA) emissions
projection for 2021 combined with cement clinker data from USGS gives an
increase of 6.8 % (range 6.6 % to 7.0 %) compared to 2020, bringing
USA 2021 emissions to around 1.4 GtC yr<inline-formula><mml:math id="M673" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (5.0 GtCO<inline-formula><mml:math id="M674" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M675" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). This
is based on separate projections for coal of <inline-formula><mml:math id="M676" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>17.1 %, oil <inline-formula><mml:math id="M677" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>9.0 %,
natural gas <inline-formula><mml:math id="M678" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.8 %, and cement <inline-formula><mml:math id="M679" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.3 %.</p>
      <p id="d1e9920">For the European Union, our projection for 2021 is for an increase of
6.3 % (range 4.3 % to 8.3 %) over 2020, with 2021 emissions around 0.8 GtC yr<inline-formula><mml:math id="M680" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (2.8 GtCO<inline-formula><mml:math id="M681" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M682" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). This is based on separate
projections for coal of <inline-formula><mml:math id="M683" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>14.6 %, oil <inline-formula><mml:math id="M684" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.7 %, natural gas <inline-formula><mml:math id="M685" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.6 %,
and cement <inline-formula><mml:math id="M686" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.3 %.</p>
      <p id="d1e9986">For India, our projection for 2021 is an increase of 11.2 % (range of
10.7 % to 11.7 %) over 2020, with 2021 emissions around 0.7 GtC yr<inline-formula><mml:math id="M687" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (2.7 GtCO<inline-formula><mml:math id="M688" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> yr<inline-formula><mml:math id="M689" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). This is based on separate projections
for coal of <inline-formula><mml:math id="M690" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>13.9 %, oil <inline-formula><mml:math id="M691" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.4 %, natural gas <inline-formula><mml:math id="M692" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.8 %, and cement
<inline-formula><mml:math id="M693" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>21.6 %.</p>
      <p id="d1e10051">For the rest of the world, the expected growth rate for 2021 is 3.2 %
(range 2.0 % to 4.3 %). This is computed using the GDP projection for
the world (excluding China, the USA, the EU, and India) of 4.4 % made by
the IMF (2022) and a decrease in <inline-formula><mml:math id="M694" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of <inline-formula><mml:math id="M695" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.7 % yr<inline-formula><mml:math id="M696" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, which is
the average over 2011–2020. The uncertainty range is based on the standard
deviation of the interannual variability in <inline-formula><mml:math id="M697" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> during 2011–2020 of
0.6 % yr<inline-formula><mml:math id="M698" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and our estimates of uncertainty in the IMF's GDP forecast
of 0.6 %. The methodology allows independent projections for coal, oil,
natural gas, cement, and other components, which add to the total emissions
in the rest of the world. The fuel-specific projected 2021 growth rates for
the rest of the world are: <inline-formula><mml:math id="M699" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.2 % (range 0.7 % to 5.8 %) for coal,
<inline-formula><mml:math id="M700" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>2.3 % (<inline-formula><mml:math id="M701" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.3 % to <inline-formula><mml:math id="M702" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.9 %) for oil, <inline-formula><mml:math id="M703" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.1 % (2.6 % to 5.7 %)
for natural gas, and <inline-formula><mml:math id="M704" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.8 % (<inline-formula><mml:math id="M705" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>2.7 % to <inline-formula><mml:math id="M706" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>6.9 %) for cement.</p>
      <p id="d1e10165">Independently, the IEA has published two forecasts of global fossil energy
CO<inline-formula><mml:math id="M707" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (i.e. a subset of fossil CO<inline-formula><mml:math id="M708" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions), the first in
April (4.8 %; IEA, 2021a) which was then revised in October to 4 % (IEA, 2021b).
In March 2022 they also published a new, preliminary estimate of 6 %
growth (IEA, 2021a). Carbon Monitor produces estimates of global emissions
with low temporal lag, and their estimates suggest that emissions were
5.1 % higher than in 2020 (Carbon Monitor, 2022).</p>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T7" specific-use="star"><?xmltex \currentcnt{6}?><label>Table 6</label><caption><p id="d1e10189">Decadal mean in the five components of the anthropogenic
CO<inline-formula><mml:math id="M709" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> budget for different periods, and last year available. All values are in
GtC yr<inline-formula><mml:math id="M710" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, and uncertainties are reported as <inline-formula><mml:math id="M711" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M712" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>.
Fossil CO<inline-formula><mml:math id="M713" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions include cement carbonation. The
table also shows the budget imbalance (<inline-formula><mml:math id="M714" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), which
provides a measure of the discrepancies among the nearly independent
estimates and has an uncertainty exceeding <inline-formula><mml:math id="M715" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1 GtC yr<inline-formula><mml:math id="M716" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. A positive imbalance means the emissions are
overestimated and/or the sinks are too small. All values are rounded to the
nearest 0.1 GtC and therefore columns do not necessarily add to zero.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.88}[.88]?><oasis:tgroup cols="9">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:colspec colnum="7" colname="col7" align="right"/>
     <oasis:colspec colnum="8" colname="col8" align="right"/>
     <oasis:colspec colnum="9" colname="col9" align="right"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry rowsep="1" namest="col2" nameend="col9" align="center">Mean (GtC yr<inline-formula><mml:math id="M732" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">1960s</oasis:entry>
         <oasis:entry colname="col3">1970s</oasis:entry>
         <oasis:entry colname="col4">1980s</oasis:entry>
         <oasis:entry colname="col5">1990s</oasis:entry>
         <oasis:entry colname="col6">2000s</oasis:entry>
         <oasis:entry colname="col7">2011–</oasis:entry>
         <oasis:entry colname="col8">2020</oasis:entry>
         <oasis:entry colname="col9">2021</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">2020</oasis:entry>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9">(Projection)</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry namest="col1" nameend="col9">Total emissions (<inline-formula><mml:math id="M733" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Fossil CO<inline-formula><mml:math id="M734" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (<inline-formula><mml:math id="M735" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)<inline-formula><mml:math id="M736" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">3.0 <inline-formula><mml:math id="M737" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2</oasis:entry>
         <oasis:entry colname="col3">4.7 <inline-formula><mml:math id="M738" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2</oasis:entry>
         <oasis:entry colname="col4">5.5 <inline-formula><mml:math id="M739" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3</oasis:entry>
         <oasis:entry colname="col5">6.3 <inline-formula><mml:math id="M740" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3</oasis:entry>
         <oasis:entry colname="col6">7.7 <inline-formula><mml:math id="M741" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col7">9.5 <inline-formula><mml:math id="M742" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col8">9.3 <inline-formula><mml:math id="M743" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col9">9.9 <inline-formula><mml:math id="M744" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Land-use change emissions (<inline-formula><mml:math id="M745" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">1.6 <inline-formula><mml:math id="M746" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col3">1.3 <inline-formula><mml:math id="M747" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col4">1.2 <inline-formula><mml:math id="M748" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col5">1.3 <inline-formula><mml:math id="M749" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col6">1.2 <inline-formula><mml:math id="M750" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col7">1.1 <inline-formula><mml:math id="M751" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col8">0.9 <inline-formula><mml:math id="M752" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col9">0.8 <inline-formula><mml:math id="M753" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Total emissions</oasis:entry>
         <oasis:entry colname="col2">4.6 <inline-formula><mml:math id="M754" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col3">5.9 <inline-formula><mml:math id="M755" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7</oasis:entry>
         <oasis:entry colname="col4">6.7 <inline-formula><mml:math id="M756" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col5">7.7 <inline-formula><mml:math id="M757" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col6">9.0 <inline-formula><mml:math id="M758" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col7">10.6 <inline-formula><mml:math id="M759" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col8">10.2 <inline-formula><mml:math id="M760" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8</oasis:entry>
         <oasis:entry colname="col9">10.7 <inline-formula><mml:math id="M761" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col9">Partitioning </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Growth rate in atmospheric CO<inline-formula><mml:math id="M762" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math id="M763" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">1.7 <inline-formula><mml:math id="M764" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.07</oasis:entry>
         <oasis:entry colname="col3">2.8 <inline-formula><mml:math id="M765" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.07</oasis:entry>
         <oasis:entry colname="col4">3.4 <inline-formula><mml:math id="M766" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.02</oasis:entry>
         <oasis:entry colname="col5">3.1 <inline-formula><mml:math id="M767" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.02</oasis:entry>
         <oasis:entry colname="col6">4.0 <inline-formula><mml:math id="M768" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.02</oasis:entry>
         <oasis:entry colname="col7">5.1 <inline-formula><mml:math id="M769" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.02</oasis:entry>
         <oasis:entry colname="col8">5.0 <inline-formula><mml:math id="M770" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2</oasis:entry>
         <oasis:entry colname="col9">5.3 <inline-formula><mml:math id="M771" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.1</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Ocean sink (<inline-formula><mml:math id="M772" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">1.1 <inline-formula><mml:math id="M773" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col3">1.3 <inline-formula><mml:math id="M774" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col4">1.8 <inline-formula><mml:math id="M775" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col5">2.0 <inline-formula><mml:math id="M776" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col6">2.2 <inline-formula><mml:math id="M777" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col7">2.8 <inline-formula><mml:math id="M778" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col8">3.0 <inline-formula><mml:math id="M779" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col9">2.9 <inline-formula><mml:math id="M780" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Terrestrial sink (<inline-formula><mml:math id="M781" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">1.2 <inline-formula><mml:math id="M782" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col3">2.0 <inline-formula><mml:math id="M783" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col4">1.8 <inline-formula><mml:math id="M784" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col5">2.3 <inline-formula><mml:math id="M785" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4</oasis:entry>
         <oasis:entry colname="col6">2.6 <inline-formula><mml:math id="M786" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5</oasis:entry>
         <oasis:entry colname="col7">3.1 <inline-formula><mml:math id="M787" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6</oasis:entry>
         <oasis:entry colname="col8">2.9 <inline-formula><mml:math id="M788" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1.0</oasis:entry>
         <oasis:entry colname="col9">3.3 <inline-formula><mml:math id="M789" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1.0</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col9">Budget imbalance </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M790" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub><mml:mo>-</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">0.6</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M791" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.2</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M792" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.2</oasis:entry>
         <oasis:entry colname="col5">0.2</oasis:entry>
         <oasis:entry colname="col6">0.1</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M793" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.3</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M794" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.8</oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M795" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.7</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M796" display="inline"><mml:mrow><mml:mo>(</mml:mo><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table><table-wrap-foot><p id="d1e10267"><inline-formula><mml:math id="M717" display="inline"><mml:msup><mml:mi/><mml:mo>*</mml:mo></mml:msup></mml:math></inline-formula> Fossil emissions excluding the cement carbonation sink amount to 3.1 <inline-formula><mml:math id="M718" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2 GtC yr<inline-formula><mml:math id="M719" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 4.7 <inline-formula><mml:math id="M720" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2 GtC yr<inline-formula><mml:math id="M721" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 5.5 <inline-formula><mml:math id="M722" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M723" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 6.4 <inline-formula><mml:math id="M724" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M725" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, 7.9 <inline-formula><mml:math id="M726" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M727" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, <?xmltex \hack{\break}?>and 9.7 <inline-formula><mml:math id="M728" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M729" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the decades 1960s to 2010s respectively and to 9.5 <inline-formula><mml:math id="M730" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M731" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for 2020.</p></table-wrap-foot></table-wrap>

</sec>
</sec>
<sec id="Ch1.S3.SS2">
  <label>3.2</label><title>Emissions from land-use changes</title>
<sec id="Ch1.S3.SS2.SSS1">
  <label>3.2.1</label><title>Historical period 1850–2020</title>
      <p id="d1e11314">Cumulative CO<inline-formula><mml:math id="M797" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from land-use changes (<inline-formula><mml:math id="M798" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) for
1850–2020 were 200 <inline-formula><mml:math id="M799" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 65 GtC (Table 8; Figs. 3, 13). The cumulative
emissions from <inline-formula><mml:math id="M800" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are particularly uncertain, with large spread among
individual estimates of 140 GtC (updated H&amp;N2017), 270 GtC (BLUE), and
195 GtC (OSCAR) for the three bookkeeping models and a similar wide estimate
of 190 <inline-formula><mml:math id="M801" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 60 GtC for the DGVMs (all cumulative numbers are rounded to
the nearest 5 GtC). These estimates are broadly consistent with indirect
constraints from vegetation biomass observations, giving a cumulative source
of 155 <inline-formula><mml:math id="M802" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 50 GtC over the 1901–2012 period (Li et al., 2017). However,
given the large spread, a best estimate is difficult to ascertain.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS2">
  <label>3.2.2</label><title>Recent period 1960–2020</title>
      <p id="d1e11378">In contrast to growing fossil emissions, CO<inline-formula><mml:math id="M803" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from land use,
land-use change, and forestry have remained relatively constant, at around
1.3 <inline-formula><mml:math id="M804" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M805" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> over the 1970–1999 period, and even show a
slight decrease over the last 20 years, reaching 1.1 <inline-formula><mml:math id="M806" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M807" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the 2011–2020 period (Table 6, Fig. 4), but with large spread across
estimates (Table 5, Fig. 7). Emissions have been relatively constant in the DGVMs
ensemble of models since the 1970s, with similar mean values until the 1990s
as the bookkeeping mean and large model spread (Table 5, Fig. 7). The DGVMs
average grows larger than the bookkeeping average in the recent decades and
shows no sign of decreasing emissions, which is, however, expected as
DGVM-based estimates include the loss of additional sink capacity, which
grows with time, while the bookkeeping estimates do not (Appendix D4).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F7" specific-use="star"><?xmltex \currentcnt{7}?><?xmltex \def\figurename{Figure}?><label>Figure 7</label><caption><p id="d1e11430">CO<inline-formula><mml:math id="M808" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> exchanges between the atmosphere and the terrestrial
biosphere as used in the global carbon budget (black with <inline-formula><mml:math id="M809" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M810" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>
uncertainty in grey shading in all panels). <bold>(a)</bold> CO<inline-formula><mml:math id="M811" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from
land-use change (<inline-formula><mml:math id="M812" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) with estimates from the three bookkeeping models
(yellow lines) and DGVMs (green) shown individually, with DGVM
ensemble means (dark green). The dashed line identifies the pre-satellite
period before the inclusion of peatland burning. <bold>(b)</bold> CO<inline-formula><mml:math id="M813" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> gross sinks
(positive, from regrowth after agricultural abandonment and wood harvesting)
and gross sources (negative, from decaying material left dead on site,
products after clearing of natural vegetation for agricultural purposes,
wood harvesting, and for BLUE, degradation from primary to secondary land
through usage of natural vegetation as rangeland, and also from emissions
from peat drainage and peat burning) from the three bookkeeping models
(yellow lines). The sum of the gross sinks and sources is <inline-formula><mml:math id="M814" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> shown in
panel <bold>(a)</bold>. <bold>(c)</bold> Land CO<inline-formula><mml:math id="M815" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M816" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) with individual DGVM
estimates (green). <bold>(d)</bold> Total atmosphere–land CO<inline-formula><mml:math id="M817" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes (<inline-formula><mml:math id="M818" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M819" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>
<inline-formula><mml:math id="M820" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), with individual DGVMs (green) and their multi-model mean (dark
green).</p></caption>
            <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f07.png"/>

          </fig>

      <p id="d1e11578"><inline-formula><mml:math id="M821" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is a net term of various gross fluxes, which comprise emissions
and removals. Gross emissions are on average 2–4 times larger than the net
<inline-formula><mml:math id="M822" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions, and remained largely constant over the last 60 years,
with a moderate increase from an average of 3.4 <inline-formula><mml:math id="M823" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9 GtC yr<inline-formula><mml:math id="M824" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
for the decade of the 1960s to an average of 3.8 <inline-formula><mml:math id="M825" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6 GtC yr<inline-formula><mml:math id="M826" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
during 2011–2020 (Fig. 7, Table 5), showing the relevance of land management
such as harvesting or rotational agriculture. Increases in gross removals,
from 1.9 <inline-formula><mml:math id="M827" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M828" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the 1960s to 2.7 <inline-formula><mml:math id="M829" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M830" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for 2011–2020, were larger than the increase in gross emissions.
Since the processes behind gross removals, foremost forest regrowth and soil
recovery, are all slow, while gross emissions include a large instantaneous
component, short-term changes in land-use dynamics, such as a temporary
decrease in deforestation, influence gross emissions dynamics more than
gross removal dynamics. It is these relative changes to each other that
explain the decrease in net <inline-formula><mml:math id="M831" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions over the last two decades
and the last few years. Gross fluxes differ more across the three
bookkeeping estimates than net fluxes, which is expected due to different
process representation; in particular, treatment of shifting cultivation,
which increases both gross emissions and removals, differs across models.</p>
      <p id="d1e11691">There is a decrease in net CO<inline-formula><mml:math id="M832" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from land-use change over the
last decade (Fig. 7, Table 6), in contrast to earlier estimates of no clear
trend across <inline-formula><mml:math id="M833" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimates (Friedlingstein et al., 2020; Hong et al.,
2021). The trend in the last decade is now about <inline-formula><mml:math id="M834" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>4 % yr<inline-formula><mml:math id="M835" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, compared
to the <inline-formula><mml:math id="M836" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.8 % yr<inline-formula><mml:math id="M837" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> reported by Friedlingstein et al. (2020). This
decrease is principally attributable to changes in <inline-formula><mml:math id="M838" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimates from
BLUE and OSCAR, which relate to changes in the underlying land-use forcing,
LUH2 (Chini et al., 2021; Hurtt et al., 2020), based on HYDE3.3 (Klein
Goldewijk et al., 2017a, b): HYDE3.3 now incorporates updated estimates of
agricultural areas by the FAO and uses multi-annual land-cover maps from
satellite remote sensing (ESA CCI Land Cover) to constrain contemporary land-cover patterns (see Appendix C2.2 for details). These changes lead to
lower global <inline-formula><mml:math id="M839" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimates in the last two decades compared to earlier
versions of the global carbon budget due most notably to lower emissions
from cropland expansion, particularly in the tropical regions. Rosan et al. (2021) showed that for Brazil, the new HYDE3.3 version is closer to
independent, regional estimates of land-use and land-cover change
(MapBiomas, 2021) with respect to spatial patterns, but it shows less
land-use and land-cover changes than these independent estimates, while
HYDE3.2-based estimates had shown higher changes and lower emissions. The
update in land-use forcing leads to a decrease in estimated emissions in
Brazil across several models after the documented deforestation peak of
2003–2004 that preceded policies and monitoring systems decreasing
deforestation rates (Rosan et al., 2021). However, estimated emissions based
on the new land-use forcing do not reflect the rise in Brazilian
deforestation in the last few years (Silva Junior et al., 2021), and associated
increasing emissions from deforestation would have been missed here. The
update in FAO agricultural areas in Brazil also implied that substantial
interannual variability reported to earlier FAO assessment and captured by
the HYDE3.2 version since 2000 was removed. Due to the asymmetry of (fast)
decay (like clearing by fire) and (slower) regrowth, such reduced
variability is expected to decrease annual emissions. Also, the approach by
Houghton and Nassikas (2017) smooths land-use area changes before
calculating carbon fluxes by a 5-year running mean, hence the three emission
estimates are in better agreement than in previous GCB estimates. However,
differences still exist, which highlight the need for accurate knowledge of
land-use transitions and their spatial and temporal variability. A further
caveat is that global land-use change data for model input does not capture
forest degradation, which often occurs on small scales or without forest
cover changes easily detectable from remote sensing and poses a growing
threat to forest area and carbon stocks that may surpass deforestation
effects (e.g. Matricardi et al., 2020; Qin et al., 2021).</p>
      <p id="d1e11775">Overall, therefore, we assign low confidence to the change towards a
decreasing trend of land-use emissions over the last two decades as seen
compared to the estimate of the global carbon budget 2020 (Friedlingstein et
al., 2020). Our approach aims at using the most up-to-date data and methods,
such as accounting for revisions of living databases of country-level
agricultural statistics from FAO or including satellite remote-sensing
information for spatial allocation. While we start from a well-documented
methodology to provide gridded land-use data (Chini et al., 2021), not all
changes in individual components are always documented, complicating the
explanation of changes from one GCB to the next. The rising number of
pan-tropical or global estimates of carbon stock changes based on satellite
remote sensing of carbon densities and forest cover changes (Fan et al., 2019; Qin et al., 2021; Xu et al., 2022; Feng et al., 2022) may seem a
promising path for independent evaluation of the land-use emissions term.
However, comparison of satellite-derived fluxes to global model estimates is
hampered for several reasons discussed by Pongratz et al. (2021). Most
importantly, satellite-based estimates usually do not distinguish between
anthropogenic drivers and natural forest cover losses (e.g. from drought or
natural wildfires), which have also increased over time in some regions,
including the tropics; ancillary information would be needed to attribute
the observed signal of vegetation or carbon stock change to different
drivers. Further, satellite-based estimates often only provide sub-component
fluxes of <inline-formula><mml:math id="M840" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, excluding soil or product pool changes. Since forest
cover loss is better detectable from space than regrowth, satellite-based
products often limit their estimates to emissions from forest loss,
neglecting carbon uptake from regrowth of forests, as may occur following
wood harvesting, abandonment, or natural disturbances; such products thus
provide a subset of the gross emissions term (Fig. 7b) and cannot be
compared to net emissions. Lastly, satellite-based fluxes typically quantify
committed instead of actual emissions, i.e. legacy CO<inline-formula><mml:math id="M841" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes from
potentially slow processes such as slash, soil carbon or product decay, or
forest regrowth are not captured at the time they actually occur but are
attributed to the time of the land-use change event (Pongratz et al., 2021).
Using data on drivers of forest cover loss to isolate fluxes from
agricultural expansion, and looking into gross emissions instead of the net
land-use change flux, Feng et al. (2022) suggest a stronger increase in
global gross emissions (though generally a smaller flux) than the
bookkeeping models do (see gross fluxes in Fig. 7b). This is in line with
Rosan et al. (2021) suggesting that the trend of net emissions in Brazil may
be underestimated by the updated land-use data (though patterns have
improved). Further studies are needed to robustly estimate the trend of
global net land-use emissions. Progress is also needed on accurate
quantifications of land-use dynamics, including less well observable
management types such as shifting cultivation and wood harvesting, and their
distinction from natural disturbances (Pongratz et al., 2021).</p>
      <p id="d1e11798">The highest land-use emissions occur in the tropical regions of all three
continents, including the Arc of Deforestation in the Amazon basin (Fig. 6b). This is related to massive expansion of cropland, particularly in the
last few decades in Latin America, Southeast Asia, and sub-Saharan Africa (Hong et al., 2021), to a substantial extent for export (Pendrill et
al., 2019). Emission intensity is high in many tropical countries,
particularly of Southeast Asia, due to high rates of land conversion in
regions of carbon-dense and often still pristine, undegraded natural forests
(Hong et al., 2021). Emissions are further increased by peat fires in
equatorial Asia (GFED4s, van der Werf et al., 2017). Uptake due to land-use
change occurs, particularly in Europe, partly related to expanding forest
area as a consequence of the forest transition in the 19th and
20th century and subsequent regrowth of forest (Fig. 6b) (Mather, 2001;
McGrath et al., 2015).</p>
      <p id="d1e11801">While the mentioned patterns are robust and supported by independent literature, we acknowledge that model spread is substantially larger on regional
than on global level, as has been shown for bookkeeping models (Bastos et al.,
2021) as well as DGVMs (Obermeier et al., 2021). A detailed analysis of
country-level or regional uncertainties globally is beyond the scope of this
study. Assessments for individual regions will be performed as part of
REgional Carbon Cycle Assessment and Processes (RECCAP2; Ciais et al., 2022)
or already exist for selected regions (e.g. for Europe Petrescu et al.,
2020, for Brazil Rosan et al., 2021).</p>
      <p id="d1e11804">National GHG inventory data (NGHGI) under the LULUCF sector or data
submitted by countries to FAOSTAT differ from the global models' definition
of <inline-formula><mml:math id="M842" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> we adopt here in that in the NGHGI reporting, the natural
fluxes (<inline-formula><mml:math id="M843" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) are counted towards <inline-formula><mml:math id="M844" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> when they occur on managed
land (Grassi et al., 2018). In order to compare our results to the NGHGI
approach, we perform a re-mapping of our <inline-formula><mml:math id="M845" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate by including the
<inline-formula><mml:math id="M846" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> over managed forest from the DGVM simulations (following Grassi
et al., 2021) to the bookkeeping <inline-formula><mml:math id="M847" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate (see Appendix C2.3).
For the 2011–2020 period, we estimate that 1.5 GtC yr<inline-formula><mml:math id="M848" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> of <inline-formula><mml:math id="M849" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
occurred on managed forests and is then reallocated to <inline-formula><mml:math id="M850" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> here, as
done in the NGHGI method. Doing so, our mean estimate of <inline-formula><mml:math id="M851" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is
reduced from a source of 1.1 GtC to a sink of <inline-formula><mml:math id="M852" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.4 GtC, very similar to the
NGHGI estimate of <inline-formula><mml:math id="M853" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.6 GtC (Table A8).</p>
      <p id="d1e11934">Though estimates between GHGI, FAOSTAT, individual process-based models, and
the mapped budget estimates still differ in value and need further analysis,
the approach taken here provides a possibility to relate the global models'
and NGHGI approach to each other routinely and thus link the anthropogenic
carbon budget estimates of land CO<inline-formula><mml:math id="M854" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes directly to the Global
Stocktake, as part of the UNFCCC Paris Agreement.</p>
</sec>
<sec id="Ch1.S3.SS2.SSS3">
  <label>3.2.3</label><title>Final year 2020</title>
      <p id="d1e11954">The global CO<inline-formula><mml:math id="M855" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from land-use change are estimated as 0.9 <inline-formula><mml:math id="M856" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC in 2020, 0.2 GtC lower than 2019, which had featured
particularly large peat and tropical deforestation and degradation fires. The
surge in deforestation fires in the Amazon, causing about 30 % higher
emissions from deforestation and degradation fires in 2019 over the previous
decade, continued into 2020 (GFED4.1s, van der Werf et al., 2017). However,
the unusually dry conditions for a non-El Niño year that occurred in
Indonesia in 2019 and led to fire emissions from peat burning, deforestation,
and degradation in equatorial Asia to be about twice as large as the average
over the previous decade (GFED4.1s, van der Werf et al., 2017) ceased in
2020. However, confidence in the annual change remains low. While the
mentioned fires are clearly attributable to land-use activity, foremost
deforestation and peat burning, and may have been reinforced by dry weather
conditions, as was the case in Indonesia in 2019, wildfires also occur
naturally. In particular, the extreme fire events in recent years in
Australia, Siberia, and California were unrelated to land-use change and are
thus not attributed to <inline-formula><mml:math id="M857" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, but to the natural land sink, and are
discussed in Sect. 3.6.2.</p>
      <p id="d1e11984">Land-use change and related emissions may have been affected by the COVID-19
pandemic (e.g. Poulter et al., 2021). Although emissions from tropical
deforestation and degradation fires have been decreasing from 2019 to 2020
on the global scale, they increased in Latin America (GFED4s; van der Werf
et al., 2017). During the period of the pandemic, environmental protection
policies and their implementation may have been weakened in Brazil (Vale et
al., 2021). In other countries, too, monitoring capacities and legal
enforcement of measures to reduce tropical deforestation have been reduced
due to budget restrictions of environmental agencies or impairments to
ground-based monitoring that prevents land grabs and tenure conflicts
(Brancalion et al., 2020; Amador-Jiménez et al., 2020). Effects of the
pandemic on trends in fire activity or forest cover changes are hard to
separate from those of general political developments and environmental
changes, and the long-term consequences of disruptions in agricultural and
forestry economic activities (e.g. Gruère and Brooks, 2020; Golar et
al., 2020; Beckman and Countryman, 2021) remain to be seen.
<?xmltex \hack{\newpage}?></p>
</sec>
<sec id="Ch1.S3.SS2.SSS4">
  <label>3.2.4</label><title>Year 2021 projection</title>
      <p id="d1e11996">With wet conditions in Indonesia and a below-average fire season in South
America our preliminary estimate of <inline-formula><mml:math id="M858" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for 2021 is substantially
lower than the 2011–2020 average. By the end of September 2021 emissions
from tropical deforestation and degradation fires were estimated to be 222
TgC, down from 347 TgC in 2019 and 288 in 2020 (315 TgC 1997–2020 average).
Peat fire emissions in equatorial Asia were estimated to be 1 TgC, down from
117 TgC in 2019 and 2 TgC in 2020 (74 TgC 1997–2020 average) (GFED4.1s, van
der Werf et al., 2017). Based on the fire emissions until the end of
September, we expect <inline-formula><mml:math id="M859" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> emissions of around 0.8 GtC in 2021. Note
that although our extrapolation is based on tropical deforestation and
degradation fires, degradation attributable to selective logging,
edge effects, or fragmentation will not be captured.</p>
</sec>
</sec>
<sec id="Ch1.S3.SS3">
  <label>3.3</label><title>Total anthropogenic emissions</title>
      <p id="d1e12030">Cumulative anthropogenic CO<inline-formula><mml:math id="M860" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions for 1850–2020 totalled 660 <inline-formula><mml:math id="M861" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 65 GtC (2420 <inline-formula><mml:math id="M862" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 240 GtCO<inline-formula><mml:math id="M863" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>), of which almost 70 % (455 GtC) occurred since 1960 and more than 30 % (205 GtC) since 2000 (Tables 6
and 8). Total anthropogenic emissions more than doubled over the last 60 years, from 4.6 <inline-formula><mml:math id="M864" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M865" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the decade of the 1960s to an
average of 10.6 <inline-formula><mml:math id="M866" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8 GtC yr<inline-formula><mml:math id="M867" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during 2011–2020.</p>
      <p id="d1e12104">The total anthropogenic CO<inline-formula><mml:math id="M868" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from fossil plus land-use change
amounted to 10.6 <inline-formula><mml:math id="M869" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8 GtC (38.9 <inline-formula><mml:math id="M870" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 2.9 GtCO<inline-formula><mml:math id="M871" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) for the
2011–2020 decade, reaching 10.2 <inline-formula><mml:math id="M872" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8 GtC (37.2 <inline-formula><mml:math id="M873" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 2.9 GtCO<inline-formula><mml:math id="M874" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) in 2020, while for 2021, we project global total anthropogenic
CO<inline-formula><mml:math id="M875" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from fossil and land-use changes to be around 10.7 GtC
(39.3 GtCO<inline-formula><mml:math id="M876" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>).</p>
      <p id="d1e12181">During the historical period 1850–2020, 30 % of historical emissions were
from land-use change and 70 % from fossil emissions. However, fossil
emissions have grown significantly since 1960 while land-use changes have
not, and consequently the contributions of land-use change to total
anthropogenic emissions were smaller during recent periods (17 % during
the period 1960–2020 and 10 % during 2011–2020).</p>

<?xmltex \floatpos{p}?><table-wrap id="Ch1.T8" orientation="landscape"><?xmltex \currentcnt{7}?><label>Table 7</label><caption><p id="d1e12188">Comparison of the projection with realized fossil CO<inline-formula><mml:math id="M877" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (EFOS). The “Actual” values are first the estimate available using actual data, and the “Projected” values refer to estimates made before the end of the year for each publication. Projections based on a different method from that described here during 2008–2014 are available in Le Quéré et al. (2016). All values are adjusted for leap years.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.9}[.9]?><oasis:tgroup cols="13">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right" colsep="1"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right" colsep="1"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:colspec colnum="7" colname="col7" align="right" colsep="1"/>
     <oasis:colspec colnum="8" colname="col8" align="right"/>
     <oasis:colspec colnum="9" colname="col9" align="right" colsep="1"/>
     <oasis:colspec colnum="10" colname="col10" align="right"/>
     <oasis:colspec colnum="11" colname="col11" align="right" colsep="1"/>
     <oasis:colspec colnum="12" colname="col12" align="right"/>
     <oasis:colspec colnum="13" colname="col13" align="right"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry rowsep="1" namest="col2" nameend="col3" align="center" colsep="1">World </oasis:entry>
         <oasis:entry rowsep="1" namest="col4" nameend="col5" align="center" colsep="1">China </oasis:entry>
         <oasis:entry rowsep="1" namest="col6" nameend="col7" align="center" colsep="1">USA </oasis:entry>
         <oasis:entry rowsep="1" namest="col8" nameend="col9" align="center" colsep="1">EU28<inline-formula><mml:math id="M886" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">h</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry rowsep="1" namest="col10" nameend="col11" align="center" colsep="1">India </oasis:entry>
         <oasis:entry rowsep="1" namest="col12" nameend="col13" align="center">Rest of world </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">Projected</oasis:entry>
         <oasis:entry colname="col3">Actual</oasis:entry>
         <oasis:entry colname="col4">Projected</oasis:entry>
         <oasis:entry colname="col5">Actual</oasis:entry>
         <oasis:entry colname="col6">Projected</oasis:entry>
         <oasis:entry colname="col7">Actual</oasis:entry>
         <oasis:entry colname="col8">Projected</oasis:entry>
         <oasis:entry colname="col9">Actual</oasis:entry>
         <oasis:entry colname="col10">Projected</oasis:entry>
         <oasis:entry colname="col11">Actual</oasis:entry>
         <oasis:entry colname="col12">Projected</oasis:entry>
         <oasis:entry colname="col13">Actual</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">2015<inline-formula><mml:math id="M887" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M888" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.6 %</oasis:entry>
         <oasis:entry colname="col3">0.06 %</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M889" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>3.9 %</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M890" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.7 %</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M891" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.5 %</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M892" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.5 %</oasis:entry>
         <oasis:entry colname="col8">–</oasis:entry>
         <oasis:entry colname="col9">–</oasis:entry>
         <oasis:entry colname="col10">–</oasis:entry>
         <oasis:entry colname="col11">–</oasis:entry>
         <oasis:entry colname="col12">1.2 %</oasis:entry>
         <oasis:entry colname="col13">1.2 %</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">(<inline-formula><mml:math id="M893" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>1.6 to 0.5)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">(<inline-formula><mml:math id="M894" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>4.6 to <inline-formula><mml:math id="M895" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.1)</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">(<inline-formula><mml:math id="M896" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>5.5 to 0.3)</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
         <oasis:entry colname="col10"/>
         <oasis:entry colname="col11"/>
         <oasis:entry colname="col12">(<inline-formula><mml:math id="M897" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.2 to 2.6)</oasis:entry>
         <oasis:entry colname="col13"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2016<inline-formula><mml:math id="M898" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M899" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.2 %</oasis:entry>
         <oasis:entry colname="col3">0.20 %</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M900" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.5 %</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M901" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.3 %</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M902" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.7 %</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M903" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.1 %</oasis:entry>
         <oasis:entry colname="col8">–</oasis:entry>
         <oasis:entry colname="col9">–</oasis:entry>
         <oasis:entry colname="col10">–</oasis:entry>
         <oasis:entry colname="col11">–</oasis:entry>
         <oasis:entry colname="col12">1.0 %</oasis:entry>
         <oasis:entry colname="col13">1.3 %</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">(<inline-formula><mml:math id="M904" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>1.0 to <inline-formula><mml:math id="M905" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.8)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">(<inline-formula><mml:math id="M906" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>3.8 to <inline-formula><mml:math id="M907" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.3)</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">(<inline-formula><mml:math id="M908" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>4.0 to <inline-formula><mml:math id="M909" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.6)</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
         <oasis:entry colname="col10"/>
         <oasis:entry colname="col11"/>
         <oasis:entry colname="col12">(<inline-formula><mml:math id="M910" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.4 to <inline-formula><mml:math id="M911" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>2.5)</oasis:entry>
         <oasis:entry colname="col13"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2017<inline-formula><mml:math id="M912" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">2.0 %</oasis:entry>
         <oasis:entry colname="col3">1.6 %</oasis:entry>
         <oasis:entry colname="col4">3.5 %</oasis:entry>
         <oasis:entry colname="col5">1.5 %</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M913" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.4 %</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M914" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.5 %</oasis:entry>
         <oasis:entry colname="col8">–</oasis:entry>
         <oasis:entry colname="col9">–</oasis:entry>
         <oasis:entry colname="col10">2.00 %</oasis:entry>
         <oasis:entry colname="col11">3.9 %</oasis:entry>
         <oasis:entry colname="col12">1.6 %</oasis:entry>
         <oasis:entry colname="col13">1.9 %</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">(<inline-formula><mml:math id="M915" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>0.8 to <inline-formula><mml:math id="M916" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.0)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">(<inline-formula><mml:math id="M917" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>0.7 to <inline-formula><mml:math id="M918" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>5.4)</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">(<inline-formula><mml:math id="M919" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>2.7 to <inline-formula><mml:math id="M920" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.0)</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
         <oasis:entry colname="col10">(<inline-formula><mml:math id="M921" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>0.2 to <inline-formula><mml:math id="M922" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.8)</oasis:entry>
         <oasis:entry colname="col11"/>
         <oasis:entry colname="col12">(0.0 to <inline-formula><mml:math id="M923" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.2)</oasis:entry>
         <oasis:entry colname="col13"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2018<inline-formula><mml:math id="M924" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">2.7 %</oasis:entry>
         <oasis:entry colname="col3">2.1 %</oasis:entry>
         <oasis:entry colname="col4">4.7 %</oasis:entry>
         <oasis:entry colname="col5">2.3 %</oasis:entry>
         <oasis:entry colname="col6">2.5 %</oasis:entry>
         <oasis:entry colname="col7">2.8 %</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M925" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.7 %</oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M926" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.1 %</oasis:entry>
         <oasis:entry colname="col10">6.3 %</oasis:entry>
         <oasis:entry colname="col11">8.0 %</oasis:entry>
         <oasis:entry colname="col12">1.8 %</oasis:entry>
         <oasis:entry colname="col13">1.7 %</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">(<inline-formula><mml:math id="M927" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>1.8 to <inline-formula><mml:math id="M928" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.7)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">(<inline-formula><mml:math id="M929" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>2.0 to <inline-formula><mml:math id="M930" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>7.4)</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">(<inline-formula><mml:math id="M931" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>0.5 to <inline-formula><mml:math id="M932" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.5)</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8">(-2.6 to <inline-formula><mml:math id="M933" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.3)</oasis:entry>
         <oasis:entry colname="col9"/>
         <oasis:entry colname="col10">(<inline-formula><mml:math id="M934" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>4.3 to <inline-formula><mml:math id="M935" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>8.3)</oasis:entry>
         <oasis:entry colname="col11"/>
         <oasis:entry colname="col12">(<inline-formula><mml:math id="M936" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>0.5 to <inline-formula><mml:math id="M937" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.0)</oasis:entry>
         <oasis:entry colname="col13"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2019<inline-formula><mml:math id="M938" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">e</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">0.5 %</oasis:entry>
         <oasis:entry colname="col3">0.1 %</oasis:entry>
         <oasis:entry colname="col4">2.6 %</oasis:entry>
         <oasis:entry colname="col5">2.2 %</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M939" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.4 %</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M940" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.6 %</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M941" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.7 %</oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M942" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>4.3 %</oasis:entry>
         <oasis:entry colname="col10">1.8 %</oasis:entry>
         <oasis:entry colname="col11">1.0 %</oasis:entry>
         <oasis:entry colname="col12">0.5 %</oasis:entry>
         <oasis:entry colname="col13">0.5 %</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">(<inline-formula><mml:math id="M943" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.3 to <inline-formula><mml:math id="M944" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.4)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">(<inline-formula><mml:math id="M945" display="inline"><mml:mo lspace="0mm">+</mml:mo></mml:math></inline-formula>0.7 to <inline-formula><mml:math id="M946" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>4.4)</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">(<inline-formula><mml:math id="M947" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>4.7 to <inline-formula><mml:math id="M948" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.1)</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8">(<inline-formula><mml:math id="M949" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>5.1 % to <inline-formula><mml:math id="M950" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.8 %)</oasis:entry>
         <oasis:entry colname="col9"/>
         <oasis:entry colname="col10">(<inline-formula><mml:math id="M951" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.7 to <inline-formula><mml:math id="M952" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3.7)</oasis:entry>
         <oasis:entry colname="col11"/>
         <oasis:entry colname="col12">(<inline-formula><mml:math id="M953" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.8 to <inline-formula><mml:math id="M954" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>1.8)</oasis:entry>
         <oasis:entry colname="col13"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2020<inline-formula><mml:math id="M955" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">f</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"><inline-formula><mml:math id="M956" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>6.7 %</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M957" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>5.4 %</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M958" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.7 %</oasis:entry>
         <oasis:entry colname="col5">1.4 %</oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M959" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>12.2 %</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M960" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>10.6 %</oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M961" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>11.3 % (EU27)</oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M962" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>10.9 %</oasis:entry>
         <oasis:entry colname="col10"><inline-formula><mml:math id="M963" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>9.1 %</oasis:entry>
         <oasis:entry colname="col11"><inline-formula><mml:math id="M964" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>7.3 %</oasis:entry>
         <oasis:entry colname="col12"><inline-formula><mml:math id="M965" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>7.4 %</oasis:entry>
         <oasis:entry colname="col13"><inline-formula><mml:math id="M966" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>7.0 %</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2021<inline-formula><mml:math id="M967" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">g</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">4.8 %</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">4.3 %</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">6.8 %</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8">6.3 %</oasis:entry>
         <oasis:entry colname="col9"/>
         <oasis:entry colname="col10">11.2 %</oasis:entry>
         <oasis:entry colname="col11"/>
         <oasis:entry colname="col12">3.2 %</oasis:entry>
         <oasis:entry colname="col13"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">(4.2 % to 5.4 %)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">(3.0 % to 5.4 %)</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">(6.6 % to 7.0 %)</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8">(4.3 % to 8.3 %)</oasis:entry>
         <oasis:entry colname="col9"/>
         <oasis:entry colname="col10">(10.7 % to 11.7 %)</oasis:entry>
         <oasis:entry colname="col11"/>
         <oasis:entry colname="col12">(2.0 % to 4.3 %)</oasis:entry>
         <oasis:entry colname="col13"/>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table><table-wrap-foot><p id="d1e12200"><inline-formula><mml:math id="M878" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula> Jackson et al. (2016) and Le Quéré et al. (2015a). <inline-formula><mml:math id="M879" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> Le Quéré et al. (2016). <inline-formula><mml:math id="M880" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula> Le Quéré et al. (2018a). <inline-formula><mml:math id="M881" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula> Le Quéré et al. (2018b). <inline-formula><mml:math id="M882" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">e</mml:mi></mml:msup></mml:math></inline-formula> Friedlingstein et al. (2019), <inline-formula><mml:math id="M883" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">f</mml:mi></mml:msup></mml:math></inline-formula> Friedlingstein et al. (2020), <inline-formula><mml:math id="M884" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">g</mml:mi></mml:msup></mml:math></inline-formula> This study (median of four reported <?xmltex \hack{\break}?> estimates, Sect. 3.1.4). <inline-formula><mml:math id="M885" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">h</mml:mi></mml:msup></mml:math></inline-formula> EU28 until 2019, EU27 from 2020.</p></table-wrap-foot></table-wrap>

<?xmltex \floatpos{t}?><table-wrap id="Ch1.T9" specific-use="star"><?xmltex \currentcnt{8}?><label>Table 8</label><caption><p id="d1e13460">Cumulative CO<inline-formula><mml:math id="M968" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> for different time
periods in gigatonnes of carbon (GtC). All uncertainties are reported as
<inline-formula><mml:math id="M969" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M970" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>. Fossil CO<inline-formula><mml:math id="M971" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
include cement carbonation. The budget imbalance
(<inline-formula><mml:math id="M972" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) provides a measure of the discrepancies among
the nearly independent estimates. All values are rounded to the nearest 5 GtC and therefore columns do not necessarily add to zero.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="6">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="right"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:colspec colnum="6" colname="col6" align="right"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">1750–2020</oasis:entry>
         <oasis:entry colname="col3">1850–2014</oasis:entry>
         <oasis:entry colname="col4">1850–2020</oasis:entry>
         <oasis:entry colname="col5">1960–2020</oasis:entry>
         <oasis:entry colname="col6">1850–2021<inline-formula><mml:math id="M982" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col6">Emissions </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Fossil CO<inline-formula><mml:math id="M983" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (<inline-formula><mml:math id="M984" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">460 <inline-formula><mml:math id="M985" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 25</oasis:entry>
         <oasis:entry colname="col3">400 <inline-formula><mml:math id="M986" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 20</oasis:entry>
         <oasis:entry colname="col4">455 <inline-formula><mml:math id="M987" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 25</oasis:entry>
         <oasis:entry colname="col5">375 <inline-formula><mml:math id="M988" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 20</oasis:entry>
         <oasis:entry colname="col6">465 <inline-formula><mml:math id="M989" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 25</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Land-use change emissions (<inline-formula><mml:math id="M990" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">235 <inline-formula><mml:math id="M991" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 75<inline-formula><mml:math id="M992" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">195 <inline-formula><mml:math id="M993" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 60<inline-formula><mml:math id="M994" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4">200 <inline-formula><mml:math id="M995" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 65<inline-formula><mml:math id="M996" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">80 <inline-formula><mml:math id="M997" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 45<inline-formula><mml:math id="M998" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">205 <inline-formula><mml:math id="M999" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 65</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Total emissions</oasis:entry>
         <oasis:entry colname="col2">690 <inline-formula><mml:math id="M1000" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 80</oasis:entry>
         <oasis:entry colname="col3">595 <inline-formula><mml:math id="M1001" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 65</oasis:entry>
         <oasis:entry colname="col4">660 <inline-formula><mml:math id="M1002" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 65</oasis:entry>
         <oasis:entry colname="col5">455 <inline-formula><mml:math id="M1003" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 45</oasis:entry>
         <oasis:entry colname="col6">670 <inline-formula><mml:math id="M1004" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 65</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col6">Partitioning </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Growth rate in atmospheric CO<inline-formula><mml:math id="M1005" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math id="M1006" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">290 <inline-formula><mml:math id="M1007" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 5</oasis:entry>
         <oasis:entry colname="col3">235 <inline-formula><mml:math id="M1008" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 5</oasis:entry>
         <oasis:entry colname="col4">270 <inline-formula><mml:math id="M1009" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 5</oasis:entry>
         <oasis:entry colname="col5">205 <inline-formula><mml:math id="M1010" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 5</oasis:entry>
         <oasis:entry colname="col6">275 <inline-formula><mml:math id="M1011" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 5</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Ocean sink (<inline-formula><mml:math id="M1012" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">180 <inline-formula><mml:math id="M1013" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 35</oasis:entry>
         <oasis:entry colname="col3">150 <inline-formula><mml:math id="M1014" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 30</oasis:entry>
         <oasis:entry colname="col4">170 <inline-formula><mml:math id="M1015" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 35</oasis:entry>
         <oasis:entry colname="col5">115 <inline-formula><mml:math id="M1016" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 25</oasis:entry>
         <oasis:entry colname="col6">170 <inline-formula><mml:math id="M1017" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 35</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Terrestrial sink (<inline-formula><mml:math id="M1018" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">215 <inline-formula><mml:math id="M1019" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 50</oasis:entry>
         <oasis:entry colname="col3">180 <inline-formula><mml:math id="M1020" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 40</oasis:entry>
         <oasis:entry colname="col4">195 <inline-formula><mml:math id="M1021" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 45</oasis:entry>
         <oasis:entry colname="col5">135 <inline-formula><mml:math id="M1022" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 25</oasis:entry>
         <oasis:entry colname="col6">200 <inline-formula><mml:math id="M1023" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 45</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col6">Budget imbalance </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M1024" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:mo>(</mml:mo><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">10</oasis:entry>
         <oasis:entry colname="col3">30</oasis:entry>
         <oasis:entry colname="col4">25</oasis:entry>
         <oasis:entry colname="col5">0</oasis:entry>
         <oasis:entry colname="col6">25</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table><table-wrap-foot><p id="d1e13506"><inline-formula><mml:math id="M973" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula> Using projections for the year 2021.
<inline-formula><mml:math id="M974" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> Cumulative <inline-formula><mml:math id="M975" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> 1750–1849 of 30 GtC based on multi-model mean of Pongratz et al. (2009), Shevliakova et al. (2009), Zaehle et al. (2011), and Van Minnen et al. (2009). 1850–2020 from the mean of BLUE (Hansis et al., 2015), OSCAR (Gasser et al., 2020), and H&amp;N2017 (Houghton and Nassikas, 2017). 1750–2020 uncertainty is estimated from standard deviation of DGVMs over 1870–2020 scaled by 1750–2020 emissions.
<inline-formula><mml:math id="M976" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula> Cumulative <inline-formula><mml:math id="M977" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> based on BLUE, OSCAR, and H&amp;N2017. Uncertainty is estimated from the standard deviation of DGVM estimates. <inline-formula><mml:math id="M978" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula> Cumulative <inline-formula><mml:math id="M979" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> based on BLUE, OSCAR, and H&amp;N2017. Uncertainty is formed from the uncertainty in annual <inline-formula><mml:math id="M980" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> over 1959–2020, which is 0.7 GtC yr<inline-formula><mml:math id="M981" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> multiplied by length of the time series.</p></table-wrap-foot></table-wrap>

</sec>
<sec id="Ch1.S3.SS4">
  <label>3.4</label><?xmltex \opttitle{Atmospheric CO${}_{{2}}$}?><title>Atmospheric CO<inline-formula><mml:math id="M1025" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula></title>
<sec id="Ch1.S3.SS4.SSS1">
  <label>3.4.1</label><title>Historical period 1850–2020</title>
      <p id="d1e14215">Atmospheric CO<inline-formula><mml:math id="M1026" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration was approximately 277 parts per million
(ppm) in 1750 (Joos and Spahni, 2008), reaching 300 ppm in the 1910s, 350 ppm
in the late 1980s, and 412.44 <inline-formula><mml:math id="M1027" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.1 ppm in 2020 (Dlugokencky
and Tans, 2022; Fig. 1). The mass of carbon in the atmosphere increased by
48 % from 590 GtC in 1750 to 876 GtC in 2020. Current CO<inline-formula><mml:math id="M1028" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentrations in the atmosphere are unprecedented in the last 2 million
years, and the current rate of atmospheric CO<inline-formula><mml:math id="M1029" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> increase is at least 10
times faster than at any other time during the last 800 000 years (Canadell
et al., 2022).</p>
</sec>
<sec id="Ch1.S3.SS4.SSS2">
  <label>3.4.2</label><title>Recent period 1960–2020</title>
      <p id="d1e14260">The growth rate in atmospheric CO<inline-formula><mml:math id="M1030" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> level increased from 1.7 <inline-formula><mml:math id="M1031" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.07 GtC yr<inline-formula><mml:math id="M1032" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the 1960s to 5.1 <inline-formula><mml:math id="M1033" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.02 GtC yr<inline-formula><mml:math id="M1034" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during
2011–2020 with important decadal variations (Table 6, Figs. 3 and 4).</p>
      <p id="d1e14310">During the last decade (2011–2020), the growth rate in atmospheric CO<inline-formula><mml:math id="M1035" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration continued to increase, albeit with large interannual
variability (Fig. 4).</p>
      <p id="d1e14322">The airborne fraction (AF), defined as the ratio of atmospheric CO<inline-formula><mml:math id="M1036" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth rate to total anthropogenic emissions,
              <disp-formula id="Ch1.E2" content-type="numbered"><label>2</label><mml:math id="M1037" display="block"><mml:mrow><mml:mi mathvariant="normal">AF</mml:mi><mml:mo>=</mml:mo><mml:mspace linebreak="nobreak" width="0.125em"/><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mo>/</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/><mml:mo>(</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub><mml:mo>)</mml:mo></mml:mrow></mml:math></disp-formula>
            provides a diagnostic of the relative strength of the land and ocean carbon
sinks in removing part of the anthropogenic CO<inline-formula><mml:math id="M1038" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> perturbation. The
evolution of AF over the last 60 years shows no significant trend, remaining at around 45 %, albeit showing a large interannual variability
driven by the year-to-year variability in <inline-formula><mml:math id="M1039" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Fig. 8). The observed
stability of the airborne fraction over the 1960–2020 period indicates that
the ocean and land CO<inline-formula><mml:math id="M1040" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sinks have been removing on average about 55 %
of the anthropogenic emissions (see Sect. 3.5 and 3.6).</p>

      <?xmltex \floatpos{p}?><fig id="Ch1.F8"><?xmltex \currentcnt{8}?><?xmltex \def\figurename{Figure}?><label>Figure 8</label><caption><p id="d1e14403">The partitioning of total anthropogenic CO<inline-formula><mml:math id="M1041" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
(<inline-formula><mml:math id="M1042" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) across <bold>(a)</bold> the atmosphere (airborne fraction), <bold>(b)</bold> land (land-borne fraction), and <bold>(c)</bold> ocean (ocean-borne fraction). Black
lines represent the central estimate, and the coloured shading represents
the uncertainty. The grey dashed lines represent the long-term average of
the airborne (44 %), land-borne (28 %), and ocean-borne (24 %)
fractions during 1959–2020.</p></caption>
            <?xmltex \igopts{width=199.169291pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f08.png"/>

          </fig>

</sec>
<sec id="Ch1.S3.SS4.SSS3">
  <label>3.4.3</label><title>Final year 2020</title>
      <p id="d1e14456">The growth rate in atmospheric CO<inline-formula><mml:math id="M1043" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration was 5.0 <inline-formula><mml:math id="M1044" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2 GtC (2.37 <inline-formula><mml:math id="M1045" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.08 ppm) in 2020 (Fig. 4; Dlugokencky and Tans, 2022),
very close to the 2011–2020 average. The 2020 decrease in <inline-formula><mml:math id="M1046" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and
<inline-formula><mml:math id="M1047" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of about 0.7 GtC propagated to an atmospheric CO<inline-formula><mml:math id="M1048" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth rate
reduction of 0.38 GtC (0.18 ppm), given the significant interannual
variability of the land carbon sink.</p>
</sec>
<sec id="Ch1.S3.SS4.SSS4">
  <label>3.4.4</label><title>Year 2021 projection</title>
      <p id="d1e14523">The 2021 growth in atmospheric CO<inline-formula><mml:math id="M1049" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration (<inline-formula><mml:math id="M1050" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) is
projected to be about 5.3 GtC (2.49 ppm) based on GLO observations until the
end of December 2021, bringing the atmospheric CO<inline-formula><mml:math id="M1051" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration to an
expected level of 414.67 ppm averaged over the year, 50 % over the
pre-industrial level.</p>
</sec>
</sec>
<sec id="Ch1.S3.SS5">
  <label>3.5</label><title>Ocean sink</title>
<sec id="Ch1.S3.SS5.SSS1">
  <label>3.5.1</label><title>Historical period 1850–2020</title>
      <p id="d1e14571">Cumulated since 1850, the ocean sink adds up to 170 <inline-formula><mml:math id="M1052" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 35 GtC, with two-thirds of this amount being taken up by the global ocean since 1960. Over
the historical period, the ocean sink increased in pace with the
anthropogenic emissions exponential increase (Fig. 3b). Since 1850, the
ocean has removed 26 % of total anthropogenic emissions.</p>
</sec>
<sec id="Ch1.S3.SS5.SSS2">
  <label>3.5.2</label><title>Recent period 1960–2020</title>
      <p id="d1e14589">The ocean CO<inline-formula><mml:math id="M1053" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink increased from 1.1 <inline-formula><mml:math id="M1054" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M1055" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the
1960s to 2.8 <inline-formula><mml:math id="M1056" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M1057" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during 2011–2020 (Table 6), with
interannual variations of the order of a few tenths of GtC yr<inline-formula><mml:math id="M1058" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Fig. 9). The ocean-borne fraction (<inline-formula><mml:math id="M1059" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:mo>(</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) has been
remarkably constant, around 25 % on average (Fig. 8). Variations around
this mean illustrate decadal variability of the ocean carbon sink. So far,
there is no indication of a decrease in the ocean-borne fraction from 1960
to 2020. The increase in the ocean sink is primarily driven by the increased
atmospheric CO<inline-formula><mml:math id="M1060" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration, with the strongest CO<inline-formula><mml:math id="M1061" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-induced
signal in the North Atlantic and the Southern Ocean (Fig. 10a). The effect
of climate change is much weaker, reducing the ocean sink globally by 0.12 <inline-formula><mml:math id="M1062" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.07 GtC yr<inline-formula><mml:math id="M1063" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> or 5 % (2011–2020, range <inline-formula><mml:math id="M1064" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.8 % to <inline-formula><mml:math id="M1065" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>7.4 %), and
does not show clear spatial patterns across the GOBMs ensemble (Fig. 10b).
This is the combined effect of change and variability in all atmospheric
forcing fields, previously attributed to wind and temperature changes in one
model (Le Quéré et al., 2010).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F9"><?xmltex \currentcnt{9}?><?xmltex \def\figurename{Figure}?><label>Figure 9</label><caption><p id="d1e14733">Comparison of the anthropogenic atmosphere–ocean CO<inline-formula><mml:math id="M1066" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux
showing the budget values of <inline-formula><mml:math id="M1067" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (black; with the uncertainty in
grey shading), individual ocean models (teal), and the ocean <inline-formula><mml:math id="M1068" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1069" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based
data products (cyan; with Watson et al. (2020) in dashed line as not used
for ensemble mean). The <inline-formula><mml:math id="M1070" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1071" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products were adjusted for the
pre-industrial ocean source of CO<inline-formula><mml:math id="M1072" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> from river input to the ocean, by
subtracting a source of 0.61 GtC yr<inline-formula><mml:math id="M1073" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to make them comparable to
<inline-formula><mml:math id="M1074" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (see Sect. 2.4). Bar-plot in the lower right illustrates the
number of <inline-formula><mml:math id="M1075" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1076" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> observations in the SOCAT v2021 database (Bakker et al.,
2021). Grey bars indicate the number of data points in SOCAT v2020, and
coloured bars the newly added observations in v2021.</p></caption>
            <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f09.png"/>

          </fig>

      <p id="d1e14843">The global net air–sea CO<inline-formula><mml:math id="M1077" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux is a residual of large natural and
anthropogenic CO<inline-formula><mml:math id="M1078" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes into and out of the ocean with distinct
regional and seasonal variations (Figs. 6 and B1). Natural fluxes dominate on
regional scales but largely cancel out when integrated globally (Gruber et
al., 2009). Mid-latitudes in all basins and the high-latitude North Atlantic
dominate the ocean CO<inline-formula><mml:math id="M1079" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> uptake where low temperatures and high wind
speeds facilitate CO<inline-formula><mml:math id="M1080" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> uptake at the surface (Takahashi et al., 2009).
In these regions, mode, intermediate, and deep-water masses are formed that
transport anthropogenic carbon into the ocean interior, thus allowing for
continued CO<inline-formula><mml:math id="M1081" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> uptake at the surface. Outgassing of natural CO<inline-formula><mml:math id="M1082" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
occurs mostly in the tropics, especially in the equatorial upwelling region,
and to a lesser extent in the North Pacific and polar Southern Ocean,
mirroring a well-established understanding of regional patterns of air–sea
CO<inline-formula><mml:math id="M1083" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> exchange (e.g. Takahashi et al., 2009; Gruber et al., 2009). These
patterns are also noticeable in the Surface Ocean CO<inline-formula><mml:math id="M1084" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> Atlas (SOCAT) dataset,
where an ocean <inline-formula><mml:math id="M1085" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1086" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> value above the atmospheric level indicates
outgassing (Fig. B1). This map further illustrates the data sparsity in the
Indian Ocean and the Southern Hemisphere in general.</p>
      <p id="d1e14936">Interannual variability of the ocean carbon sink is driven by climate
variability with a first-order effect from a stronger ocean sink during
large El Niño events (e.g. 1997–1998) (Fig. 9; Rödenbeck et al.,
2014; Hauck et al., 2020). The GOBMs show the same patterns of decadal
variability as the mean of the <inline-formula><mml:math id="M1087" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1088" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products, with a
stagnation of the ocean sink in the 1990s and a strengthening since the
early 2000s (Fig. 9, Le Quéré et al., 2007; Landschützer et al.,
2015, 2016; DeVries et al., 2017; Hauck et al., 2020; McKinley et al.,
2020). Different explanations have been proposed for this decadal
variability, ranging from the ocean's response to changes in atmospheric
wind and pressure systems (e.g. Le Quéré et al., 2007; Keppler and
Landschützer, 2019), including variations in upper ocean overturning
circulation (DeVries et al., 2017), to the eruption of Mount Pinatubo and its
effects on sea surface temperature and slowed atmospheric CO<inline-formula><mml:math id="M1089" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth
rate in the 1990s (McKinley et al., 2020). The main origin of the decadal
variability is a matter of debate with a number of studies initially
pointing to the Southern Ocean (see review in Canadell et al., 2022), but
also contributions from the North Atlantic and North Pacific
(Landschützer et al., 2016; DeVries et al., 2019) or a global signal
(McKinley et al., 2020) were proposed.</p>
      <p id="d1e14964">Although all individual GOBMs and data products fall within the
observational constraint, the ensemble means of GOBMs and data products
adjusted for the riverine flux diverge over time with a mean offset
increasing from 0.24 GtC yr<inline-formula><mml:math id="M1090" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the 1990s to 0.66 GtC yr<inline-formula><mml:math id="M1091" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the
decade 2011–2020 and reaching 1.1 GtC yr<inline-formula><mml:math id="M1092" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in 2020. The <inline-formula><mml:math id="M1093" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
trend diverges with a factor-of-2 difference since 2002 (GOBMs: 0.3 <inline-formula><mml:math id="M1094" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.1 GtC yr<inline-formula><mml:math id="M1095" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade, data products: 0.7 <inline-formula><mml:math id="M1096" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2 GtC yr<inline-formula><mml:math id="M1097" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
per decade, best estimate: 0.5 GtC yr<inline-formula><mml:math id="M1098" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade) and with a factor-of-3 since 2010 (GOBMs: 0.3 <inline-formula><mml:math id="M1099" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.1 GtC yr<inline-formula><mml:math id="M1100" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade,
data products: 0.9 <inline-formula><mml:math id="M1101" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M1102" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade, best
estimate: 0.6 GtC yr<inline-formula><mml:math id="M1103" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> per decade). The GOBM estimate is lower than
in the previous global carbon budget (Friedlingstein et al., 2020), because
one high-sink model was not available. The effect of two models (CNRM,
MOM6-COBALT) revising their estimates downwards was largely balanced by two
models revising their estimate upwards (FESOM-REcoM, PlankTOM).</p>
      <p id="d1e15116">The discrepancy between the two types of estimates stems mostly from a
larger Southern Ocean sink in the data products prior to 2001, and from a
larger <inline-formula><mml:math id="M1104" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> trend in the northern and southern extra-tropics since
then (Fig. 12). Possible explanations for the discrepancy in the Southern
Ocean could be missing winter observations and data sparsity in general
(Bushinsky et al., 2019; Gloege et al., 2021), model biases (as indicated by
the large model spread in the south, Fig. 12, and the larger model–data
mismatch, Fig. B2), or uncertainties in the regional river flux adjustment
(Hauck et al., 2020; Lacroix et al., 2020).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F10" specific-use="star"><?xmltex \currentcnt{10}?><?xmltex \def\figurename{Figure}?><label>Figure 10</label><caption><p id="d1e15132">Attribution of the atmosphere–ocean (<inline-formula><mml:math id="M1105" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and
atmosphere–land (<inline-formula><mml:math id="M1106" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) CO<inline-formula><mml:math id="M1107" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes to <bold>(a)</bold> increasing atmospheric
CO<inline-formula><mml:math id="M1108" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations and <bold>(b)</bold> changes in climate, averaged over the
previous decade 2011–2020. All data shown are from the processed-based GOBMs
and DGVMs. The sum of ocean CO<inline-formula><mml:math id="M1109" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and climate effects will not equal the
ocean sink shown in Fig. 6 which includes the <inline-formula><mml:math id="M1110" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1111" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data
products. See Appendix Sects. C3.2 and C4.1 for attribution methodology. Units
are in kgC m<inline-formula><mml:math id="M1112" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> yr<inline-formula><mml:math id="M1113" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (note the non-linear colour scale).</p></caption>
            <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f10.png"/>

          </fig>

      <p id="d1e15237">During 2010–2016, the ocean CO<inline-formula><mml:math id="M1114" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink appears to have intensified in
line with the expected increase from atmospheric CO<inline-formula><mml:math id="M1115" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (McKinley et al.,
2020). This effect is stronger in the <inline-formula><mml:math id="M1116" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1117" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products (Fig. 9,
GOBMs: <inline-formula><mml:math id="M1118" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.43 GtC yr<inline-formula><mml:math id="M1119" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, data products: <inline-formula><mml:math id="M1120" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.56 GtC yr<inline-formula><mml:math id="M1121" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). The
reduction of <inline-formula><mml:math id="M1122" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.09 GtC yr<inline-formula><mml:math id="M1123" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (range: <inline-formula><mml:math id="M1124" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.30 to <inline-formula><mml:math id="M1125" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.12 GtC yr<inline-formula><mml:math id="M1126" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) in
the ocean CO<inline-formula><mml:math id="M1127" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink in 2017 is consistent with the return to normal
conditions after the El Niño in 2015–2016, which caused an enhanced sink
in previous years. After 2017, the GOBMs ensemble mean suggests the ocean
sink levels off at about 2.5 GtC yr<inline-formula><mml:math id="M1128" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, whereas the data products'
estimate increases by 0.3 GtC yr<inline-formula><mml:math id="M1129" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> over the same period.</p>
</sec>
<sec id="Ch1.S3.SS5.SSS3">
  <label>3.5.3</label><title>Final year 2020</title>
      <p id="d1e15400">The estimated ocean CO<inline-formula><mml:math id="M1130" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink was 3.0 <inline-formula><mml:math id="M1131" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC in 2020. This is
the average of GOBMs and data products, and is a small increase of 0.02 GtC
compared to 2019, in line with the competing effects from an expected sink
strengthening from atmospheric CO<inline-formula><mml:math id="M1132" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth and expected sink weakening
from La Niña conditions. There is, however, a substantial difference
between GOBMs and <inline-formula><mml:math id="M1133" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1134" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products in their mean 2020
<inline-formula><mml:math id="M1135" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate (GOBMs: 2.5 GtC, data products: 3.5 GtC). While the
GOBMs simulate a stagnation of the sink from 2019 to 2020 (<inline-formula><mml:math id="M1136" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.02 <inline-formula><mml:math id="M1137" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.11 GtC), the data products suggest an increase by 0.06 GtC, although
not significant at the 1<inline-formula><mml:math id="M1138" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> level (<inline-formula><mml:math id="M1139" display="inline"><mml:mo lspace="0mm">±</mml:mo></mml:math></inline-formula>0.13 GtC). Four models and
four data products show an increase in <inline-formula><mml:math id="M1140" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (GOBMs up to <inline-formula><mml:math id="M1141" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.18 GtC,
data product up to <inline-formula><mml:math id="M1142" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.21 GtC), while four models and three data products
show no change or a decrease in <inline-formula><mml:math id="M1143" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (GOBMs down to <inline-formula><mml:math id="M1144" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.12 GtC,
data products down to <inline-formula><mml:math id="M1145" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.13 GtC; Fig. 9). The data products have a larger
uncertainty at the tails of the reconstructed time series (e.g. Watson et
al., 2020). Specifically, the data products' estimate of the last year is
regularly adjusted in the following release owing to the tail effect and an
incrementally increasing data availability with 1–5 years lag (Fig. 9
bottom).</p>
</sec>
<sec id="Ch1.S3.SS5.SSS4">
  <label>3.5.4</label><title>Year 2021 projection</title>
      <p id="d1e15543">Using a feed-forward neural network method (see Sect. 2.4) we project an
ocean sink of 2.9 GtC for 2021. This is a reduction of the sink by 0.1 GtC
relative to the 2020 value, which we attribute to La Niña conditions in
January to May 2021 and projections of a re-emergence of La Niña later
in the year.</p>
</sec>
<sec id="Ch1.S3.SS5.SSS5">
  <label>3.5.5</label><title>Model evaluation</title>
      <p id="d1e15555">The evaluation of the ocean estimates (Fig. B2) shows an RMSE from annually
detrended data of 1.3 to 2.8 <inline-formula><mml:math id="M1146" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">atm</mml:mi></mml:mrow></mml:math></inline-formula> for the seven <inline-formula><mml:math id="M1147" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1148" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data
products over the globe, relative to the <inline-formula><mml:math id="M1149" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1150" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> observations from the
SOCAT v2021 dataset for the period 1990–2020. The GOBMs RMSEs are larger and
range from 3.3 to 5.9 <inline-formula><mml:math id="M1151" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">atm</mml:mi></mml:mrow></mml:math></inline-formula>. The RMSEs are generally larger at high
latitudes compared to the tropics, for both the data products and the GOBMs.
The data products have RMSEs of 1.3 to 3.6 <inline-formula><mml:math id="M1152" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">atm</mml:mi></mml:mrow></mml:math></inline-formula> in the tropics, 1.3
to 2.7 <inline-formula><mml:math id="M1153" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">atm</mml:mi></mml:mrow></mml:math></inline-formula> in the north, and 2.2 to 6.1 <inline-formula><mml:math id="M1154" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">atm</mml:mi></mml:mrow></mml:math></inline-formula> in the south.
Note that the data products are based on the SOCAT v2021 database; hence the
latter are not an independent dataset for the evaluation of the data products.
The GOBM RMSEs are more spread across regions, ranging from 2.7 to 4.3 <inline-formula><mml:math id="M1155" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">atm</mml:mi></mml:mrow></mml:math></inline-formula> in the tropics, 2.9 to 6.9 <inline-formula><mml:math id="M1156" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">atm</mml:mi></mml:mrow></mml:math></inline-formula> in the north, and 6.4 to
9.8 <inline-formula><mml:math id="M1157" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi><mml:mi mathvariant="normal">atm</mml:mi></mml:mrow></mml:math></inline-formula> in the south. The higher RMSEs occur in regions with
stronger climate variability, such as the northern and southern high
latitudes (poleward of the subtropical gyres). The upper ranges of the model
RMSEs have decreased somewhat relative to Friedlingstein et al. (2020),
owing to one model with upper-end RMSE not being represented this year, and
the reduction of RMSE in one model (MPIOM-HAMOCC6), presumably related to
the inclusion of riverine carbon fluxes.</p>
      <p id="d1e15672">The additional simulation C allows the steady-state
anthropogenic carbon component (sim C – sim B) to be separated and the model flux
and DIC inventory change to be compared directly to the interior ocean estimate of Gruber
et al. (2019) without further assumptions. The GOBMs ensemble average of
steady-state anthropogenic carbon inventory change 1994–2007 amounts to 2.1 GtC yr<inline-formula><mml:math id="M1158" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and is significantly lower than the 2.6 <inline-formula><mml:math id="M1159" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M1160" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> estimated by Gruber et al. (2019). Only the three models with the
highest sink estimate fall within the range reported by Gruber et al. (2019). This suggests that most of the models underestimate anthropogenic
carbon uptake by the ocean likely due to biases in ocean carbon transport
and mixing from the surface mixed layer to the ocean interior.</p>
      <p id="d1e15706">The reported <inline-formula><mml:math id="M1161" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate from GOBMs and data products is 2.1 <inline-formula><mml:math id="M1162" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M1163" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> over the period 1994 to 2007, which is in
agreement with the ocean interior estimate of 2.2 <inline-formula><mml:math id="M1164" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M1165" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> when accounting for the climate effect on the natural CO<inline-formula><mml:math id="M1166" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux of
<inline-formula><mml:math id="M1167" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.4 <inline-formula><mml:math id="M1168" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.24 GtC yr<inline-formula><mml:math id="M1169" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Gruber et al., 2019) to match the
definition of <inline-formula><mml:math id="M1170" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> used here (Hauck et al., 2020). This comparison
depends critically on the estimate of the climate effect on the natural
CO<inline-formula><mml:math id="M1171" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux, which is smaller from the GOBMs (Sect. 3.5.2) than in
Gruber et al. (2019).</p>
</sec>
</sec>
<sec id="Ch1.S3.SS6">
  <label>3.6</label><title>Land sink</title>
<sec id="Ch1.S3.SS6.SSS1">
  <label>3.6.1</label><title>Historical period 1850–2020</title>
      <p id="d1e15830">Cumulated since 1850, the terrestrial CO<inline-formula><mml:math id="M1172" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink amounts to 195 <inline-formula><mml:math id="M1173" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 45 GtC, 30 % of total anthropogenic emissions. Over the historical period,
the sink increased in pace with the anthropogenic emissions exponential
increase (Fig. 3b).</p>
</sec>
<sec id="Ch1.S3.SS6.SSS2">
  <label>3.6.2</label><title>Recent period 1960–2020</title>
      <p id="d1e15857">The terrestrial CO<inline-formula><mml:math id="M1174" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink increased from 1.2 <inline-formula><mml:math id="M1175" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M1176" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
in the 1960s to 3.1 <inline-formula><mml:math id="M1177" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6 GtC yr<inline-formula><mml:math id="M1178" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during 2010–2019, with
important interannual variations of up to 2 GtC yr<inline-formula><mml:math id="M1179" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> generally showing
a decreased land sink during El Niño events (Fig. 7), responsible for
the corresponding enhanced growth rate in atmospheric CO<inline-formula><mml:math id="M1180" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration. The larger land CO<inline-formula><mml:math id="M1181" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink during 2010–2019 compared to
the 1960s is reproduced by all the DGVMs in response to the combined
atmospheric CO<inline-formula><mml:math id="M1182" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> increase and the changes in climate, and consistent
with constraints from the other budget terms (Table 5).</p>
      <p id="d1e15947">Over the period 1960 to present the increase in the global terrestrial
CO<inline-formula><mml:math id="M1183" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink is largely attributed to the CO<inline-formula><mml:math id="M1184" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fertilization effect in
the models (Prentice et al., 2001; Piao et al., 2009), directly stimulating
plant photosynthesis and increased plant water use in water-limited systems,
with a small negative contribution of climate change (Fig. 10). There is a
range of evidence to support a positive terrestrial carbon sink in response
to increasing atmospheric CO<inline-formula><mml:math id="M1185" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, albeit with uncertain magnitude (Walker
et al., 2021). As expected from theory the greatest CO<inline-formula><mml:math id="M1186" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> effect is
simulated in the tropical forest regions, associated with warm temperatures
and long growing seasons (Hickler et al., 2008) (Fig. 10a). However,
evidence from tropical intact forest plots indicate an overall decline in
the land sink across Amazonia (1985–2011), attributed to enhanced mortality
offsetting productivity gains (Brienen et al., 2005; Hubau et al., 2020).
During 2011–2020 the land sink is positive in all regions (Fig. 6) with the
exception of central and eastern Brazil, southwest USA and northern Mexico,
southeast Europe and central Asia, South Africa, and eastern Australia,
where the negative effects of climate variability and change (i.e. reduced
rainfall) counterbalance CO<inline-formula><mml:math id="M1187" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> effects. This is clearly visible in Fig. 10 where the effects of CO<inline-formula><mml:math id="M1188" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (Fig. 10a) and climate (Fig. 10b) as
simulated by the DGVMs are isolated. The negative effect of climate is the
strongest in most of South America, Central America, southwest USA, and
central Europe (Fig. 10b). Globally, climate change reduces the land sink by
0.45 <inline-formula><mml:math id="M1189" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.39 GtC yr<inline-formula><mml:math id="M1190" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> or 15 % (2011–2020).</p>
      <p id="d1e16024">In the past years several regions experienced record-setting fire events.
While global burned area has declined over the past decades mostly due to
declining fire activity in savannas (Andela et al., 2017), forest fire
emissions are rising and have the potential to counter the negative fire
trend in savannas (Zheng et al., 2021). Noteworthy events include the
2019–2020 Black Summer event in Australia (emissions of roughly 0.2 GtC; van
der Velde et al., 2021) and Siberia in 2021, where emissions approached 0.4 GtC or 3 times the 1997–2020 average according to GFED4s. While other
regions, including western USA and Mediterranean Europe, also experienced
intense fire seasons in 2021 their emissions are substantially lower.</p>
      <p id="d1e16027">Despite these regional negative effects of climate change on <inline-formula><mml:math id="M1191" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, the
efficiency of land to remove anthropogenic CO<inline-formula><mml:math id="M1192" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions has remained
broadly constant over the last six decades, with a land-borne fraction
(<inline-formula><mml:math id="M1193" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>/</mml:mo><mml:mo>(</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) of <inline-formula><mml:math id="M1194" display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 30 % (Fig. 8).</p>
</sec>
<sec id="Ch1.S3.SS6.SSS3">
  <label>3.6.3</label><title>Final year 2020</title>
      <p id="d1e16092">The terrestrial CO<inline-formula><mml:math id="M1195" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink from the DGVM ensemble was 2.9 <inline-formula><mml:math id="M1196" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1.0 GtC in 2020, slightly below the decadal average of 3.1 GtC yr<inline-formula><mml:math id="M1197" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Fig. 4, Table 6). We note that the DGVM estimate for 2020 is significantly
larger than the 2.1 <inline-formula><mml:math id="M1198" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9 GtC yr<inline-formula><mml:math id="M1199" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> estimate from the residual
sink from the global budget (<inline-formula><mml:math id="M1200" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)
(Table 5).</p>
</sec>
<sec id="Ch1.S3.SS6.SSS4">
  <label>3.6.4</label><title>Year 2021 projection</title>
      <p id="d1e16183">Using a feed-forward neural network method (see Sect. 2.5) we project a
land sink of 3.3 GtC for 2021. This is an increase in the land sink by 0.3 GtC relative to the 2020 value which we attribute to La Niña conditions
in 2021.</p>
</sec>
<sec id="Ch1.S3.SS6.SSS5">
  <label>3.6.5</label><title>Model evaluation</title>
      <p id="d1e16195">The evaluation of the DGVMs (Fig. B3) shows generally high skill scores
across models for runoff, and to a lesser extent for vegetation biomass,
GPP, and ecosystem respiration (Fig. B3a). Skill score was lowest
for leaf area index and net ecosystem exchange, with the widest disparity
among models for soil carbon. Further analysis of the results will be
provided separately, focusing on the strengths and weaknesses in the DGVMs
ensemble and its validity for use in the global carbon budget.</p>
</sec>
</sec>
<sec id="Ch1.S3.SS7">
  <label>3.7</label><title>Partitioning the carbon sinks</title>
<sec id="Ch1.S3.SS7.SSS1">
  <label>3.7.1</label><title>Global sinks and spread of estimates</title>
      <p id="d1e16214">In the period 2011–2020, the bottom-up view of total global carbon sinks
provided by the GCB (<inline-formula><mml:math id="M1201" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) agrees
closely with the top-down budget delivered by the atmospheric inversions.
Figure 11 shows both total sink estimates of the last decade split by land
and ocean, which match the difference between <inline-formula><mml:math id="M1202" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M1203" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> to
within 0.06–0.17 GtC yr<inline-formula><mml:math id="M1204" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for inverse models and to 0.3 GtC yr<inline-formula><mml:math id="M1205" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
for the GCB mean. The latter represents the <inline-formula><mml:math id="M1206" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> discussed in Sect. 3.8, which by design is minimal for the inverse models.</p>
      <p id="d1e16300">The distributions based on the individual models and data products reveal
substantial spread but converge near the decadal means quoted in Tables 5
and 6. Sink estimates for <inline-formula><mml:math id="M1207" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and from inverse models are mostly
non-Gaussian, while the ensemble of DGVMs appears more normally distributed
justifying the use of a multi-model mean and standard deviation for their
errors in the budget. Noteworthy is that the tails of the distributions
provided by the land and ocean bottom-up estimates would not agree with the
global constraint provided by the fossil fuel emissions and the observed
atmospheric CO<inline-formula><mml:math id="M1208" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth rate (<inline-formula><mml:math id="M1209" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). This
illustrates the power of the atmospheric joint constraint from <inline-formula><mml:math id="M1210" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and
the global CO<inline-formula><mml:math id="M1211" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> observation network it derives from.</p>
</sec>
<sec id="Ch1.S3.SS7.SSS2">
  <label>3.7.2</label><title>Total atmosphere-to-land fluxes</title>
      <p id="d1e16369">The total atmosphere-to-land fluxes (<inline-formula><mml:math id="M1212" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), calculated
here as the difference between <inline-formula><mml:math id="M1213" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from the DGVMs and <inline-formula><mml:math id="M1214" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from
the bookkeeping models, amounts to a 1.9 <inline-formula><mml:math id="M1215" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.9 GtC yr<inline-formula><mml:math id="M1216" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> sink
during 2011–2020 (Table 5). Estimates of total atmosphere-to-land fluxes
(<inline-formula><mml:math id="M1217" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) from the DGVMs alone (1.6 <inline-formula><mml:math id="M1218" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6 GtC yr<inline-formula><mml:math id="M1219" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) are consistent with this estimate and also with the global carbon
budget constraint (<inline-formula><mml:math id="M1220" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, 1.7 <inline-formula><mml:math id="M1221" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.8 GtC yr<inline-formula><mml:math id="M1222" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> Table 5). Consistent with the bookkeeping model estimates,
the DGVM-based <inline-formula><mml:math id="M1223" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is substantially lower than in Friedlingstein et
al. (2020) due to the improved land-cover forcing (see Sect. 3.2.2),
increasing their total atmosphere-to-land fluxes and hence the consistency
with the budget constraint. For the last decade (2011–2020), the inversions
estimate the net atmosphere-to-land uptake to lie within a range of 1.3 to
2.0 GtC yr<inline-formula><mml:math id="M1224" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, consistent with the GCB and DGVM estimates of <inline-formula><mml:math id="M1225" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Fig. 11, Fig. 2, top row).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F11"><?xmltex \currentcnt{11}?><?xmltex \def\figurename{Figure}?><label>Figure 11</label><caption><p id="d1e16557">The 2011–2020 decadal mean net atmosphere–ocean and
atmosphere–land fluxes derived from the ocean models and <inline-formula><mml:math id="M1226" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1227" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> products
(<inline-formula><mml:math id="M1228" display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> axis, right- and left-pointing blue triangles respectively) and from the
DGVMs (<inline-formula><mml:math id="M1229" display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> axis, green symbols), and the same fluxes estimated from the six
inversions (purple symbols on secondary <inline-formula><mml:math id="M1230" display="inline"><mml:mi>x</mml:mi></mml:math></inline-formula> and <inline-formula><mml:math id="M1231" display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> axis). The grey central
point is the mean (<inline-formula><mml:math id="M1232" display="inline"><mml:mo lspace="0mm">±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M1233" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>) of <inline-formula><mml:math id="M1234" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and (<inline-formula><mml:math id="M1235" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M1236" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>
<inline-formula><mml:math id="M1237" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) as assessed in this budget. The shaded distributions show the
density of the ensemble of individual estimates. The grey diagonal band
represents the fossil fuel emissions minus the atmospheric growth rate from
this budget (<inline-formula><mml:math id="M1238" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M1239" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M1240" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). Note that positive values are
CO<inline-formula><mml:math id="M1241" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sinks. </p></caption>
            <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f11.png"/>

          </fig>

      <?xmltex \floatpos{p}?><fig id="Ch1.F12" specific-use="star"><?xmltex \currentcnt{12}?><?xmltex \def\figurename{Figure}?><label>Figure 12</label><caption><p id="d1e16706">CO<inline-formula><mml:math id="M1242" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes between the atmosphere and the Earth's surface
separated between land and oceans, globally and in three latitude bands. The
ocean flux is <inline-formula><mml:math id="M1243" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and the land flux is the net atmosphere–land
fluxes from the DGVMs. The latitude bands are (top row) global, (second
row) north (<inline-formula><mml:math id="M1244" display="inline"><mml:mo lspace="0mm">&gt;</mml:mo></mml:math></inline-formula> 30<inline-formula><mml:math id="M1245" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N), (third row) tropics
(30<inline-formula><mml:math id="M1246" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S–30<inline-formula><mml:math id="M1247" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N), and (bottom row) south (&lt;30<inline-formula><mml:math id="M1248" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S), and over ocean (left column), over land (middle column), and
total (right column). Estimates are shown for process-based models (DGVMs
for land, GOBMs for oceans), inversion models (land and ocean), and
<inline-formula><mml:math id="M1249" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1250" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products (ocean only). Positive values indicate a flux
from the atmosphere to the land or the ocean. Mean estimates from the
combination of the process models for the land and oceans are shown (black
line) with <inline-formula><mml:math id="M1251" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1 standard deviation (1<inline-formula><mml:math id="M1252" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>) of the model ensemble
(grey shading). For the total uncertainty in the process-based estimate of
the total sink, uncertainties are summed in quadrature. Mean estimates from
the atmospheric inversions are shown (purple lines) with their full spread
(purple shading). Mean estimates from the <inline-formula><mml:math id="M1253" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1254" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products are
shown for the ocean domain (light blue lines) with their <inline-formula><mml:math id="M1255" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M1256" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>
spread (light blue shading). The global <inline-formula><mml:math id="M1257" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (upper left) and the sum
of <inline-formula><mml:math id="M1258" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in all three regions represents the anthropogenic
atmosphere-to-ocean flux based on the assumption that the pre-industrial
ocean sink was 0 GtC yr<inline-formula><mml:math id="M1259" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> when riverine fluxes are not considered. This
assumption does not hold at the regional level, where pre-industrial fluxes
can be significantly different from zero. Hence, the regional panels for
<inline-formula><mml:math id="M1260" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> represent a combination of natural and anthropogenic fluxes.
Bias correction and area weighting were only applied to global <inline-formula><mml:math id="M1261" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>;
hence the sum of the regions is slightly different from the global estimate
(<inline-formula><mml:math id="M1262" display="inline"><mml:mo lspace="0mm">&lt;</mml:mo></mml:math></inline-formula> 0.06 GtC yr<inline-formula><mml:math id="M1263" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>).</p></caption>
            <?xmltex \igopts{width=426.791339pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f12.png"/>

          </fig>

</sec>
<sec id="Ch1.S3.SS7.SSS3">
  <label>3.7.3</label><title>Total atmosphere-to-ocean fluxes</title>
      <p id="d1e16924">For the 2011–2020 period, the GOBMs (2.5 <inline-formula><mml:math id="M1264" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6 GtC yr<inline-formula><mml:math id="M1265" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) produce
a lower estimate for the ocean sink than the <inline-formula><mml:math id="M1266" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1267" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products
(3.1 <inline-formula><mml:math id="M1268" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M1269" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), which shows up in Fig. 11 as a separate
peak in the distribution from the GOBMs (triangle symbols pointing right)
and from the <inline-formula><mml:math id="M1270" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1271" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based products (triangle symbols pointing left).
Atmospheric inversions (2.6 to 3.1 GtC yr<inline-formula><mml:math id="M1272" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) also suggest higher ocean
uptake in the recent decade (Fig. 11, Fig. 12 top row). In interpreting
these differences, we caution that the riverine transport of carbon taken up
on land and outgassing from the ocean is a substantial (0.6 GtC yr<inline-formula><mml:math id="M1273" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)
and uncertain term that separates the various methods. A recent estimate of
decadal ocean uptake from observed O<inline-formula><mml:math id="M1274" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> <inline-formula><mml:math id="M1275" display="inline"><mml:mo>/</mml:mo></mml:math></inline-formula> N<inline-formula><mml:math id="M1276" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> ratios (Tohjima et al.,
2019) also points towards a larger ocean sink, albeit with large uncertainty
(2012–2016: 3.1 <inline-formula><mml:math id="M1277" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1.5 GtC yr<inline-formula><mml:math id="M1278" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>).</p>
</sec>
<sec id="Ch1.S3.SS7.SSS4">
  <label>3.7.4</label><title>Regional breakdown and interannual variability</title>
      <p id="d1e17075">Figure 12 also shows the latitudinal partitioning of the total
atmosphere-to-surface fluxes excluding fossil CO<inline-formula><mml:math id="M1279" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
(<inline-formula><mml:math id="M1280" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) according to the multi-model
average estimates from GOBMs and ocean <inline-formula><mml:math id="M1281" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1282" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based products
(<inline-formula><mml:math id="M1283" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and DGVMs (<inline-formula><mml:math id="M1284" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), and from atmospheric
inversions (<inline-formula><mml:math id="M1285" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M1286" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>).</p>
</sec>
<sec id="Ch1.S3.SS7.SSSx1" specific-use="unnumbered">
  <title>North</title>
      <p id="d1e17194">Despite being one of the most densely observed and studied regions of our
globe, annual mean carbon sink estimates in the northern extra-tropics
(north of 30<inline-formula><mml:math id="M1287" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N) continue to differ by about 0.5 GtC yr<inline-formula><mml:math id="M1288" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.
The atmospheric inversions suggest an atmosphere-to-surface sink
(<inline-formula><mml:math id="M1289" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) for 2011–2020 of 2.0 to 3.4 GtC yr<inline-formula><mml:math id="M1290" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, which is higher than the process models' estimate of 2.1 <inline-formula><mml:math id="M1291" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M1292" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Fig. 12). The GOBMs (1.1 <inline-formula><mml:math id="M1293" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2 GtC yr<inline-formula><mml:math id="M1294" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>),
<inline-formula><mml:math id="M1295" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1296" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products (1.3 <inline-formula><mml:math id="M1297" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.1 GtC yr<inline-formula><mml:math id="M1298" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), and inversion
models (0.9 to 1.5 GtC yr<inline-formula><mml:math id="M1299" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) produce consistent estimates of the ocean
sink. Thus, the difference mainly arises from the total land flux
(<inline-formula><mml:math id="M1300" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) estimate, which is 1.0 <inline-formula><mml:math id="M1301" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.4 GtC yr<inline-formula><mml:math id="M1302" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
in the DGVMs compared to 0.7 to 2.4 GtC yr<inline-formula><mml:math id="M1303" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the atmospheric
inversions (Fig. 12, second row).</p>
      <p id="d1e17391">Discrepancies in the northern land fluxes conforms with persistent issues
surrounding the quantification of the drivers of the global net land
CO<inline-formula><mml:math id="M1304" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux (Arneth et al., 2017; Huntzinger et al., 2017) and the
distribution of atmosphere-to-land fluxes between the tropics and high
northern latitudes (Baccini et al., 2017; Schimel et al., 2015; Stephens et
al., 2007; Ciais et al., 2019; Gaubert et al., 2019).</p>
      <p id="d1e17403">In the northern extra-tropics, the process models, inversions, and
<inline-formula><mml:math id="M1305" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1306" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products consistently suggest that most of the
variability stems from the land (Fig. 12). Inversions generally estimate
similar interannual variations (IAV) over land to DGVMs (0.28–0.47 vs.
0.20–0.73 GtC yr<inline-formula><mml:math id="M1307" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, averaged over 1990–2020), and they have higher
IAV in ocean fluxes (0.03–0.19 GtC yr<inline-formula><mml:math id="M1308" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) relative to GOBMs (0.03–0.05 GtC yr<inline-formula><mml:math id="M1309" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Fig. B2) and <inline-formula><mml:math id="M1310" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1311" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products (0.03–0.09 GtC yr<inline-formula><mml:math id="M1312" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>).</p>
</sec>
<sec id="Ch1.S3.SS7.SSSx2" specific-use="unnumbered">
  <title>Tropics</title>
      <p id="d1e17493">In the tropics (30<inline-formula><mml:math id="M1313" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S–30<inline-formula><mml:math id="M1314" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N), both the atmospheric
inversions and process models estimate a total carbon balance
(<inline-formula><mml:math id="M1315" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) that is close to neutral over the past
decade. The GOBMs (0.0 <inline-formula><mml:math id="M1316" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M1317" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), <inline-formula><mml:math id="M1318" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1319" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data
products (0.03 <inline-formula><mml:math id="M1320" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.2 GtC yr<inline-formula><mml:math id="M1321" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), and inversion models (<inline-formula><mml:math id="M1322" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.2 to 0.2 GtC yr<inline-formula><mml:math id="M1323" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) all indicate an approximately neutral tropical ocean flux
(see Fig. B1 for spatial patterns). DGVMs indicate a net land sink
(<inline-formula><mml:math id="M1324" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) of 0.6 <inline-formula><mml:math id="M1325" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M1326" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, whereas the
inversion models indicate a net land flux between <inline-formula><mml:math id="M1327" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.7 and 0.9 GtC yr<inline-formula><mml:math id="M1328" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, though with high uncertainty (Fig. 12, third row).</p>
      <p id="d1e17670">The tropical lands are the origin of most of the atmospheric CO<inline-formula><mml:math id="M1329" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
interannual variability (Ahlström et al., 2015), consistently among the
process models and inversions (Fig. 12). The interannual variability in the
tropics is similar among the ocean data products (0.07–0.15 GtC yr<inline-formula><mml:math id="M1330" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)
and the models (0.07–0.15 GtC yr<inline-formula><mml:math id="M1331" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Fig. B2), which is the highest
ocean sink variability of all regions. The DGVMs and inversions indicate
that atmosphere-to-land CO<inline-formula><mml:math id="M1332" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes are more variable than
atmosphere-to-ocean CO<inline-formula><mml:math id="M1333" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes in the tropics, with interannual
variability of 0.4 to 1.2 and 0.6 to 1.1 GtC yr<inline-formula><mml:math id="M1334" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> respectively.</p>
</sec>
<sec id="Ch1.S3.SS7.SSSx3" specific-use="unnumbered">
  <title>South</title>
      <p id="d1e17743">In the southern extra-tropics (south of 30<inline-formula><mml:math id="M1335" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S), the atmospheric
inversions suggest a total atmosphere-to-surface sink
(<inline-formula><mml:math id="M1336" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) for 2011–2020 of 1.6 to 1.9 GtC yr<inline-formula><mml:math id="M1337" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, slightly higher than the process models' estimate of 1.4 <inline-formula><mml:math id="M1338" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M1339" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Fig. 12). An approximately neutral total land flux
(<inline-formula><mml:math id="M1340" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) for the southern extra-tropics is estimated by both
the DGVMs (0.02 <inline-formula><mml:math id="M1341" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.05 GtC yr<inline-formula><mml:math id="M1342" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and the inversion models (sink
of <inline-formula><mml:math id="M1343" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.1 to 0.2 GtC yr<inline-formula><mml:math id="M1344" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). This means nearly all carbon uptake is due to
oceanic sinks south of 30<inline-formula><mml:math id="M1345" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S. The southern ocean flux in the
<inline-formula><mml:math id="M1346" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1347" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products (1.7 <inline-formula><mml:math id="M1348" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.1 GtC yr<inline-formula><mml:math id="M1349" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and inversion
estimates (1.4 to 1.8 GtC yr<inline-formula><mml:math id="M1350" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) is higher than in the GOBMs (1.4 <inline-formula><mml:math id="M1351" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M1352" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) (Fig. 12, bottom row). This might be explained by the
data products potentially underestimating the winter CO<inline-formula><mml:math id="M1353" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> outgassing
south of the Polar Front (Bushinsky et al., 2019), by model biases, or by
the uncertainty in the regional distribution of the river flux adjustment
(Aumont et al., 2001; Lacroix et al., 2020) applied to <inline-formula><mml:math id="M1354" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1355" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data
products and inverse models to isolate the anthropogenic <inline-formula><mml:math id="M1356" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> flux.
CO<inline-formula><mml:math id="M1357" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes from this region are more sparsely sampled by all methods,
especially in wintertime (Fig. B1).</p>
      <p id="d1e17990">The interannual variability in the southern extra-tropics is low because of
the dominance of ocean area with low variability compared to land areas. The
split between land (<inline-formula><mml:math id="M1358" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and ocean (<inline-formula><mml:math id="M1359" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) shows a
substantial contribution to variability in the south coming from the land,
with no consistency between the DGVMs and the inversions or among
inversions. This is expected due to the difficulty of separating exactly the
land and oceanic fluxes when viewed from atmospheric observations alone. The
<inline-formula><mml:math id="M1360" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> interannual variability was found to be higher in the
<inline-formula><mml:math id="M1361" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1362" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products (0.09 to 0.14 GtC yr<inline-formula><mml:math id="M1363" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) compared to GOBMs
(0.04 to 0.06 GtC yr<inline-formula><mml:math id="M1364" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) in 1990–2020 (Fig. B2). Model subsampling
experiments recently illustrated that observation-based products may
overestimate decadal variability in the Southern Ocean carbon sink by 30 %
due to data sparsity, based on one data product with the highest decadal
variability (Gloege et al., 2021).</p>
</sec>
<sec id="Ch1.S3.SS7.SSSx4" specific-use="unnumbered">
  <title>Tropical vs. northern land uptake</title>
      <p id="d1e18080">A continuing conundrum is the partitioning of the global atmosphere–land
flux between the Northern Hemisphere land and the tropical land (Stephens et
al., 2017; Pan et al., 2011; Gaubert et al., 2019). It is of importance
because each region has its own history of land-use change, climate drivers,
and impact of increasing atmospheric CO<inline-formula><mml:math id="M1365" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and nitrogen deposition.
Quantifying the magnitude of each sink is a prerequisite to understanding
how each individual driver impacts the tropical and mid- to high-latitude carbon
balance.</p>
      <p id="d1e18092">We define the north–south (N–S) difference as net atmosphere–land flux north
of 30<inline-formula><mml:math id="M1366" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N minus the net atmosphere–land flux south of 30<inline-formula><mml:math id="M1367" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N. For the
inversions, the N–S difference ranges from <inline-formula><mml:math id="M1368" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.1 to 2.9 GtC yr<inline-formula><mml:math id="M1369" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> across this year's inversion ensemble with an equal preference
across models for either a small northern land sink and a tropical land sink
(small N–S difference), a medium northern land sink and a neutral tropical
land flux (medium N–S difference), or a large northern land sink and a
tropical land source (large N–S difference).</p>
      <p id="d1e18132">In the ensemble of DGVMs the N–S difference is 0.5 <inline-formula><mml:math id="M1370" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.5 GtC yr<inline-formula><mml:math id="M1371" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, a much narrower range than the one from inversions. Only three
DGVMs have a N–S difference larger than 1.0 GtC yr<inline-formula><mml:math id="M1372" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The larger
agreement across DGVMs than across inversions is to be expected as there is
no correlation between northern and tropical land sinks in the DGVMs as
opposed to the inversions where the sum of the two regions being
well-constrained leads to an anti-correlation between these two regions. The
much smaller spread in the N–S difference between the DGVMs could help to
scrutinize the inverse models further. For example, a large northern land
sink and a tropical land source in an inversion would suggest a large
sensitivity to CO<inline-formula><mml:math id="M1373" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fertilization (the dominant factor driving the land
sinks) for northern ecosystems, which would be not mirrored by tropical
ecosystems. Such a combination could be hard to reconcile with the process
understanding gained from the DGVMs ensembles and independent measurements
(e.g. free-air CO<inline-formula><mml:math id="M1374" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> enrichment experiments). Such investigations will be
further pursued in the upcoming assessment from REgional Carbon Cycle
Assessment and Processes (RECCAP2; Ciais et al., 2022).</p>
</sec>
</sec>
<sec id="Ch1.S3.SS8">
  <label>3.8</label><title>Closing the global carbon cycle</title>
<sec id="Ch1.S3.SS8.SSS1">
  <label>3.8.1</label><title>Partitioning of cumulative emissions and sink fluxes</title>
      <p id="d1e18200">The global carbon budget over the historical period (1850–2020) is shown in
Fig. 3.</p>
      <p id="d1e18203">Emissions during the period 1850–2020 amounted to 660 <inline-formula><mml:math id="M1375" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 65 GtC and
were partitioned among the atmosphere (270 <inline-formula><mml:math id="M1376" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 5 GtC; 41 %), ocean
(170 <inline-formula><mml:math id="M1377" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 35 GtC; 26 %), and the land (195 <inline-formula><mml:math id="M1378" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 45 GtC; 30 %). The
cumulative land sink is almost equal to the cumulative land-use emissions
(200 <inline-formula><mml:math id="M1379" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 65 GtC), making the global land nearly neutral over the whole
1850–2020 period.</p>
      <p id="d1e18241">The use of nearly independent estimates for the individual terms shows a
cumulative budget imbalance of 25 GtC (4 %) during 1850–2020 (Fig. 3,
Table 8), which, if correct, suggests that emissions are slightly too high
by the same proportion (4 %) or that the combined land and ocean sinks are
slightly underestimated (by about 7 %). The bulk of the imbalance could
originate from the estimation of large <inline-formula><mml:math id="M1380" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> between the mid-1920s and
the mid-1960s which is unmatched by a growth in atmospheric CO<inline-formula><mml:math id="M1381" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration as recorded in ice cores (Fig. 3). However, the known loss of
additional sink capacity of 30–40 GtC (over the 1850–2020 period) due to
reduced forest cover has not been accounted for in our method and would
further exacerbate the budget imbalance (Sect. 2.7.4).</p>
      <p id="d1e18264">For the more recent 1960–2020 period where direct atmospheric CO<inline-formula><mml:math id="M1382" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
measurements are available, 375 <inline-formula><mml:math id="M1383" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 20 GtC (82 %) of the total
emissions (<inline-formula><mml:math id="M1384" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) were caused by fossil CO<inline-formula><mml:math id="M1385" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
emissions, and 80 <inline-formula><mml:math id="M1386" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 45 GtC (18 %) by land-use change (Table 8). The
total emissions were partitioned among the atmosphere (205 <inline-formula><mml:math id="M1387" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 5 GtC;
47 %), ocean (115 <inline-formula><mml:math id="M1388" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 25 GtC; 25 %), and the land (135 <inline-formula><mml:math id="M1389" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 25 GtC; 30 %), with a near-zero unattributed budget imbalance. All components
except land-use change emissions have significantly grown since 1960, with
important interannual variability in the growth rate in atmospheric CO<inline-formula><mml:math id="M1390" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration and in the land CO<inline-formula><mml:math id="M1391" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (Fig. 4), and some decadal
variability in all terms (Table 6). Differences with previous budget
releases are documented in Fig. B5.</p>
      <p id="d1e18358">The global carbon budget averaged over the last decade (2011–2020) is shown
in Figs. 2 and 13b and Table 6. For this time period, 90 %
of the total emissions (<inline-formula><mml:math id="M1392" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) were from fossil CO<inline-formula><mml:math id="M1393" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
emissions (<inline-formula><mml:math id="M1394" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), and 10 % from land-use change (<inline-formula><mml:math id="M1395" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). The
total emissions were partitioned among the atmosphere (47 %), ocean
(26 %), and land (29 %), with a near-zero unattributed budget imbalance
(<inline-formula><mml:math id="M1396" display="inline"><mml:mo lspace="0mm">∼</mml:mo></mml:math></inline-formula> 3 %). For single years, the budget imbalance can be
larger (Fig. 4). For 2020, the combination of our sources and sinks
estimates leads to a <inline-formula><mml:math id="M1397" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of <inline-formula><mml:math id="M1398" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.8 GtC, suggesting an underestimation of
the anthropogenic sources (potentially <inline-formula><mml:math id="M1399" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), and/or an overestimation
of the combined land and ocean sinks</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F13"><?xmltex \currentcnt{13}?><?xmltex \def\figurename{Figure}?><label>Figure 13</label><caption><p id="d1e18449">Cumulative changes over the 1850–2020 period <bold>(a)</bold> and average
fluxes over the 2011–2020 period <bold>(b)</bold> for the anthropogenic perturbation
of the global carbon cycle. See the caption of Fig. 3 for key information
and the methods in text for full details.</p></caption>
            <?xmltex \igopts{width=241.848425pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f13.png"/>

          </fig>

</sec>
<sec id="Ch1.S3.SS8.SSS2">
  <label>3.8.2</label><title>Carbon budget imbalance</title>
      <p id="d1e18472">The carbon budget imbalance (<inline-formula><mml:math id="M1400" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; Eq. 1, Fig. 4) quantifies the mismatch
between the estimated total emissions and the estimated changes in the
atmosphere, land, and ocean reservoirs. The mean budget imbalance from 1960
to 2020 is very small (average of 0.03 GtC yr<inline-formula><mml:math id="M1401" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and shows no trend
over the full time series. The process models (GOBMs and DGVMs) and
data products have been selected to match observational constraints in the
1990s, but no further constraints have been applied to their representation
of trend and variability. Therefore, the near-zero mean and trend in the
budget imbalance is seen as evidence of a coherent community understanding
of the emissions and their partitioning on those timescales (Fig. 4).
However, the budget imbalance shows substantial variability of the order of
<inline-formula><mml:math id="M1402" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1 GtC yr<inline-formula><mml:math id="M1403" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, particularly over semi-decadal timescales,
although most of the variability is within the uncertainty of the estimates.
The positive carbon imbalance during the 1960s, and early 1990s, indicates
that either the emissions were overestimated, or the sinks were
underestimated during these periods. The reverse is true for the 1970s,
1980s, and for the 2011–2020 period (Fig. 4, Table 6).</p>
      <p id="d1e18517">We cannot attribute the cause of the variability in the budget imbalance
with our analysis; we only note that the budget imbalance is unlikely to be
explained by errors or biases in the emissions alone because of its large
semi-decadal variability component, a variability that is untypical of
emissions and has not changed in the past 60 years despite a near tripling
in emissions (Fig. 4). Errors in <inline-formula><mml:math id="M1404" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M1405" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are more likely
to be the main cause for the budget imbalance. For example, underestimation
of <inline-formula><mml:math id="M1406" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> by DGVMs has been reported following the eruption of Mount
Pinatubo in 1991 possibly due to missing responses to changes in diffuse
radiation (Mercado et al., 2009). Although in GCB2021 we have for the first
time accounted for aerosol effects on solar radiation quantity and quality
(diffuse vs. direct), most DGVMs only used the former as input (i.e. total
solar radiation). Thus, the ensemble mean may not capture the full effects
of volcanic eruptions, i.e. associated with high light scattering sulfate
aerosols, on the land carbon sink (O'Sullivan et al., 2021). DGVMs are
suspected to overestimate the land sink in response to the wet decade of the
1970s (Sitch et al., 2008). Quasi-decadal variability in the ocean sink has
also been reported, with all methods agreeing on a smaller than expected
ocean CO<inline-formula><mml:math id="M1407" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink in the 1990s and a larger than expected sink in the
2000s (Fig. 9; Landschützer et al., 2016; DeVries et al., 2019; Hauck et
al., 2020; McKinley et al., 2020). Errors in sink estimates could also be
driven by errors in the climatic forcing data, particularly precipitation
for <inline-formula><mml:math id="M1408" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and wind for <inline-formula><mml:math id="M1409" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e18585">The budget imbalance (<inline-formula><mml:math id="M1410" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) was negative (<inline-formula><mml:math id="M1411" display="inline"><mml:mo lspace="0mm">-</mml:mo></mml:math></inline-formula>0.3 GtC yr<inline-formula><mml:math id="M1412" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) on average
over 2011–2020, although the B<inline-formula><mml:math id="M1413" display="inline"><mml:msub><mml:mi/><mml:mrow><mml:mi>I</mml:mi><mml:mi>M</mml:mi></mml:mrow></mml:msub></mml:math></inline-formula> uncertainty is large (1.1 GtC yr<inline-formula><mml:math id="M1414" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> over the decade). Also, the <inline-formula><mml:math id="M1415" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> shows substantial
departure from zero on yearly timescales (Fig. 4), highlighting unresolved
variability of the carbon cycle, likely in the land sink (<inline-formula><mml:math id="M1416" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), given
its large year-to-year variability (Figs. 4e and 7).</p>
      <p id="d1e18665">Both the budget imbalance (<inline-formula><mml:math id="M1417" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, Table 6) and the residual land sink
from the global budget (<inline-formula><mml:math id="M1418" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>+</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub><mml:mo>-</mml:mo><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, Table 5) include an error term due to the inconsistencies that arise from using
<inline-formula><mml:math id="M1419" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from bookkeeping models, and <inline-formula><mml:math id="M1420" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from DGVMs, most notably
the loss of additional sink capacity (see Sect. 2.7). Other differences
include a better accounting of changing land-use practices and processes in
bookkeeping models than in DGVMs, or the bookkeeping models' error of having
present-day observed carbon densities fixed in the past. That the budget
imbalance shows no clear trend towards larger values over time is an
indication that these inconsistencies probably play a minor role compared to
other errors in <inline-formula><mml:math id="M1421" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> or <inline-formula><mml:math id="M1422" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e18757">Although the budget imbalance is near zero for the recent decades, it could
be due to compensation of errors. We cannot exclude an overestimation of
CO<inline-formula><mml:math id="M1423" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions, particularly from land-use change, given their large
uncertainty, as has been suggested elsewhere (Piao et al., 2018), combined
with an underestimate of the sinks. A larger <inline-formula><mml:math id="M1424" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> would reconcile
model results with inversion estimates for fluxes in the total land during
the past decade (Fig. 12; Table 5). Likewise, a larger <inline-formula><mml:math id="M1425" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is also
possible given the higher estimates from the data products (see Sect. 3.1.2, Figs. 9 and 12) and the recently suggested upward correction of
the ocean carbon sink (Watson et al., 2020, Fig. 9). If <inline-formula><mml:math id="M1426" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> were
to be based on data products alone, with all data products including the
Watson et al. (2020) adjustment, this would result in a 2011–2020
<inline-formula><mml:math id="M1427" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of nearly 4 GtC yr<inline-formula><mml:math id="M1428" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, outside of the range supported by the
atmospheric inversions, with a negative <inline-formula><mml:math id="M1429" display="inline"><mml:mrow><mml:msub><mml:mi>B</mml:mi><mml:mi mathvariant="normal">IM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of more than 1 GtC yr<inline-formula><mml:math id="M1430" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> indicating that a closure of the budget could only be achieved
with either anthropogenic emissions being larger and/or the net land sink
being substantially smaller than estimated here. More integrated use of
observations in the Global Carbon Budget, either on their own or for further
constraining model results, should help resolve some of the budget imbalance
(Peters et al., 2017).</p>
</sec>
</sec>
</sec>
<sec id="Ch1.S4">
  <label>4</label><title>Tracking progress towards mitigation targets</title>
      <p id="d1e18860">Fossil CO<inline-formula><mml:math id="M1431" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions growth peaked at <inline-formula><mml:math id="M1432" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>3 % yr<inline-formula><mml:math id="M1433" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> during the
2000s, driven by the rapid growth in Chinese emissions. In the last decade,
however, the growth rate for the preceding 10 years has slowly declined,
reaching a low <inline-formula><mml:math id="M1434" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>0.4 % yr<inline-formula><mml:math id="M1435" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> from 2012–2021 (including the 2020 global
decline and the expected 2021 emissions rebound). While this slowdown in
global fossil CO<inline-formula><mml:math id="M1436" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions growth is welcome, it is far from what is
needed to be consistent with the temperature goals of the Paris Agreement.</p>
      <p id="d1e18920">Since the 1990s, the average growth rate of fossil CO<inline-formula><mml:math id="M1437" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions has
continuously declined across the group of developed countries of the
Organisation for Economic Co-operation and Development (OECD), with
emissions peaking in around 2005 and now declining at around 1 % yr<inline-formula><mml:math id="M1438" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
(Le Quéré et al., 2021). In the decade 2010–2019, territorial fossil
CO<inline-formula><mml:math id="M1439" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions decreased significantly (at the 95 % confidence level)
in 23 countries whose economies grew significantly (also at the 95 %
confidence level): Barbados, Belgium, Croatia, Czech Republic, Denmark,
Finland, France, Germany, Israel, Japan, Luxembourg, North Macedonia, Malta,
Mexico, the Netherlands, Slovakia, Slovenia, Solomon Islands, Sweden,
Switzerland, Tuvalu, United Kingdom, and USA (updated from Le
Quéré et al., 2019). Altogether, these 23 countries contributed
2.5 GtC yr<inline-formula><mml:math id="M1440" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> over the last decade, about one-quarter of world CO<inline-formula><mml:math id="M1441" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
fossil emissions. Consumption-based emissions are also falling significantly
in 15 of these countries (Belgium, Croatia, Czech Republic, Denmark,
Finland, France, Germany, Israel, Japan, Mexico, the Netherlands, Slovenia,
Sweden, United Kingdom, and USA). Figure 14 shows that the emission
declines in the USA and the EU27 are primarily driven by increased
decarbonization (CO<inline-formula><mml:math id="M1442" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions per unit energy) in the last decade
compared to the previous, with smaller contributions in the EU27 from
slightly weaker economic growth and slightly larger declines in energy per
GDP. These countries have stable or declining energy use and so
decarbonization policies replace existing fossil fuel infrastructure (Le
Quéré et al., 2019).</p>

      <?xmltex \floatpos{t}?><fig id="Ch1.F14" specific-use="star"><?xmltex \currentcnt{14}?><?xmltex \def\figurename{Figure}?><label>Figure 14</label><caption><p id="d1e18986">Kaya decomposition of the main drivers of fossil CO<inline-formula><mml:math id="M1443" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
emissions, considering population, GDP per person, energy per GDP, and
CO<inline-formula><mml:math id="M1444" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions per energy use, for China <bold>(a)</bold>, USA <bold>(b)</bold>, EU27
<bold>(c)</bold>, India <bold>(d)</bold>, the rest of the world <bold>(e)</bold>, and the
world <bold>(f)</bold>. Black dots are the annual fossil CO<inline-formula><mml:math id="M1445" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
growth rate, coloured bars are the contributions from the different drivers.
A general trend is that population and GDP growth put upward pressure on
emissions, while energy per GDP and more recently CO<inline-formula><mml:math id="M1446" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions per
energy put downward pressure on emissions. The changes during 2020 led to a
stark contrast to previous years, with different drivers in each region.</p></caption>
        <?xmltex \igopts{width=455.244094pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f14.png"/>

      </fig>

      <p id="d1e19051">In contrast, fossil CO<inline-formula><mml:math id="M1447" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions continue to grow in non-OECD
countries, although the growth rate has slowed from over 5 % yr<inline-formula><mml:math id="M1448" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
during the 2000s to around 2 % yr<inline-formula><mml:math id="M1449" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the last decade. A large part
of this slowdown in non-OECD countries is due to China, which has seen
emissions growth declining from nearly 10 % yr<inline-formula><mml:math id="M1450" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the 2000s to
2 % yr<inline-formula><mml:math id="M1451" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the last decade. Excluding China, non-OECD emissions grew
at 3 % yr<inline-formula><mml:math id="M1452" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the 2000s compared to 2 % yr<inline-formula><mml:math id="M1453" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the last
decade. Figure 14 shows that compared to the previous decade, China has had
weaker economic growth in the last decade and a larger decarbonization rate,
with more rapid declines in energy per GDP which are now back to levels
during the 1990s. India and the rest of the world have strong economic
growth that is not compensated by decarbonization or declines in energy per
GDP, implying fossil CO<inline-formula><mml:math id="M1454" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions continue to grow. Despite the high
deployment of renewables in some countries (e.g. India), fossil energy
sources continue to grow to meet growing energy demand (Le Quéré et
al., 2019).</p>
      <p id="d1e19145">Globally, fossil CO<inline-formula><mml:math id="M1455" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions growth is slowing, and this is primarily
due to the emergence of climate policy and emission declines in OECD
countries (Eskander and Fankhauser, 2020). At the aggregated global level,
decarbonization shows a strong and growing signal in the last decade, with
smaller contributions from lower economic growth and declines in energy per
GDP. Despite the slowing growth in global fossil CO<inline-formula><mml:math id="M1456" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions,
emissions are still growing, far from the reductions needed to meet the
ambitious climate goals of the UNFCCC Paris agreement.</p>
      <p id="d1e19166">We update the remaining carbon budget assessed by the IPCC AR6 (Canadell et
al., 2022), accounting for the 2020 and estimated 2021 emissions from fossil
fuel combustion (<inline-formula><mml:math id="M1457" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and land-use changes (<inline-formula><mml:math id="M1458" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). From January
2022, the remaining carbon (50 % likelihood) for limiting global warming
to 1.5, 1.7, and 2 <inline-formula><mml:math id="M1459" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>C is estimated to
amount to 120, 210, and 350 GtC (420, 770, 1270 GtCO<inline-formula><mml:math id="M1460" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>). These numbers
include an uncertainty based on model spread (as in IPCC AR6), which is
reflected through the percent likelihood of exceeding the given temperature
threshold. These remaining amounts correspond respectively to about 11, 20,
and 32 years from the beginning of 2022, at the 2021 level of total CO<inline-formula><mml:math id="M1461" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
emissions. Reaching net-zero CO<inline-formula><mml:math id="M1462" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions by 2050 entails cutting
total anthropogenic CO<inline-formula><mml:math id="M1463" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions by about 0.4 GtC (1.4 GtCO<inline-formula><mml:math id="M1464" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>)
each year on average, comparable to the decrease during 2020.</p>
</sec>
<sec id="Ch1.S5">
  <label>5</label><title>Discussion</title>
      <p id="d1e19254">Each year when the global carbon budget is published, each flux component is
updated for all previous years to consider corrections that are the result
of further scrutiny and verification of the underlying data in the primary
input datasets. Annual estimates may be updated with improvements in data
quality and timeliness (e.g. to eliminate the need for extrapolation of
forcing data such as land use). Of all terms in the global budget, only the
fossil CO<inline-formula><mml:math id="M1465" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions and the growth rate in atmospheric CO<inline-formula><mml:math id="M1466" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration are based primarily on empirical inputs supporting annual
estimates in this carbon budget. The carbon budget imbalance, yet an
imperfect measure, provides a strong indication of the limitations in
observations in understanding and representing processes in models, and/or
in the integration of the carbon budget components.</p>
      <p id="d1e19275">The persistent unexplained variability in the carbon budget imbalance limits
our ability to verify reported emissions (Peters et al., 2017) and suggests
we do not yet have a complete understanding of the underlying carbon cycle
dynamics on annual to decadal timescales. Resolving most of this unexplained
variability should be possible through different and complementary
approaches. First, as intended with our annual updates, the imbalance as an
error term is reduced by improvements of individual components of the global
carbon budget that follow from improving the underlying data and statistics
and by improving the models through the resolution of some of the key
uncertainties detailed in Table 9. Second, additional clues to the origin
and processes responsible for the variability in the budget imbalance could
be obtained through a closer scrutiny of carbon variability in light of
other Earth system data (e.g. heat balance, water balance), and the use of
a wider range of biogeochemical observations to better understand the
land–ocean partitioning of the carbon imbalance (e.g. oxygen, carbon
isotopes). Finally, additional information could also be obtained through
higher resolution and process knowledge at the regional level, and through
the introduction of inferred fluxes such as those based on satellite
CO<inline-formula><mml:math id="M1467" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> retrievals. The limit of the resolution of the carbon budget
imbalance is yet unclear, but most certainly not yet reached given the
possibilities for improvements that lie ahead.</p>

<?xmltex \floatpos{p}?><table-wrap id="Ch1.T10" specific-use="star"><?xmltex \currentcnt{9}?><label>Table 9</label><caption><p id="d1e19290">Major known sources of uncertainties in each component of the Global Carbon Budget, defined as input data or processes that have a demonstrated effect of at least <inline-formula><mml:math id="M1468" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.3 GtC yr<inline-formula><mml:math id="M1469" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.9}[.9]?><oasis:tgroup cols="5">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="3.6cm"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="3.2cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="3.6cm"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="5" colname="col5" align="justify" colwidth="3.4cm"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Source of uncertainty</oasis:entry>
         <oasis:entry colname="col2">Timescale (years)</oasis:entry>
         <oasis:entry colname="col3">Location</oasis:entry>
         <oasis:entry colname="col4">Status</oasis:entry>
         <oasis:entry colname="col5">Evidence</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col5" align="left">Fossil CO<inline-formula><mml:math id="M1474" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (EFOS; Sect. 2.1) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Energy statistics</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">global, but mainly China and major developing countries</oasis:entry>
         <oasis:entry colname="col4">see Sect. 2.1</oasis:entry>
         <oasis:entry colname="col5">Korsbakken et al. (2016); Guan et al. (2012)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Carbon content of coal</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">global, but mainly China and major developing countries</oasis:entry>
         <oasis:entry colname="col4">see Sect. 2.1</oasis:entry>
         <oasis:entry colname="col5">Liu et al. (2015)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">System boundary</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">all countries</oasis:entry>
         <oasis:entry colname="col4">see Sect. 2.1</oasis:entry>
         <oasis:entry colname="col5">Andrew (2020a)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col5" align="left">Net land-use change flux (<inline-formula><mml:math id="M1475" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; Sect. 2.2) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Land-cover and land-use<?xmltex \hack{\hfill\break}?>change statistics</oasis:entry>
         <oasis:entry colname="col2">continuous</oasis:entry>
         <oasis:entry colname="col3">global; in particular tropics</oasis:entry>
         <oasis:entry colname="col4">see Sect. 2.2</oasis:entry>
         <oasis:entry colname="col5">Houghton et al. (2012);<?xmltex \hack{\hfill\break}?>Gasser et al. (2020)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Sub-grid-scale transitions</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">global</oasis:entry>
         <oasis:entry colname="col4">see Table A1</oasis:entry>
         <oasis:entry colname="col5">Wilkenskjeld et al. (2014)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Vegetation biomass</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">global; in particular tropics</oasis:entry>
         <oasis:entry colname="col4">see Table A1</oasis:entry>
         <oasis:entry colname="col5">Houghton et al. (2012)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Forest degradation (fire,<?xmltex \hack{\hfill\break}?>selective logging)</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">tropics</oasis:entry>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5">Aragão et al. (2018); Qin et al. (2020)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Wood and crop harvest</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">global; SE Asia</oasis:entry>
         <oasis:entry colname="col4">see Table A1</oasis:entry>
         <oasis:entry colname="col5">Arneth et al. (2017); Erb et al. (2018)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Peat burning<inline-formula><mml:math id="M1476" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">multi-decadal trend</oasis:entry>
         <oasis:entry colname="col3">global</oasis:entry>
         <oasis:entry colname="col4">see Table A1</oasis:entry>
         <oasis:entry colname="col5">van der Werf et al. (2010, 2017)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Loss of additional sink <?xmltex \hack{\hfill\break}?>capacity</oasis:entry>
         <oasis:entry colname="col2">multi-decadal trend</oasis:entry>
         <oasis:entry colname="col3">global</oasis:entry>
         <oasis:entry colname="col4">not included; see<?xmltex \hack{\hfill\break}?>Appendix D1.4</oasis:entry>
         <oasis:entry colname="col5">Pongratz et al. (2014);<?xmltex \hack{\hfill\break}?>Gasser et al. (2020), Obermeier et al. (2021)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col5" align="left">Atmospheric growth rate (GATM; Sect. 2.3) no demonstrated uncertainties larger than <inline-formula><mml:math id="M1477" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.3 GtC yr<inline-formula><mml:math id="M1478" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula><inline-formula><mml:math id="M1479" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col5" align="left">Ocean sink (<inline-formula><mml:math id="M1480" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; Sect. 2.4) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Sparsity in surface <inline-formula><mml:math id="M1481" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1482" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula><?xmltex \hack{\hfill\break}?>observations</oasis:entry>
         <oasis:entry colname="col2">mean, decadal variability and trend</oasis:entry>
         <oasis:entry colname="col3">global, in particular Southern Hemisphere</oasis:entry>
         <oasis:entry colname="col4">see Sect. 3.5.2</oasis:entry>
         <oasis:entry colname="col5">Gloege et al. (2021),<?xmltex \hack{\hfill\break}?>Denvil-Sommer et<?xmltex \hack{\hfill\break}?>al. (2019), Bushinsky et al. (2019)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Riverine carbon outgassing and its anthropogenic perturbation</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">global, in particular partitioning between tropics and south</oasis:entry>
         <oasis:entry colname="col4">see Sect. 2.4 (anthropogenic perturbations<?xmltex \hack{\hfill\break}?>not included)</oasis:entry>
         <oasis:entry colname="col5">Aumont et al. (2001), Resplandy et al. (2018), Lacroix et al. (2020)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Interior ocean<?xmltex \hack{\hfill\break}?>anthropogenic carbon<?xmltex \hack{\hfill\break}?>storage</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">global</oasis:entry>
         <oasis:entry colname="col4">see Sect. 3.5.5</oasis:entry>
         <oasis:entry colname="col5">Gruber et al. (2019)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Near-surface temperature<?xmltex \hack{\hfill\break}?>and salinity gradients</oasis:entry>
         <oasis:entry colname="col2">mean on all timescales</oasis:entry>
         <oasis:entry colname="col3">global</oasis:entry>
         <oasis:entry colname="col4">see Sect. 3.8.2</oasis:entry>
         <oasis:entry colname="col5">Watson et al. (2020)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col5" align="left">Land sink (<inline-formula><mml:math id="M1483" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; Sect. 2.5) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Strength of CO<inline-formula><mml:math id="M1484" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fertilization</oasis:entry>
         <oasis:entry colname="col2">multi-decadal trend</oasis:entry>
         <oasis:entry colname="col3">global</oasis:entry>
         <oasis:entry colname="col4">see Sect. 2.5</oasis:entry>
         <oasis:entry colname="col5">Wenzel et al. (2016); <?xmltex \hack{\hfill\break}?>Walker et al. (2021)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Response to variability in <?xmltex \hack{\hfill\break}?>temperature and rainfall</oasis:entry>
         <oasis:entry colname="col2">annual to decadal</oasis:entry>
         <oasis:entry colname="col3">global; in particular tropics</oasis:entry>
         <oasis:entry colname="col4">see Sect. 2.5</oasis:entry>
         <oasis:entry colname="col5">Cox et al. (2013); Jung et al. (2017); Humphrey et al. (2018, 2021)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Nutrient limitation and<?xmltex \hack{\hfill\break}?>supply</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Tree mortality</oasis:entry>
         <oasis:entry colname="col2">annual</oasis:entry>
         <oasis:entry colname="col3">global in particular tropics</oasis:entry>
         <oasis:entry colname="col4">see Sect. 2.5</oasis:entry>
         <oasis:entry colname="col5">Hubau et al. (2021); <?xmltex \hack{\hfill\break}?>Brienen et al. (2020)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Response to diffuse<?xmltex \hack{\hfill\break}?>radiation</oasis:entry>
         <oasis:entry colname="col2">annual</oasis:entry>
         <oasis:entry colname="col3">global</oasis:entry>
         <oasis:entry colname="col4">see Sect. 2.5</oasis:entry>
         <oasis:entry colname="col5">Mercado et al. (2009); <?xmltex \hack{\hfill\break}?>O'Sullivan et al. (2021)</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table><table-wrap-foot><p id="d1e19312"><inline-formula><mml:math id="M1470" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula> As result of interactions between land use and climate. <inline-formula><mml:math id="M1471" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> The uncertainties in GATM have been estimated as <inline-formula><mml:math id="M1472" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.2 GtC yr<inline-formula><mml:math id="M1473" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, although the conversion of the growth rate into<?xmltex \hack{\break}?> a global annual flux assuming instantaneous mixing throughout the atmosphere introduces additional errors that have not yet been quantified.</p></table-wrap-foot></table-wrap>

      <p id="d1e19903">Estimates of global fossil CO<inline-formula><mml:math id="M1485" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from different datasets are in
relatively good agreement when the different system boundaries of these
datasets are considered (Andrew, 2020a). But while estimates of <inline-formula><mml:math id="M1486" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
are derived from reported activity data requiring much fewer complex
transformations than some other components of the budget, uncertainties
remain, and one reason for the apparently low variation between datasets is
precisely the reliance on the same underlying reported energy data. The
budget excludes some sources of fossil CO<inline-formula><mml:math id="M1487" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions, which available
evidence suggests are relatively small (<inline-formula><mml:math id="M1488" display="inline"><mml:mo lspace="0mm">&lt;</mml:mo></mml:math></inline-formula> 1 %). We have added
emissions from lime production in China and the US, but these are still
absent in most other non-Annex I countries, and before 1990 in other Annex I
countries. Further changes to <inline-formula><mml:math id="M1489" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> this year are documented by Andrew
and Peters (2021).</p>
      <p id="d1e19953">Estimates of <inline-formula><mml:math id="M1490" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> suffer from a range of intertwined issues, including
the poor quality of historical land-cover and land-use change maps, the
rudimentary representation of management processes in most models, and the
confusion in methodologies and boundary conditions used across methods
(e.g. Arneth et al., 2017; Pongratz et al., 2014; see also Sect. 2.7.4 on
the loss of sink capacity; Bastos et al., 2021). Uncertainties in current
and historical carbon stocks in soils and vegetation also add uncertainty in
the <inline-formula><mml:math id="M1491" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimates. Unless a major effort to resolve these issues is
made, little progress is expected in the resolution of <inline-formula><mml:math id="M1492" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. This is
particularly concerning given the growing importance of <inline-formula><mml:math id="M1493" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for
climate mitigation strategies, and the large issues in the quantification of
the cumulative emissions over the historical period that arise from large
uncertainties in <inline-formula><mml:math id="M1494" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e20011">By adding the DGVM estimates of CO<inline-formula><mml:math id="M1495" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes due to environmental change
from countries' managed forest areas (part of <inline-formula><mml:math id="M1496" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in this budget)
to the budget <inline-formula><mml:math id="M1497" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate, we successfully reconciled the large gap
between our <inline-formula><mml:math id="M1498" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate and the land-use flux from NGHGIs using the
approach described in Grassi et al. (2021). This latter estimate has been
used in the recent UNFCCC's Synthesis Report on Nationally Determined
Contribution (UNFCCC, 2021b) to enable the total national emission estimates
to be comparable with those of the IPCC. However, while Grassi et al. (2021)
used only one DGVM, here 17 DGVMs are used, thus providing a more robust
value to be used as potential adjustment in the policy context, e.g. to
help assessing the collective countries' progress towards the goal of the
Paris Agreement and avoiding double-accounting for the sink in managed
forests. In the absence of this adjustment, collective progress would hence
appear better than it is (Grassi et al., 2021).</p>
      <p id="d1e20056">The comparison of GOBMs, data products, and inversions highlights substantial
discrepancy in the Southern Ocean (Fig. 12, Hauck et al., 2020). The
long-standing sparse data coverage of <inline-formula><mml:math id="M1499" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1500" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> observations in the Southern
compared to the Northern Hemisphere (e.g. Takahashi et al., 2009) continues
to exist (Bakker et al., 2016, 2021, Fig. B1) and to lead to substantially
higher uncertainty in the <inline-formula><mml:math id="M1501" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate for the Southern Hemisphere
(Watson et al., 2020; Gloege et al., 2021). This discrepancy, which also
hampers model improvement, points to the need for increased high-quality
<inline-formula><mml:math id="M1502" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1503" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> observations, especially in the Southern Ocean. At the same time,
model uncertainty is illustrated by the large spread of individual GOBM
estimates (indicated by shading in Fig. 12) and highlights the need for
model improvement. Further uncertainty stems from the regional distribution
of the river flux adjustment term being based on one model study yielding
the largest riverine outgassing flux south of 20<inline-formula><mml:math id="M1504" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S (Aumont et
al., 2001), with a recent study questioning this distribution (Lacroix et
al., 2020). The diverging trends in <inline-formula><mml:math id="M1505" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from different methods is a
matter of concern, which is unresolved. The assessment of the net
land–atmosphere exchange from DGVMs and atmospheric inversions also shows
substantial discrepancy, particularly for the estimate of the total land
flux over the northern extra-tropics. This discrepancy highlights the
difficulty of quantifying complex processes (CO<inline-formula><mml:math id="M1506" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fertilization, nitrogen
deposition and fertilizers, climate change and variability, land management,
etc.) that collectively determine the net land CO<inline-formula><mml:math id="M1507" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux. Resolving the
differences in the Northern Hemisphere land sink will require the
consideration and inclusion of larger volumes of observations.</p>
      <p id="d1e20141">We provide metrics for the evaluation of the ocean and land models and the
atmospheric inversions (Figs. B2 to B4). These metrics expand the use of
observations in the global carbon budget, helping (1) to support improvements
in the ocean and land carbon models that produce the sink estimates, and (2) to constrain the representation of key underlying processes in the models
and to allocate the regional partitioning of the CO<inline-formula><mml:math id="M1508" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes. However,
GOBM skills have changed little since the introduction of the ocean model
evaluation. An additional simulation this year allows for direct comparison
with interior ocean anthropogenic carbon estimates and suggests that the
models underestimate anthropogenic carbon uptake and storage. This is an
initial step towards the introduction of a broader range of observations
that we hope will support continued improvements in the annual estimates of
the global carbon budget.</p>
      <p id="d1e20153">We assessed before that a sustained decrease of <inline-formula><mml:math id="M1509" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1 % in global emissions
could be detected at the 66 % likelihood level after a decade only (Peters
et al., 2017). Similarly, a change in behaviour of the land and/or ocean
carbon sink would take as long to detect, and much longer if it emerges more
slowly. To continue reducing the carbon imbalance on annual to decadal timescales, regionalizing the carbon budget and integrating multiple variables
are powerful ways to shorten the detection limit and ensure the research
community can rapidly identify issues of concern in the evolution of the
global carbon cycle under the current rapid and unprecedented changing
environmental conditions.</p>
</sec>
<sec id="Ch1.S6" sec-type="conclusions">
  <label>6</label><title>Conclusions</title>
      <p id="d1e20171">The estimation of global CO<inline-formula><mml:math id="M1510" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions and sinks is a major effort by
the carbon cycle research community that requires a careful compilation and
synthesis of measurements, statistical estimates, and model results. The
delivery of an annual carbon budget serves two purposes. First, there is a
large demand for up-to-date information on the state of the anthropogenic
perturbation of the climate system and its underpinning causes. A broad
stakeholder community relies on the datasets associated with the annual
carbon budget including scientists, policy makers, businesses, journalists,
and non-governmental organizations engaged in adapting to and mitigating
human-driven climate change. Second, over the last decades we have seen
unprecedented changes in the human and biophysical environments (e.g.
changes in the growth of fossil fuel emissions, impact of COVID-19 pandemic,
Earth's warming, and strength of the carbon sinks), which call for frequent
assessments of the state of the planet, a better quantification of the
causes of changes in the contemporary global carbon cycle, and an improved
capacity to anticipate its evolution in the future. Building this scientific
understanding to meet the extraordinary climate mitigation challenge
requires frequent, robust, transparent, and traceable datasets and methods
that can be scrutinized and replicated. This paper via “living data” helps
to keep track of new budget updates.</p>
</sec>
<sec id="Ch1.S7">
  <label>7</label><title>Data availability</title>
      <p id="d1e20191">The data presented here are made available in the belief that their wide
dissemination will lead to greater understanding and new scientific insights
into how the carbon cycle works, how humans are altering it, and how we can
mitigate the resulting human-driven climate change. Full contact details and
information on how to cite the data shown here are given at the top of each
page in the accompanying database and summarized in Table 2.</p>
      <p id="d1e20194">The accompanying database includes two Excel files organized in the
following spreadsheets:</p>
      <p id="d1e20197">The file Global_Carbon_Budget_2021v1.0.xlsx includes the following:
<list list-type="order"><list-item>
      <p id="d1e20202">summary;</p></list-item><list-item>
      <p id="d1e20206">the global carbon budget (1959–2020);</p></list-item><list-item>
      <p id="d1e20210">the historical global carbon budget (1750–2020);</p></list-item><list-item>
      <p id="d1e20214">global CO<inline-formula><mml:math id="M1511" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from fossil fuels and cement production by fuel
type, and the per capita emissions (1959–2020);</p></list-item><list-item>
      <p id="d1e20227">CO<inline-formula><mml:math id="M1512" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from land-use change from the individual methods and
models (1959–2020);</p></list-item><list-item>
      <p id="d1e20240">ocean CO<inline-formula><mml:math id="M1513" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink from the individual ocean models and <inline-formula><mml:math id="M1514" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1515" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based
products (1959–2020);</p></list-item><list-item>
      <p id="d1e20269">terrestrial CO<inline-formula><mml:math id="M1516" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink from the DGVMs (1959–2020).</p></list-item></list><?xmltex \hack{\newpage}?>
The file National_Carbon_Emissions_2021v1.0.xlsx includes the following:
<list list-type="order"><list-item>
      <p id="d1e20285">summary;</p></list-item><list-item>
      <p id="d1e20289">territorial country CO<inline-formula><mml:math id="M1517" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from fossil CO<inline-formula><mml:math id="M1518" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
(1959–2020);</p></list-item><list-item>
      <p id="d1e20311">consumption country CO<inline-formula><mml:math id="M1519" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from fossil CO<inline-formula><mml:math id="M1520" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions and
emissions transfer from the international trade of goods and services
(1990–2019) using CDIAC/UNFCCC data as reference;</p></list-item><list-item>
      <p id="d1e20333">emissions transfers (Consumption minus territorial emissions; 1990–2019);</p></list-item><list-item>
      <p id="d1e20337">country definitions;</p></list-item><list-item>
      <p id="d1e20341">details of disaggregated countries;</p></list-item><list-item>
      <p id="d1e20345">details of aggregated countries.</p></list-item></list>
Both spreadsheets are published by the Integrated Carbon Observation System
(ICOS) Carbon Portal and are available at <ext-link xlink:href="https://doi.org/10.18160/gcp-2021" ext-link-type="DOI">10.18160/gcp-2021</ext-link> (Friedlingstein et al., 2021). National
emissions data are also available from the Global Carbon Atlas
(<uri>http://www.globalcarbonatlas.org/</uri>, last access: 11 March 2022) and from Our
World in Data (<uri>https://ourworldindata.org/CO2-emissions</uri>, last access: 11
March 2022).</p><?xmltex \hack{\clearpage}?>
</sec>

      
      </body>
    <back><app-group>

<app id="App1.Ch1.S1">
  <?xmltex \currentcnt{A}?><label>Appendix A</label><title>Supplementary tables</title><?xmltex \hack{\begin{turn}{90}\begin{minipage}{.95\textheight}}?><?xmltex \floatpos{H}?><table-wrap id="App1.Ch1.S1.T11" position="anchor"><?xmltex \def\@captype{table}?><?xmltex \currentcnt{A1}?><label>Table A1</label><caption><p id="d1e20374">Comparison of the processes included in the bookkeeping method and DGVMs in their estimates of <inline-formula><mml:math id="M1521" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M1522" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. See Table 4 for model references. All models include deforestation and forest regrowth after abandonment of agriculture (or from afforestation activities on agricultural land). Processes relevant for <inline-formula><mml:math id="M1523" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> are only described for the DGVMs used with land-cover change in this study. n/a – not applicable </p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.6}[.6]?><oasis:tgroup cols="21">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="left" colsep="1"/>
     <oasis:colspec colnum="5" colname="col5" align="left"/>
     <oasis:colspec colnum="6" colname="col6" align="left"/>
     <oasis:colspec colnum="7" colname="col7" align="left"/>
     <oasis:colspec colnum="8" colname="col8" align="left"/>
     <oasis:colspec colnum="9" colname="col9" align="left"/>
     <oasis:colspec colnum="10" colname="col10" align="left"/>
     <oasis:colspec colnum="11" colname="col11" align="left"/>
     <oasis:colspec colnum="12" colname="col12" align="left"/>
     <oasis:colspec colnum="13" colname="col13" align="left"/>
     <oasis:colspec colnum="14" colname="col14" align="left"/>
     <oasis:colspec colnum="15" colname="col15" align="left"/>
     <oasis:colspec colnum="16" colname="col16" align="left"/>
     <oasis:colspec colnum="17" colname="col17" align="left"/>
     <oasis:colspec colnum="18" colname="col18" align="left"/>
     <oasis:colspec colnum="19" colname="col19" align="left"/>
     <oasis:colspec colnum="20" colname="col20" align="left"/>
     <oasis:colspec colnum="21" colname="col21" align="left"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry rowsep="1" namest="col2" nameend="col4" align="center" colsep="1">Bookkeeping models </oasis:entry>
         <oasis:entry rowsep="1" namest="col5" nameend="col21" align="center">DGVMs </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">H&amp;N</oasis:entry>
         <oasis:entry colname="col3">BLUE</oasis:entry>
         <oasis:entry colname="col4">OSCAR</oasis:entry>
         <oasis:entry colname="col5">CABLE-</oasis:entry>
         <oasis:entry colname="col6">CLASSIC</oasis:entry>
         <oasis:entry colname="col7">CLM5.0</oasis:entry>
         <oasis:entry colname="col8">DLEM</oasis:entry>
         <oasis:entry colname="col9">IBIS</oasis:entry>
         <oasis:entry colname="col10">ISAM</oasis:entry>
         <oasis:entry colname="col11">ISBA-</oasis:entry>
         <oasis:entry colname="col12">JSBACH</oasis:entry>
         <oasis:entry colname="col13">JULES-</oasis:entry>
         <oasis:entry colname="col14">LPJ-</oasis:entry>
         <oasis:entry colname="col15">LPJ</oasis:entry>
         <oasis:entry colname="col16">LPX-</oasis:entry>
         <oasis:entry colname="col17">OCNv2</oasis:entry>
         <oasis:entry colname="col18">ORCHIDEEv3</oasis:entry>
         <oasis:entry colname="col19">SDGVM</oasis:entry>
         <oasis:entry colname="col20">VISIT</oasis:entry>
         <oasis:entry colname="col21">YIBs</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5">POP</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
         <oasis:entry colname="col10"/>
         <oasis:entry colname="col11">CTRIP<inline-formula><mml:math id="M1524" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">h</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12"/>
         <oasis:entry colname="col13">ES</oasis:entry>
         <oasis:entry colname="col14">GUESS</oasis:entry>
         <oasis:entry colname="col15"/>
         <oasis:entry colname="col16">Bern</oasis:entry>
         <oasis:entry colname="col17"/>
         <oasis:entry colname="col18"/>
         <oasis:entry colname="col19"/>
         <oasis:entry colname="col20"/>
         <oasis:entry colname="col21"/>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col21" align="left">Processes relevant for <inline-formula><mml:math id="M1525" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Wood harvest and<?xmltex \hack{\hfill\break}?>forest degradation<inline-formula><mml:math id="M1526" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">yes</oasis:entry>
         <oasis:entry colname="col3">yes</oasis:entry>
         <oasis:entry colname="col4">yes</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">yes</oasis:entry>
         <oasis:entry colname="col8">yes</oasis:entry>
         <oasis:entry colname="col9">yes</oasis:entry>
         <oasis:entry colname="col10">yes</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">yes</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">yes</oasis:entry>
         <oasis:entry colname="col15">yes</oasis:entry>
         <oasis:entry colname="col16">no<inline-formula><mml:math id="M1527" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col17">yes</oasis:entry>
         <oasis:entry colname="col18">yes</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">yes</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Shifting cultivation/ <?xmltex \hack{\hfill\break}?>Sub-grid-scale<?xmltex \hack{\hfill\break}?>transitions</oasis:entry>
         <oasis:entry colname="col2">no<inline-formula><mml:math id="M1528" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">yes</oasis:entry>
         <oasis:entry colname="col4">yes</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">yes</oasis:entry>
         <oasis:entry colname="col8">no</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">no</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">yes</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">yes</oasis:entry>
         <oasis:entry colname="col15">yes</oasis:entry>
         <oasis:entry colname="col16">no<inline-formula><mml:math id="M1529" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col17">no</oasis:entry>
         <oasis:entry colname="col18">no</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">yes</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Cropland harvest <?xmltex \hack{\hfill\break}?>(removed, R, or<?xmltex \hack{\hfill\break}?>added to litter, L)</oasis:entry>
         <oasis:entry colname="col2">yes (R) (z)</oasis:entry>
         <oasis:entry colname="col3">yes (R) (z)</oasis:entry>
         <oasis:entry colname="col4">yes (R)</oasis:entry>
         <oasis:entry colname="col5">yes (R)</oasis:entry>
         <oasis:entry colname="col6">yes  (l)</oasis:entry>
         <oasis:entry colname="col7">yes (R)</oasis:entry>
         <oasis:entry colname="col8">yes</oasis:entry>
         <oasis:entry colname="col9">yes (R)</oasis:entry>
         <oasis:entry colname="col10">yes</oasis:entry>
         <oasis:entry colname="col11">yes (R<inline-formula><mml:math id="M1530" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>L)</oasis:entry>
         <oasis:entry colname="col12">yes (R<inline-formula><mml:math id="M1531" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>L)</oasis:entry>
         <oasis:entry colname="col13">yes (R)</oasis:entry>
         <oasis:entry colname="col14">yes (R)</oasis:entry>
         <oasis:entry colname="col15">yes  (l)</oasis:entry>
         <oasis:entry colname="col16">yes (R)</oasis:entry>
         <oasis:entry colname="col17">yes (R<inline-formula><mml:math id="M1532" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>L)</oasis:entry>
         <oasis:entry colname="col18">yes (R)</oasis:entry>
         <oasis:entry colname="col19">yes (R)</oasis:entry>
         <oasis:entry colname="col20">yes (R)</oasis:entry>
         <oasis:entry colname="col21">yes (L)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Peat fires</oasis:entry>
         <oasis:entry colname="col2">yes</oasis:entry>
         <oasis:entry colname="col3">yes</oasis:entry>
         <oasis:entry colname="col4">yes</oasis:entry>
         <oasis:entry colname="col5">no</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">yes</oasis:entry>
         <oasis:entry colname="col8">no</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">no</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">no</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">no</oasis:entry>
         <oasis:entry colname="col15">no</oasis:entry>
         <oasis:entry colname="col16">no</oasis:entry>
         <oasis:entry colname="col17">no</oasis:entry>
         <oasis:entry colname="col18">no</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">no</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Fire as a<?xmltex \hack{\hfill\break}?>management  tool</oasis:entry>
         <oasis:entry colname="col2">yes (z)</oasis:entry>
         <oasis:entry colname="col3">yes (z)</oasis:entry>
         <oasis:entry colname="col4">yes<inline-formula><mml:math id="M1533" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">no</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">no</oasis:entry>
         <oasis:entry colname="col8">no</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">no</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">no</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">no</oasis:entry>
         <oasis:entry colname="col15">no</oasis:entry>
         <oasis:entry colname="col16">no</oasis:entry>
         <oasis:entry colname="col17">no</oasis:entry>
         <oasis:entry colname="col18">no</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">no</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">N fertilization</oasis:entry>
         <oasis:entry colname="col2">yes (z)</oasis:entry>
         <oasis:entry colname="col3">yes (z)</oasis:entry>
         <oasis:entry colname="col4">yes<inline-formula><mml:math id="M1534" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">no</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">yes</oasis:entry>
         <oasis:entry colname="col8">yes</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">yes</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">no</oasis:entry>
         <oasis:entry colname="col13">yes<inline-formula><mml:math id="M1535" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">k</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col14">yes</oasis:entry>
         <oasis:entry colname="col15">no</oasis:entry>
         <oasis:entry colname="col16">yes</oasis:entry>
         <oasis:entry colname="col17">yes</oasis:entry>
         <oasis:entry colname="col18">yes</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">no</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Tillage</oasis:entry>
         <oasis:entry colname="col2">yes (z)</oasis:entry>
         <oasis:entry colname="col3">yes (z)</oasis:entry>
         <oasis:entry colname="col4">yes<inline-formula><mml:math id="M1536" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">no</oasis:entry>
         <oasis:entry colname="col6">yes<inline-formula><mml:math id="M1537" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">g</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">no</oasis:entry>
         <oasis:entry colname="col8">no</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">no</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">no</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">yes</oasis:entry>
         <oasis:entry colname="col15">no</oasis:entry>
         <oasis:entry colname="col16">no</oasis:entry>
         <oasis:entry colname="col17">no</oasis:entry>
         <oasis:entry colname="col18">yes<inline-formula><mml:math id="M1538" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">g</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">no</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Irrigation</oasis:entry>
         <oasis:entry colname="col2">yes (z)</oasis:entry>
         <oasis:entry colname="col3">yes (z)</oasis:entry>
         <oasis:entry colname="col4">yes<inline-formula><mml:math id="M1539" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">no</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">yes</oasis:entry>
         <oasis:entry colname="col8">yes</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">yes</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">no</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">yes</oasis:entry>
         <oasis:entry colname="col15">no</oasis:entry>
         <oasis:entry colname="col16">no</oasis:entry>
         <oasis:entry colname="col17">no</oasis:entry>
         <oasis:entry colname="col18">no</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">no</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Wetland drainage</oasis:entry>
         <oasis:entry colname="col2">yes (z)</oasis:entry>
         <oasis:entry colname="col3">yes (z)</oasis:entry>
         <oasis:entry colname="col4">yes<inline-formula><mml:math id="M1540" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">no</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">no</oasis:entry>
         <oasis:entry colname="col8">no</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">yes</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">no</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">no</oasis:entry>
         <oasis:entry colname="col15">no</oasis:entry>
         <oasis:entry colname="col16">no</oasis:entry>
         <oasis:entry colname="col17">no</oasis:entry>
         <oasis:entry colname="col18">no</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">no</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Erosion</oasis:entry>
         <oasis:entry colname="col2">yes (z)</oasis:entry>
         <oasis:entry colname="col3">yes (z)</oasis:entry>
         <oasis:entry colname="col4">yes<inline-formula><mml:math id="M1541" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">no</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">no</oasis:entry>
         <oasis:entry colname="col8">yes</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">no</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">no</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">no</oasis:entry>
         <oasis:entry colname="col15">no</oasis:entry>
         <oasis:entry colname="col16">no</oasis:entry>
         <oasis:entry colname="col17">no</oasis:entry>
         <oasis:entry colname="col18">no</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">yes</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Peat drainage</oasis:entry>
         <oasis:entry colname="col2">yes</oasis:entry>
         <oasis:entry colname="col3">yes</oasis:entry>
         <oasis:entry colname="col4">yes</oasis:entry>
         <oasis:entry colname="col5">no</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">no</oasis:entry>
         <oasis:entry colname="col8">no</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">no</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">no</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">no</oasis:entry>
         <oasis:entry colname="col15">no</oasis:entry>
         <oasis:entry colname="col16">no</oasis:entry>
         <oasis:entry colname="col17">no</oasis:entry>
         <oasis:entry colname="col18">no</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">no</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Grazing and mowing harvest (removed, r, or added to litter, l)</oasis:entry>
         <oasis:entry colname="col2">yes (r) (z)</oasis:entry>
         <oasis:entry colname="col3">yes (r) (z)</oasis:entry>
         <oasis:entry colname="col4">yes (r)</oasis:entry>
         <oasis:entry colname="col5">yes (r)</oasis:entry>
         <oasis:entry colname="col6">no</oasis:entry>
         <oasis:entry colname="col7">no</oasis:entry>
         <oasis:entry colname="col8">no</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">yes (l)</oasis:entry>
         <oasis:entry colname="col11">no</oasis:entry>
         <oasis:entry colname="col12">yes (l)</oasis:entry>
         <oasis:entry colname="col13">no</oasis:entry>
         <oasis:entry colname="col14">yes (r)</oasis:entry>
         <oasis:entry colname="col15">yes (l)</oasis:entry>
         <oasis:entry colname="col16">no</oasis:entry>
         <oasis:entry colname="col17">yes (r<inline-formula><mml:math id="M1542" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>l)</oasis:entry>
         <oasis:entry colname="col18">no</oasis:entry>
         <oasis:entry colname="col19">no</oasis:entry>
         <oasis:entry colname="col20">no</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col21" align="left">Processes also relevant for <inline-formula><mml:math id="M1543" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (in addition to CO<inline-formula><mml:math id="M1544" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fertilization and climate) </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Fire simulation <?xmltex \hack{\hfill\break}?>and/or suppression</oasis:entry>
         <oasis:entry colname="col2">n/a</oasis:entry>
         <oasis:entry colname="col3">n/a</oasis:entry>
         <oasis:entry colname="col4">n/a</oasis:entry>
         <oasis:entry colname="col5">no</oasis:entry>
         <oasis:entry colname="col6">yes</oasis:entry>
         <oasis:entry colname="col7">yes</oasis:entry>
         <oasis:entry colname="col8">no</oasis:entry>
         <oasis:entry colname="col9">yes</oasis:entry>
         <oasis:entry colname="col10">no</oasis:entry>
         <oasis:entry colname="col11">yes</oasis:entry>
         <oasis:entry colname="col12">yes</oasis:entry>
         <oasis:entry colname="col13">yes</oasis:entry>
         <oasis:entry colname="col14">yes</oasis:entry>
         <oasis:entry colname="col15">yes</oasis:entry>
         <oasis:entry colname="col16">yes</oasis:entry>
         <oasis:entry colname="col17">no</oasis:entry>
         <oasis:entry colname="col18">no</oasis:entry>
         <oasis:entry colname="col19">yes</oasis:entry>
         <oasis:entry colname="col20">yes</oasis:entry>
         <oasis:entry colname="col21">no</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Carbon-nitrogen<?xmltex \hack{\hfill\break}?>interactions, <?xmltex \hack{\hfill\break}?>including N<?xmltex \hack{\hfill\break}?>deposition</oasis:entry>
         <oasis:entry colname="col2">n/a</oasis:entry>
         <oasis:entry colname="col3">n/a</oasis:entry>
         <oasis:entry colname="col4">n/a</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
         <oasis:entry colname="col6">no<inline-formula><mml:math id="M1545" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">f</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">yes</oasis:entry>
         <oasis:entry colname="col8">yes</oasis:entry>
         <oasis:entry colname="col9">no</oasis:entry>
         <oasis:entry colname="col10">yes</oasis:entry>
         <oasis:entry colname="col11">no<inline-formula><mml:math id="M1546" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">e</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col12">yes</oasis:entry>
         <oasis:entry colname="col13">yes</oasis:entry>
         <oasis:entry colname="col14">yes</oasis:entry>
         <oasis:entry colname="col15">no</oasis:entry>
         <oasis:entry colname="col16">yes</oasis:entry>
         <oasis:entry colname="col17">yes</oasis:entry>
         <oasis:entry colname="col18">yes</oasis:entry>
         <oasis:entry colname="col19">yes<inline-formula><mml:math id="M1547" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col20">no</oasis:entry>
         <oasis:entry colname="col21">no<inline-formula><mml:math id="M1548" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">f</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\end{minipage}\end{turn}}?><?xmltex \hack{\clearpage}?><?xmltex \floatpos{p}?><table-wrap id="App1.Ch1.S1.T12" specific-use="star" orientation="landscape"><?xmltex \currentcnt{A2}?><label>Table A2</label><caption><p id="d1e21806">Comparison of the processes and model set-up for the global ocean biogeochemistry models for their estimates of <inline-formula><mml:math id="M1549" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. See Table 4 for model references. NA – not available</p></caption><oasis:table frame="top"><?xmltex \begin{scaleboxenv}{.78}[.78]?><oasis:tgroup cols="9">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="5" colname="col5" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="6" colname="col6" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="7" colname="col7" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="8" colname="col8" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="9" colname="col9" align="justify" colwidth="2.8cm"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">NEMO-PlankTOM12</oasis:entry>
         <oasis:entry colname="col3">NEMO-PISCES (IPSL)</oasis:entry>
         <oasis:entry colname="col4">MICOM-HAMOCC (NorESM1-OCv1.2)</oasis:entry>
         <oasis:entry colname="col5">MPIOM-HAMOCC6</oasis:entry>
         <oasis:entry colname="col6">FESOM-2.1-REcoM2</oasis:entry>
         <oasis:entry colname="col7">NEMO3.6-PISCESv2-gas (CNRM)</oasis:entry>
         <oasis:entry colname="col8">MOM6-COBALT (Princeton)</oasis:entry>
         <oasis:entry colname="col9">CESM-ETHZ</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col9" align="left">Spin-up procedure </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Initialization of<?xmltex \hack{\hfill\break}?>carbon chemistry</oasis:entry>
         <oasis:entry colname="col2">GLODAPv1 <?xmltex \hack{\hfill\break}?>corrected for anthropogenic carbon from Sabine et al. (2004)</oasis:entry>
         <oasis:entry colname="col3">GLODAPv2</oasis:entry>
         <oasis:entry colname="col4">GLODAP v1 (pre-industrial DIC)</oasis:entry>
         <oasis:entry colname="col5">initialization from<?xmltex \hack{\hfill\break}?>previous model<?xmltex \hack{\hfill\break}?>simulations</oasis:entry>
         <oasis:entry colname="col6">GLODAPv2 alkalinity and pre-industrial DIC</oasis:entry>
         <oasis:entry colname="col7">GLODAPv2</oasis:entry>
         <oasis:entry colname="col8">GLODAPv2 for Alkalinity and DIC. DIC is corrected to 1959 level for simulation A and C and corrected to pre-industrial level for simulation B using Khatiwala et al. (2009, 2013)</oasis:entry>
         <oasis:entry colname="col9">GLODAPv2<?xmltex \hack{\hfill\break}?>pre-industrial</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Pre-industrial spin-up<?xmltex \hack{\hfill\break}?>prior to 1850? If yes, how long?</oasis:entry>
         <oasis:entry colname="col2">spin-up 1750–1947</oasis:entry>
         <oasis:entry colname="col3">spin-up starting in 1836 with 3 loops of JRA55</oasis:entry>
         <oasis:entry colname="col4">1000 year spin-up</oasis:entry>
         <oasis:entry colname="col5">yes, <inline-formula><mml:math id="M1550" display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 2000 years</oasis:entry>
         <oasis:entry colname="col6">50 years</oasis:entry>
         <oasis:entry colname="col7">long spin-up <?xmltex \hack{\hfill\break}?>(<inline-formula><mml:math id="M1551" display="inline"><mml:mo lspace="0mm">&gt;</mml:mo></mml:math></inline-formula> 1000 years)</oasis:entry>
         <oasis:entry colname="col8">Other biogeochemical tracers are initialized from a GFDL-<?xmltex \hack{\hfill\break}?>ESM2M spin-up <?xmltex \hack{\hfill\break}?>(<inline-formula><mml:math id="M1552" display="inline"><mml:mo lspace="0mm">&gt;</mml:mo></mml:math></inline-formula> 1000 years)</oasis:entry>
         <oasis:entry colname="col9">spin-up 1655–1849</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric forcing<?xmltex \hack{\hfill\break}?>for pre-industrial<?xmltex \hack{\hfill\break}?>spin-up</oasis:entry>
         <oasis:entry colname="col2">looping NCEP year 1990</oasis:entry>
         <oasis:entry colname="col3">JRA55</oasis:entry>
         <oasis:entry colname="col4">CORE-I (normal<?xmltex \hack{\hfill\break}?>year) forcing</oasis:entry>
         <oasis:entry colname="col5">spin-up with omip <?xmltex \hack{\hfill\break}?>climatology to reach steady state with the rivers</oasis:entry>
         <oasis:entry colname="col6">JRA55-do v.1.5.0 <?xmltex \hack{\hfill\break}?>repeated year 1961</oasis:entry>
         <oasis:entry colname="col7">JRA55-do</oasis:entry>
         <oasis:entry colname="col8">GFDL-ESM2M internal forcing</oasis:entry>
         <oasis:entry colname="col9">COREv2 forcing until 1835, three cycles of conditions from <?xmltex \hack{\hfill\break}?>1949–2009 from <?xmltex \hack{\hfill\break}?>1835–1850: JRA <?xmltex \hack{\hfill\break}?>forcing</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric forcing <?xmltex \hack{\hfill\break}?>for historical spin-up 1850–1958 for simulation A</oasis:entry>
         <oasis:entry colname="col2">1750–1947: looping NCEP year 1990; 1948–2020: NCEP</oasis:entry>
         <oasis:entry colname="col3">1836–1958: looping full JRA55 reanalysis</oasis:entry>
         <oasis:entry colname="col4">CORE-I (normal-year) forcing; from 1948 onwards NCEP-R1 with CORE-II corrections</oasis:entry>
         <oasis:entry colname="col5">NCEP 6-hourly cyclic forcing (10 years starting from 1948) with CO<inline-formula><mml:math id="M1553" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> at 278 ppm and rivers</oasis:entry>
         <oasis:entry colname="col6">JRA55-do-v1.5.0 repeated year 1961</oasis:entry>
         <oasis:entry colname="col7">JRA55-do<?xmltex \hack{\hfill\break}?>cycling year 1958</oasis:entry>
         <oasis:entry colname="col8">JRA55-do-v1.5 repeat year 1959 (71 years)</oasis:entry>
         <oasis:entry colname="col9">JRA55 version 1.3, repeat cycle between 1958–2018.</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric CO<inline-formula><mml:math id="M1554" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula><?xmltex \hack{\hfill\break}?>for historical spin-up 1850–1958 for<?xmltex \hack{\hfill\break}?>simulation A</oasis:entry>
         <oasis:entry colname="col2">provided by the GCP; converted to <inline-formula><mml:math id="M1555" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1556" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> temperature formulation (Sarmiento et al., 1992), monthly resolution</oasis:entry>
         <oasis:entry colname="col3">xCO<inline-formula><mml:math id="M1557" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB, global mean, annual resolution, converted to <inline-formula><mml:math id="M1558" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1559" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with sea-level pressure and water vapour pressure</oasis:entry>
         <oasis:entry colname="col4">xCO<inline-formula><mml:math id="M1560" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB, converted to <inline-formula><mml:math id="M1561" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1562" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with sea level pressure and water vapour correction</oasis:entry>
         <oasis:entry colname="col5">provided by the GCB</oasis:entry>
         <oasis:entry colname="col6">xCO<inline-formula><mml:math id="M1563" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB, converted to <inline-formula><mml:math id="M1564" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1565" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with sea-level pressure and water vapour pressure, global mean, monthly resolution</oasis:entry>
         <oasis:entry colname="col7">xCO<inline-formula><mml:math id="M1566" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB, converted to <inline-formula><mml:math id="M1567" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1568" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with constant sea-level pressure and water vapour pressure, global mean, yearly resolution</oasis:entry>
         <oasis:entry colname="col8">xCO<inline-formula><mml:math id="M1569" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> at year 1959 level (315 ppm), converted to <inline-formula><mml:math id="M1570" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1571" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with sea-level pressure and water vapour pressure, global mean, yearly resolution</oasis:entry>
         <oasis:entry colname="col9">xCO<inline-formula><mml:math id="M1572" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB (new version 2021), converted to <inline-formula><mml:math id="M1573" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1574" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with atmospheric pressure, and locally determined water vapour pressure from SST and SSS (100 % saturation)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric forcing<?xmltex \hack{\hfill\break}?>for control spin-up 1850–1958 for<?xmltex \hack{\hfill\break}?>simulation B</oasis:entry>
         <oasis:entry colname="col2">1750–2020: looping<?xmltex \hack{\hfill\break}?>NCEP 1990</oasis:entry>
         <oasis:entry colname="col3">1836–1958: looping <?xmltex \hack{\hfill\break}?>full JRA55 reanalysis</oasis:entry>
         <oasis:entry colname="col4">CORE-I (normal<?xmltex \hack{\hfill\break}?>year) forcing</oasis:entry>
         <oasis:entry colname="col5">NCEP 1957 <?xmltex \hack{\hfill\break}?>fixed forcing,<?xmltex \hack{\hfill\break}?>CO<inline-formula><mml:math id="M1575" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> <inline-formula><mml:math id="M1576" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 278 ppm <?xmltex \hack{\hfill\break}?>and rivers</oasis:entry>
         <oasis:entry colname="col6">JRA55-do-v1.5.0 <?xmltex \hack{\hfill\break}?>repeat year 1961</oasis:entry>
         <oasis:entry colname="col7">JRA55-do <?xmltex \hack{\hfill\break}?>cycling  year 1958</oasis:entry>
         <oasis:entry colname="col8">JRA55-do-v1.5 repeat year 1959 (71 years)</oasis:entry>
         <oasis:entry colname="col9">normal-year forcing created from JRA-55 version 1.3, NYF <inline-formula><mml:math id="M1577" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> climatology with anomalies from the year 2001</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric CO<inline-formula><mml:math id="M1578" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> for control spin-up 1850–1958 for simulation B</oasis:entry>
         <oasis:entry colname="col2">constant 278 ppm;<?xmltex \hack{\hfill\break}?>converted to <inline-formula><mml:math id="M1579" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1580" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> temperature formulation (Sarmiento et al., 1992), monthly resolution</oasis:entry>
         <oasis:entry colname="col3">xCO<inline-formula><mml:math id="M1581" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> of 286.46 ppm, converted to <inline-formula><mml:math id="M1582" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1583" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with constant sea-level pressure and water vapour pressure</oasis:entry>
         <oasis:entry colname="col4">xCO<inline-formula><mml:math id="M1584" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> of 278 ppm, <?xmltex \hack{\hfill\break}?>converted to <inline-formula><mml:math id="M1585" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1586" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with seal level pressure and water vapour correction</oasis:entry>
         <oasis:entry colname="col5">278, no conversion,<?xmltex \hack{\hfill\break}?>assuming constant<?xmltex \hack{\hfill\break}?>standard sea level <?xmltex \hack{\hfill\break}?>pressure</oasis:entry>
         <oasis:entry colname="col6">xCO<inline-formula><mml:math id="M1587" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> of 278 ppm,<?xmltex \hack{\hfill\break}?>converted to <inline-formula><mml:math id="M1588" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1589" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with sea-level pressure and water vapour pressure</oasis:entry>
         <oasis:entry colname="col7">xCO<inline-formula><mml:math id="M1590" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> of 286.46 ppm, converted to <inline-formula><mml:math id="M1591" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1592" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with constant sea-level pressure and water vapour pressure</oasis:entry>
         <oasis:entry colname="col8">xCO<inline-formula><mml:math id="M1593" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> of 278 ppm,<?xmltex \hack{\hfill\break}?>converted to <inline-formula><mml:math id="M1594" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1595" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with sea-level pressure and water vapour pressure</oasis:entry>
         <oasis:entry colname="col9">xCO<inline-formula><mml:math id="M1596" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB for 1850, converted to <inline-formula><mml:math id="M1597" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1598" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with atmospheric pressure, and locally determined water vapour pressure from SST and SSS (100 % saturation)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{p}?><table-wrap id="App1.Ch1.S1.T13" specific-use="star" orientation="landscape"><?xmltex \currentcnt{A2}?><label>Table A2</label><caption><p id="d1e22610">Continued.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.78}[.78]?><oasis:tgroup cols="9">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="2.5cm"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="2.5cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="2.5cm"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="2.5cm"/>
     <oasis:colspec colnum="5" colname="col5" align="justify" colwidth="2.5cm"/>
     <oasis:colspec colnum="6" colname="col6" align="justify" colwidth="2.5cm"/>
     <oasis:colspec colnum="7" colname="col7" align="justify" colwidth="2.5cm"/>
     <oasis:colspec colnum="8" colname="col8" align="justify" colwidth="2.5cm"/>
     <oasis:colspec colnum="9" colname="col9" align="justify" colwidth="2.5cm"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">NEMO-PlankTOM12</oasis:entry>
         <oasis:entry colname="col3">NEMO-PISCES (IPSL)</oasis:entry>
         <oasis:entry colname="col4">MICOM-HAMOCC (NorESM1-OCv1.2)</oasis:entry>
         <oasis:entry colname="col5">MPIOM-HAMOCC6</oasis:entry>
         <oasis:entry colname="col6">FESOM-2.1-REcoM2</oasis:entry>
         <oasis:entry colname="col7">NEMO3.6-PISCESv2-gas (CNRM)</oasis:entry>
         <oasis:entry colname="col8">MOM6-COBALT (Princeton)</oasis:entry>
         <oasis:entry colname="col9">CESM-ETHZ</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col9" align="left">Simulation A </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric<?xmltex \hack{\hfill\break}?>forcing for <?xmltex \hack{\hfill\break}?>simulation   A</oasis:entry>
         <oasis:entry colname="col2">NCEP</oasis:entry>
         <oasis:entry colname="col3">JRA55-v1.4 then <?xmltex \hack{\hfill\break}?>1.5 for 2020.</oasis:entry>
         <oasis:entry colname="col4">NCEP-R1 with <?xmltex \hack{\hfill\break}?>CORE-II<?xmltex \hack{\hfill\break}?>corrections</oasis:entry>
         <oasis:entry colname="col5">till1948: continue<?xmltex \hack{\hfill\break}?>from A_spinup with cyclic NCEP forcing (1948<inline-formula><mml:math id="M1599" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>10) and increasing CO<inline-formula><mml:math id="M1600" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> <inline-formula><mml:math id="M1601" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M1602" display="inline"><mml:mo>&gt;</mml:mo></mml:math></inline-formula> GCBA-1777-1948<?xmltex \hack{\hfill\break}?>-1948-2020: with<?xmltex \hack{\hfill\break}?>transient NCEP<?xmltex \hack{\hfill\break}?>forcing and <?xmltex \hack{\hfill\break}?>transient monthly<?xmltex \hack{\hfill\break}?>CO<inline-formula><mml:math id="M1603" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">JRA55-do-v1.5.0</oasis:entry>
         <oasis:entry colname="col7">JRA55-do</oasis:entry>
         <oasis:entry colname="col8">JRA55-do-v1.5.0 1959–2019 and<?xmltex \hack{\hfill\break}?>JRA55-do-v1.5.0.1b for<?xmltex \hack{\hfill\break}?>2020</oasis:entry>
         <oasis:entry colname="col9">JRA-55 version 1.3</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric CO<inline-formula><mml:math id="M1604" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> for simulation A</oasis:entry>
         <oasis:entry colname="col2">provided by the<?xmltex \hack{\hfill\break}?>GCP; converted<?xmltex \hack{\hfill\break}?>to <inline-formula><mml:math id="M1605" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1606" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> temperature formulation (Sarmiento et al., 1992), monthly<?xmltex \hack{\hfill\break}?>resolution</oasis:entry>
         <oasis:entry colname="col3">xCO<inline-formula><mml:math id="M1607" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided <?xmltex \hack{\hfill\break}?>by the GCB, global mean, annual resolution, converted to <inline-formula><mml:math id="M1608" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1609" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>  with<?xmltex \hack{\hfill\break}?>sea-level pressure and water vapour<?xmltex \hack{\hfill\break}?>pressure</oasis:entry>
         <oasis:entry colname="col4">xCO<inline-formula><mml:math id="M1610" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB, converted to <inline-formula><mml:math id="M1611" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1612" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula><?xmltex \hack{\hfill\break}?>with sea level <?xmltex \hack{\hfill\break}?>pressure and water vapour correction</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">xCO<inline-formula><mml:math id="M1613" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB, converted to <inline-formula><mml:math id="M1614" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1615" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with sea-level <?xmltex \hack{\hfill\break}?>pressure and water vapour pressure, <?xmltex \hack{\hfill\break}?>global mean,<?xmltex \hack{\hfill\break}?>monthly resolution</oasis:entry>
         <oasis:entry colname="col7">xCO<inline-formula><mml:math id="M1616" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB, converted to <inline-formula><mml:math id="M1617" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1618" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula><?xmltex \hack{\hfill\break}?>with constant sea-level pressure and water vapour pressure, global mean, yearly resolution</oasis:entry>
         <oasis:entry colname="col8">xCO<inline-formula><mml:math id="M1619" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB, converted to <inline-formula><mml:math id="M1620" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1621" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula><?xmltex \hack{\hfill\break}?>with sea-level <?xmltex \hack{\hfill\break}?>pressure and water vapour pressure, <?xmltex \hack{\hfill\break}?>global mean, yearly resolution</oasis:entry>
         <oasis:entry colname="col9">xCO<inline-formula><mml:math id="M1622" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB (new version 2021),<?xmltex \hack{\hfill\break}?>converted to <inline-formula><mml:math id="M1623" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1624" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with atmospheric pressure, and locally determined water vapour pressure from SST and SSS (100 % saturation)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col9" align="left">Simulation B </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric<?xmltex \hack{\hfill\break}?>forcing for<?xmltex \hack{\hfill\break}?>simulation B</oasis:entry>
         <oasis:entry colname="col2">NCEP 1990</oasis:entry>
         <oasis:entry colname="col3">NA</oasis:entry>
         <oasis:entry colname="col4">CORE-I (normal <?xmltex \hack{\hfill\break}?>year) forcing</oasis:entry>
         <oasis:entry colname="col5">1948–2020: <?xmltex \hack{\hfill\break}?>continue with<?xmltex \hack{\hfill\break}?>B_spinup with<?xmltex \hack{\hfill\break}?>fixed NCEP<?xmltex \hack{\hfill\break}?>forcing 1957,<?xmltex \hack{\hfill\break}?>CO<inline-formula><mml:math id="M1625" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> <inline-formula><mml:math id="M1626" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 278 ppm and rivers</oasis:entry>
         <oasis:entry colname="col6">JRA55-do-v1.5.0 repeat year 1961</oasis:entry>
         <oasis:entry colname="col7">JRA55-do cycling <?xmltex \hack{\hfill\break}?>year 1958</oasis:entry>
         <oasis:entry colname="col8">JRA55-do-v1.5.0 repeat year 1959</oasis:entry>
         <oasis:entry colname="col9">normal-year forcing created from JRA-55 version 1.3, NYF <inline-formula><mml:math id="M1627" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> climatology with anomalies from the year 2001</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric CO<inline-formula><mml:math id="M1628" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> <?xmltex \hack{\hfill\break}?>for simulation B</oasis:entry>
         <oasis:entry colname="col2">constant 278 ppm; converted to <inline-formula><mml:math id="M1629" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1630" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> temperature formulation (Sarmiento et al., 1992), monthly resolution</oasis:entry>
         <oasis:entry colname="col3">NA</oasis:entry>
         <oasis:entry colname="col4">xCO<inline-formula><mml:math id="M1631" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> of 278 ppm, converted to <inline-formula><mml:math id="M1632" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1633" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with sea level pressure and water vapour correction</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">xCO<inline-formula><mml:math id="M1634" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> of 278 ppm, converted to<?xmltex \hack{\hfill\break}?> <inline-formula><mml:math id="M1635" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1636" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with <?xmltex \hack{\hfill\break}?>sea-level pressure <?xmltex \hack{\hfill\break}?>and water vapour<?xmltex \hack{\hfill\break}?>pressure</oasis:entry>
         <oasis:entry colname="col7">xCO<inline-formula><mml:math id="M1637" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> of<?xmltex \hack{\hfill\break}?>286.46 ppm, <?xmltex \hack{\hfill\break}?>converted to <inline-formula><mml:math id="M1638" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1639" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula><?xmltex \hack{\hfill\break}?>with constant <?xmltex \hack{\hfill\break}?>sea-level pressure and water vapour <?xmltex \hack{\hfill\break}?>pressure</oasis:entry>
         <oasis:entry colname="col8">xCO<inline-formula><mml:math id="M1640" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> of 278 ppm, converted to <inline-formula><mml:math id="M1641" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1642" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with sea-level<?xmltex \hack{\hfill\break}?>pressure and water vapour pressure</oasis:entry>
         <oasis:entry colname="col9">xCO<inline-formula><mml:math id="M1643" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> as provided by the GCB for 1850, converted to <inline-formula><mml:math id="M1644" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1645" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> with atmospheric pressure, and locally determined water vapour pressure from SST and SSS (100 % saturation)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col9" align="left">Model specifics </oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Physical ocean <?xmltex \hack{\hfill\break}?>model</oasis:entry>
         <oasis:entry colname="col2">NEMOv3.6-ORCA2</oasis:entry>
         <oasis:entry colname="col3">NEMOv3.6-eORCA1L75</oasis:entry>
         <oasis:entry colname="col4">MICOM (NorESM1-OCv1.2)</oasis:entry>
         <oasis:entry colname="col5">MPIOM</oasis:entry>
         <oasis:entry colname="col6">FESOM-2.1</oasis:entry>
         <oasis:entry colname="col7">NEMOv3.6-GELATOv6-eORCA1L75</oasis:entry>
         <oasis:entry colname="col8">MOM6-SIS2</oasis:entry>
         <oasis:entry colname="col9">CESMv1.3 (ocean model based on<?xmltex \hack{\hfill\break}?>POP2)</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Biogeochemistry model</oasis:entry>
         <oasis:entry colname="col2">PlankTOM12</oasis:entry>
         <oasis:entry colname="col3">PISCESv2</oasis:entry>
         <oasis:entry colname="col4">HAMOCC (NorESM1-OCv1.2)</oasis:entry>
         <oasis:entry colname="col5">HAMOCC6</oasis:entry>
         <oasis:entry colname="col6">REcoM-2-M</oasis:entry>
         <oasis:entry colname="col7">PISCESv2-gas</oasis:entry>
         <oasis:entry colname="col8">COBALTv2</oasis:entry>
         <oasis:entry colname="col9">BEC (modified and extended)</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{p}?><table-wrap id="App1.Ch1.S1.T14" specific-use="star" orientation="landscape"><?xmltex \currentcnt{A2}?><label>Table A2</label><caption><p id="d1e23367">Continued.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.78}[.78]?><oasis:tgroup cols="9">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="5" colname="col5" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="6" colname="col6" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="7" colname="col7" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="8" colname="col8" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="9" colname="col9" align="justify" colwidth="2.8cm"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">NEMO-PlankTOM12</oasis:entry>
         <oasis:entry colname="col3">NEMO-PISCES (IPSL)</oasis:entry>
         <oasis:entry colname="col4">MICOM-HAMOCC (NorESM1-OCv1.2)</oasis:entry>
         <oasis:entry colname="col5">MPIOM-HAMOCC6</oasis:entry>
         <oasis:entry colname="col6">FESOM-2.1-REcoM2</oasis:entry>
         <oasis:entry colname="col7">NEMO3.6-PISCESv2-gas (CNRM)</oasis:entry>
         <oasis:entry colname="col8">MOM6-COBALT (Princeton)</oasis:entry>
         <oasis:entry colname="col9">CESM-ETHZ</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Horizontal resolution</oasis:entry>
         <oasis:entry colname="col2">2<inline-formula><mml:math id="M1646" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> longitude, 0.3 to 1.5<inline-formula><mml:math id="M1647" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> latitude</oasis:entry>
         <oasis:entry colname="col3">1<inline-formula><mml:math id="M1648" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> longitude, 0.3 to<?xmltex \hack{\hfill\break}?>1<inline-formula><mml:math id="M1649" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> latitude</oasis:entry>
         <oasis:entry colname="col4">1<inline-formula><mml:math id="M1650" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> longitude, 0.17 to 0.25 latitude (nominally 1<inline-formula><mml:math id="M1651" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col5">1.5<inline-formula><mml:math id="M1652" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">unstructured multi-<?xmltex \hack{\hfill\break}?>resolution mesh. <?xmltex \hack{\hfill\break}?>CORE-mesh, with 20–120 km resolution. Highest resolution north of 50<inline-formula><mml:math id="M1653" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N, intermediate in the equatorial belt and Southern Ocean, lowest in the subtropical gyres</oasis:entry>
         <oasis:entry colname="col7">1<inline-formula><mml:math id="M1654" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> longitude, 0.3 to 1<inline-formula><mml:math id="M1655" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> latitude</oasis:entry>
         <oasis:entry colname="col8">0.5<inline-formula><mml:math id="M1656" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> longitude, 0.25 to 0.5<inline-formula><mml:math id="M1657" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> latitude</oasis:entry>
         <oasis:entry colname="col9">1.125<inline-formula><mml:math id="M1658" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> longitude, <?xmltex \hack{\hfill\break}?>latitude  varying from<?xmltex \hack{\hfill\break}?>0.53<inline-formula><mml:math id="M1659" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> in the extra-<?xmltex \hack{\hfill\break}?>tropics to 0.27<inline-formula><mml:math id="M1660" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> near <?xmltex \hack{\hfill\break}?>the Equator</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Vertical resolution</oasis:entry>
         <oasis:entry colname="col2">31 levels</oasis:entry>
         <oasis:entry colname="col3">75 levels, 1 m at the<?xmltex \hack{\hfill\break}?>surface</oasis:entry>
         <oasis:entry colname="col4">51 isopycnic layers <inline-formula><mml:math id="M1661" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> 2 layers representing a bulk mixed layer</oasis:entry>
         <oasis:entry colname="col5">40 levels, layer thickness increase with <?xmltex \hack{\hfill\break}?>depth</oasis:entry>
         <oasis:entry colname="col6">46 levels, 10 m spacing in the top 100 m</oasis:entry>
         <oasis:entry colname="col7">75 levels, 1 m at <?xmltex \hack{\hfill\break}?>surface</oasis:entry>
         <oasis:entry colname="col8">75 levels hybrid coordinates, 2 m at surface</oasis:entry>
         <oasis:entry colname="col9">60 levels <?xmltex \hack{\hfill\break}?>(<inline-formula><mml:math id="M1662" display="inline"><mml:mi>z</mml:mi></mml:math></inline-formula> coordinates)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Total ocean area on <?xmltex \hack{\hfill\break}?>native grid (km<inline-formula><mml:math id="M1663" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">3.6080E<inline-formula><mml:math id="M1664" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col3">3.6270E<inline-formula><mml:math id="M1665" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col4">3.6006E<inline-formula><mml:math id="M1666" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col5">3.6598E<inline-formula><mml:math id="M1667" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col6">3.6475E<inline-formula><mml:math id="M1668" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col7">3.6270E<inline-formula><mml:math id="M1669" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>14</oasis:entry>
         <oasis:entry colname="col8">3.6110E<inline-formula><mml:math id="M1670" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col9">3.5926E<inline-formula><mml:math id="M1671" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Ocean area on native grid (km<inline-formula><mml:math id="M1672" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>) – north</oasis:entry>
         <oasis:entry colname="col2">6.2646E<inline-formula><mml:math id="M1673" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">6.2049E<inline-formula><mml:math id="M1674" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07</oasis:entry>
         <oasis:entry colname="col5">6.4440E<inline-formula><mml:math id="M1675" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">6.3971E<inline-formula><mml:math id="M1676" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>13</oasis:entry>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Ocean area on native grid (km<inline-formula><mml:math id="M1677" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>) – tropics</oasis:entry>
         <oasis:entry colname="col2">1.1051E<inline-formula><mml:math id="M1678" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">1.9037E<inline-formula><mml:math id="M1679" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col5">1.9248E<inline-formula><mml:math id="M1680" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">1.9025E<inline-formula><mml:math id="M1681" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>14</oasis:entry>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Ocean area on native grid (km<inline-formula><mml:math id="M1682" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>) – south</oasis:entry>
         <oasis:entry colname="col2">1.8766E<inline-formula><mml:math id="M1683" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">1.0765E<inline-formula><mml:math id="M1684" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col5">1.0986E<inline-formula><mml:math id="M1685" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">1.0848E<inline-formula><mml:math id="M1686" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>14</oasis:entry>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Gas-exchange parameterization</oasis:entry>
         <oasis:entry colname="col2">Quadratic exchange formulation (function of <inline-formula><mml:math id="M1687" display="inline"><mml:mrow><mml:mi>T</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">0.3</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mi>U</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>)</mml:mo><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>; Wanninkhof (1992, Eq. 8); Sweeney et al. (2007)</oasis:entry>
         <oasis:entry colname="col3">see Orr et al. (2017): <inline-formula><mml:math id="M1688" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> parameterized from Wanninkhof (1992), with <inline-formula><mml:math id="M1689" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi>a</mml:mi><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo><mml:mo>×</mml:mo><mml:msup><mml:mi>u</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mi mathvariant="italic">_</mml:mi><mml:mtext>ice</mml:mtext><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> with <inline-formula><mml:math id="M1690" display="inline"><mml:mi>a</mml:mi></mml:math></inline-formula> from Wanninkhof (2014)</oasis:entry>
         <oasis:entry colname="col4">see Orr et al. (2017): <inline-formula><mml:math id="M1691" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> parameterized from Wanninkhof (1992), with <inline-formula><mml:math id="M1692" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi>a</mml:mi><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo><mml:mo>×</mml:mo><mml:msup><mml:mi>u</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mi mathvariant="italic">_</mml:mi><mml:mtext>ice</mml:mtext><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> with <inline-formula><mml:math id="M1693" display="inline"><mml:mrow><mml:mi>a</mml:mi><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0</mml:mn></mml:mrow></mml:math></inline-formula>.337 following the OCMIP2 protocols</oasis:entry>
         <oasis:entry colname="col5">Gas transfer velocity formulation and parameter set-up of Wanninkhof (2014), including updated Schmidt number parameterizations for CO<inline-formula><mml:math id="M1694" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> to comply with OMIP protocol (Orr et al., 2017)</oasis:entry>
         <oasis:entry colname="col6">see Orr et al. (2017): <inline-formula><mml:math id="M1695" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> parameterized from Wanninkhof (1992), with <inline-formula><mml:math id="M1696" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi>a</mml:mi><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo><mml:mo>×</mml:mo><mml:msup><mml:mi>u</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mi mathvariant="italic">_</mml:mi><mml:mtext>ice</mml:mtext><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> with <inline-formula><mml:math id="M1697" display="inline"><mml:mi>a</mml:mi></mml:math></inline-formula> from Wanninkhof (2014)</oasis:entry>
         <oasis:entry colname="col7">see Orr et al. (2017): <inline-formula><mml:math id="M1698" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> parameterized from Wanninkhof (1992), with <inline-formula><mml:math id="M1699" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi>a</mml:mi><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo><mml:mo>×</mml:mo><mml:msup><mml:mi>u</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mi mathvariant="italic">_</mml:mi><mml:mtext>ice</mml:mtext><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> with <inline-formula><mml:math id="M1700" display="inline"><mml:mi>a</mml:mi></mml:math></inline-formula> from Wanninkhof (2014)</oasis:entry>
         <oasis:entry colname="col8">see Orr et al. (2017): <inline-formula><mml:math id="M1701" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> parameterized from Wanninkhof (1992), with <inline-formula><mml:math id="M1702" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi>a</mml:mi><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo><mml:mo>×</mml:mo><mml:msup><mml:mi>u</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mi mathvariant="italic">_</mml:mi><mml:mtext>ice</mml:mtext><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula> with <inline-formula><mml:math id="M1703" display="inline"><mml:mi>a</mml:mi></mml:math></inline-formula> from Wanninkhof (2014)</oasis:entry>
         <oasis:entry colname="col9">Gas exchange is parameterized using the Wanninkhof (1992) quadratic wind speed dependency formulation, but with the coefficient scaled down to reflect the recent <inline-formula><mml:math id="M1704" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">14</mml:mn></mml:msup></mml:math></inline-formula>C inventories. Concretely, we used a coefficient a of <inline-formula><mml:math id="M1705" display="inline"><mml:mn mathvariant="normal">0.31</mml:mn></mml:math></inline-formula> cm h<inline-formula><mml:math id="M1706" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> s<inline-formula><mml:math id="M1707" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula> m<inline-formula><mml:math id="M1708" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to read 0.31<inline-formula><mml:math id="M1709" display="inline"><mml:mrow><mml:msup><mml:mi>u</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>-</mml:mo><mml:mi>f</mml:mi><mml:mi mathvariant="italic">_</mml:mi><mml:mtext>ice</mml:mtext><mml:mo>)</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Time step</oasis:entry>
         <oasis:entry colname="col2">96 min</oasis:entry>
         <oasis:entry colname="col3">45 min</oasis:entry>
         <oasis:entry colname="col4">3200 s</oasis:entry>
         <oasis:entry colname="col5">60 min</oasis:entry>
         <oasis:entry colname="col6">45 min</oasis:entry>
         <oasis:entry colname="col7">15 min</oasis:entry>
         <oasis:entry colname="col8">30 min</oasis:entry>
         <oasis:entry colname="col9">3757 s</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Output frequency</oasis:entry>
         <oasis:entry colname="col2">monthly</oasis:entry>
         <oasis:entry colname="col3">monthly</oasis:entry>
         <oasis:entry colname="col4">monthly/daily</oasis:entry>
         <oasis:entry colname="col5">monthly</oasis:entry>
         <oasis:entry colname="col6">monthly</oasis:entry>
         <oasis:entry colname="col7">monthly</oasis:entry>
         <oasis:entry colname="col8">monthly</oasis:entry>
         <oasis:entry colname="col9">monthly</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">CO<inline-formula><mml:math id="M1710" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> chemistry<?xmltex \hack{\hfill\break}?>routines</oasis:entry>
         <oasis:entry colname="col2">following Broecker (1982)</oasis:entry>
         <oasis:entry colname="col3">mocsy</oasis:entry>
         <oasis:entry colname="col4">following Dickson et al. (2007)</oasis:entry>
         <oasis:entry colname="col5">as in Ilyina et <?xmltex \hack{\hfill\break}?>al. (2013) adapted to comply with OMIP<?xmltex \hack{\hfill\break}?>protocol (Orr et al.,<?xmltex \hack{\hfill\break}?>2017).</oasis:entry>
         <oasis:entry colname="col6">mocsy</oasis:entry>
         <oasis:entry colname="col7">mocsy</oasis:entry>
         <oasis:entry colname="col8">mocsy</oasis:entry>
         <oasis:entry colname="col9">OCMIP2 (Orr et al., 2017)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">River carbon input<?xmltex \hack{\hfill\break}?>(PgC yr<inline-formula><mml:math id="M1711" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">60.24 Tmol yr<inline-formula><mml:math id="M1712" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>; 0.723 PgC yr<inline-formula><mml:math id="M1713" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">0.61 PgC yr<inline-formula><mml:math id="M1714" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4">0</oasis:entry>
         <oasis:entry colname="col5">0.77 PgC yr<inline-formula><mml:math id="M1715" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">0</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M1716" display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 0.611 PgC yr<inline-formula><mml:math id="M1717" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M1718" display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 0.15 PgC yr<inline-formula><mml:math id="M1719" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9">0.33 PgC yr<inline-formula><mml:math id="M1720" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Burial/net flux<?xmltex \hack{\hfill\break}?>into the sediment<?xmltex \hack{\hfill\break}?>(PgC yr<inline-formula><mml:math id="M1721" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">0.723 PgC yr<inline-formula><mml:math id="M1722" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">0.59 GtC yr<inline-formula><mml:math id="M1723" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4">around 0.54</oasis:entry>
         <oasis:entry colname="col5">around 0.44 PgC yr<inline-formula><mml:math id="M1724" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">0</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M1725" display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 0.656 GtC yr<inline-formula><mml:math id="M1726" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M1727" display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 0.18 PgC yr<inline-formula><mml:math id="M1728" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9">0.21 PgC yr<inline-formula><mml:math id="M1729" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{p}?><table-wrap id="App1.Ch1.S1.T15" specific-use="star" orientation="landscape"><?xmltex \currentcnt{A3}?><label>Table A3</label><caption><p id="d1e24907">Description of ocean data products used for assessment of <inline-formula><mml:math id="M1730" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. See Table 4 for references.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.75}[.75]?><oasis:tgroup cols="9">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="2cm"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="5" colname="col5" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="6" colname="col6" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="7" colname="col7" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="8" colname="col8" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="9" colname="col9" align="justify" colwidth="3cm"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">Jena-MLS</oasis:entry>
         <oasis:entry colname="col3">MPI-SOMFFN</oasis:entry>
         <oasis:entry colname="col4">CMEMS-LSCE-FFNN</oasis:entry>
         <oasis:entry colname="col5">CSIR-ML6</oasis:entry>
         <oasis:entry colname="col6">Watson et al.</oasis:entry>
         <oasis:entry colname="col7">NIES-NN</oasis:entry>
         <oasis:entry colname="col8">JMA-MLR</oasis:entry>
         <oasis:entry colname="col9">OS-ETHZ-GRaCER</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Method</oasis:entry>
         <oasis:entry colname="col2">Spatio-temporal interpolation (update of Rödenbeck et al., 2013, version oc_v2021). Specifically, the sea-air CO<inline-formula><mml:math id="M1731" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes and the <inline-formula><mml:math id="M1732" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1733" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> field are numerically linked to each other and to the spatio-temporal field of ocean-internal carbon sources/sinks through process parameterizations, and the ocean-internal source/sink field is then fit to the SOCATv2021 <inline-formula><mml:math id="M1734" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1735" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data (Bakker et al., 2021). The fit includes a multi-linear regression against environmental drivers to bridge data gaps, and interannually explicit corrections to represent the data signals more completely.</oasis:entry>
         <oasis:entry colname="col3">2-step neural network method where in a first step the global ocean is clustered into 16 biogeochemical provinces (one stand-alone province for the Arctic Ocean – see Landschützer et al., 2020) using a self-organizing map (SOM). In a second step, the non-linear relationship between available <inline-formula><mml:math id="M1736" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1737" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements from the SOCAT database (Bakker et al., 2016) and environmental predictor data (SST, SSS, MLD, CHL <inline-formula><mml:math id="M1738" display="inline"><mml:mi>a</mml:mi></mml:math></inline-formula>, atmospheric CO<inline-formula><mml:math id="M1739" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> – see Landschützer et al., 2016) are established using a feed-forward neural network (FFN) for each province separately. The established relationship is then used to fill the existing data gaps (see Landschützer et al., 2013, 2016).</oasis:entry>
         <oasis:entry colname="col4">An ensemble of neural network models trained on 100 subsampled datasets from the Surface Ocean CO<inline-formula><mml:math id="M1740" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> Atlas v2021 (SOCATv2021, Bakker et al., 2021). Like the original data, subsamples are distributed after interpolation on <inline-formula><mml:math id="M1741" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula> grid cells along ship tracks. Sea surface salinity, temperature, sea surface height, mixed layer depth, atmospheric CO<inline-formula><mml:math id="M1742" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> mole fraction, chlorophyll <inline-formula><mml:math id="M1743" display="inline"><mml:mi>a</mml:mi></mml:math></inline-formula>, <inline-formula><mml:math id="M1744" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1745" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> climatology, latitude, and longitude are used as predictors. The models are used to reconstruct sea surface <inline-formula><mml:math id="M1746" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1747" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and convert to air–sea CO<inline-formula><mml:math id="M1748" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes (see the proposed ensemble-based approach and analysis in Chau et al., 2020, 2022).</oasis:entry>
         <oasis:entry colname="col5">An ensemble average of six machine learning estimates of surface ocean <inline-formula><mml:math id="M1749" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1750" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> using the approach described in Gregor et al. (2019) with the updated product using SOCAT v2021 (Bakker et al., 2016). All ensemble members use a cluster-regression approach. Two different cluster configurations are used: (1) based on <inline-formula><mml:math id="M1751" display="inline"><mml:mi>K</mml:mi></mml:math></inline-formula>-means clustering; (2) Fay and McKinley (2014)'s CO<inline-formula><mml:math id="M1752" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> biomes. Three regression algorithms are used: (1) gradient-boosted decision trees; (2) feed-forward neural network; (3) support vector regression. The product of the cluster configurations and the regression algorithms results in an ensemble with six members; hence the CSIR-ML6.</oasis:entry>
         <oasis:entry colname="col6">Derived from the SOCAT(v2021) <inline-formula><mml:math id="M1753" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1754" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> database, but corrected to the subskin temperature of the ocean as measured by satellite, using the methodology described by Goddijn-Murphy et al. (2015). A correction to the flux calculation is also applied for the cool and salty surface skin. In other respects the product uses interpolation of the data using the two-step neural network based on MPI-SOMFFN: in the first step the ocean is divided into a monthly climatology of 16 biogeochemical provinces using a SOM, In the second step a feed-forward neural network establishes non-linear relationships between <inline-formula><mml:math id="M1755" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1756" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and SST, SSS, mixed layer depth(MLD) and atmospheric xCO<inline-formula><mml:math id="M1757" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> in each of the 16 provinces. Further description in Watson et al. (2020).</oasis:entry>
         <oasis:entry colname="col7">A feed-forward neural network model was used to reconstruct monthly global surface ocean CO<inline-formula><mml:math id="M1758" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations <inline-formula><mml:math id="M1759" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1760" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> meshes and estimate air–sea CO<inline-formula><mml:math id="M1761" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes. The target variable is the per cruise weighted <inline-formula><mml:math id="M1762" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1763" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> mean of SOCAT 2021. Feature variables include sea surface temperature (SST), salinity, chlorophyll <inline-formula><mml:math id="M1764" display="inline"><mml:mi>a</mml:mi></mml:math></inline-formula>, mixed layer depth, and the monthly anomaly of SST. See Zeng et al. (2014).</oasis:entry>
         <oasis:entry colname="col8">Fields of total alkalinity (TA) were estimated by using a multiple linear regressions (MLR) method based on GLODAPv2.2021 and satellite observation data. <?xmltex \hack{\hfill\break}?>TA <inline-formula><mml:math id="M1765" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M1766" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>(SSDH, SSS). <?xmltex \hack{\hfill\break}?>SOCATv2021 <inline-formula><mml:math id="M1767" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1768" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data were converted to total dissolved inorganic carbon (DIC) concentrations in combination with the TA, and then fields of DIC were estimated by using a MLR method based on the DIC and satellite observation data. <?xmltex \hack{\hfill\break}?>DIC <inline-formula><mml:math id="M1769" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M1770" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>(SSDH, SST, SSS, log(Chl), log(MLD), time).</oasis:entry>
         <oasis:entry colname="col9">OceanSODA-ETHZ's Geospatial Random Cluster Ensemble Regression is a two-step cluster-regression approach, where multiple clustering instances with slight variations are run to create an ensemble of estimates (n_membersd <inline-formula><mml:math id="M1771" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 16). We use <inline-formula><mml:math id="M1772" display="inline"><mml:mi>K</mml:mi></mml:math></inline-formula>-means clustering (n_clusters <inline-formula><mml:math id="M1773" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 21) for the clustering step and a combination of gradient-boosted trees (n_members <inline-formula><mml:math id="M1774" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 8) and Feed-forward neural networks (n_members <inline-formula><mml:math id="M1775" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula> 8) to estimate SOCAT v2021 <inline-formula><mml:math id="M1776" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1777" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>. Clustering is performed on the following variables: SOCOM_ <inline-formula><mml:math id="M1778" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1779" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>_climatology, SST_clim, MLD_clim, CHL_clim. Regression is performed on the following variables: xCO<inline-formula><mml:math id="M1780" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>atm, SST, SST_anomaly, SSS, CHL, MLD, u10_wind, v10_wind, sea-ice changes, SSH (note that the latter two variables are an update from Gregor and Gruber, 2021).</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Gas-exchange parameterization</oasis:entry>
         <oasis:entry colname="col2">Quadratic exchange <?xmltex \hack{\hfill\break}?>formulation (<inline-formula><mml:math id="M1781" display="inline"><mml:mrow><mml:mi>k</mml:mi><mml:mo>×</mml:mo><mml:msup><mml:mi>U</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>) (Wanninkhof, 1992) with the transfer coefficient <inline-formula><mml:math id="M1782" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula> scaled to match a global mean transfer rate of 16.5 cm h<inline-formula><mml:math id="M1783" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> by Naegler (2009).</oasis:entry>
         <oasis:entry colname="col3">Quadratic exchange<?xmltex \hack{\hfill\break}?>formulation (<inline-formula><mml:math id="M1784" display="inline"><mml:mrow><mml:mi>k</mml:mi><mml:mo>×</mml:mo><mml:msup><mml:mi>U</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>) (Wanninkhof, 1992) with the transfer coefficient <inline-formula><mml:math id="M1785" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula> scaled to match a global mean transfer rate of 16.5 cm h<inline-formula><mml:math id="M1786" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (calculated over the full period 1982–2020).</oasis:entry>
         <oasis:entry colname="col4">Quadratic exchange<?xmltex \hack{\hfill\break}?>formulation (<inline-formula><mml:math id="M1787" display="inline"><mml:mrow><mml:mi>k</mml:mi><mml:mo>×</mml:mo><mml:msup><mml:mi>U</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>) (Wanninkhof., 2014) with the transfer coefficient <inline-formula><mml:math id="M1788" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula> scaled to match a global mean transfer rate of 16.5 cm h<inline-formula><mml:math id="M1789" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Naegler, 2009).</oasis:entry>
         <oasis:entry colname="col5">Quadratic formulation<?xmltex \hack{\hfill\break}?> <inline-formula><mml:math id="M1790" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi>a</mml:mi><mml:mo>×</mml:mo><mml:msup><mml:mi>u</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>). We use scaled <inline-formula><mml:math id="M1791" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for ERA5 reanalysis wind data, which are scaled globally to 16.5 cm h<inline-formula><mml:math id="M1792" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (after Naegler, 2009) like in Fay and Gregor et al. (2021).</oasis:entry>
         <oasis:entry colname="col6">Nightingale et al.<?xmltex \hack{\hfill\break}?>(2000) formulation: <?xmltex \hack{\hfill\break}?> <inline-formula><mml:math id="M1793" display="inline"><mml:mrow><mml:mi>K</mml:mi><mml:mo>=</mml:mo><mml:mo>(</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">600</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup><mml:mo>)</mml:mo><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">0.333</mml:mn><mml:mo>×</mml:mo><mml:mi>U</mml:mi><mml:mo>+</mml:mo><mml:mn mathvariant="normal">0.222</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mi>U</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>)</mml:mo></mml:mrow></mml:math></inline-formula>.</oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M1794" display="inline"><mml:mrow><mml:msub><mml:mi>K</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mn mathvariant="normal">0.251</mml:mn><mml:mo>×</mml:mo><mml:mi>W</mml:mi><mml:mi>n</mml:mi><mml:mi>d</mml:mi><mml:mo>×</mml:mo><mml:mi>W</mml:mi><mml:mi>n</mml:mi><mml:mi>d</mml:mi><mml:mo>/</mml:mo><mml:msqrt><mml:mrow><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660.0</mml:mn><mml:mo>)</mml:mo></mml:mrow></mml:msqrt></mml:mrow></mml:math></inline-formula> (Wanninkhof, 2014).</oasis:entry>
         <oasis:entry colname="col8">Quadratic exchange<?xmltex \hack{\hfill\break}?>formulation (<inline-formula><mml:math id="M1795" display="inline"><mml:mrow><mml:mi>k</mml:mi><mml:mo>×</mml:mo><mml:msup><mml:mi>U</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>) (Wanninkhof, 2014) with the transfer coefficient <inline-formula><mml:math id="M1796" display="inline"><mml:mi>k</mml:mi></mml:math></inline-formula> scaled to match a global mean transfer rate of 16.5 cm h<inline-formula><mml:math id="M1797" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (Naegler, 2009) under fitted to the JRA55 wind field.</oasis:entry>
         <oasis:entry colname="col9">Quadratic formulation<?xmltex \hack{\hfill\break}?>of bulk air–sea CO<inline-formula><mml:math id="M1798" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux: <?xmltex \hack{\hfill\break}?> <inline-formula><mml:math id="M1799" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi>a</mml:mi><mml:mo>×</mml:mo><mml:msup><mml:mi>u</mml:mi><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:mo>(</mml:mo><mml:mi>S</mml:mi><mml:mi>c</mml:mi><mml:mo>/</mml:mo><mml:mn mathvariant="normal">660</mml:mn><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">0.5</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula>  <?xmltex \hack{\hfill\break}?>We use individually scaled <inline-formula><mml:math id="M1800" display="inline"><mml:mrow><mml:msub><mml:mi>k</mml:mi><mml:mi mathvariant="normal">w</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>'s for JRA55, ERA5, and NCEP-R1, which are all scaled globally to 16.5 cm h<inline-formula><mml:math id="M1801" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (after Naegler, 2009). See Fay and Gregor et al. (2021).</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{p}?><table-wrap id="App1.Ch1.S1.T16" specific-use="star" orientation="landscape"><?xmltex \currentcnt{A3}?><label>Table A3</label><caption><p id="d1e25949">Continued.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.73}[.73]?><oasis:tgroup cols="9">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="2.5cm"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="5" colname="col5" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="6" colname="col6" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="7" colname="col7" align="justify" colwidth="3cm"/>
     <oasis:colspec colnum="8" colname="col8" align="justify" colwidth="3.2cm"/>
     <oasis:colspec colnum="9" colname="col9" align="justify" colwidth="3.2cm"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">Jena-MLS</oasis:entry>
         <oasis:entry colname="col3">MPI-SOMFFN</oasis:entry>
         <oasis:entry colname="col4">CMEMS-LSCE-FFNN</oasis:entry>
         <oasis:entry colname="col5">CSIR-ML6</oasis:entry>
         <oasis:entry colname="col6">Watson et al.</oasis:entry>
         <oasis:entry colname="col7">NIES-NN</oasis:entry>
         <oasis:entry colname="col8">JMA-MLR</oasis:entry>
         <oasis:entry colname="col9">OS-ETHZ-GRaCER</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Wind product</oasis:entry>
         <oasis:entry colname="col2">JMA55-do reanalysis</oasis:entry>
         <oasis:entry colname="col3">ERA 5</oasis:entry>
         <oasis:entry colname="col4">ERA5</oasis:entry>
         <oasis:entry colname="col5">ERA5</oasis:entry>
         <oasis:entry colname="col6">CCMP wind product, <inline-formula><mml:math id="M1802" display="inline"><mml:mrow><mml:mn mathvariant="normal">0.25</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">0.25</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1803" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1804" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 6-hourly, from which we calculate mean and mean square winds over <inline-formula><mml:math id="M1805" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1806" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> and 1-month intervals. CCMP product does not cover years 1985–1987, for which we use a monthly climatology calculated as the means of 1988–1991.</oasis:entry>
         <oasis:entry colname="col7">ERA5</oasis:entry>
         <oasis:entry colname="col8">JRA55</oasis:entry>
         <oasis:entry colname="col9">JRA55, ERA5, NCEP1</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Spatial resolution</oasis:entry>
         <oasis:entry colname="col2">2.5<inline-formula><mml:math id="M1807" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> longitude <inline-formula><mml:math id="M1808" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2<inline-formula><mml:math id="M1809" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> latitude</oasis:entry>
         <oasis:entry colname="col3"><inline-formula><mml:math id="M1810" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1811" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M1812" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1813" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1814" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1815" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6"><inline-formula><mml:math id="M1816" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1817" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7"><inline-formula><mml:math id="M1818" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1819" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col8"><inline-formula><mml:math id="M1820" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1821" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M1822" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1823" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Temporal <?xmltex \hack{\hfill\break}?>resolution</oasis:entry>
         <oasis:entry colname="col2">daily</oasis:entry>
         <oasis:entry colname="col3">monthly</oasis:entry>
         <oasis:entry colname="col4">monthly</oasis:entry>
         <oasis:entry colname="col5">monthly</oasis:entry>
         <oasis:entry colname="col6">monthly</oasis:entry>
         <oasis:entry colname="col7">monthly</oasis:entry>
         <oasis:entry colname="col8">monthly</oasis:entry>
         <oasis:entry colname="col9">monthly</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric CO<inline-formula><mml:math id="M1824" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Spatially and temporally varying field based on atmospheric CO<inline-formula><mml:math id="M1825" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data from 169 stations (Jena CarboScope atmospheric inversion sEXTALL_v2021).</oasis:entry>
         <oasis:entry colname="col3">Atmospheric <inline-formula><mml:math id="M1826" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1827" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>_wet calculated from the NOAA ESRL marine boundary layer xCO<inline-formula><mml:math id="M1828" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and the NCEP sea level pressure with the moisture correction by Dickson et al. (2007) (details and references can be obtained from Appendix A3 in Landschützer et al., 2013).</oasis:entry>
         <oasis:entry colname="col4">Spatially and monthly varying fields of atmospheric <inline-formula><mml:math id="M1829" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1830" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> computed from CO<inline-formula><mml:math id="M1831" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> mole fraction (Chevallier, 2013; CO<inline-formula><mml:math id="M1832" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> atmospheric inversion from the Copernicus Atmosphere Monitoring Service), and atmospheric dry-air pressure which is derived from monthly surface pressure (ERA5) and water vapour pressure fitted by Weiss and Price (1980).</oasis:entry>
         <oasis:entry colname="col5">The NOAA's marine boundary layer product for the mole fraction of carbon dioxide (xCO<inline-formula><mml:math id="M1833" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) is linearly interpolated onto a 1<inline-formula><mml:math id="M1834" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1835" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M1836" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> grid and resampled from weekly to monthly. Basically, xCO<inline-formula><mml:math id="M1837" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> is multiplied by ERA5 mean sea level pressure (MSLP), and a water vapour pressure correction is applied to MSLP using the equation from Dickson et al. (2007). This results in monthly 1<inline-formula><mml:math id="M1838" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1839" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M1840" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> atmospheric <inline-formula><mml:math id="M1841" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1842" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>.</oasis:entry>
         <oasis:entry colname="col6">Atmospheric <inline-formula><mml:math id="M1843" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1844" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (wet) calculated from NOAA marine boundary layer XCO<inline-formula><mml:math id="M1845" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and NCEP sea level pressure, with <inline-formula><mml:math id="M1846" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>H<inline-formula><mml:math id="M1847" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>O calculated from Cooper et al. (1998). (2019 XCO<inline-formula><mml:math id="M1848" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> marine boundary values were not available at submission so we used preliminary values, estimated from 2018 values and increase at Mauna Loa.)</oasis:entry>
         <oasis:entry colname="col7">NOAA Greenhouse Gas Marine Boundary Layer Reference. <uri>https://gml.noaa.gov/ccgg/mbl/mbl.html</uri> (last access: 11 March 2022)</oasis:entry>
         <oasis:entry colname="col8">Atmospheric xCO<inline-formula><mml:math id="M1849" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fields of JMA-GSAM inversion model (Maki et al., 2010; Nakamura et al., 2015) were used. They were converted to <inline-formula><mml:math id="M1850" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1851" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> by using JRA55 sea level pressure. xCO<inline-formula><mml:math id="M1852" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fields in 2020 were not available at this stage, and we use observation data of obspack_CO<inline-formula><mml:math id="M1853" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>_1 _NRT_v6.1.1 _2021-05-17 (Di Sarra et al., 2021) to estimate the increase from 2019 to 2020.</oasis:entry>
         <oasis:entry colname="col9">NOAA's marine boundary layer product for xCO<inline-formula><mml:math id="M1854" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> is linearly interpolated onto a <inline-formula><mml:math id="M1855" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1856" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> grid and resampled from weekly to monthly. xCO<inline-formula><mml:math id="M1857" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> is multiplied by ERA5 mean sea level pressure, where the latter corrected for water vapour pressure using Dickson et al. (2007). This results in monthly <inline-formula><mml:math id="M1858" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup><mml:mo>×</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula><inline-formula><mml:math id="M1859" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1860" display="inline"><mml:mi>p</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1861" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>atm.</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Total ocean area on native grid (km<inline-formula><mml:math id="M1862" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>)</oasis:entry>
         <oasis:entry colname="col2">3.63E<inline-formula><mml:math id="M1863" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col3">3.63E<inline-formula><mml:math id="M1864" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col4">3.46E<inline-formula><mml:math id="M1865" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col5">3.48E<inline-formula><mml:math id="M1866" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col6">3.51E<inline-formula><mml:math id="M1867" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col7">3.28E<inline-formula><mml:math id="M1868" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08 <?xmltex \hack{\hfill\break}?>(3.23E<inline-formula><mml:math id="M1869" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08 to<?xmltex \hack{\hfill\break}?>3.35E<inline-formula><mml:math id="M1870" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08, <?xmltex \hack{\hfill\break}?>depending on ice cover)</oasis:entry>
         <oasis:entry colname="col8">3.05E<inline-formula><mml:math id="M1871" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08 <?xmltex \hack{\hfill\break}?>(2.98E<inline-formula><mml:math id="M1872" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08 to 3.15E<inline-formula><mml:math id="M1873" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08, depending on ice cover)</oasis:entry>
         <oasis:entry colname="col9">3.55E<inline-formula><mml:math id="M1874" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Method to <?xmltex \hack{\hfill\break}?>extend product to<?xmltex \hack{\hfill\break}?>full global ocean<?xmltex \hack{\hfill\break}?>coverage</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">Arctic and marginal<?xmltex \hack{\hfill\break}?>seas added <?xmltex \hack{\hfill\break}?>following Landschützer et al. (2020). <?xmltex \hack{\hfill\break}?>Previously applied<?xmltex \hack{\hfill\break}?>coastal cut (1<inline-formula><mml:math id="M1875" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula><?xmltex \hack{\hfill\break}?>off coast) was dropped</oasis:entry>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8">We used the same <?xmltex \hack{\hfill\break}?>method as Fay et <?xmltex \hack{\hfill\break}?>al. (2021a)</oasis:entry>
         <oasis:entry colname="col9">Method has near full<?xmltex \hack{\hfill\break}?>coverage</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Ocean area on <?xmltex \hack{\hfill\break}?>native grid (km<inline-formula><mml:math id="M1876" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>) – North</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">5.4545E<inline-formula><mml:math id="M1877" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07</oasis:entry>
         <oasis:entry colname="col5">5.0528E<inline-formula><mml:math id="M1878" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07</oasis:entry>
         <oasis:entry colname="col6">5.0700E<inline-formula><mml:math id="M1879" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8">3.90E<inline-formula><mml:math id="M1880" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07 <?xmltex \hack{\hfill\break}?>(3.75E<inline-formula><mml:math id="M1881" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07 to 4.09E<inline-formula><mml:math id="M1882" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07, depending on ice cover)</oasis:entry>
         <oasis:entry colname="col9">5.9771E<inline-formula><mml:math id="M1883" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Ocean area on <?xmltex \hack{\hfill\break}?>native grid (km<inline-formula><mml:math id="M1884" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>) – tropics</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">1.8875E<inline-formula><mml:math id="M1885" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col5">1.8933E<inline-formula><mml:math id="M1886" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col6">1.9230E<inline-formula><mml:math id="M1887" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8">1.74E<inline-formula><mml:math id="M1888" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col9">1.8779E<inline-formula><mml:math id="M1889" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Ocean area on <?xmltex \hack{\hfill\break}?>native grid (km<inline-formula><mml:math id="M1890" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>) – south</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">1.0241E<inline-formula><mml:math id="M1891" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col5">1.0767E<inline-formula><mml:math id="M1892" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col6">1.0868E<inline-formula><mml:math id="M1893" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8">9.20E<inline-formula><mml:math id="M1894" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07 <?xmltex \hack{\hfill\break}?>(8.47E<inline-formula><mml:math id="M1895" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>07 to 1.02E<inline-formula><mml:math id="M1896" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08, depending on ice cover)</oasis:entry>
         <oasis:entry colname="col9">1.0705E<inline-formula><mml:math id="M1897" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>08</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{t}?><table-wrap id="App1.Ch1.S1.T17" specific-use="star"><?xmltex \currentcnt{A4}?><label>Table A4</label><caption><p id="d1e27161">Comparison of the inversion set-up and input fields for the atmospheric inversions. Atmospheric inversions include the full CO<inline-formula><mml:math id="M1898" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes, including the anthropogenic and pre-industrial fluxes. Hence they need to be adjusted for the pre-industrial flux of CO<inline-formula><mml:math id="M1899" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> from the land to the ocean that is part of the natural carbon cycle before they can be compared with <inline-formula><mml:math id="M1900" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M1901" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from process models. See Table 4 for references.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.75}[.75]?><oasis:tgroup cols="7">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="5" colname="col5" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="6" colname="col6" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="7" colname="col7" align="justify" colwidth="2.8cm"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">CarbonTracker <?xmltex \hack{\hfill\break}?>Europe (CTE)</oasis:entry>
         <oasis:entry colname="col3">Jena CarboScope</oasis:entry>
         <oasis:entry colname="col4">Copernicus <?xmltex \hack{\hfill\break}?>Atmosphere<?xmltex \hack{\hfill\break}?>Monitoring Service<?xmltex \hack{\hfill\break}?>(CAMS)</oasis:entry>
         <oasis:entry colname="col5">UoE</oasis:entry>
         <oasis:entry colname="col6">CMS-Flux</oasis:entry>
         <oasis:entry colname="col7">NISMON-CO<inline-formula><mml:math id="M1906" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula></oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Version number</oasis:entry>
         <oasis:entry colname="col2">CTE2021</oasis:entry>
         <oasis:entry colname="col3">sEXTocNEET_v2021</oasis:entry>
         <oasis:entry colname="col4">v20r2</oasis:entry>
         <oasis:entry colname="col5">In situ</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">v2021.1</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Observations</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Atmospheric observations</oasis:entry>
         <oasis:entry colname="col2">Hourly resolution <?xmltex \hack{\hfill\break}?>(well-mixed <?xmltex \hack{\hfill\break}?>conditions) obspack GLOBALVIEWplus v6.1 and<?xmltex \hack{\hfill\break}?>NRT_v6.1.1<inline-formula><mml:math id="M1907" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Flasks and hourly<?xmltex \hack{\hfill\break}?>from various<?xmltex \hack{\hfill\break}?>institutions (outliers removed by <inline-formula><mml:math id="M1908" display="inline"><mml:mrow><mml:mn mathvariant="normal">2</mml:mn><mml:mi mathvariant="italic">σ</mml:mi></mml:mrow></mml:math></inline-formula> <?xmltex \hack{\hfill\break}?>criterion)</oasis:entry>
         <oasis:entry colname="col4">Hourly resolution <?xmltex \hack{\hfill\break}?>(well-mixed<?xmltex \hack{\hfill\break}?>conditions) obspack <?xmltex \hack{\hfill\break}?>GLOBALVIEWplus v6.1 and <?xmltex \hack{\hfill\break}?>NRT_v6.1.1<inline-formula><mml:math id="M1909" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula>,<?xmltex \hack{\hfill\break}?>WDCGG, RAMCES and ICOS ATC</oasis:entry>
         <oasis:entry colname="col5">Hourly resolution <?xmltex \hack{\hfill\break}?>(well-mixed<?xmltex \hack{\hfill\break}?>conditions) obspack GLOBALVIEWplus v6.1 and <?xmltex \hack{\hfill\break}?>NRT_v6.1.1<inline-formula><mml:math id="M1910" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">ACOS-GOSAT v9 (6) retrievals between July 2009 and Dec 2014 and OCO-2 b10 (7) retrievals between Jan 2015 to Dec 2015. In addition, surface flask observations from remote sites were also assimilated from GLOBALVIEWplus v6.1 and NRT_v6.1.1.</oasis:entry>
         <oasis:entry colname="col7">Hourly resolution<?xmltex \hack{\hfill\break}?>(well-mixed <?xmltex \hack{\hfill\break}?>conditions) obspack <?xmltex \hack{\hfill\break}?>GLOBALVIEWplus v6.1 and<?xmltex \hack{\hfill\break}?>NRT_v6.1.1<inline-formula><mml:math id="M1911" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Period covered</oasis:entry>
         <oasis:entry colname="col2">2001–2020</oasis:entry>
         <oasis:entry colname="col3">1957–2020</oasis:entry>
         <oasis:entry colname="col4">1979–2021</oasis:entry>
         <oasis:entry colname="col5">2001–2020</oasis:entry>
         <oasis:entry colname="col6">2010–2020</oasis:entry>
         <oasis:entry colname="col7">1990–2020</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Prior fluxes</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Biosphere and fires</oasis:entry>
         <oasis:entry colname="col2">SIBCASA biosphere<inline-formula><mml:math id="M1912" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> with 2019–2020<?xmltex \hack{\hfill\break}?>climatological, GFAS fires</oasis:entry>
         <oasis:entry colname="col3">No prior</oasis:entry>
         <oasis:entry colname="col4">ORCHIDEE <?xmltex \hack{\hfill\break}?>(climatological), GFEDv4.1s</oasis:entry>
         <oasis:entry colname="col5">CASA v1.0, climatology after 2016 and<?xmltex \hack{\hfill\break}?>GFED4.0</oasis:entry>
         <oasis:entry colname="col6">yearly repeating <?xmltex \hack{\hfill\break}?>CARDAMOM biosphere<inline-formula><mml:math id="M1913" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>fires</oasis:entry>
         <oasis:entry colname="col7">VISIT and <?xmltex \hack{\hfill\break}?>GFEDv4.1s</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Ocean</oasis:entry>
         <oasis:entry colname="col2">oc_v2020<?xmltex \hack{\hfill\break}?>(Rödenbeck et al., <?xmltex \hack{\hfill\break}?>2014), with updates, For 2020: climatology based on years 2015–2019</oasis:entry>
         <oasis:entry colname="col3">oc_v2021 (Rödenbeck et al., 2014) with updates</oasis:entry>
         <oasis:entry colname="col4">CMEMS Copernicus ocean fluxes (Denvil-Sommer et al., 2019), with updates</oasis:entry>
         <oasis:entry colname="col5">Takahashi<?xmltex \hack{\hfill\break}?>climatology</oasis:entry>
         <oasis:entry colname="col6">MOM6</oasis:entry>
         <oasis:entry colname="col7">JMA global ocean <?xmltex \hack{\hfill\break}?>mapping (Iida et al., 2015)</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Fossil fuels</oasis:entry>
         <oasis:entry colname="col2">GCP-GridFEDv2021.1 (Jones et al., 2021b) for 2000–2018, GCP-GridFEDv2021.2 for 2019<inline-formula><mml:math id="M1914" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula>2020<inline-formula><mml:math id="M1915" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">GCP-GridFEDv2021.2 (Jones et al., 2021b)<inline-formula><mml:math id="M1916" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4">GCP-GridFEDv2021.2 (Jones et al., 2021b)<inline-formula><mml:math id="M1917" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">GCP-GridFEDv2021.2 (Jones et al., 2021b)<inline-formula><mml:math id="M1918" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">GCP-GridFEDv2021.2 (Jones et al., 2021b)<inline-formula><mml:math id="M1919" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">GCP-GridFEDv2021.2 (Jones et al., 2021b)<inline-formula><mml:math id="M1920" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Transport and optimization</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Transport model</oasis:entry>
         <oasis:entry colname="col2">TM5</oasis:entry>
         <oasis:entry colname="col3">TM3</oasis:entry>
         <oasis:entry colname="col4">LMDZ v6</oasis:entry>
         <oasis:entry colname="col5">GEOS-CHEM</oasis:entry>
         <oasis:entry colname="col6">GEOS-CHEM</oasis:entry>
         <oasis:entry colname="col7">NICAM-TM</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Weather forcing</oasis:entry>
         <oasis:entry colname="col2">ECMWF</oasis:entry>
         <oasis:entry colname="col3">NCEP</oasis:entry>
         <oasis:entry colname="col4">ECMWF</oasis:entry>
         <oasis:entry colname="col5">MERRA2</oasis:entry>
         <oasis:entry colname="col6">MERRA-2</oasis:entry>
         <oasis:entry colname="col7">JRA55</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Horizontal resolution</oasis:entry>
         <oasis:entry colname="col2">Global: 3<inline-formula><mml:math id="M1921" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1922" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 2<inline-formula><mml:math id="M1923" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>,<?xmltex \hack{\hfill\break}?>Europe: 1<inline-formula><mml:math id="M1924" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1925" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M1926" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula>,<?xmltex \hack{\hfill\break}?>North America: <?xmltex \hack{\hfill\break}?>1<inline-formula><mml:math id="M1927" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1928" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M1929" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col3">Global: 4<inline-formula><mml:math id="M1930" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1931" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 5<inline-formula><mml:math id="M1932" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4">Global: 3.75<inline-formula><mml:math id="M1933" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1934" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 1.875<inline-formula><mml:math id="M1935" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col5">Global: 4<inline-formula><mml:math id="M1936" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1937" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 5<inline-formula><mml:math id="M1938" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col6">Global: 4<inline-formula><mml:math id="M1939" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M1940" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 5<inline-formula><mml:math id="M1941" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col7">isocahedral grid:<?xmltex \hack{\hfill\break}?> <inline-formula><mml:math id="M1942" display="inline"><mml:mo>∼</mml:mo></mml:math></inline-formula> 225 km</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Optimization</oasis:entry>
         <oasis:entry colname="col2">Ensemble Kalman<?xmltex \hack{\hfill\break}?>filter</oasis:entry>
         <oasis:entry colname="col3">Conjugate<?xmltex \hack{\hfill\break}?>gradient <?xmltex \hack{\hfill\break}?>(re-ortho-normalization)<inline-formula><mml:math id="M1943" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4">Variational</oasis:entry>
         <oasis:entry colname="col5">Ensemble Kalman <?xmltex \hack{\hfill\break}?>filter</oasis:entry>
         <oasis:entry colname="col6">Variational</oasis:entry>
         <oasis:entry colname="col7">Variational</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table><table-wrap-foot><p id="d1e27204"><inline-formula><mml:math id="M1902" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula> Cox et al. (2021); Di Sarra et al. (2021). <inline-formula><mml:math id="M1903" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> van der Velde et al. (2014). <inline-formula><mml:math id="M1904" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula> GCP-GridFEDv2021.2 (Jones et al., 2021b) is an update through the year 2020 of the GCP-GridFED <?xmltex \hack{\break}?> dataset presented by Jones et al. (2021a). <inline-formula><mml:math id="M1905" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula> Ocean prior not optimized.</p></table-wrap-foot></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{t}?><table-wrap id="App1.Ch1.S1.T18" specific-use="star"><?xmltex \currentcnt{A5}?><label>Table A5</label><caption><p id="d1e27993">Attribution of <inline-formula><mml:math id="M1944" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1945" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements for the year 2020 included in SOCATv2021 (Bakker et al., 2016, 2021) to inform ocean <inline-formula><mml:math id="M1946" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M1947" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.85}[.85]?><oasis:tgroup cols="6">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="4.6cm"/>
     <oasis:colspec colnum="3" colname="col3" align="right"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="4.2cm"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:colspec colnum="6" colname="col6" align="left"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Platform</oasis:entry>
         <oasis:entry colname="col2">Regions</oasis:entry>
         <oasis:entry colname="col3">No. of</oasis:entry>
         <oasis:entry colname="col4">Principal</oasis:entry>
         <oasis:entry colname="col5">No. of</oasis:entry>
         <oasis:entry colname="col6">Platform</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">name</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">measurements</oasis:entry>
         <oasis:entry colname="col4">investigators</oasis:entry>
         <oasis:entry colname="col5">datasets</oasis:entry>
         <oasis:entry colname="col6">type</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1"><italic>1 degree</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">8652</oasis:entry>
         <oasis:entry colname="col4">Gutekunst, S.</oasis:entry>
         <oasis:entry colname="col5">2</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Allure of the Seas</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, tropical Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">19 321</oasis:entry>
         <oasis:entry colname="col4">Wanninkhof, R.; Pierrot, D.</oasis:entry>
         <oasis:entry colname="col5">8</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Atlantic Explorer</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic</oasis:entry>
         <oasis:entry colname="col3">15 665</oasis:entry>
         <oasis:entry colname="col4">Bates, N.</oasis:entry>
         <oasis:entry colname="col5">11</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Atlantic Sail</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">25 082</oasis:entry>
         <oasis:entry colname="col4">Steinhoff, T.; Körtzinger, A.</oasis:entry>
         <oasis:entry colname="col5">6</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Aurora Australis</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean</oasis:entry>
         <oasis:entry colname="col3">14 316</oasis:entry>
         <oasis:entry colname="col4">Tilbrook, B.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Bjarni Saemundsson</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">3269</oasis:entry>
         <oasis:entry colname="col4">Benoit-Cattin A.; Ólafsdóttir, S. R.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>BlueFin</italic></oasis:entry>
         <oasis:entry colname="col2">North Pacific, tropical Pacific, coastal</oasis:entry>
         <oasis:entry colname="col3">76 505</oasis:entry>
         <oasis:entry colname="col4">Alin, S. R.; Feely, R. A.</oasis:entry>
         <oasis:entry colname="col5">12</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Cap San Lorenzo</italic></oasis:entry>
         <oasis:entry colname="col2">Tropical Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">12 417</oasis:entry>
         <oasis:entry colname="col4">Lefèvre, N.</oasis:entry>
         <oasis:entry colname="col5">2</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Celtic Explorer</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">18 617</oasis:entry>
         <oasis:entry colname="col4">Cronin, M.</oasis:entry>
         <oasis:entry colname="col5">6</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Colibri</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, tropical Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">13 402</oasis:entry>
         <oasis:entry colname="col4">Lefèvre, N.</oasis:entry>
         <oasis:entry colname="col5">2</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Equinox</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">25 052</oasis:entry>
         <oasis:entry colname="col4">Wanninkhof, R.; Pierrot, D.</oasis:entry>
         <oasis:entry colname="col5">11</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>F. G. Walton Smith</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">10 460</oasis:entry>
         <oasis:entry colname="col4">Rodriguez, C.; Millero, F. J.; Pierrot, D.; Wanninkhof, R.</oasis:entry>
         <oasis:entry colname="col5">6</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Finnmaid</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">253 894</oasis:entry>
         <oasis:entry colname="col4">Rehder, G.; Glockzin, M.</oasis:entry>
         <oasis:entry colname="col5">11</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Flora</italic></oasis:entry>
         <oasis:entry colname="col2">Tropical Pacific</oasis:entry>
         <oasis:entry colname="col3">4099</oasis:entry>
         <oasis:entry colname="col4">Wanninkhof, R.; Pierrot, D.</oasis:entry>
         <oasis:entry colname="col5">2</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>G.O. Sars</italic></oasis:entry>
         <oasis:entry colname="col2">Arctic, North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">75 833</oasis:entry>
         <oasis:entry colname="col4">Skjelvan, I.</oasis:entry>
         <oasis:entry colname="col5">7</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>GAKOA_149W_60N</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">68</oasis:entry>
         <oasis:entry colname="col4">Cross, J. N.; Monacci, N. M.</oasis:entry>
         <oasis:entry colname="col5">3</oasis:entry>
         <oasis:entry colname="col6">Mooring</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Gulf Challenger</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">2717</oasis:entry>
         <oasis:entry colname="col4">Salisbury, J.; Vandemark, D.; Hunt, C.</oasis:entry>
         <oasis:entry colname="col5">3</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Healy</italic></oasis:entry>
         <oasis:entry colname="col2">Arctic, North Pacific, coastal</oasis:entry>
         <oasis:entry colname="col3">16 943</oasis:entry>
         <oasis:entry colname="col4">Sweeney, C.; Newberger, T.; Sutherland, S. C.; Munro, D. R.</oasis:entry>
         <oasis:entry colname="col5">4</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Henry B. Bigelow</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">14 436</oasis:entry>
         <oasis:entry colname="col4">Wanninkhof, R.; Pierrot, D.</oasis:entry>
         <oasis:entry colname="col5">4</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Heron Island</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">768</oasis:entry>
         <oasis:entry colname="col4">Tilbrook B.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Mooring</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>James Clark Ross</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean</oasis:entry>
         <oasis:entry colname="col3">2000</oasis:entry>
         <oasis:entry colname="col4">Kitidis, V.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>James Cook</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, tropical Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">46 710</oasis:entry>
         <oasis:entry colname="col4">Theetaert, H.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>KC_BUOY</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">1983</oasis:entry>
         <oasis:entry colname="col4">Evans, W.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Mooring</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Laurence M. Gould</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean</oasis:entry>
         <oasis:entry colname="col3">25 414</oasis:entry>
         <oasis:entry colname="col4">Sweeney, C.; Newberger, T.; Sutherland, S. C.; Munro, D. R.</oasis:entry>
         <oasis:entry colname="col5">4</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Maria. S. Merian</italic></oasis:entry>
         <oasis:entry colname="col2">Tropical Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">35 806</oasis:entry>
         <oasis:entry colname="col4">Ritschel, M.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Marion Dufresne</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean, Indian</oasis:entry>
         <oasis:entry colname="col3">4709</oasis:entry>
         <oasis:entry colname="col4">Lo Monaco, C.; Metzl, N.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Nathaniel B. Palmer</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean, tropical Pacific</oasis:entry>
         <oasis:entry colname="col3">34 357</oasis:entry>
         <oasis:entry colname="col4">Sweeney, C.; Newberger, T.; Sutherland, S. C.; Munro, D. R.</oasis:entry>
         <oasis:entry colname="col5">3</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>New Century 2</italic></oasis:entry>
         <oasis:entry colname="col2">North Pacific, tropical Pacific, tropical Atlantic, North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">27 793</oasis:entry>
         <oasis:entry colname="col4">Nakaoka, S.-I.</oasis:entry>
         <oasis:entry colname="col5">14</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Nuka Arctica</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">26 576</oasis:entry>
         <oasis:entry colname="col4">Becker, M.; Olsen, A.</oasis:entry>
         <oasis:entry colname="col5">6</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Oscar Dyson</italic></oasis:entry>
         <oasis:entry colname="col2">Arctic, North Pacific, coastal</oasis:entry>
         <oasis:entry colname="col3">28 196</oasis:entry>
         <oasis:entry colname="col4">Alin, S. R.; Feely, R. A.</oasis:entry>
         <oasis:entry colname="col5">6</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Quadra Island Field Station</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">78 098</oasis:entry>
         <oasis:entry colname="col4">Evans, W.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Mooring</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Ronald H. Brown</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean, tropical Atlantic, North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">51 611</oasis:entry>
         <oasis:entry colname="col4">Wanninkhof, R.; Pierrot, D.</oasis:entry>
         <oasis:entry colname="col5">6</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Saildrone1030</italic></oasis:entry>
         <oasis:entry colname="col2">North Atlantic, tropical Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">4080</oasis:entry>
         <oasis:entry colname="col4">Skjelvan, I.; Fiedler, B.; Pfeil, B.; Jones, S. D.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Saildrone</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Sea Explorer</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean, tropical Atlantic, North Atlantic, coastal</oasis:entry>
         <oasis:entry colname="col3">89 896</oasis:entry>
         <oasis:entry colname="col4">Landschützer, P.; Tanhua, T.</oasis:entry>
         <oasis:entry colname="col5">6</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Sikuliaq</italic></oasis:entry>
         <oasis:entry colname="col2">Arctic, North Pacific, coastal</oasis:entry>
         <oasis:entry colname="col3">36 278</oasis:entry>
         <oasis:entry colname="col4">Sweeney, C.; Newberger, T.; Sutherland, S. C.; Munro, D. R.</oasis:entry>
         <oasis:entry colname="col5">10</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Simon Stevin</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">16 448</oasis:entry>
         <oasis:entry colname="col4">Gkritzalis, T.</oasis:entry>
         <oasis:entry colname="col5">4</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Soyo Maru</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">46 280</oasis:entry>
         <oasis:entry colname="col4">Ono, T.</oasis:entry>
         <oasis:entry colname="col5">2</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Tangaroa</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean, tropical Pacific</oasis:entry>
         <oasis:entry colname="col3">121 135</oasis:entry>
         <oasis:entry colname="col4">Currie, K. I.</oasis:entry>
         <oasis:entry colname="col5">13</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>TAO110W_0N</italic></oasis:entry>
         <oasis:entry colname="col2">Tropical Pacific</oasis:entry>
         <oasis:entry colname="col3">1518</oasis:entry>
         <oasis:entry colname="col4">Sutton, A. J.</oasis:entry>
         <oasis:entry colname="col5">3</oasis:entry>
         <oasis:entry colname="col6">Mooring</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Tavastland</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">4214</oasis:entry>
         <oasis:entry colname="col4">Willstrand Wranne, A., Steinhoff, T.</oasis:entry>
         <oasis:entry colname="col5">5</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Thomas G. Thompson</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean, tropical Atlantic</oasis:entry>
         <oasis:entry colname="col3">1317</oasis:entry>
         <oasis:entry colname="col4">Alin, S. R.; Feely, R. A.</oasis:entry>
         <oasis:entry colname="col5">1</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Trans Carrier</italic></oasis:entry>
         <oasis:entry colname="col2">Coastal</oasis:entry>
         <oasis:entry colname="col3">24 135</oasis:entry>
         <oasis:entry colname="col4">Omar, A. M.</oasis:entry>
         <oasis:entry colname="col5">13</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Trans Future 5</italic></oasis:entry>
         <oasis:entry colname="col2">Southern Ocean, coastal</oasis:entry>
         <oasis:entry colname="col3">16 404</oasis:entry>
         <oasis:entry colname="col4">Nakaoka, S.-I.; Nojiri, Y.</oasis:entry>
         <oasis:entry colname="col5">15</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><italic>Wakataka Maru</italic></oasis:entry>
         <oasis:entry colname="col2">North Pacific, Coastal</oasis:entry>
         <oasis:entry colname="col3">101 327</oasis:entry>
         <oasis:entry colname="col4">Tadokoro, K.; Ono, T.</oasis:entry>
         <oasis:entry colname="col5">7</oasis:entry>
         <oasis:entry colname="col6">Ship</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{t}?><table-wrap id="App1.Ch1.S1.T19" specific-use="star"><?xmltex \currentcnt{A6}?><label>Table A6</label><caption><p id="d1e29119">Aircraft measurement programmes archived by Cooperative Global Atmospheric Data Integration Project (CGADIP; Cox et al., 2021) that contribute to the evaluation of the atmospheric inversions (Fig. B4).</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.88}[.88]?><oasis:tgroup cols="5">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="4.2cm"/>
     <oasis:colspec colnum="3" colname="col3" align="left"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="4.4cm"/>
     <oasis:colspec colnum="5" colname="col5" align="left"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Site</oasis:entry>
         <oasis:entry colname="col2">Measurement programme</oasis:entry>
         <oasis:entry colname="col3">Specific</oasis:entry>
         <oasis:entry colname="col4">Data</oasis:entry>
         <oasis:entry colname="col5">Used in</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">code</oasis:entry>
         <oasis:entry colname="col2">name in Obspack</oasis:entry>
         <oasis:entry colname="col3">DOI</oasis:entry>
         <oasis:entry colname="col4">providers</oasis:entry>
         <oasis:entry colname="col5">2021</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">AAO</oasis:entry>
         <oasis:entry colname="col2">Airborne Aerosol Observatory, Bondville, Illinois</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ACG</oasis:entry>
         <oasis:entry colname="col2">Alaska Coast Guard</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; McKain, K.; Karion, A.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ACT</oasis:entry>
         <oasis:entry colname="col2">Atmospheric Carbon and<?xmltex \hack{\hfill\break}?>Transport – America</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.; Baier, B; Montzka, S.; Davis, K.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ALF</oasis:entry>
         <oasis:entry colname="col2">Alta Floresta</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Gatti, L. V.; Gloor, E.; Miller, J. B.;</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">AOA</oasis:entry>
         <oasis:entry colname="col2">Aircraft Observation of<?xmltex \hack{\hfill\break}?>Atmospheric trace gases by JMA</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">ghg_obs@met.kishou.go.jp</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BGI</oasis:entry>
         <oasis:entry colname="col2">Bradgate, Iowa</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BNE</oasis:entry>
         <oasis:entry colname="col2">Beaver Crossing, Nebraska</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BRZ</oasis:entry>
         <oasis:entry colname="col2">Berezorechka, Russia</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sasakama, N.; Machida, T.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CAR</oasis:entry>
         <oasis:entry colname="col2">Briggsdale, Colorado</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CMA</oasis:entry>
         <oasis:entry colname="col2">Cape May, New Jersey</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CON</oasis:entry>
         <oasis:entry colname="col2">CONTRAIL (Comprehensive<?xmltex \hack{\hfill\break}?>Observation Network for TRace<?xmltex \hack{\hfill\break}?>gases by AIrLiner)</oasis:entry>
         <oasis:entry colname="col3"><ext-link xlink:href="https://doi.org/10.17595/20180208.001" ext-link-type="DOI">10.17595/20180208.001</ext-link></oasis:entry>
         <oasis:entry colname="col4">Machida, T.; Matsueda, H.; Sawa, Y.; Niwa, Y.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">CRV</oasis:entry>
         <oasis:entry colname="col2">Carbon in Arctic Reservoirs Vulnerability Experiment (CARVE)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Karion, A.; Miller, J. B.; Miller, C. E.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">DND</oasis:entry>
         <oasis:entry colname="col2">Dahlen, North Dakota</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ESP</oasis:entry>
         <oasis:entry colname="col2">Estevan Point, British Columbia</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">ETL</oasis:entry>
         <oasis:entry colname="col2">East Trout Lake, Saskatchewan</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">FWI</oasis:entry>
         <oasis:entry colname="col2">Fairchild, Wisconsin</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">GSFC</oasis:entry>
         <oasis:entry colname="col2">NASA Goddard Space Flight<?xmltex \hack{\hfill\break}?>Center Aircraft Campaign</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Kawa, S. R.; Abshire, J. B.; Riris, H.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HAA</oasis:entry>
         <oasis:entry colname="col2">Molokai Island, Hawaii</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HFM</oasis:entry>
         <oasis:entry colname="col2">Harvard University Aircraft<?xmltex \hack{\hfill\break}?>Campaign</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Wofsy, S. C.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HIL</oasis:entry>
         <oasis:entry colname="col2">Homer, Illinois</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HIP</oasis:entry>
         <oasis:entry colname="col2">HIPPO (HIAPER Pole-to-Pole Observations)</oasis:entry>
         <oasis:entry colname="col3"><ext-link xlink:href="https://doi.org/10.3334/CDIAC/HIPPO_010" ext-link-type="DOI">10.3334/CDIAC/HIPPO_010</ext-link></oasis:entry>
         <oasis:entry colname="col4">Wofsy, S. C.; Stephens, B. B.; Elkins, J. W.; Hintsa, E. J.; Moore, F.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">IAGOS-CARIBIC</oasis:entry>
         <oasis:entry colname="col2">In-service Aircraft for a Global<?xmltex \hack{\hfill\break}?>Observing System</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Obersteiner, F.; Boenisch., H; Gehrlein, T.; Zahn, A.; Schuck, T.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">INX</oasis:entry>
         <oasis:entry colname="col2">INFLUX (Indianapolis Flux <?xmltex \hack{\hfill\break}?>Experiment)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.; Shepson, P. B.; Turnbull, J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">LEF</oasis:entry>
         <oasis:entry colname="col2">Park Falls, Wisconsin</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">NHA</oasis:entry>
         <oasis:entry colname="col2">Offshore Portsmouth, New<?xmltex \hack{\hfill\break}?>Hampshire (Isles of Shoals)</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">OIL</oasis:entry>
         <oasis:entry colname="col2">Oglesby, Illinois</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PFA</oasis:entry>
         <oasis:entry colname="col2">Poker Flat, Alaska</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">RBA-B</oasis:entry>
         <oasis:entry colname="col2">Rio Branco</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Gatti, L. V.; Gloor, E.; Miller, J. B.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">RTA</oasis:entry>
         <oasis:entry colname="col2">Rarotonga</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">SCA</oasis:entry>
         <oasis:entry colname="col2">Charleston, South Carolina</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">SGP</oasis:entry>
         <oasis:entry colname="col2">Southern Great Plains, Oklahoma</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.; Biraud, S.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">TAB</oasis:entry>
         <oasis:entry colname="col2">Tabatinga</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Gatti, L. V.; Gloor, E.; Miller, J. B.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">TGC</oasis:entry>
         <oasis:entry colname="col2">Offshore Corpus Christi, Texas</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">THD</oasis:entry>
         <oasis:entry colname="col2">Trinidad Head, California</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">WBI</oasis:entry>
         <oasis:entry colname="col2">West Branch, Iowa</oasis:entry>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Sweeney, C.; Dlugokencky, E. J.</oasis:entry>
         <oasis:entry colname="col5">yes</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{p}?><table-wrap id="App1.Ch1.S1.T20" specific-use="star" orientation="landscape"><?xmltex \currentcnt{A7}?><label>Table A7</label><caption><p id="d1e29806">Main methodological changes in the global carbon budget since first publication. Methodological changes introduced in one year are kept for the following years unless noted. Empty cells mean there were no methodological changes introduced that year.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.8}[.8]?><oasis:tgroup cols="9">
     <oasis:colspec colnum="1" colname="col1" align="left"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="4" colname="col4" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="5" colname="col5" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="6" colname="col6" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="7" colname="col7" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="8" colname="col8" align="justify" colwidth="2.8cm"/>
     <oasis:colspec colnum="9" colname="col9" align="justify" colwidth="2.8cm"/>
     <oasis:thead>
       <oasis:row>
         <oasis:entry colname="col1">Publication year</oasis:entry>
         <oasis:entry rowsep="1" namest="col2" nameend="col4" align="center">Fossil fuel emissions </oasis:entry>
         <oasis:entry rowsep="1" colname="col5">LUC emissions</oasis:entry>
         <oasis:entry rowsep="1" namest="col6" nameend="col8" align="center">Reservoirs </oasis:entry>
         <oasis:entry colname="col9">Uncertainty and other <?xmltex \hack{\hfill\break}?>changes</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">Global</oasis:entry>
         <oasis:entry colname="col3">Country (territorial)</oasis:entry>
         <oasis:entry colname="col4">Country (consumption)</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6">Atmosphere</oasis:entry>
         <oasis:entry colname="col7">Ocean</oasis:entry>
         <oasis:entry colname="col8">Land</oasis:entry>
         <oasis:entry colname="col9"/>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2006<inline-formula><mml:math id="M1959" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">Split in regions</oasis:entry>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2007<inline-formula><mml:math id="M1960" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1961" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> based on FAO-FRA 2005; constant<?xmltex \hack{\hfill\break}?> <inline-formula><mml:math id="M1962" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for 2006</oasis:entry>
         <oasis:entry colname="col6">1959–1979 data from Mauna Loa; data after 1980 from global average</oasis:entry>
         <oasis:entry colname="col7">Based on one ocean model tuned to reproduced observed 1990s sink</oasis:entry>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"><inline-formula><mml:math id="M1963" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M1964" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> provided for all components</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2008<inline-formula><mml:math id="M1965" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5">Constant <inline-formula><mml:math id="M1966" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for<?xmltex \hack{\hfill\break}?>2007</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2009<inline-formula><mml:math id="M1967" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">Split between Annex B and non-Annex B</oasis:entry>
         <oasis:entry colname="col4">Results from an independent study discussed</oasis:entry>
         <oasis:entry colname="col5">Fire-based emission anomalies used for<?xmltex \hack{\hfill\break}?>2006–2008</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">Based on four ocean models normalized<?xmltex \hack{\hfill\break}?>to observations with constant delta</oasis:entry>
         <oasis:entry colname="col8">First use of five <?xmltex \hack{\hfill\break}?>DGVMs to compare with budget residual</oasis:entry>
         <oasis:entry colname="col9"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2010<inline-formula><mml:math id="M1968" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">e</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Projection for current year based on GDP</oasis:entry>
         <oasis:entry colname="col3">Emissions for top<?xmltex \hack{\hfill\break}?>emitters</oasis:entry>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1969" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> updated with FAO-FRA 2010</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2011<inline-formula><mml:math id="M1970" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">f</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">Split between Annex B and non-Annex B</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7"/>
         <oasis:entry colname="col8"/>
         <oasis:entry colname="col9"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2012<inline-formula><mml:math id="M1971" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">g</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">129 countries from <?xmltex \hack{\hfill\break}?>1959</oasis:entry>
         <oasis:entry colname="col4">129 countries and<?xmltex \hack{\hfill\break}?>regions from 1990–2010 based on<?xmltex \hack{\hfill\break}?>GTAP8.0</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1972" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for 1997–2011 includes interannual anomalies from fire-based emissions</oasis:entry>
         <oasis:entry colname="col6">All years from global average</oasis:entry>
         <oasis:entry colname="col7">Based on 5 ocean<?xmltex \hack{\hfill\break}?>models normalized to observations with <?xmltex \hack{\hfill\break}?>ratio</oasis:entry>
         <oasis:entry colname="col8">10 DGVMs available for <inline-formula><mml:math id="M1973" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>; First use of four models to compare with <inline-formula><mml:math id="M1974" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9"/>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2013<inline-formula><mml:math id="M1975" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">h</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">250 countries</oasis:entry>
         <oasis:entry colname="col4">134 countries and regions 1990–2011 based on GTAP8.1, with detailed estimates for years 1997, 2001, 2004, and 2007</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1976" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for 2012 estimated from 2001–2010 average</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">Based on six models compared with two data products to year 2011</oasis:entry>
         <oasis:entry colname="col8">Coordinated DGVM experiments for<?xmltex \hack{\hfill\break}?> <inline-formula><mml:math id="M1977" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M1978" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col9">Confidence levels; <?xmltex \hack{\hfill\break}?>cumulative emissions; budget from 1750</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2014<inline-formula><mml:math id="M1979" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">i</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">3 years of BP <?xmltex \hack{\hfill\break}?>data</oasis:entry>
         <oasis:entry colname="col3">3 years of BP <?xmltex \hack{\hfill\break}?>data</oasis:entry>
         <oasis:entry colname="col4">Extended to 2012<?xmltex \hack{\hfill\break}?>with updated GDP data</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1980" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for 1997–2013 includes interannual anomalies from fire-based emissions</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">Based on seven<?xmltex \hack{\hfill\break}?>models</oasis:entry>
         <oasis:entry colname="col8">Based on 10 models</oasis:entry>
         <oasis:entry colname="col9">Inclusion of breakdown of the sinks in three latitude bands and comparison with three atmospheric inversions</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">2015<inline-formula><mml:math id="M1981" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Projection for current year based January–August data</oasis:entry>
         <oasis:entry colname="col3">National emissions<?xmltex \hack{\hfill\break}?>from UNFCCC extended to 2014 also provided</oasis:entry>
         <oasis:entry colname="col4">Detailed estimates<?xmltex \hack{\hfill\break}?>introduced for 2011 based on GTAP9</oasis:entry>
         <oasis:entry colname="col5"/>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">Based on eight<?xmltex \hack{\hfill\break}?>models</oasis:entry>
         <oasis:entry colname="col8">Based on 10 models with assessment of minimum realism</oasis:entry>
         <oasis:entry colname="col9">The decadal uncertainty for the DGVM ensemble mean now uses <inline-formula><mml:math id="M1982" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M1983" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> of the decadal spread across models</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">2016<inline-formula><mml:math id="M1984" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">k</mml:mi></mml:msup></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">2 years of BP data</oasis:entry>
         <oasis:entry colname="col3">Added three small countries; China's emissions from 1990 from BP data (this release only)</oasis:entry>
         <oasis:entry colname="col4"/>
         <oasis:entry colname="col5">Preliminary <inline-formula><mml:math id="M1985" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula><?xmltex \hack{\hfill\break}?>using FRA-2015<?xmltex \hack{\hfill\break}?>shown for comparison; use of five <?xmltex \hack{\hfill\break}?>DGVMs</oasis:entry>
         <oasis:entry colname="col6"/>
         <oasis:entry colname="col7">Based on seven<?xmltex \hack{\hfill\break}?>models</oasis:entry>
         <oasis:entry colname="col8">Based on 14 <?xmltex \hack{\hfill\break}?>models</oasis:entry>
         <oasis:entry colname="col9">Discussion of projection for full budget for current year</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table><table-wrap-foot><p id="d1e29809"><inline-formula><mml:math id="M1948" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">a</mml:mi></mml:msup></mml:math></inline-formula> Raupach et al. (2007). <inline-formula><mml:math id="M1949" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">b</mml:mi></mml:msup></mml:math></inline-formula> Canadell et al. (2007). <inline-formula><mml:math id="M1950" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">c</mml:mi></mml:msup></mml:math></inline-formula> GCP (2007). <inline-formula><mml:math id="M1951" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">d</mml:mi></mml:msup></mml:math></inline-formula> Le Quéré et al. (2009). <inline-formula><mml:math id="M1952" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">e</mml:mi></mml:msup></mml:math></inline-formula> Friedlingstein et al. (2010). <inline-formula><mml:math id="M1953" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">f</mml:mi></mml:msup></mml:math></inline-formula> Peters et al. (2012b). <inline-formula><mml:math id="M1954" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">g</mml:mi></mml:msup></mml:math></inline-formula> Le Quéré et al. (2013), Peters et al. (2013). <inline-formula><mml:math id="M1955" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">h</mml:mi></mml:msup></mml:math></inline-formula> Le Quéré et al. (2014).<?xmltex \hack{\break}?> <inline-formula><mml:math id="M1956" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">i</mml:mi></mml:msup></mml:math></inline-formula> Le Quéré et al. (2015a). <inline-formula><mml:math id="M1957" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">j</mml:mi></mml:msup></mml:math></inline-formula> Le Quéré et al. (2015b) <inline-formula><mml:math id="M1958" display="inline"><mml:msup><mml:mi/><mml:mi mathvariant="normal">k</mml:mi></mml:msup></mml:math></inline-formula> Le Quéré et al. (2016)</p></table-wrap-foot></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{t}?><table-wrap id="App1.Ch1.S1.T21" specific-use="star"><?xmltex \currentcnt{A8}?><label>Table A8</label><caption><p id="d1e30585">Mapping of global carbon cycle models' land flux definitions to the definition of the LULUCF net flux used in national reporting to UNFCCC. Non-intact lands are used here as proxy for “managed lands” in the country reporting.</p></caption><oasis:table frame="topbot"><oasis:tgroup cols="5">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="4cm"/>
     <oasis:colspec colnum="2" colname="col2" align="justify" colwidth="4cm"/>
     <oasis:colspec colnum="3" colname="col3" align="justify" colwidth="4cm"/>
     <oasis:colspec colnum="4" colname="col4" align="right"/>
     <oasis:colspec colnum="5" colname="col5" align="right"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">2001–2010</oasis:entry>
         <oasis:entry colname="col5">2011–2020</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"><inline-formula><mml:math id="M1986" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from bookkeeping <?xmltex \hack{\hfill\break}?>estimates (from Table 5)</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">1.21</oasis:entry>
         <oasis:entry colname="col5">1.13</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M1987" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2">Total (from Table 5)</oasis:entry>
         <oasis:entry colname="col3">from DGVMs</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M1988" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>2.54</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1989" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>3.06</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">on non-forest lands</oasis:entry>
         <oasis:entry colname="col3">from DGVMs</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M1990" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.90</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1991" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.14</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">on non-intact forest</oasis:entry>
         <oasis:entry colname="col3">from DGVMs</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M1992" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.27</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1993" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.50</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2">on intact land (intact forest only for DGVMs)</oasis:entry>
         <oasis:entry colname="col3">from DGVMs</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M1994" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.37</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1995" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.42</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">from ORCHIDEE-MICT</oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M1996" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.29</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M1997" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>1.47</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1"><inline-formula><mml:math id="M1998" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> on non-intact lands<?xmltex \hack{\hfill\break}?>plus <inline-formula><mml:math id="M1999" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">from DGVMs and bookkeeping <inline-formula><mml:math id="M2000" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></oasis:entry>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M2001" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.06</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M2002" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.37</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1"/>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3">from ORCHIDEE-MICT</oasis:entry>
         <oasis:entry colname="col4">1.00</oasis:entry>
         <oasis:entry colname="col5">0.61</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">National greenhouse gas<?xmltex \hack{\hfill\break}?>inventories (LULUCF)</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4"><inline-formula><mml:math id="M2003" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.43</oasis:entry>
         <oasis:entry colname="col5"><inline-formula><mml:math id="M2004" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.57</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">FAOSTAT (LULUCF)</oasis:entry>
         <oasis:entry colname="col2"/>
         <oasis:entry colname="col3"/>
         <oasis:entry colname="col4">0.39</oasis:entry>
         <oasis:entry colname="col5">0.20</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{t}?><table-wrap id="App1.Ch1.S1.T22" specific-use="star"><?xmltex \currentcnt{A9}?><label>Table A9</label><caption><p id="d1e30936">Funding supporting the production of the various components of the global carbon budget in addition to the authors' supporting institutions (see also the Acknowledgements).</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.9}[.9]?><oasis:tgroup cols="2">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="12cm"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Funder and grant number (where relevant)</oasis:entry>
         <oasis:entry colname="col2">Author initials</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">Australia, Integrated Marine Observing System (IMOS)</oasis:entry>
         <oasis:entry colname="col2">BT</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Australian National Environment Science Program (NESP)</oasis:entry>
         <oasis:entry colname="col2">JGC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Belgium, FWO (Flanders Research Foundation, contract IRI I001019N)</oasis:entry>
         <oasis:entry colname="col2">TG</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">BNP Paribas Foundation through Climate &amp; Biodiversity initiative, philanthropic grant for developments of the Global Carbon Atlas</oasis:entry>
         <oasis:entry colname="col2">PC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Canada, Tula Foundation</oasis:entry>
         <oasis:entry colname="col2">WE</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">China, National Natural Science Foundation (grant no. 41975155)</oasis:entry>
         <oasis:entry colname="col2">XY</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Commonwealth Scientific and Industrial Organization (CSIRO) – Climate Science Centre</oasis:entry>
         <oasis:entry colname="col2">JGC, JK</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC Copernicus Atmosphere Monitoring Service implemented by ECMWF on behalf of the European Commission</oasis:entry>
         <oasis:entry colname="col2">FC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC Copernicus Marine Environment Monitoring Service implemented by Mercator Ocean</oasis:entry>
         <oasis:entry colname="col2">TTTC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (4C; grant no. 821003)</oasis:entry>
         <oasis:entry colname="col2">PF, RMA, SS, GPP, PC, JIK, TI, LB, PL, LG, SL, NG</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (CHE; grant no. 776186)</oasis:entry>
         <oasis:entry colname="col2">MWJ</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (CoCO<inline-formula><mml:math id="M2005" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>: grant no. 958927)</oasis:entry>
         <oasis:entry colname="col2">RMA, GPP</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (COMFORT: grant no. 820989)</oasis:entry>
         <oasis:entry colname="col2">DCEB, LG</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (CONSTRAIN: grant no. 820829)</oasis:entry>
         <oasis:entry colname="col2">RS, PMF, TG</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (CRESCENDO: grant no. 641816)</oasis:entry>
         <oasis:entry colname="col2">RS, EJ AJPS, TI</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (ESM2025 – Earth System Models for the Future; grant agreement no. 101003536).</oasis:entry>
         <oasis:entry colname="col2">RS, TG, TI, LB, BD</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (EuroSea: grant no. 862626)</oasis:entry>
         <oasis:entry colname="col2">SDJ</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (JERICO-S3: grant no. 871153)</oasis:entry>
         <oasis:entry colname="col2">GR</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (QUINCY; grant no. 647204)</oasis:entry>
         <oasis:entry colname="col2">SZ</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (RINGO: grant no. 730944)</oasis:entry>
         <oasis:entry colname="col2">DCEB</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EC H2020 (VERIFY: grant no. 776810)</oasis:entry>
         <oasis:entry colname="col2">MWJ, RMA, GPP, PC, JIK, NV, GG</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">EFG International</oasis:entry>
         <oasis:entry colname="col2">TT</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">European Space Agency Climate Change Initiative ESA-CCI RECCAP2 project 655 (ESRIN/4000123002/18/I-NB)</oasis:entry>
         <oasis:entry colname="col2">PF, SS, PC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">European Space Agency OceanSODA project (grant no. 4000112091/14/I-LG)</oasis:entry>
         <oasis:entry colname="col2">LG</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">France, ICOS (Integrated Carbon Observation System) France</oasis:entry>
         <oasis:entry colname="col2">NL</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">France, Institut de Recherche pour le Développement (IRD)</oasis:entry>
         <oasis:entry colname="col2">NL</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Germany, Blue Ocean and Federal Ministry of Education (BONUS INTEGRAL; grant no. 03F0773A)</oasis:entry>
         <oasis:entry colname="col2">GR</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Germany, Deutsche Forschungsgemeinschaft (DFG) under Germany's Excellence Strategy – EXC 2037 “Climate, Climatic Change, and Society” – project number: 390683824</oasis:entry>
         <oasis:entry colname="col2">TI</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Germany, Federal Ministry for Education and Research (BMBF)</oasis:entry>
         <oasis:entry colname="col2">GR</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Germany, GEOMAR Helmholtz Centre for Ocean Research</oasis:entry>
         <oasis:entry colname="col2">SKL</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Germany, German Federal Ministry of Education and Research under project “DArgo2025” (03F0857C)</oasis:entry>
         <oasis:entry colname="col2">AK</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Germany, Helmholtz Association ATMO programme</oasis:entry>
         <oasis:entry colname="col2">PA</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Germany, Helmholtz Young Investigator Group Marine Carbon and Ecosystem Feedbacks in the Earth System (MarESys), grant number VH-NG-1301</oasis:entry>
         <oasis:entry colname="col2">JH, OG</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Germany, ICOS (Integrated Carbon Observation System) Germany</oasis:entry>
         <oasis:entry colname="col2">GR, NL</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Hapag-Lloyd</oasis:entry>
         <oasis:entry colname="col2">TT</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Ireland, Marine Institute</oasis:entry>
         <oasis:entry colname="col2">MC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Japan, Environment Research and Technology Development Fund of the Ministry of the Environment (JPMEERF21S20810)</oasis:entry>
         <oasis:entry colname="col2">YN</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Japan, Global Environmental Research Coordination System, Ministry of the Environment (grant number E1751)</oasis:entry>
         <oasis:entry colname="col2">SN, TO, CW</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Kuehne <inline-formula><mml:math id="M2006" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> Nagel International AG</oasis:entry>
         <oasis:entry colname="col2">TT</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Mediterranean Shipping Company (MSc)</oasis:entry>
         <oasis:entry colname="col2">TT</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Monaco, Fondation Prince Albert II de Monaco</oasis:entry>
         <oasis:entry colname="col2">TT</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Monaco, Yacht Club de Monaco</oasis:entry>
         <oasis:entry colname="col2">TT</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">NASA Interdisciplinary Research in Earth Science Program.</oasis:entry>
         <oasis:entry colname="col2">BP</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Netherlands Organization for Scientific Research (NWO; grant no. SH-312, 17616)</oasis:entry>
         <oasis:entry colname="col2">WP</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">New Zealand, NIWA MBIE Core funding</oasis:entry>
         <oasis:entry colname="col2">KIC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Norway, Norwegian Research Council (grant no. 270061)</oasis:entry>
         <oasis:entry colname="col2">JS</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Norway, Research Council of Norway, ICOS (Integrated Carbon Observation System) Norway and OTC (Ocean Thematic Centre) (grant no. 245927)</oasis:entry>
         <oasis:entry colname="col2">SKL, MB, SDJ</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">PEAK6 Investments</oasis:entry>
         <oasis:entry colname="col2">SKL</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Saildrone Inc.</oasis:entry>
         <oasis:entry colname="col2">SKL</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{t}?><table-wrap id="App1.Ch1.S1.T23" specific-use="star"><?xmltex \currentcnt{A9}?><label>Table A9</label><caption><p id="d1e31432">Continued.</p></caption><oasis:table frame="topbot"><?xmltex \begin{scaleboxenv}{.9}[.9]?><oasis:tgroup cols="2">
     <oasis:colspec colnum="1" colname="col1" align="justify" colwidth="13cm"/>
     <oasis:colspec colnum="2" colname="col2" align="left"/>
     <oasis:thead>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">Funder and grant number (where relevant)</oasis:entry>
         <oasis:entry colname="col2">Author initials</oasis:entry>
       </oasis:row>
     </oasis:thead>
     <oasis:tbody>
       <oasis:row>
         <oasis:entry colname="col1">South Africa, Department of Science and Innovation</oasis:entry>
         <oasis:entry colname="col2">LD</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">South Africa, National Science Foundation</oasis:entry>
         <oasis:entry colname="col2">LD</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Swiss National Science Foundation (grant no. 200020_172476)</oasis:entry>
         <oasis:entry colname="col2">SL</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UK Royal Society (grant no. RP<inline-formula><mml:math id="M2007" display="inline"><mml:mo>\</mml:mo></mml:math></inline-formula>R1<inline-formula><mml:math id="M2008" display="inline"><mml:mo>\</mml:mo></mml:math></inline-formula>191063)</oasis:entry>
         <oasis:entry colname="col2">CLQ</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UK, CLASS ERC funding</oasis:entry>
         <oasis:entry colname="col2">TG</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UK, National Centre for Atmospheric Science (NCAS)</oasis:entry>
         <oasis:entry colname="col2">PCM</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UK, Natural Environment Research Council (SONATA: grant no. NE/P021417/1)</oasis:entry>
         <oasis:entry colname="col2">DW</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UK, Natural Environmental Research Council (NE/R016518/1)</oasis:entry>
         <oasis:entry colname="col2">LF</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UK, Newton Fund, Met Office Climate Science for Service Partnership Brazil (CSSP Brazil)</oasis:entry>
         <oasis:entry colname="col2">AJWi</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UK, Royal Society: The European Space Agency OCEANFLUX projects</oasis:entry>
         <oasis:entry colname="col2">AJWa</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UK, University of Reading Research Endowment Trust Fund</oasis:entry>
         <oasis:entry colname="col2">PCM</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">USA, Department of Commerce, Office of Oceanic and Atmospheric Research (OAR)'s / National Oceanic and Atmospheric Administration (NOAA)'s Global Ocean Monitoring and Observation Program (GOMO)</oasis:entry>
         <oasis:entry colname="col2">DRM, CS, DP, RW, SRA, RAF, AJS, NRB</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">USA, Department of Commerce, Office of Oceanic and Atmospheric Research (OAR)'s / National Oceanic and Atmospheric Administration (NOAA)'s Ocean Acidification Program</oasis:entry>
         <oasis:entry colname="col2">DP, RW, SRA, RAF, AJS</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">USA, Department of Energy, Office of Science and BER prg. (grant no. DE-SC000 0016323)</oasis:entry>
         <oasis:entry colname="col2">AKJ</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">USA, Department of Energy, SciDac (DESC0012972)</oasis:entry>
         <oasis:entry colname="col2">GCH, LPC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">USA, NASA Carbon Monitoring System programme and OCO Science team programme (80NM0018F0583).</oasis:entry>
         <oasis:entry colname="col2">JL</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">USA, NASA Interdisciplinary Research in Earth Science (IDS) (80NSSC17K0348)</oasis:entry>
         <oasis:entry colname="col2">GCH, LPC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">USA, National Science Foundation (grant number 1903722)</oasis:entry>
         <oasis:entry colname="col2">HT</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">USA, National Science Foundation (grant number PLR 1543457)</oasis:entry>
         <oasis:entry colname="col2">DRM, CS</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry colname="col1">USA, Princeton University Environmental Institute and the NASA OCO<inline-formula><mml:math id="M2009" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> science team, grant number 80NSSC18K0893.</oasis:entry>
         <oasis:entry colname="col2">LR</oasis:entry>
       </oasis:row>
       <oasis:row rowsep="1">
         <oasis:entry namest="col1" nameend="col2" align="left">Computing resources </oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">bwHPC, High Performance Computing Network of the State of Baden-Württemberg, Germany</oasis:entry>
         <oasis:entry colname="col2">PA</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Cheyenne supercomputer, Computational and Information Systems Laboratory (CISL) at National Center for Atmospheric Research (NCAR)</oasis:entry>
         <oasis:entry colname="col2">DK</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Deutsches Klimarechenzentrum (allocation bm0891)</oasis:entry>
         <oasis:entry colname="col2">JEMSN, JP</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">HPC cluster Aether at the University of Bremen, financed by DFG within the scope of the Excellence Initiative</oasis:entry>
         <oasis:entry colname="col2">ITL, WP</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">MRI (FUJITSU Server PRIMERGY CX2550M5)</oasis:entry>
         <oasis:entry colname="col2">YN</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">NIES (SX-Aurora)</oasis:entry>
         <oasis:entry colname="col2">YN</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">NIES supercomputer system</oasis:entry>
         <oasis:entry colname="col2">EK</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Supercomputer “Gadi” of the National Computational Infrastructure (NCI), Australia</oasis:entry>
         <oasis:entry colname="col2">JK</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">Supercomputing time was provided by the Météo-France/DSI supercomputing centre.</oasis:entry>
         <oasis:entry colname="col2">RS, BD</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">TGCC under allocation 2019-A0070102201 made by GENCI</oasis:entry>
         <oasis:entry colname="col2">FC</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UEA High Performance Computing Cluster, UK</oasis:entry>
         <oasis:entry colname="col2">MWJ, CLQ, DRW</oasis:entry>
       </oasis:row>
       <oasis:row>
         <oasis:entry colname="col1">UNINETT Sigma2, National Infrastructure for High Performance Computing and Data Storage in Norway (NN2980K/NS2980K)</oasis:entry>
         <oasis:entry colname="col2">JS</oasis:entry>
       </oasis:row>
     </oasis:tbody>
   </oasis:tgroup><?xmltex \end{scaleboxenv}?></oasis:table></table-wrap>

<?xmltex \hack{\clearpage}?>
</app>

<app id="App1.Ch1.S2">
  <?xmltex \currentcnt{B}?><label>Appendix B</label><title>Supplementary figures</title>

      <?xmltex \floatpos{h!}?><fig id="App1.Ch1.S2.F15"><?xmltex \currentcnt{B1}?><?xmltex \def\figurename{Figure}?><label>Figure B1</label><caption><p id="d1e31793">Ensemble mean air–sea CO<inline-formula><mml:math id="M2010" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux from <bold>(a)</bold> global ocean
biogeochemistry models and <bold>(b)</bold> <inline-formula><mml:math id="M2011" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2012" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products, averaged over
2011–2020 period (kgC m<inline-formula><mml:math id="M2013" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> yr<inline-formula><mml:math id="M2014" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>). Positive numbers indicate a flux
into the ocean. <bold>(c)</bold> Gridded SOCAT v2021 <inline-formula><mml:math id="M2015" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2016" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements, averaged over
the 2011–2020 period (<inline-formula><mml:math id="M2017" display="inline"><mml:mrow class="unit"><mml:mi mathvariant="normal">µ</mml:mi></mml:mrow></mml:math></inline-formula>atm). In <bold>(a)</bold> model simulation A is shown. The
data products represent the contemporary flux, i.e. including outgassing of
riverine carbon, which is estimated to amount to 0.615 GtC yr<inline-formula><mml:math id="M2018" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p></caption>
        <?xmltex \hack{\hsize\textwidth}?>
        <?xmltex \igopts{width=298.753937pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f15.png"/>

      </fig>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{h!}?><fig id="App1.Ch1.S2.F16"><?xmltex \currentcnt{B2}?><?xmltex \def\figurename{Figure}?><label>Figure B2</label><caption><p id="d1e31906">Evaluation of the GOBMs and data products using the root
mean squared error (RMSE) for the period 1990 to 2020, between the
individual surface ocean <inline-formula><mml:math id="M2019" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2020" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> mapping schemes and the SOCAT v2021
database. The <inline-formula><mml:math id="M2021" display="inline"><mml:mi>y</mml:mi></mml:math></inline-formula> axis shows the amplitude of the interannual variability
(A-IAV, taken as the standard deviation of a detrended time series
calculated as a 12-month running mean over the monthly flux time series,
Rödenbeck et al., 2015). Results are presented for the globe, north
(<inline-formula><mml:math id="M2022" display="inline"><mml:mo lspace="0mm">&gt;</mml:mo></mml:math></inline-formula> 30<inline-formula><mml:math id="M2023" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N), tropics (30<inline-formula><mml:math id="M2024" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S–30<inline-formula><mml:math id="M2025" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N),
and south (<inline-formula><mml:math id="M2026" display="inline"><mml:mo lspace="0mm">&lt;</mml:mo></mml:math></inline-formula> 30<inline-formula><mml:math id="M2027" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> S) for the GOBMs (see legend circles) and
for the <inline-formula><mml:math id="M2028" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2029" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products (star symbols). The <inline-formula><mml:math id="M2030" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2031" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based
data products use the SOCAT database and therefore are not independent from
the data (see Sect. 2.4.1).</p></caption>
        <?xmltex \hack{\hsize\textwidth}?>
        <?xmltex \igopts{width=369.885827pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f16.png"/>

      </fig>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{h!}?><fig id="App1.Ch1.S2.F17"><?xmltex \currentcnt{B3}?><?xmltex \def\figurename{Figure}?><label>Figure B3</label><caption><p id="d1e32028">Evaluation of the DGVMs using the International Land
Model Benchmarking system (ILAMB; Collier et al., 2018) <bold>(a)</bold> absolute
skill scores and <bold>(b)</bold> skill scores relative to other models. The
benchmarking is done with observations for vegetation biomass (Saatchi et
al., 2011; and GlobalCarbon unpublished data; Avitabile et al., 2016), GPP
(Jung et al., 2010; Lasslop et al., 2010), leaf area index (De Kauwe et al.,
2011; Myneni et al., 1997), net ecosystem exchange (Jung et al.,
2010; Lasslop et al., 2010), ecosystem respiration (Jung et al., 2010; Lasslop
et al., 2010), soil carbon (Hugelius et al., 2013; Todd-Brown et al., 2013),
evapotranspiration (De Kauwe et al., 2011), and runoff (Dai and Trenberth,
2002). For each model–observation comparison a series of error metrics are
calculated, scores are then calculated as an exponential function of each
error metric, and finally for each variable the multiple scores from different
metrics and observational datasets are combined to give the overall
variable scores shown in <bold>(a)</bold>. Overall variable scores increase
from 0 to 1 with improvements in model performance. The set of error metrics
vary with dataset and can include metrics based on the period mean, bias,
root mean squared error, spatial distribution, interannual variability, and
seasonal cycle. The relative skill score shown in <bold>(b)</bold> is a
<inline-formula><mml:math id="M2032" display="inline"><mml:mi>Z</mml:mi></mml:math></inline-formula> score, which indicates in units of standard deviation the model scores
relative to the multi-model mean score for a given variable. Grey boxes
represent missing model data.</p></caption>
        <?xmltex \hack{\hsize\textwidth}?>
        <?xmltex \igopts{width=412.564961pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f17.png"/>

      </fig>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{h!}?><fig id="App1.Ch1.S2.F18"><?xmltex \currentcnt{B4}?><?xmltex \def\figurename{Figure}?><label>Figure B4</label><caption><p id="d1e32061">Evaluation of the atmospheric inversion products. The
mean of the model minus observations is shown for four latitude bands in
three periods: <bold>(a)</bold> 2001–2010, <bold>(b)</bold> 2011–2020, <bold>(c)</bold> 2001–2020. The
six models are compared to independent CO<inline-formula><mml:math id="M2033" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements made onboard
aircraft over many places of the world between 2 and 7 km above sea level.
Aircraft measurements archived in the Cooperative Global Atmospheric Data
Integration Project (CGADIP; Cox et al., 2021) from sites, campaigns, or
programmes that cover at least 9 months between 2001 and 2020 and that have
not been assimilated have been used to compute the biases of the
differences in four 45<inline-formula><mml:math id="M2034" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> latitude bins. Land and ocean data are
used without distinction, and observation density varies strongly with
latitude and time as seen in the lower panels.</p></caption>
        <?xmltex \hack{\hsize\textwidth}?>
        <?xmltex \igopts{width=412.564961pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f18.png"/>

      </fig>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{h!}?><fig id="App1.Ch1.S2.F19"><?xmltex \currentcnt{B5}?><?xmltex \def\figurename{Figure}?><label>Figure B5</label><caption><p id="d1e32102">Comparison of the estimates of each component of the
global carbon budget in this study (black line) with the estimates released
annually by the GCP since 2006. Grey shading shows the uncertainty bounds
representing <inline-formula><mml:math id="M2035" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1 standard deviation of the current global carbon
budget, based on the uncertainty assessments described in Appendix C.
CO<inline-formula><mml:math id="M2036" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from <bold>(a)</bold> fossil CO<inline-formula><mml:math id="M2037" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions (<inline-formula><mml:math id="M2038" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) and <bold>(b)</bold> land-use change (<inline-formula><mml:math id="M2039" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), as well as their partitioning among <bold>(c)</bold> the
atmosphere (<inline-formula><mml:math id="M2040" display="inline"><mml:mrow><mml:msub><mml:mi>G</mml:mi><mml:mi mathvariant="normal">ATM</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), <bold>(d)</bold> the land (<inline-formula><mml:math id="M2041" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>), and <bold>(e)</bold> the ocean
(<inline-formula><mml:math id="M2042" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). See legend for the corresponding years, and Tables 3 and A7
for references. The budget year corresponds to the year when the budget was
first released. All values are in GtC yr<inline-formula><mml:math id="M2043" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p></caption>
        <?xmltex \hack{\hsize\textwidth}?>
        <?xmltex \igopts{width=384.112205pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f19.png"/>

      </fig>

<?xmltex \hack{\clearpage}?><?xmltex \floatpos{h!}?><fig id="App1.Ch1.S2.F20"><?xmltex \currentcnt{B6}?><?xmltex \def\figurename{Figure}?><label>Figure B6</label><caption><p id="d1e32226">Changes in the HYDE/LUH2 land-use forcing from last
year's global carbon budget (Friedlingstein et al., 2020, in blue) to this
year (orange). Shown are year-to-year changes in cropland area <bold>(b)</bold> and pasture area <bold>(c)</bold>. To illustrate the relevance of the
update in the land-use forcing to the recent trends in <inline-formula><mml:math id="M2044" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, <bold>(a)</bold> shows the land-use emission estimate from the bookkeeping model BLUE
(original model output, i.e. excluding peat fire and drainage emissions).</p></caption>
        <?xmltex \hack{\hsize\textwidth}?>
        <?xmltex \igopts{width=355.659449pt}?><graphic xlink:href="https://essd.copernicus.org/articles/14/1917/2022/essd-14-1917-2022-f20.png"/>

      </fig>

<?xmltex \hack{\clearpage}?>
</app>

<app id="App1.Ch1.S3">
  <?xmltex \currentcnt{C}?><label>Appendix C</label><title>Extended methodology</title>
<sec id="App1.Ch1.S3.SS1">
  <label>C1</label><?xmltex \opttitle{Methodology fossil fuel CO${}_{{{2}}}$ emissions
($E_{{\mathrm{FOS}}}$)}?><title>Methodology fossil fuel CO<inline-formula><mml:math id="M2045" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
(<inline-formula><mml:math id="M2046" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</title>
<sec id="App1.Ch1.S3.SS1.SSS1">
  <label>C1.1</label><title>Cement carbonation</title>
      <p id="d1e32302">From the moment it is created, cement begins to absorb CO<inline-formula><mml:math id="M2047" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> from the
atmosphere, a process known as “cement carbonation”. We estimate this
CO<inline-formula><mml:math id="M2048" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink, as the average of two studies in the literature (Cao et al.,
2020; Guo et al., 2021). Both studies use the same model, developed by Xi et
al. (2016), with different parameterizations and input data, with the
estimate of Guo and colleagues being a revision of Xi et al. (2016). The
trends of the two studies are very similar. Modelling cement carbonation
requires estimation of a large number of parameters, including the different
types of cement material in different countries, the lifetime of the
structures before demolition, of cement waste after demolition, and the
volumetric properties of structures, among others (Xi et al., 2016).
Lifetime is an important parameter because demolition results in the
exposure of new surfaces to the carbonation process. The main reasons for
differences between the two studies appear to be the assumed lifetimes of
cement structures and the geographic resolution, but the uncertainty bounds
of the two studies overlap. In the present budget, we include the cement
carbonation carbon sink in the fossil CO<inline-formula><mml:math id="M2049" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emission component
(<inline-formula><mml:math id="M2050" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>).</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSS2">
  <label>C1.2</label><title>Emissions embodied in goods and services</title>
      <p id="d1e32351">CDIAC, UNFCCC, and BP national emission statistics “include greenhouse gas
emissions and removals taking place within national territory and offshore
areas over which the country has jurisdiction” (Rypdal et al., 2006) and
are called territorial emission inventories. Consumption-based emission
inventories allocate emissions to products that are consumed within a
country and are conceptually calculated as the territorial emissions minus
the “embodied” territorial emissions to produce exported products plus the
emissions in other countries to produce imported products (consumption <inline-formula><mml:math id="M2051" display="inline"><mml:mo>=</mml:mo></mml:math></inline-formula>
territorial – exports <inline-formula><mml:math id="M2052" display="inline"><mml:mo>+</mml:mo></mml:math></inline-formula> imports). Consumption-based emission attribution
results (e.g. Davis and Caldeira, 2010) provide additional information to
territorial-based emissions that can be used to understand emission drivers
(Hertwich and Peters, 2009) and quantify emission transfers by the trade of
products between countries (Peters et al., 2011b). The consumption-based
emissions have the same global total but reflect the trade-driven movement
of emissions across the Earth's surface in response to human activities. We
estimate consumption-based emissions from 1990–2018 by enumerating the
global supply chain using a global model of the economic relationships
between economic sectors within and between every country (Andrew and
Peters, 2013; Peters et al., 2011a). Our analysis is based on the economic
and trade data from the Global Trade and Analysis Project (GTAP; Narayanan
et al., 2015), and we make detailed estimates for the years 1997 (GTAP
version 5), 2001 (GTAP6), 2004, 2007, and 2011 (GTAP9.2), covering 57
sectors and 141 countries and regions. The detailed results are then
extended into an annual time series from 1990 to the latest year of the
gross domestic product (GDP) data (2018 in this budget), using GDP data by
expenditure in the current exchange rate of US dollars (USD; from the UN
National Accounts Main Aggregrates Database; UN, 2021) and time series of
trade data from GTAP (based on the methodology in Peters et al., 2011a). We
estimate the sector-level CO<inline-formula><mml:math id="M2053" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions using the GTAP data and
methodology, include the flaring and cement emissions from CDIAC, and then
scale the national totals (excluding bunker fuels) to match the emission
estimates from the carbon budget. We do not provide a separate uncertainty
estimate for the consumption-based emissions, but based on model comparisons
and sensitivity analysis, they are unlikely to be significantly different
than for the territorial emission estimates (Peters et al., 2012a).</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSS3">
  <label>C1.3</label><?xmltex \opttitle{Uncertainty assessment for $E_{{\mathrm{FOS}}}$}?><title>Uncertainty assessment for <inline-formula><mml:math id="M2054" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></title>
      <p id="d1e32396">We estimate the uncertainty of the global fossil CO<inline-formula><mml:math id="M2055" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions at <inline-formula><mml:math id="M2056" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>5 % (scaled down from the published <inline-formula><mml:math id="M2057" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>10 % at <inline-formula><mml:math id="M2058" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>2<inline-formula><mml:math id="M2059" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>
to the use of <inline-formula><mml:math id="M2060" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M2061" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> bounds reported here; Andres et al., 2012).
This is consistent with a more detailed analysis of uncertainty of <inline-formula><mml:math id="M2062" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>8.4 % at <inline-formula><mml:math id="M2063" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>2<inline-formula><mml:math id="M2064" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> (Andres et al., 2014) and at the high-end of
the range of <inline-formula><mml:math id="M2065" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>5 %–10 % at <inline-formula><mml:math id="M2066" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>2<inline-formula><mml:math id="M2067" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> reported by Ballantyne
et al. (2015). This includes an assessment of uncertainties in the amounts
of fuel consumed, the carbon and heat contents of fuels, and the combustion
efficiency. While we consider a fixed uncertainty of <inline-formula><mml:math id="M2068" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>5 % for all
years, the uncertainty as a percentage of emissions is growing with time
because of the larger share of global emissions from emerging economies and
developing countries (Marland et al., 2009). Generally, emissions from
mature economies with good statistical processes have an uncertainty of only
a few per cent (Marland, 2008), while emissions from strongly developing
economies such as China have uncertainties of around <inline-formula><mml:math id="M2069" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>10 % (for
<inline-formula><mml:math id="M2070" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M2071" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>; Gregg et al., 2008; Andres et al., 2014). Uncertainties
of emissions are likely to be mainly systematic errors related to underlying
biases of energy statistics and to the accounting method used by each
country.</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSS4">
  <label>C1.4</label><title>Growth rate in emissions</title>
      <p id="d1e32531">We report the annual growth rate in emissions for adjacent years (in percent
per year) by calculating the difference between the two years and then
normalizing to the emissions in the first year:
(<inline-formula><mml:math id="M2072" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>(<inline-formula><mml:math id="M2073" display="inline"><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:math></inline-formula>) <inline-formula><mml:math id="M2074" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M2075" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>(<inline-formula><mml:math id="M2076" display="inline"><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>))<inline-formula><mml:math id="M2077" display="inline"><mml:mrow><mml:mo>/</mml:mo><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>(<inline-formula><mml:math id="M2078" display="inline"><mml:mrow><mml:msub><mml:mi>t</mml:mi><mml:mn mathvariant="normal">0</mml:mn></mml:msub></mml:mrow></mml:math></inline-formula>) <inline-formula><mml:math id="M2079" display="inline"><mml:mrow><mml:mo>×</mml:mo><mml:mn mathvariant="normal">100</mml:mn></mml:mrow></mml:math></inline-formula> %. We apply a leap-year
adjustment where relevant to ensure valid interpretations of annual growth
rates. This affects the growth rate by about 0.3 % yr<inline-formula><mml:math id="M2080" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> (<inline-formula><mml:math id="M2081" display="inline"><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">366</mml:mn></mml:mrow></mml:math></inline-formula>) and causes
calculated growth rates to go up approximately 0.3 % if the first year is
a leap year and down 0.3 % if the second year is a leap year.
<?xmltex \hack{\newpage}?>
The relative growth rate of <inline-formula><mml:math id="M2082" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> over time periods of greater than 1 year can be rewritten using its logarithm equivalent as follows:
              <disp-formula id="App1.Ch1.S3.E3" content-type="numbered"><label>C1</label><mml:math id="M2083" display="block"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:mo>(</mml:mo><mml:mi>ln⁡</mml:mi><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mspace width="0.125em" linebreak="nobreak"/></mml:mrow><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
            Here we calculate relative growth rates in emissions for multi-year periods
(e.g. a decade) by fitting a linear trend to ln(<inline-formula><mml:math id="M2084" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) in Eq. (2), reported
in percent per year.</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSS5">
  <label>C1.5</label><?xmltex \opttitle{Emissions projection for $E_{{\mathrm{FOS}}}$}?><title>Emissions projection for <inline-formula><mml:math id="M2085" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></title>
      <p id="d1e32749">To gain insight into emission trends for 2021, we provide an assessment of
global fossil CO<inline-formula><mml:math id="M2086" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions, <inline-formula><mml:math id="M2087" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, by combining individual
assessments of emissions for China, USA, the EU, and India (the four
countries and regions with the largest emissions), and the rest of the world. We
provide full year estimates for two datasets: IEA (2021b) and our own
analysis. This approach differs from last year where we used four
independent estimates including our own, because of the unique circumstances
related to the COVID-19 pandemic. This year's analysis is more in line with
earlier budgets.</p>
      <p id="d1e32772">Previous editions of the Global Carbon Budget (GCB) have estimated year-to-date (YTD) emissions, and performed projections, using sub-annual energy
consumption data from a variety of sources depending on the country or
region. The YTD estimates have then been projected to the full year using
specific methods for each country or region. The methods described in detail
below.</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSSx1" specific-use="unnumbered">
  <title>China</title>
      <p id="d1e32781">We use the growth in total fossil CO<inline-formula><mml:math id="M2088" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions in 2021
reported by the National Bureau of Statistics (NBS) in their 2022
Statistical Communique (NBS, 2022). This report includes growth rates of
energy consumption for coal, oil, and natural gas as well as the growth in
cement production, which are used to determine the changes in emissions from
these four categories.</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSSx2" specific-use="unnumbered">
  <title>USA</title>
      <p id="d1e32799">We use emissions estimated by the U.S. Energy Information
Administration (EIA) in their Short-Term Energy Outlook (STEO) for emissions
from fossil fuels to get both a YTD and a full-year projection (EIA, 2022).
The STEO also includes a near-term forecast based on an energy forecasting
model which is updated monthly (last update with preliminary data through
September 2021) and takes into account expected temperatures, household
expenditures by fuel type, energy markets, policies, and other effects. We
combine this with our estimate of emissions from cement production using the
monthly U.S. cement clinker production data from USGS for January–June 2021,
assuming changes in cement production over the first part of the year apply
throughout the year.</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSSx3" specific-use="unnumbered">
  <title>India</title>
      <p id="d1e32808">We use monthly emissions estimates for India updated from
Andrew (2020b) through August 2021. These estimates are derived from many
official monthly energy and other activity data sources to produce direct
estimates of national CO<inline-formula><mml:math id="M2089" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions, without the use of proxies.
Emissions from coal are then extended to September using a regression
relationship based on power generated from coal, coal dispatches by Coal
India Ltd., the composite PMI, time, and days per month. For the last 3–4
months of the year, each series is extrapolated assuming typical trends.</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSSx4" specific-use="unnumbered">
  <title>EU</title>
      <p id="d1e32826">We use a refinement to the methods presented by Andrew (2021),
deriving emissions from monthly energy data reported by Eurostat. Some data
gaps are filled using data from the Joint Organisations Data Initiative
(JODI, 2022). Sub-annual cement production data are limited, but data for
Germany and Poland, the two largest producers, suggest a small decline. For
fossil fuels this provides estimates through July. We extend coal emissions
through September using a regression model built from generation of power
from hard coal, power from brown coal, total power generation, and the
number of working days in Germany and Poland, the two biggest coal consumers
in the EU. These are then extended through the end of the year assuming
typical trends. We extend oil emissions by building a regression model
between our monthly CO<inline-formula><mml:math id="M2090" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> estimates and oil consumption reported by the EIA
for Europe in its Short-Term Energy Outlook (October edition), and then
using this model with EIA's monthly forecasts. For natural gas, the strong
seasonal signal allows the use of the bias-adjusted Holt–Winters exponential
smoothing method (Chatfield, 1978).</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSSx5" specific-use="unnumbered">
  <title>Rest of the world</title>
      <p id="d1e32845">We use the close relationship between the growth
in GDP and the growth in emissions (Raupach et al., 2007) to project
emissions for the current year. This is based on a simplified Kaya identity,
whereby <inline-formula><mml:math id="M2091" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (GtC yr<inline-formula><mml:math id="M2092" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) is decomposed by the product of GDP (USD yr<inline-formula><mml:math id="M2093" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and the fossil fuel carbon intensity of the economy (<inline-formula><mml:math id="M2094" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>;
GtC USD<inline-formula><mml:math id="M2095" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) as follows:
              <disp-formula id="App1.Ch1.S3.E4" content-type="numbered"><label>C2</label><mml:math id="M2096" display="block"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>=</mml:mo><mml:mi mathvariant="normal">GDP</mml:mi><mml:mo>×</mml:mo><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub><mml:mo>.</mml:mo></mml:mrow></mml:math></disp-formula>
            Taking a time derivative of Eq. (3) and rearranging gives the following:
              <disp-formula id="App1.Ch1.S3.E5" content-type="numbered"><label>C3</label><mml:math id="M2097" display="block"><mml:mrow><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>=</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mi mathvariant="normal">GDP</mml:mi></mml:mfrac></mml:mstyle><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mi mathvariant="normal">dGDP</mml:mi><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>+</mml:mo><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mn mathvariant="normal">1</mml:mn><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:mfrac></mml:mstyle><mml:mstyle displaystyle="true"><mml:mfrac style="display"><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow><mml:mrow><mml:mi mathvariant="normal">d</mml:mi><mml:mi>t</mml:mi></mml:mrow></mml:mfrac></mml:mstyle><mml:mo>,</mml:mo></mml:mrow></mml:math></disp-formula>
            where the left-hand term is the relative growth rate of <inline-formula><mml:math id="M2098" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, and the
right-hand terms are the relative growth rates of GDP and <inline-formula><mml:math id="M2099" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>,
respectively, which can simply be added linearly to give the overall growth
rate.</p>
      <p id="d1e33030">The <inline-formula><mml:math id="M2100" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is based on GDP in constant PPP (purchasing power parity) from
the International Energy Agency (IEA) up to 2017 (IEA/OECD, 2019) and
extended using the International Monetary Fund (IMF) growth rates through
2020 (IMF, 2022). Interannual variability in <inline-formula><mml:math id="M2101" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the largest source
of uncertainty in the GDP-based emissions projections. We thus use the
standard deviation of the annual <inline-formula><mml:math id="M2102" display="inline"><mml:mrow><mml:msub><mml:mi>I</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> for the period 2009–2019 as a
measure of uncertainty, reflecting a <inline-formula><mml:math id="M2103" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M2104" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> as in the rest of
the carbon budget.</p>
</sec>
<sec id="App1.Ch1.S3.SS1.SSSx6" specific-use="unnumbered">
  <title>World</title>
      <p id="d1e33086">The global total is the sum of each of the countries and
regions.</p>
</sec>
</sec>
<sec id="App1.Ch1.S3.SS2">
  <label>C2</label><?xmltex \opttitle{Methodology CO${}_{{2}}$ emissions from land use, land-use
change, and forestry ($E_{{\mathrm{LUC}}}$)}?><title>Methodology CO<inline-formula><mml:math id="M2105" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from land use, land-use
change, and forestry (<inline-formula><mml:math id="M2106" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</title>
      <p id="d1e33119">The net CO<inline-formula><mml:math id="M2107" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux from land use, land-use change, and forestry
(<inline-formula><mml:math id="M2108" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, called land-use change emissions in the rest of the text)
includes CO<inline-formula><mml:math id="M2109" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes from deforestation, afforestation, logging and
forest degradation (including harvest activity), shifting cultivation (cycle
of cutting forest for agriculture, then abandoning), and regrowth of forests
following wood harvest or abandonment of agriculture. Emissions from peat
burning and drainage are added from external datasets (see Sect. C2.1
below). Only some land-management activities are included in our land-use
change emissions estimates (Table A1). Some of these activities lead to
emissions of CO<inline-formula><mml:math id="M2110" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> to the atmosphere, while others lead to CO<inline-formula><mml:math id="M2111" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
sinks. <inline-formula><mml:math id="M2112" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is the net sum of emissions and removals due to all
anthropogenic activities considered. Our annual estimate for 1960–2020 is
provided as the average of results from three bookkeeping approaches
(Sect. C2.1 below): an estimate using the Bookkeeping of Land Use
Emissions model (Hansis et al., 2015; hereafter BLUE) and one using the
compact Earth system model OSCAR (Gasser et al., 2020), both BLUE and OSCAR
being updated here to new land-use forcing covering the time period until
2020, and an updated version of the estimate published by Houghton and
Nassikas (2017) (hereafter updated H&amp;N2017). All three datasets are then
extrapolated to provide a projection for 2021 (Sect. C2.5 below). In
addition, we use results from dynamic global vegetation models (DGVMs; see
Sect. 2.5 and Table 4) to help quantify the uncertainty in <inline-formula><mml:math id="M2113" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Sect. C2.4), and thus better characterize our understanding. Note
that in this budget, we use the scientific <inline-formula><mml:math id="M2114" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> definition, which
counts fluxes due to environmental changes on managed land towards
<inline-formula><mml:math id="M2115" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, as opposed to the national greenhouse gas inventories under the
UNFCCC, which include them in <inline-formula><mml:math id="M2116" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and thus often report smaller
land-use emissions (Grassi et al., 2018; Petrescu et al., 2020). However, we
provide a methodology of mapping of the two approaches to each other further
below (Sect. C2.3).
<?xmltex \hack{\newpage}?></p>
<sec id="App1.Ch1.S3.SS2.SSS1">
  <label>C2.1</label><title>Bookkeeping models</title>
      <p id="d1e33233">Land-use change CO<inline-formula><mml:math id="M2117" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions and uptake fluxes are calculated by three
bookkeeping models. These are based on the original bookkeeping approach of
Houghton (2003) that keeps track of the carbon stored in vegetation and
soils before and after a land-use change (transitions between various
natural vegetation types, croplands, and pastures). Literature-based
response curves describe decay of vegetation and soil carbon, including
transfer to product pools of different lifetimes, as well as carbon uptake
due to regrowth. In addition, the bookkeeping models represent long-term
degradation of primary forest as lowered standing vegetation and soil carbon
stocks in secondary forests and include forest management practices such as
wood harvests.</p>
      <p id="d1e33245">BLUE and the updated H&amp;N2017 exclude land ecosystems' transient response
to changes in climate, atmospheric CO<inline-formula><mml:math id="M2118" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, and other environmental factors
and base the carbon densities on contemporary data from literature and
inventory data. Since carbon densities thus remain fixed over time, the
additional sink capacity that ecosystems provide in response to
CO<inline-formula><mml:math id="M2119" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fertilization and some other environmental changes is not captured
by these models (Pongratz et al., 2014). On the contrary, OSCAR includes
this transient response, and it follows a theoretical framework (Gasser and
Ciais, 2013) that allows the separation of bookkeeping land-use emissions and the
loss of additional sink capacity. Only the former is included here, while
the latter is discussed in Appendix D4. The bookkeeping models differ in (1) computational units (spatially explicit treatment of land-use change for
BLUE, regional- or mostly country-level for the updated H&amp;N2017 and OSCAR),
(2) processes represented (see Table A1), and (3) carbon densities assigned
to vegetation and soil of each vegetation type (literature-based for the
updated H&amp;N2017 and BLUE, calibrated to DGVMs for OSCAR). A notable
difference between models exists with respect to the treatment of shifting
cultivation. The update of H&amp;N2017 changed the approach over the earlier
H&amp;N2017 version: H&amp;N2017 had assumed the “excess loss” of tropical
forests (i.e. when FRA indicated a forest loss larger than the increase in
agricultural areas from FAO) resulted from converting forests to croplands
at the same time older croplands were abandoned. Those abandoned croplands
began to recover to forests after 15 years. The updated H&amp;N2017 now
assumes that forest loss in excess of increases in cropland and pastures
represented an increase in shifting cultivation. When the excess loss of
forests was negative, it was assumed that shifting cultivation was returned
to forest. Historical areas in shifting cultivation were extrapolated taking
into account country-based estimates of areas lying fallow in 1980 (FAO/UNEP,
1981) and expert opinion (from Heinimann et al., 2017). In contrast, the
BLUE and OSCAR models include sub-grid-scale transitions between all
vegetation types. Furthermore, the updated H&amp;N2017 assume conversion of
natural grasslands to pasture, while BLUE and OSCAR allocate pasture
proportionally on all natural vegetation that exists in a grid cell. This is
one reason for generally higher emissions in BLUE and OSCAR. Bookkeeping
models do not directly capture carbon emissions from peat fires, which can
create large emissions and interannual variability due to synergies of
land-use and climate variability in Southeast Asia, particularly during
El-Niño events, nor emissions from the organic layers of drained peat
soils. To correct for this, the updated H&amp;N2017 includes carbon emissions
from burning and draining of peatlands in Indonesia, Malaysia, and Papua New
Guinea (based on the Global Fire Emission Database, GFED4s; van der Werf et
al., 2017, for fire and Hooijer et al., 2010, for drainage). Further, estimates of
carbon losses from peatlands in extra-tropical regions are added from Qiu et
al. (2021). We add GFED4s peat fire emissions to BLUE and OSCAR output as
well as the global FAO peat drainage emissions 1990–2018 from croplands and
grasslands (Conchedda and Tubiello, 2020), keeping post-2018 emissions
constant. We linearly increase tropical drainage emissions from 0 in 1980,
consistent with H&amp;N2017's assumption, and keep emissions from the often
old drained areas of the extra-tropics constant pre-1990. This adds 9.0 GtC
for FAO compared to 5.6 GtC for Hooijer et al. (2010). Peat fires add
another 2.0 GtC over the same period.</p>
      <p id="d1e33266">The three bookkeeping estimates used in this study differ with respect to
the land-use change data used to drive the models. The updated H&amp;N2017
base their estimates directly on the Forest Resource Assessment of the FAO
which provides statistics on forest-area change and management at intervals
of 5 years currently updated until 2020 (FAO, 2020). The data are based on
country reporting to FAO and may include remote-sensing information in more
recent assessments. Changes in land use other than forests are based on
annual, national changes in cropland and pasture areas reported by FAO
(FAOSTAT, 2021). On the other hand, BLUE uses the harmonized land-use change
data LUH2-GCB2021 covering the entire 850–2020 period (an update to the
previously released LUH2 v2h dataset; Hurtt et al., 2017,
2020), which was also used as input to the DGVMs (Sect. C2.2). It
describes land-use change, also based on the FAO data as described in
Sect. C2.2 as well as the HYDE3.3 dataset (Klein Goldewijk et al., 2017a, b), but provided at a quarter-degree spatial resolution, considering
sub-grid-scale transitions between primary forest, secondary forest, primary
non-forest, secondary non-forest, cropland, pasture, rangeland, and urban
land (Hurtt et al., 2020; Chini et al., 2021). LUH2-GCB2021 provides a
distinction between rangelands and pasture, based on inputs from HYDE. To
constrain the models' interpretation on whether rangeland implies the
original natural vegetation to be transformed to grassland or not (e.g.
browsing on shrubland), a forest mask was provided with LUH2-GCB2021; forest
is assumed to be transformed to grasslands, while other natural vegetation
remains (in case of secondary vegetation) or is degraded from primary to
secondary vegetation (Ma et al., 2020). This is implemented in BLUE. OSCAR
was run with both LUH2-GCB2021 and FAO/FRA (as used by Houghton and
Nassikas, 2017), where emissions from the latter were extended beyond 2015
with constant 2011–2015 average values. The best-guess OSCAR estimate used
in our study is a combination of results for LUH2-GCB2021 and FAO/FRA
land-use data and a large number of perturbed parameter simulations weighted
against an observational constraint. All three bookkeeping estimates were
extended from 2020 to provide a projection for 2021 by adding the annual
change in emissions from tropical deforestation and degradation and peat
burning and drainage to the respective model's estimate for 2020 (van der
Werf et al., 2017; Conchedda and Tubiello, 2020).</p>
      <p id="d1e33269">For <inline-formula><mml:math id="M2120" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from 1850 onwards we average the estimates from BLUE, the
updated H&amp;N2017 and OSCAR. For the cumulative numbers starting 1750 an
average of four earlier publications is added (30 <inline-formula><mml:math id="M2121" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 20 PgC 1750–1850,
rounded to nearest 5; Le Quéré et al., 2016).</p>
      <p id="d1e33291">We provide estimates of the gross land-use change fluxes from which the
reported net land-use change flux, <inline-formula><mml:math id="M2122" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, is derived as a sum. Gross
fluxes are derived internally by the three bookkeeping models: gross
emissions stem from decaying material left dead on site and from products
after clearing of natural vegetation for agricultural purposes, wood
harvesting, emissions from peat drainage and peat burning, and, for BLUE,
additionally from degradation from primary to secondary land through usage
of natural vegetation as rangeland. Gross removals stem from regrowth after
agricultural abandonment and wood harvesting. Gross fluxes for the updated
H&amp;N2017 2016–2020 and for the 2021 projection of all three models were
based on a regression of gross sources (including peat emissions) to net
emissions for recent years.</p>
      <p id="d1e33305">Due to an artefact in the HYDE3.3 dataset expressed as an abrupt shift in
the pattern of pastures and rangelands in 1960, the year 1960 exhibits much
larger gross transitions between natural vegetation and pastures and rangelands
than prior and subsequent years. Although these gross transitions cancel out in
terms of net area changes causing large abrupt transitions, an unrealistic
peak in emissions occurs around 1960 in BLUE and OSCAR. To correct for this,
we replace the estimates for 1959–1961 by the average of 1958 and 1962 in
both BLUE and OSCAR. Abrupt transitions will immediately influence gross
emissions, which have a larger instantaneous component. Processes with
longer timescales, such as slow legacy emissions and regrowth, are
inseparable from the carbon dynamics due to subsequent land-use change
events. We therefore do not adjust gross removals, but only gross emissions
to match the corrected net flux. Since DGVM estimates are only used for an
uncertainty range of <inline-formula><mml:math id="M2123" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, which is independent of land-use changes, no
correction is applied to the DGVM data.</p>
</sec>
<sec id="App1.Ch1.S3.SS2.SSS2">
  <label>C2.2</label><title>Dynamic global vegetation models (DGVMs)</title>
      <p id="d1e33327">Land-use change CO<inline-formula><mml:math id="M2124" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions have also been estimated using an
ensemble of 17 DGVM simulations. The DGVMs account for deforestation and
regrowth, the most important components of <inline-formula><mml:math id="M2125" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, but they do not
represent all processes resulting directly from human activities on land
(Table A1). All DGVMs represent processes of vegetation growth and
mortality, as well as decomposition of dead organic matter associated with
natural cycles, and include the vegetation and soil carbon response to
increasing atmospheric CO<inline-formula><mml:math id="M2126" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration and to climate variability and
change. Most models explicitly simulate the coupling of carbon and nitrogen
cycles and account for atmospheric N deposition and N fertilizers (Table A1). The DGVMs are independent from the other budget terms except for their
use of atmospheric CO<inline-formula><mml:math id="M2127" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration to calculate the fertilization
effect of CO<inline-formula><mml:math id="M2128" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> on plant photosynthesis.</p>
      <p id="d1e33377">DGVMs that do not simulate sub-grid-scale transitions (i.e. net land-use
emissions; see Table A1) used the HYDE land-use change dataset (Klein
Goldewijk et al., 2017a, b), which provides annual (1700–2019),
half-degree, fractional data on cropland and pasture. The data are based on
the available annual FAO statistics of change in agricultural land area
available until 2015. The new HYDE3.3 cropland and grazing land dataset which
now in addition to having FAO country-level statistics is constrained spatially
based on multi-year satellite land-cover maps from ESA CCI LC. Data from
HYDE3.3 are based on a FAO which includes yearly data from 1961 up to and
including the year 2017. After the year 2017 HYDE extrapolates the cropland,
pasture, and urban data linearly based on the trend over the previous 5 years, to generate data until the year 2020. HYDE also uses satellite
imagery from ESA-CCI from 1992–2018 for more detailed yearly allocation
of cropland and grazing land, with the ESA area data scaled to match the FAO
annual totals at country level. The 2018 map is also used for the 2019–2020
period. The original 300 m resolution data from ESA were aggregated to a
5 arcmin resolution according to the classification scheme as described
in Klein Goldewijk et al. (2017a). DGVMs that simulate sub-grid-scale
transitions (i.e. gross land-use emissions; see Table A1) also use the
LUH2-GCB2021 dataset, an update of the more comprehensive harmonized
land-use dataset (Hurtt et al., 2020), that further includes fractional
data on primary and secondary forest vegetation, as well as all underlying
transitions between land-use states (850–2020; Hurtt et al., 2011, 2017,
2020; Chini et al., 2021; Table A1). This new dataset is of quarter-degree
fractional areas of land-use states and all transitions between those
states, including a new wood harvest reconstruction and new representation of
shifting cultivation, crop rotations, and management information including
irrigation and fertilizer application. The land-use states include five
different crop types in addition to the pasture–rangeland split discussed
before. Wood harvest patterns are constrained with Landsat-based tree cover
loss data (Hansen et al., 2013). Updates of LUH2-GCB2021 over last year's
version (LUH2-GCB2020) are using the most recent HYDE/FAO release (covering
the time period up to 2021 included). We also use the most recent FAO wood
harvest data for all years from 1961 to 2019. After the year 2019 we
extrapolated the wood harvest data until the year 2020. The HYDE3.3
population data are also used to extend the wood harvest time series back in
time. Other wood harvest inputs (for years prior to 1961) remain the same in
LUH2. With the switch from HYDE3.2 to HYDE3.3 changes in the land-use
forcing compared to the version used in the GCB2020 (Friedlingstein et al.,
2020) are pronounced. They are thus compared in Fig. 6b and their relevance
for land-use emissions discussed in Sect. 3.4.2. DGVMs implement land-use
change differently (e.g. an increased cropland fraction in a grid cell can
either be at the expense of grassland or shrubs, or forest, the latter
resulting in deforestation; land-cover fractions of the non-agricultural
land differ between models). Similarly, model-specific assumptions are
applied to convert deforested biomass or deforested area, and other forest
product pools into carbon, and different choices are made regarding the
allocation of rangelands as natural vegetation or pastures.</p>
      <p id="d1e33380">The difference between two DGVM simulations (see Sect. C4.1 below), one
forced with historical changes in land-use and a second with time-invariant
pre-industrial land cover and pre-industrial wood harvest rates, allows
quantification of the dynamic evolution of vegetation biomass and soil
carbon pools in response to land-use change in each model (<inline-formula><mml:math id="M2129" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). Using
the difference between these two DGVM simulations to diagnose <inline-formula><mml:math id="M2130" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
means the DGVMs account for the loss of additional sink capacity (around 0.4 <inline-formula><mml:math id="M2131" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M2132" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>; see Sect. 2.7.4, Appendix D4), while the bookkeeping
models do not.</p>
      <p id="d1e33424">As a criterion for inclusion in this carbon budget, we only retain models
that simulate a positive <inline-formula><mml:math id="M2133" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> during the 1990s, as assessed in the IPCC
AR4 (Denman et al., 2007) and AR5 (Ciais et al., 2013). All DGVMs met this
criterion, although one model was not included in the <inline-formula><mml:math id="M2134" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate
from DGVMs as it exhibited a spurious response to the transient land-cover
change forcing after its initial spin-up.</p>
</sec>
<sec id="App1.Ch1.S3.SS2.SSS3">
  <label>C2.3</label><?xmltex \opttitle{Mapping of national GHG inventory data to $E_{{\mathrm{LUC}}}$}?><title>Mapping of national GHG inventory data to <inline-formula><mml:math id="M2135" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></title>
      <p id="d1e33469">An approach was implemented to reconcile the large gap between <inline-formula><mml:math id="M2136" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from
bookkeeping models and land use, land-use change, and forestry (LULUCF) from
national GHG inventories (NGHGIs) (see Table A8). This gap is due to different
approaches to calculating “anthropogenic” CO<inline-formula><mml:math id="M2137" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes related to
land-use change and land management (Grassi et al., 2018). In particular, the
land sinks due to environmental change on managed lands are treated as
non-anthropogenic in the global carbon budget, while they are generally
considered as anthropogenic in NGHGIs (“indirect anthropogenic fluxes”;
Eggleston et al., 2006). Building on previous studies (Grassi et al., 2021),
the approach implemented here adds the DGVM estimates of CO<inline-formula><mml:math id="M2138" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes
due to environmental change from countries' managed forest area (part of the
<inline-formula><mml:math id="M2139" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) to the original <inline-formula><mml:math id="M2140" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> flux. This sum is expected to be
conceptually more comparable to LULUCF than simply <inline-formula><mml:math id="M2141" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e33535"><inline-formula><mml:math id="M2142" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> data are taken from bookkeeping models, in line with the global carbon
budget approach. To determine <inline-formula><mml:math id="M2143" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> on managed forest, the following
steps were taken: Spatially gridded data of “natural” forest NBP (net biome productivity) (<inline-formula><mml:math id="M2144" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, i.e. due to environmental change and excluding land-use change
fluxes) were obtained with S2 runs from DGVMs up to 2019 from the TRENDY v9
dataset. Results were first masked with the Hansen forest map (Hansen et al., 2013), with a 20 % tree cover and following the FAO definition of forest
(isolated pixels with maximum connectivity less than 0.5 ha are excluded),
and then further masked with the “intact” forest map for the year 2013,
i.e. forest areas characterized by no remotely detected signs of human
activity (Potapov et al., 2017). This way, we obtained the <inline-formula><mml:math id="M2145" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in
“intact” and “non-intact” forest area, which previous studies (Grassi et al., 2021) indicated to be a good proxy, respectively, for “unmanaged” and
“managed” forest area in the NGHGI. Note that only four models (CABLE-POP,
CLASSIC, YIBs and ORCHIDEE-CNP) had forest NBP at grid cell level. Two
models (OCN and ISBA-CTRIP) provided forest NEP and simulated disturbances
at pixel level that were used as basis, in addition to forest cover
fraction, to estimate forest NBP. For the other DGVMs, when a grid cell had
forest, all the NBP was allocated to forest.</p>
      <p id="d1e33581">LULUCF data from NGHGIs are from Grassi et al. (2021) until 2017, updated
until 2019 for UNFCCC Annex I countries. For non-Annex I countries, the
years 2018 and 2019 were assumed to be equal to the average 2013–2017. These
data include all CO<inline-formula><mml:math id="M2146" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes from land considered managed, which in
principle encompasses all land uses (forest land, cropland, grassland,
wetlands, settlements, and other land), changes among them, and emissions from
organic soils and from fires. In practice, although almost all Annex I
countries report all land uses, many non-Annex I countries report only on
deforestation and forest land, and few countries report on other land
uses. In most cases, NGHGIs include most of the natural response to recent
environmental change, because they use direct observations (e.g. national
forest inventories) that do not allow the separation of direct and indirect
anthropogenic effects (Eggleston et al., 2006).</p>
      <p id="d1e33594">To provide additional, largely independent assessments of fluxes on
unmanaged vs. managed lands, we include a DGVM that allows diagnosis of fluxes
from unmanaged vs. managed lands by tracking vegetation cohorts of different
ages separately. This model, ORCHIDEE-MICT (Yue et al., 2018), was run using
the same LUH2 forcing as the DGVMs used in this budget (Sect. 2.5) and the
bookkeeping models BLUE and OSCAR (Sect. 2.2). Old-aged forest was
classified as primary forest after a certain threshold of carbon density was
reached again, and the model-internal distinction between primary and
secondary forest used as proxies for unmanaged vs. managed forests;
agricultural lands are added to the latter to arrive at total managed land.</p>
      <p id="d1e33597">Table A8 shows the resulting mapping of global carbon cycle models' land flux
definitions to that of the NGHGI (discussed in Sect. 3.2.2). ORCHIDEE-MICT
estimates for <inline-formula><mml:math id="M2147" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> on intact forests are expected to be higher than those based
on DGVMs in combination with the NGHGI managed and unmanaged forest data because
the unmanaged forest area, with about 27 mio km<inline-formula><mml:math id="M2148" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>, is estimated to be
substantially larger by ORCHIDEE-MICT than that, with less than 10 mio km<inline-formula><mml:math id="M2149" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>, by
the NGHGI, while managed forest area is estimated to be smaller (22 compared
to 32 mio km<inline-formula><mml:math id="M2150" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>). Related to this, <inline-formula><mml:math id="M2151" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> on non-intact lands plus
<inline-formula><mml:math id="M2152" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> is a larger source estimated by ORCHIDEE-MICT compared to the NGHGI.
We also show as comparison FAOSTAT emissions totals (FAO, 2021), which
include emissions from net forest conversion and fluxes on forest land
(Tubiello et al., 2021) as well as CO<inline-formula><mml:math id="M2153" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from peat drainage and
peat fires.</p>
</sec>
<sec id="App1.Ch1.S3.SS2.SSS4">
  <label>C2.4</label><?xmltex \opttitle{Uncertainty assessment for $E_{{\mathrm{LUC}}}$}?><title>Uncertainty assessment for <inline-formula><mml:math id="M2154" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></title>
      <p id="d1e33689">Differences between the bookkeeping models and DGVMs originate from
three main sources: the different methodologies, which among others lead to
inclusion of the loss of additional sink capacity in DGVMs (see Appendix D1.4), the underlying land-use/land-cover dataset, and the different
processes represented (Table A1). We examine the results from the DGVMs and of the bookkeeping method and use the resulting variations as a
way to characterize the uncertainty in <inline-formula><mml:math id="M2155" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e33703">Despite these differences, the <inline-formula><mml:math id="M2156" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimate from the DGVMs multi-model
mean is consistent with the average of the emissions from the bookkeeping
models (Table 5). However, there are large differences among individual DGVMs
(standard deviation at around 0.5 GtC yr<inline-formula><mml:math id="M2157" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>; Table 5), between the
bookkeeping estimates (average difference 1850–2020 BLUE-updated H&amp;N2017
of 0.8 GtC yr<inline-formula><mml:math id="M2158" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, BLUE-OSCAR of 0.4 GtC yr<inline-formula><mml:math id="M2159" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, OSCAR-updated
H&amp;N2017 of 0.3 GtC yr<inline-formula><mml:math id="M2160" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), and between the updated estimate of
H&amp;N2017 and its previous model version (Houghton et al., 2012). A
factorial analysis of differences between BLUE and H&amp;N2017 attributed
them particularly to differences in carbon densities between natural and
managed vegetation or primary and secondary vegetation (Bastos et al.,
2021). Earlier studies additionally showed the relevance of the different
land-use forcing as applied (in updated versions) also in the current study
(Gasser et al., 2020).</p>
      <p id="d1e33765">The uncertainty in <inline-formula><mml:math id="M2161" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> of <inline-formula><mml:math id="M2162" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.7 GtC yr<inline-formula><mml:math id="M2163" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> reflects our best
value judgement that there is at least 68 % chance (<inline-formula><mml:math id="M2164" display="inline"><mml:mo lspace="0mm">±</mml:mo></mml:math></inline-formula>1<inline-formula><mml:math id="M2165" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>) that the true land-use change emission lies within the given range, for the
range of processes considered here. Prior to the year 1959, the uncertainty
in <inline-formula><mml:math id="M2166" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> was taken from the standard deviation of the DGVMs. We assign
low confidence to the annual estimates of <inline-formula><mml:math id="M2167" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> because of the
inconsistencies among estimates and of the difficulties of quantifying some of
the processes in DGVMs.</p>
</sec>
<sec id="App1.Ch1.S3.SS2.SSS5">
  <label>C2.5</label><?xmltex \opttitle{Emissions projections for $E_{{\mathrm{LUC}}}$}?><title>Emissions projections for <inline-formula><mml:math id="M2168" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></title>
      <p id="d1e33854">We project the 2021 land-use emissions for BLUE, the updated H&amp;N2017, and
OSCAR, starting from their estimates for 2020 assuming unaltered peat
drainage, which has low interannual variability, and the highly variable
emissions from peat fires, tropical deforestation, and degradation as
estimated using active fire data (MCD14ML; Giglio et al., 2016). The
latter scale almost linearly with GFED over large areas (van der Werf et
al., 2017) and thus allow for tracking fire emissions in deforestation and
tropical peat zones in near-real time.</p>
</sec>
</sec>
<sec id="App1.Ch1.S3.SS3">
  <label>C3</label><?xmltex \opttitle{Methodology ocean CO${}_{{{2}}}$ sink ($S_{{\mathrm{OCEAN}}}$)}?><title>Methodology ocean CO<inline-formula><mml:math id="M2169" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M2170" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</title>
<sec id="App1.Ch1.S3.SS3.SSS1">
  <label>C3.1</label><title>Observation-based estimates</title>
      <p id="d1e33894">We primarily use the observational constraints assessed by IPCC of a mean
ocean CO<inline-formula><mml:math id="M2171" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink of 2.2 <inline-formula><mml:math id="M2172" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M2173" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the 1990s (90 %
confidence interval; Ciais et al., 2013) to verify that the GOBMs provide a
realistic assessment of <inline-formula><mml:math id="M2174" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. This is based on indirect observations
with seven different methodologies and their uncertainties, using the
methods that are deemed most reliable for the assessment of this quantity
(Denman et al., 2007; Ciais et al., 2013). The observation-based estimates
use the ocean–land CO<inline-formula><mml:math id="M2175" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink partitioning from observed atmospheric
CO<inline-formula><mml:math id="M2176" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and O<inline-formula><mml:math id="M2177" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> <inline-formula><mml:math id="M2178" display="inline"><mml:mo>/</mml:mo></mml:math></inline-formula> N<inline-formula><mml:math id="M2179" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration trends (Manning and Keeling,
2006;  Keeling and Manning, 2014), an oceanic inversion method constrained by
ocean biogeochemistry data (Mikaloff Fletcher et al., 2006), and a method
based on penetration timescale for chlorofluorocarbons (McNeil et al.,
2003). The IPCC estimate of 2.2 GtC yr<inline-formula><mml:math id="M2180" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the 1990s is consistent
with a range of methods (Wanninkhof et al., 2013). We refrain from using the
IPCC estimates for the 2000s (2.3 <inline-formula><mml:math id="M2181" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M2182" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>), and the period
2002–2011 (2.4 <inline-formula><mml:math id="M2183" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.7 GtC yr<inline-formula><mml:math id="M2184" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Ciais et al., 2013) as these are
based on trends derived mainly from models and one data product (Ciais et
al., 2013). Additional constraints summarized in AR6 (Canadell et al., 2022)
are the interior ocean anthropogenic carbon change (Gruber et al., 2019) and
ocean sink estimate from atmospheric CO<inline-formula><mml:math id="M2185" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and O<inline-formula><mml:math id="M2186" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> <inline-formula><mml:math id="M2187" display="inline"><mml:mo>/</mml:mo></mml:math></inline-formula> N<inline-formula><mml:math id="M2188" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (Tohjima
et al., 2019) which are used for model evaluation and discussion,
respectively.</p>
      <p id="d1e34066">We also use eight estimates of the ocean CO<inline-formula><mml:math id="M2189" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink and its variability
based on surface ocean <inline-formula><mml:math id="M2190" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2191" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> maps obtained by the interpolation of
surface ocean <inline-formula><mml:math id="M2192" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2193" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements from 1990 onwards due to severe
restriction in data availability prior to 1990 (Fig. 9). These estimates
differ in many respects: they use different maps of surface <inline-formula><mml:math id="M2194" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2195" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>,
different atmospheric CO<inline-formula><mml:math id="M2196" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations, wind products and different
gas-exchange formulations as specified in Table A3. We refer to them as
<inline-formula><mml:math id="M2197" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2198" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based flux estimates. The measurements underlying the surface
<inline-formula><mml:math id="M2199" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2200" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> maps are from the Surface Ocean CO<inline-formula><mml:math id="M2201" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> Atlas version 2021
(SOCATv2021; Bakker et al., 2021), which is an update of version 3 (Bakker
et al., 2016) and contains quality-controlled data through 2020 (see data
attribution Table A5). Each of the estimates uses a different method to then
map the SOCAT v2021 data to the global ocean. The methods include a
data-driven diagnostic method (Rödenbeck et al., 2013; referred to here
as Jena-MLS), three neural network models (Landschützer et al., 2014;
referred to as MPI-SOMFFN; Chau et al., 2022; Copernicus Marine Environment
Monitoring Service, referred to here as CMEMS-LSCE-FFNN; and Zeng et al.,
2014; referred to as NIES-FNN), two cluster regression approaches (Gregor et
al., 2019; referred to here as CSIR-ML6; and Gregor and Gruber, 2021,
referred to as OS-ETHZ-GRaCER), and a multi-linear regression method (Iida
et al., 2021; referred to as JMA-MLR). The ensemble mean of the
<inline-formula><mml:math id="M2202" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2203" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based flux estimates is calculated from these seven mapping
methods. Further, we show the flux estimate of Watson et al. (2020), who also
use the MPI-SOMFFN method to map the adjusted <inline-formula><mml:math id="M2204" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2205" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data to the globe,
but resulting in a substantially larger ocean sink estimate, owing to a
number of adjustments they applied to the surface ocean <inline-formula><mml:math id="M2206" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2207" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data and
the gas-exchange parameterization. Concretely, these authors adjusted the
SOCAT <inline-formula><mml:math id="M2208" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2209" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> downward to account for differences in temperature between
the depth of the ship intake and the relevant depth right near the surface
and included a further adjustment to account for the cool surface skin
temperature effect. The Watson et al. flux estimate hence differs from the
others by their choice of adjusting the flux to a cool, salty ocean surface
skin. Watson et al. (2020) showed that this temperature adjustment leads to
an upward correction of the ocean carbon sink, up to 0.9 GtC yr<inline-formula><mml:math id="M2210" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>,
that, if correct, should be applied to all <inline-formula><mml:math id="M2211" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2212" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based flux estimates.
So far, this adjustment is based on a single line of evidence and hence
associated with low confidence until further evidence is available. The
Watson et al. flux estimate presented here is therefore not included in the
ensemble mean of the <inline-formula><mml:math id="M2213" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2214" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based flux estimates. This choice will be
re-evaluated in upcoming budgets based on further lines of evidence.</p>
      <p id="d1e34288">The CO<inline-formula><mml:math id="M2215" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux from each <inline-formula><mml:math id="M2216" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2217" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based product is either already at or
above 98 % areal coverage (Jena-MLS, OS-ETHZ-GRaCER), filled by the
data provider (using Fay et al., 2021, method for JMA-MLR; and
Landschützer et al., 2020, methodology for MPI-SOMFFN) or scaled for the
remaining products by the ratio of the total ocean area covered by the
respective product to the total ocean area (<inline-formula><mml:math id="M2218" display="inline"><mml:mrow><mml:mn mathvariant="normal">361.9</mml:mn><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">10</mml:mn><mml:mn mathvariant="normal">6</mml:mn></mml:msup></mml:mrow></mml:math></inline-formula> km<inline-formula><mml:math id="M2219" display="inline"><mml:msup><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msup></mml:math></inline-formula>) from ETOPO1
(Amante and Eakins, 2009; Eakins and Sharman, 2010). In products where the
covered area varies with time (e.g. CMEMS-LSCE-FFNN) we use the maximum
area coverage. The lowest coverage is 93 % (NIES-NN), resulting in a
maximum adjustment factor of 1.08 (Table A3, Hauck et al., 2020).</p>
      <p id="d1e34340">We further use results from two diagnostic ocean models, Khatiwala et al. (2013) and DeVries (2014), to estimate the anthropogenic carbon accumulated
in the ocean prior to 1959. The two approaches assume constant ocean
circulation and biological fluxes, with <inline-formula><mml:math id="M2220" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimated as a response
in the change in atmospheric CO<inline-formula><mml:math id="M2221" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration calibrated to
observations. The uncertainty in cumulative uptake of <inline-formula><mml:math id="M2222" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>20 GtC
(converted to <inline-formula><mml:math id="M2223" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 1<inline-formula><mml:math id="M2224" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>) is taken directly from the IPCC's review
of the literature (Rhein et al., 2013), or about <inline-formula><mml:math id="M2225" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>30 % for the
annual values (Khatiwala et al., 2009).</p>
</sec>
<sec id="App1.Ch1.S3.SS3.SSS2">
  <label>C3.2</label><title>Global ocean biogeochemistry models (GOBMs)</title>
      <p id="d1e34400">The ocean CO<inline-formula><mml:math id="M2226" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink for 1959–2019 is estimated using eight GOBMs (Table A2). The GOBMs represent the physical, chemical, and biological processes
that influence the surface ocean concentration of CO<inline-formula><mml:math id="M2227" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and thus the
air–sea CO<inline-formula><mml:math id="M2228" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux. The GOBMs are forced by meteorological reanalysis and
atmospheric CO<inline-formula><mml:math id="M2229" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration data available for the entire time
period. They mostly differ in the source of the atmospheric forcing data
(meteorological reanalysis), spin-up strategies, and in their horizontal and
vertical resolutions (Table A2). All GOBMs except one (CESM-ETHZ) do not
include the effects of anthropogenic changes in nutrient supply (Duce et
al., 2008). They also do not include the perturbation associated with
changes in riverine organic carbon (see Sect. 2.7.3).</p>
      <p id="d1e34439">Three sets of simulations were performed with each of the GOBMs. Simulation
A applied historical changes in climate and atmospheric CO<inline-formula><mml:math id="M2230" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration. Simulation B is a control simulation with constant
atmospheric forcing (normal-year or repeated-year forcing) and constant
pre-industrial atmospheric CO<inline-formula><mml:math id="M2231" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration. Simulation C is forced
with historical changes in atmospheric CO<inline-formula><mml:math id="M2232" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration, but repeated
year or normal-year atmospheric climate forcing. To derive <inline-formula><mml:math id="M2233" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> from
the model simulations, we subtracted the annual time series of the control
simulation B from the annual time series of simulation A. Assuming that
drift and bias are the same in simulations A and B, we thereby correct for
any model drift. Further, this difference also removes the natural steady-state flux (assumed to be 0 GtC yr<inline-formula><mml:math id="M2234" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> globally without rivers) which is
often a major source of biases. Simulation B of IPSL had to be treated
differently as it was forced with constant atmospheric CO<inline-formula><mml:math id="M2235" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> but observed
historical changes in climate. For IPSL, we fitted a linear trend to the
simulation B and subtracted this linear trend from simulation A. This
approach assures that the interannual variability is not removed from IPSL
simulation A.</p>
      <p id="d1e34502">The absolute correction for bias and drift per model in the 1990s varied
between <inline-formula><mml:math id="M2236" display="inline"><mml:mo>&lt;</mml:mo></mml:math></inline-formula> 0.01 and 0.26 GtC yr<inline-formula><mml:math id="M2237" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, with six models
having positive biases, and one model having essentially no bias (NorESM).
The remaining model (MPI) uses riverine input and therefore simulates
outgassing in simulation B, i.e. a seemingly negative bias. By subtracting
simulation B, the ocean carbon sink of the MPI model also follows the
definition of <inline-formula><mml:math id="M2238" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. This correction reduces the model mean ocean
carbon sink by 0.03 GtC yr<inline-formula><mml:math id="M2239" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> in the 1990s. The ocean models cover
99 % to 101 % of the total ocean area, so that area scaling is not
necessary.</p>
</sec>
<sec id="App1.Ch1.S3.SS3.SSS3">
  <label>C3.3</label><?xmltex \opttitle{GOBM evaluation and uncertainty assessment for $S_{{\mathrm{OCEAN}}}$}?><title>GOBM evaluation and uncertainty assessment for <inline-formula><mml:math id="M2240" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></title>
      <p id="d1e34566">The ocean CO<inline-formula><mml:math id="M2241" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink for all GOBMs and the ensemble mean falls within
90 % confidence of the observed range, or 1.5 to 2.9 GtC yr<inline-formula><mml:math id="M2242" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the
1990s (Ciais et al., 2013) after applying adjustments. An exception is the
MPI model, which simulates a low ocean carbon sink of 1.38 GtC yr<inline-formula><mml:math id="M2243" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for
the 1990s in simulation A owing to the inclusion of riverine carbon flux.
After adjusting to the GCB's definition of <inline-formula><mml:math id="M2244" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> by subtracting
simulation B, the MPI model falls into the observed range with an estimated
sink of 1.69 GtC yr<inline-formula><mml:math id="M2245" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p>
      <p id="d1e34625">The GOBMs and data products have been further evaluated using the fugacity
of sea surface CO<inline-formula><mml:math id="M2246" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math id="M2247" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2248" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>) from the SOCAT v2021 database (Bakker et
al., 2016, 2021). We focused this evaluation on the root mean squared error
(RMSE) between observed and modelled <inline-formula><mml:math id="M2249" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2250" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> and on a measure of the
amplitude of the interannual variability of the flux (modified after
Rödenbeck et al., 2015). The RMSE is calculated from detrended annually
and regionally averaged time series calculated from GOBMs and data product
<inline-formula><mml:math id="M2251" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2252" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> subsampled to open ocean (water depth <inline-formula><mml:math id="M2253" display="inline"><mml:mo>&gt;</mml:mo></mml:math></inline-formula> 400 m) SOCAT
sampling points to measure the misfit between large-scale signals (Hauck et
al., 2020) The amplitude of the <inline-formula><mml:math id="M2254" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> interannual variability (A-IAV)
is calculated as the temporal standard deviation of the detrended CO<inline-formula><mml:math id="M2255" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
flux time series (Rödenbeck et al., 2015; Hauck et al., 2020). These
metrics are chosen because RMSE is the most direct measure of data–model
mismatch and the A-IAV is a direct measure of the variability of <inline-formula><mml:math id="M2256" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
on interannual timescales. We apply these metrics globally and by latitude
bands. Results are shown in Fig. B2 and discussed in Sect. 3.5.5.</p>
      <p id="d1e34724">We quantify the 1<inline-formula><mml:math id="M2257" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> uncertainty around the mean ocean sink of
anthropogenic CO<inline-formula><mml:math id="M2258" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> by assessing random and systematic uncertainties for
the GOBMs and data products. The random uncertainties are taken from the
ensemble standard deviation (0.3 GtC yr<inline-formula><mml:math id="M2259" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for GOBMs, 0.3 GtC yr<inline-formula><mml:math id="M2260" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for data products). We derive the GOBMs' systematic uncertainty
by the deviation of the DIC inventory change 1994–2007 from the Gruber et al. (2019) estimate (0.5 GtC yr<inline-formula><mml:math id="M2261" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) and suggest these are related to
physical transport (mixing, advection) into the ocean interior. For the
data products, we consider systematic uncertainties stemming from
uncertainty in <inline-formula><mml:math id="M2262" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2263" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> observations (0.2 GtC yr<inline-formula><mml:math id="M2264" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Takahashi et
al., 2009; Wanninkhof et al., 2013), gas-transfer velocity (0.2 GtC yr<inline-formula><mml:math id="M2265" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Ho et al., 2011; Wanninkhof et al., 2013; Roobaert et al.,
2018), wind product (0.1 GtC yr<inline-formula><mml:math id="M2266" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Fay et al., 2021), river flux
adjustment (0.2 GtC yr<inline-formula><mml:math id="M2267" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Jacobson et al., 2007; Resplandy et al.,
2018), and <inline-formula><mml:math id="M2268" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2269" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> mapping (0.2 GtC yr<inline-formula><mml:math id="M2270" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Landschützer et al.,
2014). Combining these uncertainties as their squared sums, we assign an
uncertainty of <inline-formula><mml:math id="M2271" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.6 GtC yr<inline-formula><mml:math id="M2272" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to the GOBMs ensemble mean and an
uncertainty of <inline-formula><mml:math id="M2273" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.5 GtC yr<inline-formula><mml:math id="M2274" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to the data-product ensemble
mean. These uncertainties are propagated as <inline-formula><mml:math id="M2275" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula>(<inline-formula><mml:math id="M2276" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub><mml:mo>)</mml:mo><mml:mo>=</mml:mo><mml:mo>(</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:msup><mml:mn mathvariant="normal">2</mml:mn><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">0.6</mml:mn><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>+</mml:mo><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:msup><mml:mn mathvariant="normal">2</mml:mn><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:mo>×</mml:mo><mml:msup><mml:mn mathvariant="normal">0.5</mml:mn><mml:mn mathvariant="normal">2</mml:mn></mml:msup><mml:msup><mml:mo>)</mml:mo><mml:mrow><mml:mn mathvariant="normal">1</mml:mn><mml:mo>/</mml:mo><mml:mn mathvariant="normal">2</mml:mn></mml:mrow></mml:msup></mml:mrow></mml:math></inline-formula> GtC yr<inline-formula><mml:math id="M2277" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and
result in an <inline-formula><mml:math id="M2278" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.4 GtC yr<inline-formula><mml:math id="M2279" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> uncertainty around the best
estimate of <inline-formula><mml:math id="M2280" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>.</p>
      <p id="d1e35025">We examine the consistency between the variability of the model-based and
the <inline-formula><mml:math id="M2281" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2282" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products to assess confidence in <inline-formula><mml:math id="M2283" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>. The
interannual variability of the ocean fluxes (quantified as A-IAV, the
standard deviation after detrending, Fig. B2) of the seven <inline-formula><mml:math id="M2284" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2285" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based
data products plus the Watson et al. (2020) product for 1990–2020 ranges
from 0.16 to 0.26 GtC yr<inline-formula><mml:math id="M2286" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> with the lower estimates by the three
ensemble methods (CSIR-ML6, CMEMS-LSCE-FFNN, OS-ETHZ-GRaCER). The
inter-annual variability in the GOBMs ranges between 0.10 and 0.19 GtC yr<inline-formula><mml:math id="M2287" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>; hence there is overlap with the lower A-IAV estimates of three
data products.</p>
      <p id="d1e35096">Individual estimates (both GOBMs and data products) generally produce a
higher ocean CO<inline-formula><mml:math id="M2288" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink during strong El Niño events. There is
emerging agreement between GOBMs and data products on the patterns of
decadal variability of <inline-formula><mml:math id="M2289" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> with a global stagnation in the 1990s and
an extra-tropical strengthening in the 2000s (McKinley et al., 2020; Hauck
et al., 2020). The central estimates of the annual flux from the GOBMs and
the <inline-formula><mml:math id="M2290" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2291" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based data products have a correlation <inline-formula><mml:math id="M2292" display="inline"><mml:mi>r</mml:mi></mml:math></inline-formula> of 0.94 (1990–2020).
The agreement between the models and the data products reflects some
consistency in their representation of underlying variability since there is
little overlap in their methodology or use of observations.</p>
</sec>
</sec>
<sec id="App1.Ch1.S3.SS4">
  <label>C4</label><?xmltex \opttitle{Methodology land CO${}_{{{2}}}$ sink ($S_{\mathrm{LAND}}$)}?><title>Methodology land CO<inline-formula><mml:math id="M2293" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (<inline-formula><mml:math id="M2294" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>)</title>
<sec id="App1.Ch1.S3.SS4.SSS1">
  <label>C4.1</label><title>DGVM simulations</title>
      <p id="d1e35179">The DGVM runs were forced by either the merged monthly Climate
Research Unit (CRU) and 6-hourly Japanese 55-year Reanalysis (JRA-55) dataset or by the monthly CRU dataset, both providing observation-based
temperature, precipitation, and incoming surface radiation on a
0.5<inline-formula><mml:math id="M2295" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> <inline-formula><mml:math id="M2296" display="inline"><mml:mo>×</mml:mo></mml:math></inline-formula> 0.5<inline-formula><mml:math id="M2297" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> grid and updated to 2020 (Harris et al.,
2014, 2020). The combination of CRU monthly data with 6-hourly forcing from
JRA-55 (Kobayashi et al., 2015) is performed with methodology used in
previous years (Viovy, 2016) adapted to the specifics of the JRA-55 data.</p>
      <p id="d1e35207">New to this budget is the revision of incoming short-wave radiation fields
to take into account aerosol impacts and the division of total radiation
into direct and diffuse components as summarized below.</p>
      <p id="d1e35210">The diffuse fraction dataset offers 6-hourly distributions of the diffuse
fraction of surface shortwave fluxes over the period 1901–2020. Radiative
transfer calculations are based on monthly-averaged distributions of
tropospheric and stratospheric aerosol optical depth and 6-hourly
distributions of cloud fraction. Methods follow those described in the
Methods section of Mercado et al. (2009), but with updated input datasets.</p>
      <p id="d1e35213">The time series of speciated tropospheric aerosol optical depth is taken
from the historical and RCP8.5 simulations by the HadGEM2-ES climate model
(Bellouin et al., 2011). To correct for biases in HadGEM2-ES, tropospheric
aerosol optical depths are scaled over the whole period to match the global
and monthly averages obtained over the period 2003–2020 by the CAMS
Reanalysis of atmospheric composition (Inness et al., 2019), which
assimilates satellite retrievals of aerosol optical depth.</p>
      <p id="d1e35217">The time series of stratospheric aerosol optical depth is taken from the
Sato et al. (1993) climatology, which has been updated to 2012. Years
2013–2020 are assumed to be background years and so replicate the background
year 2010. That assumption is supported by the Global Space-based
Stratospheric Aerosol Climatology time series (1979–2016; Thomason et al.,
2018). The time series of cloud fraction is obtained by scaling the 6-hourly
distributions simulated in the Japanese Reanalysis (Kobayashi et al., 2015)
to match the monthly-averaged cloud cover in the CRU TS v4.03 dataset
(Harris et al., 2021). Surface radiative fluxes account for
aerosol–radiation interactions from both tropospheric and stratospheric
aerosols, and for aerosol–cloud interactions from tropospheric aerosols,
except mineral dust. Tropospheric aerosols are also assumed to exert
interactions with clouds.</p>
      <p id="d1e35220">The radiative effects of those aerosol–cloud interactions are assumed to
scale with the radiative effects of aerosol–radiation interactions of
tropospheric aerosols, using regional scaling factors derived from
HadGEM2-ES. Diffuse fraction is assumed to be 1 in cloudy sky conditions. Atmospheric
constituents other than aerosols and clouds are set to a constant standard
mid-latitude summer atmosphere, but their variations do not affect the
diffuse fraction of surface shortwave fluxes.</p>
      <p id="d1e35223">In summary, the DGVM forcing data include time-dependent gridded climate
forcing, global atmospheric CO<inline-formula><mml:math id="M2298" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (Dlugokencky and Tans, 2022), gridded
land-cover changes (see Appendix C2.2), and gridded nitrogen deposition and
fertilizers (see Table A1 for specific models details).</p>
      <p id="d1e35235">Four simulations were performed with each of the DGVMs. Simulation 0 (S0) is
a control simulation which uses fixed pre-industrial (year 1700) atmospheric
CO<inline-formula><mml:math id="M2299" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations, cycles early 20th century (1901–1920) climate, and
applies a time-invariant pre-industrial land-cover distribution and
pre-industrial wood harvest rates. Simulation 1 (S1) differs from S0 by
applying historical changes in atmospheric CO<inline-formula><mml:math id="M2300" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentration and N inputs.
Simulation 2 (S2) applies historical changes in atmospheric CO<inline-formula><mml:math id="M2301" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration, N inputs, and climate, while applying time-invariant
pre-industrial land-cover distribution and pre-industrial wood harvest
rates. Simulation 3 (S3) applies historical changes in atmospheric CO<inline-formula><mml:math id="M2302" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration, N inputs, climate, and land-cover distribution and wood
harvest rates.</p>
      <p id="d1e35274">S2 is used to estimate the land sink component of the global carbon budget
(<inline-formula><mml:math id="M2303" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>). S3 is used to estimate the total land flux but is not used in
the global carbon budget. We further separate <inline-formula><mml:math id="M2304" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> into contributions
from CO<inline-formula><mml:math id="M2305" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> (<inline-formula><mml:math id="M2306" display="inline"><mml:mo lspace="0mm">=</mml:mo></mml:math></inline-formula> S1 <inline-formula><mml:math id="M2307" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> S0) and climate (<inline-formula><mml:math id="M2308" display="inline"><mml:mo lspace="0mm">=</mml:mo></mml:math></inline-formula> S2 <inline-formula><mml:math id="M2309" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> S1 <inline-formula><mml:math id="M2310" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> S0).</p>
</sec>
<sec id="App1.Ch1.S3.SS4.SSS2">
  <label>C4.2</label><?xmltex \opttitle{DGVM evaluation and uncertainty assessment for $S_{{\mathrm{LAND}}}$}?><title>DGVM evaluation and uncertainty assessment for <inline-formula><mml:math id="M2311" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula></title>
      <p id="d1e35363">We apply three criteria for minimum DGVM realism by including only those
DGVMs with (1) steady state after spin-up; (2) global net land flux
(<inline-formula><mml:math id="M2312" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> <inline-formula><mml:math id="M2313" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula> <inline-formula><mml:math id="M2314" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>) that is an atmosphere-to-land carbon flux over the
1990s ranging between <inline-formula><mml:math id="M2315" display="inline"><mml:mo>-</mml:mo></mml:math></inline-formula>0.3 and 2.3 GtC yr<inline-formula><mml:math id="M2316" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, within 90 % confidence
of constraints by global atmospheric and oceanic observations (Keeling and
Manning, 2014; Wanninkhof et al., 2013); and (3) global <inline-formula><mml:math id="M2317" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> that is a
carbon source to the atmosphere over the 1990s, as already mentioned in
Sect. C2.2. All 17 DGVMs meet these three criteria.</p>
      <p id="d1e35426">In addition, the DGVM results are also evaluated using the International
Land Model Benchmarking system (ILAMB; Collier et al., 2018). This
evaluation is provided here to document, encourage, and support model
improvements through time. ILAMB variables cover key processes that are
relevant for the quantification of <inline-formula><mml:math id="M2318" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and resulting aggregated
outcomes. The selected variables are vegetation biomass, gross primary
productivity, leaf area index, net ecosystem exchange, ecosystem
respiration, evapotranspiration, soil carbon, and runoff (see Fig. B3 for
the results and for the list of observed databases). Results are shown in
Fig. B3 and discussed in Sect. 3.6.5.</p>
      <p id="d1e35440">For the uncertainty for <inline-formula><mml:math id="M2319" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, we use the standard deviation of the
annual CO<inline-formula><mml:math id="M2320" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink across the DGVMs, averaging to about <inline-formula><mml:math id="M2321" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.6 GtC yr<inline-formula><mml:math id="M2322" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the period 1959 to 2019. We attach a medium confidence level
to the annual land CO<inline-formula><mml:math id="M2323" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink and its uncertainty because the estimates
from the residual budget and averaged DGVMs match well within their
respective uncertainties (Table 5).</p>
</sec>
</sec>
<sec id="App1.Ch1.S3.SS5">
  <label>C5</label><title>Methodology atmospheric inversions</title>
      <p id="d1e35501">Six atmospheric inversions (details of each in Table A4) were used to infer
the spatio-temporal distribution of the CO<inline-formula><mml:math id="M2324" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> flux exchanged between the
atmosphere and the land or oceans. These inversions are based on Bayesian
inversion principles with prior information on fluxes and their
uncertainties. They use very similar sets of surface measurements of
CO<inline-formula><mml:math id="M2325" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> time series (or subsets thereof) from various flask and in situ
networks. One inversion system also used satellite xCO<inline-formula><mml:math id="M2326" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> retrievals from
GOSAT and OCO-2.</p>
      <p id="d1e35531">Each inversion system uses different methodologies and input data but is
rooted in Bayesian inversion principles. These differences mainly concern
the selection of atmospheric CO<inline-formula><mml:math id="M2327" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data and prior fluxes, as well as the
spatial resolution, assumed correlation structures, and mathematical
approach of the models. Each system uses a different transport model, which
was demonstrated to be a driving factor behind differences in atmospheric
inversion-based flux estimates, and specifically their distribution across
latitudinal bands (Gaubert et al., 2019; Schuh et al., 2019).</p>
      <p id="d1e35543">The inversion systems prescribe same global fossil fuel emissions for
<inline-formula><mml:math id="M2328" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, specifically the GCP's Gridded Fossil Emissions Dataset version
2021 (GCP-GridFEDv2021.2; Jones et al., 2021b), which is an update through
2020 of the first version of GCP-GridFED presented by Jones et al. (2021a).
GCP-GridFEDv2021.2 scales gridded estimates of CO<inline-formula><mml:math id="M2329" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from
EDGARv4.3.2 (Janssens-Maenhout et al., 2019) within national territories to
match national emissions estimates provided by the GCP for the years
1959–2020, which were compiled following the methodology described in
Appendix C1 based on all information available on 31 July 2021 (Robbie Andrew, personal communication, 2021). Typically, the GCP-GridFED adopts the seasonal variation in
emissions (the monthly distribution of annual emissions) from EDGAR and
applies small corrections based on heating or cooling degree days to account
for the effects of inter-annual climate variability on the seasonality
emissions (Jones et al., 2021a). However, strategies taken to deal with the
COVID-19 pandemic during 2020 mean that the seasonality of emissions
diverged substantially in 2020 from a typical year. To account for this
change, GCP-GridFEDv2021.2 adopts the national seasonality in emissions from
Carbon Monitor (Liu et al., 2020a, b) during the years 2019–2020 (Jones et al., 2021b).</p>
      <p id="d1e35566">The consistent use of GCP-GridFEDv2021.2 for <inline-formula><mml:math id="M2330" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> ensures a close
alignment with the estimate of <inline-formula><mml:math id="M2331" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> used in this budget assessment,
enhancing the comparability of the inversion-based estimate with the flux
estimates deriving from DGVMs, GOBMs, and <inline-formula><mml:math id="M2332" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2333" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>-based methods. To account
for small differences in regridding, and the use of a slightly earlier file
version (GCP-GridFEDv2021.1) for 2000–2018 in CarbonTracker Europe, small
fossil fuel corrections were applied to all inverse models to make the
estimated uptake of atmospheric CO<inline-formula><mml:math id="M2334" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fully consistent. Finally, we note that
GCP-GridFEDv2021.2 includes emissions from cement production, but it does
not include the cement carbonation CO<inline-formula><mml:math id="M2335" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink (Xi et al., 2016; Cao et
al., 2020; Guo et al., 2021) that is applied to the GCB estimate of <inline-formula><mml:math id="M2336" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>
in Table 6.</p>
      <p id="d1e35638">The land and ocean CO<inline-formula><mml:math id="M2337" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes from atmospheric inversions contain
anthropogenic perturbation and natural pre-industrial CO<inline-formula><mml:math id="M2338" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes. On
annual timescales, natural pre-industrial fluxes are primarily land
CO<inline-formula><mml:math id="M2339" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sinks and ocean CO<inline-formula><mml:math id="M2340" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sources corresponding to carbon taken up
on land, transported by rivers from land to ocean, and outgassed by the
ocean. These pre-industrial land CO<inline-formula><mml:math id="M2341" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sinks are thus compensated over
the globe by ocean CO<inline-formula><mml:math id="M2342" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sources corresponding to the outgassing of
riverine carbon inputs to the ocean, using the exact same numbers and
distribution as described for the oceans in Sect. 2.4. To facilitate the
comparison, we adjusted the inverse estimates of the land and ocean fluxes
per latitude band with these numbers to produce historical perturbation
CO<inline-formula><mml:math id="M2343" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes from inversions. Finally, for the presentation of the
comparison in Fig. 11 we modified the fossil-fuel-corrected and riverine-adjusted
land sinks from the inversions further, by removing a 0.2 GtC yr<inline-formula><mml:math id="M2344" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>
CO<inline-formula><mml:math id="M2345" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> sink that is ascribed to cement carbonation in the GCB, rather than
to terrestrial ecosystems. The latter is not applied in the inversion
products released through GCB or the original data portals of these
products.</p>
      <p id="d1e35726">All participating atmospheric inversions are checked for consistency with
the annual global growth rate, as both are derived from the global surface
network of atmospheric CO<inline-formula><mml:math id="M2346" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> observations. In this exercise, we use the
conversion factor of 2.086 GtC ppm<inline-formula><mml:math id="M2347" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> to convert the inverted carbon fluxes to
mole fractions, as suggested by Prather (2012). This number is specifically
suited for the comparison to surface observations that do not respond
uniformly, nor immediately, to each year's summed sources and sinks. This
factor is therefore slightly smaller than the GCB conversion factor in Table 1 (2.142 GtC ppm<inline-formula><mml:math id="M2348" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>, Ballantyne et al., 2012). Overall, the inversions agree
with the growth rate with biases between 0.03–0.08 ppm (0.06–0.17 GtC yr<inline-formula><mml:math id="M2349" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>) on the decadal average.</p>
      <p id="d1e35774">The atmospheric inversions are also evaluated using vertical profiles of
atmospheric CO<inline-formula><mml:math id="M2350" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> concentrations (Fig. B4). More than 30 aircraft
programmes over the globe, either regular programmes or repeated surveys over at
least 9 months, have been used in order to draw a robust picture of the
model performance (with space–time data coverage irregular and denser in the
0–45<inline-formula><mml:math id="M2351" display="inline"><mml:msup><mml:mi/><mml:mo>∘</mml:mo></mml:msup></mml:math></inline-formula> N latitude band; Table A6). The six models are compared to
the independent aircraft CO<inline-formula><mml:math id="M2352" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements between 2 and 7 km above sea
level between 2001 and 2020. Results are shown in Fig. B4, where the
inversions generally match the atmospheric mole fractions to within 0.6 ppm
at all latitudes, except for CarbonTracker Europe in 2010–2020 over the more sparsely
sampled Southern Hemisphere.</p>
</sec>
</app>

<app id="App1.Ch1.S4">
  <?xmltex \currentcnt{D}?><label>Appendix D</label><title>Processes not included in the global carbon budget </title>
<sec id="App1.Ch1.S4.SS1">
  <label>D1</label><?xmltex \opttitle{Contribution of anthropogenic CO and CH${}_{{{4}}}$ to the
global carbon budget}?><title>Contribution of anthropogenic CO and CH<inline-formula><mml:math id="M2353" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> to the
global carbon budget</title>
      <p id="d1e35830">Equation (1) includes only partly the net input of CO<inline-formula><mml:math id="M2354" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> to the
atmosphere from the chemical oxidation of reactive carbon-containing gases
from sources other than the combustion of fossil fuels, such as (1) cement
process emissions, since these do not come from combustion of fossil fuels;
(2) the oxidation of fossil fuels; and (3) the assumption of immediate oxidation
of vented methane in oil production. However, it omits any other
anthropogenic carbon-containing gases that are eventually oxidized in the
atmosphere, such as anthropogenic emissions of CO and CH<inline-formula><mml:math id="M2355" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula>. An attempt
is made in this section to estimate their magnitude and identify the sources
of uncertainty. Anthropogenic CO emissions are from incomplete fossil fuel
and biofuel burning and deforestation fires. The main anthropogenic
emissions of fossil CH<inline-formula><mml:math id="M2356" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> that matter for the global (anthropogenic)
carbon budget are the fugitive emissions of coal, oil, and gas sectors (see
below). These emissions of CO and CH<inline-formula><mml:math id="M2357" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> contribute a net addition of
fossil carbon to the atmosphere.</p>
      <p id="d1e35869">In our estimate of <inline-formula><mml:math id="M2358" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> we assumed (Sect. 2.1.1) that all the fuel
burned is emitted as CO<inline-formula><mml:math id="M2359" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>, thus CO anthropogenic emissions associated
with incomplete fossil fuel combustion and its atmospheric oxidation into
CO<inline-formula><mml:math id="M2360" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> within a few months are already counted implicitly in <inline-formula><mml:math id="M2361" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and
should not be counted twice (same for <inline-formula><mml:math id="M2362" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and anthropogenic CO
emissions by deforestation fires). Anthropogenic emissions of fossil
CH<inline-formula><mml:math id="M2363" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> are, however, not included in <inline-formula><mml:math id="M2364" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, because these fugitive
emissions are not included in the fuel inventories. Yet they contribute to
the annual CO<inline-formula><mml:math id="M2365" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth rate after CH<inline-formula><mml:math id="M2366" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> gets oxidized into
CO<inline-formula><mml:math id="M2367" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>. Emissions of fossil CH<inline-formula><mml:math id="M2368" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> represent 30 % of total
anthropogenic CH<inline-formula><mml:math id="M2369" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> emissions (Saunois et al., 2020; their top-down
estimate is used because it is consistent with the observed CH<inline-formula><mml:math id="M2370" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> growth
rate), that is 0.083 GtC yr<inline-formula><mml:math id="M2371" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> for the decade 2008–2017. Assuming steady
state, an amount equal to this fossil CH<inline-formula><mml:math id="M2372" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> emission is all converted to
CO<inline-formula><mml:math id="M2373" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> by OH oxidation, thus explaining 0.083 GtC yr<inline-formula><mml:math id="M2374" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> of the global
CO<inline-formula><mml:math id="M2375" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth rate with an uncertainty range of 0.061 to 0.098 GtC yr<inline-formula><mml:math id="M2376" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>  taken from the min–max of top-down estimates in Saunois et al. (2020). If this min–max range is assumed to be 2<inline-formula><mml:math id="M2377" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> because Saunois
et al. (2020) did not account for the internal uncertainty of their min and
max top-down estimates, it translates into a 1<inline-formula><mml:math id="M2378" display="inline"><mml:mi mathvariant="italic">σ</mml:mi></mml:math></inline-formula> uncertainty of
0.019 GtC yr<inline-formula><mml:math id="M2379" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>.</p>
      <p id="d1e36089">Other anthropogenic changes in the sources of CO and CH<inline-formula><mml:math id="M2380" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> from
wildfires, vegetation biomass, wetlands, ruminants, or permafrost changes
are similarly assumed to have a small effect on the CO<inline-formula><mml:math id="M2381" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth rate.
The CH<inline-formula><mml:math id="M2382" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">4</mml:mn></mml:msub></mml:math></inline-formula> and CO emissions and sinks are published and analysed
separately in the Global Methane Budget and Global Carbon Monoxide Budget
publications, which follow a similar approach to that presented here
(Saunois et al., 2020; Zheng et al., 2019).</p>
</sec>
<sec id="App1.Ch1.S4.SS2">
  <label>D2</label><?xmltex \opttitle{Contribution of other carbonates to CO${}_{{{2}}}$ emissions}?><title>Contribution of other carbonates to CO<inline-formula><mml:math id="M2383" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions</title>
      <p id="d1e36137">Although we do account for cement carbonation (a carbon sink), the
contribution of emissions of fossil carbonates (carbon sources) other than
cement production is not systematically included in estimates of <inline-formula><mml:math id="M2384" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>,
except at the national level where they are accounted for in the UNFCCC
national inventories. The missing processes include CO<inline-formula><mml:math id="M2385" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions
associated with the calcination of lime and limestone outside cement
production. Carbonates are also used in various industries, including in
iron and steel manufacture and in agriculture. They are found naturally in
some coals. CO<inline-formula><mml:math id="M2386" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> emissions from fossil carbonates other than cement are
estimated to amount to about 1 % of <inline-formula><mml:math id="M2387" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">FOS</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> (Crippa et al., 2019),
though some of these carbonate emissions are included in our estimates
(e.g. via UNFCCC inventories).</p>
</sec>
<sec id="App1.Ch1.S4.SS3">
  <label>D3</label><title>Anthropogenic carbon fluxes in the land-to-ocean aquatic
continuum</title>
      <p id="d1e36188">The approach used to determine the global carbon budget refers to the mean,
variations, and trends in the perturbation of CO<inline-formula><mml:math id="M2388" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> in the atmosphere,
referenced to the pre-industrial era. Carbon is continuously displaced from
the land to the ocean through the land–ocean aquatic continuum (LOAC)
comprising freshwaters, estuaries, and coastal areas (Bauer et al., 2013;
Regnier et al., 2013). A substantial fraction of this lateral carbon flux is
entirely “natural” and is thus a steady-state component of the
pre-industrial carbon cycle. We account for this pre-industrial flux where
appropriate in our study (see Appendix C3). However, changes in
environmental conditions and land-use change have caused an increase in the
lateral transport of carbon into the LOAC – a perturbation that is relevant
for the global carbon budget presented here.</p>
      <p id="d1e36200">The results of the analysis of Regnier et al. (2013) can be summarized in
two points of relevance for the anthropogenic CO<inline-formula><mml:math id="M2389" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> budget. First, the
anthropogenic perturbation of the LOAC has increased the organic carbon
export from terrestrial ecosystems to the hydrosphere by as much as 1.0
<inline-formula><mml:math id="M2390" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula>0.5 GtC yr<inline-formula><mml:math id="M2391" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> since pre-industrial times, mainly owing to
enhanced carbon export from soils. Second, this exported anthropogenic
carbon is partly respired through the LOAC, partly sequestered in sediments
along the LOAC, and to a lesser extent transferred to the open ocean where
it may accumulate or be outgassed. The increase in storage of land-derived
organic carbon in the LOAC carbon reservoirs (burial) and in the open ocean
combined is estimated by Regnier et al. (2013) at 0.65 <inline-formula><mml:math id="M2392" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.35 GtC yr<inline-formula><mml:math id="M2393" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula>. The inclusion of LOAC-related anthropogenic CO<inline-formula><mml:math id="M2394" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes
should affect estimates of <inline-formula><mml:math id="M2395" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">LAND</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> and <inline-formula><mml:math id="M2396" display="inline"><mml:mrow><mml:msub><mml:mi>S</mml:mi><mml:mi mathvariant="normal">OCEAN</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> in Eq. (1) but does
not affect the other terms. Representation of the anthropogenic perturbation
of LOAC CO<inline-formula><mml:math id="M2397" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> fluxes is, however, not included in the GOBMs and DGVMs used
in our global carbon budget analysis presented here.</p>
</sec>
<sec id="App1.Ch1.S4.SS4">
  <label>D4</label><title>Loss of additional land sink capacity</title>
      <p id="d1e36299">Historical land-cover change was dominated by transitions from vegetation
types that can provide a large carbon sink per area unit (typically,
forests) to others less efficient in removing CO<inline-formula><mml:math id="M2398" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> from the atmosphere
(typically, croplands). The resultant decrease in land sink, called the
“loss of additional sink capacity”, can be calculated as the difference
between the actual land sink under changing land cover and the
counterfactual land sink under pre-industrial land cover. This term is not
accounted for in our global carbon budget estimate. Here, we provide a
quantitative estimate of this term to be used in the discussion. Seven of
the DGVMs used in Friedlingstein et al. (2019) performed additional
simulations with and without land-use change under cycled pre-industrial
environmental conditions. The resulting loss of additional sink capacity
amounts to 0.9 <inline-formula><mml:math id="M2399" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.3 GtC yr<inline-formula><mml:math id="M2400" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> on average over 2009–2018 and 42 <inline-formula><mml:math id="M2401" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 16 GtC accumulated between 1850 and 2018 (Obermeier et al., 2021).
OSCAR, emulating the behaviour of 11 DGVMs, finds values of the loss of
additional sink capacity of 0.7 <inline-formula><mml:math id="M2402" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 0.6 GtC yr<inline-formula><mml:math id="M2403" display="inline"><mml:msup><mml:mi/><mml:mrow><mml:mo>-</mml:mo><mml:mn mathvariant="normal">1</mml:mn></mml:mrow></mml:msup></mml:math></inline-formula> and 31 <inline-formula><mml:math id="M2404" display="inline"><mml:mo>±</mml:mo></mml:math></inline-formula> 23 GtC for the same time period (Gasser et al., 2020). Since the DGVM-based
<inline-formula><mml:math id="M2405" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula> estimates are only used to quantify the uncertainty around the
bookkeeping models' <inline-formula><mml:math id="M2406" display="inline"><mml:mrow><mml:msub><mml:mi>E</mml:mi><mml:mi mathvariant="normal">LUC</mml:mi></mml:msub></mml:mrow></mml:math></inline-formula>, we do not add the loss of additional sink capacity
to the bookkeeping estimate.</p>
</sec>
</app>
  </app-group><notes notes-type="authorcontribution"><title>Author contributions</title>

      <p id="d1e36391">PF, MWJ, MOS, CLQ, RMA, DCEB, JH, GPP, WP, JP, and SS designed the study,
conducted the analysis, and wrote the paper with input from JGC, PC, and RBJ.
RMA, GPP, and JIK produced the fossil fuel emissions and their uncertainties
and analysed the emissions data. DG and GM provided fossil fuel emission
data. JP, TG, CS, and RAH provided the bookkeeping land-use change emissions.
JH, LB, OG, NG, TI, LR, JS, RS, and DW provided an update of the global ocean
biogeochemical models. SRA, TTTC, LD, LG, YI, PL, CR, AJW, and JZ provided an
update of the ocean <inline-formula><mml:math id="M2407" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2408" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data products, with synthesis by JH. MB, NRB,
KIC, MC, WE, RAF, SRA, TG, AK, NL, SKL, DRM, ClS, CoS, SN, CW, TO, DP, GR,
AJS, BT, TT, CW, and RW provided ocean <inline-formula><mml:math id="M2409" display="inline"><mml:mi>f</mml:mi></mml:math></inline-formula>CO<inline-formula><mml:math id="M2410" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements for the year
2020, with synthesis by DCEB and SDJ. PA, BD, AKJ, DK, EK, JK, SL, PCM, JRM,
JEMSN, BP, HT, NV, AJW, WY, XY, and SZ provided an update of the dynamic
global vegetation models, with synthesis by SS. WP, FC, LF, ITL, JL, YN, and
CR provided an updated atmospheric inversion, developed the protocol, and
produced the evaluation, with synthesis by WP. RMA provided predictions of
the 2021 emissions and atmospheric CO<inline-formula><mml:math id="M2411" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> growth rate. PL provided the
predictions of the 2021 ocean and land sinks. LPC, GCH, KKG, TMS, and GRvdW
provided forcing data for land-use change. GG, FT, and CY provided data for
the land-use change NGHGI mapping. PPT provided key atmospheric CO<inline-formula><mml:math id="M2412" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
data. MWJ produced the historical record of atmospheric CO<inline-formula><mml:math id="M2413" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>
concentration and growth rate, including the atmospheric CO<inline-formula><mml:math id="M2414" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> forcing.
MOS and NB produced the aerosol diffuse radiative forcing for the DGVMs. IH
provided the climate forcing data for the DGVMs. ER provided the evaluation
of the DGVMs. MWJ provided the emissions prior for use in the inversion
models. XD provided seasonal emissions data for years 2019–2020 for the
emission prior. MWJ and MOS developed a new data management pipeline which
automates many aspects of the data collation, analysis, plotting, and
synthesis. PF, MWJ, and MOS revised all figures, tables, text, and/or numbers
to ensure the update was clear from the 2020 edition and in line with the Global Carbon Atlas (<uri>http://globalcarbonatlas.org</uri>, last access: 11 March 2022).</p>
  </notes><notes notes-type="competinginterests"><title>Competing interests</title>

      <p id="d1e36469">At least one of the (co-)authors is a member of the editorial board of <italic>Earth System Science Data</italic>. The peer-review process was guided by an independent editor, and the authors have also no other competing interests to declare.</p>
  </notes><notes notes-type="disclaimer"><title>Disclaimer</title>

      <p id="d1e36479">Publisher's note: Copernicus Publications remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.</p>
  </notes><ack><title>Acknowledgements</title><p id="d1e36485">We thank all people and institutions who provided the data used in this
global carbon budget 2021 and the Global Carbon Project members for their
input throughout the development of this publication. We thank Nigel Hawtin
for producing Figs. 2 and 13. We thank Omar Jamil and Freddy
Wordingham for technical support. We thank Ed Dlugokencky for providing
atmospheric CO<inline-formula><mml:math id="M2415" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> measurements. We thank Vivek Arora, Ian G. C. Ashton,
Erik Buitenhuis, Fatemeh Cheginig, Christian Ethé, Marion Gehlen,
Lonneke Goddijn-Murphy, Thomas Holding, Fabrice Lacroix, Enhui Liao, Pedro M. S.
Monteiro, Naiquing Pan, Tristan Quaife, Shijie Shu, Jamie D. Shutler, Jade
Skye, Anthony Walker, and David K. Woolf for their involvement in the
development, use, and analysis of the models and data products used here. We
thank Markus Ritschel, Carmen Rodriguez, Claire Lo Monaco, Nicolas Metzl,
Vassilis Kitidis, Sören Gutekunst, Anne Willstrand Wranne, Tobias
Steinhoff, Jessica N. Cross, Natalie M. Monacci, Alice Benoit-Cattin,
Sólveig R. Ólafsdóttir, Joe Salisbury, Doug Vandemark, and
Christopher W. Hunt, who contributed to the provision of surface ocean
CO<inline-formula><mml:math id="M2416" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> observations for the year 2020 (see Table A5). We also thank
Benjamin Pfeil, Rocío Castaño-Primo, Camilla Landa, and Maren
Karlsen of the Ocean Thematic Centre of the EU Integrated Carbon Observation
System (ICOS) Research Infrastructure; Kevin O'Brien and Eugene Burger of
NOAA's Pacific Marine Environmental Laboratory; and Alex Kozyr of NOAA's
National Centers for Environmental Information, for their contribution to
surface ocean CO<inline-formula><mml:math id="M2417" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data and metadata management. We thank the
scientists, institutions, and funding agencies responsible for the
collection and quality control of the data in SOCAT as well as the
International Ocean Carbon Coordination Project (IOCCP), the Surface Ocean
Lower Atmosphere Study (SOLAS), and the Integrated Marine Biosphere Research
(IMBeR) programme for their support. We thank data providers ObsPack
GLOBALVIEWplus v6.1 and NRT v6.1.1 for atmospheric CO<inline-formula><mml:math id="M2418" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> observations. We
thank the individuals and institutions that provided the databases used for
the models evaluations used here. We thank Fortunat Joos, Samar Khatiwala,
and Timothy DeVries for providing historical data. Nicolas Vuichard thanks the whole
ORCHIDEE group.  Yosuke Niwa thanks CSIRO, EC, EMPA, FMI, IPEN, JMA, LSCE, NCAR, NIES,
NILU, NIWA, NOAA, SIO, and TU/NIPR for providing data for NISMON-CO<inline-formula><mml:math id="M2419" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula>. We
thank Kevin Bowman (NASA JPL) for contribution to the CMS-Flux results.  Junjie Liu
thanks the Jet Propulsion Laboratory, California Institute of Technology.
This is PMEL contribution 5317. Steve D. Jones thanks the data management team at the
Bjerknes Climate Data Centre. Wiley Evans thanks the Tula Foundation for funding
support. Australian ocean CO<inline-formula><mml:math id="M2420" display="inline"><mml:msub><mml:mi/><mml:mn mathvariant="normal">2</mml:mn></mml:msub></mml:math></inline-formula> data were sourced from Australia's
Integrated Marine Observing System (IMOS); IMOS is enabled by the National
Collaborative Research Infrastructure Strategy (NCRIS). Margot Cronin thanks Anthony
English, Clynt Gregory, and Gordon Furey (P&amp;O Maritime Services) as well as
Tobias Steinhoff for their support. Nathalie Lefèvre thanks the crew of the Cap San
Lorenzo and the US IMAGO of IRD Brest for technical support. Gregor Rehder is grateful
for the skilful technical support of Michael Glockzin and Bernd Sadkowiak. Matthew W. Jones
thanks Anthony J. De-Gol for his technical and conceptual assistance with
the development of GCP-GridFED. We thank Ana Bastos and Joana Melo for
helpful comments on land-use emission estimates. FAOSTAT is funded by FAO
member states through their contributions to the FAO Regular Programme, and data
contributions by national experts are greatly acknowledged. The views
expressed in this paper are the authors' only and do not necessarily reflect
those of FAO. Finally, we thank all funders who have supported the
individual and joint contributions to this work (see Table A9), as well as
the reviewers of this paper and previous versions, and the many
researchers who have provided feedback.</p></ack><notes notes-type="financialsupport"><title>Financial support</title>

      <p id="d1e36545">For a list of all funders that have
supported this research, please refer to Table A9.</p>
  </notes><notes notes-type="reviewstatement"><title>Review statement</title>

      <p id="d1e36551">This paper was edited by David Carlson and reviewed by Hélène Peiro and one anonymous referee.</p>
  </notes><ref-list>
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